CN109604319A - The combined governance packet of fortification of plants extraction repairing heavy metal pollution farming land - Google Patents
The combined governance packet of fortification of plants extraction repairing heavy metal pollution farming land Download PDFInfo
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- CN109604319A CN109604319A CN201811608538.5A CN201811608538A CN109604319A CN 109604319 A CN109604319 A CN 109604319A CN 201811608538 A CN201811608538 A CN 201811608538A CN 109604319 A CN109604319 A CN 109604319A
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B09—DISPOSAL OF SOLID WASTE; RECLAMATION OF CONTAMINATED SOIL
- B09C—RECLAMATION OF CONTAMINATED SOIL
- B09C1/00—Reclamation of contaminated soil
- B09C1/08—Reclamation of contaminated soil chemically
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B09—DISPOSAL OF SOLID WASTE; RECLAMATION OF CONTAMINATED SOIL
- B09C—RECLAMATION OF CONTAMINATED SOIL
- B09C1/00—Reclamation of contaminated soil
- B09C1/10—Reclamation of contaminated soil microbiologically, biologically or by using enzymes
- B09C1/105—Reclamation of contaminated soil microbiologically, biologically or by using enzymes using fungi or plants
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B09—DISPOSAL OF SOLID WASTE; RECLAMATION OF CONTAMINATED SOIL
- B09C—RECLAMATION OF CONTAMINATED SOIL
- B09C2101/00—In situ
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Abstract
The present invention provides a kind of combined governance packets of fortification of plants extraction repairing heavy metal pollution farming land, the combined governance packet is made of heavy metallic activation material, vegetable seeds, fertilizer and fertile soil, wherein for activated material individually at packet, vegetable seeds, fertilizer and fertile soil are mixed into packet.Plant choosing is type hyperaccumulative plant of one's native land.Present invention application is easy, swift to operate, can the habitat characteristics according to needed for farming land heavy metal in soil contamination class and content, plant growth, selectively adjust the type and dosage, plant variety, the ratio of planting patterns and various composition of activated material.The combined governance packet overcomes the weakness in previous experiences, solves the problems, such as the plant extraction recovery technique application under the conditions of different pollution conditions, different zones, Different climate, improves planting effect, enhances the ability of plant absorption heavy metal.The combined governance packet has good application value in farming land contaminated soil remediation.
Description
Technical field
The invention belongs to farming land heavy metal pollution regulation field, a huge sum of money is repaired in the fortification of plants extraction for being related to specific composition
Belong to the combined governance packet of pollution farming land.
Background technique
For heavy metal pollution farming land soil, more safely and effectively repair mode is phytoremediation, at low cost, secondary dirt
Contaminate it is easily controllable, and vegetation formed after have effects that protect surface soil, reduce corrode, slow down soil erosion and landscape reparation, can
Large-area applications are in heavy metal pollution farming land soil.In phytoremediation field, studies and what application was more is planted so that ultraproduct is tired
Plant extraction technology based on object.Currently, reported accumulation has more than 500, but most of ultraproducts with hyperaccumulative plant kind
Tired plant narrow application range, root system is shallow, and biomass is small, so that the time required for repairing polluted soil is very long.In addition, plant
Enrichment and tolerance are limited, and plant growth is vulnerable to such environmental effects, so needing the habitat characteristics according to each department
Suitable type hyperaccumulative plant of one's native land is selected, and enhancements appropriate is selected to improve hyperaccumulative plant repairing performance, is had with this
Effect makes up the limitation of phytoremediation.Strengthen in hyperaccumulative plant extraction restoration of soil polluted by heavy metal, skill is induced with chelating agent
Art, the research of microbial association technology and application are more, wherein the effect stability of chelating agent, can large area use.So taking
Strengthen super enriching plant extraction with chelating agent induced activation to repair, is the recovery technique that there is long term growth to be worth.
