IL42867A - Method and compositions for zinc electroplating - Google Patents

Method and compositions for zinc electroplating

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Publication number
IL42867A
IL42867A IL42867A IL4286773A IL42867A IL 42867 A IL42867 A IL 42867A IL 42867 A IL42867 A IL 42867A IL 4286773 A IL4286773 A IL 4286773A IL 42867 A IL42867 A IL 42867A
Authority
IL
Israel
Prior art keywords
nitrogen
heterocyclic compound
containing heterocyclic
integer
composition
Prior art date
Application number
IL42867A
Original Assignee
M & T Chemicals Inc
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by M & T Chemicals Inc filed Critical M & T Chemicals Inc
Publication of IL42867A publication Critical patent/IL42867A/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C25ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25DPROCESSES FOR THE ELECTROLYTIC OR ELECTROPHORETIC PRODUCTION OF COATINGS; ELECTROFORMING; APPARATUS THEREFOR
    • C25D3/00Electroplating: Baths therefor
    • C25D3/02Electroplating: Baths therefor from solutions
    • C25D3/22Electroplating: Baths therefor from solutions of zinc

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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • Materials Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Electroplating And Plating Baths Therefor (AREA)
  • Pyridine Compounds (AREA)
  • Compounds Of Alkaline-Earth Elements, Aluminum Or Rare-Earth Metals (AREA)
  • Compositions Of Oxide Ceramics (AREA)

Abstract

1394637 Additives for bright zinc electroplating baths M & T CHEMICALS Inc 24 Sept 1973 [26 Sept 1972] 44715/73 Heading C7B A bright zinc electro-deposit is produced from an aqueous bath containing (1) at least one zinc ion yielding compound, (2) at least one bathsoluble surfactant selected from substituted or unsubstituted polyethers or non-aromatic heterocyclic nitrogen compounds and (3) at least one aromatic non-carbonyl heterocyclic nitrogen compound. Component (2) may be a polyalkoxylated alkyl phenol, a quarternary imidazolinium compound, polyvinyl pyrrolidone or a polyethylene- or polypropylene glycol which may carry C(5-25) alkyl end groups. Component (3) may be pyridine, quinoline, izoquinoline or acridine or a derivative thereof. General formulae for and long lists of components (2) and (3) are given. Concentrations of 1-25 g/l and 0.001-4 g/l respectively of these components may be used in a weight ratio of 100-1 to 0.5-1. Plating conditions may include a bath temperature of 10-60‹C, a c.d. of 0.5- 5A/dm<SP>2</SP>, a pH of 1-10, a plating time of 0.5-120 min and a plating thickness of 0.25-25 microns Barrel plating may be used. The plated substrate may be steel, Fe, Cu, brass, bronze, Ni or Ag and may be a thin coating on a non-conductive substrate. Specified baths contain (1) ZnSo 4 or ZnCl 2 and NH 4 Cl optionally with citric acid and NH 4 OH as buffer or (2) Zn and NH 4 sulphamates and NH 4 OH buffer, in addition to the components (2) and (3) above. The plated zinc may be chromated by conversion coating. [GB1394637A]

Claims (9)

