AU600255B2 - Novel polymer barrier blends - Google Patents
Novel polymer barrier blends Download PDFInfo
- Publication number
- AU600255B2 AU600255B2 AU68691/87A AU6869187A AU600255B2 AU 600255 B2 AU600255 B2 AU 600255B2 AU 68691/87 A AU68691/87 A AU 68691/87A AU 6869187 A AU6869187 A AU 6869187A AU 600255 B2 AU600255 B2 AU 600255B2
- Authority
- AU
- Australia
- Prior art keywords
- polymer
- blend
- organic liquid
- polymers
- vapor
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Ceased
Links
- 229920000642 polymer Polymers 0.000 title claims description 95
- 239000000203 mixture Substances 0.000 title claims description 53
- 230000004888 barrier function Effects 0.000 title claims description 37
- 239000007788 liquid Substances 0.000 claims description 43
- -1 poly(hexamethylene adipamide) Polymers 0.000 claims description 26
- 229920001577 copolymer Polymers 0.000 claims description 23
- 238000004132 cross linking Methods 0.000 claims description 23
- 238000000034 method Methods 0.000 claims description 23
- 150000002978 peroxides Chemical class 0.000 claims description 22
- 239000007822 coupling agent Substances 0.000 claims description 21
- 238000002156 mixing Methods 0.000 claims description 21
- VGGSQFUCUMXWEO-UHFFFAOYSA-N Ethene Chemical compound C=C VGGSQFUCUMXWEO-UHFFFAOYSA-N 0.000 claims description 20
- 239000005977 Ethylene Substances 0.000 claims description 20
- 229920002959 polymer blend Polymers 0.000 claims description 20
- 230000035699 permeability Effects 0.000 claims description 18
- 230000008569 process Effects 0.000 claims description 17
- 239000004952 Polyamide Substances 0.000 claims description 11
- 229920002647 polyamide Polymers 0.000 claims description 11
- 229920002302 Nylon 6,6 Polymers 0.000 claims description 9
- 125000000524 functional group Chemical group 0.000 claims description 8
- 230000005855 radiation Effects 0.000 claims description 8
- 229920000139 polyethylene terephthalate Polymers 0.000 claims description 7
- 239000005020 polyethylene terephthalate Substances 0.000 claims description 7
- 150000002148 esters Chemical class 0.000 claims description 6
- 229920002292 Nylon 6 Polymers 0.000 claims description 5
- 150000008064 anhydrides Chemical class 0.000 claims description 5
- 125000003178 carboxy group Chemical group [H]OC(*)=O 0.000 claims description 5
- 150000004985 diamines Chemical class 0.000 claims description 5
- 239000006185 dispersion Substances 0.000 claims description 5
- 229920000728 polyester Polymers 0.000 claims description 5
- NINIDFKCEFEMDL-UHFFFAOYSA-N Sulfur Chemical group [S] NINIDFKCEFEMDL-UHFFFAOYSA-N 0.000 claims description 4
- 239000003795 chemical substances by application Substances 0.000 claims description 4
- 229920001038 ethylene copolymer Polymers 0.000 claims description 4
- 239000000945 filler Substances 0.000 claims description 4
- 125000002887 hydroxy group Chemical group [H]O* 0.000 claims description 4
- 229920003023 plastic Polymers 0.000 claims description 4
- 239000004033 plastic Substances 0.000 claims description 4
- 239000005077 polysulfide Substances 0.000 claims description 4
- 229920001021 polysulfide Polymers 0.000 claims description 4
- 150000008117 polysulfides Polymers 0.000 claims description 4
