TW581751B - Compound for organic EL (electroluminescent) device and organic EL device using it - Google Patents

Compound for organic EL (electroluminescent) device and organic EL device using it Download PDF

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TW581751B
TW581751B TW091108294A TW91108294A TW581751B TW 581751 B TW581751 B TW 581751B TW 091108294 A TW091108294 A TW 091108294A TW 91108294 A TW91108294 A TW 91108294A TW 581751 B TW581751 B TW 581751B
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biphenylyl
naphthyl
tolyl
hhh
group
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TW091108294A
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Tetsuji Fujita
Sumiko Kitagawa
Tetsuji Inoue
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Tdk Corp
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Description

581751 A7 B7 經濟部智惡財產局員工消費合作钍印賢 五、發明説明（ί 【發明之技術領域】 本發明係有關有機電致（電場發光）發光元件，詳細 言之，即有關對由有機化合物所構成之薄膜上附加電場使 其放出亮光之元件所使用之化合物。 【先前技術】 有機電致發光元件，爲一具有將含有螢光性有機化合 物之薄膜，挾夾於電子注入電極與正孔注入電極之構成， 且於前記薄膜上注入電子與正孔後所產生之再鍵結而生成 激發子（exiton)，並利用此激發子鈍化之際所釋放之光（ 螢光、磷光）進行發光之元件。 有機電致發光元件之特徵，係可於1 0 V左右之電壓 下發出1 0 0至1 0 0 0 0 c d /m2之高亮度之面亮光， 又，選擇螢光物質之種類後亦可得到藍色至紅色之發光。 有機電致發光元件可得到任意發光色之方法例如摻雜 法，例如蒽結晶中摻雜有微量1 ，2，3，4 _四氫蒽時 ，可使發光色由藍色變爲綠色之報告（Jpn. J. Appl. Phys.， 10,527( 197 1 ))。又，於具有層合構造之有機薄膜電致發 光元件中，於具有發光機能之主體物質（host material)中 ，微量混入可配合該發光反應而發出與主體物質不同發光 之螢光色素作爲摻雜劑而形成發光層，而形成可由綠色變 化至橙〜紅色發光色之報告（特開昭6 3 — 2 6 4 6 9 2 號）〇 有關黃〜紅色長波長發光中，作爲發光材料或摻雜劑 (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -4- 581751 A7 B7 五、發明説明（j 材料者例如，可進行紅色振盪之雷射色素（ E P〇2 8 1 3 8 1號）、顯示出激態絡合物發光之化合 物（特開平2 - 2 5 5 7 8 8號公報）、驼化合物（特開 平3 - 79 1號公報）、香豆素化合物（特開平3 — 7 9 2號公報）、二胺基伸甲基系化合物（特開平3 - 1 6 2 4 8 1號公報）、噻噸化合物（特開平3 - 177486號公報）、共軛系高分子與墊子輸送性化合 物之混合物（特開平6 - 7 3 3 7 4號公報）、四方系化 合物（Squarylium )(特開平6 - 9 3 2 5 7號公報）、噁 二唑系化合物（特開平6 - 145146號公報）、芘系 化合物（特開平6 - 240246號公報）等。 又，例如熒蒽衍生物具有極高之螢光量子產率等內容 係記載於 J· Am. Chem. Soc 1996，118，2374-2379 頁之內容 中，特開平1 0 — 3 3 0 2 9 5號公報與特開平11一 2 3 3 2 6 1號公報中則記載於各種主體材料中，摻雜由 熒蒽所衍生之二苯駢〔f · f ’ 〕二茚〔1，2，3 - cd:l’ ，2’ ，3 ’一 lm〕驼衍生物衍生物作爲發 光層所得之有機電致發光元件。 其他發光材料例如縮合多環芳香族化合物（特開平5 -32966號公報，特開平5 — 214334號公報） 等。又，摻雜材料例如各種縮合多環芳香族化合物（特開 平5 — 258859號公報）等。 > 但，前述以往之螢光材料中可得到近乎純藍色發光之 例子極少，但欲實現高品位之全彩顯示器時，急需開發出 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） (請先閲讀背面之注意事項再填寫本頁) 、τ 經濟部智慧財產局工消費合作Ti印製 581751 A7 B7 五、發明説明（3 •-種高效率的純藍系螢光材料。 (請先閲讀背面之注意事項再填寫本頁) 【發明之槪要】 本發明係提供一種可得到充分亮度之發光，特別是長 波長下之發光，優良之發色純度，特別是可用於全彩顯示 器之充分發色純度’且該良好發光性能經過長期使用亦具 有優良耐久性之有機電致發光元件用化合物，及有機電致 發光元件爲發明之目的。 上記目的，係依以下內容而達成。 (1 ) 一種有機電致發光元件用化合物，其係具有下 式（1)所示之基本骨架； X π — Y …（1 ) 〔式（1)中’ X爲下目己式（2)所不化合物，其可 爲相同或不同；Y爲單鍵或爲經取代或未取代之芳基、或 由雜環基所形成之連結基，η爲2或3之整數]
Rs R7 經濟部智慈財凌局員工消費合作社印製
X (2) 〔式（2)中’尺：至！^與a至d爲氫、院基、可具 有取代基之芳基、可具有取代基之烯丙基、可具有取代基 之雜環基、胺基、或可具有取代基之芳基胺基之任一者〕 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -6 - 581751 經濟部智总財產局員工消費合作社印製 (11)如（1)至（6)中任〜項之有機電致發光 元件用化合物，其係具有下記式（B)所示基本骨架；
(日） A7 B7 五、發明説明（g
Hi Cl
〔式（3 c)中，Ri至R8與ax至di、Rh至 與a 2至d2爲氫、烷基、可具有取代基之芳基、可具 有取代基之烯丙基、可具有取代基之雜環基、胺基、或可 具有取代基之芳基胺基之任一者，Y爲單鍵、取代或未取 代之芳基、或由雜環所形成之連結基〕。 (1 0)如（1)至（6)中任一項之有機電致發光 元件用化合物，其係具有下記式（A)所示基本骨架； 巳2曱1 眾11斤12
㈧
Rl6 穴 15 〔式（A)中’ Ri至[^與尺"至Ri?爲氫、院基 、取代或未取代之芳基、或雜環基〕。 爲氫、烷基 本紙張尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） (請先閲讀背面之注意事項再填寫本頁)
-9 581751 A7 B7 五、發明説明（} 、取代或未取代之芳基、或雜環基〕。 (1 2 )如（1 )至（6 )中任〜項之有機電致發光 元件用化合物，其係具有下記式（E )所示基本骨架；
(E) 1至R i 8爲氫、烷基 、取代或未取代之芳基、或雜環基〕。 (1 3)如（1)至（6)中任〜項之有機電致發光 元件用化合物，其係具有下記式（Η )所示基本骨架；
‘18 17 (Η) (請先閱讀背面之注意事項再填寫本頁) 經濟部晳慧財產局員工消費合作社印製 〔式（Η)中，Ri至R8與R 、取代或未取代之芳基、或雜環基〕。 (1 4 )如（1 )至（6 )中任〜項之有機電致發光 元件用化合物，其係具有下記式（X )所示基本骨架； 至R 1 8爲氨、院基
12 (X) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -10· 581751 爲氫、烷基 5)如（1)至（6)中任〜項之有機電致發光
(z) A7 B7 五、發明説明（g 〔式（X)中，尺1至尺8與RugR 取代或未取代之芳基、或雜環基〕。 7爲氫、烷基 、取代或未取代之芳基、或雜環基〕。 (16)如（1)至（6)中任〜項之有機電致發光 元件用化合物，其係具有下記式（AAa，）所示基本骨 架； (請先閲讀背面之注意事項再填寫本頁)
經濟部皙慧时產局貨工消费合作社印焚 〔式（AA.A )中 ’ RiMRs、與 Rii 至 r "爲 氫、烷基、可具有取代基之芳基、可具有取代基之烯丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 基之任一者〕。 (1 7)如（1 )至（6 )中任一項之有機電致發光 元件用化合物，其係具有下記式（BBB，）所示基本骨 架； 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -11 - 581751 A7 B7 五、發明説明（g
(BBB’) 8、與Rll至Rl8爲 氫、烷基、可具有取代基之芳基、可具有取代基之烯丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 基之任一者〕。 (18)如（1)至（6)中任一項之有機電致發光 元件用化合物，其係具有下記式（cc：(：，）所示基本骨 架；
(CCC.) (請先閲讀背面之注意事項再填寫本頁) 〔式（CCC’ ）中，Ri至R8、與爲 經濟部智慈財4^8工消費合作钍印製 氫、烷基、可具有取代基之芳基、可具有取代基之烯丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 基之任一者〕。 (19)如（1)至（6)中任一項之有機電致發光 元件用化合物，其係具有下記式（DDD，）所示基本骨 架； 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -12-
581751 A7 __B7 五、發明説明（）〇 (DDD，） 〔式（DDD’ ）中，Ri 至 R8、與 Rii 至 R18 爲 氫、烷基、可具有取代基之芳基、可具有取代基之烯丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 基之任~1者〕° (2 0)如（1 )至（6 )中任一項之有機電致發光 元件用化合物，其係具有下記式（EEE，）所示基本骨 架； (請先閲讀背面之注意事項再填寫本頁)
經濟部智恶財產局S工消費合作社印裝 〔式（EEE )中’ Ri至R8、與Rii至Ri8爲 氣、烷基、可具有取代基之芳基、可具有取代基之烯丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 基之任一者〕。 (21)如（1)至（6)中任一項之有機電致發光 元件用化合物，其係具有下記式（RRR，）所示基本骨 架； 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -13- 581751 經濟部智慈財產局資工消費合作社印製 A7 B7五、發明説明（ (2 5)如（24)之有機電致發光元件，其中，前 記蒽系衍生物係作爲發光層之主體材料。 (26)如（23)至（25)之有機電致發光元件 ，其中，前記有機電致發光元件用化合物係以摻雜劑形式 含有。 (2 7)如（2 3)至（2 6)之有機電致發光元件 ，其中，前記有機電致發光元件用化合物係包含於發光層 中。 (2 8)如（2 3)至（2 5)之有機電致發光元件 ，其中，前記有機電致發光元件用化合物係包含於電子輸 送層中。 (2 9)如（2 3)至（28)之有機電致發光元件 ，其中，前記有機電致發光元件用化合物係包含於正孔注 入輸送層中。 (3 0)如（2 3)至（2 9)之有機電致發光元件 ，其係具有由2種以上發光材料所形成之2種以上發光極 大波長者。 【圖示之簡單說明】 圖1:本發明之有機電致發光元件基本構造之槪略截 面圖。 圖2 :質譜分析圖。 圖3 :紅外線吸收光譜圖。 圖4:NMR光譜圖。 (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -15- 581751 A7 B7 五、發明説明（ 圖5:實施例1之元件的發光光譜圖。 圖6:實施例11之元件的發光光譜圖。 圖7 :實施例1 2之元件的發光光譜圖。 圖8:實施例13之元件的發光光譜圖。 【較佳實施態樣之說明】 本發明有機電致發光元件用化合物，係具有下記式（ 1 )所示之基本骨架； X π — Y 广 1 、 …（1 ) 〔式（1)中’X爲下記式（2)所示化合物，其可 爲相同或不同；Y爲單鍵或爲經取代或未取代之芳基、或 由雜環基所形成之連結基，η爲2或3之整數〕 (請先閲讀背面之注意事項再填寫本頁)
X
Rs R? (2) 經濟部智慧財產局a(工消費合作社印製 〔式（2)中’ 111至1^8與3至d爲氫、烷基、可具 有取代基之芳基、可具有取代基之烯丙基、可具有取代基 之雜環基、胺基、或可具有取代基之芳基胺基之任一者〕 以下，將對上記式（1 )所示化合物作更進一步之描 述 式（1 )中’ X爲上記式（2)所示化合物，各X可 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -16- 581751 A7 B7 五、發明説明（）4 (請先閲讀背面之注意事項再填寫本頁) 爲相同或不同。即，X爲上記式（2 )所示之化合物時， 其可爲相同或不同之化合物，又以相同化合物爲佳。η = 3時’ 3種X可爲各自不同之化合物。 式（2)中，111至1^8與3至a爲氫、烷基、可具有 取代基之芳基、可具有取代基之烯丙基、可具有取代基之 雜環基、胺基、或可具有取代基之芳基胺基之任一者。又 ’較佳者爲甲基、乙基、丙基、苯基、甲苯基、聯苯基、 萘基、硫苯基、吡啶基、吡咯基、苯乙烯基、三苯胺基、 苯胺基中之任一者，其中又以甲基、苯基、甲苯基、聯苯 基、蔡基、二本胺基、苯胺基中之任一者爲更佳。
Ri至R8與a至d，可各自爲相同或不同。又，鄰接 之R 1至R 8與a至d間亦可形成縮合環。 特別是R 7、R 8之部位，因構造上具有高反應活性， 故以具有取代基爲佳。若將R 7、R 8部位以取代基保護時 ’可使化合物得到化學上之安定性，而防止電致發光元件 時材料之劣化情形。特別是R 7、R 8部位中，以至少一方 具有取代基者爲佳，又以兩方皆具有取代基者爲更佳。 經濟部智惡財4局a(工消費合作社印製 R 7、R 8之取代基種類，例如上記所例示之內容，又 以烷基、芳基、烯丙基、雜環等爲佳。 又，R7、R8可因導入取代基種類之不同，而可敏感 地影響發光波長。因此，適當地選擇導入R 7、R 8部位之 取代基時，可控制發光之波長。 表示X數目的η，可爲2或3之整數，較佳者爲n = 2。n = 3時，會使昇華性降低，使得於昇華時產生熱分 本紙張尺度適用中國國家標準（CNS ) A4規格（21〇X297公釐） 581751 A7 B7 五、發明説明（ί8 本發明化合物之較佳例示，例如下述內容所示 (請先閲讀背面之注意事項再填寫本頁) 經濟部智慧財產局Μ工消費合作社印製 本纸張尺度適用中國國家標準（CNS ) Α4規格（210X297公釐） -21 - 經濟部智慈財產局員工消費合作社印製 581751 A7 B7 五、發明説明（30) 其中，又以下記式（A) 、( B ) 、( E ) 、( Η ) 、（X)、（ZW(AAA’）、（BBB’）、（ CCC’ ）、（DDD’ ）、（EEE’ ）、（RRR， )、（s s s ’ ）所示化合物爲佳。
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、1T 線 本紙張尺度適用中國國家標隼（CNS ) A4規格（210X297公釐） -63- 581751 A7 B7 五、發明説明（61 )
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p-biphenylyl (p-聯苯基) H3C o-tolyl (〇·甲苯基） CH3 rrvtolyl (m·甲苯基） -〇"CH3 p-lolyl (>甲 x 基）
L·H \ ± :P E-140 E-141 E-142 E-143 E-144 E-145 E-146 E-147 * E-148 E-149 E-150 E-151 E-152 E-153 E-154 E-155 E-156 E-157 E-158 E-159 E-160 E-161 E-162 E-163 E-164 E-165 E-166 E-167 E-168 E-169 E-170 E-171 E-172 E-173 E-174 Ε·175· E-176 E-177 E-178 E-179 E-180 E-181 E-182 E-183 E-184 E-185 E-186 ' E-187 E-188 E-189 E-190
