CN108572382B - Method for measuring and calculating H' (0.07) in beta-gamma mixed radiation field - Google Patents
Method for measuring and calculating H' (0.07) in beta-gamma mixed radiation field Download PDFInfo
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- G01T—MEASUREMENT OF NUCLEAR OR X-RADIATION
- G01T1/00—Measuring X-radiation, gamma radiation, corpuscular radiation, or cosmic radiation
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- Y02E30/00—Energy generation of nuclear origin
- Y02E30/30—Nuclear fission reactors
Abstract
The invention belongs to the technical field of radiation monitoring, and relates to a beta-gamma mixed radiation fieldThe method of (1). The measuring and calculating method comprises the following steps: 1) by passingMeasurement of monitorNumerical values, corrected to obtainNumerical values according to correctionNumerically determining the directed dose equivalent rate of gamma ray contribution2) By beta-spectral measurement, determinationCalibration factor N of monitor in beta radiation fieldβA value; 3) determination by gamma spectrometryCalibration factor N of monitor in gamma radiation fieldγA value; 4) according toDirect measurement of monitor, combinedNβAnd NγValue, the directed dose equivalent rate of the beta ray contribution is calculated5)Andadding to obtain the measured positionThe value is obtained. The method solves the problem of the beta-gamma mixed radiation fieldThe difficulty of accurate measurement is improvedThe accuracy of measurement and can provide powerful data support for radiation evaluation and radiation protection actions.
Description
Technical Field
Background
With the development of nuclear energy and the wide application of nuclear technology, the weak penetrating radiation has wide harmThe method is widely applied to various fields such as nuclear industry, radiology, nuclear technology application and the like. Although radiation is in many cases more easily shielded to reduce extraneous radiation to personnel, personnel working in radiation fields where weak penetrating radiation makes a larger share and is not easily shielded, such as fuel element manufacturing plants, after-treatment plants and parts of the work site of nuclear power plants, may still be exposed to a larger dose of radiation to their extremities, skin. In order to evaluate the weak penetrating radiation condition of workers in a site with nuclear radiation, the directional dose equivalent rate of the site needs to be accurately monitored in advanceNumerical values. The monitoring data provides basis for decision-making of radiation protection actions, and radiation protection professionals can make decisions according to monitored placesThe numerical value is measured, reasonable and feasible protective measures are taken, the weak penetrating radiation dose borne by staff in a radiation place is reduced, and the risk of skin burn is reduced.
The international committee for radiation and measurement (ICRU) definition of the targeted dose equivalent rate is: the directional dose equivalent H' (d, Ω) at a point in the radiation field is the dose equivalent produced by the corresponding extended field at a depth d on a radius of the ICRU sphere in the specified direction Ω. The ICRU recommends d 0.07mm for weak penetrating radiation, denoted H' (0.07).
Currently, site directed dose equivalent rates are measuredThe instrument has poor energy response characteristics, and cannot directly measure and accurately give the radiation in the beta-gamma mixed radiation fieldNumerical values, thus for mixed beta-gamma radiation fieldsHas been an accurate measurement in the field of radiation monitoringA difficult problem, which is also a weak link to be solved urgently in the radiation protection field.
Disclosure of Invention
The invention aims to provide a beta-gamma mixed radiation fieldTo solve the problem of beta-gamma mixed radiation fieldDifficulty in accurate measurement, improvementThe accuracy of measurement and provide powerful data support for radiation evaluation and radiation protection actions.
To achieve this, in a basic embodiment, the invention provides a mixed beta-gamma radiation fieldThe measuring and calculating method of (2), said measuring and calculating method comprising the steps of:
1) by passingMeasurement of monitorNumerical values, corrected to obtainNumerical values according to correctionNumerically determining the directed dose equivalent rate of gamma ray contribution
2) Determination by beta-spectral measurementCalibration factor N of monitor in beta radiation fieldβA value;
3) determination by gamma spectrometryCalibration factor N of monitor in gamma radiation fieldγA value;
4) according toDirect measurement of monitor, combinedNβAnd NγValue, calculating the directed dose equivalent rate of the beta ray contribution
In a preferred embodiment, the present invention provides a mixed beta-gamma radiation fieldThe method for measuring and calculating, wherein the method described in step 1)The performance of the monitor meets the requirements of the metrological verification regulation JJJG 393-2003 on X and gamma radiation equivalent (rate) meters and monitors for radiation protection.