Plant growth needs advantageous ecological environmental condition, and soil texture is good, nutrient supply is sufficient and coordinates, soil is protected
Water is good with nutrient preserving capability, is wherein most important three Xiang Yinsu.The planting plants seed in heavy metal pollution farming land soil, hair
Bud and growth restriction cause germination percentage low with survival rate, and phytomass is few, thus must take soil structure improved addictive appropriate with
Reasonable broadcast application measure.And in large area repair heavy metal pollution farming land, implement soil structure improved addictive, plant step by step
Sowing, broadcast application, are lost a large amount of manpower and material resources.To improve working efficiency, vegetable seeds is improved in heavy metal
Biomass, the increase hyperaccumulative plant extraction absorption huge sum of money for polluting germination percentage and survival rate in farming land soil, increasing plant
The ability of category, is badly in need of the new product of one kind or technology solves problem above.
Summary of the invention
The present invention sowed etc. for broadcast application and seed implement step by step take time and effort, plant extraction recovery technique is applicable in model
The problems such as small is enclosed, a kind of combined governance packet of fortification of plants extraction repairing heavy metal pollution farming land is provided, overcomes previous
Weakness in experience improves planting effect, enhances the ability of plant absorption heavy metal.
The present invention is realized with following technical solution:
The combined governance packet of fortification of plants extraction repairing heavy metal pollution farming land of the present invention is by heavy metallic activation material, plant species
Son, fertilizer and fertile soil are combined.
The heavy metallic activation material is based on the stable chelating agent of activation effect, including artificial synthesized chelating agent and day
Right chelating agent, specifically by EDTA, EDDS, DTPA, EGTA, dimercaptosuccinic acid, ammonium dihydrogen phosphate, tartaric acid, malic acid, apple
Sour sodium, citric acid, sodium citrate, the one or more of thiosulfate compound.
The heavy metallic activation bill of materials alone becomes packet.
The vegetable seeds selects the seed of type hyperaccumulative plant of one's native land, i.e., within the scope of farming land region to be repaired
The native plants kind of heavy metal effect is tired out with ultraproduct.
The vegetable seeds, fertilizer and fertile soil are mixed into packet.
The mass percentage that interior each ingredient is wrapped in the mixing is as follows: vegetable seeds 20%~40%, fertilizer 20%~40% are remaining
Amount is fertile soil, and the sum of mass percentage of each component is 100%.
For example in Southwestern China area, the type heavy metal hyperaccumulative plant of one's native land that can choose and corresponding activated material are such as
Under:
For cadmium pollution farming land, the type hyperaccumulative plant of one's native land that can preferentially select have bog marshcress herb (Rorippa globosa), three
Leaf beggar-ticks (Bidens pilosaVar. radiata), wild crowndaisy chrysanthemum (Crassocephalum crepidioides), Xiang
Certain herbaceous plants with big flowers (Helianthus annuus), hollyhock (Althaea rosea), black nightshade (Solanum nigrum), Phytolacca acinosa
(Phytolacca acinosa), ramie (Boehmeria nivea), strengthen the activated material of the above hyperaccumulative plant extraction cadmium
There are EDTA, citric acid, tartaric acid, malic acid etc.;
For arsenic pollution farming land, the type hyperaccumulative plant of one's native land that can preferentially select have ciliate desert-grass (Pteris vittata), tiltedly
Plumage brake fern (Pteris oshimensis), brake fern (Pteris cretica), strengthen the above hyperaccumulative plant extraction arsenic
Activated material has EDTA, citric acid, tartaric acid etc.;