Ri r2 r3 r4 Rs r7 R8 o-tolyl H H H H H H o-tolyl Ph H H Ph H H o-tolyl H Ph Ph H H H o-tolyl H H H H Ph H o-tolyl H H H H H Ph o-tolyl H H H H 1-naphthyl H o-tolyl H H H H H 1-naphthyl o-tolyl H H H H 2-naphthyl H o-tolyl H H H H H 2-naphthyl o-tolyl H H H H o-biphenylyl H o-tolyl H H H H H o-biphenylyl o-tolyl H H H H m-biphenylyl H o-tolyl H H H H H m-biphenylyl o-toiyi H H H H p-biphenylyl H o-tolyl H H H H H p-biphenylyl o-tolyl H H H H o-tolyl H o-tolyl H H H H H o-toJyl m-tolyl H H H H H H m-tolyl Ph H H Ph H H m-tolyl H Ph Ph H H H m-tolyl H H H H Ph H m-tolyl H H H H H Ph m-tolyl H H H H 1-naphthyl H m-tolyl H H H H H 1-naphthyl m-tolyl H H H H 2-naphlhyl H m-tolyl H H H H H 2-naphthyl m-tolyl H H H H o-biphenylyl H m-tolyl H H H H H o-biphenylyl m-tolyl H H H H m-biphenylyl H m-tolyl H H H H H m-biphenylyl m-tolyl H H H H p-biphenylyl H m-tolyl H H H H H p-biphenylyl m-tolyl H H H H m-tolyl H m-tolyl H H H H H m-tolyl p-tolyl H H H H H H p-tolyl Ph H H Ph H H p-tolyl H Ph • Ph H H H p-tolyl H H H H Ph H p-tolyl H H H H H Ph p-tolyl H H H H 1-naphthyl H p-tolyl H H H H H 1-naphthyl p-tolyl H H H H 2-naphthyl H p-tolyl H H H H H 2-naphthyl p-tolyl H H H H o-biphenylyl H p-tolyl H H H H H o-biphenylyl p-tolyl H H H H m-biphenylyl H p-tolyl H H H H H m-biphenylyl p-tolyl H H H H p-biphenylyl H p-tolyl H H H H H p-biphenylyl p-tolyl H H K H p-tolyl H p-tolyl H H H H H p-tolyl (請先閲讀背面之注意事項再填寫本頁) 裝· 訂 線 本紙伕尺度適用中國國家標準（CNS〉A4規格（210X297公釐） -64 - 581751 A7 B7 五、發明説明（62 )
R5 R4 3 R E-191 E-192 E-193 E-194 E-195 E-196 E-197 E-198 E-199 E-200 E-201 E-202 E-203 E-204 E-205 E-206 E-207 E-208 E-209 E-210 E-211 E-212 E-213 E-214 E-215 E-216 E-217 x E-218 〇-〇 E-219 o-biphenylyl E-220 • (°"聯苯基）£-221 E-222 E-223
C0 1-naphthy丨（l·萘基) 2-naphthyl (2-菜基) oc5 m-biphenylyl (m·聯苯基) E-224 E-225 E-226 E-227 E-228 H3Ch E-229 -(3 E-230 〇4〇丨y丨（〇·甲苯基）E-231 CH3 Ε·232 E-233 \^/ c m-tolyl (m-甲苯基） 厂v E-236 E-237 p-tolyl (p*甲苯基）E-238 E-239 E-240 E-241 E-242 E-243 E-244 E-245 E-246 E-247 E-248 E-249 E-250 p-biphenylyl (P·聯苯基)
DPA
~〇N o
TPA o
Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph. 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphlhyl o-biphenylyl m-biphenylyl p-biphenylyi Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenyiyl p-biphenylyl Ph 1-naphtyl 2*naphthyl o-biphenylyl m-biphenylyl p-biphenylyl
H3H3H3H3H39 UH3H3 • HHHHHHHH H HHH HH HHHHHHH HHHHHHH HH^nHH HHH HH HHHHHHHH HH H HH HHHHHHH Η H HHH HHHHH H HHH HH Η H HH HH Η HHHHHHHHHHHHH HHHHHHHHHHHH
HHHHHHHH HHHHHHH Η HHHHH HH HHHH Η H hhhh HHHHH
HHHHHHHH
Η Η Η HH HHHH HH Η Η Η HHH HHHHH HHHHHHH Η HHHHH HHHHHHHH HHHH Η H HHHH H HHHH Η H R7I hhhhhhhhhs^^ s>^^hhhh hhhh H -CH3 -CH3 •CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 H H H H H H DPA DPA DPA DPA DPA DPA H H H H H H TPA TPA TPA TPA TPA TPA. •R8η η η hh η η η h
Η Η Η Η Η Η Η Η Η -CH3 -CH3 •CH3 •CH3 -CH3 -CH3 -CH3 -CH3 -CH3 •CH3 -CH3 -CH3 :CH3 -CH3 -CH3 -CH3 -CH3 •CH3 DPA DPA DPA DPA DPA DPA H H H H H H TPA TPA TPA 丁 PA TPA TPA H H H H H H (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) Α4規格（210X297公釐） -65- 581751 A7 B7 五、發明説明（63 )
2-naphthyl (2-蔡基）ob o-biphenylyl (〇·聯苯基）o-d m-biphenyly丨（m-聯苯基）f-23 p-biphenyly丨（p·聯苯基）
Nw L·
00 1-naphthyl (1-蔡基） Ri r2 F-1 Η H F-2 Ph H F-3 Ph Ph F-4 Ph H F-5 Ph H F-6 Ph H F-7 Ph H F-8 Ph .H F-9 Ph H F-10 Ph H F-11 Ph .H F-12 Ph H F-13 Ph H F-14 Ph H F-15 Ph H F-16 Ph H F-17 Ph H F-18 Ph H F-19 Ph H F-20 Ph H F-21 Ph H F-22 Ph H F-23 Ph H F-24 Ph H F-25 1-naphlhyl H F-26 1-naphthyl Ph F-27 1-naphthyl H F-28 1-naphthyl H F-29 1-naphthyl H F-30 1-naphthyl H F-31 1-naphthyl H F-32 1-naphthyl H F-33 1-naphthyl H F-34 1-naphthyl H F-35 1-naphthyl H F-36 1-naphthyl H F-37 1-naphthyl H F-38 1-naphlhyl H F-39 1-naphthyl H F-40 1-naphthyi H F-41 1-naphlhyl H F-42 1-naphlhyl H F-43 1-naphlhyl H F-44 1-naphlhyl H F-45 1-naphthyl H F-46 1-naphthyl H F-47 .1-naphthyl H r5 r7 r8 ^ hhh^h^hhhhhhhhhhhhhhhhhh hh^h^hhhhhhhhhhhhhhhhhh R3HHHphphHHHHHHHHHHHHHHHHHHH HHphphHHHHHHHHHHHHHHHHHHH H H H H H H Ph H H H H H H H H H H H H Ph H H H Ph H Ph Ph H 1-naphthyl H H H 1-naphthyl H 1-naphthyl 1-naphthyl H 2-naphthyl H H H 2-naphthyl H 2-naphthyl 2-naphthyl H o-biphenylyl H H H o-biphenylyl H o-biphenylyl o-biphenylyl H m-biphenylyl H H H m-biphenylyl H m-biphenylyl m-biphenylyl H p-biphenylyl H H H p-biphenylyl H .p-biphenylyl p-biphenylyl H H H Ph H H H H H H H H H H H H Ph H H H Ph H Ph Ph H 1-naphthyl H H H 1-riaphthyI H 1-naphlhyl 1-naphthyl H 2-naphthyl H H H 2-naphthyl H 2-naphthyl 2-naphthyl H o-bfphenylyl H H H o-biphenylyl H o-biphenylyl o-biphenylyl H m-blphenylyl H H H m-biphenylyl H m-biphenylyl m-biphenylyl H p-biphenylyl H H H p-biphenylyl H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本纸張尺度適用中國國家標準（CNS ) A4規格（21〇X297公釐） -66- 581751 A7 B7 五、發明説明（64 )
〇τ6 L 土 Pίί 00 1-naphthyl (1-^S) 2-naphthyl (2-蔡基） ob 种 o-biphenylyl (°·聯本基） p-biphenylyl (p·聯苯基） Ri r2 R3 R4 r5 Ry Re F-48 2-naphthyl. H H H H H H F-49 2-naphthyl Ph H H Ph H H F-50 2-naphthyl H Ph Ph H H H F-51 2-naphthyl H Ph H H H H F-52 2-naphthyl H H Ph H H H. F-53 2-naphthyl H H H H Ph H F-54 2-naphthyl H H H H H Ph F-55 2-naphthyl H H H H Ph Ph F-56 2-naphthyl H H H H 1-naphthyl H F-57 2-naphthyl H H H H H 1-naphthyl F-58 2-naphthyl H H H H 1-naphthyl 1-naphthyl F-59 2naphthyi H H H H 2-naphthyl H F-60 2-naphthyl H H H H H 2-naphthyl F-61 2-naphthyl H H H H 2-naphthyl 2-naphthyl F-62 2-naphthyl H H H H o-biphenylyl H F-63 2-naphthyl H H H H H o-biphenylyl F-64 2-naphthyl H H H H o-biphenylyl o-biphenylyl F-65 2-naphthyl H H H H m-biphenylyl H F-66 2-naphlhyl H H H H H m-biphenylyl F^7 2-naphlhyl H H H H m-biphenylyl m-biphenylyl F-68 2-naphthyl H H H H p-biphenylyl H F-69 2-naphthyl H H H H H p-biphenylyl F-70 2-naphthyl H H H H p-biphenylyl p-biphenylyl F-71 o-biphenylyl H H H H H H F-72 o-biphenylyl Ph H * H Ph H H F-73 o-biphenyfyl H Ph Ph H H H F-74 o-biphenylyl H Ph H H H H F-75 o-biphenylyl H H Ph H H H R76 o-biphenylyl H H H H Ph H F-77 o-biphenylyl H H H H H Ph F-78 o-biphenylyl H H H H Ph Ph F-79 o-biphenylyl H H H H 1-naphthyl H F-80 o-biphenylyl H H H H .H 1-naphlhyl F-81 o-biphenylyl H H H H 1-naphlhyl 1-naphthyl F-82 o-biphenylyl H H H H 2-naphthyl H F-83 o-biphenylyl H H H H H 2-naphlhyl F-84 o-biphenylyl H H H H 2-naphthyl 2-naphthyl F-85 o-biphenylyl H H H H o-biphenylyl H F-86 o-biphenylyl H H H H H o-biphenylyl F-87 o-biphenylyl H H H H o-biphenylyl o-biphenylyl F-88 o-biphenylyl H H H H m-biphenylyl H F-89 o-biphenyJyl H H H H H m-biphenylyl F-90 o-biphenylyl H H H H m-biphenylyl m-biphenylyl F-91 o-biphenylyl H H H H p-biphenylyl H F-92 o-biphenylyl H H H H H • p-biphenylyl F-93 o-biphenylyl H H H H p-biphenylyl p-biphenylyl ---------辦衣------IT------0 (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） -67- 581751 A7 B7 五、發明説明（65 )
o-biphenylyl (ο-聯苯基）FM12 F-113 F-114 m-biphenylyl P 川 (m-聯苯基）卜·Ί10 F-116 od p-blphenyly丨（p-聯苯基〕 F-117 F-118 F-119 F-120 F-121 F-122 F-123 F-124 F-125 F-126 F-127 F-128 F-129 Μ 30 F-131 F-132 F-133 F-134 F-135 F-136 F-137 F-138 F-139 m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl R2 · r4 r5 r7 Re Η Η Η Η Η H Fh Η Η Ph Η H Η Ph Ph Η Η H hi Ph Η Η Η H Η Η Ph Η Η H Η Η Η Η Ph H Η Η Η Η Η Ph Η Η Η Η Ph Ph Η Η Η Η 1-naphthyl H Η Η Η Η Η 1-naphthyl Η Η Η Η 1-naphthyl 1-naphthyl Η Η Η Η 2-naphthyl H Η Η Η Η Η 2-naphthyl Η Η Η Η 2-naphthyl 2-naphthyl Η Η Η Η o-biphenylyl H Η Η Η Η Η o-biphenylyl Η Η Η Η o-biphenylyl o-biphenylyl Η Η Η Η m-biphenylyl H Η Η Η Η H m-biphenylyl Η Η Η Η m-biphenylyl .m-biphenylyl Η Η Η Η p-biphenylyl H Η Η Η Η H p-biphenylyl Η Η Η Η p-biphenylyl p-biphenylyl Η Η Η Η H H Ph Η Η Ph H H Η Ph Ph Η H H Η Ph Η Η H H Η Η Ph Η H H Η Η Η Η Ph H Η Η Η Η H Ph Η Η .Η Η Ph Ph Η Η Η Η 1-naphthyl H Η Η Η Η H 1-naphthyl Η Η Η Η 1-naphthyl ' 1-naphthyl Η Η Η Η 2-naphthyl H Η Η Η Η H 2-naphthyl Η Η Η Η 2-naphthyl 2-naphthyl Η Η Η Η o-biphenylyl H Η Η Η Η H o-biphenylyl Η Η Η Η o-biphenylyl o-biphenylyl Η Η Η Η m-biphenylyl H Η Η Η Η H m-biphenylyl Η Η Η Η m-biphenylyl m-biphenylyl Η Η Η Η p-biphenylyl H Η Η Η Η H p-biphenylyl Η Η Η Η p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) -裝·
、1T 線 本紙張尺度適用中國國家標準（CNS ) Α4%格（210X29*7公釐） -68- 581751
A B7 五、發明説明（66 )
