JP2006257381A - Water-soluble metal-containing paint composition - Google Patents

Water-soluble metal-containing paint composition Download PDF

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JP2006257381A
JP2006257381A JP2005244348A JP2005244348A JP2006257381A JP 2006257381 A JP2006257381 A JP 2006257381A JP 2005244348 A JP2005244348 A JP 2005244348A JP 2005244348 A JP2005244348 A JP 2005244348A JP 2006257381 A JP2006257381 A JP 2006257381A
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metal
powder
water
coating composition
soluble metal
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Taisei Shin
泰正 辛
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    • E—FIXED CONSTRUCTIONS
    • E03—WATER SUPPLY; SEWERAGE
    • E03B—INSTALLATIONS OR METHODS FOR OBTAINING, COLLECTING, OR DISTRIBUTING WATER
    • E03B11/00—Arrangements or adaptations of tanks for water supply
    • E03B11/02—Arrangements or adaptations of tanks for water supply for domestic or like local water supply
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B65—CONVEYING; PACKING; STORING; HANDLING THIN OR FILAMENTARY MATERIAL
    • B65D—CONTAINERS FOR STORAGE OR TRANSPORT OF ARTICLES OR MATERIALS, e.g. BAGS, BARRELS, BOTTLES, BOXES, CANS, CARTONS, CRATES, DRUMS, JARS, TANKS, HOPPERS, FORWARDING CONTAINERS; ACCESSORIES, CLOSURES, OR FITTINGS THEREFOR; PACKAGING ELEMENTS; PACKAGES
    • B65D88/00—Large containers
    • B65D88/26—Hoppers, i.e. containers having funnel-shaped discharge sections
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B65—CONVEYING; PACKING; STORING; HANDLING THIN OR FILAMENTARY MATERIAL
    • B65D—CONTAINERS FOR STORAGE OR TRANSPORT OF ARTICLES OR MATERIALS, e.g. BAGS, BARRELS, BOTTLES, BOXES, CANS, CARTONS, CRATES, DRUMS, JARS, TANKS, HOPPERS, FORWARDING CONTAINERS; ACCESSORIES, CLOSURES, OR FITTINGS THEREFOR; PACKAGING ELEMENTS; PACKAGES
    • B65D88/00—Large containers
    • B65D88/74—Large containers having means for heating, cooling, aerating or other conditioning of contents

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  • Engineering & Computer Science (AREA)
  • Mechanical Engineering (AREA)
  • Structural Engineering (AREA)
  • Health & Medical Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Hydrology & Water Resources (AREA)
  • Public Health (AREA)
  • Water Supply & Treatment (AREA)
  • Paints Or Removers (AREA)

Abstract

<P>PROBLEM TO BE SOLVED: To provide a water-soluble metal-containing paint composition which is free from problems that a conventional metallic coating paint and a metallic coating method embrace, and allows the metal to exhibit the inherent feeling and color. <P>SOLUTION: The water-soluble metal-containing paint composition comprises 100 wt% of a metallic paint powder and 30 wt% of an acrylate binder, wherein the metallic paint powder comprises 85-96 wt% of a metallic powder, 2-8 wt% of a glass powder, and 2-7 wt% of a melamine cyanurate powder. <P>COPYRIGHT: (C)2006,JPO&NCIPI

Description

本発明は水溶性塗料組成物に関し、特に金属粉末、ガラスパウダー及びメラミン系難燃材（Melamine Cyanurate）粉末をアクリル系バインダーと混合して被塗布体に塗布可能な液状難燃金属を含有する塗料組成物に関する。   TECHNICAL FIELD The present invention relates to a water-soluble paint composition, and in particular, a paint containing a liquid flame retardant metal that can be applied to a substrate by mixing metal powder, glass powder, and melamine flame retardant powder (Melamine Cyanurate) powder with an acrylic binder. Relates to the composition.

通常、被塗布体に金属質感を表現する方法としては、金属ペイント（Metallic paint）を塗布したり、塗布鍍金、または蒸着するなどの方式、もしくは直に金属を溶かして被塗布体に噴射する熱スプレー（Thermo spray）方式などがある。   Usually, as a method of expressing the metallic texture on the coated body, a method such as applying metallic paint, coating plating, or vapor deposition, or directly melting the metal and injecting it onto the coated body There is a spray (Thermo spray) method.