1. CLAIMS: 1. A method of producing bright, or brilliant zinc electrodeposits free of"spores" and/or striations over a wide current density range which comprises passing current from an anode to a metal cathode through an aqueous bath composition containing at least one zinc compound providing zinc ions for electroplating zinc, (a) at least one bath soluble surfactant selected from the group consisting of bath soluble polyethers , substituted polyethers, and substituted non-aromatic nitrogen heterocyclic surfactants; and (b) at least one aromatic, non-carbonyl, nitrogen-containing heterocyclic compound for a time period sufficient to deposit a bright zinc electro- deposit upon said cathode.
2. The method as claimed in Claim 1 wherein at least one nitrogen-containing heterocyclic compound is of the formula wherein each R is independently hydrogen, alkyl, alkenyl, alkoxy, alkylamine, alkylsulfonic acid or salts thereof, sulfonic acid or salts thereof, halogen, amine, hydroxyl, mer capto, nitrile, benzyl, or phenylalkyl (where m is an integer 0 to );n is an integer z is 0 or 1; Y is oxygen, allyl, propargyl, benzyl, an alkoxy group, alkyl sulfonic acid -(CH2)p-S03®(where p is an integer of from 1 to 4), an oxyalkylsulfonic acid, quinaldinyl, p-phenoxybenzyl or a halogenated alkeneyl radical and X" represents an anionic radical or the anionic moiety of Y or R provided that when Y is N-oxide x" is absent.
3. The method as claimed in Claim 2 wherein at least one nitrogen-containing heterocyclic compound is N-(2,3-dichlo o-2-propenyl)-pyridinium chloride. k . The method as claimed in Claim 2 wherein at least one nitrogen-containing heterocyclic compound is N-propargyl-2-(n-propan-3-ol)-pyr idinium bromide. 5. The method as claimed in Claim 2 wherein at least one nitrogen-containing heterocyclic compound is 2-mercapto-4-methylpyridine . 6. The method as claimed in Claim 2 wherein at least one nitrogen-containing heterocyclic compound is -cyanopyr idine-N-oxide. 7. The method as claimed in Claim 2 wherein at least one nitrogen-containing heterocyclic compound is 4-cyanopyridine . 8. The method as claimed in Claim 2 wherein at least one nitrogen-containing heterocyclic compound is 3-pyridylsulfonic acid. 9. The method as claimed in Claim 1 wherein at least one nitrogen-containing heterocyclic compound is of the formula wherein each R is independently hydrogen, alkyl, alkenyl, alkoxy, alkylamine, alkylsulfonic acid or salts thereof, sulfonic acid or salts thereof, halogen, amine, hydroxyl, mer- capto, nitrile, benzyl, or phenylalkyl (where m is an integer 0 to ;n is an integer 0 to 3; z is 0 or 1; Y is oxygen, allyl, propargyl, benzyl, an alkoxy group, alkyl sulfonic acid -(CH2)p-S03:( here p is an integer of from 1 to *0, an oxyalkylsulfonic acid, quinaldinyl, p-phenoxybenzyl, or a halogenated alkeneyl radical and X" represents an anionic radical or the anionic moiety of Y or R provided that when Y is N-oxide X" is absent. 10. The method as claimed in Claim 9 wherein at least one nitrogen-containing heterocyclic compound is quinoline. The method as claimed in Claim 9 wherein at least one nitrogen-containing heterocyclic compound is N-allylquinolinium bromide. The method as claimed in Claim 9 wherein at least one nitrogen-containing heterocyclic compound N-(2,3-dichloro-2-pr openyD-quinolinium iodide. 13. The method as claimed in Claim 1 wherein at least one nitrogen-containing heterocyclic compound is of the formula wherein each R is independently hydrogen, alkyl, alkenyl, alkoxy, alkylamine, alkylsulfonic acid or salts thereof, sulfonic acid or salts thereof, halogen, amine, hydroxyl, mercapto, nitrile, benzyl, or phenylalkyl (where m is an integer 0 to 4); n is an integer 0 to 3; z is 0 or 1; Y is oxygen, allyl, propargyl, benzyl, an alkoxy group, alkyl sulfonic acid -CCH2 )p-S03®(where p is an integer of from 1 to 4), an oxyalkylsulfonic acid, quinaldinyl, p-phenoxybenzyl, or a halogenated alkeneyl radical, and X~ represents an anionic radical or the anionic moiety of Y or R provided that when Y is N-oxide X" is absent. 1
4. The method as claimed in Claim 13 wherein at least one nitrogen-containing heterocyclic compound is isoquinoline. 1
5. The method as claimed in Claim 13 wherein at least one nitrogen-containing heterocyclic compound is isoquinoline-N-oxide. 1
6. The method as claimed in Claim 13 wherein at least one nitrogen-containing heterocyclic compound is N-allylisoquinolinium bromide. 1
7. The method as claimed in Claim 13 wherein at least one nitrogen-containing heterocyclic compound is N-(2,3-dichloro-2-propenyl)-isoquinolinium iodide. 1
