US2079803A - Soluble oil - Google Patents

Soluble oil Download PDF

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US2079803A
US2079803A US740454A US74045434A US2079803A US 2079803 A US2079803 A US 2079803A US 740454 A US740454 A US 740454A US 74045434 A US74045434 A US 74045434A US 2079803 A US2079803 A US 2079803A
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oil
soluble
acid
acids
oils
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Expired - Lifetime
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US740454A
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John B Holtzclaw
Winning Carl
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Standard Oil Development Co
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Standard Oil Development Co
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Priority claimed from US725083A external-priority patent/US2049043A/en
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Priority to US740454A priority Critical patent/US2079803A/en
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Classifications

    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06MTREATMENT, NOT PROVIDED FOR ELSEWHERE IN CLASS D06, OF FIBRES, THREADS, YARNS, FABRICS, FEATHERS OR FIBROUS GOODS MADE FROM SUCH MATERIALS
    • D06M7/00Treating fibres, threads, yarns, fabrics, or fibrous goods made of other substances with subsequent freeing of the treated goods from the treating medium, e.g. swelling, e.g. polyolefins
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2201/00Inorganic compounds or elements as ingredients in lubricant compositions
    • C10M2201/02Water
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2203/00Organic non-macromolecular hydrocarbon compounds and hydrocarbon fractions as ingredients in lubricant compositions
    • C10M2203/10Petroleum or coal fractions, e.g. tars, solvents, bitumen
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2205/00Organic macromolecular hydrocarbon compounds or fractions, whether or not modified by oxidation as ingredients in lubricant compositions
    • C10M2205/14Synthetic waxes, e.g. polythene waxes
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2205/00Organic macromolecular hydrocarbon compounds or fractions, whether or not modified by oxidation as ingredients in lubricant compositions
    • C10M2205/16Paraffin waxes; Petrolatum, e.g. slack wax
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2205/00Organic macromolecular hydrocarbon compounds or fractions, whether or not modified by oxidation as ingredients in lubricant compositions
    • C10M2205/17Fisher Tropsch reaction products
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2205/00Organic macromolecular hydrocarbon compounds or fractions, whether or not modified by oxidation as ingredients in lubricant compositions
    • C10M2205/17Fisher Tropsch reaction products
    • C10M2205/173Fisher Tropsch reaction products used as base material
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2205/00Organic macromolecular hydrocarbon compounds or fractions, whether or not modified by oxidation as ingredients in lubricant compositions
    • C10M2205/18Natural waxes, e.g. ceresin, ozocerite, bees wax, carnauba; Degras
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2207/00Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
    • C10M2207/02Hydroxy compounds
    • C10M2207/021Hydroxy compounds having hydroxy groups bound to acyclic or cycloaliphatic carbon atoms
    • C10M2207/022Hydroxy compounds having hydroxy groups bound to acyclic or cycloaliphatic carbon atoms containing at least two hydroxy groups
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2207/00Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
    • C10M2207/40Fatty vegetable or animal oils
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2207/00Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
    • C10M2207/40Fatty vegetable or animal oils
    • C10M2207/404Fatty vegetable or animal oils obtained from genetically modified species
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2215/00Organic non-macromolecular compounds containing nitrogen as ingredients in lubricant Compositions
    • C10M2215/02Amines, e.g. polyalkylene polyamines; Quaternary amines
    • C10M2215/04Amines, e.g. polyalkylene polyamines; Quaternary amines having amino groups bound to acyclic or cycloaliphatic carbon atoms
    • C10M2215/042Amines, e.g. polyalkylene polyamines; Quaternary amines having amino groups bound to acyclic or cycloaliphatic carbon atoms containing hydroxy groups; Alkoxylated derivatives thereof
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2219/00Organic non-macromolecular compounds containing sulfur, selenium or tellurium as ingredients in lubricant compositions
    • C10M2219/04Organic non-macromolecular compounds containing sulfur, selenium or tellurium as ingredients in lubricant compositions containing sulfur-to-oxygen bonds, i.e. sulfones, sulfoxides
    • C10M2219/044Sulfonic acids, Derivatives thereof, e.g. neutral salts
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10NINDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
    • C10N2030/00Specified physical or chemical properties which is improved by the additive characterising the lubricating composition, e.g. multifunctional additives
    • C10N2030/12Inhibition of corrosion, e.g. anti-rust agents or anti-corrosives
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10NINDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
    • C10N2040/00Specified use or application for which the lubricating composition is intended
    • C10N2040/20Metal working
    • C10N2040/22Metal working with essential removal of material, e.g. cutting, grinding or drilling
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10NINDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
    • C10N2040/00Specified use or application for which the lubricating composition is intended
    • C10N2040/46Textile oils
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10NINDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
    • C10N2050/00Form in which the lubricant is applied to the material being lubricated
    • C10N2050/01Emulsions, colloids, or micelles
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06MTREATMENT, NOT PROVIDED FOR ELSEWHERE IN CLASS D06, OF FIBRES, THREADS, YARNS, FABRICS, FEATHERS OR FIBROUS GOODS MADE FROM SUCH MATERIALS
    • D06M2200/00Functionality of the treatment composition and/or properties imparted to the textile material
    • D06M2200/40Reduced friction resistance, lubricant properties; Sizing compositions

