JP4324674B2 - Viburnum pericarp manufacturing method, viburnum pericarp manufacturing apparatus, viburnum pericarp extract, antioxidants derived from viburnum pericarp, powdered material derived from viburnum pericarp and processed products using viburnum pericarp - Google Patents

Viburnum pericarp manufacturing method, viburnum pericarp manufacturing apparatus, viburnum pericarp extract, antioxidants derived from viburnum pericarp, powdered material derived from viburnum pericarp and processed products using viburnum pericarp Download PDF

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JP4324674B2
JP4324674B2 JP2004338715A JP2004338715A JP4324674B2 JP 4324674 B2 JP4324674 B2 JP 4324674B2 JP 2004338715 A JP2004338715 A JP 2004338715A JP 2004338715 A JP2004338715 A JP 2004338715A JP 4324674 B2 JP4324674 B2 JP 4324674B2
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邦久 岩井
一 松江
昭夫 小野寺
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地方独立行政法人青森県産業技術センター
昭夫 小野寺
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本発明はガマズミ果肉皮の製造方法、ガマズミ果肉皮製造装置、ガマズミ果肉皮抽出物、ガマズミ果肉皮由来抗酸化剤、ガマズミ果肉皮由来粉末状素材およびガマズミ果肉皮使用加工品に係り、ガマズミ果汁製造工程において産する種子と果肉皮からなる搾汁残渣から果肉皮のみを効率的に分離でき、かつその技術に基づいて、主にアントシアニン、アントシアニン誘導体、クロロゲン酸およびクロロゲン酸誘導体等の抗酸化活性など種々の有用な生理活性物質を提供することのできる、ガマズミ果肉皮の製造方法、ガマズミ果肉皮製造装置、ガマズミ果肉皮抽出物、ガマズミ果肉皮由来抗酸化剤、ガマズミ果肉皮由来粉末状素材およびガマズミ果肉皮使用加工品に関する。   The present invention relates to a method for producing viburnum pericarp, an apparatus for producing viburnum pericarp, a viburnum pericarp extract, an antioxidant derived from viburnum pericarp, a powdered material derived from viburnum pericarp and a processed product using viburnum pericarp, It is possible to efficiently separate only the flesh peel from the squeezed residue consisting of seeds and flesh peel produced in the process, and based on the technology, mainly antioxidant activity such as anthocyanins, anthocyanin derivatives, chlorogenic acid and chlorogenic acid derivatives, etc. Viburnum pericarp manufacturing method, viburnum pericarp manufacturing apparatus, viburnum pericarp extract, viburnum pericarp-derived antioxidant, viburnum pericarp-derived powdery material and viburnum that can provide various useful physiologically active substances It relates to processed products using pulp.

ガマズミは、山野に自生するスイカズラ科の落葉低木である。本願の約10年前から本願発明者の一人・小野寺らが、青森県三戸郡三戸町において、ガマズミの畑への栽培を試みてそれに成功し、果汁100%飲料を開発した。本願発明者の岩井、松江および小野寺はガマズミ果実の生理機能の共同研究に着手し、その結果、ガマズミ果実に強い抗酸化活性があることを見出した。そこで、ガマズミ果実抽出物 (果汁) をラットに投与し、水浸拘束ストレスを負荷した場合の胃潰瘍発生を抑制することを明らかにした (非特許文献1)。さらに、岩井らはラットを用いた実験から、ガマズミ果汁が実験的糖尿病の症状進行を抑制すること (非特許文献2)、またそれらの活性成分の分子構造を同定するとともに、その生化学的作用機序を明らかにした (非特許文献3、4)。それらの結果より、ガマズミ果汁に含まれるアントシアニン誘導体、クロロゲン酸、クロロゲン酸誘導体およびケルセチン等が、抗酸化活性および種々の生理作用の主要な成分であることを活性の検討および各種機器分析を用いた構造解析から、分子構造レベルで明らかにした。   Viburnum is a deciduous shrub of the family Lonicera that grows naturally in the mountains. About 10 years before this application, Onodera et al., One of the inventors of this application, succeeded in cultivation in a field of viburnum in Sannohe-cho, Sannohe-gun, Aomori Prefecture, and developed a 100% fruit juice drink. The inventors of the present invention, Iwai, Matsue and Onodera, started joint research on physiological functions of viburnum fruits, and as a result, found that viburnum fruits have strong antioxidant activity. Thus, it was clarified that viburnum fruit extract (fruit juice) was administered to rats to suppress the occurrence of gastric ulcer when water immersion restraint stress was applied (Non-patent Document 1). In addition, Iwai et al., From experiments using rats, showed that viburnum juice suppressed the progression of experimental diabetes symptoms (Non-Patent Document 2), identified the molecular structure of these active ingredients, and their biochemical effects. The mechanism was clarified (Non-Patent Documents 3 and 4). From these results, we examined the activity of anthocyanin derivatives, chlorogenic acid, chlorogenic acid derivatives and quercetin contained in viburnum juice as the main components of antioxidant activity and various physiological functions, and used various instrumental analyzes. Clarified at the molecular structure level from structural analysis.

これらの研究成果をきっかけに、科学的な根拠に基づいたガマズミ果実の有用な生理作用が知られるようになり、飲料開発時にはわずか数百kgであった果実の収穫量が、2003年には10tを超えるまでに発展し、現在、三戸町の周辺町村でもガマズミの栽培および飲料の生産が手掛けられている。また、本願出願人が公表した事実をそのまま記載した後発の特許出願例も存在する (特許文献1参照)。   As a result of these research results, the physiological effects of viburnum fruits based on scientific grounds became known, and the yield of fruits, which was only a few hundred kg at the time of beverage development, was 10 tons in 2003. The viburnum is grown and beverages are being produced in neighboring towns and villages in Sannohe. There is also a later patent application example that directly describes the facts published by the applicant of the present application (see Patent Document 1).

K.Iwai, et al., Int. J. Food Sci. Nutr., 52, 443-451 (2001)K. Iwai, et al., Int. J. Food Sci. Nutr., 52, 443-451 (2001) K.Iwai, et al., J. Agric, Food Chem., 52, 1002-1007 (2004)K. Iwai, et al., J. Agric, Food Chem., 52, 1002-1007 (2004) M.Y.Kim, et al., J. Agric. Food Chem., 51, 6173-6177 (2003)M.Y.Kim, et al., J. Agric. Food Chem., 51, 6173-6177 (2003) K.Iwai, et al., J. Sci. Food Agric., 83, 1593-1599 (2003)K. Iwai, et al., J. Sci. Food Agric., 83, 1593-1599 (2003) 特願2001-158136Japanese Patent Application 2001-158136

さて、本願発明者らにより1996年から販売されているガマズミ果汁飲料(商品名「ジョミ」)は、ガマズミ果実を原料とした無添加の100%果汁飲料製品であるが、その製造は、ガマズミ果実を油圧式圧搾機で圧搾して得られる果汁原液を、加温、瓶充填、および加熱殺菌の各工程を経ることによって行われる。この圧搾工程には約2時間を要し、ろ布を用いたろ過によって果実20kg から約12L の果汁原液が得られ、約10kgの搾汁残渣が生じる。   The viburnum juice drink (trade name “Jomi”) sold by the inventors of the present application since 1996 is an additive-free 100% fruit juice drink product using viburnum fruit as a raw material. The juice concentrate obtained by squeezing with a hydraulic press is performed through each step of heating, bottle filling, and heat sterilization. This pressing process takes about 2 hours, and a fruit stock solution of about 12 L is obtained from 20 kg of fruit by filtration using a filter cloth, resulting in about 10 kg of juice residue.