00 1-naphthyl (1-萘基) 2-naphthyl (2-^¾)ob o-biphenylyl (0-聯苯基）od m-biphenylyl (m-聯苯基） p-biphenylyl • (p·聯苯基） o-toly丨（〇·甲苯基） CH3 m-tolyl如·甲苯基） -〇ch3 • p-bly丨少甲茏基） F-140 F-141 F-142 F-143 F-144 F-145 F-146 F-147 F-148 F-149 F-150 F-151 F-162 F-153 E-154 F-155 F-156 F-157 F-158 F-159 E-160 F-161 F-162 F-163 F-164 F-165 F-166 F-167 F-168 F-169 F-170 F-171 F-172 F-173 F-174 F-175 F-176 F-177 F-17B F-179 F-180 F-181 F-182 F-183 F-184 F-185 F-186 F-187 F-188 F-189 F-190 o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-to&l o-tolyl o-tolyl o-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl Holy! p-tolyl p-tolyl p-tolyl p-iolyl p-tolyl p-tolyl p-tolyl p-lolyl H phhh hhhhhhhhhhhhh^ hhhhhhhhhhhhhhh hhh hhhhhhhhhhhh H h^hh hhhhhhhhhhhhhh ^hhhhhhhhhhhhhh hh^hhhhhhhhhhhhhh H H^HH hhhhhhhhhhh hhh hhhhhhhhhhhhhhh hh^hhhhhhhhhhhhhh D^-- H ^hhh hhhhhhhhhhhhhh hhhhhhhhhhhhhhh h^hhhhhhhhhhhhhhh r7 Re Η Η Η Η Η Η Ph Η Η Ph 1-naphthyl Η Η 1-naphthyl 2-naphthyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p-biphenylyl o-tolyl Η Η o-tolyl Η Η Η Η Η Η Ph Η Η Ph 1-naphthyl Η Η 1-naphthyl 2-naphthyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-blphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p-biphenylyl m-tolyl Η Η m-tolyl Η Η Η Η Η Η Ph . Η Η Ph 1-naphthyl Η Η 1-naphthyl 2-naphthyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p-biphenylyl p-tolyl Η Η p-tolyl (請先閲讀背面之注意事項再填寫本頁) •裝· 訂 線 本紙沬尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -69- 581751 Α7Β7 五、發明説明（67 )
F-191 F-192 . F-193 F-194 F-195 F-196 F-197 F-198 F-199 F-200 F-201 F-202 F-203 F-204 F-205 F-206 F-207 E-20B F-209. F-210 F-211 F-212 F-213 F-214 F-215 F-216 F-217 F-218 F-219 o-biphenylyJ F-220 (〇»聯苯基） F-222 m-biphenylyl ^23 (m·瞰苯基） F-225 F-226 F-227 F-228 F-229 F-230 F-231 F-232 F-233 Π， F-234 m-tolyl (m·甲苯基）ρ·235 -〇CH3 F：23? p*tolyl . (p·甲苯基）F-238 F-239 F-240 F-241 F-242 F-243 F-244 F-245 F-246 F-247 F-248 F-249 F-250 C0 1- naphthyl ,οσ 2- naphlhy 丨(2·萊基）ob o-biphenyly (ο-ϊod p-biphenylyl (p·聯苯基） o-tolyl (〇*甲苯基i CH3
DPA
TPA
Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl 0- tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyI 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphlyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl 0- lolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphlhyl o-biphenylyl m-blphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl IΗ3Η3Η3Η3Η3Η3Η3Η3Η3ΗΗΗΗΗ ηηηηηηηηηηηηηηη Η Η Η ΗΗ Η ηηηηηηηηηηηη ηηηηηηηηηηηηη F--C-C-C-C.C9-C9-C R2I ΗΗΗ ΗΗ ηηηηηηηη η ΗΗΗ ΗΗΗΗΗ Η ΗΗΗ ΗΗΗΗ ΗΗΗΗΗ ΗΗΗΗΗΗΗΗ ΗΗΗΗ Η ΗΗΗΗΗΗΗΗ ΗΗΗΗ R^- ^^^^^ηηηηηηηηηηηηη ηηηηηηηη ηηηηηηηηηηηηηηηηηηηηηηηηηηηηηη r5
Re Η Η Η ΗΗ ΗΗΗΗΗΗΗ Η Η ΗΗΗ ΗΗΗΗΗ ΗΗΗΗΗΗΗ Η ΗΗ ΗΗ Η ΗΗΗΗΗΗΗΗ ΗΗΗΗ Η Η ΗΗΗΗΗΗΗΗΗΗΗ HHHHH HHHH-CH:CCHH3-CH3-CH3-CH3-CH3-CH3-CH3HHHH hhhhhch-ch.ch-ch.ch-ch:cchhhchhhhhhdpadpa^dpadpahhhhhhtpatpatpatpatpatpa
H H H
H H H H H H H H H H H H H -CH3 «CH3 •CH3 -CH3 •CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 •CH3 -CH3 •CH3 -CH3 -CH3 •CH3 -CH3 DPA DPA DPA DPA DPA DPA H H H H H H TPA TPA TPA TPA TPA TPA H H H H H H (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X 297公釐） -70 581751 A7 B7
G-25 G-47 Ri r2 r3 r5 r6 R7 Re Η H H H H H H Ph H H H Ph H H Ph Ph H H Ph H H Ph H H Ph Ph H H Ph Ph H Ph Ph H H Ph H Ph H Ph H H Ph H H H Ph Ph H Ph H H H Ph H Ph Ph H H H Ph Ph Ph Ph H H H Ph 1-naphthyl H Ph H H H Ph H 1-naphlhyl Ph H H H Ph 1-naphthyl 1-naphthyl Ph .H H H Ph 2-naphthyl H Ph H H H Ph H 2-naphlhyl Ph H H H Ph 2-naphthyl 2-naphthyl Ph H H H Ph o-blphenylyl H Ph H H H Ph H o-biphenylyl Ph H H H Ph o-biphenylyl o-biphenylyl Ph H H H Ph m-biphenylyl H Ph H H H Ph H m-biphenylyl Ph H H H Ph m-biphenylyl m-biphenylyi Ph H H H Ph p-biphenylyl H Ph H H H Ph H p-biphenylyl Ph H H H Ph p-biphenylyl p-biphenylyl 1-naphthyl H H H 1-naphthyl H H 1-naphthyl Ph H H 1-naphthyl H H 1-naphlhyl H H Ph 1-naphthyl H H 1-naphthyl Ph H Ph 1-naphthyl H H 1-naphthyl H Ph H 1-naphthyl H H 1-naphthyl H H H 1-naphthyl Ph H 1-naphthyl H H H 1-naphlhyl H Ph 1-naphthyl H H H 1-naphthyl Ph Ph 1-naphthyl H H H 1-naphthyl 1-naphthyl H 1-naphthyl H H H 1-naphthyl H 1-naphlhyl 1-naphthyl H H H 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl H H H 1-naphthyl 2-naphthyl H 1-naphthyl H H H 1-naphlhyl H 2-naphthyl 1-naphthyl H H H 1-naphthyl 2-naphthyl 2-naphthyl 1-naphthyl H H H 1-naphthyl o-biphenylyl H 1-naphthyl H H H 1-naphthyl H o-biphenyiyl 1-naphthyl H H H 1-naphthyl o-biphenylyl o-biphenylyl 1-naphthyl H H H 1-naphthyl m-biphenylyl H 1-naphthyl H H H 1-naphthyl H m-biphenylyl 1-naphthyl H H H 1-naphthyl m-biphenylyl m-biphenylyl 1-naphthyl H H H 1-naphthyl p-biphenylyl H 1-naphthyl H H H 1-naphthyl H p-biphenylyl 1-naphthyl H H H 1-naphthyl p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 五、發明説明（68 ) C0 1-naphlhy丨（1-萘基） 2-naphthyl (2·蔡基） ob 奸· o-bipheny丨yl (〇-聯本基） p-biphenylyl (P~聯苯基) 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -71 - 581751 A7 B7 五、發明説明（69 )尽2尽1 ^ Ββ 85 3Ί r7-
06 1- naphthy丨（1-萘基）οσ 一. 2- naph〖hyl (2-萘基）o-b 作 o-biphenyly丨（〇-聯本基） G-48 G-49 (3-50 G-51 G-52 G-53 G-54 G-55 G-56 G-57 G-58 G-59 G-60 G-61 G-62 G-63 G-64 G-65 G-66 G-67 G-68 od •奸— m-bipheny丨yl (m-聯苯基）g-69 G-70 p-biphenylyl (p·聯苯基） G-71 G-72 G-73 G-74 G-75 G-76 G-77 G-78 G-79 G-80 G-81 G-82 G-83 G-84 G-85 G-86 G-87 G-88 G-89 G-90 G-91 G-92 G-93 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthy! 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl o-blphenylyl o-biphenylyl o-biphenylyl o-bipheny)yl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenytyl r2 ^3 r5 Re r7 Re Η Η Η 2-naphthyl H H Ph Η Η 2-naphthyl H H Η Η Ph 2-naphthyl H H Ph Η Ph 2-naphthyl H H Η Ph Η 2-naphthyl H H Η Η Η 2-naphthyl Ph H Η Η Η 2-naphthyl H Ph Η Η Η 2-naphthyl Ph Ph Η Η Η 2-naphthyl 1-naphthyl H Η Η Η 2-naphthyl H 1-naphthyl Η Η Η 2-naphthyl 1-naphthyl 1-naphthyl Η Η Η 2-naphthyl 2-naphthyl H Η Η Η 2-naphlhyl H 2-naphthyl Η Η Η 2-naphthyl 2-naphthyl 2-naphthyl Η Η Η 2-naphthyl o-biphenylyl H Η Η Η 2-naphthy) H o-biphenylyl Η Η Η 2-naphthyl o-biphenylyl o-biphenylyl Η Η Η 2-naphthyl m-biphenylyl H Η Η Η 2-naphthyl H m-biphenylyl Η Η Η 2-naphthyl m-biphenylyl m-biphenylyl Η Η Η 2-naphthyl p-biphenylyl H Η Η Η 2-naphthyl H p-biphenylyl Η Η Η 2-naphthyl p-biphenylyl p-biphenylyl Η Η Η o-biphenylyl H H Ph Η Η o-biphenylyl H H Η Η Ph o-biphenylyl H H Ph Η Ph o-blphenylyl H H Η Ph Η o-biphenylyl H H Η Η Η o-biphenylyl Ph H Η Η Η o-biphenylyl H Ph Η Η Η o-biphenylyl Ph Ph Η Η Η o-biphenylyl 1-naphthyl H Η Η Η o-biphenylyl H 1-naphthyl Η Η Η o-biphenylyl 1-naphthyl 1-naphthyl Η Η Η o-biphenylyl 2-naphthyl H Η Η Η o-biphenylyl H 2-naphthyl Η Η Η o-biphenylyl 2-naphthyl 2-naphthyl Η Η Η o-biphenylyl o-biphenylyl H Η Η Η o-biphenylyl H o-biphenylyl Η Η Η o-biphenylyl o-biphenylyl o-biphenylyl Η Η Η o-biphenylyl m-biphenylyl H Η Η Η o-biphenylyl H m-biphenylyl Η Η Η o-biphenylyl m-biphenylyl m-biphenylyl Η Η Η o-biphenylyl p-blphenylyl H Η Η Η o-biphenylyl H p-biphenylyl Η Η Η o-biphenylyl p-biphenylyl p-biphenyly! 訂 線 (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -72- 581751 A7 B7 五、發明説明（70 )
Ra Ο. R1 r2 R3 r5 Re Ry Re H7 00 G-94 m-biphenylyl H H H m-biphenylyl H H 孩6 G-95 m-biphenylyl Ph H H m-biphenylyl H H G-96 m-biphenylyl H H Ph m-biphenylyl H H G-97 m-biphenylyl Ph H Ph m-biphenylyl H H Re-<>Ri G-98 m-biphenylyl H Ph H m-biphenylyl H H G-99 m-biphenylyl H H H m-biphenylyl Ph H G-100 m-biphenylyl H H H m-biphenylyl H Ph CX3 G-101 m-biphenylyl H H H m-biphenylyl Ph Ph ττ R7 Re G-102 m-biphenylyl H H H m-biphenylyl 1-naphthyl H XypcG G-103 m-biphenylyl H H H m-biphenylyl H 1-naphthyl G-104 m-biphenylyl H H H m-biphenylyl 1-naphthyl 1-naphthyl G-105 m-biphenylyl H H H m-biphenylyl 2-naphthyl H G-106 m-blphenylyl H H H m-biphenylyl H 2-naphthyl G-107 m-biphenylyl H H H m-biphenylyl 2-naphthyl 2-naphthyl G-108 m-biphenylyl H H H m-biphenylyl o-biphenylyl H 00 G-109 m-biphenylyl H H H m-biphenylyl H o-biphenylyl G-110 m-biphenylyl H H H m-biphenylyl o-biphenylyl o-biphenylyl G-111 m-biphenylyl H H H m-biphenylyl m-biphenylyl H 1-naphthy丨（丨·萘基)(3-112 m-biphenylyl H H H m-biphenylyl H m-biphenylyl ΓΤΎ G-113 m-biphenyjyl H H H m-biphenylyl m-biphenylyl m-biphenylyl G-114 m-biphenylyl H H H m-biphenylyl p-biphenylyl H 2-naphthyl (2-^S) g-1 15 m-biphenylyl H H H m-biphenylyl H p-biphenylyl ob o-biphenylyl G-116 m-biphenylyl H H H m-biphenylyl p-biphenylyl p-biphenylyl G-117 P^phenylyf H H H p-biphenylyl H H (〇·聯苯基: od * G-118 P-biphenylyl Ph H H p-biphenylyl H H G-119 P-biphenylyl H H Ph p-biphenylyl H . H m-biphenylyl G-120 p-biphenylyl Ph H Ph p-biphenylyl H H (m-聯苯基、G-121 p-biphenylyl H Ph H p-biphenylyl H H G-122 p-biphenylyl H H H p-biphenylyl Ph H \mtm/ \ im ¥ p-biphenylyl G-123 p-biphenylyl H H H p-biphenylyl H Ph (p>聯苯基） G-124 P-biphenylyl H H H p-biphenylyl Ph Ph G-125 p-biphenylyl H H H p-biphenylyl 1-naphthyl H G-126 p-biphenylyl H H H p-biphenylyl H 1-naphthyl G-127 p-biphenyJyl H H H p-biphenylyl 1-naphthyl 1-naphthyl G-128 — H H H p-biphenylyl 2-naphthyl H G-129 P-biphenyly) H H H p-biphenylyl H 2-naphthyl G-130 p-biphenylyl H H H p-biphenylyl 2-naphthyl 2-naphthyl G-131 p-biphenylyl H H H p-biphenylyl o-biphenylyi H G-132 p-biphenylyl H H H p-biphenylyl H o-biphenylyl G-133 p-biphenylyl H H H p-biphenylyl o-biphenylyl o-biphenylyl G-134 p-biphenylyl H H H p-biphenyly! m-biphenylyl H G-135 p-biphenylyl H H H p-biphenylyl H m-biphenylyl G-136 p-biphenylyl H H H p-biphenylyl m-biphenylyl m-biphenylyl G-137 p-biphenylyl H H H p-biphenylyl p-biphenylyl H G-138 p-biphenylyl H H H p-biphenylyl H p-biphenylyl G-139 p-biphenylyl H H H p-biphenylyl p-biphenylyl p-biphenylyl ---------批衣------1T------線 (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中囷國家標準（CNS ) A4規格（21〇χ297公釐） -73- 581751