金属ペイントは、油性溶剤に金属粉末を少量添加して、染料で金属の固有色を表現する方式であるが、これは被塗布体に金属固有の質感や色を表現するには十分ではない。   Metal paint is a method in which a small amount of metal powder is added to an oil-based solvent and the inherent color of the metal is expressed with a dye. However, this is not sufficient to express the texture and color inherent to the metal on the substrate.

鍍金や蒸着などの方式は、一般的に鍍金対象物の種類によって複雑な前処理過程を必要とし、また対象物の化学的、物理的性質によって多くの制限を受ける。   Methods such as plating and vapor deposition generally require a complicated pretreatment process depending on the type of plating object, and are subject to many limitations depending on the chemical and physical properties of the object.

熱スプレー方式は、金属の固有の質感表現ができるが、金属を溶融点以上に加熱した後、スプレーする方式として、高価な装備及び技術が必要であると共に、熱による被塗布体の変形及び滅失などの多くの制約を受ける。   The thermal spray method can express the unique texture of metal, but it requires expensive equipment and technology as a method of spraying after heating the metal to the melting point or higher, and deformation and loss of the coated object due to heat. Subject to many restrictions.

従って、本発明は前記のような従来技術の問題点を解消するために創案するものである。
本発明の目的は、前記のような従来の金属塗装塗料及び他の金属塗装方法が有している問題点を解消し、金属が有する固有の質感及び色をそのまま生かす水溶性金属含有塗料組成物を提供することである。 Therefore, the present invention is devised to solve the problems of the prior art as described above.
An object of the present invention is to solve the problems of the conventional metal coating paint and other metal coating methods as described above, and to use the water-soluble metal-containing coating composition that makes use of the unique texture and color of the metal as it is. Is to provide.

前記目的を実現するために、本発明の水溶性金属含有塗料組成物は、 金属粉末８５〜９６重量％、ガラスパウダー２〜８重量％及びメラミンシアヌレート粉末２〜７重量％を含む金属塗料粉末及びその金属塗料粉末の総重量に対して３０重量％のアクリレート結合剤を含む。
前記金属塗料粉末は、好ましくは、金属粉末９５重量％、ガラスパウダー３重量％及びメラミンシアヌレート粉末２重量％を含有するのがよい。
前記金属は、銅、青銅、黄銅、鉄、ニッケル、アルミニウム、金、銀からなる群より選ばれる少なくとも１つの金属であって、特に 銅、青銅、もしくは黄銅を用いるのが好ましい。
前記金属粉末の大きさは１０〜３００μmであり、ガラスパウダーの大きさは１００〜３００μmであり、そしてメラミンシアヌレートの大きさは１０μm以下である。
前記アクリレート結合剤としては、Ｃ１−Ｃ６のアクリル酸アルキルエステルを用いるのが好ましく、特にアクリル酸メチルを用いるのがより好ましい。
本発明による水溶性金属含有塗料組成物は、スプレー、筆塗装、パター塗装などを用いることができ、その塗装方法に特別な制約を受けない。また、木材、金属、ポリビニルクロライド（ＰＶＣ）、ウレタン、メラミン発砲フォームなどのある素材にも適用ができて適用対象にも制約を受けない。
また、本発明の組成物は、水溶性で油性金属含有塗料と違って揮発性有機化合物や他の有害な環境ホルモンが発生しない。 To achieve the above object, the water-soluble metal-containing coating composition of the present invention comprises a metal coating powder comprising 85 to 96% by weight of metal powder, 2 to 8% by weight of glass powder, and 2 to 7% by weight of melamine cyanurate powder. And 30 wt% acrylate binder based on the total weight of the metal paint powder.
The metal paint powder preferably contains 95% by weight of metal powder, 3% by weight of glass powder and 2% by weight of melamine cyanurate powder.
The metal is at least one metal selected from the group consisting of copper, bronze, brass, iron, nickel, aluminum, gold, and silver, and it is particularly preferable to use copper, bronze, or brass.
The metal powder has a size of 10 to 300 μm, the glass powder has a size of 100 to 300 μm, and the melamine cyanurate has a size of 10 μm or less.
The acrylate binder is preferably a C1-C6 alkyl acrylate ester, and more preferably methyl acrylate.
The water-soluble metal-containing coating composition according to the present invention can be sprayed, brush-painted, putter-painted, etc., and is not subject to any particular restrictions on the coating method. Moreover, it can be applied to certain materials such as wood, metal, polyvinyl chloride (PVC), urethane, melamine foam, and is not restricted by the application target.
In addition, the composition of the present invention does not generate volatile organic compounds and other harmful environmental hormones, unlike water-soluble and oily metal-containing paints.