In a preferred embodimentIn the scheme, the invention provides a beta-gamma mixed radiation fieldThe method for measuring and calculating in (1), wherein the correction method in step 1) comprises: for an energy response of better than + -30% in the range of 40keV to 1.5MeV and for a dose rate linearity of better than + -10% in its effective rangeMonitor according to standard radiation fieldResults of the monitor's verification/calibration, usingBy multiplying the value directly measured by the monitor by a calibration factor obtained by verification/calibration, a correction of the measuring point is obtainedNumerical values.
In a preferred embodiment, the present invention provides a mixed beta-gamma radiation fieldThe method for measuring and calculating in (1), wherein the correction method in step 1) comprises:
for an energy response in the range 40keV to 1.5MeV of more than + -30%Monitor according toThe result of the monitor is determined/calibrated in the X, gamma standard radiation field, and the result can be obtainedCalibration factor for measuring X-ray and gamma-ray radiation fields with different energies by monitorA seed;
according to the field gamma measurement spectrum, the energy characteristics of the measured gamma ray can be known, and the energy point can be found in the standard radiation field calibration resultThe calibration factor of the monitor measurements is,the direct measurement value of the monitor being multiplied by the calibration factor to obtain a correction of the measurement pointNumerical values.
In a preferred embodiment, the present invention provides a mixed beta-gamma radiation fieldWherein the correction in step 1) is made when the energy of the gamma-rays emitted by the radionuclide in the beta-gamma mixed radiation field is above 40keVThe numerical value isThe value is obtained.
In a preferred embodiment, the present invention provides a mixed beta-gamma radiation fieldThe method for measuring and calculating, wherein N is described in the step 2)βThe determination method of the value is as follows:
measuring a beta radiation spectrum in a beta-gamma mixed radiation field by using a beta spectrometer, measuring a spectrum 1 when a probe is exposed, measuring a spectrum 2 at the same position when 5mm of aluminum is added in front of the probe, and respectively correcting the spectrum 1 and the spectrum 2 in dead time and subtracting to obtain a pure beta ray fluence spectrum of a measuring point;
then the pure beta ray fluence spectrumComparing the measured spectrum with that of a beta spectrometer in a pure beta radiation field, finding out a standard reference spectrum similar to that of a beta-gamma mixed radiation field, and taking a calibration factor, namely N, in the beta radiation field corresponding to the standard reference spectrumβThe value is obtained.
In a preferred embodiment, the invention provides a mixed beta-gamma radiation fieldWherein the pure beta radiation field is90Sr-90Y、85Kr and/or147The radiation field of Pm.
In a preferred embodiment, the present invention provides a mixed beta-gamma radiation fieldThe method for measuring and calculating, wherein N is described in the step 3)γThe determination method of the value is as follows:
measuring the gamma-ray energy spectrum of the beta-gamma mixed radiation field by using a gamma spectrometer, or measuring the gamma-ray energy spectrum after sampling the beta-gamma mixed radiation field on site, and combining the energy of the gamma-ray of the measured fieldThe monitor calibrates the result in the standard X, gamma radiation field, finds out the calibration factor of the energy point close to the site in the standard radiation field, and the calibration factor isN of monitor at the actual measurement pointγThe value is obtained.
In a preferred embodiment, the present invention provides a mixed beta-gamma radiation fieldThe method of (1), wherein the measurement is carried out in the range of 40keV to 1.5MeVThe monitor has good response to gamma ray energyAt + -30%, if the gamma radiation energy of the measured field is of various types and the gamma ray energy is in the range of 40keV-1.5MeV, it can be selectedMonitor is arranged at137The calibration factor given by calibration in the Cs radiation field is used as N for calculationγThe value is obtained.
