KR101972632B1 - 고체 산화물 연료 전지용 점성 밀봉 유리 조성물 - Google Patents

고체 산화물 연료 전지용 점성 밀봉 유리 조성물 Download PDF

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Publication number
KR101972632B1
KR101972632B1 KR1020157004531A KR20157004531A KR101972632B1 KR 101972632 B1 KR101972632 B1 KR 101972632B1 KR 1020157004531 A KR1020157004531 A KR 1020157004531A KR 20157004531 A KR20157004531 A KR 20157004531A KR 101972632 B1 KR101972632 B1 KR 101972632B1
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mol
sealant
glass
less
sofc
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Korean (ko)
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KR20150052017A (ko
Inventor
김철운
리차드 케이. 브로우
Original Assignee
엠오-싸이 코포레이션
더 큐레이터스 오브 더 유니버시티 오브 미주리
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    • C—CHEMISTRY; METALLURGY
    • C03—GLASS; MINERAL OR SLAG WOOL
    • C03C—CHEMICAL COMPOSITION OF GLASSES, GLAZES OR VITREOUS ENAMELS; SURFACE TREATMENT OF GLASS; SURFACE TREATMENT OF FIBRES OR FILAMENTS MADE FROM GLASS, MINERALS OR SLAGS; JOINING GLASS TO GLASS OR OTHER MATERIALS
    • C03C3/00—Glass compositions
    • C03C3/04—Glass compositions containing silica
    • C03C3/062—Glass compositions containing silica with less than 40% silica by weight
    • C03C3/064—Glass compositions containing silica with less than 40% silica by weight containing boron
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M50/00—Constructional details or processes of manufacture of the non-active parts of electrochemical cells other than fuel cells, e.g. hybrid cells
    • H01M50/10—Primary casings; Jackets or wrappings
    • H01M50/183—Sealing members
    • H01M50/186—Sealing members characterised by the disposition of the sealing members
    • C—CHEMISTRY; METALLURGY
    • C03—GLASS; MINERAL OR SLAG WOOL
    • C03C—CHEMICAL COMPOSITION OF GLASSES, GLAZES OR VITREOUS ENAMELS; SURFACE TREATMENT OF GLASS; SURFACE TREATMENT OF FIBRES OR FILAMENTS MADE FROM GLASS, MINERALS OR SLAGS; JOINING GLASS TO GLASS OR OTHER MATERIALS
    • C03C3/00—Glass compositions
    • C03C3/04—Glass compositions containing silica
    • C03C3/062—Glass compositions containing silica with less than 40% silica by weight
    • C03C3/064—Glass compositions containing silica with less than 40% silica by weight containing boron
    • C03C3/066—Glass compositions containing silica with less than 40% silica by weight containing boron containing zinc
    • C—CHEMISTRY; METALLURGY
    • C03—GLASS; MINERAL OR SLAG WOOL
    • C03C—CHEMICAL COMPOSITION OF GLASSES, GLAZES OR VITREOUS ENAMELS; SURFACE TREATMENT OF GLASS; SURFACE TREATMENT OF FIBRES OR FILAMENTS MADE FROM GLASS, MINERALS OR SLAGS; JOINING GLASS TO GLASS OR OTHER MATERIALS
    • C03C3/00—Glass compositions
    • C03C3/04—Glass compositions containing silica
    • C03C3/062—Glass compositions containing silica with less than 40% silica by weight
    • C03C3/064—Glass compositions containing silica with less than 40% silica by weight containing boron
    • C03C3/068—Glass compositions containing silica with less than 40% silica by weight containing boron containing rare earths
    • C—CHEMISTRY; METALLURGY
    • C03—GLASS; MINERAL OR SLAG WOOL
    • C03C—CHEMICAL COMPOSITION OF GLASSES, GLAZES OR VITREOUS ENAMELS; SURFACE TREATMENT OF GLASS; SURFACE TREATMENT OF FIBRES OR FILAMENTS MADE FROM GLASS, MINERALS OR SLAGS; JOINING GLASS TO GLASS OR OTHER MATERIALS
    • C03C8/00—Enamels; Glazes; Fusion seal compositions being frit compositions having non-frit additions
    • C03C8/02—Frit compositions, i.e. in a powdered or comminuted form
    • C—CHEMISTRY; METALLURGY
    • C03—GLASS; MINERAL OR SLAG WOOL
    • C03C—CHEMICAL COMPOSITION OF GLASSES, GLAZES OR VITREOUS ENAMELS; SURFACE TREATMENT OF GLASS; SURFACE TREATMENT OF FIBRES OR FILAMENTS MADE FROM GLASS, MINERALS OR SLAGS; JOINING GLASS TO GLASS OR OTHER MATERIALS
    • C03C8/00—Enamels; Glazes; Fusion seal compositions being frit compositions having non-frit additions
    • C03C8/02—Frit compositions, i.e. in a powdered or comminuted form
    • C03C8/04—Frit compositions, i.e. in a powdered or comminuted form containing zinc
    • C—CHEMISTRY; METALLURGY
    • C03—GLASS; MINERAL OR SLAG WOOL
    • C03C—CHEMICAL COMPOSITION OF GLASSES, GLAZES OR VITREOUS ENAMELS; SURFACE TREATMENT OF GLASS; SURFACE TREATMENT OF FIBRES OR FILAMENTS MADE FROM GLASS, MINERALS OR SLAGS; JOINING GLASS TO GLASS OR OTHER MATERIALS
    • C03C8/00—Enamels; Glazes; Fusion seal compositions being frit compositions having non-frit additions
    • C03C8/24—Fusion seal compositions being frit compositions having non-frit additions, i.e. for use as seals between dissimilar materials, e.g. glass and metal; Glass solders
    • H01M2/06—
    • H01M2/08—
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M50/00—Constructional details or processes of manufacture of the non-active parts of electrochemical cells other than fuel cells, e.g. hybrid cells
    • H01M50/10—Primary casings; Jackets or wrappings
    • H01M50/183—Sealing members
    • H01M50/19—Sealing members characterised by the material
    • H01M50/191—Inorganic material
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0271—Sealing or supporting means around electrodes, matrices or membranes
    • H01M8/028—Sealing means characterised by their material
    • H01M8/0282—Inorganic material
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0271—Sealing or supporting means around electrodes, matrices or membranes
    • H01M8/0286—Processes for forming seals
    • C—CHEMISTRY; METALLURGY
    • C03—GLASS; MINERAL OR SLAG WOOL
    • C03C—CHEMICAL COMPOSITION OF GLASSES, GLAZES OR VITREOUS ENAMELS; SURFACE TREATMENT OF GLASS; SURFACE TREATMENT OF FIBRES OR FILAMENTS MADE FROM GLASS, MINERALS OR SLAGS; JOINING GLASS TO GLASS OR OTHER MATERIALS
    • C03C2207/00—Compositions specially applicable for the manufacture of vitreous enamels
    • C03C2207/04—Compositions specially applicable for the manufacture of vitreous enamels for steel
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M2008/1293—Fuel cells with solid oxide electrolytes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0017—Non-aqueous electrolytes
    • H01M2300/0065—Solid electrolytes
    • H01M2300/0068—Solid electrolytes inorganic
    • H01M2300/0071—Oxides
    • H01M2300/0074—Ion conductive at high temperature
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204—Non-porous and characterised by the material
    • H01M8/0206—Metals or alloys
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10—Energy storage using batteries
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells

Landscapes

  • Chemical & Material Sciences (AREA)
  • General Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Geochemistry & Mineralogy (AREA)
  • Materials Engineering (AREA)
  • Organic Chemistry (AREA)
  • Electrochemistry (AREA)
  • Manufacturing & Machinery (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Inorganic Chemistry (AREA)
  • Glass Compositions (AREA)
  • Fuel Cell (AREA)
KR1020157004531A 2012-07-23 2013-07-23 고체 산화물 연료 전지용 점성 밀봉 유리 조성물 Active KR101972632B1 (ko)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
US201261674692P 2012-07-23 2012-07-23
US61/674,692 2012-07-23
PCT/US2013/051691 WO2014018536A1 (en) 2012-07-23 2013-07-23 Viscous sealing glass compositions for solid oxide fuels cells

Publications (2)

Publication Number Publication Date
KR20150052017A KR20150052017A (ko) 2015-05-13
KR101972632B1 true KR101972632B1 (ko) 2019-04-25

Family

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KR1020157004531A Active KR101972632B1 (ko) 2012-07-23 2013-07-23 고체 산화물 연료 전지용 점성 밀봉 유리 조성물

Country Status (7)

Country Link
US (1) US9530991B2 (https=)
EP (1) EP2875537B1 (https=)
JP (1) JP6328111B2 (https=)
KR (1) KR101972632B1 (https=)
ES (1) ES2887360T3 (https=)
IN (1) IN2015DN01487A (https=)
WO (1) WO2014018536A1 (https=)