本発明の水溶性金属含有塗料組成物は、既存の金属質感ペイントや油性金属含有塗料と違って、揮発性有機化合物や他の有害な環境ホルモンが発生せず、常温乾燥形で熱処理をする既存方式とは大きく異なる。
また、ガラスパウダーの添加により、表面の耐磨耗性が上昇して硬度が高まり、磨耗による損傷を防止する効果があり、また、メラミン系難燃材の添加によって難燃２等級に該当する難燃効果を期待することができる。
本発明の水溶性金属含有塗料組成物は、また、スプレー、筆塗装、パター塗装などの使用に対しても制約を受ず、また、木材、金属、ポリビニルクロライド（ＰＶＣ）、ウレタン、メラミン発砲フォームなどのある素材にも適用ができて適用対象にも制約を受けない。このため、低価格の原資材を用いて高価格の製品を生産することができ、製品の付加価値を高めることができる。 The water-soluble metal-containing paint composition of the present invention is different from existing metal texture paints and oil-based metal-containing paints, and does not generate volatile organic compounds or other harmful environmental hormones. It is very different from the method.
In addition, the addition of glass powder increases the wear resistance of the surface and increases the hardness, thereby preventing damage due to wear. Also, the addition of melamine-based flame retardants makes it difficult to meet the second grade of flame resistance. A fuel effect can be expected.
The water-soluble metal-containing coating composition of the present invention is not restricted for use in spraying, brush painting, putter painting, etc., and wood, metal, polyvinyl chloride (PVC), urethane, melamine foamed foam It can also be applied to certain materials and is not subject to restrictions. For this reason, a high-priced product can be produced using low-priced raw materials, and the added value of the product can be increased.

本発明は、各々固有の性質を保有した金属粉末、ガラスパウダー、メラミン系難燃材及び水溶性アクリル系バインダーを混合、組成して低価な費用及び努力で高価な金属質感及び色を有する水溶性難燃金属塗料含有組成物を製造する。
本発明による液状の水溶性難燃金属含有塗料組成物は、大きさ１０〜３００μmの金属粉末８５〜９６重量％、大きさ１００〜３００μmのガラスパウダー２〜８重量％及び大きさ１０μm以下のメラミン系難燃材粉末２〜７重量％を含有する金属塗料粉末の総重量に対してアクリル系結合剤３０重量％と混合して製造する。 The present invention mixes and composes metal powders, glass powders, melamine flame retardants and water-soluble acrylic binders each having unique properties to form a water-soluble water with an expensive metal texture and color at low cost and effort. A flame retardant metal paint-containing composition is produced.
The liquid water-soluble flame-retardant metal-containing coating composition according to the present invention comprises 85 to 96% by weight of metal powder having a size of 10 to 300 μm, 2 to 8% by weight of glass powder having a size of 100 to 300 μm, and melamine having a size of 10 μm or less. It is manufactured by mixing with 30% by weight of an acrylic binder based on the total weight of the metal paint powder containing 2 to 7% by weight of the flame retardant powder.

本発明に適用された金属粉末は、 被塗布体に金属質感を表すために用いられたもので、銅、青銅、黄銅、鉄、ニッケル、アルミニウム、金、銀などの粉末を用いることができ、特に銅を用いるのが好ましい。
前記金属粉末を８５重量％以下で用いた場合、所望の金属の質感が十分現れず、また９６重量％以上で用いた場合には、 被塗布体の質感が非常に厚ぼったくなったり、表面の美麗性を害してしまう。 The metal powder applied to the present invention is used to express the metal texture on the coated body, and powders of copper, bronze, brass, iron, nickel, aluminum, gold, silver, etc. can be used, It is particularly preferable to use copper.
When the metal powder is used in an amount of 85% by weight or less, the desired metal texture does not appear sufficiently, and when it is used in an amount of 96% by weight or more, the texture of the coated body becomes very thick or the surface is beautiful. It will harm the sex.