7 7 A B 五、發明説明（71 ) r2
甲B
Rl C0 1-naphlhy丨（1·萘基） 2-naphthyl (2·蒂基） ob o-biphenylyl (〇>聯苯基） 〇τ6 m-blphenylyl (m-聯苯基) p-biphenylyl (p·脚苯基） o^toly丨（〇·田苯基） CH3 m-tolyl (m·甲苯基） ~〇~ch3 p-tolyl (p·甲苯基） G-140 o-lolyl G-141 o-tolyl G-142 o-tolyl G-143 o-tolyl G-144 o-tolyl G-145 o-tolyl G-146 o-tolyl G-147 o-toly) G-148 o-tolyl G-149 o-tolyl G-150 o-tolyl G-151 o-tolyl G-152 o-tolyl G-153 o-tolyl G-154 o-tolyl G-155 o-tolyl G-156 o-tolyl G-157 m-tolyl G-158 m-tolyl G-159 m-tolyl G-160 m-tolyl G-161 m-tolyl G-162 m-tolyl G-163 m-tolyl G-164 m-tolyl G-165 m-tolyl G-166 m-tolyl G-167 m-tolyl G-168 m-tolyl G-169 m-tolyl G-17Q m-tolyl G-171 m-tolyl G-172 m-tolyl G-173 m-tolyl G-174 p-tolyl G-175 p-tolyl G-176 p-tolyl G-177 p-tolyl G-178 p-tolyl G-179 p-tolyl G-180 p-tolyl G-181 p-tolyl G-182 p-tolyl G-183 p-tolyl G-184 p-tolyl G-185 p-tolyl G-186 p-tolyl G-187 p-tolyl G-188 p-tolyl G-189 p-tolyl G-190 p-to!yl
H ^HHH hhhhhhhhhhhhhh HHHHHHHHHHHHHHHHphHHHHHHHHHHHHHHH ps R3 Η ^HHH Η HHH HHHHHHH HH^ HHHHHHHHHHHHHHHΉέΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗ H H^HH hhhhhhhhhhhhhh ^hhhhhhhhhhhhhh hh^hhhhhhhhhhhhhh r6 · r7 Re o-tolyl H H o-tolyl H H o-tolyl H H o-tolyl Ph H o-tolyl H Ph o-tolyl 1-naphthyl H o-tolyl H 1-naphthyl o-tolyl 2-naphthyl H o-tolyl . H 2-naphthyl o-tolyl o-biphenylyl H o-tolyl H o-biphenylyl o-tolyl m-biphenylyl H o-tolyl H m-biphenylyl o-tolyl p-biphenylyl H o-tolyl H p-biphenylyl o-tolyl o-tolyl H o-tolyl H o-tolyl m-tolyl H H m-tolyl H H m-toiyl H H m-tolyl Ph H m-tolyl H Ph m-tolyl 1-naphthyl H m-tolyl H 1-naphthyl m-tolyl 2-naphthyl H m-tolyl H 2-naphthyl m-tolyl o-biphenylyl H m-tolyl H o-biphenylyl m-tolyl m-biphenylyl H m-tolyl H m-biphenylyl m-tolyl p-biphenylyl H m-tolyl H p-biphenylyl m-tolyl m-tolyl H m-tolyl H m-tolyl p-tolyl H H p-toly! H H p-tolyl H H p-tolyl Ph H p-tolyl H Ph p-tolyl 1-naphthyl H p-lolyl H 1-naphthyl p-tolyl 2-naphthyl H p-tolyl H 2-naphthyl p-tolyl o-biphenylyl H p-tolyl H o-biphenylyl p-tolyl m-biphenylyl H p-tolyl H m-biphenylyl p-tolyl p-biphenylyl H p-tolyl H p-biphenylyl p-tolyl p-tolyl H p-tolyl H p-tolyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -74- 581751 五、發明説明（72 ) r3 R5 Rs R7
Rb
TypeG
r2 C0 1-naphthyl (1-萊基） 2-naphthy丨（2-莱基） ob o^biphenyly丨（〇·聯苯基） o-d m-biphenylyl (m-聯苯基） p-biphenylyl (p·聯苯基） o-to)yl (〇·甲苯基） -oCH3 nrvtdyl (m·甲苯基） -〇ch3 p-tolyt (p·甲苯基） DPA TPA G-191 Ph H G-192 1-naphtyl H G-193 2-naphthyl H G-194 o-biphenylyl H G-195 m-biphenylyl H G-196 p-biphenylyl H G-197 o-tolyl H G-198 m-tolyl H G-199 p-tolyl H G-200 Ph H G-201 1-naphtyl H G-202 2-naphthyl H G-203 o-biphenylyl H G-204 m-biphenylyl H G-205 p-biphenylyl H G-206 o-tolyl H G-207 m-tolyl H G-208 p-tolyl H G-209 Ph H G-210 G-211 G-212 1- naphtyl 2- naphthyl o-bipnenylyl H H H G-213 m-biphenylyl H G-214 p-biphenylyl H G-215 o-tolyl H G-216 m-tolyl H G-217 p-tolyl H G-218 Ph H. <3-219 1-naptity! H G-220 2-naphthyl H G-221 o-biphenylyl H G-222 m-biphenylyl H G-223 p-biphenylyi H G-224 o-tolyl H G-225 m-tolyl H G-226 p-tolyl H G-227 Ph H G-228 1-naphlyl H G-229 2-naphthyl H G-230 o-biphenylyl * H G-231 m-biphenylyl H G-232 p-biphenylyl H G-233 Ph H G-234 G-235 G-236 G-237 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl H H H H G-238 p-biphenylyl H G-239 Ph H G-240 1-naphtyl H G-241 2-naphthyl H G-242 o-biphenylyl H G-243 m-biphenyiyl H G-244 p-biphenylyl H <3-245 Ph H G-246 1-naphlyl H G-247 2-naphthyl H G-248 o-biphenylyl H G-249 m-biphenylyl H G-250 p-biphenylyl H
-CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 H H H H H H H H H H H H H H H H H H H H H Η Η ΗΗ Η ΗΗΗΗΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗΗ
HHHHH ηηηηηηη Η Η ΗΗΗ ΗΗΗΗΗ ΗΗΗΗΗΗΗΗ Η Η Η Η Η ΗΗΗΗΗΗΗΗ ΗΗΗΗ Η Η ΗΗΗΗΗΗΗΗΗΗΗ · Ph H 1-naphtyl H 2-naphthyl H o-biphenylyl H m-biphenylyl H p-biphenylyl H o-tolyl H m-tolyl H p-tolyl H Ph -CH3 1-naphtyl •CH3 2-naphthyl -CHS o-biphenylyl -CH3 m-biphenylyl -CH3 p-biphenylyl -CH3 o-tolyl -CH3 m-tolyl -CH3 p-tolyl -CH3 Ph H 1-naphtyl H 2-naphthvl o-biphenylyl H H m-biphenylyl H p-biphenylyl H o-tolyl m-tolyl H H p-tolyl H Ph -CH3 1-naphtyl •CH3 2-naphthyl -CH3 o-biphenylyl •CH3 m-biphenylyl -CH3 p-biphenylyl -CH3 o-tolyl -CH3 m-tolyl -CH3 p-tolyl -CH3 Ph H 1-naphlyl H 2-naphthvl o-biphenylyl H H · m-biphenylyl H p-biphenylyl H Ph DPA 1-naphlyl. DPA 2-naphthyl o-biphenylyl m-biphenylyl DPA DPA DPA p-biphenylyl DPA Ph . H 1-naphtyl H 2-naphthyl H o-biphenylyl H m-biphenylyl H p-biphenylyl H Ph TPA 1-naphtyl TPA 2-naphthyl TPA o-biphenylyl TPA m-biphenylyl TPA p-biphenylyl TPA
H H H
H H H H H H H H H H H H H •CH3 -CH3 -CH3 -CH3 •CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 . •CH3 •CH3 •CH3 •CH3 -CH3 DPA DPA DPA DPA DPA DPA H H H H H H •TPA TPA TPA TPA TPA TPA H H H H H H (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） 75 581751 A7 B7 五、發明説明（73 )
r8 «7 C0 1-naphthy丨 0-蔡基） otolyl (°·申苯基） ch3 n-tolyl (m·甲苯基） -〇CH3 p-tolyl 〇>·甲苯基） 2-naphthyl (2-蔡基） o-b丨phenylyl (0-聯苯基） od 抑 m-b丨phenyly丨（m-聯本基） p-biphenylyl (p·聯苯基） h3c Ri G-251 Ph G-252 Ph G-253 Ph G-254 Ph G-255 Ph G-256 Ph G-257 Ph . G-258 Ph G-259 1-naphthyl G-260 1-naphthyl G-261 1-naphthyl G-262 1-naphthyl G-263 1-naphthyl G-264 1-naphthyl G-265 1-naphthyl G-266 2-naphthyl G-267 2-naphthyl G-268 2-naphthyl G-269 2-naphthyl G-270 2-naphthyl G-271 2-naphthyl G-272 o-biphenylyl G-273 o-biphenylyl G-274 o-biphenylyl G-276 o-biphenylyl G-276 o-blphenylyl G-277 m-biphenylyl G-278 m-biphenylyl G-279 G-280 m-biphenylyl m-biphenylyl G-281 p-biphenylyl G-282 p-biphenylyl G-283 p-biphenylyl G-284 0-tolyly G-285 0-tolyly G-286 m-tolyly r3hhhh hhhhhh hhhhhhhhhhhhhhhhhh hh hhhh hh r2hhhh hhhhhhhhhhhhhhh hhhhhhhhh hh hhhh hh Η 1-naphthyl Η 2-naphthyl Η •o-biphenylyl Η m-biphenylyl Η p-biphenylyl Η 0-tolyly Η m-tolyl Η p-tolyl Η 2-naphthyl Η o-biphenylyl Η m-biphenylyl Η p-biphenylyl Η 0-tolyly Η m-tolyl Η p-tolyl Η o-biphenylyl Η m-biphenylyl Η p-biphenylyl Η 0-tolyly Η m-tolyl Η p-tolyl Η m-biphenyly! Η p-biphenylyl Η 0-tolyly Η m-tolyl Η p-tolyl Η p-biphenylyl Η 0-tolyly Η m-tolyl p-tolyl Η 0-tolyly Η m-tolyl Η p-tolyl Η m-tolyl Η p-tolyl Η p-tolyl hhhhhhhhhhhhhhhhhhhhhhhhhhhhhh hhhh hh
Ra hhhhhhhhhhhhhhhhhhhhhhhhhhhhhh hhhhhh ^-- (請先閲讀背面之注意事項再填寫本頁)