- 150000003254 radicals Chemical group 0.000 claims description 4
- 229910052717 sulfur Inorganic materials 0.000 claims description 4
- 239000011593 sulfur Substances 0.000 claims description 4
- UGFAIRIUMAVXCW-UHFFFAOYSA-N Carbon monoxide Chemical compound [O+]#[C-] UGFAIRIUMAVXCW-UHFFFAOYSA-N 0.000 claims description 3
- 229920001328 Polyvinylidene chloride Polymers 0.000 claims description 3
- 229910002091 carbon monoxide Inorganic materials 0.000 claims description 3
- 150000001875 compounds Chemical class 0.000 claims description 3
- JBKVHLHDHHXQEQ-UHFFFAOYSA-N epsilon-caprolactam Chemical compound O=C1CCCCCN1 JBKVHLHDHHXQEQ-UHFFFAOYSA-N 0.000 claims description 3
- 239000000178 monomer Substances 0.000 claims description 3
- 239000002245 particle Substances 0.000 claims description 3
- 150000004965 peroxy acids Chemical class 0.000 claims description 3
- 229920002239 polyacrylonitrile Polymers 0.000 claims description 3
- 229920001470 polyketone Polymers 0.000 claims description 3
- 229920000874 polytetramethylene terephthalate Polymers 0.000 claims description 3
- 229920000915 polyvinyl chloride Polymers 0.000 claims description 3
- 239000004800 polyvinyl chloride Substances 0.000 claims description 3
- 239000005033 polyvinylidene chloride Substances 0.000 claims description 3
- 239000007787 solid Substances 0.000 claims description 3
- NLHHRLWOUZZQLW-UHFFFAOYSA-N Acrylonitrile Chemical compound C=CC#N NLHHRLWOUZZQLW-UHFFFAOYSA-N 0.000 claims description 2
- XTXRWKRVRITETP-UHFFFAOYSA-N Vinyl acetate Chemical compound CC(=O)OC=C XTXRWKRVRITETP-UHFFFAOYSA-N 0.000 claims description 2
- 239000011343 solid material Substances 0.000 claims description 2
- 150000001735 carboxylic acids Chemical class 0.000 claims 1
- 150000002118 epoxides Chemical class 0.000 claims 1
- CTQNGGLPUBDAKN-UHFFFAOYSA-N O-Xylene Chemical compound CC1=CC=CC=C1C CTQNGGLPUBDAKN-UHFFFAOYSA-N 0.000 description 18
- 239000008096 xylene Substances 0.000 description 18
- 238000012360 testing method Methods 0.000 description 9
- 239000008188 pellet Substances 0.000 description 7
- XMNIXWIUMCBBBL-UHFFFAOYSA-N 2-(2-phenylpropan-2-ylperoxy)propan-2-ylbenzene Chemical compound C=1C=CC=CC=1C(C)(C)OOC(C)(C)C1=CC=CC=C1 XMNIXWIUMCBBBL-UHFFFAOYSA-N 0.000 description 6
- 239000000155 melt Substances 0.000 description 6
- 239000004698 Polyethylene Substances 0.000 description 5
- 229930195733 hydrocarbon Natural products 0.000 description 5
- 150000002430 hydrocarbons Chemical class 0.000 description 5
- 229920000573 polyethylene Polymers 0.000 description 5
- 239000004215 Carbon black (E152) Substances 0.000 description 4
- 230000007423 decrease Effects 0.000 description 4
- 238000001125 extrusion Methods 0.000 description 4
- 238000001000 micrograph Methods 0.000 description 4
- YXFVVABEGXRONW-UHFFFAOYSA-N Toluene Chemical compound CC1=CC=CC=C1 YXFVVABEGXRONW-UHFFFAOYSA-N 0.000 description 3
- 230000000052 comparative effect Effects 0.000 description 3
- 230000000694 effects Effects 0.000 description 3
- 229920006242 ethylene acrylic acid copolymer Polymers 0.000 description 3
- 239000000463 material Substances 0.000 description 3
- 229920003145 methacrylic acid copolymer Polymers 0.000 description 3