ガマズミ果実搾汁残渣(以下、単に「搾汁残渣」ともいう)を温風乾燥機を用いて70〜80℃の温度下で8〜9時間乾燥させることによって、約9.3kgの乾燥搾汁残渣 (収量約46.5%) が得られる(乾燥温度は、上記温度より低温で行うと乾燥に長い時間を要し、高温で行うと乾燥時間は若干短縮できるが、成分の変質を生じる可能性がある。上記温度条件によれば、有用物質が比較的分解せず、しかも腐敗を防止することができる)。この搾汁残渣は、主にガマズミの果肉皮と種子が密着した状態よりなる。   About 9.3 kg of dried juice is obtained by drying viburnum fruit juice residue (hereinafter also simply referred to as “juice residue”) at a temperature of 70-80 ° C. for 8-9 hours using a warm air dryer. A residue (yield of about 46.5%) is obtained. (Drying temperature takes a long time if it is performed at a temperature lower than the above temperature. If it is performed at a high temperature, the drying time can be shortened slightly, but the components may be altered. According to the above temperature conditions, useful substances are not relatively decomposed and can be prevented from decaying). This squeezed residue mainly consists of a state where the viburnum peel and seed are in close contact.

こうして、製造過程において常時産業廃棄物として発生するガマズミ果実搾汁残渣の量は、ガマズミ果汁飲料の製造量の増加とともに増大しており、従来はこれをすべて廃棄処分してきた。しかし、今後も果実生産量は増加すると見込まれており、残渣の処分が問題になることは避けられない。また、残渣の有効利用はゼロエミッションの配慮からも重要であり、利用法の開発は生産者側および消費者側からも強く望まれている。   Thus, the amount of viburnum fruit juice residue that is always generated as industrial waste during the production process has increased with the increase in the production amount of viburnum fruit juice beverage, and all of this has been disposed of in the past. However, fruit production is expected to increase in the future, and it is unavoidable that disposal of the residue becomes a problem. In addition, the effective use of residues is important from the viewpoint of zero emissions, and the development of usage is strongly desired by producers and consumers.

本発明が解決しようとする課題は、上記従来技術の状況を踏まえ、かつその問題点を除き、ガマズミ果汁製造工程において産する種子と果肉皮からなる搾汁残渣から果肉皮のみを効率的に分離し、かつその技術に基づいて、主にアントシアニン、アントシアニン誘導体、クロロゲン酸およびクロロゲン酸誘導体等の抗酸化活性など種々の有用な生理活性物質を抽出物や添加食品等の諸形態で提供することのできる、ガマズミ果肉皮の製造方法、ガマズミ果肉皮製造装置、ガマズミ果肉皮抽出物、ガマズミ果肉皮由来抗酸化剤、ガマズミ果肉皮由来粉末状素材およびガマズミ果肉皮使用加工品を提供することである。   The problem to be solved by the present invention is based on the above-mentioned state of the art, and, except for the problems, efficiently separates only the flesh peel from the juice residue consisting of seeds and flesh peel produced in the viburnum juice production process. In addition, based on the technology, various useful physiologically active substances such as anthocyanins, anthocyanin derivatives, chlorogenic acid and chlorogenic acid derivatives are useful in various forms such as extracts and added foods. It is possible to provide a method for producing viburnum peel, an apparatus for producing viburnum peel, an extract of viburnum peel, an antioxidant derived from viburnum peel, a powdered material derived from viburnum peel, and a processed product using viburnum peel.

本願発明者は上記課題について、下記の通り検討した。すなわち;
ガマズミ果実搾汁残渣について、XYZ−dish法 (K.Iwai, et al., Food Sci. Biotechnol., 10, 513-520 (2001)、およびK.Iwai, et al., Food Sci. Biotechnol., 10, 508-512 (2001)) によって抗酸化活性を調べると、活性酸素種を過酸化水素とした時の搾汁残渣1g当たりの抗酸化活性は3.87±0.75 unit、水酸化ラジカルに対する搾汁残渣1g当たりの抗酸化活性は5.60±0.94 unitと、果汁の抗酸化活性 (過酸化水素に対して1mL当たり0.689±0.043 unit、水酸化ラジカルに対して1mL当たり3.621±0.363 unit) 以上の抗酸化活性が存在していることを見出した。
表1に、各抗酸化活性測定結果を示す。
The inventor of the present application examined the above problems as follows. Ie;
For viburnum fruit juice residue, XYZ-dish method (K.Iwai, et al., Food Sci. Biotechnol., 10, 513-520 (2001), and K.Iwai, et al., Food Sci. Biotechnol., 10, 508-512 (2001)), the antioxidant activity per gram of squeezed residue when reactive oxygen species was hydrogen peroxide was 3.87 ± 0.75 unit, squeezed residue against hydroxyl radical Antioxidant activity per gram is 5.60 ± 0.94 units, and antioxidant activity of fruit juice (0.689 ± 0.043 unit per mL for hydrogen peroxide, 3.621 ± 0.363 unit per mL for hydroxyl radical) Found that exists.
Table 1 shows the measurement results of each antioxidant activity.

Figure 0004324674
Figure 0004324674

つまり本願発明者は、ガマズミ搾汁残渣に果汁と同様の抗酸化作用を見出し、しかも、果汁に含まれていてガマズミ果汁飲料の有益な作用の活性物質とされるアントシアニン誘導体、クロロゲン酸、クロロゲン酸誘導体等の成分が搾汁残渣中の果肉皮部分に多量に含まれることを見出し、残渣から果肉皮と種子を分離することによって果汁に匹敵する果肉皮の効果的活用が可能であることを見出して、本発明に至った。すなわち、上記課題を解決するための手段として本願で特許請求もしくは少なくとも開示される発明は、以下のとおりである。   In other words, the present inventor has found an antioxidant effect similar to fruit juice in viburnum juice residue, and an anthocyanin derivative, chlorogenic acid, chlorogenic acid, which is contained in fruit juice and is an active substance of beneficial effects of viburnum juice beverage It is found that components such as derivatives are contained in a large amount in the pulp skin part of the juice residue, and the fruit skin skin comparable to the fruit juice can be effectively used by separating the fruit skin and seeds from the residue. Thus, the present invention has been achieved. That is, the invention claimed or at least disclosed in the present application as means for solving the above-described problems is as follows.

