CN106058289A - Temperature-controlled microbial fuel cell - Google Patents
Temperature-controlled microbial fuel cell Download PDFInfo
- Publication number
- CN106058289A CN106058289A CN201610559346.4A CN201610559346A CN106058289A CN 106058289 A CN106058289 A CN 106058289A CN 201610559346 A CN201610559346 A CN 201610559346A CN 106058289 A CN106058289 A CN 106058289A
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- China
- Prior art keywords
- fuel cell
- temperature
- cathode
- microbiological fuel
- temperature control
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Classifications
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- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/16—Biochemical fuel cells, i.e. cells in which microorganisms function as catalysts
-
- H—ELECTRICITY
- H01—ELECTRIC ELEMENTS
- H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
- H01M8/00—Fuel cells; Manufacture thereof
- H01M8/04—Auxiliary arrangements, e.g. for control of pressure or for circulation of fluids
- H01M8/04298—Processes for controlling fuel cells or fuel cell systems
- H01M8/04694—Processes for controlling fuel cells or fuel cell systems characterised by variables to be controlled
- H01M8/04701—Temperature
- H01M8/04731—Temperature of other components of a fuel cell or fuel cell stacks
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
- Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
- Y02E60/30—Hydrogen technology
- Y02E60/50—Fuel cells
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
- Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
- Y02P70/50—Manufacturing or production processes characterised by the final manufactured product
Abstract
The invention discloses a temperature-controlled microbial fuel cell which comprises a cell body and an ion exchange membrane, wherein the ion exchange membrane is arranged in the middle of the cell body and divides the cell body into an anode chamber and a cathode chamber; an anode body is arranged in the anode chamber; a cathode body is arranged in the cathode chamber, and an opening is formed in the upper end of the cathode chamber; the anode body is inoculated with anaerobic microorganisms; the cathode body is inoculated with aerobic microorganisms or is not inoculated with microorganisms; the anode body is connected with the cathode body through an external resistance to form a closed loop; both the anode body and the cathode body are connected with a temperature control system; the temperature control system comprises a direct current power supply, a temperature controller and a temperature sensor. According to the invention, the surface temperatures of the anode body and the cathode body of the microbial fuel cell can be quickly regulated and controlled, so that the biological activities of the microorganisms are improved, and the reduction reaction of an electron acceptor on the cathode body is accelerated, therefore, the performance of the microbial fuel cell is improved; the temperature-controlled microbial fuel cell is simple in structure and convenient for the expansion of chemical industry production and application.
Description
Technical field
The present invention relates to a kind of battery, particularly relate to a kind of temperature control microbiological fuel cell, belong to green bio energy skill
Art field.
Background technology
Microbiological fuel cell (Microbial Fuel Cell, MFC) is made up of anode chamber and cathode chamber, room, the two poles of the earth it
Between be separated by by ion exchange membrane.Anode microorganism degradation of organic substances under anaerobic environment produces electronics, proton and carbon dioxide;
Electric transmission arrives biological-cathode to anode by external circuit load, and proton is arrived negative electrode by ion exchange membrane by anode chamber
Room;Cathode chamber electron acceptor oxygen obtains electronics and proton at negative electrode and is reduced into water, thus produces electric current.Microbial fuel
Battery is a kind of New Green Energy source technology, obtains in year studying extensively and profoundly nearly youngster, for solving energy shortage and sewage disposal
Provide a new way.
Up to the present, the actual performance of the microbiological fuel cell in laboratory is than ideal performance or much lower.Micro-
The electricity generation performance of biological fuel cell produces to be affected by several factors.The product electricity of microbiological fuel cell include several mainly
Process: the metabolism of microorganism, electronics are delivered to anode from cell, proton transfers to electron acceptor negative electrode and negative electrode from anode
Reduction reaction, in these parts, each small details directly influences the performance of microbiological fuel cell.
The low transformation efficiency of microorganism in battery, even under optimum growth speed, microbial transformation efficiency with
And and electrode between electron transmission the slowest.And high temperature can speed up almost all of kinetics, including biology
With chemistry.Can improve electronics transformation efficiency in microorganism by the method heated up, the activation reducing electrode reaction is damaged
Lose.