- 229940117841 methacrylic acid copolymer Drugs 0.000 description 3
- 239000000126 substance Substances 0.000 description 3
- 229920001897 terpolymer Polymers 0.000 description 3
- 230000004580 weight loss Effects 0.000 description 3
- QPFMBZIOSGYJDE-UHFFFAOYSA-N 1,1,2,2-tetrachloroethane Chemical compound ClC(Cl)C(Cl)Cl QPFMBZIOSGYJDE-UHFFFAOYSA-N 0.000 description 2
- OZAIFHULBGXAKX-UHFFFAOYSA-N 2-(2-cyanopropan-2-yldiazenyl)-2-methylpropanenitrile Chemical compound N#CC(C)(C)N=NC(C)(C)C#N OZAIFHULBGXAKX-UHFFFAOYSA-N 0.000 description 2
- KUBDPQJOLOUJRM-UHFFFAOYSA-N 2-(chloromethyl)oxirane;4-[2-(4-hydroxyphenyl)propan-2-yl]phenol Chemical compound ClCC1CO1.C=1C=C(O)C=CC=1C(C)(C)C1=CC=C(O)C=C1 KUBDPQJOLOUJRM-UHFFFAOYSA-N 0.000 description 2
- KAKZBPTYRLMSJV-UHFFFAOYSA-N Butadiene Chemical compound C=CC=C KAKZBPTYRLMSJV-UHFFFAOYSA-N 0.000 description 2
- VTYYLEPIZMXCLO-UHFFFAOYSA-L Calcium carbonate Chemical compound [Ca+2].[O-]C([O-])=O VTYYLEPIZMXCLO-UHFFFAOYSA-L 0.000 description 2
- 229920006051 Capron® Polymers 0.000 description 2
- VZCYOOQTPOCHFL-OWOJBTEDSA-N Fumaric acid Chemical compound OC(=O)\C=C\C(O)=O VZCYOOQTPOCHFL-OWOJBTEDSA-N 0.000 description 2
- 229920000339 Marlex Polymers 0.000 description 2
- CERQOIWHTDAKMF-UHFFFAOYSA-N Methacrylic acid Chemical compound CC(=C)C(O)=O CERQOIWHTDAKMF-UHFFFAOYSA-N 0.000 description 2
- BAPJBEWLBFYGME-UHFFFAOYSA-N Methyl acrylate Chemical compound COC(=O)C=C BAPJBEWLBFYGME-UHFFFAOYSA-N 0.000 description 2
- PPBRXRYQALVLMV-UHFFFAOYSA-N Styrene Chemical compound C=CC1=CC=CC=C1 PPBRXRYQALVLMV-UHFFFAOYSA-N 0.000 description 2
- 229920006102 Zytel® Polymers 0.000 description 2
- 239000002253 acid Substances 0.000 description 2
- 239000004927 clay Substances 0.000 description 2
- 238000013329 compounding Methods 0.000 description 2
- 150000001993 dienes Chemical class 0.000 description 2
- 238000010101 extrusion blow moulding Methods 0.000 description 2
- 230000006872 improvement Effects 0.000 description 2
- 238000012545 processing Methods 0.000 description 2
- 229920005989 resin Polymers 0.000 description 2
- 239000011347 resin Substances 0.000 description 2
- 239000002904 solvent Substances 0.000 description 2
- SMZOUWXMTYCWNB-UHFFFAOYSA-N 2-(2-methoxy-5-methylphenyl)ethanamine Chemical compound COC1=CC=C(C)C=C1CCN SMZOUWXMTYCWNB-UHFFFAOYSA-N 0.000 description 1
- NIXOWILDQLNWCW-UHFFFAOYSA-N 2-Propenoic acid Natural products OC(=O)C=C NIXOWILDQLNWCW-UHFFFAOYSA-N 0.000 description 1
- CFVWNXQPGQOHRJ-UHFFFAOYSA-N 2-methylpropyl prop-2-enoate Chemical compound CC(C)COC(=O)C=C CFVWNXQPGQOHRJ-UHFFFAOYSA-N 0.000 description 1
- IEPRKVQEAMIZSS-UHFFFAOYSA-N Di-Et ester-Fumaric acid Natural products CCOC(=O)C=CC(=O)OCC IEPRKVQEAMIZSS-UHFFFAOYSA-N 0.000 description 1
- IEPRKVQEAMIZSS-WAYWQWQTSA-N Diethyl maleate Chemical compound CCOC(=O)\C=C/C(=O)OCC IEPRKVQEAMIZSS-WAYWQWQTSA-N 0.000 description 1
- JIGUQPWFLRLWPJ-UHFFFAOYSA-N Ethyl acrylate Chemical compound CCOC(=O)C=C JIGUQPWFLRLWPJ-UHFFFAOYSA-N 0.000 description 1
- VVQNEPGJFQJSBK-UHFFFAOYSA-N Methyl methacrylate Chemical compound COC(=O)C(C)=C VVQNEPGJFQJSBK-UHFFFAOYSA-N 0.000 description 1
- 229920001007 Nylon 4 Polymers 0.000 description 1
- 229920000393 Nylon 6/6T Polymers 0.000 description 1