、1T 線 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -76- 581751 A7 B7 五、發明説明（74 ) 經濟部智您时/1^7"^工消費合作社印^ R1 r2 R3 R5 Re r7 Re 00 Η.Γ H H H H H H H Ri-Hr6 h·2 Ph H H H Ph H H R2-〇-R5 H'3 Ph Ph H H Ph H H Ph H H Ph Ph H H Q R3 H-5 Ph Ph H Ph Ph H H R>yR2 H-6 Ph H Ph H Ph H H R >tR H-7 Ph H H H Ph Ph H 1Y H'8 Ph H H H Ph H Ph TypeH ¢¢3 h-9 Ph H H. H Ph Ph Ph R7 Rb H-10 Ph H H H Ph 1-naphthyl H H-11 Ph H H H Ph H 1-naphthyl rvX Η·12 Ph H H H Ph 1-naphthyl 1-naphthyl H-13 Ph H H H Ph 2-naphthyl H 1-naphthyl (1-蔡基） Ph H H H Ph H 2-naphthyl H-15 Ph H H H Ph 2-naphthyJ 2-naphthyl H-16 Ph H H H Ph o-biphenylyl H 2-naphthyl (2-萘基）H>>17 Ph H H H Ph H o-biphenylyl V H-18 Ph H H H Ph o-biphenylyl o-blphenylyl 〇〇 H-19 Ph H H H Ph m-biphenyJyl H o-biphenylyl (〇·聯苯基）h-20 Ph H H H Ph H m-biphenylyl H-21 Ph H H H Ph m-biphenylyl m-biphenylyl ryri η-22 Ph H H H Ph p-biphenyly) H m-b〗phenyly丨（m-聯苯基） Ph H H H Ph H p-biphenylyl H-24 Ph H H H Ph p-biphenylyl p-biphenylyl ChCh Η·25 1-naphthyl H H H 1-naphthyl H H p-biphenylyl (p-聯苯基）H-26 1-naphthyl Ph H H 1-naphthyl H H H-27 1-naphthyl H H . Ph 1-naphthyl H H Η·28 1-naphthyl Ph H .Ph 1-naphthyl H H H-29 1-naphthyl H Ph H 1-naphthyl H H H-30 1-naphthyl H H H 1-naphthyl Ph H H-31 .1-naphthyl H H H 1-naphthyl H Ph H-32 1-naphthyl H H H 1-naphthyl Ph Ph H-33 1-naphthyl H H H 1-naphthyl 1-naphthyl H H-34 1-naphthyl H H H 1-naphthyl H 1-naphthyl H-35 1-naphthyl H H H 1-naphthyl 1-naphthyl 1-naphthyl H-36 1-naphthyl H H H 1-naphlhyl 2-naphthyl H H-37 1-naphthyl H H H 1-naphthyl H 2-naphthyl • H-38 1-naphthyl H H H 1-naphthyl 2-naphthyl 2-naphlhyl H-39 1-naphthyl H H H 1-naphthyl o-biphenylyl H HMO 1-naphthyl H H H 1-naphthyl H o-biphenylyl H-41 1-naphthyl H H H 1-naphthyl o-biphenylyl o-biphenylyl H-42 1-naphthyl H H H 1-naphthyl m-biphenylyl H H-43 1-naphthyl H H H 1-naphthyl H m-biphenylyl H-44 1-naphthyl H H H 1-naphthyl m-biphenylyl m-biphenylyl H-45 1-naphthyl H H H 1-naphthyl p-biphenylyl H HM6 1-naphthyl H H H 1-naphthyl H p-biphenylyl H-47 1-naphthyl H H H 1-naphthyl p-biphenylyl p-biphenylyl ---------f------IT------0 (請先閲讀背面之注意事項再填寫本頁) 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -77- 581751 A7 B7 75 p-biphenyly丨（P-聯苯基） Ri r2 r3 Rs Re r7 Ra H-48 2-naphthyl H H H 2-naphthyl H H H-49 2-naphthyl Ph H H 2-naphthyl H H H-50 2-naphthyl H H Ph 2-naphthyl H H H-51 2-naphthyl Ph H Ph 2-naphthyl H H H-52 2-naphthyl H Ph H • 2-naphthyl H H H-53 2-naphthyl H H H 2-naphthyl Ph H H-54 2-naphthyl H H H 2-naphthyl H Ph Η·55 2-naphthyl H H H 2-naphthyl Ph Ph Η-56 2-naphthyl H H H 2-naphthyl 1-naphthyl H Η-57 2-naphthyl H H H 2-naphlhyl H 1-naphthyl Η-58 2-naphthyl H H H 2-naphthyl 1-naphthyl 1-naphthyl Η-59 2-naphthyl H H H 2-naphthyl 2-naphthyl H Η-60 2-naphthyl H H H 2-naphthyl H 2-naphthyl Η-61 2-naphthyl H H H 2-naphthyl 2-naphthyl 2-naphlhyI Η-62 2-naphthyl H H H 2-naphthyl o-biphenylyl H Η·63 2-naphthyl H H H 2-naphthyl H o-biphenylyl Η-64 2-naphthyl H H H 2-naphthyl o-biphenylyl o-biphenylyl Η-65 2-naphthyl H H H 2-naphthyl m-biphenylyl H Η·66 2-naphthyl H H H 2-naphthyl H m-biphenylyl Η-67 2-naphthyl H H H 2-naphthyl m-biphenylyl m-biphenylyl Η-68 2-naphthyl H H H 2-naphthyl p-biphenylyl H Η-69 2-naphthyl H H H 2-naphthyl .H p-biphenylyl Η-70 2-naphthyl H H H 2-naphthyl p-biphenylyl p-biphenylyl Η-71 o-biphenylyl H H H o-biphenylyl H H Η-72 o-biphenylyl Ph H H o-biphenylyl H . H Η-73 o-biphenylyl H H Ph o-biphenylyl H H Η-74 o-biphenylyl Ph H Ph o-biphenylyl H H Η-75 o-biphenylyl H Ph H o-biphenylyl H H Η-76 o-biphenylyl H H H o-biphenylyt Ph H Η-77 o-biphenylyl H H H o-biphenylyl H Ph Η-78 o-biphenylyl H H H o-biphenylyl Ph Ph · Η-79 o-biphenylyl H H H o-biphenylyl 1-naphthyl H Η-ΒΟ o-biphenylyl H H H o-biphenylyl H 1-naphthyl Η-81 o-biphenylyl H H H o-biphenylyl 1-naphthyl 1-naphlhyl Η-82 o-biphenylyl H H H o-biphenylyl 2-naphthyl H Η-83 o-biphenylyl H H H o-biphenylyl H 2-naphthyl Η-84 o-biphenylyl H H H o-biphenylyl 2-naphthyl 2-naphthyl Η·85 o-biphenylyl H H H o-biphenylyl o-biphenylyl H Η-Β6 o-biphenylyl H H H o-biphenylyl H o-biphenylyl Η·87 o-biphenylyl H H H o-biphenylyl o-biphenylyl o-biphenylyl Η-8Θ o-biphenylyl H H H o-biphenylyl m-biphenylyl H Η-89 o-biphenylyl H H H o-biphenylyl H m-biphenylyl Η-90 o-biphenylyl H H H o-biphenyly! m-biphenylyl m-biphenylyl Η-91 o-biphenylyl H H H o-biphenylyl p-biphenylyl H Η-92 o-biphenylyl H H H o-biphenylyl H p-biphenylyl Η·93 o-biphenylyl H H H o-biphenylyl p-biphenylyl p-biphenylyl 訂 線 (請先閲讀背面之注意事項再填寫本頁) 五、發明説明（
〇6 1- naphthy丨（1·萘基） 〇〇r 2- naphthyl (2·蔡基） cvb 抑 o-biphenylyl (〇·聯本基） od * m-biphenylyl (m-聯苯基) 本紙張尺度適用中國國家標率（CNS ) A4規格（210X297公釐） -78- 581751 A7 B7 五、發明説明（ 76
R1 逯濟部智您財4¾¾工消費合作钍印製 H-94 H-95 H-96 H-97 H-98 H-99 H-100 Η·101 Η-102 Η-103 Η-104 Η-105 Η-106 Η-107 Η-108 , Η-109 fYS Η-110 Η-111 1.naphthyl 0·菜基）Η·112 Η·113 Η-114 2-naphthyl (2·系基）Η·115 \ Η-116 〇-C) n o-bipheny丨yl (〜塒本基&117 y H-118 〇〇 謂 m-biphenylyl H-120 (m-聯苯基）H-121OO, HhT23 p-biphenylyl H*123 (p·聯苯i) H-124 H-125 H-126 H-127 H-128 H-129 H-130 H-131 H-132 H-133 H-134 H-135 H-136 H-137 H-138 H-139 p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyJ p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl m-biphenylyl m-blphenylyl m-biphenylyl r2 r3 R5 R6 r7 Re Η Η Η m-biphenylyl H H Ph Η Η m-biphenylyl H H Η Η Ph m-biphenylyl H H Ph Η Ph m-biphenylyl H H Η Ph Η m-biphenylyl H H Η Η Η m-biphenylyl Ph H Η Η Η m-biphenylyl H Ph Η Η Η m-biphenylyl Ph Ph Η Η Η m-biphenylyl 1-naphthyl H Η • Η Η m-biphenylyl H 1-naphthyl Η •Η Η • m-blphenylyl 1-naphthyl 1-naphthyl Η Η Η m-biphenylyl 2-naphthyl H Η Η Η m-biphenylyl H 2-naphthyt Η Η Η m-biphenylyl 2-naphthyl 2-naphthyl Η Η Η m-biphenylyl o-biphenylyl H Η Η Η m-biphenylyl .H o-biphenylyl Η Η Η m-biphenylyl o-biphenylyl o-biphenylyl Η Η Η m-biphenylyl m-biphenylyl H Η Η Η m-biphenyiyl H m-biphenylyl Η Η Η m-biphenylyl m-biphenylyl m-biphenylyl Η Η Η m-biphenylyl p-biphenylyl H Η Η Η m-biphenylyl H p-biphenylyl Η Η Η m-biphenylyt p-biphenylyl p_biphenylyl Η Η Η p-biphenylyl H H Ph Η Η p-biphenylyl H H Η Η Ph p-biphenylyl H H Ph Η Ph p-biphenylyl H H Η Ph Η p-biphenylyl H H Η Η Η p-biphenylyi Ph H Η Η Η p-biphenylyl H Ph Η Η Η p-biphenylyl Ph Ph Η Η Η p-biphenylyl 1-naphthyl H Η Η Η p-biphenylyl H 1-naphthyl Η Η Η p-biphenylyl 1-naphthyl 1-naphthyl Η Η Η p-biphenylyl 2-naphthyl H Η Η Η p-biphenylyl H 2-naphthyl Η Η Η p-biphenylyl 2-naphthyl 2-naphthyl Η Η Η p-biphenylyl o-biphenylyl H Η Η Η p-biphenylyl H o-biphenylyl Η Η Η p-biphenylyl o-biphenylyl o-biphenylyl Η Η Η p-biphenylyl m-biphenylyl H Η Η Η p-biphenylyl H m-biphenylyl Η Η Η p-biphenylyl m-biphenylyl m-biphenylyl Η Η Η p-biphenylyl p-biphenylyl H Η Η Η p-biphenylyl H p-biphenylyl Η Η Η p-biphenylyl p-biphenylyl p-biphenylyl ---------裝-- (請先閲讀背面之注意事項再填寫本頁) 訂 線 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -79- 581751
7 7 A B 五、發明説明（ 77
H-140 H-141 H-142 H-143 H-144 H-145 H-146 H-147 H-148 H-149 H-150 H-151 H-152 H-153 H-154 H-155 H-156 H-157 1- naphthyl H"158 (1-秦基）H-159 〇y η， 2- naphthyl Η*161 (2-萘基）Η-162 厂Η·163 Η-164 o-biphenylyl (〇·聯苯基）Η·165 / Η-166 〇〇 Η-167 m-biphenylyl Η-168 (m·聯苯基）η·169 〇〇 _ (Ρ·聯苯基）Η·172 h3c C0 Η-173 ~Λ-/ Η-174• o-tolyl (〇·甲苯基）η-175 ch3 經濟部智慧时是笱爵工消黃合作钍印^ Η-176
Ri o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-lolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl prolyl p-tolyi p-tolyl p-tolyl p-tolyl p-tolyl r2
Η ^HHH HHHH HHHHHHH HH^ HHHHHHHHHHHHHHH H^HHHHHHHHHHHHHHH R6 R5 ο o ooo oooooo<soooo-o-mm mmmmmmmmmmmmmm'm-Mp-p-p-p-p-p-p-ciLp-p-p-p-p-p-p-p* Η ^HHH Η HHH HHHHHHH HH^ HHHHHHHHHHHHHHH H^HHHHHHHHHHHHHHH H h^hh hhhhhhhhhhhhhh ^hhhhhhhhhhhhhh hh^hhhhhh hhhhhhhh r7 Re Η Η Η Η Η Η Ph Η Η Ph 1-naphthyl Η Η 1-naphthyl 2-naphthyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p-biphenylyl o-tolyl Η Η o-tolyl Η Η Η Η Η Η Ph Η Η 'Ph 1-naphthyl Η Η 1-naphthyl 2-naphthyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-blphenylyl Η Η p-biphenylyl m-tolyl Η Η m-tolyl Η Η Η Η Η Η Ph Η Η Ph 1-naphthyl Η Η 1-naphthyl 2-naphthyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p-biphenylyl p-tolyl Η Η p-tolyl (請先閲讀背面之注意事項再填寫本頁) 本纸張尺度適用中國®家標準（CNS ) A4規格（210X297公釐） -80- 581751 A 7 B7 五、發明説明（78 )
C0 ob o-biphenyly (〇聯潷 od
1-naphthyl (1·菜基) 2-naphthyl (2-萘基） m-biphenylyl (m-聯苯基） Ri H-191 Ph Η·192 1-naphtyl Η-193 2-naphlhyl Η-194 Η-195 o-biphenylyl m-biphenylyl Η-196 p-biphenylyl Η-197 Η-198 o-tolv) m-tolyl Η-199 p-tolyl Η-200 Ph Η-201 1-naphtyl Η-202 2-naphthyl Η-203 o-biphenylyl Η-204 m-biphenylyl Η-205 p-biphenylyl Η-206 o-tolyl Η-207 m-tolyl Η-208 p-tolyl Η-209 Ph Η-210 Η-211 Η-212 1- naphtyl 2- naphthyl o-bipnenylyl Η-213 m-biphenylyl Η-214 p-biphenylyl Η-215 o-tolyl Η-216 m-tolyl Η-217 p-toly) Η-218 Ph Η-219 1-naphtyl Η-220 2-naphthyl Η-221 o-biphenylyl Η-222 m-biphenylyl Η-223 p-blphenylyl Η-224 o-tolyl Η-225 m-tolyl r2 H H H
Re
H H H H H H H H H H H H H H
H H H H H H
-CH3 -CH3 -CH3 -CH3 -CH3 •CH3 -CH3 -CH3 -CH3 H H H H H H H H H H H H 唆耷巿r4;5rl^t!Hx.^:^^;t^^^ H-226 H-227 H-228 H-229 ^ H-230 丨（〇·甲苯基）H-231 CH H-232 H-233 Vi. m*»、H-234 m-loly 丨(m·甲苯基） ^ H-236 --Q-CH3 H-237 p-tolyl 少甲苯基） H-239 H-240 H-241 H-242 H-243 H-244 H-245 H-246 H-247 H-248 H-249 H-250
p-biphenylyl (p·聯苯基) H3C 0^,0
DPA
心g TPA