(1) 一粒ごとに種子に薄く果肉皮が密着し一体となっているガマズミ果実搾汁残渣を、該ガマズミ果実搾汁残渣各粒間相互の研磨作用を行える精米機様構造で処理することによって、アントシアニン、クロロゲン酸ならびにその誘導体をより多く含有する果肉皮を、種子をほとんど損傷せずに種子から分離することにより行う、 ガマズミ果肉皮の製造方法。
(2) 一粒ごとに種子に薄く果肉皮が密着し一体となっているガマズミ果実搾汁残渣を後記分離部へ供給する原料供給口と、供給される該ガマズミ果実搾汁残渣を種子とガマズミ果肉皮とに分離する分離部と、分離された該ガマズミ果肉皮を受ける果肉皮受け部と、およびこれらを包含してなる筐体とからなるガマズミ果肉皮製造装置であって、該分離部は、該ガマズミ果実搾汁残渣を回転させつつこれに精米機の様に該ガマズミ果実搾汁残渣各粒間相互における研磨作用を施すロータと、該ロータにおける作用により剥離されたガマズミ果肉皮を種子をほとんど損傷することなく種子と分離して該果肉皮受け部へ排出するための網状筒型容器を備えている、ガマズミ果肉皮製造装置。
(3) (1)に記載の製造方法により得られるガマズミ果肉皮を抽出してなる、ガマズミ果肉皮の抽出物。
(4) (1)に記載の製造方法により得られるガマズミ果肉皮を用いてなる、ガマズミ果肉皮由来抗酸化剤。
(5) (1)に記載の製造方法により得られるガマズミ果肉皮を用いてなる、ガマズミ果肉皮由来粉末状素材。
(6) (5)に記載のガマズミ果肉皮由来粉末状素材を用いてなる、錠剤、顆粒、カプセルその他の形態のサプリメント。
(7) (3)に記載のガマズミ果肉皮抽出物または請求項5に記載のガマズミ果肉皮由来粉末状素材を用いてなる、食品、飲料または着色料。
(1) Treating viburnum fruit juice residue, in which the pericarp is thinly attached to the seed for each grain, with a rice milling machine-like structure capable of mutual polishing action between the grains of viburnum fruit juice residue. A method for producing viburnum pericarp, comprising separating the pericarp containing more anthocyanin, chlorogenic acid and derivatives thereof from the seed with little damage to the seed .
(2) A raw material supply port for supplying a viburnum fruit juice residue, in which the pericarp is thinly attached to the seed for each grain, to the separation unit described later, and the viburnum fruit juice residue to be fed is used as a seed and a viburnum. A viburnum peel production apparatus comprising a separation part that separates into flesh skin, a flesh skin receiving part that receives the separated viburnum skin, and a casing that includes these parts, wherein the separation part comprises: a rotor performing polishing action at the mutual between said Viburnum fruit juice remaining渣各particle like a rice mill to while rotating the Viburnum fruit juice residue, a seeds Viburnum pulp skin which is peeled off by the action of the rotor A viburnum peel production apparatus comprising a reticulated tubular container for separating from a seed and discharging it to the pulp peel receiving part with almost no damage .
(3) An extract of viburnum pericarp obtained by extracting viburnum pericarp obtained by the production method according to (1) .
(4) A viburnum pericarp-derived antioxidant comprising the viburnum pericarp obtained by the production method according to (1) .
(5) A viburnum pericarp-derived powdery material obtained by using the viburnum pericarp obtained by the production method according to (1) .
(6) A supplement in the form of a tablet, granule, capsule or the like, using the powdery material derived from viburnum pericarp according to (5).
(7) A food, beverage or colorant comprising the viburnum pericarp extract according to (3) or the viburnum pericarp derived powdery material according to claim 5.

本発明のガマズミ果肉皮の製造方法、ガマズミ果肉皮製造装置、ガマズミ果肉皮抽出物、ガマズミ果肉皮由来抗酸化剤、ガマズミ果肉皮由来粉末状素材およびガマズミ果肉皮使用加工品は上述のように構成されるため、これによれば、ガマズミ果汁製造工程において産する種子と果肉皮からなる搾汁残渣から果肉皮のみを効率的に分離することができ、その技術に基づいて、主にアントシアニン、アントシアニン誘導体、クロロゲン酸およびクロロゲン酸誘導体等の抗酸化活性など種々の有用な生理活性物質を、抽出物や添加食品、抗酸化剤等の諸形態で提供することができる。   The method for producing viburnum pericarp of the present invention, viburnum pericarp manufacturing apparatus, viburnum pericarp extract, antibiotic derived from viburnum pericarp, powdered material derived from viburnum pericarp and processed product using viburnum pericarp as described above Therefore, according to this, it is possible to efficiently separate only the flesh peel from the juice residue consisting of seeds and flesh peel produced in the viburnum juice production process, and based on that technology, mainly anthocyanins and anthocyanins Various useful physiologically active substances such as antioxidants such as derivatives, chlorogenic acid and chlorogenic acid derivatives can be provided in various forms such as extracts, additive foods, antioxidants and the like.

また、ガマズミ果汁飲料の製造量の増加とともに増大し、従来廃棄処分されてきた搾汁残渣について、ゼロエミッション化が可能となる。   Moreover, it increases with the increase in the production amount of a viburnum fruit juice drink, and the squeeze residue that has been conventionally disposed of can be made zero emission.

その上、従来はジュース製造用途のみしかなかったガマズミ果実を、本発明によって粉末状素材化でき、種々の付加価値製品を応用開発することができる。   Moreover, viburnum fruit, which has been used only for juice production in the past, can be made into a powdery material according to the present invention, and various value-added products can be applied and developed.

以下、本発明を図面も用いつつ詳細に説明する。
まず本願発明のうち、上記(1)および(2)の発明完成の経緯について、さらに述べる。
搾汁残渣は種子と果肉皮からなっており、そのどちらに抗酸化を示す物質が得られるかが重要である。すなわち、強い抗酸化活性を示す部分のみを物理的に分離することができれば、抗酸化力を有する成分を濃縮した食品素材になり得ることから、それらの分離を試みた。ほぼ球形に近い生の果実は、果汁を得るための圧搾によって扁平となり、さらに乾燥した残渣は皺を生じている。しかし、単純な圧搾のため、果皮が裂けるなどの損傷はほとんどなく、また、本来の生果実が直径5mm前後の小ささであることから、搾汁残渣といっても一粒一粒は種子に薄く果肉と果皮が密着したものとなっている。そのため、この残渣を種子と果肉および果皮に分離することは非常な困難が予想されたが、本願発明者は搾汁残渣の形状が玄米に非常に似た形態であることに着目し、精米器様構造を利用した分離を試みた。その結果、精米器様構造の利用によって効率的に搾汁残渣を種子と果肉皮に分離することが可能となり、しかも種子をほとんど損傷しないことから、種子の主要な成分である脂質の混入を防ぐことも可能となった。また処理量が多い場合には、この分離製造工程を並列に配した機器によって、効率的に、無駄なく、精度良く制御された形で、しかも安定的にガマズミ果肉皮の分離分別に対応する製造が可能になった。
Hereinafter, the present invention will be described in detail with reference to the drawings.
First of all, the background of the completion of the inventions (1) and (2) will be further described.
The squeezed residue is composed of seeds and flesh skin, and it is important which of them can obtain a substance exhibiting antioxidant properties. That is, if only a portion exhibiting strong antioxidant activity can be physically separated, it can be a food material in which components having antioxidant power are concentrated. The raw fruit, which is almost spherical, is flattened by pressing to obtain fruit juice, and the dried residue is wrinkled. However, due to simple pressing, there is almost no damage such as tearing of the skin, and since the original raw fruit is as small as about 5 mm in diameter, each squeezed residue is a seed. Thinly, the flesh and skin are in close contact. For this reason, it was expected that it would be very difficult to separate the residue into seeds, pulp and skin, but the present inventor paid attention to the fact that the shape of the squeezed residue was very similar to brown rice, Separation using a similar structure was attempted. As a result, it is possible to efficiently separate the juice residue into seeds and flesh skin by using a rice mill-like structure, and since it hardly damages the seeds, it prevents contamination of lipids, which are the main components of seeds. It became possible. In addition, when the amount of processing is large, manufacturing that can efficiently separate, separate, and separate the viburnum pericarp by using a device with this separation manufacturing process arranged in parallel, efficiently, without waste, and accurately controlled. Became possible.