In a preferred embodiment, the invention provides a mixed beta-gamma radiation fieldThe method of measuring and calculating, wherein in step 4)The calculation method of (2) is shown in the following formula (3):
The invention has the beneficial effect that the beta-gamma mixed radiation field of the invention is utilizedThe method can be used for the directional dose equivalent rate measurement of nuclear facility sites, particularly the measurement of the directional dose equivalent rate of sites emitting gamma rays and having higher beta radiation, and solves the problem of the beta-gamma mixed radiation fieldDifficulty in accurate measurement, improvementThe accuracy of measurement and can provide powerful data support for radiation evaluation and radiation protection actions.
Drawings
FIG. 1 is an exemplary beta-gamma hybrid radiation field of the present inventionIs a flow chart of the measurement and calculation method.
FIG. 2 is a graph of the conversion coefficients of photon fluence to ambient dose equivalents and directed dose equivalents as referred to in the detailed description.
Fig. 3 is a gamma spectrum of a cold end seal liner wipe sample of a nuclear power plant 1SG (steam generator) in an example of an application of the embodiment.
Fig. 4 is a pure beta-ray fluence spectrum of a seal liner wipe sample at the cold end of a nuclear power plant 1SG (steam generator) in an example of an application of an embodiment.
FIG. 5 is an exemplary embodiment of an exemplary application85Beta fluence spectrum of kr standard radiation field.
Detailed Description
The following further describes embodiments of the present invention with reference to the accompanying drawings.
Exemplary beta-gamma mixed radiation field of the inventionThe method of measurement and calculation of (2) is shown in FIG. 1. Due to the sameThe response of the monitor to beta rays and gamma rays is different, and the monitor cannot be directly usedThe monitor can accurately measure the beta-gamma mixed fieldValues, in the processing of measurement data, based onThe values directly measured by the monitor need to be calculated by gamma ray and beta ray pair respectivelyThe contribution of (a), namely:
the method comprises the following steps:
With better energy response and dose rate linearityThe monitor is verified/calibrated in X and gamma standard radiation fields, and the performance of the monitor meets the requirements of JJJG 393-2003. For in-situ beta-gamma mixed radiation fieldNumerical values, using after verification/calibrationThe monitor measures the measurement, and the corrected measurement point can be calculated by multiplying the directly measured value by the calibration factor given in the certificate of verification/calibration according to the verification/calibration result in the standard radiation fieldNumerical values. If it is notIf the energy response of the measuring instrument is slightly poor and the field gamma radiation energy is known, the energy response can be further corrected according to the result of the verification/calibration certificate.
For gamma rays with energies above 300keV, as shown in fig. 2, the international radiation unit is consistent with the conversion coefficients reported by the measurement commission as ICRU43, which reports fluence to ambient dose equivalents and fluence to directed dose equivalents H' (0.07); for gamma rays with energies below 300keV, the conversion coefficients differ slightly. However, the air kerma K according to the monoenergetic photon given in GB/T12162.3aTo the surrounding dose equivalent H*(10) And a conversion factor for the directed dose equivalent H' (0.07), as shown in Table 1, in the range of 30keV to 300keV, and a ratio of the two in the range of 0.9 to 1.1, indicating the same point in the radiation field around which the dose equivalent H is present*(10) And the agreed true value for the targeted dose equivalent H' (0.07) do not differ by more than 10%. The energy of gamma rays emitted by the radionuclide in the actual nuclear facility site is basically above 30 keV. Therefore, the directional dose equivalent rate of the gamma ray contribution is calculatedWhen, the following relationship can be considered to exist:
therefore, only the field measurement is needed and the correction is carried out through the calibration factor, and the measurement point is accurately obtainedThe measured place can be obtained by valueThe value is obtained.