8. The method as claimed in Claim 13 wherein at least one nitrogen-containing heterocyclic compound is N-benzylisoquinolinium chloride. yl, 21. The method as claimed in Claim 19 wherein at least one nitrogen-containing heterocyclic compound is l,3-di-(4,4' -pyridyDpropane. 22. The method as claimed in Claim 1 wherein at least one nitrogen-containing heterocyclic compound is of the formula wherein each R is independently hydrogen, alkyl, alkenyl, alkoxy, alkylamine, alkylsulf onic acid or salts thereof, sulfonic acid or salts thereof, halogen, amine, hydroxyl, mercapto, nitrile, benzyl, or phenylalkyl (where m is an integer 0 to 4) n is an integer 0 to 3; z is 0 or 1; Y is oxygen, allyl, propargyl, benzyl, an alkoxy group, alkyl sulfonic acid -(CH2)p-S03®( where p is an integer of from 1 to ), an oxyalkylsulf onic acid, quinaldinyl, p-phenoxybenzyl or a halogenated alkeneyl radical and X" represents an anionic radical or the anionic moiety of Y or R provided that when Y is N-oxide X" is absent. 23. The method as claimed in Claim 22 wherein at least one nitrogen-containing heterocyclic compound is acridine. 24. The method as claimed in Claim 1 wherein at least one nitrogen-containing heterocyclic compound is of the formula wherein each R is independently hydrogen, alkyl, alkenyl, alkoxy, alkylamine, alkylsulfonic acid or salts thereof, sulfonic acid or salts thereof, halogen, amine, hydroxyl, mercapto, nitrile, benzyl, or phenylalkyl (where m is an integer 0 to * ; n is an integer 0 to 3; R" is a bifunctional radical and X represents an anionic radical or the anionic moiety of R. n at at formula: an at formula: teger at formula: 50. in Claim 1 wherein at a quaternary imidazo- ated fatty acid radical, metal carboxylate, ting of alkyl alcoholate, boxylic acid and alkali boxylic acids, and A" is ulfate or sulfamate anion. in Claim 1 wherein at a polyvinylpyrrolidone 50 to 5000, 31. A composition for providing bright, or brilliant zinc electrodeposits free of "spores" and/or striations over a wide current density range which comprises an aqueous bath composition containing at least one zinc compound providing zinc ions for electroplating zinc, (a) at least one bath-soluble surfactant selected from the group consisting of bath-soluble polyethers, substituted polyethers, and substituted non-aromatic nitrogen heterocyclic surfactants; and (b) at least one aromatic, non-carbonyl, nitrogen-containing heterocyclic compound. 32. A composition as claimed in Claim 31 wherein at least one nitrogen-containing heterocyclic compound is of the formula: wherein each R is independently hydrogen, alkyl, alkenyl, alkoxy, alkylamine, alkylsulfonic acid or salts thereof, sulfonic acid or salts thereof, halogen, amine, hydroxyl, mercapto, nitrile, benzyl, or phenylalkyl (where m is an integer 0 to ¾) n is an integer 0 to 3; z is O or 1; Y is oxygen, allyl, propargyl, benzyl, an alkoxy group, alkyl sulfonic acid -(CH2)p-S03®(where p is an integer of from 1 to 4), an oxyalkylsulfonic acid, quinaldinyl, p-phenoxybenzyl or a halogenated alkeneyl radical and X" represents an anionic radical or the anionic moiety of Y or R provided that when Y is N-oxide X" is absent. 33. A composition as claimed in Claim 32 wherein at least one nitrogen-containing heterocyclic compound is N-(2,3-dichlo o-2-p openyl")-pyr idinium chloride. 34. A composition as claimed in Claim 32 wherein at least one nitrogen-containing heterocyclic compound is N-pr opargy1-2- (n-propan-3-ol)-py idinium bromide. 35. A composition as claimed in Claim 32 wherein at least one nitrogen-containing heterocyclic compound is 2-mer capto- -methylpyridine. 36. A composition as claimed in Claim 32 wherein at least one nitrogen-containing heterocyclic compound is -cyanopyridine-N-oxide . 37. A composition as claimed in Claim 32 wherein at least one nitrogen-containing heterocyclic compound is 4-cyanopyridine . 38. A composition as claimed in Claim 32 wherein at least one nitrogen-containing heterocyclic compound is 3-pyr idylsulfonic acid. 3