図1は、本発明のガマズミ果肉皮の製造方法を示すフロー図、また、
図2は、本発明のガマズミ果肉皮製造装置の機構の基本構成例を示す説明図である。
図1に示すように、本ガマズミ果肉皮製造方法では、一粒ごとに種子と果肉皮とが密着し一体となっているガマズミ果実搾汁残渣1を適宜の温度条件下乾燥して乾燥搾汁残渣2を得(P1)、該乾燥搾汁残渣2に対して、各粒間の摩擦作用または研磨作用を利用することによって、アントシアニン、クロロゲン酸ならびにその誘導体をより多く含有する果肉皮3を種子4から分離する(P2)ことにより、 ガマズミ果肉皮3が得られる。乾燥には温風乾燥機を用いることができる。また、その際の温度条件としては、前述の通り、70〜80℃、8〜9時間の条件を好適に用いることができる。
FIG. 1 is a flowchart showing a method for producing a viburnum skin of the present invention,
FIG. 2 is an explanatory diagram showing a basic configuration example of the mechanism of the viburnum peel manufacturing apparatus of the present invention.
As shown in FIG. 1, in this viburnum peel manufacturing method, the viburnum fruit squeezed residue 1 in which the seed and the flesh peel are in close contact with each other and dried is dried under a suitable temperature condition. Residue 2 is obtained (P1), and the dried squeezed residue 2 is seeded with flesh peel 3 containing more anthocyanins, chlorogenic acid and derivatives thereof by utilizing the frictional action or polishing action between the grains. By separating from 4 (P2), a viburnum pericarp 3 is obtained. A hot air dryer can be used for drying. Moreover, as temperature conditions in that case, as above-mentioned, the conditions of 70-80 degreeC and 8-9 hours can be used suitably.

図においてP2の各粒間の摩擦作用または研磨作用利用による分離には、精米機様構造等を用いて行うことができる。また、分離製造されたガマズミ果肉皮3は、これを必要に応じて粉末化(P3)してガマズミ果肉皮由来粉末状素材5とするなどして、各種加工食品等素材とすることができる。   In the figure, separation by using frictional action or polishing action between the grains of P2 can be performed using a rice mill-like structure or the like. In addition, the separated viburnum skin 3 can be made into various processed food materials, for example, by pulverizing (P3) as needed to obtain a viburnum skin-derived powdery material 5.

図2に示すように本例ガマズミ果肉皮製造装置100は、一粒ごとに種子と果肉皮とが一体となっているガマズミ果実搾汁残渣(乾燥搾汁残渣)を後記分離部20へ供給する原料供給口10と、供給される該ガマズミ果実搾汁残渣を種子とガマズミ果肉皮とに分離する分離部20と、分離された該ガマズミ果肉皮を受ける果肉皮受け部30と、およびこれらを包含してなる筐体(図示せず)とからなるガマズミ果肉皮製造装置100であって、該分離部20は、モータ50により回転されて、該ガマズミ果実搾汁残渣を回転させつつこれに研磨もしくは摩擦作用を施すスクリュー型等のロータ24と、該作用により剥離されたガマズミ果肉皮を種子と分離して該果肉皮受け部30へ排出するための網状筒型容器28を備えて構成される。ここで、該網状筒型容器28の網構造は、分離された果肉皮は通すが種子は通さないサイズの網目のものが用いられる。   As shown in FIG. 2, the example viburnum peel manufacturing apparatus 100 supplies a viburnum fruit juice residue (dried juice residue) in which seeds and fruit skin are integrated for each grain to the separation unit 20 described later. A raw material supply port 10, a separation unit 20 for separating the viburnum fruit juice residue supplied into seeds and viburnum skin, a flesh skin receiving portion 30 for receiving the separated viburnum skin, and the like A viburnum peel manufacturing apparatus 100 comprising a casing (not shown) formed by the separation part 20 being rotated by a motor 50 and polishing or polishing the viburnum fruit juice residue. A rotor 24 such as a screw type that performs a frictional action, and a mesh-like cylindrical container 28 for separating the viburnum flesh peeled by the action from the seeds and discharging them to the flesh peel receiving portion 30 are configured. Here, the mesh structure of the mesh-like cylindrical container 28 is a mesh having a size that allows the separated flesh skin to pass but does not allow seeds to pass.

本装置100は上述のように構成されるため、乾燥搾汁残渣は原料供給口10から分離部20へと供給され、分離部20のロータ24によって回転されながら研磨もしくは摩擦作用が施され、それによって種子とガマズミ果肉皮とが分離され、分離された該ガマズミ果肉皮は網状筒型容器28を通して排出されて果肉皮受け部30によって受けられる。このようにして分離製造されたガマズミ果肉皮は、良好に種子とは分離され、しかもほとんど損傷がない状態のものが得られる。本発明製造方法・製造装置では、一定の、しかも多様なサイズの分離果肉皮を製造することができる。   Since the apparatus 100 is configured as described above, the dried juice residue is supplied from the raw material supply port 10 to the separation unit 20 and is subjected to polishing or friction while being rotated by the rotor 24 of the separation unit 20. The seeds and the viburnum pericarp are separated by the above, and the separated viburnum pericarp is discharged through the reticulated cylindrical container 28 and received by the pericarp skin receiving portion 30. The viburnum pericarp thus separated and produced is well separated from the seeds, and can be obtained with little damage. In the manufacturing method and the manufacturing apparatus of the present invention, it is possible to manufacture separated and peeled skins of various sizes.