Definitions

  • Example 3 About .03% of water was thoroughly mixed into the soluble oil prepared in Example 2. The product was uniform and showed no tendency to gel.
  • a non-gelling emulsifiable textile oil composition consisting essentially of a mineral ofl, about 7% of oil-soluble sulfonate emulsifier derived from petroleum hydrocarbons and about 1.5% of triethanolamine oleate.

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  • Engineering & Computer Science (AREA)
  • Textile Engineering (AREA)
  • Colloid Chemistry (AREA)

Description

Patented May 11, 1937 1 SOLUBLE on.
John B. Holtzclaw, Roselle, and Carl Winning,
Elizabeth, N. J., assignors to Standard Oil De-- velopment- Company, a corporation of Delaware No Drawing. Application August 18, 1934,
' Serial No. 140,454
9 Claims. (Cl. 8'3-9) This invention relates to a novel soluble oil and methods of preparing and using same.
Broadly, the invention .consists in preparing a soluble oil by blending together an oil, oil-soluble sulfonates derived from petroleum hydrocarbons, alcohol amines and carboxylic acids.
-In co-pending application Serial No. 725,086, filed May 11, 1934 by Karl T. Steik and Stewart C. Fulton, there is disclosed and claimed broadly, an emulsifying agent comprising a major proportion of oil-soluble sulfonates and a minor proportion of alcohol amine soap. That application also contains specific claims on an emulsifying agent comprising a major proportion of oil-soluble sulfonate and a minor proportion of alcohol amine sulfonate.
One object of the present invention is to claim one of the other species, a composition comprise ing an alcohol amine soap of a carboxylic acid,
disclosed in the co-pending application.
It is a further object of the present invention to disclose and claim a method of stabilizing soluble oils or emulsions prepared by use of either of the species referred to, namely, the combination of oil-soluble sulfonates with either an alcohol amine sulfonate or ,with an alcohol amine soap of a carboxylic acid. According to the present invention, this stabilization is accomplished by the use of a, slight excess of the alcohol amine over the stoichiometric amount required to combine with the carboxylic or sulfonic acid used. I
It is known in the prior art that soluble oils, capable of forming emulsions when subsequently mixed with water, can be formed by dissolving in a suitable oil, such as a mineral lubricating oil or a'mineral white oil, the oil-soluble alkali soaps of sulfonic acids derived from petroleum hydrocarbons, as for instance the so-called mahogany soaps, obtained as a result of 'treating a mineral lubricating oil fraction with strong sulfuric acid for the preparation of white oil. However, in preparing soluble oils of that type, a relatively large amount ofoil-soluble sulfonates must be used and, according to the presentinvention, this amount may be greatly reduced by substituting inpart therefona small amount of an alcohol amine soap of a carboxylic acid, or a mixture of an alcohol amine and a carboxylic acid. The oil-soluble 'sulfonates may be'obtained or purified by any of the known methods-but it is particularly preferred, for the present invention, to use oil-soluble sulfonates prepared according to the method described and claimed in co-pending application Serial No. 626,233 filed July 29, 1932 by Hyym E. Buc', now Patent 1,981,799 which comprises isolating oil-soluble sulfonates directly from the alcoholic aqueous solution (resulting from the extraction of the acidtreated oil with alcohol) by agitating with alkali carbonates, drawing off and filtering the upper layer and evaporating the filtrate to dryness. Instead of, or in addition to, the pure or impure mahogany soap, any variety of related sulfonates, which are reasonably soluble in the oil base, may be used, such as sulfonated lard oil, Turkey red oil, sulfated higher fatty alcohols, etc.
Triethanolamine is the preferred alcohol amine as it is available commercially. The product on the market usually consists of a mixture of mono-, di-, and triethanolamine, although pure triethanolamine may be used if desired. Also, other. alcohol amines and their mixtures maybe used; for instance, propanolamines, etc. One feature of the present invention is the use of a slight excess of alcohol amine over the amount required to neutralize or combine with the carboxylic acid. This excess amine produces more stable emulsions.
0f the carboxylic acids, oleic is generally the most satisfactory, and for a high grade product, the better grades of oleic acid are preferred. Other. fatty acids of similar molecular weight (palmitic, lauric, stearic, behenic, etc., linoleic, linolenic, etc.) may be used, also naphthenic acids, rosin acids, or acids formed by the oxidation of oils and waxes, but, in general, it is preferred to use acids having-morethan 6 carbon atoms and, better still, more than 12 carbon atoms if a single acid is used. Low melting point acids are preferred when fluid products are desired. Highly unsaturated acids are tobe avoided where an extra high resistance to oxidation is desired. Mixed acids may also be used, such as those obtained by the oxidation of high molecular weight oils and waxes, particularly parafiin wax. These fatty acids may be used in the free stage or chemically combined with the alcohol amines.