9. A composition as claimed in Claim 31 wherein at least one nitrogen-containing heterocyclic compound is of the formula: wherein each R is independently hydrogen, alkyl, alkenyl, alkoxy, alkylamine, alkylsulfonic acid or salts thereof, sulfonic acid or salts thereof, halogen, amine, hydroxyl, mer- capto, nitrile, benzyl, or phenylalkyl (where m is an integer 0 to 4);n is an integer 0 to 3; z is 0 or 1; Y is oxygen, allyl, propargyl, benzyl, an alkoxy group, alkyl sulfonic acid -(CH2 )p-S03®(where p is an integer of from 1 to 4), an oxyalkylsulfonic acid, quinaldinyl, p-phenoxybenzyl, or a halogenated alkeneyl radical and X" represents an anionic radical or the anionic moiety of Y or R provided that when Y is N-oxide X" is absent. 40. A composition as claimed in Claim 39 wherein at least one nitrogen-containing heterocyclic compound is quinoline. 41. A composition as claimed in Claim 39 wherein at least one nitrogen-containing heterocyclic compound is N-allylquinolinium bromide. 42. A composition as claimed in Claim 39 wherein at least one nitrogen-containing heterocyclic compound is 43. A composition as claimed in Claim 31 wherein at least one nitrogen-containing heterocyclic compound is of the formula: wherein each R is independently hydrogen, alkyl, alkenyl, alkoxy, alkylamine, alkylsulfonic acid or salts thereof, sulfonic acid or salts thereof, halogen, amine, hydroxyl, mercapto, nitrile, benzyl, or phenylalkyl (where m is an integer 0 to 4); n is an integer 0 to 3; z is 0 or 1; Y is oxygen, allyl, propargyl, benzyl, an alkoxy group, alkyl sulfonic acid -CCH2)p-S03®(where p is an integer of from 1 to 4), and oxyalkylsulfonic acid, quinaldinyl p-phenoxybenzyl, or a halogenated alkeneyl radical, and X" represents an anionic radical or the anionic moiety of Y or R provided that when Y is N-oxide X" is absent. 44. A composition as claimed in Claim 43 wherein at least one nitrogen-containing heterocyclic compound is isoquinoline . 45. A composition as claimed in Claim 43 wherein at least one nitrogen-containing heterocyclic compound is isoquinoline-N-oxide. 46. A composition as claimed in Claim 3 wherein at least one nitrogen-containing heterocyclic compound is N-allylisoquinolinium bromide. 47. A composition as claimed in Claim 43 wherein at least one nitrogen-containing heterocyclic compound is N-(2,3-d chloro-2-pr openyD-isoquinolinium iodide . 48. A composition as claimed in Claim 43 wherein at least one nitrogen-containing heterocyclic compound is N-benzylisoquinolinium chloride. 49. A composition as claimed in Claim 31 wherein at least one nitrogen-containing heterocyclic compound is of the formula wherein each R is independently hydrogen, alkyl, akenyl, alkoxy, alkylamine, alkylsulfonic acid or salts thereof, sulfonic acid or salts thereof, halogen, amine, hydroxyl, mercapto, nitrile, benzyl, or phenylalkyl (where m is an integer 0 to 4) n is an integer 0 to 3; R' is a divalent alkylene, divalent alkeneylene, secondary amine, or a direct bond between two heterocyclic rings; z is 0 or 1; Y is oxygen, allyl, propargyl, benzyl, an alkoxy group, alkyl sulfonic acid -(CH2)p-S03®(where p is an integer of from 1 to 4), an oxyalkylsulfonic acid, quinaldinyl, p-phenoxybenzyl or a halogenated alkeneyl radical and X~ represents an anionic radical or the anionic moiety of Y or R provided that when Y is N-oxide x" is absent. 50. A composition as claimed in Claim 49 wherein at least one nitrogen-containing heterocyclic compound is l,3-di-( ,4' -pyridyl-Ν,Ν' -oxide)-n-propane. 51. A composition as claimed in Claim 9 wherein least one nitrogen-containing heterocyclic compound is 3-di-(* , -pyridyl) propane. A composition as claimed in Claim 31 wherein at least one nitrogen-containing heterocyclic compound is of the formula wherein each R is independently hydrogen, alkyl, alkenyl, alkoxy, alkylamine, alkylsulfonic acid or salts thereof, sulfonic acid or salts thereof, halogen, amine, hydroxyl, mercapto, nitrile, benzyl, or phenylalkyl (where m is an integer 0 to 4) n is an integer 0 to 3; z is 0 or 1; Y is oxygen, allyl, propargyl, benzyl, an alkoxy group, alkyl sulfonic acid -(CH2)p-S03®(where p is an integer of from 1 to * , an oxyalkylsulfonic acid, quinaldinyl, p-phenoxybenzyl or a halogenated alkeneyl radical and X" represents an anionic radical or the anionic moity of Y or R provided that when Y is N-oxide X" is absent . 53. A composition as claimed in Claim 52 wherein at least one nitrogen-containing heterocyclic compound is acridine. 5b. A composition as claimed in Claim 31 wherein at least one nitrogen-containing heterocyclic compound is of the formula wherein each R is independently hydrogen, alkyl, alkenyl, alkoxy, alkylamine, alkylsulfonic acid or salts thereof, sulfonic acid or salts thereof, halogen, amine, hydroxyl, mercapto, nitrile, benzyl, or phenylalkyl (where m is an integer 0 to 4); n is an integer .0 to 3; R" is a bifunctional radical such as and X" represents an anionic radical or the anionic moiety of R.
IL42867A 1972-09-26 1973-08-01 Method and compositions for zinc electroplating IL42867A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US00293659A US3821095A (en) 1972-09-26 1972-09-26 Zinc electroplating process and electrolyte therefor

