CN102257182B - 用于还原分子氧的电化学方法 - Google Patents

用于还原分子氧的电化学方法 Download PDF

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Publication number
CN102257182B
CN102257182B CN200980150665.8A CN200980150665A CN102257182B CN 102257182 B CN102257182 B CN 102257182B CN 200980150665 A CN200980150665 A CN 200980150665A CN 102257182 B CN102257182 B CN 102257182B
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China
Prior art keywords
nitrogen
carbon nanotubes
doped carbon
electrode
oxygen
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Expired - Fee Related
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CN200980150665.8A
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English (en)
Chinese (zh)
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CN102257182A (zh
Inventor
J.阿斯曼
A.沃尔夫
L.姆莱齐科
A.卡彭科
V.米歇尔
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Covestro Deutschland AG
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Bayer Pharma AG
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    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B82—NANOTECHNOLOGY
    • B82Y—SPECIFIC USES OR APPLICATIONS OF NANOSTRUCTURES; MEASUREMENT OR ANALYSIS OF NANOSTRUCTURES; MANUFACTURE OR TREATMENT OF NANOSTRUCTURES
    • B82Y30/00—Nanotechnology for materials or surface science, e.g. nanocomposites
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B1/00—Electrolytic production of inorganic compounds or non-metals
    • C25B1/01—Products
    • C25B1/14—Alkali metal compounds
    • C25B1/16—Hydroxides
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B1/00—Electrolytic production of inorganic compounds or non-metals
    • C25B1/01—Products
    • C25B1/34—Simultaneous production of alkali metal hydroxides and chlorine, oxyacids or salts of chlorine, e.g. by chlor-alkali electrolysis
    • C25B1/46—Simultaneous production of alkali metal hydroxides and chlorine, oxyacids or salts of chlorine, e.g. by chlor-alkali electrolysis in diaphragm cells
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
    • C25B11/04—Electrodes; Manufacture thereof not otherwise provided for characterised by the material
    • C25B11/042—Electrodes formed of a single material
    • C25B11/043—Carbon, e.g. diamond or graphene
    • C25B11/044—Impregnation of carbon
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B15/00—Operating or servicing cells
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B15/00—Operating or servicing cells
    • C25B15/02—Process control or regulation
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B9/00—Cells or assemblies of cells; Constructional parts of cells; Assemblies of constructional parts, e.g. electrode-diaphragm assemblies; Process-related cell features
    • C25B9/17—Cells comprising dimensionally-stable non-movable electrodes; Assemblies of constructional parts thereof
    • C25B9/19—Cells comprising dimensionally-stable non-movable electrodes; Assemblies of constructional parts thereof with diaphragms
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J21/00—Catalysts comprising the elements, oxides, or hydroxides of magnesium, boron, aluminium, carbon, silicon, titanium, zirconium, or hafnium
    • B01J21/18—Carbon
    • B01J21/185—Carbon nanotubes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M12/00—Hybrid cells; Manufacture thereof
    • H01M12/04—Hybrid cells; Manufacture thereof composed of a half-cell of the fuel-cell type and of a half-cell of the primary-cell type
    • H01M12/06—Hybrid cells; Manufacture thereof composed of a half-cell of the fuel-cell type and of a half-cell of the primary-cell type with one metallic and one gaseous electrode
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/36—Hydrogen production from non-carbon containing sources, e.g. by water electrolysis

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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Nanotechnology (AREA)
  • Automation & Control Theory (AREA)
  • General Physics & Mathematics (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Condensed Matter Physics & Semiconductors (AREA)
  • Composite Materials (AREA)
  • Physics & Mathematics (AREA)
  • Catalysts (AREA)
  • Carbon And Carbon Compounds (AREA)
  • Oxygen, Ozone, And Oxides In General (AREA)
  • Electrolytic Production Of Non-Metals, Compounds, Apparatuses Therefor (AREA)
  • Electrodes For Compound Or Non-Metal Manufacture (AREA)
CN200980150665.8A 2008-12-18 2009-12-05 用于还原分子氧的电化学方法 Expired - Fee Related CN102257182B (zh)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
DE102008063727A DE102008063727A1 (de) 2008-12-18 2008-12-18 Elektrochemisches Verfahren zur Reduktion molekularen Sauerstoffs
DE102008063727.0 2008-12-18
PCT/EP2009/008699 WO2010069490A1 (de) 2008-12-18 2009-12-05 Elektrochemisches verfahren zur reduktion molekularen sauerstoffs

Publications (2)

Publication Number Publication Date
CN102257182A CN102257182A (zh) 2011-11-23
CN102257182B true CN102257182B (zh) 2015-05-20