For lead contamination farming land, the type hyperaccumulative plant of one's native land that can preferentially select have white lotus wormwood artemisia (Artemisia sacrorum), bidens pilosa (Bidens pilosaVar. radiate), wild crowndaisy chrysanthemum (Crassocephalum crepidioides), sunflower (Helianthus annuus L.) Thlaspi (Thlaspi arvense), leaf mustard (Brassica
Juncea), ramie (Boehmeria nivea(L.) Gaudich.), white back maple (Buddleja asiatica), tuber fern
(Nephrolepis auriculata), buckwheat (Fagopyrum esculentum), alfalfa (Medicago sativa),
The activated material for strengthening the above hyperaccumulative plant extraction lead has EDTA, citric acid, tartaric acid, malic acid etc.;
For pollution of chromium farming land, the type hyperaccumulative plant of one's native land that can preferentially select have Leersia Sw (Leersia hexandra),
Hemarthria compressa (Hemarthria compressa), fake rice (Leersia japonica), Chinese pennisetum (Pennisetum alopecuroides), the activated material for strengthening the above hyperaccumulative plant extraction of chromium has EDTA, citric acid, ammonium citrate etc.;
For zinc pollution farming land, the type hyperaccumulative plant of one's native land that can preferentially select have leaf mustard (Brassica juncea), open country Tong
Wormwood artemisia (Crassocephalum crepidioides), sunflower (Helianthus annuus), Sedum alfredii Hance (Sedum alfredii), the activated material for strengthening the above hyperaccumulative plant extracting zinc has EDTA;
For Cu-W ore deposit farming land, the type hyperaccumulative plant of one's native land that can preferentially select have leaf mustard (Brassica juncea), duck plantar
Grass (Commelina communis), castor-oil plant (Ricinus communis), water chestnut (Heleocharis dulcis), Festuca Arundinacea
(Festuca elat), Pteridium revolutum (Bl.) Naka (Pteridium revolutum), strengthens the activated material of the above hyperaccumulative plant extracting copper
There are EDTA, EDDS, citric acid, tartaric acid and malic acid.
Combined governance packet of the present invention is directly used, activated material therein promotes the activity of heavy metal in soil, therein
Fertilizer, fertile soil directly can provide nutrition and environment needed for growth course for seed, improve plant survival rate and biology
Amount, it is final to realize the target for reducing farming land heavy metal in soil content.
The invention has the following beneficial effects:
(1) product of the present invention can manually or mechanically be spread fertilizer over the fields, swift to operate using simplicity, overcome broadcast application in previous experiences,
The weakness taken time and effort is implemented in seed sowing etc. step by step.
(2) present invention can the habitat characteristics according to needed for farming land The Heavy Metal Contaminated Soil type and degree, plant growth,
The selectively type and dosage, plant variety, planting patterns of adjustment activated material and the ratio of various composition, solve difference
The problem of plant extraction recovery technique under the conditions of pollution condition, different zones, Different climate is applied.
(3) present invention improves planting effect using type hyperaccumulative plant of one's native land and heavy metallic activation material, enhances
The ability of plant absorption heavy metal.
(4) present invention is applied widely, has good application value in farming land contaminated soil remediation.
Specific embodiment
Embodiment 1
Certain dry farming farming land soil regime are as follows: cement, red soil, pH value 5.9, cadmium (Cd) content average out to 16.02mg/kg surpass
Cross farming land risk control value (5.5 < pH≤6.5,2.0 mg/kg of cadmium).
Heavy metallic activation material is citric acid, sodium citrate, EDTA, tartaric acid, malic acid, natrium malicum, plant variety
For Phytolacca acinosa (Phytolacca acinosa), fertilizer is particle humic acid, and fertile soil is pine needle fertile soil.
Administer Phytolacca acinosa seed quality percentage 40% in packet, particle humic acid 30%, pine needle fertile soil 30%.