本発明に適用されたガラスパウダーは、遠心力法または火炎法で生産された単繊維パウダーを用いることができ、これは本発明の塗料組成物に優れた耐熱性、耐火性及び電気絶縁性を提供するためのものである。
前記ガラスパウダーを２重量％以下で用いた場合、その本来の目的である優れた耐熱性、耐火性及び電気絶縁性を提供することができず、また８重量％以上で用いた場合には、被塗布体の表面の美麗性を害してしまう。 As the glass powder applied to the present invention, a single fiber powder produced by a centrifugal force method or a flame method can be used, which has excellent heat resistance, fire resistance and electrical insulation properties to the coating composition of the present invention. It is for providing.
When the glass powder is used in an amount of 2% by weight or less, it cannot provide excellent heat resistance, fire resistance and electrical insulation, which are its original purposes, and when it is used in an amount of 8% by weight or more, The beauty of the surface of the coated body will be damaged.

本発明に適用されたメラミン系難燃材としては、メラミンシアヌレート（分子式：Ｃ6Ｈ9Ｎ9Ｏ3）を用いることができ、これは燃焼中に窒素ガスを放出して酸素の供給を遮断したり希釈させて燃焼の進行を抑制する作用をする。
前記メラミン系難燃材を２重量％以下で用いた場合、その本来の目的である燃焼性を得ることができず、また７重量％以上で用いた場合には、被塗布体の表面の美麗性を害してしまう。 Melamine cyanurate (molecular formula: C 6 H 9 N 9 O 3 ) can be used as the melamine-based flame retardant applied in the present invention, which releases nitrogen gas during combustion to supply oxygen. Blocks or dilutes to suppress the progress of combustion.
When the melamine flame retardant is used at 2% by weight or less, the original combustibility cannot be obtained, and when it is used at 7% by weight or more, the surface of the coated body is beautiful. It will harm the sex.

本発明に適用されたアクリル系結合剤は、粘度３００〜５００ｃＰ（２５℃）であるのが好ましい。また前記アクリル系結合剤としては、例えば、アクリル酸メチル、アクリル酸エチル、アクリル酸プロピル、アクリル酸ブチル、アクリル酸ペンチル、アクリル酸へキシルなどのＣ１−Ｃ６のアクリル酸アルキルエステルを用いるのが好ましく、より好ましくはアクリル酸メチル（ＣＨ2＝ＣＨＣＯＯＣＨ3）である。 The acrylic binder applied to the present invention preferably has a viscosity of 300 to 500 cP (25 ° C.). Further, as the acrylic binder, for example, it is preferable to use C1-C6 alkyl acrylate such as methyl acrylate, ethyl acrylate, propyl acrylate, butyl acrylate, pentyl acrylate, hexyl acrylate and the like. And more preferably methyl acrylate (CH 2 ═CHCOOCH 3 ).

本発明の水溶性金属含有塗料組成物は、低温、低速の一般攪拌器を用いて結合剤→メラミン系難燃材粉末→ガラスパウダー→金属粉末の順に攪拌器に混入して常温２５℃で攪拌して製造する。
前記方法は水溶性、常温乾燥形に他の硬化剤やシンナーなどを添加しない。 The water-soluble metal-containing coating composition of the present invention is mixed in a stirrer in the order of binder → melamine flame retardant powder → glass powder → metal powder using a low temperature, low speed general stirrer and stirred at room temperature at 25 ° C. To manufacture.
The above method does not add any other curing agent or thinner to the water-soluble, room temperature dry form.

前記のようにして得られた本発明による水溶性金属含有塗料組成物は、各々相違な特性を有する金属粉末、ガラスパウダー及びメラミン系難燃材粉末をアクリル系結合剤と結合することによって、金属が有する特有の質感及び色を表現し、同時にガラスパウダーが有する絶縁性及び耐熱性と共に、メラミン系難燃材粉末の吸着性及び難燃性を有し、さらに被塗布体表面の美麗さを保持する耐磨耗性などを有する多機能性塗料組成物である。   The water-soluble metal-containing coating composition according to the present invention obtained as described above is obtained by combining metal powder, glass powder and melamine flame retardant powder, each having different characteristics, with an acrylic binder. Represents the unique texture and color of glass, and at the same time has the insulating properties and heat resistance of glass powder, as well as the adsorptivity and flame retardancy of melamine-based flame retardant powder, and also maintains the beauty of the coated surface It is a multifunctional coating composition having wear resistance and the like.