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CN200980150665.8A Expired - Fee Related CN102257182B (zh) 2008-12-18 2009-12-05 用于还原分子氧的电化学方法

Country Status (7)

Country Link
US (2) US20110233071A1 (enExample)
EP (1) EP2379782B1 (enExample)
JP (1) JP5607064B2 (enExample)
CN (1) CN102257182B (enExample)
DE (1) DE102008063727A1 (enExample)
SG (1) SG172041A1 (enExample)
WO (1) WO2010069490A1 (enExample)

Families Citing this family (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE102009058833A1 (de) * 2009-12-18 2011-06-22 Bayer Technology Services GmbH, 51373 Stickstoff-dotierte Kohlenstoffnanoröhrchen mit Metall-Nanopartikeln
DE102009058832A1 (de) 2009-12-18 2011-06-30 Bayer Technology Services GmbH, 51373 Verfahren zur elektrochemischen Sauerstoffreduktion im Alkalischen
JP5638433B2 (ja) 2011-03-24 2014-12-10 株式会社東芝 電解装置および冷蔵庫
JP6281906B2 (ja) * 2014-05-15 2018-02-21 国立大学法人 名古屋工業大学 空気極、金属空気電池、並びに窒素がドープされたカーボンナノチューブ及び空気極の製造方法
DE102014218368A1 (de) 2014-09-12 2016-03-17 Covestro Deutschland Ag Sauerstoffverzehrelektrode und Verfahren zu ihrer Herstellung
DE102014218367A1 (de) 2014-09-12 2016-03-17 Covestro Deutschland Ag Sauerstoffverzehrelektrode und Verfahren zu ihrer Herstellung
CN107196020A (zh) * 2017-06-03 2017-09-22 太原理工大学 氮掺杂碳纳米管阵列/碳纤维材料空气电极的制备方法

Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN1620528A (zh) * 2001-01-29 2005-05-25 威廉马歇莱思大学 用重氮化合物衍生碳纳米管的方法及其复合材料

Family Cites Families (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPS5669384A (en) * 1979-11-09 1981-06-10 Asahi Glass Co Ltd Preparation of caustic alkali
US20070275160A1 (en) * 2003-10-10 2007-11-29 Stephen Maldonado Carbon Nanostructure-Based Electrocatalytic Electrodes
DE102006007147A1 (de) * 2006-02-16 2007-08-23 Bayer Technology Services Gmbh Verfahren zur kontinuierlichen Herstellung von Katalysatoren
JP5068029B2 (ja) * 2006-03-31 2012-11-07 株式会社日鉄技術情報センター 酸素還元複合触媒及びその製造方法並びにこれを用いた燃料電池
US7629285B2 (en) * 2006-10-31 2009-12-08 University Of South Carolina Carbon-based composite electrocatalysts for low temperature fuel cells
DE102007062421A1 (de) 2007-12-20 2009-06-25 Bayer Technology Services Gmbh Verfahren zur Herstellung von Stickstoff-dotierten Kohlenstoffnanoröhrchen
JP2010009807A (ja) * 2008-06-25 2010-01-14 Nec Corp 空気極用燃料電池触媒、その製造方法、電極および燃料電池

Patent Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN1620528A (zh) * 2001-01-29 2005-05-25 威廉马歇莱思大学 用重氮化合物衍生碳纳米管的方法及其复合材料

Non-Patent Citations (4)

* Cited by examiner, † Cited by third party
Title
nitrogen-doped carbon nanostructures and their composites as catalytic materials for proten exchange membrane fuel cell;SHAO,et.al;《applied catalysis B:environmental》;20071012;第79卷(第1期);第89-99页 *
oxygen reduction reaction activity and surface properties of nanostructured nitrogen-containing carbon;P.H.MATTER,et.al;《journal of molecular catalysis A:chemical》;20060909;第264卷;第73-81页 *
surface modification of carbons for enhanced electrochemical activity;X.CHU.et.al;《material science and engineering》;19970905;第49卷;第53-60页 *
the role of nanostructure in nitrogen_conatining carbon catalysts for the oxygen reduction reaction;P.H.MATTER,et.al;《journal of catalysis》;20060210;第239卷;第83-96页 *

Also Published As

Publication number Publication date
CN102257182A (zh) 2011-11-23
WO2010069490A1 (de) 2010-06-24
JP5607064B2 (ja) 2014-10-15
DE102008063727A1 (de) 2010-06-24
US20170107634A1 (en) 2017-04-20
US20110233071A1 (en) 2011-09-29
EP2379782A1 (de) 2011-10-26
SG172041A1 (en) 2011-07-28
EP2379782B1 (de) 2013-07-10
JP2012512328A (ja) 2012-05-31

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