1 group of control group and 5 groups of experimental groups be set, control group is directly to sow Phytolacca acinosa seed, experimental group 1 be Phytolacca acinosa seed and
According to the 4:3:3 mixed planting of mass ratio, experimental group 2 is Phytolacca acinosa seed and humic acid, pine needle humic for humic acid, pine needle fertile soil
4:3:3 mixed planting and sprinkling 0.5 mmol/L citric acid solution of the soil according to mass ratio, experimental group 3 is Phytolacca acinosa seed and humic
Acid, pine needle fertile soil are according to the 4:3:3 mixed planting and 0.5 mmol/L sodium citrate solution of sprinkling, experimental group 4 of mass ratio
Phytolacca acinosa seed and humic acid, pine needle fertile soil according to mass ratio 4:3:3 mixed planting and spray 0.25 mmol/L EDTA and
0.25 mmol/L natrium malicum solution, experimental group 5 be Phytolacca acinosa seed and humic acid, pine needle fertile soil according to mass ratio 4:3:3
Mixed planting simultaneously sprays 0.25 mmol/L tartaric acid and 0.25 mmol/L malic acid solution.Control group is each with two groups of experimental groups
Group is respectively provided with 3 repetitions, and each repetition is set as a cell, and 6 groups are arranged 18 cells altogether, and the plot area of each test is
2.25m2(1.5m × 1.5m).
Test starts from mid-February, ploughs deeply cultivated 20~30cm first, dries one week, starts to plant in mid or late Febuary.
Phytolacca acinosa plantation carries out sowing and field weeding management according to the conventional method of general dry land crop.Each cell inside trade
Spacing is planted in 20cm in land, and 5-8 seed is spread in 49 kinds of plant holes of average design in average each cell, every bunch planting, after emergence between
Seedling, every cave stay 1 ~ 2 plant of seedling.Crop cycle is 90 days.The 30th day after plant plantation, experimental group, which is spread fertilizer over the fields, was prepared as aqueous solution
Heavy metallic activation material.
Field management: it is short of seedling according to field Routine Management mode thinning, polishing, weeding, watering, top dressing etc..Late May,
Plant is harvested, aerial part recycles simultaneously under ground portion.
Continuous plantation 3 years.
The variation of cadmium content is shown in Table 1 in soil.
Total cadmium content changes unit: mg/kg in 1 soil of table
Group | Before plantation | First Year | Second year | Third year |
Control group | 16.02 | 15.69 | 15.24 | 15.43 |
Experimental group 1 | 16.02 | 14.88 | 14.01 | 13.58 |
Experimental group 2 | 16.02 | 14.34 | 12.76 | 11.62 |
Experimental group 3 | 16.02 | 14.86 | 14.05 | 13.46 |
Experimental group 4 | 16.02 | 14.67 | 13.74 | 13.02 |
Experimental group 5 | 16.02 | 14.02 | 12.67 | 11.65 |
The plant height of Phytolacca acinosa such as table 2.
The average height unit of 2 Phytolacca acinosa plant of table: m
Group | First Year | Second year | Third year |
Control group | 0.51 | 0.52 | 0.78 |
Experimental group 1 | 0.73 | 0.89 | 1.02 |
Experimental group 2 | 0.92 | 0.94 | 1.06 |
Experimental group 3 | 0.75 | 0.84 | 0.86 |
Experimental group 4 | 0.60 | 0.68 | 0.70 |
Experimental group 5 | 0.94 | 0.98 | 0.96 |
Embodiment 2
Certain dry farming farming land soil regime are as follows: cement, red soil, pH value 6.4,71.40 mg/kg of copper content average out to are more than
Farming land risk screening value (5.5 < pH≤6.5,50 mg/kg of copper).
Heavy metallic activation material be EDDS, citric acid, DTPA, EGTA, plant variety be leaf mustard (Brassica juncea), fertilizer is pig manure decomposed manure, and fertile soil is pine needle fertile soil.
Administer juncea seeds mass percent 20% in packet, pig manure decomposed manure 40%, pine needle fertile soil 40%.