本装置100は、玄米を精米するための精米機様の構造を有する。したがって、従来公知の精米機を適宜使用して、本発明の目的を達成することもできる。特に大量の搾汁残渣を連続的かつ効率的に処理するために、本装置100の構成を複数並列させたシステムを構成してもよい。   The apparatus 100 has a rice mill-like structure for milling brown rice. Therefore, the object of the present invention can be achieved by appropriately using a conventionally known rice mill. In particular, in order to process a large amount of squeezed residue continuously and efficiently, a system in which a plurality of configurations of the apparatus 100 are arranged in parallel may be configured.

本装置は、乾燥搾汁残渣はその表面すなわちガマズミ果肉皮が削られて分離されながら排出される構成をとることができるが、この場合、その削り具合を調整できる機構を備えたものとすることができる。かかる機構はたとえば、排出部におけるバネ仕掛けによって削り具合を加減する方式を始めとして、従来の精米機構造に用いられている適宜の精米歩合調整機構を使用して構成することができる。また原料供給口は、原料の詰まりを有効に防止するのに充分な広さにこれを設計することももちろんできる。さらに原料供給口には、円滑な供給の行える原料搬入路とするために、ロータに接触しないような位置に上方から下垂する細目の棒を用いる、もしくは設けることもできる。   This device can take a structure in which the dried juice residue is discharged while its surface, i.e., the viburnum skin skin is scraped and separated, but in this case, it shall have a mechanism that can adjust the shaving condition. Can do. Such a mechanism can be configured, for example, using an appropriate rice milling rate adjusting mechanism used in a conventional rice milling machine structure, including a method of adjusting the degree of shaving by a spring mechanism in the discharge unit. It is of course possible to design the raw material supply port so that it is wide enough to effectively prevent clogging of the raw material. Furthermore, in order to provide a raw material carry-in path that allows smooth supply, a thin rod that hangs down from above can be used or provided at a position that does not contact the rotor.

分離した果肉皮の有用性を確認するため、分離果肉皮の抗酸化活性をXYZ-dish法で測定すると、過酸化水素に対して41.54 unit、および水酸化ラジカルに対して56.18 unit (いずれも分離果肉皮1 gあたり) の活性が得られた。これは、元の搾汁残渣の活性 (過酸化水素に対して3.87 unit、水酸化ラジカルに対して5.60 unit) に比べて10倍以上高いものであった。したがって、この分離法によって、抗酸化活性を有している搾汁残渣から活性の存在する部分のみを選択的に得ることが可能になった。
表2に、搾汁残渣および分離果肉皮の抗酸化活性測定結果を示す。
In order to confirm the usefulness of the separated flesh skin, the antioxidant activity of the separated flesh skin was measured by the XYZ-dish method. 41.54 units for hydrogen peroxide and 56.18 units for hydroxyl radicals (both separated) Activity per 1 g of pulp skin). This was more than 10 times higher than the activity of the original juice residue (3.87 units for hydrogen peroxide and 5.60 units for hydroxyl radicals). Therefore, this separation method makes it possible to selectively obtain only the active portion from the juice residue having antioxidant activity.
Table 2 shows the measurement results of the antioxidant activity of the juice residue and the separated pulp skin.

Figure 0004324674
Figure 0004324674

さらに、すでに果汁中の有用成分が同定されていることに基づいて、その主要成分であるシアニジン誘導体およびクロロゲン酸が、本願に係る搾汁残渣および分離果肉皮に存在するか否かをHPLC法による定量分析によって検討した。その結果、シアニジン誘導体は残渣および分離果肉皮1 g中にそれぞれ0.057および0.117 mgが含まれており、果汁1 mL中濃度0.235 mgに比べると少ないものの、残渣の中では分離果肉皮に多く含まれていることが分かった。さらに、クロロゲン酸は残渣および分離果肉皮1 g中にそれぞれ1.552および3.150 mg含まれており、これは果汁1 mL中濃度1.018 mgに比べても多く、シアニジン誘導体と同様に果肉皮に多く含まれていることを明らかにした。したがって、この分離方法によって、残渣中に含まれる活性成分を特異的に多く含む部分を選択的に分離することを可能とした。
表3に、それぞれのシアニジン誘導体およびクロロゲン酸濃度測定結果を示す。
Furthermore, based on the fact that useful components in fruit juice have already been identified, whether or not the cyanidin derivative and chlorogenic acid, which are the main components, are present in the squeezed residue and separated pulp skin according to the present application is determined by HPLC. It was examined by quantitative analysis. As a result, the cyanidin derivative contained 0.057 and 0.117 mg in 1 g of residue and separated pulp skin, respectively, which is less than the concentration of 0.235 mg in 1 mL of fruit juice, but contained in the separated pulp skin in the residue. I found out. In addition, chlorogenic acid is contained in 1.552 and 3.150 mg in 1 g of residue and isolated pulp skin, respectively, which is higher than the concentration of 1.018 mg in 1 mL of fruit juice and as much in the pulp skin as in cyanidin derivatives. Made clear. Therefore, this separation method makes it possible to selectively separate a portion containing a large amount of the active ingredient contained in the residue.
Table 3 shows each cyanidin derivative and chlorogenic acid concentration measurement results.

Figure 0004324674
Figure 0004324674

上述のように、上記の搾汁残渣の抗酸化活性を向上させるために、残渣から種子と果肉皮を分離する方法が発明され、分離した果肉皮が有用成分を特異的に多く含む部分であることが証明された。
表4に、分離果肉皮の一般的栄養成分分析結果を示す。
As described above, in order to improve the antioxidant activity of the above juice residue, a method for separating seeds and flesh peel from the residue was invented, and the separated flesh peel is a part containing a large amount of useful components. It was proved.
Table 4 shows the general nutritional component analysis results of the separated flesh skin.

Figure 0004324674
Figure 0004324674

表4に示す通り、分離果肉皮は水分4.5%、粗タンパク質5.3%、粗脂肪3.8%、灰分1.8%、食物繊維59.8%およびその他の炭水化物24.8%で構成され、ビタミンCは検出されなかったことから、分離果肉皮の強い抗酸化作用は上記のアントシアニン誘導体およびクロロゲン酸によるものであることが示された。これらの成分は、すでに本願出願人による研究においてその有用性が明らかとなっており、またこの分離果肉皮を大量に含む餌を実験動物に2週間与えた場合に、体重、摂食量、臓器重量および血液生化学値に何ら異常は見られなかったことから、ガマズミ搾汁残渣の有用成分を濃縮した食品素材となり得ることが証明された。   As shown in Table 4, the isolated pericarp was composed of 4.5% moisture, 5.3% crude protein, 3.8% crude fat, 1.8% ash, 59.8% dietary fiber and 24.8% other carbohydrates, and no vitamin C was detected. From the results, it was shown that the strong antioxidant action of the isolated flesh peel was due to the above-mentioned anthocyanin derivatives and chlorogenic acid. The usefulness of these ingredients has already been clarified in the study by the applicant of the present application, and when a diet containing a large amount of this isolated flesh peel is given to experimental animals for 2 weeks, the body weight, food intake, organ weight In addition, since no abnormality was found in the blood biochemical values, it was proved that it could be a food material in which useful components of viburnum juice residue were concentrated.