Being generally all to utilize oxygen as the electron acceptor of reduction reaction in negative electrode in microbiological fuel cell, oxygen is also
Former kinetic factor is also a restriction factor of microbiological fuel cell performance.Intensification can improve mass transfer speed,
Accelerate the electrode reaction of negative electrode, thus improve the performance of battery.
By in whole for the microbiological fuel cell tank being placed on temperature regulating device, it is possible to obtain stable isoperibol,
Chinese patent literary composition CN101916871A discloses the temperature regulating device of a kind of microbiological fuel cell, by tank, baffle plate, titanium heating
Pipe, thermocouple, water circulating pump, semiconductor cooler and electrical equipment control instrument are constituted;Tank is rectangle structure and is provided with into water
Mouth and outlet, inboard wall of cistern is provided with baffle plate slot;Baffle plate is rectangular slab and has rectangle water flow hole;Titanium add heat pipe and
Thermocouple is fixed in tank;Water circulating pump water inlet is connected with sink outlet by pipeline, and water circulating pump outlet passes through
Pipeline is connected with semiconductor cooler water inlet, and semiconductor cooler outlet is connected with tank water inlet by pipeline;Titanium adds
Heat pipe, thermocouple, water circulating pump and semiconductor cooler are connected with electrical equipment control instrument by wire respectively.This device can root
According to reaction temperature need realize the rising of temperature and reduction, the further investigation for microbiological fuel cell operation process condition carries
For strong experiment condition, but in the case of microbiological fuel cell volume ratio is relatively big, particularly during Treating Municipal Sewage
Needing the battery of large volume, the time required for overall temperature control acquisition equilibrium temperature is long, makes whole microbiological fuel cell overall
External energy required for constant temperature is huge.The present invention devises a kind of temperature control microbiological fuel cell.Utilize the present invention, not only may be used
With monitoring anode of microbial fuel cell and cathode surface temperature, and can quickly regulate and control anode and negative electrode by temperature control circuit
Surface temperature.The present invention can improve the biological activity of microorganism, accelerates the reduction reaction of electron acceptor on negative electrode, thus improves
The performance of microbiological fuel cell, reduces decomposing organic pollutant required time.Compare with heating whole microbiological fuel cell,
Little energy needed for the present invention, it is possible to greatly reduce the cost that microbiological fuel cell heats up.Microorganism of the present invention
Fuel-cell device simple in construction, it is simple to extension commercial production and application.
Summary of the invention
It is an object of the invention to propose a kind of temperature control microbiological fuel cell, control Microbial fuel by temperature control circuit
The anode bodies of battery and cathode surface temperature, improve the biological activity of microorganism, accelerates the reduction of electron acceptor on negative electrode anti-
Should, thus improve the performance of microbiological fuel cell, reduce decomposing organic pollutant required time;Energy needed for the present invention
Few, it is possible to greatly reduce the cost that microbiological fuel cell heats up;Microbial fuel cell unit structure of the present invention
Simply, it is simple to extension commercial production and application.
The technical solution adopted in the present invention: a kind of temperature control microbiological fuel cell, exchanges including battery body and ion
Film, described ion exchange membrane is arranged in the middle part of described battery body and described battery body is divided into anode chamber and cathode chamber, institute
It is provided with anode bodies in stating anode chamber, is provided with cathode in described cathode chamber and described cathode chamber upper end arranges opening, institute
State anode bodies inoculation anaerobe, cathode inoculation aerobic microbiological or not microbe inoculation, described anode bodies and described the moon
Polar body connects formation closed-loop path by external resistance, and described anode bodies and described cathode are respectively connected with temperature-controlling system.
Preferably, described temperature-controlling system includes DC source, temperature controller and temperature sensor, described DC source with
The power end of described temperature controller connects, the temperature signal receiving terminal of described temperature controller and the temperature of described temperature sensor
Degree signal output part connects, and described temperature sensor is arranged on described anode bodies and described cathode outer surface.
Preferably, described anode bodies and described cathode are by internal layer heating plate, intermediate layer thermal conductive insulator and outer layer electricity
Pole active body composition.
Preferably, described heating plate is metal material or nonmetallic materials or alloy material.
Preferably, described thermal conductive insulator can be heat-conducting silicone grease, heat conduction adhesive tape, heat conduction mica sheet, thermal conductive ceramic plate,
One or more in heat conduction silica gel sheet.