1 group of control group and 3 groups of experimental groups be set, control group is directly to sow juncea seeds, experimental group 1 be juncea seeds and
According to the 1:2:2 mixed planting of mass ratio, experimental group 2 is that juncea seeds and pig manure are rotten for pig manure decomposed manure, pine needle fertile soil
The 1:2:2 mixed planting and sprinkling 0.25 mmol/L citric acid and 0.25 of ripe organic fertilizer, pine needle fertile soil according to mass ratio
Mmol/LEDDS solution, experimental group 3 be juncea seeds and pig manure decomposed manure, pine needle fertile soil according to mass ratio 1:2:2
Mixed planting simultaneously sprays 0. 25 mmol/L DTPA and 0.25 mmol/L EGTA solution.The each group of control group and 3 groups of experimental groups
3 repetitions are respectively provided with, each repetition is set as a cell, and 4 groups are arranged 12 cells altogether, and the plot area of each test is
2.25m2(1.5m × 1.5m).
Test ploughs deeply cultivated 20~30cm since early August first, dries one week, starts to plant mid-August.
Leaf mustard plantation carries out sowing and field weeding management according to the conventional method of general dry land crop.Mustard in each cell
Colza plants spacing in 20cm, and 3-5 seed is spread in 49 kinds of plant holes of average design in average each cell, every bunch planting, after emergence between
Seedling, every cave stay 1 plant of seedling.Crop cycle is 60 days.The 20th day after plant plantation, experimental group spread fertilizer over the fields the weight for being prepared as aqueous solution
Metal activation material.
Field management: it is short of seedling according to field Routine Management mode thinning, polishing, weeding, sprays insecticide, watering, top dressing etc..
Mid-October, plant is harvested, aerial part recycles simultaneously under ground portion.
Continuous plantation 3 years.
The variation of copper content is shown in Table 3 in soil.
Total copper content changes unit: mg/kg in 3 soil of table
Group | Before plantation | First Year | Second year | Third year |
Control group | 71.40 | 69.34 | 67.94 | 66.93 |
Experimental group 1 | 71.40 | 66.92 | 64.03 | 62.27 |
Experimental group 2 | 71.40 | 65.32 | 61.77 | 59.39 |
Experimental group 3 | 71.40 | 65.89 | 62.40 | 60.11 |
The plant height of leaf mustard such as table 4.
The average height unit of 4 leaf mustard plant of table: m
Group | First Year | Second year | Third year |
Control group | 0.29 | 0.30 | 0.28 |
Experimental group 1 | 0.43 | 0.46 | 0.51 |
Experimental group 2 | 0.44 | 0.45 | 0.48 |
Experimental group 3 | 0.38 | 0.39 | 0.42 |
Embodiment 3
Certain dry farming farming land soil regime are as follows: rendzinas, pH value 5.3,231.26 mg/kg of lead content average out to are more than agriculture
Land used risk screening value (pH≤5.5, lead 70mg/kg).
Heavy metallic activation material is citric acid, tartaric acid, dimercaptosuccinic acid, ammonium dihydrogen phosphate, thiosulfate, plant
Kind be bidens pilosa (Bidens pilosaVar. radiate), fertilizer is pig manure decomposed manure, and fertile soil is pine
Needle fertile soil.
Administer bidens pilosa seed quality percentage 30% in packet, pig manure decomposed manure 20%, pine needle fertile soil 50%.
1 group of control group and 4 groups of experimental groups are set, and control group is directly to sow bidens pilosa seed, and experimental group 1 is three leaves
According to the 3:2:5 mixed planting of mass ratio, experimental group 2 is three leaves for Bidens bipinnata grass seed and pig manure decomposed manure, pine needle fertile soil
The 3:2:5 mixed planting and sprinkling 0.25 of Bidens bipinnata grass seed and pig manure decomposed manure, pine needle fertile soil according to mass ratio
Mmol/L citric acid and 0.25 mmol/L dimercaptosuccinic acid solution, experimental group 3 are bidens pilosa seed and pig manure is decomposed has
Machine fertilizer, pine needle fertile soil are according to the 3:2:5 mixed planting of mass ratio and 0. 25 mmol/L tartaric acid of sprinkling and 0.25 mmol/
L ammonium dihydrogen phosphate, experimental group 4 are bidens pilosa seed and pig manure decomposed manure, pine needle fertile soil according to mass ratio
3:2:5 mixed planting and spray 0. 25 mmol/L citric acids and 0.25 mmol/L thiosulfate solution.Control group with
The each group of 4 groups of experimental groups is respectively provided with 3 repetitions, and each repetition is set as a cell, and 5 groups are arranged 15 cells, Mei Geshi altogether
The plot area tested is 2.25m2(1.5m × 1.5m).