H H p-tolyl H Ph H 1- naphtyl H 2- naphthyl H o-biphenylyl H m-biphenylyl H p-biphenylyl H Ph H 1- naphtyl H 2- naphlhyl H o-biphenylyl H m-biphenylyl H p-biphenylyl H Ph H 1- naphlyl H 2- naphlhyl H o-biphenylyl H m-blphenylyl H p-biphenylyi H Ph H 1- naphtyl H 2- naphthyi H o-biphenylyl H m-biphenyiyl H p-biphenylyl H hhhhhhh h hhhhh hhhhhhhh hhhh h h hhhhhhhhhhh H HH HH hhhhhhh h h hhh hhhhh hhhhhhh h hhhhh hhhhhhhhhhhhhhhhhhhhhhhhh
Ph 1- naphtyl 2- naphthyl •o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p>to)yl 1- naphty) 2- naphthyl o-bipnenylyl · m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyt o-biphenylyl m-biphenylyl p-biphenyiyl Ph 1- naphtyl 2- naphthyl o-bipnenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl Orbiphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-blphenylyl
7J £223333333 R_ HHHHHHHHH-CH-CH-CH-CH-CH-CH-CH-CH-CHHHHH HHHH Η -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 Η Η Η Η Η Η DPA DPA DPA DPA DPA DPA Η Η Η Η Η Η ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ
Rol HH Η HH Η Η Η Η Η Η Η Η Η Η Η Η Η -CH3 -CH3 -CH3 •CH3 -CH3 -CH3 •CH3 -CH3 -CH3 •CH3 -CH3 -CH3 •CH3 •CH3 -CH3 -CH3 •CH3 -CH3 DPA DPA DPA DPA DPA DPA Η Η Η Η ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ Η· Η Η Η Η Η (請先閲讀背面之注意事項再填寫本頁) •裝· 訂 線 本紙法尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -81 - 581751 A7 B7 五、發明説明（ 79
o-biphenylyl (〇雎苯基） j H-278 〇〇 H-279 m-biphenylyl H-280 (m-聯苯基）η·281 H-282 p-biphenylyl H-283 ㈣玉基）H-284 H3C H-285 H-286 o-tolyl (°*甲苯基） .ch3
Rj Ph Ph Ph Ph Ph Ph Ph Ph 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1- naphthyl 2- naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl O-tolyly O-tolyly m-tolyly R2 ηηηη η ηηηηηηηηηηηηηη ηηηηηηηηη ηη ηηηη η η Η Η Η Η ηηηηηηηηηηηηηη Η ηηηηηηηηη ηη ηηηη η η ΗΗΗΗ ηηηηηη ΗΗΗΗΗΗΗΗΗ ηηηηηηηηη ηη ηηηη ηη
Rs 1- naphthyl 2- naphthyl o-biphenyly) m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl 2-naphthyl p-biphenylyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl o-biphenylyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl p-biphenylyl O-tolyly m-tolyl p-tolyl O-tolyly m-tolyl p-tolyl m-tolyl p-tolyl p-tolyl ^ Η Η Η Η Η ηηηηηηηηη ηη ηηηηηηηηη ΗΗ Η ΗΗ Η Η Η Η Η Η ^-- (請先閲讀背面之注意事項再填寫本頁) 訂 線 m-tolyl (m·田苯基） -〇ch3 p-tolyl (p·甲苯基） 本纸伕尺度適用中國國家標準（CNS ) Α4規格（210Χ297公釐） -82- 581751 A7 B7 經濟部智慧財4^7員工消黃合作钍印災 五、發明説明 (80 ) R1 r2 Rs Re r7 r8 Ι·1 Η H H H H H H l-2 Ph H H H Ph H H R1-\>R6 I-3 Ph Ph H H Ph H H r2-^>r5 1-4 Ph H H Ph Ph H H 1-5 Ph Ph H Ph Ph H H Q 1-6 Ph H Ph H Ph H H Ο Ο 1-7 Ph H H H Ph Ph H Typd 1-8 Ph H H H Ph H Ph R5-V/-R2 ρ 1-9 Ph H H H Ph Ph Ph MO Ph H H H Ph 1-naphthyl H Cx) M1 Ph H H H Ph H 1-naphthyl M2 Ph H H H Ph 1-naphthyl 1-naphthyl M3 Ph H H H Ph 2-naphthyl H CO M4 Ph H H H Ph H 2-naphthyl • 1-naph«iy丨（1-萘基） 1-15 Ph H H H Ph 2-naphthyl 2-naphthyl 卜16 Ph H H H Ph o-blphenylyl H OCX Μ 7 , Ph H H H Ph H o-biphenylyl 2-naphthyl (2-蔡基） 1-18 Ph H H H Ph o-biphenylyl o-biphenylyl Μ9 Ph H H H Ph m-biphenylyl H ob Ι-20 Ph H H H Ph H m-biphenylyl o-Wphenylyl (〇聯苯基） 1-21 Ph H H H Ph m-biphenylyl m-biphenylyl Ι-22 Ph H H H Ph p-biphenylyl H y-v/—( Ι-23 Ph H H H Ph H p-biphenylyl 1-24 Ph H H H Ph p-biphenylyl p-biphenylyl m-biphenylyl (m-聯本基） 1-25 1-naphthyl H H H 1-naphthyl H H 1-26 1-naphthyl Ph H H 1-naphthyl H H p-biphenyly丨（p·聯苯基} 1-27 1-naphthyl H H Ph 1-naphthyl H H 1-28 1-naphthyl Ph H Ph 1-naphthyl H H 1-29 1-naphthyl H Ph H 1-naphlhyl H H 卜30 1-naphthyl H H H 1-naphthyl Ph H 卜31 • 1-naphthyl H H H 1-naphthyl H Ph 1-32 1-naphthyl H H H 1-naphthyl Ph Ph 1-33 1-naphthyl H H H 1-naphthyl 1-naphthyl H 1-34 1-naphthyl H H H 1-naphthyl H 1-naphthyi 1-35 1-naphthyl H H H 1-naphlhyl 1-naphthyl 1-naphlhyl 1-36 1-naphthyl H H H 1-naphthyl 2-naphthyl H 1-37 1-naphthyl H H H 1-naphthyl H 2-naphthyl 1-38 1-naphthyl H H H 1-naphthyl 2-naphthyl 2-naphthyl 1-39 1-naphthyl H H H 1-naphthyl o-biphenylyl H 1-40 1-naphthyl H H H 1-naphthyl H o-biphenylyl 1-41 1-naphthyl H H H 1-naphthyl obiphenylyl o-biphenylyl Ι-42 1-naphthyl H H H 1-naphlhyl m-biphenylyl H M3 1-naphthyl H H H 1-naphlhyl H m-biphenylyl Ι-44 1-naphthyl H H H 1-naphthyl m-biphenylyl m-biphenylyl Μ5 1-naphthyl H H H 1-naphthyl p-biphenylyl H 1-46 1-naphthyl H H H 1-naphthyl H p-biphenylyl Μ7 1-naphthyl H H H 1-naphthyl p-biphenylyl p-biphenylyl 裝 訂 線 (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家揉準（CNS ) A4规格（210X297公釐） -83- 581751 A7 B7
1- naphthy丨（1-萘基）丨·59 1-60 C0 經濟部智慧財走局貨工消費合作社印災
Ri r2 r3 R5 Re r7 Re 2-naphthyl H H H 2-naphthyl H H 2-naphthyl Ph H H 2-naphthyl H H 2-naphthyl H H P\ 1 2-naphthyl H H 2-naphthyi Ph H PI· )2-naphthyl H H 2-naphthyl H Ph H 2-naphthyl H H 2-naphthyl H H H 2-naphthyl Ph H 2-naphthyl H H H 2-naphthyl H Ph 2-naphthyl H H H 2-naphthyl Ph Ph 2-naphthyl H H H 2-naphthyl 1-naphthyl H 2-naphthyl H H H 2-naphthyl H 1-naphthyl 2-naphthyl H H H 2-naphthyl 1-naphthyl 1 -naphthyl 2-naphthyl H H H 2-naphthyl 2-naphthyl H 2-naphthyl H H H 2-naphthyl H 2-naphthyl 2-naphthyl H H H 2-naphthyl 2-naphlhyl 2-naphthyi 2-naphthyl H H H 2-naphthyl o-biphenylyl H 2-naphthyl H H H 2-naphthyl H o-biphenylyl 2-naphthyl H H H 2-naphthyl o-biphenylyl o-biphenylyl 2-naphthyl H H H 2-naphlhyl m-biphenylyl H 2-naphthyl H H H 2-naph!hyl H m-biphenylyl 2-naphthyl H H H 2-naphthyl m-biphenylyl m-biphenylyl 2-naphthyl H H H 2-naphthyl p-biphenylyl H 2-naphthyl H H H 2-naphthyl H p-biphenylyl 2rnaphthyl H H H 2-naphthyl p-biphenylyl p-biphenylyl o-biphenylyl H H H o-biphenylyl H H o-biphenyly| Ph H H o-biphenylyl H H o-biphenylyl H H Ph o-biphenylyl H H o-biphenylyl Ph H Ph o-biphenylyl H H o-biphenylyl H Ph H o-biphenylyl H H o-biphenylyl H H H o-biphenylyl Ph H o-biphenylyl H H H o-biphenylyl H Ph o-biphenylyl H H H o-biphenylyl Ph Ph o-biphenylyl H H H o-biphenylyl 1-naphthyl H o-biphenyiyi H H H o-biphenylyi H 1-naphthyl o-blphenylyt H H H o-biphenylyl 1-naphthyl 1-naphthyl o-biphenylyl H H H o-biphenylyl 2-naphthyl H o-biphenylyl H H H o-biphenylyl H 2-naphthyl o-biphenylyl H H H o-biphenylyl 2-naphthyl 2-naphthyl o-blphenyly) H H H o-biphenylyl o-biphenylyl H o-biphenylyl H H H o-biphenylyl H o-biphenylyl o-biphenylyl H H H o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl H H H o-biphenylyl m-biphenylyl H o-blphenylyl H H H o-biphenylyl H m-biphenylyl o-biphenylyl H H H o-biphenylyl m-biphenylyl m-biphenylyl o-biphenylyl H H H o-biphenylyl p-biphenylyl H o-biphenylyl H H H o-biphenylyl H p-biphenylyl o-biphenylyl H H H o-biphenylyl p-biphenylyl p-biphenylyl ---------裝------訂------線 (請先閲讀背面之注意事項再填寫本頁) 五、發明説明（81 M8 I-49 I-50 1-51 1-52 1-53 1-54 1-55 1-56 1-57 !-58 (XX 丨-61 2- naphthy丨（2-萘基）μ62 [-63 o-b 丨::; o^biphenylyl (〇-聯苯基） )-66 ./ I-67 CVO I-68 m-biphenylyl (m·聯苯基}卜69 I-70 〇〇 丨71 p-biphenylyl (p·聯苯基） 卜72 卜73 I-74 !-75 I-76 I-77 Ι·78 Ι·79 Ι-80 1-81 Ι-82 Ι-83 Ι-84 Ι-85 丨·86 Ι·87 Ι·8Θ Ι-Θ9 1-90 1*91 I-S2 I-S3 本紙張尺度適用中國國豕榡率（CNS ) Α4規格（210x297公釐） -84- 581751 A7 B7 五、發明説明（82 )
Ri r2 r5 r6 r7 Rb 1-94 m-biphenylyl H H H m-biphenylyl H H W 1-95 m-biphenylyl Ph H H m-biphenylyl H H R1-\>R6 1-96 m-biphenylyl H H Ph m-biphenylyl H H R2-<>R5 1-97 m-biphenylyl Ph H Ph m-biphenylyl H H 1-98 m-biphenylyl H Ph H m-biphenylyl H H Q 1-99 m-biphenylyl H H H m-biphenylyl Ph H 〇 MOO m-biphenylyl H H H m-biphenylyl H Ph Typel ^ Jr M01 m-biphenylyl H H H m-biphenylyl Ph Ph rO 1-102 m-biphenylyl H H H m-biphenylyl 1-naphlhyl H Μ 03 m-biphenylyl •H H H m-biphenylyl H 1-naphthyl c: ώ Μ04 m-biphenylyl H H H m-biphenylyl 1-naphthyl 1-naphthyl R7 Re Μ 05 m-biphenylyl H H H m-biphenylyl 2-naphthyl H Μ 06 m-biphenylyl H H H m-biphenylyl H . 2-naphthyl 1-107 m-biphenylyl H H H m-biphenylyl 2-naphthyl 2-naphthyl 1-108 m-biphenylyl H H H m-biphenylyl o-biphenylyl H 1-109 m-biphenylyl H H H m-biphenylyl H o-biphenylyl 〇6 1-110 m-biphenylyl H H H m-biphenylyl o-biphenylyl o-biphenylyl 1-111 m-biphenylyl H H H m-biphenylyl m-biphenylyl H 1-naphthyl· (1-系圣） Μ12 m-biphenylyl H H H m-biphenylyl .H m-biphenylyl 1-113 m-biphenylyl H H H m-biphenylyl m-biphenylyl m-biphenylyl 1-114 m-biphenylyl H H H m-biphenylyl p-biphenylyl H 2-naphthyl (2·奈圣） Μ15 m-biphenylyl H H H m-biphenylyl H p-biphenylyl 1-116 m-biphenylyl H H H m-biphenylyl p-biphenylyl p-biphenylyl o«biphenyly丨（°·聯苯基) 1-117 p-bipheny(yl H H H p-biphenylyl H H orf Μ18 p-biphenylyl Ph H H p-biphenylyl H H 1-119 p-biphenylyl H H Ph p-biphenylyl H H m-biphenyly丨(m·聯苯基）卜 12D p-biphenylyl Ph H Ph p-biphenylyl H H 1-121 p-biphenylyl H Ph H p-biphenylyl H H Μ22 p-biphenylyl H H H p-biphenylyl Ph H phbiphepyly 丨(p·聯苯基） 卜123 p-biphenylyl H H H p-biphenylyl H Ph 1-124 p-biphenylyl H H H p-biphenylyl Ph Ph Μ 25 p-biphenylyl H H H p-biphenylyl 1-naphthyl H Μ 26 p-biphenylyl H H H p-biphenylyl H 1-naphthyl Μ27 p-biphenylyl H H H p-biphenylyl 1-naphthyl 1-naphthyl 1-128 p-biphenylyl H H H p-biphenylyl 2-naphthyl H 1-129 p-biphenylyl H H H p-biphenylyl H 2-naphthyl Μ30 p-biphenylyl H H H p-biphenylyl 2-naphthyl 2-naphthyl 1-131 p-biphenylyl H H H p-biphenylyl o-biphenyiyl H Μ 32 p-biphenylyl H H H p-biphenylyl· H o-biphenylyl Μ 33 p-biphenylyl H H H p-biphenylyl o-biphenylyl o-biphenylyl Μ 34 p-biphenylyl H H H p-biphenylyl m-biphenylyl H 1-135 p-biphenylyl H H H p-biphenylyl H m-biphenylyl Μ 36 p-biphenylyl H H H p-biphenylyl m-biphenylyl m-biphenylyl 1-137 p-biphenylyl H H H p-biphenylyl p-biphenylyl H 1-138 p-biphenylyl H H H p-biphenylyl H p-biphenylyl Μ39 p-biphenylyl H H H p-biphenylyl p-biphenylyl p-biphenylyl II 裝 I 訂 I I I線 (請先閲讀背面之注意事項再填寫本頁)· 本纸乐尺度適用中國國家標準（CNS ) A4说格（210X297公簸） -85- 581751 A7 B7 五、發明説明（83 ) R2 R3 ^5