Preferably, described electrode active gonosome can be carbon slurry, carbon cloth, graphite flake, carbon paste, CNT, Graphene, stainless
Steel, titanium sheet material.
Preferably, described closed-loop path includes wire, external resistance and voltmeter.
Preferably, described temperature sensor can be critesistor or thermocouple.
Preferably, the quantity of described temperature sensor wires is at least two.
Preferably, the quantity of described temperature controller is one or two.
Compared with prior art, the invention has the beneficial effects as follows: the present invention can rapidly regulating and controlling microbial fuel cell sun
Polar body and the temperature on cathode surface, improve the biological activity of microorganism, accelerates the reduction reaction of electron acceptor on negative electrode, thus
Improve the performance of microbiological fuel cell, reduce decomposing organic pollutant required time;With traditional heating whole microorganism combustion
Material battery is compared, the little energy needed for the present invention, it is possible to greatly reduce the cost that microbiological fuel cell heats up;Institute of the present invention
The microbial fuel cell unit simple in construction stated, it is simple to extension commercial production and application.
Accompanying drawing explanation
Fig. 1 is the structural representation of the present invention a kind of temperature control microbiological fuel cell.
Fig. 2 is the structural representation of one one kinds of temperature control microbiological fuel cells of the embodiment of the present invention.
Detailed description of the invention
Technical scheme is further illustrated below in conjunction with specific embodiment.
As it is shown in figure 1, a kind of temperature control microbiological fuel cell, including battery body 1 and ion exchange membrane 2, described ion
Exchange membrane 2 is arranged in the middle part of described battery body 1 and described battery body 1 is divided into anode chamber 3 and cathode chamber 4, described anode
It is provided with anode bodies in room 3, is provided with cathode in described cathode chamber 4 and described cathode chamber 4 upper end arranges opening 14, be used for
Enter for atmospheric gas;Described anode bodies inoculation anaerobe 5, cathode inoculation aerobic microbiological or not microbe inoculation,
Described anode bodies and described cathode connect formation closed-loop path 7 by external resistance 6, and described anode bodies and described cathode all connect
It is connected to temperature-controlling system.
Described temperature-controlling system includes DC source 8, temperature controller 9 and temperature sensor 10, described DC source 8 and institute
The power end stating temperature controller 9 connects, the temperature signal receiving terminal of described temperature controller 9 and described temperature sensor 10
Temperature signal outfan connects, and described temperature sensor 10 is arranged on described anode bodies and described cathode outer surface, described sun
Polar body and described cathode are formed with outer electrode active body 13 by internal layer heating plate 11, intermediate layer thermal conductive insulator 12, institute
Stating heating plate 11 is metal material or nonmetallic materials or alloy material, and described closed-loop path includes wire 7, external resistance 6 and electricity
Pressure table 15.
In the concrete technical scheme of the present invention, in temperature-controlling system, DC source 8 is responsible for providing unidirectional current, temperature sensing
Device 10 measures anode bodies and the temperature on cathode surface and feeds back to temperature controller 9, and temperature controller 9 is applied to by regulation
Internal layer heating plate 11 size of current of anode bodies and cathode controls anode bodies and the temperature on cathode surface;Described internal layer
Heating plate 11 can be metal material such as copper sheet, nickel sheet, iron plate etc., can be nonmetallic materials such as carbon plate etc., it is also possible to be to close
Gold copper-base alloy such as iron-nickel alloy sheet, nichrome film, iron-nickel-chromium sheet etc..
Described thermal conductive insulator 12 can be heat-conducting silicone grease, heat conduction adhesive tape, heat conduction mica sheet, thermal conductive ceramic plate, heat conduction
One or more in silica gel sheet, described electrode active gonosome can be carbon slurry, carbon cloth, graphite flake, carbon paste, CNT, graphite
Alkene, rustless steel, titanium sheet material, described temperature sensor 10 can be critesistor or thermocouple, and described temperature sensor 10 is drawn
The quantity of line is at least two, and the quantity of described temperature controller 9 is one or two.The described anode bodies inoculation micro-life of anaerobism
Thing, anaerobe 5 can be Actinobacillus succinogenes, Aeromonas hydrophila, Clostridium beijerinckii, Shewanella putrefaciens etc., negative electrode
Body inoculation aerobic microbiological or not microbe inoculation;Anode microbial decomposition metabolism Organic substance produces electronics, and electronics passes through dispatch from foreign news agency
Road moves to cathode chamber 4, and oxygen and electronics and the proton that passes through from anode chamber 3, at cathode chamber 4 water generation reaction, produce simultaneously
Electric energy;Described temperature sensor 10 can be critesistor such as Pt100, Pt1000, Pt10000, Cu50, NTC, PTC etc., it is possible to
To be thermocouple such as K-type thermocouple, J-type thermocouple, T-shaped thermocouple, S type thermocouple, Type B thermocouple etc..