The oil to be used as a base in preparing the soluble oils, according to the present invention, may be a mineral oil or fatty oil, such as vegetable, animal or-fish oil of proper viscosity (generally between that of a very light spindle oiland a heavy lubricating oil). The mineral oil may be either lightly refined as by distillation, solvent extraction, clay treating or treatment with dilute acid, or other chemical treating agent, or it may be a highly refined or so-called' white oil, such as the products on the market known as Nujol and Marco]. These oils may be used as such or toit is not intended that the invention should be limited to the above proportions.
For the sake of illustration, a number of examples of the invention are given herewith:
Example 1 Percent 7.0 1.5 Balance Oil-soluble sulfonate 'Ih'iethanolamineoleate on This soluble oil was found to have an emulsifying power equivalent to that of a similar oil containing 14% of oil-soluble sulfonate, but containing no triethanolamine oleate.
Example 2 Oil-soluble sulfonate.
Triethanolamine oleate 1.5 Excess (free) triethanolamine 0.2 Oil (mineral white oil called Marcol) Balance This soluble oil was found to produce emulsions which were even more stable than those produced in Example 1.
Example 3 About .03% of water was thoroughly mixed into the soluble oil prepared in Example 2. The product was uniform and showed no tendency to gel.
Example 4 Percent Sulfonated lard oil 20 Triethanolamine oleate 2 Oil 7 Balance 100 Soluble oils prepared according to this invention may be used for any known uses, such as wool oils or other textile oils, for making cutting oils and as a stock solution for preparing emulsions by dilution or addition of water.
It is not intended that the. invention be limited by any of theexamples given, nor by any thecries suggested for the operation of the invention, but only by the appended claims in which it is Percent intended to claim all novelty inherent in the invention as broadly as the prior art permits.
We claim:
1. A. non-gelling emulsifiable textile oil composition consisting of at least of a mineral oil, an oil soluble sulfonate emulsifier, a lower aliphatic alcohol amine having less than 7 carbon atoms, and a carboxylic acid having more than 6 carbon atoms. Q v
2. Composition according to claim 1 in which the amine is triethanolamine and the acid is oleic acid.
3. Composition according to claim 1 in which the acid is a fatty acid having more than 12 carbon atoms. I
'4. Composition according to claim 1 in which the amine ispresent in quantity slightly more than. sufficient to combine with the carboxylic acid.
5. A non-gelling emulsifiable textile oil composition consisting of at least 80% of a mineral oil, an oil-soluble sulfonate emulsifier, a fatty acid having more than 6 carbon atoms and triethanclamine, the amount of the latter being slightly in excess of the stoichiometric amount required to combine with the fatty acid.
6..A' non-gelling emulsifiable textile oil composition consisting of to of a mineral oil,
5 to 10% of the sodium soaps of oil-soluble sulfonic acids derived from treatment of' petroleum lubricating oil with strong sulfuric acid, 0.1 to 2% of a lower aliphatic alcohol amine having less than 7 carbon atoms and 0.1 to 5% of a fatty acid having more than 6 carbon atoms, the amount of the alcohol amine being at least the stoichiometric amount required to combine with the fatty acid.
7. A non-gelling emulsifiable textile oil composition consisting essentially of a mineral ofl, about 7% of oil-soluble sulfonate emulsifier derived from petroleum hydrocarbons and about 1.5% of triethanolamine oleate.
8. A non-gelling emulsifiable textile oil composition consisting essentially of a mineral oil, about 7% of oil-soluble sulfonate emulsifier derived from petroleum hydrocarbons, about 1.5% of triethanolamine oleate and about 0.2% of free trlethanolamine. v
9. An emulsion comprising a major proportion of water and a minor proportion of a non-gelling emulsifiable textile oil composition consisting of at least 80% of a mineral oil, oil-soluble sulfonates derived'from petroleum hydrocarbons and present in an amount insumcient to maintain a stable emulsion if used as sole emulsifier, a small amount of a carboxylic acid having more than 6 carbon atoms and a lower aliphatic alcohol amine having less than seven carbon atoms.
JOHN B. HOLTZCLAW. CARL WINNING.
US740454A 1934-05-11 1934-08-18 Soluble oil Expired - Lifetime US2079803A (en)