1-140 1-141 M42 1-143 1-144 1-145 1-146 1-147 1-148 卜149 1-150 1-151 1-152 卜153 1-154 M55 1-156 1-157 1-158 1-159 〇y 刚 2-naphthyl (2-菜基）M61 1-162 1-163 ττ u —, , 1-164 α-biphenylyl (〇聯苯基） / 1-166 〇〇 丨-167 m-biphenylyl 1-168 C0 1-naphthyl (1-萊基） ob o-tolyl o-iolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl
H Ph H H * H H H H H H H H H H H H H H Ph H H H R H H H H H H H Ph H H H H H H H H H . H H H H H H H Ph
H H Ph H H H H H H H H H H H H H H H H Ph H Η H
H H H H H H H H
H H H H H H H H o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl otolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl R7 Re Η Η .Η Η Η Η Ph Η Η Ph 1-naphthyl Η Η 1-naphthyl 2-naphthyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p-biphenylyl
o-tolyl H H H H Ph H 1- naphthyl H 2- naphthyl H
H o-tolyl H H H H Ph H 1- naphthyl H 2- naphthyl H o-biphenylyl H (請先閲讀背面之注意事項再填寫本頁) .裝· ,11
o-tolyl (〇*甲苯基） CH3 m-tdyl m-tolyl o-biphenylyl m-tolyl H m-tolyl m-biphenylyl (m-甲苯基） -〇CH3 prolyl (p·甲苯基） 卜169 m-tolyl H H H · m-tolyl H m-biphenylyl 1-170 m-tolyl H H H m-tolyl p-biphenylyl H 1-171 m-tolyl H H H m-tolyl H p-biphenylyl 1-172 m-tolyl H H H m-tolyl m-toiyl H 1-173 m-tolyl H H H m-tolyl H m-tolyl 1-174 p-tolyl H H H p-tolyl H H Μ75 p-tolyf Ph H Ph p-tolyl H H 1-176 p-tolyl H Ph H p-tolyl H H 1-177 p-tolyl H H H p-tolyl Ph H 卜178 p-tolyl H H K p-tolyl H Ph 1-179 p-tolyl H H H p-tolyl 1-naphthyl H 1-180 p-tolyl · H H H p-tolyl H 1-naphthyl 1-181 p-tolyl H H H p*toly· 2-naphthyl H Μ 82 p-tolyl H H H p-tolyl H 2-naphthyl 1-183 p-tolyl H H H p-tdyl o-biphenylyl H 1-184 p-tolyl H H H p-tolyl H o-biphenylyl 1-185 p-tolyl H H H p-tolyl m-biphenylyl H 1-186 p-tolyl H H H p-tolyl H . m-biphenylyl Ι·187 p-tolyl H H H p-tolyl p-biphenylyl H 1-188 p-tolyl H H H p-tolyl H p-biphenylyl 1-189 p-lolyl H H H p-tolyl p-tolyl H 1-190 p-tolyl H H H p-tolyl H p-tolyl 線 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -86- 581751 A7 B7 五、發明説明（84 ) R2 R3 R5 Re r7 R81
M91 1-192 1-193 1-194 1-195 1-196 1-197 1-198 1-199 I-200 1-201 I-202 I-203 I-204 I-205 卜206 I-207 I-208 I-209 1-210 1-211 . 1-212 1-213 1-214 1-215 1-216 1-217 1-218 1-219 o-biphenylyl I-220 (〇·聯苯基）μ221 )-222 m-biphenylyl •卜 223 • (m-脚苯基、丨·224 Ι-225 C0 1-naphthyl d 2-naphthyl (2-^S) o-b o-biphenyly (o*fod ..... Ι-226 p-biphenylyl |227 (ρ聯苯基）丨-228 H3cw I-229 -Q I-230 o-tolyl (0-^¾¾) 1-231 CH3 1-232 1-233 m-tolyl J.235 广、 1-236 -〇-CH3 1-237 p*tc?lyl 訃甲茏基）1-238 1-239 DPA 溫
心g TPA 1-244 1-245 1-246 1-247 1-248 1-249 1-250
Ph 1- naphtyl 2- napht^l o-biphenylyl m-biphenylyl p-biphenylyl 0- tolyl m-toiyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-blphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2>naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl 0- tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl .Ph 1- naphtyl · 2- naphlhyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenyiyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl
H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H
-CH3 -CH3 -CH3 >CH3 -CH3 -CH3 -CH3 •CH3· •CH3 H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H H HHH HH hhhhhhhh h hhhhhhhh hhhhhhh h hh hhh hhhhhhhh hhhh h h hhhhhhhhhhh
Ph 1- naphtyl 2- naphthyJ 0- biphenylyl m-biphenyly! p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-bipnenyly! m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-faiphenylyl Ph 1- naphtyl 2- naphthyi o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphlyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl
H H H
H H H H -CH3 -CH3 •CH3 •CH3 -CH3 -CH3 -CH3 -CH3 -CH3 H H H H H H H H H •CH3 -CH3 -CH3 -CH3 •CH3 •CH3 •CH3 -CH3 -CH3 H H H H H H DPA DPA DPA DPA DPA DPA H H H H H H TPA TPA TPA TPA TPA TPA
HHHHH HHHHHHH Η Η HHHH
H3H3H3H3H3H3H3H3H3H3H3H3iHHHHHHPAPAPAH
HHHH (請先閲讀背面之注意事項再填寫本頁) 本紙乐尺度適用中國國家標準（CNS ) A4現格（210X297公釐） -87- 581751 A7 B7 五、發明説明（85 )
C0 1-naphthyl (1-蒂基） 2-naphthyl (2·系基）卜 I-\^r\J . I. o-biphenyly丨（《>%苯基）I. I· N—/V-/ |· m-biphenylyl (ηη·聯苯基）
卜286 Ri r2 r3 Rs r6 Ry Rs Ph H H. H 1-naphthyl H H Ph H H H 2-naphthyl H H Ph H H H o-biphenylyl H hi Ph H H H m-biphenylyl H H Ph H H H p-biphenylyl H H Ph H H H O-tolyly H H Ph H H H m-tolyl H H Ph H H H p-tolyl H H 1-naphthyl H H H 2-naphthyl H H 1-naphthyl H H H o-biphenylyl H H 1-naphthyl H H H m-biphenylyl H H 1-naphthyl H H H p-biphenylyl H H 1-naphthyl H H H O-tolyly H H 1-naphthyl H H H m-tolyl H H 1-naphthyl H H H p-tolyl H H 2-naphthyl H H H o-biphenylyl H H 2-naphthyl H H H m-biphenylyl H H 2-naphthyl H H H p-biphenylyl H H 2-naphthyl H H H O-tolyly H H 2-naphthyl H H H m-tolyl H H 2-naphthyl H H H p-tolyl H H o-biphenylyl H H H m-biphenylyl H H o-biphenylyl H H H p-biphenylyl H H o-biphenylyl H H H O-tolyly H H o-biphenylyl H H H m-tolyl H H o-biphenylyl H H H p-tolyl H H m-biphenylyl H H H p-biphenylyl H H m-biphenylyl H H H O-tolyly H H m-biphenylyl m-biphenylyl H H H H H H m-tolyl p-tolyl H H H H p-biphenylyl H .H H O-tolyly H H p-biphenylyl H H H m-toJyl H H p-biphenylyl H H H p-tolyl H H O-tolyly H H H m-tolyl H H O-tolyly H H H p-tolyl H H m-tolyly H H H p-tolyl H H (請先閱讀背面之注意事項再填寫本頁) -裝·
、1T 線 〇t〇|y| (〇甲苯基） ph3 m-tolyl (m•甲苯基） -〇CH3 · p-tplyl (ρ·甲苯基） •88- 本纸張尺度適用中國國家標隼（CNS ) Α4規格（210X297公釐） 581751 A7B7 五、發明説明（86 )
J-1 J-2 J-3 J-4 J-7 J-8 J-9 J-10 , J-11 C0 — J_12 1- naphthyl (1·蔡基）丄13 J-14 CCT 一 J·15 2- naphthyl (2-萘基）J-16 J-17ob Γΐ9 o-bipheny)y丨（〇聯苯基） J-20 / J-21 〇-〇 J-22 m-biphenylyl (m-聯苯基)j-23 J-24 p-biphenyly丨（P~聯苯基) J-25 J-26 J-27 J-28 J-29 J-30 J-31 J-32 J-33 J^4 J-35 J-36 J-37 J-38 J-39 J-40 J-41 J-42 J-43 J-44 J-45 J-46 J-47
Ri r2 R3 r5 Ry Re Η H H H H H H .Ph H H H Ph H H Ph Ph H H Ph H H Ph H •H Ph Ph H H Ph Ph H Ph Ph H H Ph H Ph H Ph H H Ph H H H Ph Ph H Ph H H H Ph H Ph Ph H H H Ph Ph Ph Ph H H H Ph 1-naphthyl H Ph H H H Ph H 1-naphthyl Ph H H H Ph 1-naphthyl 1-naphthyl Ph H H H Ph 2-naphthyl H Ph H H H Ph H 2-naphthyl Ph H H H Ph 2-naphtbyl 2-naphthyl Ph H H H Ph o-biphenylyl H Ph H H H Ph H o-biphenylyl Ph H H H Ph o-biphenylyl o-biphenylyl Ph H H H Ph m-biphenylyl H Ph H H H Ph H m-blphenylyl Ph H H H Ph m-biphenylyl m-biphenylyl Ph H H H Ph p-biphenylyl H Ph H H H Ph H p-biphenylyl Ph H H H Ph p-biphenylyl p-biphenylyl 1-naphthyl H H H 1-naphthyl H H 1-naphthyl Ph H H 1-naphthyl H H 1-naphthyl H H Ph 1-naphthyl H H 1-naphthyl Ph H Ph 1-naphthyl H H 1-naphthyl H Ph H 1-naphthyl H H 1-naphthyl H H H 1-naphthyl Ph H 1-naphthyl H H H 1-naphthyl H ' Ph 1-naphthyl H H H 1-naphthyl Ph Ph 1-naphthyl H H H 1-naphthyl 1-naphthyl H 1-naphthyl H H H 1-naphthyl H 1-naphthyl 1-naphthyl • H H H 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl H H H. 1-naphthyl 2-naphthyl H 1-naphthyl H H H 1-naphthyl H 2-naphthyl 1-naphthyl H H H 1-naphlhyl 2-naphthyl 2-naphthyl 1-naphthyl H H H 1-naphthyl o-biphenylyl H 1-naphthyl H H H 1-naphthyl H o-biphenylyl 1-naphthyl H H H 1-naphthyl o-biphenylyl o-biphenylyl 1-naphthyl H H H 1-naphthyl m-biphenylyl H 1-naphthyl H H H 1-naphthyl H m-biphenylyl 1-naphthyl · H H H 1-naphthyl m-blphenylyl m-biphenylyl 1-naphthyl H H H 1-naphthyl p-biphenylyl H 1-naphthyl H H H 1-naphthyl H p-biphenylyl 1-naphthyl H H H 1-naphthyl p-biphenylyl p-biphenylyl I 裝 訂 線 (請先閲讀背面之注意事項再填寫本頁) 泰紙張尺度適用中國國家標準（CMS ) A4規格（210X297公嫠） -89- 581751 A7 B7 五、發明説明（87 )