The present invention can regulating and controlling microbial anode of fuel cell body and the temperature on cathode surface rapidly, improve microorganism
Biological activity, accelerates the reduction reaction of electron acceptor on cathode, thus improves the performance of microbiological fuel cell, reduce and decompose
Organic pollution required time;Compare with heating whole microbiological fuel cell, the little energy needed for the present invention, it is possible to significantly drop
The cost that low microbiological fuel cell heats up;Microbial fuel cell unit simple in construction of the present invention, it is simple to expand
Chemical industry produces and application.
Embodiment one
As in figure 2 it is shown, a kind of temperature control microbiological fuel cell, including battery body 1 and ion exchange membrane 2, described ion
Exchange membrane 2 is arranged in the middle part of described battery body 1 and described battery body 1 is divided into anode chamber 3 and cathode chamber 4, described anode
It is provided with anode bodies in room 3, is provided with cathode in described cathode chamber 4 and described cathode chamber 4 upper end arranges opening 14, described
Anode bodies inoculation anaerobe 5, cathode inoculation aerobic microbiological or not microbe inoculation, described anode bodies and described negative electrode
Body connects formation closed-loop path 7 by external resistance 6, and described anode bodies and described cathode are respectively connected with temperature-controlling system.
Described temperature-controlling system includes DC source 8, temperature controller 9 and temperature sensor 10, described DC source 8 and institute
The power end stating temperature controller 9 connects, the temperature signal receiving terminal of described temperature controller 9 and described temperature sensor 10
Temperature signal outfan connects, and described temperature sensor 10 is arranged on described anode bodies and described cathode outer surface, described sun
Polar body and described cathode are formed with outer electrode active body 13 by internal layer heating plate 11, intermediate layer thermal conductive insulator 12, institute
Stating heating plate 11 is metal material or nonmetallic materials or alloy material, and described closed-loop path includes wire 7, external resistance 6 and electricity
Pressure table 15.
During concrete practicality: modify last layer thermal conductive insulator 12 at heating plate 11 outer layer, and repair in thermal conductive insulator 12
Decorations last layer electrode active gonosome 13, and temperature sensor 10 is fixed on electrode active gonosome 13 surface by epoxide-resin glue.Right
For anode bodies, in addition it is also necessary to inoculate anaerobe 5 at anode bodies electrode active gonosome.Anode bodies and cathode lay respectively at sun
Room, pole 3 and cathode chamber 4, separated by cation exchange membrane 2 between two Room.Anode bodies and cathode are by wire 7 and external resistance 6
Connecting and form closed-loop path, voltmeter 15 is for detecting and control the voltage of closed-loop path.Output voltage passes through data acquisition unit
It is automatically logged in computer.In temperature-controlling system, DC source 8 is connected with temperature controller 9 offer unidirectional current, temperature sensing
Device 10 measures anode bodies and the temperature on cathode surface and feeds back to temperature controller 10, and temperature controller 10 is exported by regulation
The size of electric current controls anode bodies and the temperature on cathode surface.Cathode chamber 4 is in unlimited atmospheric environment, and sets inducing QI
Pipe enters from cathode chamber 4 upper end for air.Anode chamber 3 adds can the organic wastewater of biochemical treatment make it be in airtight anaerobism
In environment, the oxidation operation in waste water is decomposed and produces electronics, proton by metabolism by the electricity microorganism of producing in anode chamber 3,
Electronics transfers to negative electrode through external circuit, and proton is diffused into cathode chamber 4 via cation exchange membrane, the oxygen in cathode chamber 4 with from
Anode bodies is delivered to the electronics of cathode chamber 4 by wire and enters the proton combination generation water of cathode chamber through cation exchange membrane
Realize electricity generation process.
In a preferred embodiment of the present invention, described heating plate 11 is copper sheet.