Test ploughs deeply cultivated 20~30cm since early March first, dries one week, starts to plant mid-March.
Bidens pilosa plantation carries out sowing and field weeding management according to the conventional method of general dry land crop.It is each small
6-8 kind is spread in bidens pilosa plantation spacing 49 kinds of plant holes of average design, every bunch planting in 20cm, average each cell in area
Son, thinning after emergence, every cave stay 2-3 plants of seedling.Crop cycle is 90 days.The 30th day after plant plantation, the experimental group system of spreading fertilizer over the fields
Standby is the heavy metallic activation material of aqueous solution.
Field management: it is short of seedling according to field Routine Management mode thinning, polishing, weeding, watering, top dressing etc..Mid-June,
Plant is harvested, aerial part recycles simultaneously under ground portion.
Continuous plantation 3 years.
The variation of lead content is shown in Table 5 in soil.
Total lead content changes unit: mg/kg in 5 soil of table
Group | Before plantation | First Year | Second year | Third year |
Control group | 231.26 | 224.59 | 220.05 | 215.99 |
Experimental group 1 | 231.26 | 216.75 | 207.39 | 199.61 |
Experimental group 2 | 231.26 | 206.94 | 187.42 | 172.70 |
Experimental group 3 | 231.26 | 211.10 | 193.59 | 178.74 |
Experimental group 4 | 231.26 | 216.97 | 203.11 | 190.14 |
The plant height of bidens pilosa such as table 6.
The average height unit of 6 bidens pilosa plant of table: m
Group | First Year | Second year | Third year |
Control group | 0.61 | 0.63 | 0.58 |
Experimental group 1 | 0.85 | 0.89 | 0.91 |
Experimental group 2 | 0.84 | 0.90 | 0.90 |
Experimental group 3 | 0.87 | 0.89 | 0.88 |
Experimental group 4 | 0.78 | 0.84 | 0.82 |
These are only the preferred embodiment of the present invention, is not intended to restrict the invention, and comes for those skilled in the art
It says, the invention may be variously modified and varied.All within the spirits and principles of the present invention, made any modification, equivalent
Replacement, improvement etc., should all be included in the protection scope of the present invention.
Claims (6)
1. fortification of plants extraction repairing heavy metal pollution farming land combined governance packet, it is characterised in that: the combined governance packet by
Heavy metallic activation material, vegetable seeds, fertilizer and fertile soil form.
2. combined governance packet according to claim 1, it is characterised in that: the heavy metallic activation material be EDTA,
EDDS, DTPA, EGTA, dimercaptosuccinic acid, ammonium dihydrogen phosphate, tartaric acid, malic acid, natrium malicum, citric acid, citric acid
Sodium, the one or more of thiosulfate compound.
3. combined governance packet according to claim 2, it is characterised in that: the heavy metallic activation bill of materials alone becomes packet.
4. combined governance packet according to claim 1, it is characterised in that: the vegetable seeds, which is that type ultraproduct of one's native land is tired, plants
The seed of object.
5. combined governance packet according to claim 1, it is characterised in that: vegetable seeds, fertilizer and the fertile soil is mixed
Synthesis packet.
6. combined governance packet according to claim 5, it is characterised in that: mixing wraps the mass percentage of interior each ingredient such as
Under: vegetable seeds 20%~40%, fertilizer 20%~40%, surplus are fertile soil, and the sum of mass percentage of each component is 100%.
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Cited By (1)
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CN113351640A (en) * | 2021-06-03 | 2021-09-07 | 西安理工大学 | Method for repairing cadmium and lead combined polluted soil by combining chelating agent with ryegrass |
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