ガマズミ果汁飲料はビタミンCも豊富で、栄養補助食品ともなり得るが、液体であるため加工食品に利用できる範囲は飲料等に限定されていた。本発明により得られるガマズミ搾汁残渣由来の分離果肉皮は、有用成分を豊富に含み、安全でしかも固体であるため、これをさらに粉末化するなど、食品に利用しやすい形態にした食品素材の製造も行うことができる。また、本発明により得られる分離果肉皮は、種子の主成分である脂肪分の混入が非常に少ないため、脂肪の酸化による分離果肉皮そのものの劣化も抑えられることから、様々な用途にも安定に使用することができる。
つまり、本発明のガマズミ搾汁残渣から成る抗酸化剤は、上述した分離方法によって抗酸化活性が濃縮され、活性成分の含有量も搾汁残渣より多い、果肉皮由来のものである。
Viburnum juice drink is rich in vitamin C and can be a nutritional supplement, but because it is liquid, the range that can be used for processed food has been limited to beverages and the like. The isolated flesh skin derived from viburnum juice residue obtained by the present invention contains abundant useful ingredients, is safe and solid, and therefore is a food material made into a form that can be easily used for food, such as further powdering. Manufacturing can also be performed. In addition, since the separated pulp skin obtained by the present invention contains very little fat, which is the main component of the seeds, it is also possible to suppress degradation of the separated pulp skin itself due to oxidation of fat. Can be used for
That is, the antioxidant consisting of the viburnum juice residue of the present invention is derived from the flesh skin, where the antioxidant activity is concentrated by the separation method described above, and the content of the active ingredient is also greater than the juice residue.

本発明を用いれば、下記実施例にも一部を記載する通り、ガマズミ果実搾汁残渣から分離されたガマズミ果肉皮を用い、これを抽出してなるガマズミ果肉皮の抽出物(上記(3)の発明)、ガマズミ果肉皮由来抗酸化剤(上記(4)の発明)、ガマズミ果肉皮由来粉末状素材(上記(5)の発明、これは、赤色系の粉末である)、錠剤・顆粒・カプセルその他の形態のサプリメント(上記(6)の発明)、あるいはまたガマズミ果実搾汁残渣・それから分離されたガマズミ果肉皮抽出物・もしくはガマズミ果肉皮由来粉末状素材を用いてなる食品・飲料もしくは着色料(上記(7)の発明)等を、構成することができる。   According to the present invention, as described in part in the examples below, an extract of viburnum pericarp formed by using viburnum pericarp isolated from viburnum fruit juice residue (above (3) Invention), viburnum pericarp-derived antioxidant (invention (4) above), viburnum pericarp-derived powdery material (invention (5) above, which is a red powder), tablets, granules, Supplements in capsule form or other forms (invention (6) above), or viburnum fruit juice residue, viburnum pericarp extract isolated from it, or food / beverage or coloring using viburnum pericarp-derived powdered material The fee (the invention of (7) above) and the like can be configured.

アントシアニンやクロロゲン酸を豊富に含む分離果肉皮は、乳鉢や各種粉砕機で容易に粉末状にすることができる。したがって上述の通り、従来のジュース製造用途を超え、粉末状素材として使用することができる。しかも、赤色系天然色素として食品に着色することも可能である。近年、ソテツの赤色系添加物が発ガン性を有するなど問題となっているが、本発明の着色料はアントシアニン系色素などの抗酸化成分を豊富に含有するものであり、すでに動物試験でその有用性と安全性が十分証明されており、充分に従来の天然色素に代替することができる。   The separated flesh skin rich in anthocyanins and chlorogenic acid can be easily powdered with a mortar or various pulverizers. Therefore, as above-mentioned, it can be used as a powder-form raw material beyond the conventional juice manufacture use. Moreover, it is possible to color food as a red natural pigment. In recent years, red additives of cycad have become a problem such as having carcinogenicity, but the colorant of the present invention contains abundant antioxidant components such as anthocyanin pigments and has already been confirmed in animal tests. Its usefulness and safety are well proven, and it can be sufficiently replaced by conventional natural pigments.

また、種子から物理的に分離された果肉皮は、脂肪分が少ないために劣化が進み難いだけでなく、その目的とする食品の形態や用途により多様な大きさの粒子に粉末化することが可能であるため、アントシアニンやクロロゲン酸化合物を含有する抗酸化食品を調理、加工、成形することにより摂取することが可能である。
In addition, the flesh peel physically separated from the seeds is not easy to deteriorate because of its low fat content, but it can be pulverized into particles of various sizes depending on the form and use of the intended food. since possible, cooking antioxidant food containing anthocyanins and chlorogenic acid compounds, machining, it is possible to ingest by molding.

以下の実施例1〜5−2は、ガマズミ果肉皮由来粉末状素材を利用した粉末状加工食品を製造する場合の実施例である。本発明が、これら実施例に限定されないことはいうまでもない。
<実施例1>
ガマズミ分離果肉皮を焙煎したハーブ茶。焙煎前水分4.5%の分離果肉皮50 gを焙煎 (焙煎時間15分間) 後、水分3.5%以下にして得られた粉末加工食品は、色が赤褐色で焙煎後の芳ばしい香りがし、熱湯を用いて溶出して飲用した場合にはハーブ的風味があり、味は苦みもなくまろやかであった。
Examples 1 to 5-2 below are examples in the case of producing a powdered processed food using a viburnum flesh skin derived powdery material. It goes without saying that the present invention is not limited to these examples.
<Example 1>
Herbal tea with roasted viburnum peel. After roasting 50 g of separated peels with a moisture content of 4.5% before roasting (roasting time 15 minutes), the processed powdered food with a moisture content of 3.5% or less has a reddish brown color and a fragrant flavor after roasting. When elution was performed using hot water, it had a herbal flavor and the taste was mild without bitterness.

<実施例2>
ナシ、リンゴ等の果物をベースに一定量のガマズミ分離果肉皮を入れることにより、赤褐色とコクのある風味を増した焼き菓子。焼き菓子用型にバターを薄く塗り、グラニュー糖をまぶしておき、予めオーブンは設定温度にしておく。一方、リンゴやナシの果物は皮を剥き、10〜12等分に切断し、鍋にバターを溶かし、果物を弱火で炒め、全体にバターが馴染んだら砂糖を加える。果物から水分が出てくるので、そのまま焦がさないように表面が透き通るまで煮詰め、最初に用意した焼型にバランスよく並べる。焼き菓子の生地は、生クリーム200 cc、牛乳50 cc、卵3個、砂糖100 g、薄力粉20 g、ガマズミ分離果肉皮粉末50 gを十分かき混ぜることにより作り、果物を並べ入れた型に流し込む。これを予め180度前後にしておいたオーブンに入れ、45分前後焼くと適度に赤褐色とコクのある風味を有した焼き菓子を製造することができる。
<Example 2>
A baked confectionery with a rich reddish brown and rich flavor by adding a certain amount of viburnum separated flesh skin based on fruits such as pears and apples. Apply a thin layer of butter on the mold for baked confectionery, sprinkle with granulated sugar, and keep the oven at a preset temperature. On the other hand, peel the apples and pears, cut them into 10-12 pieces, melt the butter in a pan, stir the fruits over low heat, and add the sugar when the butter is fully mixed. Since moisture comes out from the fruits, boil until the surface is clear so that it does not burn as it is, and arrange it in a well-balanced manner on the first prepared baking mold. The dough for baked confectionery is made by thoroughly mixing 200 cc of fresh cream, 50 cc of milk, 3 eggs, 100 g of sugar, 20 g of weak flour, and 50 g of viburnum separated pulp skin powder, and poured into a mold in which fruits are arranged. When this is put in an oven set at about 180 degrees and baked for about 45 minutes, a baked confectionery with a moderately reddish brown and rich flavor can be produced.