本発明による水溶性金属含有塗料組成物は、被塗布体に、一般的なスプレー、筆塗装、パター塗装などの塗装方法によって塗布することができ、塗装方法には、特に制約を受けない。   The water-soluble metal-containing coating composition according to the present invention can be applied to a substrate by a general coating method such as spraying, brush painting, or putter coating, and the coating method is not particularly limited.

また、本発明による水溶性金属含有塗料組成物は、木材、金属、ポリビニルクロライド（ＰＶＣ）、ウレタン、メラミン発砲フォームなどのある素材にも適用することができ、適用対象にも制約を受けない。   Moreover, the water-soluble metal-containing coating composition according to the present invention can be applied to a certain material such as wood, metal, polyvinyl chloride (PVC), urethane, melamine foam, and is not restricted by the application target.

本発明による水溶性金属含有塗料組成物の乾燥時間は３〜５時間であって、１８〜２４時間後、完全に硬化される。
塗料組成物が完全に硬化した後、金属加工用サンドペーパー、ブラシ、グラインダーなどで研磨し、金属光沢剤の塗布などで仕上げ作業をする。 The water-soluble metal-containing coating composition according to the present invention has a drying time of 3 to 5 hours, and is completely cured after 18 to 24 hours.
After the coating composition is completely cured, it is polished with a sandpaper for metal processing, a brush, a grinder, etc., and finished by applying a metallic brightener.

本発明による水溶性金属含有塗料組成物の実施例を図１および図２にを示す。
図１は、実施例１であり、ＰＶＣ板の上に銅含有金属塗料（銅粉末５００ｇ、ガラスパウダー１５ｇ、メラミン系難燃材粉末１０ｇを１６０ｇの水溶性アクリル系バインダーと混合）を筆及びスポイラーで塗布した後、腐食処理して研磨処理した製品として、銅が有する質感及び色を表したものである。
図２は、実施例２であり、木製彫刻品の上に青銅含有金属塗料（青銅粉末５００ｇ、ガラスパウダー１５ｇ、メラミン系難燃材粉末１０ｇを１６０ｇ水溶性アクリル系バインダーと混合）をスプレーで塗布した後、腐食処理して研磨処理した製品として、青銅が有する質感及び色を表したものである。 Examples of the water-soluble metal-containing coating composition according to the present invention are shown in FIGS.
FIG. 1 shows Example 1, in which a copper-containing metal paint (500 g of copper powder, 15 g of glass powder, 10 g of melamine-based flame retardant powder is mixed with 160 g of a water-soluble acrylic binder) on a PVC plate and a spoiler After the coating, the texture and color of copper as a product subjected to corrosion treatment and polishing treatment are shown.
FIG. 2 shows a second embodiment in which a bronze-containing metal paint (500 g of bronze powder, 15 g of glass powder, and 10 g of melamine-based flame retardant powder mixed with 160 g of a water-soluble acrylic binder) is sprayed onto a wooden sculpture. After that, the texture and color of bronze are expressed as a product subjected to corrosion treatment and polishing treatment.

上記実施例１、２に示す通り、本発明による水溶性金属含有塗料組成物は、木材、金属、ポリビニルクロライド（ＰＶＣ）、ウレタン、メラミン発砲フォームなどのある素材にも適用ができ、スプレー、筆塗装、パター塗装など塗装方法に制約を受けないことが分かった。   As shown in Examples 1 and 2 above, the water-soluble metal-containing coating composition according to the present invention can also be applied to materials such as wood, metal, polyvinyl chloride (PVC), urethane, melamine foam, and the like. It was found that there are no restrictions on painting methods such as painting and putter painting.

本発明にかかる実施形態の一例を示すＰＶＣ板上に塗布した場合の表面を表す図である。It is a figure showing the surface at the time of apply | coating on the PVC board which shows an example of embodiment concerning this invention. 本発明にかかる実施形態の一例を示す木製品上に塗布した場合の図である。It is a figure at the time of apply | coating on the wooden product which shows an example of embodiment concerning this invention.