Publications (1)

Publication Number Publication Date
IL42867A true IL42867A (en) 1976-02-29

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Application Number Title Priority Date Filing Date
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Country Status (15)

Country Link
US (1) US3821095A (en)
JP (1) JPS4972138A (en)
BE (1) BE804733A (en)
CA (1) CA1020901A (en)
CH (1) CH601501A5 (en)
CS (1) CS166677B2 (en)
DE (1) DE2348190A1 (en)
ES (1) ES419035A1 (en)
FR (1) FR2200370B1 (en)
GB (1) GB1394637A (en)
IL (1) IL42867A (en)
IT (1) IT1005144B (en)
NL (1) NL7313268A (en)
NO (1) NO134529C (en)
ZA (1) ZA735205B (en)

Families Citing this family (11)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB1578168A (en) * 1976-03-12 1980-11-05 Cilag Chemie Pyridyl alkylsulphonic acid derivatives and their use in electroplating baths
JPS52111820A (en) * 1976-03-18 1977-09-19 Furukawa Electric Co Ltd:The Electro-deposition of zinc
US4138294A (en) * 1977-12-06 1979-02-06 M&T Chemicals Inc. Acid zinc electroplating process and composition
US4137133A (en) * 1977-12-15 1979-01-30 M&T Chemicals Inc. Acid zinc electroplating process and composition
CA1134317A (en) * 1978-01-16 1982-10-26 Sylvia Martin Zinc electroplating bath
US4170526A (en) * 1978-01-16 1979-10-09 Oxy Metal Industries Corporation Electroplating bath and process
FR2422736A1 (en) * 1978-01-25 1979-11-09 Oxy Metal Industries Corp Aq. cyanide-free zinc electroplating bath - contg. quat. heterocyclic salt as brightener and leveller and opt. polyether
EP0037634A1 (en) * 1980-02-28 1981-10-14 Albright &amp; Wilson Limited Zinc plating baths and additives therefor
JPS62287093A (en) * 1986-06-05 1987-12-12 Okuno Seiyaku Kogyo Kk Electric zinc-nickel alloy plating bath
DE102004061255B4 (en) * 2004-12-20 2007-10-31 Atotech Deutschland Gmbh Process for the continuous operation of acidic or alkaline zinc or zinc alloy baths and apparatus for carrying it out
US8388824B2 (en) * 2008-11-26 2013-03-05 Enthone Inc. Method and composition for electrodeposition of copper in microelectronics with dipyridyl-based levelers

Also Published As

Publication number Publication date
CA1020901A (en) 1977-11-15
GB1394637A (en) 1975-05-21
CS166677B2 (en) 1976-03-29
FR2200370A1 (en) 1974-04-19
US3821095A (en) 1974-06-28
ES419035A1 (en) 1976-03-01
PL94161B1 (en) 1977-07-30
BE804733A (en) 1974-01-02
NO134529C (en) 1976-10-27
ZA735205B (en) 1974-07-31
NO134529B (en) 1976-07-19
IT1005144B (en) 1976-08-20
DE2348190A1 (en) 1974-04-04
CH601501A5 (en) 1978-07-14
NL7313268A (en) 1974-03-28
JPS4972138A (en) 1974-07-12
FR2200370B1 (en) 1980-02-08
AU6048173A (en) 1975-03-20

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