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US740454A US2079803A (en) 1934-05-11 1934-08-18 Soluble oil

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Cited By (12)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2422075A (en) * 1944-08-31 1947-06-10 Texas Co Stabilized lubricating emulsions
US2431010A (en) * 1941-07-19 1947-11-18 Standard Oil Dev Co Soluble cutting oil
US2474325A (en) * 1943-04-07 1949-06-28 Jr Thomas T Rodgers Aqueous lubricant
US2565403A (en) * 1948-04-27 1951-08-21 Standard Oil Dev Co Textile oils
US2575399A (en) * 1948-10-07 1951-11-20 Celanese Corp Textile lubricant
DE886881C (en) * 1949-09-04 1953-08-17 Bobingen Ag Fuer Textil Faser Sizing agents for the textile industry
US2695272A (en) * 1952-05-21 1954-11-23 Standard Oil Dev Co Soluble metalworking oil
US2807864A (en) * 1954-06-24 1957-10-01 Eastman Kodak Co Composition and process for treating yarn
US2999064A (en) * 1959-02-11 1961-09-05 Master Chemical Corp Stable aqueous cutting fluid
US3071544A (en) * 1959-08-14 1963-01-01 Sun Oil Co Emulsifiable mixtures of mineral oil and esters
US3311561A (en) * 1964-12-14 1967-03-28 Sun Oil Co Water-in-oil emulsions
US3442805A (en) * 1966-08-31 1969-05-06 Swift & Co Lubricating composition

Cited By (12)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2431010A (en) * 1941-07-19 1947-11-18 Standard Oil Dev Co Soluble cutting oil
US2474325A (en) * 1943-04-07 1949-06-28 Jr Thomas T Rodgers Aqueous lubricant
US2422075A (en) * 1944-08-31 1947-06-10 Texas Co Stabilized lubricating emulsions
US2565403A (en) * 1948-04-27 1951-08-21 Standard Oil Dev Co Textile oils
US2575399A (en) * 1948-10-07 1951-11-20 Celanese Corp Textile lubricant
DE886881C (en) * 1949-09-04 1953-08-17 Bobingen Ag Fuer Textil Faser Sizing agents for the textile industry
US2695272A (en) * 1952-05-21 1954-11-23 Standard Oil Dev Co Soluble metalworking oil
US2807864A (en) * 1954-06-24 1957-10-01 Eastman Kodak Co Composition and process for treating yarn
US2999064A (en) * 1959-02-11 1961-09-05 Master Chemical Corp Stable aqueous cutting fluid
US3071544A (en) * 1959-08-14 1963-01-01 Sun Oil Co Emulsifiable mixtures of mineral oil and esters
US3311561A (en) * 1964-12-14 1967-03-28 Sun Oil Co Water-in-oil emulsions
US3442805A (en) * 1966-08-31 1969-05-06 Swift & Co Lubricating composition

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