- 241001482237 Pica Species 0.000 description 1
- 101000870345 Vasconcellea cundinamarcensis Cysteine proteinase 1 Proteins 0.000 description 1
- 239000004957 Zytel Substances 0.000 description 1
- 239000000654 additive Substances 0.000 description 1
- 230000002411 adverse Effects 0.000 description 1
- 150000001298 alcohols Chemical class 0.000 description 1
- XAGFODPZIPBFFR-UHFFFAOYSA-N aluminium Chemical compound [Al] XAGFODPZIPBFFR-UHFFFAOYSA-N 0.000 description 1
- 229910052782 aluminium Inorganic materials 0.000 description 1
- RWCCWEUUXYIKHB-UHFFFAOYSA-N benzophenone Chemical compound C=1C=CC=CC=1C(=O)C1=CC=CC=C1 RWCCWEUUXYIKHB-UHFFFAOYSA-N 0.000 description 1
- 239000012965 benzophenone Substances 0.000 description 1
- 229910000019 calcium carbonate Inorganic materials 0.000 description 1
- 239000006229 carbon black Substances 0.000 description 1
- 125000002915 carbonyl group Chemical group [*:2]C([*:1])=O 0.000 description 1
- 238000006243 chemical reaction Methods 0.000 description 1
- 229920006037 cross link polymer Polymers 0.000 description 1
- 239000003431 cross linking reagent Substances 0.000 description 1
- LDCRTTXIJACKKU-ONEGZZNKSA-N dimethyl fumarate Chemical compound COC(=O)\C=C\C(=O)OC LDCRTTXIJACKKU-ONEGZZNKSA-N 0.000 description 1
- 229960004419 dimethyl fumarate Drugs 0.000 description 1
- 238000010894 electron beam technology Methods 0.000 description 1
- 239000003995 emulsifying agent Substances 0.000 description 1
- 150000002170 ethers Chemical class 0.000 description 1
- 229920005648 ethylene methacrylic acid copolymer Polymers 0.000 description 1
- 229940117927 ethylene oxide Drugs 0.000 description 1
- 238000002474 experimental method Methods 0.000 description 1
- 239000001530 fumaric acid Substances 0.000 description 1
- 239000008187 granular material Substances 0.000 description 1
- 150000008282 halocarbons Chemical class 0.000 description 1
- 229920001903 high density polyethylene Polymers 0.000 description 1
- 239000004700 high-density polyethylene Substances 0.000 description 1
- 238000011065 in-situ storage Methods 0.000 description 1
- 238000010348 incorporation Methods 0.000 description 1
- 239000004434 industrial solvent Substances 0.000 description 1
- 150000002576 ketones Chemical class 0.000 description 1
- FPYJFEHAWHCUMM-UHFFFAOYSA-N maleic anhydride Chemical compound O=C1OC(=O)C=C1 FPYJFEHAWHCUMM-UHFFFAOYSA-N 0.000 description 1
- 239000011159 matrix material Substances 0.000 description 1
- 229920005623 miscible polymer blend Polymers 0.000 description 1
- 125000004108 n-butyl group Chemical group [H]C([H])([H])C([H])([H])C([H])([H])C([H])([H])* 0.000 description 1
- 150000002924 oxiranes Chemical class 0.000 description 1
- 238000005453 pelletization Methods 0.000 description 1
- PNJWIWWMYCMZRO-UHFFFAOYSA-N pent‐4‐en‐2‐one Natural products CC(=O)CC=C PNJWIWWMYCMZRO-UHFFFAOYSA-N 0.000 description 1
- 125000000864 peroxy group Chemical group O(O*)* 0.000 description 1
- 239000000049 pigment Substances 0.000 description 1
- 229920000232 polyglycine polymer Polymers 0.000 description 1
- 229920000098 polyolefin Polymers 0.000 description 1
- 230000002028 premature Effects 0.000 description 1
- 230000009467 reduction Effects 0.000 description 1