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* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP6521064B2 (ja) * 2015-06-09 2019-05-29 日産自動車株式会社 固体酸化物型燃料電池
KR20170032856A (ko) * 2015-09-15 2017-03-23 주식회사 엘지화학 고체산화물 연료전지 실링재용 조성물, 이를 이용한 실링재 및 이의 제조방법
JP6636814B2 (ja) * 2016-02-09 2020-01-29 株式会社ノリタケカンパニーリミテド ガラス組成物およびその利用
KR102427387B1 (ko) * 2017-10-24 2022-07-29 주식회사 엘지화학 고체 산화물 연료 전지용 실링재 조성물, 이로 제조된 실링재를 갖는 고체 산화물 연료 전지 및 이의 실링방법
JP7016028B2 (ja) * 2018-04-03 2022-02-04 パナソニックＩｐマネジメント株式会社 燃料電池
KR20190127426A (ko) * 2018-05-04 2019-11-13 엘지전자 주식회사 실링 유리 조성물 및 이를 이용한 고체산화물 연료 전지
KR102217226B1 (ko) * 2018-11-02 2021-02-18 엘지전자 주식회사 실링 유리 조성물 및 이를 이용한 고체산화물 연료 전지
KR102185975B1 (ko) * 2018-11-29 2020-12-02 엘지전자 주식회사 실링 유리 조성물 및 이를 이용한 고체산화물 연료 전지
KR102244554B1 (ko) * 2020-02-07 2021-04-26 부산대학교 산학협력단 자가치유 특성을 갖는 유리의 제조 방법
JP7349950B2 (ja) * 2020-03-30 2023-09-25 大阪瓦斯株式会社 シール部材の修復方法及び燃料電池システム
CN118919797B (zh) * 2024-10-09 2025-02-11 中国石油大学(华东) 具有长寿命密封界面的sofc或soec及其制备方法

Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20060063659A1 (en) 2004-09-21 2006-03-23 General Electric Company Alkali-Free Composite Sealant Materials for Solid Oxide Fuel Cells
US20090318278A1 (en) 2008-06-19 2009-12-24 Nihon Yamamura Glass Co., Ltd. Composition for sealing glass

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EP0132810A1 (en) * 1983-07-25 1985-02-13 E.I. Du Pont De Nemours And Company Borosilicate glass composition
US5922444A (en) * 1992-10-27 1999-07-13 Ngk Spark Plug Co., Ltd. Glaze composition
US5453331A (en) 1994-08-12 1995-09-26 University Of Chicago Compliant sealants for solid oxide fuel cells and other ceramics
US5637261A (en) * 1994-11-07 1997-06-10 The Curators Of The University Of Missouri Aluminum nitride-compatible thick-film binder glass and thick-film paste composition
US6124224A (en) * 1998-09-02 2000-09-26 Ferro Corporation High temperature sealing glass
US6362119B1 (en) * 1999-06-09 2002-03-26 Asahi Glass Company, Limited Barium borosilicate glass and glass ceramic composition
KR100590968B1 (ko) 2004-01-05 2006-06-19 현대자동차주식회사 고체산화물 연료전지용 유리/세라믹 섬유 밀봉재와 이의제조방법
CA2579781A1 (en) * 2004-09-22 2007-01-04 Battelle Memorial Institute High strength insulating joints for solid oxide fuel cells and other high temperature applications and method of making
US20060063057A1 (en) * 2004-09-22 2006-03-23 Battelle Memorial Institute High strength insulating metal-to-metal joints for solid oxide fuel cells and other high temperature applications and method of making
US7897530B2 (en) 2008-01-14 2011-03-01 Atomic Energy Council-Institute Of Nuclear Energy Research Glass-ceramic sealant for planar solid oxide fuel cells
US7989374B2 (en) 2008-05-15 2011-08-02 Corning Incorporated Non-contaminating, electro-chemically stable glass frit sealing materials and seals and devices using such sealing materials
FR2946043B1 (fr) * 2009-05-27 2011-06-24 Centre Nat Rech Scient Composition vitreuse autocicatrisante, procede de preparation et utilisations.

Patent Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20060063659A1 (en) 2004-09-21 2006-03-23 General Electric Company Alkali-Free Composite Sealant Materials for Solid Oxide Fuel Cells
US20090318278A1 (en) 2008-06-19 2009-12-24 Nihon Yamamura Glass Co., Ltd. Composition for sealing glass

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* Cited by examiner, † Cited by third party
Title
Effect of additives on the thermal properties(i n t e r n a t i o n a l j o u rna l o f hydrogen energy 3 4 ( 2 0 0 9 ) 8 2 3 5 - 8 2 4 4)*
Wettability and Interfacial Reaction between Glass Sealants and Ferritic Steel(J.G.Heinrich and C. Aneziris, Proc. 10th ECerS Conf., Göller Verlag, Baden-Baden, 2007, 871-879)*

Also Published As

Publication number Publication date
WO2014018536A1 (en) 2014-01-30
US20150125780A1 (en) 2015-05-07
JP2015529621A (ja) 2015-10-08
JP6328111B2 (ja) 2018-05-23
IN2015DN01487A (https=) 2015-07-03
ES2887360T3 (es) 2021-12-22
EP2875537B1 (en) 2021-09-01
KR20150052017A (ko) 2015-05-13
US9530991B2 (en) 2016-12-27
EP2875537A1 (en) 2015-05-27
EP2875537A4 (en) 2016-03-23

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