TABLE 1 monoenergetic photons Ka-H*(10) And Ka-H' (0.07) conversion factor
And (3) measuring a field beta radiation spectrum by using a beta spectrometer, and if the field dosage rate is very high, wiping, sampling and measuring. During measurement, the spectrum 1 is measured when the probe is exposed, and because the beta spectrometer has certain response to the gamma rays, the beta rays and the gamma rays in the spectrum contribute together during fluence spectrum. Spectrum 2 was measured at the same location with 5mm aluminum (enough to absorb all beta rays) in front of the probe, spectrum 2 being the fluence spectrum of pure gamma rays. And (3) performing dead time correction and subtraction on the spectrum 1 and the spectrum 2 respectively to obtain the fluence spectrum of the pure beta ray of the measuring point. After the beta fluence spectrum is obtained, the beta fluence spectrum is compared with a beta spectrometer in a pure beta radiation field (generally, the beta fluence spectrum is measured in a pure beta radiation field)90Sr-90Y、85Kr、147Pm), and finding out a standard reference spectrum similar to the field measurement spectrum.When the measurement result of the monitor is calculated, the calibration factor N of the monitor isβGet it rightAnd calibrating the result of the monitor in the beta radiation field corresponding to the standard reference spectrum.
To pairThe monitor is calibrated in the standard X and gamma radiation fields to determineThe monitor is linear in energy response characteristic and dose rate to gamma radiation and gives a calibration factor. When the radiation field measurement is carried out, a gamma spectrometer can be used for measuring the field gamma energy spectrum, and a sampling measurement method can also be adopted for measuring the energy spectrumAfter the energy characteristics of the gamma rays in the field, combiningThe monitor calibrates the result in the standard X and gamma radiation fields to determineN used by the monitor at the actual measurement pointγThe value is obtained. If it is notThe monitor responds well to gamma ray energy (in the range of 40keV to 1.5MeV,the response of the monitor to gamma ray energy is better than +/-30 percent), and the gamma ray energy on site has various types, and the monitor is generally used137The calibration factor given by calibration in the Cs radiation field is taken as NγThe value is obtained.
Directed dose equivalent rate for beta ray contribution in beta-gamma mixed fieldMeasurement results, need to be taken fromThe contribution of gamma-ray is deducted from the direct measurement value of the monitor, the dosage rate of the residual beta-ray contribution is multiplied by the calibration factor in the beta radiation field, and then the measurement point can be obtainedThe value is obtained. Specifically, the following formula is calculated:
wherein: m isDirect measurement of the monitor; n is a radical of hydrogenγIs composed ofA calibration factor of the monitor in a gamma radiation field; n is a radical ofβIs composed ofThe measurement instrument calibrates the factor in the beta radiation field.
In the formula (3)M、The units of the three are the same and are mu Sv/h or mSv/h. 6)Numerical determination
According to the calculation results of the formula (2) and the formula (3), the sum of the formula (1) is used for calculating the beta-gamma mixed radiation field of the measuring pointThe value is obtained.
In the above exemplary beta-gamma mixed radiation field of the present inventionThe specific application of the measuring and calculating method is as follows:
sealing lining plate surface for 1SG (1# steam generator) cold end during overhaul of certain nuclear power stationThe values are measured, and the specific measurement calculation process is as follows:
1 RADIAGEM2000 type X and gamma dose rate instrument is selected, and the energy response of the instrument is better than +/-16% within the range of 40keV-1.5MeV through measurement; dose rates are linear better than + -10% over the range of 1 μ Sv/h-100 mSv/h. Use of theThe monitor measures the reading of the 1SG cold-end sealing lining plate as 268 MuSv/h, and a gamma spectrum of the 1SG cold-end sealing lining plate wiping sample measured by using a gamma spectrometer is shown in figure 3, and as can be seen from figure 3, the energy of gamma rays emitted by radioactive nuclides on the sealing lining plate is mainly more than 200 keV. Thus, the positionThe measured value of the monitor can be directly used137Correction of the calibration factor for Cs byMonitor is arranged at137As can be seen from the calibration results in the Cs standard radiation field, the calibration factor is 1.02 when the dose rate is near 268. mu. Sv/h. The 1SG cold end sealing the liner plate surfaceThe corrected value was 268 × 1.02 ═ 273 μ Sv/h.