- 230000000630 rising effect Effects 0.000 description 1
- 238000010561 standard procedure Methods 0.000 description 1
- 239000000454 talc Substances 0.000 description 1
- 229910052623 talc Inorganic materials 0.000 description 1
- KKEYFWRCBNTPAC-UHFFFAOYSA-L terephthalate(2-) Chemical compound [O-]C(=O)C1=CC=C(C([O-])=O)C=C1 KKEYFWRCBNTPAC-UHFFFAOYSA-L 0.000 description 1
- 229920006029 tetra-polymer Polymers 0.000 description 1
- VZCYOOQTPOCHFL-UHFFFAOYSA-N trans-butenedioic acid Natural products OC(=O)C=CC(O)=O VZCYOOQTPOCHFL-UHFFFAOYSA-N 0.000 description 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J3/00—Processes of treating or compounding macromolecular substances
- C08J3/20—Compounding polymers with additives, e.g. colouring
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L101/00—Compositions of unspecified macromolecular compounds
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J3/00—Processes of treating or compounding macromolecular substances
- C08J3/02—Making solutions, dispersions, lattices or gels by other methods than by solution, emulsion or suspension polymerisation techniques
- C08J3/09—Making solutions, dispersions, lattices or gels by other methods than by solution, emulsion or suspension polymerisation techniques in organic liquids
- C08J3/11—Making solutions, dispersions, lattices or gels by other methods than by solution, emulsion or suspension polymerisation techniques in organic liquids from solid polymers
Landscapes
- Chemical & Material Sciences (AREA)
- Health & Medical Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Organic Chemistry (AREA)
- Dispersion Chemistry (AREA)
- Processes Of Treating Macromolecular Substances (AREA)
- Compositions Of Macromolecular Compounds (AREA)
- Manufacture Of Macromolecular Shaped Articles (AREA)
Applications Claiming Priority (2)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| US82957386A | 1986-02-14 | 1986-02-14 | |
| US829573 | 1986-02-14 |
Publications (2)
| Publication Number | Publication Date |
|---|---|
| AU6869187A AU6869187A (en) | 1987-08-20 |
| AU600255B2 true AU600255B2 (en) | 1990-08-09 |
Family
ID=25254895
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| AU68691/87A Ceased AU600255B2 (en) | 1986-02-14 | 1987-02-11 | Novel polymer barrier blends |
Country Status (12)
| Country | Link |
|---|---|
| EP (1) | EP0238197A3 (en, 2012) |
| JP (1) | JPS62246934A (en, 2012) |
| KR (1) | KR900003917B1 (en, 2012) |
| CN (1) | CN87101919A (en, 2012) |
| AU (1) | AU600255B2 (en, 2012) |
| BR (1) | BR8700659A (en, 2012) |
| CA (1) | CA1282514C (en, 2012) |
| DK (1) | DK73387A (en, 2012) |
| FI (1) | FI870626A7 (en, 2012) |
| IL (1) | IL81567A (en, 2012) |
| IN (1) | IN166034B (en, 2012) |
| NZ (1) | NZ219273A (en, 2012) |
Families Citing this family (4)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US5147930A (en) * | 1989-11-16 | 1992-09-15 | Rohm And Haas Company | Polymer blends with enhanced properties |
| US5208083A (en) * | 1989-11-16 | 1993-05-04 | Rohm And Haas Company | Polymer blends with enhanced properties |
| DE4031389C2 (de) * | 1990-10-04 | 1993-12-09 | Mudder H Europlast | Verwendung einer Polymermasse aus Polyester und einem Ethylen-Methacrylsäure-Copolymerisat |