Claims (7)

金属粉末８５〜９６重量％、ガラスパウダー２〜８重量％及びメラミンシアヌレート粉末２〜７重量％を含む金属塗料粉末、及びその金属塗料粉末の総重量に対して３０重量％のアクリレート結合剤を含むことを特徴とする水溶性金属含有塗料組成物。 Metal paint powder comprising 85-96 wt% metal powder, 2-8 wt% glass powder and 2-7 wt% melamine cyanurate powder, and 30 wt% acrylate binder based on the total weight of the metal paint powder A water-soluble metal-containing coating composition comprising: 前記金属が、銅、青銅、黄銅、鉄、ニッケル、アルミニウム、金、銀からなる群より選ばれる少なくとも１つの金属であることを特徴とする請求項１記載の水溶性金属含有塗料組成物。 The water-soluble metal-containing coating composition according to claim 1, wherein the metal is at least one metal selected from the group consisting of copper, bronze, brass, iron, nickel, aluminum, gold, and silver. 前記金属粉末の大きさが１０〜３００μm、ガラスパウダーの大きさが１００〜３００μm、及びメラミンシアヌレートの大きさが１０μm以下であることを特徴とする請求項１記載の水溶性金属含有塗料組成物。 The water-soluble metal-containing coating composition according to claim 1, wherein the metal powder has a size of 10 to 300 µm, the glass powder has a size of 100 to 300 µm, and the melamine cyanurate has a size of 10 µm or less. . 前記金属塗料粉末が、金属粉末９５重量％、ガラスパウダー３重量％及びメラミンシアヌレート粉末２重量％を含むことを特徴とする請求項１記載の水溶性金属含有塗料組成物。 The water-soluble metal-containing coating composition according to claim 1, wherein the metal coating powder contains 95% by weight of metal powder, 3% by weight of glass powder, and 2% by weight of melamine cyanurate powder. 前記アクリレート結合剤が、Ｃ１−Ｃ６のアクリル酸アルキルエステルであることを特徴とする請求項１記載の水溶性金属含有塗料組成物。 The water-soluble metal-containing coating composition according to claim 1, wherein the acrylate binder is a C1-C6 alkyl acrylate ester. 前記アクリレート結合剤が、アクリル酸メチルであることを特徴とする請求項５記載の水溶性金属含有塗料組成物。 The water-soluble metal-containing coating composition according to claim 5, wherein the acrylate binder is methyl acrylate. 攪拌器に、結合剤→メラミン系難燃材粉末→ガラスパウダー→金属粉末の順に混入して常温２５℃で攪拌して製造することを特徴とする水溶性金属含有塗料組成物の製造方法。
A method for producing a water-soluble metal-containing coating composition comprising mixing in a stirrer in the order of binder → melamine flame retardant powder → glass powder → metal powder and stirring at room temperature of 25 ° C.
JP2005244348A 2005-03-16 2005-08-25 Water-soluble metal-containing paint composition Pending JP2006257381A (en)

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CN102993873A (en) * 2012-12-27 2013-03-27 海南红杉科创实业有限公司 Interior wall heat insulation coating
CN107216748A (en) * 2017-08-04 2017-09-29 浙江喜泽荣制漆有限公司 A kind of aqueous emulation copper coating and preparation method thereof
CN109897523A (en) * 2019-02-20 2019-06-18 张建初 A kind of preparation method of environmental protection scratch-resistant hand-feeling coating

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KR100935657B1 (en) * 2007-12-11 2010-01-07 (주)코스페이스 Terminal for vehicle and method for controlling terminal for vehicle

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* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN102993873A (en) * 2012-12-27 2013-03-27 海南红杉科创实业有限公司 Interior wall heat insulation coating
CN107216748A (en) * 2017-08-04 2017-09-29 浙江喜泽荣制漆有限公司 A kind of aqueous emulation copper coating and preparation method thereof
CN107216748B (en) * 2017-08-04 2019-03-29 浙江喜泽荣制漆有限公司 Aqueous emulation copper coating of one kind and preparation method thereof
CN109897523A (en) * 2019-02-20 2019-06-18 张建初 A kind of preparation method of environmental protection scratch-resistant hand-feeling coating

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