According to the gamma spectrum measurement result of the wiping sample of the 1SG cold-end sealing lining plate, the energy of gamma rays emitted by the radioactive nuclide on the equipment is above 40 keV. Therefore, it can be calculated according to the formula (2)
The method is characterized in that a beta spectrometer is used for measuring a beta radiation spectrum of a 1SG cold-end sealing lining plate wiping sample, the spectrum 1 is measured when a probe is exposed, and the beta ray and the gamma ray contribute together during the fluence spectrum of the spectrum because the beta spectrometer also has certain response to the gamma ray. Spectrum 2 was measured at the same location with 5mm aluminum (enough to absorb all beta rays) in front of the probe, spectrum 2 being the fluence spectrum of pure gamma rays. The dead time correction is performed on the spectrum 1 and the spectrum 2 respectively, and the dead time correction is subtracted, so that the fluence spectrum of the pure beta ray at the measuring point can be obtained, and is shown in fig. 4. After the beta fluence spectrum is obtained, the beta fluence spectrum is compared with a beta spectrometer in a pure beta radiation field (generally, the beta fluence spectrum is measured in a pure beta radiation field)90Sr-90Y、85Kr、147Pm), finding out the on-site measured spectrum and85the energy distribution ranges of the Kr standard spectra (as shown in fig. 5) are similar. ThenWhen the measurement result of the monitor is calculated, the calibration factor N of the monitor isβIs selectedMonitor is arranged at85Calibration factor 1.02 in Kr standard radiation field.
To pairThe monitor is calibrated in standard X and gamma radiation fields, and the energy response of the monitor is better than +/-30% within the range of 60keV-1.5 MeV; dose rates are better than + -5% linear over the range of 1. mu.Sv/h-100 mSv/h. Gamma spectra from 1SG cold end seal liner wipe (see fig. 3) on the seal linerThe gamma ray energy emitted by the radionuclide is mainly above 200 keV. Thus, the positionThe measured value of the monitor can be directly used137Correction of the calibration factor for Cs byMonitor is arranged at137The calibration result in the Cs standard radiation field shows that the calibration factor is 1.96 when the dosage rate is close to 268 MuSv/h. Calculating 1SG cold end seal liner surfaceWhen value, N is selectedγThe value was 1.96.
For a beta-gamma mixed field emitted by a 1SG cold-end sealed lining plate,the monitor directly measures M to be 2.98mSv/h, wherein the directional dose equivalent rate of the beta ray contributionCan be calculated by the formula (3), i.e.
Calculated according to the aboveBy adding the two, the 1SG cold end sealing liner surface can be determinedThe value 273+2897 ═ 3170 μ Sv/h.
7) Measurement uncertainty assessment
For field measurement and calculationThe numerical value is calculated by using a formula (1), and the uncertainty of the numerical value is mainly derived from the following parts:
(1) measuringTime, the uncertainty introduced by the calibration factor N: from the calibration certificate, U-7% (k-2) is derived, so that the uncertainty introduced by the calibration factor into class B is U1=3.5%;
(2) MeasuringTime, the uncertainty introduced by the calibration factor N: from the calibration certificate, U-7% (k-2) is derived, so that the uncertainty introduced by the calibration factor into class B is U2=3.5%;
(3) Uncertainty introduced by field measurement data repeatability: according to the field monitoring data, the repeatability of the instrument monitoring data can be less than 1%. 6 readings are measured on site, so that the range of A-type uncertainty repeatedly introduced by field measurement data can be obtained
(4) Uncertainty introduced by the instrument linear response: according toAt 1. mu. Sv.h-1-100mSv·h-1Within the range, the relative intrinsic error of the instrument is within ± 5%. Assuming measured dataThe uncertainty introduced by instrument dose rate linearity is
(5)Introduced uncertainty: in the calculation ofWhen usingThe uncertainty of the measured value of (2) mainly comprises the following two parts: calibration factor N-introduced uncertainty: from the calibration certificate, U-5% (k-2) is derived, so that the uncertainty introduced by the calibration factor into class B is U52.5 percent; uncertainty introduced by field measurement data repeatability: due to the fact that repeatability of the measuring instrument is different under the conditions of different dosage rates, according to field monitoring data, repeatability of the monitoring data can reach 9% at most when the dosage rate is low. The actual field measurement is carried out for 6 times, so that the range of the A-type uncertainty introduced by the repeatability of the field measurement data is obtained
Synthetic uncertainty: the uncertainty components of the above six parts can be known in the fieldSynthetic standard uncertainty of monitoring dataIts relative expansion uncertainty U is 15% (k 2).