| US5188784A (en) * | 1990-10-16 | 1993-02-23 | The Royal Institution For The Advancement Of Learning (Mcgill University) | Process for laminar pollymer extrusion |
Citations (3)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| AU555779B2 (en) * | 1982-01-29 | 1986-10-09 | Toyo Seikan Kaisha Ltd. | Ethylene/sadonified vinyl ester copolymer blend with polyamide |
| AU569104B2 (en) * | 1983-08-22 | 1988-01-21 | E.I. Du Pont De Nemours And Company | Ethylene - cooh ionomer composition |
| AU576637B2 (en) * | 1985-05-02 | 1988-09-01 | Rensselaer Polytechnic Institute | Two polymer matrix by evaporation of organic polymer solution |
Family Cites Families (5)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| JPS5231898B2 (en, 2012) * | 1972-05-10 | 1977-08-18 | ||
| US4410482A (en) * | 1979-03-06 | 1983-10-18 | E. I. Du Pont De Nemours & Co. | Process for making laminar articles of polyolefin and a condensation polymer |
| GB8320270D0 (en) * | 1983-07-27 | 1983-09-01 | Raychem Ltd | Polymer composition |
| JPS6096631A (ja) * | 1983-10-31 | 1985-05-30 | Toyoda Gosei Co Ltd | ポリアミド−ゴムブレンド組成物 |
| DE3443959A1 (de) * | 1984-12-01 | 1986-06-12 | Basf Ag, 6700 Ludwigshafen | Thermoplastische formmassen |
-
1987
- 1987-02-10 IN IN115/CAL/87A patent/IN166034B/en unknown
- 1987-02-10 CA CA000529367A patent/CA1282514C/en not_active Expired - Lifetime
- 1987-02-11 AU AU68691/87A patent/AU600255B2/en not_active Ceased
- 1987-02-12 BR BR8700659A patent/BR8700659A/pt not_active Application Discontinuation
- 1987-02-13 EP EP87301253A patent/EP0238197A3/en not_active Withdrawn
- 1987-02-13 IL IL81567A patent/IL81567A/xx unknown
- 1987-02-13 DK DK073387A patent/DK73387A/da not_active Application Discontinuation
- 1987-02-13 FI FI870626A patent/FI870626A7/fi not_active Application Discontinuation
- 1987-02-13 NZ NZ219273A patent/NZ219273A/xx unknown
- 1987-02-14 CN CN198787101919A patent/CN87101919A/zh active Pending
- 1987-02-14 JP JP62030720A patent/JPS62246934A/ja active Pending
- 1987-02-14 KR KR1019870001229A patent/KR900003917B1/ko not_active Expired
Patent Citations (3)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| AU555779B2 (en) * | 1982-01-29 | 1986-10-09 | Toyo Seikan Kaisha Ltd. | Ethylene/sadonified vinyl ester copolymer blend with polyamide |
| AU569104B2 (en) * | 1983-08-22 | 1988-01-21 | E.I. Du Pont De Nemours And Company | Ethylene - cooh ionomer composition |
| AU576637B2 (en) * | 1985-05-02 | 1988-09-01 | Rensselaer Polytechnic Institute | Two polymer matrix by evaporation of organic polymer solution |
Also Published As
| Publication number | Publication date |
|---|---|
| DK73387D0 (da) | 1987-02-13 |
| DK73387A (da) | 1987-08-15 |
| IL81567A0 (en) | 1987-09-16 |
| IN166034B (en, 2012) | 1990-03-03 |
| EP0238197A2 (en) | 1987-09-23 |
| CA1282514C (en) | 1991-04-02 |
| NZ219273A (en) | 1989-06-28 |
| KR870007964A (ko) | 1987-09-23 |
| FI870626L (fi) | 1987-08-15 |
| EP0238197A3 (en) | 1990-03-14 |
| AU6869187A (en) | 1987-08-20 |
| BR8700659A (pt) | 1987-12-15 |
| FI870626A0 (fi) | 1987-02-13 |
| FI870626A7 (fi) | 1987-08-15 |
| JPS62246934A (ja) | 1987-10-28 |
| KR900003917B1 (ko) | 1990-06-04 |
| CN87101919A (zh) | 1987-09-02 |
| IL81567A (en) | 1990-09-17 |
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