これと同様にして、ガマズミ分離果肉皮粉末を小麦粉、そば粉、うるち米粉などと練り合わせることによって、各種の煎餅のような焼き菓子を製造することができる。   In the same manner, various kinds of baked confectionery such as rice crackers can be produced by kneading viburnum separated pulp and skin powder with wheat flour, buckwheat flour, glutinous rice flour and the like.

<実施例3>
食物繊維や抗酸化成分入りパスタやラーメンなどの麺の製造。最初に卵黄3個、かん水20cc、塩20gをむらなくよく混ぜる。これにラーメン用の薄力粉950 gとガマズミ分離果肉皮50 gを加え、まんべんなく混ぜ合わせる。この時、混ぜ合わせを良くするために足で踏みつけてもよい。十分こねた後、収縮性のラップ資材等に包み30分ほど熟成させ、その後表面に打ち粉をまぶしながら麺棒で延ばし、まとめる。最終的に厚さ2 mm以下に延ばし、幅を15?20 cmにそろえ好みの幅に切り、打ち粉を振りながら切断した麺生地がくっつかないように粉をまぶし、数回両手でもむようにする。これを茹でるとガマズミ果肉皮入のラーメンが製造、調理できる。
<Example 3>
Manufacture of noodles such as pasta and ramen with dietary fiber and antioxidants. First, mix 3 yolks, 20cc brine, and 20g salt thoroughly. Add 950 g of flour for ramen and 50 g of viburnum separated flesh skin and mix thoroughly. At this time, you may step on your feet to improve mixing. After kneading sufficiently, wrap it in shrinkable wrapping material, etc., mature for about 30 minutes, and then spread it with a rolling pin while dusting the surface. Finally, extend it to a thickness of 2 mm or less, cut it to a width of 15 to 20 cm, and sprinkle the flour so that the cut noodle dough does not stick to it, and peel it with both hands several times. Boiled noodles can be made and cooked with viburnum pulp.

<実施例4>
ガマズミ分離果肉皮粉末を果実酒や果実酢として加工する。ガマズミ分離果肉皮を果実酒や果実酢にすることで、鮮やかな赤紫色の果実酒や果実酢となり、色や香りを楽しませてくれる。その果実酒や酢には抗酸化成分が溶出し、ガマズミのこれまで報告されてきた生理機能の効果を十分に得ることができる。製造方法としては、すでに醸造したアルコールや酢酸にガマズミ分離果肉皮粉末を浸漬する方法と、ガマズミ分離果肉皮粉末をアルコール発酵原料として使用する方法があり、ガマズミ分離果肉皮単独でもアルコール発酵は可能であるが、補糖すれば、より効率的に発酵が進む。
<Example 4>
Processed viburnum separated flesh skin powder as fruit liquor or fruit vinegar. By making viburnum separated fruit skins into fruit liquor or fruit vinegar, it becomes a vivid red-purple fruit liquor or fruit vinegar that will delight in color and aroma. Antioxidant components are eluted in the fruit wine and vinegar, and the effects of physiological functions of viburnum that have been reported so far can be sufficiently obtained. There are two methods of manufacturing: the method of immersing the viburnum separated flesh skin powder in already brewed alcohol or acetic acid, and the method of using the viburnum separated flesh skin powder as an alcoholic fermentation raw material. However, if sugar is supplemented, fermentation proceeds more efficiently.

<実施例5−1>
ガマズミ分離果肉皮粉末をサプリメントに加工する。ガマズミ分離果肉皮をポットミル等で微粉末化し、これに糖類等の添加剤(賦形剤) 等を適度に加え、均一に充分に混合する。これを打錠機に供し、打錠・成型することによってガマズミ分離果肉皮を主成分とするガマズミ錠剤を製造することができる。錠剤は糖衣コーティング等により、甘みや光沢を加えることができる。
<Example 5-1>
Processed viburnum separated flesh skin powder into a supplement. The viburnum-separated flesh skin is pulverized with a pot mill or the like, and additives (excipients) such as sugars are added to this, and mixed uniformly and thoroughly. By applying this to a tableting machine, and tableting and molding, a viburnum tablet comprising a viburnum-separated pulp skin as a main component can be produced. Tablets can be sweetened or glossed by sugar coating or the like.

<実施例5−2>
ガマズミ分離果肉皮と添加剤を充分混合したものに適度に水分を加えてさらに混合し、押し出し造粒機で1ミリ径程度のペレットに造粒する。これをさらにマルメライザー等で球状に整形することにより、ガマズミ顆粒を製造することができる。ガマズミ分離果肉皮単独あるいは糖類等の添加剤と均一かつ充分に混合したものを、乾燥状態でカプセル充填することにより、ガマズミカプセルを製造することができる。
<Example 5-2>
A mixture of viburnum-separated flesh peel and additives is mixed with moderate water, and the mixture is further granulated into pellets with a diameter of about 1 mm using an extrusion granulator. Viburnum granules can be produced by further shaping this into a spherical shape with a Malmerizer or the like. Viburnum capsules can be produced by filling capsules in a dry state with a viburnum-separated pericarp alone or a mixture thoroughly and thoroughly mixed with additives such as sugars.

これらサプリメントは、打錠機、造粒機等にあわせて大きさを変えることができるとともに、添加剤の種類や量を変えることによってガマズミ分離果肉皮の含有量やサプリメントの味、摂取時の食感等を調節することができる。これらのガマズミサプリメントは、ガマズミ分離果肉皮の抗酸化成分および食物繊維を補充できることが特徴である。   These supplements can be sized according to the tableting machine, granulator, etc., and by changing the type and amount of additives, the content of viburnum peeled skin, the taste of the supplement, the food at the time of intake The feeling can be adjusted. These viburnum supplements are characterized by being able to supplement antioxidant components and dietary fiber of viburnum isolated flesh skin.

その他、分離果肉皮入りジャムやジュースなどに加工することによって、長期保存も可能な各種加工食品の材料としても利用できる。またヨーグルトなどに加えて醗酵させることによりガマズミの赤紫色のアントシアニンが溶出した美しい色彩と抗酸化活性の高いヨーグルトを加工製造することができる。   In addition, it can be used as a material for various processed foods that can be stored for a long period of time by processing into jam or juice with separated pulp skin. In addition to yogurt and the like, it is possible to process and produce a yogurt with a beautiful color and a high antioxidative activity, in which viburnum reddish purple anthocyanin is eluted.