It will be apparent to those skilled in the art that various changes and modifications may be made in the present invention without departing from the spirit and scope of the invention. Thus, if such modifications and variations of the present invention fall within the scope of the claims of the present invention and their equivalents, the present invention is intended to include such modifications and variations. The foregoing examples or embodiments are merely illustrative of the present invention, which may be embodied in other specific forms or in other specific forms without departing from the spirit or essential characteristics thereof. The described embodiments are, therefore, to be considered in all respects as illustrative and not restrictive. The scope of the invention should be indicated by the appended claims, and any changes that are equivalent to the intent and scope of the claims are also intended to be included within the scope of the invention.
Claims (5)
1. In a beta-gamma mixed radiation fieldThe measuring and calculating method is characterized by comprising the following steps:
1) by passingMeasurement of monitorNumerical values, corrected to obtainNumerical values according to correctionNumerically determining the directed dose equivalent rate of gamma ray contribution
2) Determination by beta-spectral measurementCalibration factor N of monitor in beta radiation fieldβA value;
3) determination by gamma spectrometryCalibration factor N of monitor in gamma radiation fieldγA value;
4) according toDirect measurement of monitor, combinedNβAnd NγValue, calculating the directed dose equivalent rate of the beta ray contribution
wherein:
n described in step 2)βThe determination method of the value is as follows:
measuring a beta radiation spectrum in a beta-gamma mixed radiation field by using a beta spectrometer, measuring a spectrum 1 when a probe is exposed, measuring a spectrum 2 at the same position when 5mm of aluminum is added in front of the probe, and respectively correcting the spectrum 1 and the spectrum 2 in dead time and subtracting to obtain a pure beta ray fluence spectrum of a measuring point;
then comparing the pure beta ray fluence spectrum with the spectrum measured by a beta spectrometer in a pure beta radiation field,finding out a standard reference spectrum similar to the measured spectrum of the beta-gamma mixed radiation field, and taking a calibration factor in the beta radiation field corresponding to the standard reference spectrum, namely NβThe value of the sum of the values,
the pure beta radiation field is90Sr-90Y、85Kr and/or147The radiation field of the Pm,
n described in step 3)γThe determination method of the value is as follows:
measuring the gamma-ray energy spectrum of the beta-gamma mixed radiation field by using a gamma spectrometer, or measuring the gamma-ray energy spectrum after sampling the beta-gamma mixed radiation field on site, and combining the energy of the gamma-ray of the measured fieldThe monitor calibrates the result in the standard X, gamma radiation field, finds out the calibration factor of the energy point close to the site in the standard radiation field, and the calibration factor isN of monitor at the actual measurement pointγThe value of the sum of the values,
in the range of 40keV to 1.5MeV whenThe response of the monitor to gamma-ray energy is better than +/-30%, and if the gamma-ray energy of the detected place is of various types and the gamma-ray energy is in the range of 40keV-1.5MeV, the monitor can be selectedMonitor is arranged at137The calibration factor given by calibration in the Cs radiation field is used as N for calculationγThe value of the one or more of the one,
3. The method for measuring and calculating according to claim 1, wherein the correction in step 1) is: for an energy response of better than + -30% in the range of 40keV to 1.5MeV and for a dose rate linearity of better than + -10% in its effective rangeMonitor according to standard radiation fieldResults of the monitor's verification/calibration, usingBy multiplying the value directly measured by the monitor by a calibration factor obtained by verification/calibration, a correction of the measuring point is obtainedNumerical values.
4. The method for measuring and calculating according to claim 1, wherein the correction in step 1) is:
more than + -30% for energy response in the range of 40keV to 1.5MeVIsMonitor according toThe result of the monitor is determined/calibrated in the X, gamma standard radiation field, and the result can be obtainedThe monitor measures the calibration factors of X-ray and gamma-ray radiation fields with different energies;
according to the field gamma measurement spectrum, the energy characteristics of the measured gamma ray can be known, and the energy point can be found in the standard radiation field calibration resultThe calibration factor of the monitor measurements is,the direct measurement value of the monitor being multiplied by the calibration factor to obtain a correction of the measurement pointNumerical values.
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