WO2020060887A3 - Réseau organométallique inspiré d'une enzyme - Google Patents

Réseau organométallique inspiré d'une enzyme Download PDF

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Publication number
WO2020060887A3
WO2020060887A3 PCT/US2019/051211 US2019051211W WO2020060887A3 WO 2020060887 A3 WO2020060887 A3 WO 2020060887A3 US 2019051211 W US2019051211 W US 2019051211W WO 2020060887 A3 WO2020060887 A3 WO 2020060887A3
Authority
WO
WIPO (PCT)
Prior art keywords
metal
organic framework
inspired
enzyme
mof
Prior art date
Application number
PCT/US2019/051211
Other languages
English (en)
Other versions
WO2020060887A2 (fr
WO2020060887A9 (fr
Inventor
Omar M. Yaghi
Gabor A. Somorjai
Jayeon BAEK
Bunyarat RUNGTAWEEVORANIT
Original Assignee
The Regents Of The University Of California
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by The Regents Of The University Of California filed Critical The Regents Of The University Of California
Publication of WO2020060887A2 publication Critical patent/WO2020060887A2/fr
Publication of WO2020060887A3 publication Critical patent/WO2020060887A3/fr
Publication of WO2020060887A9 publication Critical patent/WO2020060887A9/fr

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Classifications

    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C29/00—Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring
    • C07C29/48—Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring by oxidation reactions with formation of hydroxy groups
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
    • B01J31/1691—Coordination polymers, e.g. metal-organic frameworks [MOF]
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
    • B01J31/18—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes containing nitrogen, phosphorus, arsenic or antimony as complexing atoms, e.g. in pyridine ligands, or in resonance therewith, e.g. in isocyanide ligands C=N-R or as complexed central atoms
    • B01J31/1805—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes containing nitrogen, phosphorus, arsenic or antimony as complexing atoms, e.g. in pyridine ligands, or in resonance therewith, e.g. in isocyanide ligands C=N-R or as complexed central atoms the ligands containing nitrogen
    • B01J31/181—Cyclic ligands, including e.g. non-condensed polycyclic ligands, comprising at least one complexing nitrogen atom as ring member, e.g. pyridine
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
    • B01J31/22—Organic complexes
    • B01J31/2204—Organic complexes the ligands containing oxygen or sulfur as complexing atoms
    • B01J31/2208—Oxygen, e.g. acetylacetonates
    • B01J31/2226—Anionic ligands, i.e. the overall ligand carries at least one formal negative charge
    • B01J31/223—At least two oxygen atoms present in one at least bidentate or bridging ligand
    • B01J31/2239—Bridging ligands, e.g. OAc in Cr2(OAc)4, Pt4(OAc)8 or dicarboxylate ligands
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2531/00—Additional information regarding catalytic systems classified in B01J31/00
    • B01J2531/02—Compositional aspects of complexes used, e.g. polynuclearity
    • B01J2531/0213—Complexes without C-metal linkages
    • B01J2531/0216—Bi- or polynuclear complexes, i.e. comprising two or more metal coordination centres, without metal-metal bonds, e.g. Cp(Lx)Zr-imidazole-Zr(Lx)Cp
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2531/00—Additional information regarding catalytic systems classified in B01J31/00
    • B01J2531/10—Complexes comprising metals of Group I (IA or IB) as the central metal
    • B01J2531/16—Copper
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2531/00—Additional information regarding catalytic systems classified in B01J31/00
    • B01J2531/40—Complexes comprising metals of Group IV (IVA or IVB) as the central metal
    • B01J2531/48—Zirconium
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/003—Catalysts comprising hydrides, coordination complexes or organic compounds containing enzymes
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P20/00—Technologies relating to chemical industry
    • Y02P20/50—Improvements relating to the production of bulk chemicals
    • Y02P20/52—Improvements relating to the production of bulk chemicals using catalysts, e.g. selective catalysts

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Inorganic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Catalysts (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Abstract

Des catalyseurs à réseau de coordination organométallique (MOF) comprennent des ligands à base d'imidazole métalatés qui forment un complexe métal-oxygène réactif dans le MOF.
PCT/US2019/051211 2018-09-19 2019-09-16 Réseau organométallique inspiré d'une enzyme WO2020060887A2 (fr)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
US201862733591P 2018-09-19 2018-09-19
US62/733,591 2018-09-19

Publications (3)

Publication Number Publication Date
WO2020060887A2 WO2020060887A2 (fr) 2020-03-26
WO2020060887A3 true WO2020060887A3 (fr) 2020-04-23
WO2020060887A9 WO2020060887A9 (fr) 2020-05-22

Family

ID=69888684

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/US2019/051211 WO2020060887A2 (fr) 2018-09-19 2019-09-16 Réseau organométallique inspiré d'une enzyme

Country Status (1)

Country Link
WO (1) WO2020060887A2 (fr)

Families Citing this family (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN112553186B (zh) * 2020-12-25 2023-08-18 华南理工大学 一种铜基金属有机框架材料固定化漆酶及其制备方法和应用
CN113262650B (zh) * 2021-04-23 2022-09-30 中国工程物理研究院材料研究所 用于氢同位素净化的二维mof膜及其制备方法和应用
CN114231518A (zh) * 2021-12-17 2022-03-25 浙江工业大学 一种固定化碳酸酐酶及其在制备二氧化碳吸收剂中的应用
CN114984242A (zh) * 2022-05-17 2022-09-02 刘天龙 通过泛素-蛋白酶体途径与自噬双抑制治疗肿瘤的方法
CN116139936B (zh) * 2023-04-17 2023-07-04 四川大学 一种碳酸酐酶人造酶及其制备方法和应用

Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20120259117A1 (en) * 2009-06-19 2012-10-11 The Regents Of The University Of California Organo-metallic frameworks and methods of making same
US20130023403A1 (en) * 2011-03-03 2013-01-24 University Of South Florida Metal organic materials as biomimetic enzymes
WO2017066328A1 (fr) * 2015-10-12 2017-04-20 The University Of Chicago Stabilisation de catalyseurs métalliques actifs au niveau de nœuds de structure organométallique pour des transformations organiques hautement efficaces
US20170173572A1 (en) * 2014-03-28 2017-06-22 The University Of Chicago Chiral ligand-based metal-organic frameworks for broad-scope asymmetric catalysis

Patent Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20120259117A1 (en) * 2009-06-19 2012-10-11 The Regents Of The University Of California Organo-metallic frameworks and methods of making same
US20130023403A1 (en) * 2011-03-03 2013-01-24 University Of South Florida Metal organic materials as biomimetic enzymes
US20170173572A1 (en) * 2014-03-28 2017-06-22 The University Of Chicago Chiral ligand-based metal-organic frameworks for broad-scope asymmetric catalysis
WO2017066328A1 (fr) * 2015-10-12 2017-04-20 The University Of Chicago Stabilisation de catalyseurs métalliques actifs au niveau de nœuds de structure organométallique pour des transformations organiques hautement efficaces

Also Published As

Publication number Publication date
WO2020060887A2 (fr) 2020-03-26
WO2020060887A9 (fr) 2020-05-22

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