本発明は上述のように構成されるため、これによれば、ガマズミ果汁製造工程において産する種子と果肉皮からなる搾汁残渣から果肉皮のみを効率的に分離することができ、その技術に基づいて、種々の有用な生理活性物質を抽出物や添加食品、抗酸化剤等の諸形態で提供することができる。また、ガマズミ果汁飲料の製造量の増加とともに増大し、従来廃棄処分されてきた搾汁残渣について、ゼロエミッション化が可能となる。特に、従来はジュース製造用途のみしかなかったガマズミ果実を、本発明によって粉末状素材化でき、種々の付加価値製品を応用開発することができる。したがって、農業・農産加工業、食品製造業、その他関連産業分野において利用価値が高い発明である。   Since the present invention is configured as described above, according to this, it is possible to efficiently separate only the flesh peel from the juice residue consisting of seeds and flesh peel produced in the viburnum juice manufacturing process. Based on this, various useful physiologically active substances can be provided in various forms such as an extract, an additive food, and an antioxidant. Moreover, it increases with the increase in the production amount of a viburnum fruit juice drink, and the squeeze residue that has been conventionally disposed of can be made zero emission. In particular, viburnum fruit, which has conventionally only been used for juice production, can be made into a powdery material according to the present invention, and various value-added products can be applied and developed. Therefore, the invention has high utility value in the fields of agriculture / agricultural processing, food manufacturing, and other related industries.

本発明のガマズミ果肉皮の製造方法を示すフロー図である。It is a flowchart which shows the manufacturing method of the viburnum pericarp of this invention. 本発明のガマズミ果肉皮製造装置の機構の基本構成例を示す説明図である。It is explanatory drawing which shows the example of a basic composition of the mechanism of the viburnum peel manufacturing apparatus of this invention.

符号の説明Explanation of symbols

1…ガマズミ果実搾汁残渣
2…乾燥搾汁残渣
3…果肉皮
4…種子
5…ガマズミ果肉皮由来粉末状素材
100…ガマズミ果肉皮製造装置
10…原料供給口
20…分離部
24…ロータ
28…網状筒型容器
30…果肉皮受け部
50…モータ
P1搾汁残渣を乾燥させる過程
P2…種子と果肉皮の分離過程
P3…粉末化過程
DESCRIPTION OF SYMBOLS 1 ... Viburnum fruit squeezed residue 2 ... Dry squeezed residue 3 ... Flesh peel 4 ... Seed 5 ... Viburnum flesh peel derived powdery material 100 ... Viburnum flesh peel production apparatus 10 ... Raw material supply port 20 ... Separation part 24 ... Rotor 28 ... Reticulated cylindrical container 30 ... pulp skin receiving part 50 ... motor P1 ... process of drying juice residue P2 ... separation process of seed and pulp skin P3 ... powdering process

Claims (7)

一粒ごとに種子に薄く果肉皮が密着し一体となっているガマズミ果実搾汁残渣を、該ガマズミ果実搾汁残渣各粒間相互の研磨作用を行える精米機様構造で処理することによって、アントシアニン、クロロゲン酸ならびにその誘導体をより多く含有する果肉皮を、種子をほとんど損傷せずに種子から分離することにより行う、 ガマズミ果肉皮の製造方法。 By treating the viburnum fruit juice residue, in which the pericarp is thinly attached to the seed for each grain, with a rice milling machine-like structure capable of polishing each grain of the viburnum fruit juice residue, anthocyanins are obtained. A method for producing viburnum pericarp, comprising separating a pericarp containing more chlorogenic acid and derivatives thereof from the seed with little damage to the seed . 一粒ごとに種子に薄く果肉皮が密着し一体となっているガマズミ果実搾汁残渣を後記分離部へ供給する原料供給口と、供給される該ガマズミ果実搾汁残渣を種子とガマズミ果肉皮とに分離する分離部と、分離された該ガマズミ果肉皮を受ける果肉皮受け部と、およびこれらを包含してなる筐体とからなるガマズミ果肉皮製造装置であって、該分離部は、該ガマズミ果実搾汁残渣を回転させつつこれに精米機の様に該ガマズミ果実搾汁残渣各粒間相互における研磨作用を施すロータと、該ロータにおける作用により剥離されたガマズミ果肉皮を種子をほとんど損傷することなく種子と分離して該果肉皮受け部へ排出するための網状筒型容器を備えている、ガマズミ果肉皮製造装置。 The raw material supply port for supplying the viburnum fruit juice residue, which is thinly attached to the seed for each grain and integrated into the seed portion, to the separation unit, and the viburnum fruit juice residue supplied to the seed and viburnum peel A viburnum peel manufacturing apparatus comprising: a separation part that separates into pieces; a flesh skin receiving part that receives the separated viburnum peel; and a casing that includes these parts; and the separation part comprises the viburnum Rotating the fruit juice residue, rotating the viburnum fruit juice residue between each grain like a rice milling machine, and the seeds of the viburnum flesh peeled by the action of the rotor are almost damaged. An apparatus for producing a viburnum pulp skin, comprising a reticulated cylindrical container for separating the seeds and discharging them to the pulp skin receiver without any separation. 請求項1に記載の製造方法により得られるガマズミ果肉皮を抽出してなる、ガマズミ果肉皮の抽出物。 An extract of viburnum pericarp obtained by extracting viburnum pericarp obtained by the production method according to claim 1 . 請求項1に記載の製造方法により得られるガマズミ果肉皮を用いてなる、ガマズミ果肉皮由来抗酸化剤。 A viburnum pericarp-derived antioxidant comprising the viburnum pericarp obtained by the production method according to claim 1 . 請求項1に記載の製造方法により得られるガマズミ果肉皮を用いてなる、ガマズミ果肉皮由来粉末状素材。 A powdery raw material derived from viburnum pericarp using the viburnum pericarp obtained by the production method according to claim 1 . 請求項5に記載のガマズミ果肉皮由来粉末状素材を用いてなる、錠剤、顆粒、カプセルその他の形態のサプリメント。 A supplement in the form of a tablet, granule, capsule or the like, using the powdered raw material derived from viburnum pericarp according to claim 5. 請求項3に記載のガマズミ果肉皮抽出物または請求項5に記載のガマズミ果肉皮由来粉末状素材を用いてなる、食品、飲料または着色料。
A food, beverage or colorant comprising the viburnum pericarp extract according to claim 3 or the viburnum pericarp derived powdery material according to claim 5.
JP2004338715A 2004-11-24 2004-11-24 Viburnum pericarp manufacturing method, viburnum pericarp manufacturing apparatus, viburnum pericarp extract, antioxidants derived from viburnum pericarp, powdered material derived from viburnum pericarp and processed products using viburnum pericarp Expired - Fee Related JP4324674B2 (en)

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