In a preferred embodiment of the present invention, described thermal conductive insulator 12 is heat-conducting silicone grease.
In a preferred embodiment of the present invention, described electrode active gonosome 13 is starched for carbon, and is modified by screen printing technique
In thermal conductive insulator 12.
In a preferred embodiment of the present invention, described temperature sensor 10 is Pt1000, goes between as three-wire system.
Beneficial effect: utilize the present invention, is possible not only to monitor anode of microbial fuel cell body and cathode surface temperature,
And can quickly regulate and control anode bodies and cathode surface temperature by temperature-controlling system.The present invention can improve the biology of microorganism
Activity, accelerates the reduction reaction of electron acceptor on cathode, thus improves the performance of microbiological fuel cell, reduce decomposition organic
Pollutant required time.Compare with heating whole microbiological fuel cell, the little energy needed for the present invention, it is possible to greatly reduce
The cost that microbiological fuel cell heats up.Microbial fuel cell unit simple in construction of the present invention, it is simple to expand chemical industry
Industry produces and application.
For a person skilled in the art, can technical scheme as described above and design, make other each
Plant corresponding change and deformation, and all these changes and deforms the protection model that all should belong to the claims in the present invention
Within enclosing.
Claims (10)
1. a temperature control microbiological fuel cell, it is characterised in that: including battery body and ion exchange membrane, described ion exchanges
Film is arranged in the middle part of described battery body and described battery body is divided into anode chamber and cathode chamber, is provided with in described anode chamber
Anode bodies, is provided with cathode in described cathode chamber and described cathode chamber upper end arranges opening, described anode bodies inoculation anaerobism
Microorganism, cathode inoculation aerobic microbiological or not microbe inoculation, described anode bodies and described cathode are by external resistance even
Connecing formation closed-loop path, described anode bodies and described cathode are respectively connected with temperature-controlling system.
A kind of temperature control microbiological fuel cell the most according to claim 1, it is characterised in that: described temperature-controlling system includes directly
Stream power supply, temperature controller and temperature sensor, described DC source is connected with the power end of described temperature controller, described temperature
The temperature signal receiving terminal of degree controller is connected with the temperature signal outfan of described temperature sensor, and described temperature sensor sets
Put at described anode bodies and described cathode outer surface.
A kind of temperature control microbiological fuel cell the most according to claim 2, it is characterised in that: described anode bodies and described the moon
Polar body is formed with outer electrode active body by internal layer heating plate, intermediate layer thermal conductive insulator.
4. according to a kind of temperature control microbiological fuel cell described in Claims 2 or 3, it is characterised in that: described heating plate is gold
Belong to material or nonmetallic materials or alloy material.
A kind of temperature control microbiological fuel cell the most according to claim 3, it is characterised in that: described thermal conductive insulator can
To be one or more in heat-conducting silicone grease, heat conduction adhesive tape, heat conduction mica sheet, thermal conductive ceramic plate, heat conduction silica gel sheet.
A kind of temperature control microbiological fuel cell the most according to claim 1, it is characterised in that: described electrode active gonosome is permissible
It is carbon slurry, carbon cloth, graphite flake, carbon paste, CNT, Graphene, rustless steel, titanium sheet material.
A kind of temperature control microbiological fuel cell the most according to claim 1, it is characterised in that: described closed-loop path includes leading
Line, external resistance and voltmeter.
A kind of temperature control microbiological fuel cell the most according to claim 2, it is characterised in that: described temperature sensor is permissible
It is critesistor or thermocouple.
A kind of temperature control microbiological fuel cell the most according to claim 1, it is characterised in that: described temperature sensor wires
Quantity be at least two.
A kind of temperature control microbiological fuel cell the most according to claim 1, it is characterised in that: described temperature controller
Quantity is one or two.
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Cited By (3)
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CN107959037A (en) * | 2017-12-05 | 2018-04-24 | 苏州喷声电子科技有限公司 | It is a kind of that there is the microbiological fuel cell pond for adjusting temperature |
CN112547791A (en) * | 2020-11-12 | 2021-03-26 | 江苏大地益源环境修复有限公司 | Pollutant remediation method and device for strengthening microbial fuel cell by using Seebeck effect |
CN113740402A (en) * | 2021-07-27 | 2021-12-03 | 中国科学院重庆绿色智能技术研究院 | BOD measures intelligent sensor |
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