J-48 J-49 J-50 J-51 J-52 J-53 J-54 J-55 J-56 , J-57 J-58 1- naphthyl (1-萘基）上59 J-60CCX 如 2- naphthyl (2-蔡基） J-63 J-64 J-65 J-66 / J-67 CHD J-68 m-biphenylyl(m-聯苯基)」·69 J-70 o-biphenylyl (〇聯苯基广 p-biphenylyl (p·聯苯基) L· 卩ti J-71 J-72 J-73 J-74 J-75 J-76 J-77 J-78 J-79 J-80 J-81 J-82 J-83 J-84 J-85 J-86 J-87 J-88 J-89 J-90 J-91 J-92 J-93
Ri r2 r3 r5 Re r7 r8 2-naphihyl H H H 2-naphthyl H H 2-naphthyl Ph H H 2-naphthyJ H H 2-naphthyl H H Ph 2-naphthyl H H 2-naphthyl Ph H Ph 2-naphthyl H H 2-naphthyl H Ph H 2-naphthyl H H 2-naphthyl H H H 2-naphthyl Ph H 2-naphlhyl H H H 2-naphthyl .H Ph 2-naphthyl H H H 2-naphthyl Ph Ph 2-naphthyl H H H 2-naphthyl 1-naphthyl H 2-naphthyl H H H 2-naphthyl H 1-naphthyl 2-naphthyl H H H 2-naphthyl 1-naphthyl .1-naphthyl 2-naphthyl H H H 2-naphthyl 2-naphthyl H 2-naphthyl H H H 2-naphlhyl H 2-naphthyl 2-naphthyl H H H 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl H H . H 2-naphthyl o-biphenylyl H 2-naphthyl H H H 2-naphtiTyl H o-biphenylyl 2-naphthyl H H H 2-naphthyl o-biphenylyl o-biphenylyl 2-naphthyl H H H 2-naphthyl m-biphenylyl H 2-naphthyl H H H 2-naphthyl H m-biphenylyl 2-naphthyl H H H 2-naphthyl m-biphenylyl m-biphenylyl 2-naphthyl H H H 2-naphthyl p-biphenylyl H 2-naphthyl H H H 2-naphthyl H p-biphenylyl 2-naphthyl H H H 2-naphthyl p-biphenylyl p-biphenylyl o-biphenylyl H H H o-biphenylyl H H o-biphenylyl Ph H H o-biphenylyl H H o-biphenylyl H H Ph o-biphenylyl H H o-biphenylyl Ph H Ph o-biphenylyl H H o-biphenylyl H Ph H o-biphenylyl H H o-biphenylyl H H H o-biphenylyl Ph H o-biphenylyl H H H o-blphenylyl H Ph o-biphenylyl H H H o-biphenylyl Ph Ph o-biphenylyl H H H o-biphenylyl 1-naphthyl H o-biphenylyl H H H o-biphenylyl H 1-naphthyl o-biphenylyl H H H o-biphenylyl 1-naphthyl · 1-naphthyl o-biphenylyl H H H o-biphenylyl 2-naphthyl H o-biphenylyl H H H o-biphenylyl H 2-naphthyl o-biphenylyl H H H o-biphenylyl 2-naphthyl 2-naphthyl o-biphenylyl H H H o-biphenylyl o-biphenylyl H o-biphenylyl H H H o-biphenyiyl H o-biphenylyl o-biphenylyl H H H o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl H H H o-biphenylyl m-biphenylyl H o-biphenylyl H H H o-biphenylyl H m-biphenylyl o-biphenylyl H H H o-biphenylyl m-biphenylyl m-biphenylyl o-biphenylyl H H H o-biphenylyl p-biphenylyl H o-biphenylyl H H H o-biphenylyl H p-biphenylyl o-biphenylyl H H H o-biphenylyl p-biphenylyl p-biphenylyl 裝 訂 線 (請先閱讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -90 - 581751 A7 B7 五、發明説明（88 )
οό 1-naphlhy丨 U-萘基） 2-naph丨hy丨（2-蔡基） J-106 J-107 J-108 J-109 J-110 J-111 J-112 J-113 J-114 J-115 J-116
土 P ob o-biphenylyl (〇_聯苯基）J-117 」 J-118 〇〇 州19 nvbiphenylyl (m-聯苯基)J-120 J-121 GK> J-122 p-Wphenyly丨（p·聯苯基） J-124 J-125 J-126 J-127 J-128 J-129 J-130 J-131 J-132 J-133 J-134 J-135 J-136 J-137 J-138 J-139
Ri r2 Rs Re r7 '.Re m-biphenylyl H H H m-biphenylyl H H m-biphenylyl Ph H 卜I m-biphenylyl H H m-biphenylyl H H Ph m-biphenylyl H H m-biphenylyl Ph H Ph m-biphenylyl H H m-biphenylyl H Ph H m-biphenylyl H H m-biphenylyl H H H m-biphenylyl Ph H m-biphenylyl H H H m-biphenylyl H Ph m-biphenylyl H H H m-biphenylyl Ph Ph m-biphenylyl H H H m-biphenylyl 1-naphthyl H m-biphenylyl H H H m-biphenylyl H 1-naphthyl m-biphenylyl H H H m-biphenylyl 1-naphthyl 1-naphthyl m-biphenylyl H H H m-biphenylyl 2-naphthyl H m-biphenylyl H H H m-biphenylyl H 2-naphthyl m-biphenylyl H H H m-biphenylyl 2-naphthyl 2-naphthyl m-biphenylyl H H H m-biphenylyl o-biphenylyl H m-biphenylyl H H H m-biphenylyl H o-biphenylyl m-biphenylyl H H H m-biphenylyl o-biphenylyl o-biphenylyl m-biphenylyl H H H m-blphenylyl m-biphenylyl H m-biphenylyl H H H m-biphenylyl H m-biphenylyl m-blphenylyl H H H m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl H H H m-biphenylyl p-biphenylyl H m-biphenylyl H H H m-biphenylyl H p-biphenylyl m-biphenylyl H H H m-biphenyiyl p-biphenylyl p-biphenylyl p-biphenylyl H H H p-biphenylyl H H p-biphenylyl Ph H H p-biphenylyl H H p-biphenyiyl H H Ph p-biphenylyl H H p-biphenylyl Ph H Ph p-biphenylyl H H p-blphenylyl H Ph H p-biphenylyl H H p-biphenylyl H H H p>biphenyiyl Ph H p-biphenylyl H H H p-biphenylyl H Ph p-biphenylyl H H H p-biphenylyl * Ph Ph p-biphenylyl H H H p-biphenylyl 1-naphlhyl H p-blphenylyl H H H p-biphenylyl H 1-naphthyl p-biphenylyl H H H p-biphenylyj 1-naphthyl 1-naphthyl p-biphenylyl H H H p-biphenylyl 2-naphthyl H p-biphenylyl H H H p-biphenylyl H 2-naphthyl p-biphenylyl H H H p-biphenylyl 2-naphthyl 2-naphthyl p-biphenylyl H H H p-biphenylyl o-biphenylyl H p-biphenylyl H H H p-biphenylyl H o-biphenylyl p-biphenylyl H H H p-biphenylyl o-biphenylyl o-biphenylyl p-biphenylyl H H H p-biphenylyl m-biphenylyl H p-biphenylyl H H H p-biphenylyl H m-biphenylyl p-biphenylyl H H H p-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl H H H p-biphenylyl p-biphenylyl H p-biphenylyl H H H p-biphenylyl H p-biphenylyl p-biphenylyl H H H p-biphenylyl p-biphenylyl p-biphenylyl ---------批衣------、玎------線 (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -91 - 581751 A7 B7 五、發明説明（89 r7
C0 1-naphthyl α-蒂基） 2-naphthyl o-b o-biphenylj (o-d m-biphenylyl (m-聯苯基） p-biphenylyl otolyl (〇·甲苯基） PH3
I | (m·甲苯基） _-ch3 p-tolyl (p*田苯基） J-140 J-141 J-142 J-143 J-144 J-145 J-146 J-147 J-148 J-149 J-150 J-151 J-152 J-153 J-154 J-155 J-156 J-157 J-158 J-159 J-160 J-161 J-162 J-163 J-164 J-165 J-166 J-167 J-168 J-169 J-170 J-171 J-172 J-173 J-174 J-175 J-176 J-177 J-178 J-179 J-180 J-181 J-182 J-183 J-184 J-185 J-186 J-187 J-188 J-189 J-190 o-tolyl o-tolyl o»tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-toly! m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl p-to(yl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyi p-tolyl p-tolyl p-tolyl p-tolyl p-toly) p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl
H Ph H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H H
Η H H Ph Ph H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H H Ph Ph H H
H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H
H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H H o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl
H H H Ph H 1- naphthyl H 2- naphthyl H 0- biphenylyl H m-biphenylyl H p-biphenylyl H o-tolyl H H H H Ph H 1- naphthyl H 2- naphthyl H 0- biphenylyl H m-biphenylyl H p-biphenylyJ H m-tolyl H H H H Ph H 1- naphthyl H 2- naphthyl H o-biphenylyl H m-biphenylyl H p-biphenylyl H p-tolyl H H H H H Ph H 1- naphthyl H 2- naphthyl H 0- biphenylyl H m-biphenylyl H p-biphenylyl H o-tolyl H H H H Ph H 1- naphthyl H 2- naphthyl H 0- biphenylyl H m-biphenylyl H p-biphenylyl H m-tolyl H H H H Ph H 1- naphthyl H 2- naphthyl H o-biphenylyl H m-biphenylyl H p-biphenylyl H p-tolyl (請先閲讀背面之注意事項再填寫本頁) 本纸張尺度適用中國國家標準（CNS ) A4说格（210X297公釐） -92- 581751 A7 B7 五、發明説明（9〇 )
R5 Rg R7
R8I ι P h才 L h匚s. \ 土 J-191 J-192 J-193 J-194 J-195 J-196 J-197 J-19B J-199 J-200 J-201 J-202 J-203 J-204 J-205 J-206 J-207 J-208 , J-209 J-210GO j-211 J-212 1- naphthyl (1-蒂基）」213 J-214 J-215 2- naphthyl (2-mm) *J*216 J-217 J-218 J-219 J-220 J-221 J-222 J-223 J-224 J-225 J-226 J-227 J-228 J-229 J-230 J-231 J-232 J-233 J-234 J-235 J-236 J-237 J-238 J-239 J-240 J-241 J-242 J-243 J-244 J-245 J-246 J-247 J-248 J-249 J-250 ob o-biphenylyl (0-聯苯基)od m-biphenylyl (m-聯苯基）
p-biphenyiyl (p*聯苯基） H3C otolyl ί〇·甲苯基） CH3 nvtolyl <m·甲苯基） -〇ch3 p»tolyl (p·甲苯 ϊ)
DPA
TPA
Ph 1- naphlyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl 0- tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-blphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl 0- tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyi p-biphenylyl Ph 1- naphtyl 2- naphthyl oblphenyiyl m-biphenylyl p-biphenylyl Ph 1- naphlyl 2- naphthyl o-biphenylyl m-biphenylyi p-biphenylyl ^ HHH ΗΗ HHHHHHH Η Η HHH HHHHH Η HHH HHHH HHHHH HHHHHHHHHHHHHHHHHHHHHHHHH •CH3 Η Ph H -CH3 Η 1-naphtyl H -CH3 Η 2-naphthyl H •CH3 -CH3 Η Η o-biphenylyl m-biphenylyl H H •CH3 Η p-biphenylyl H -CH3 Η o-tolyl H •CH3 Η m-tolyl H •CH3 Η p-tolyl H Η Η Ph •CH3 Η • Η 1-naphtyl •CH3 Η Η 2-naphthyl -CH3 Η Η o-biphenylyl -CH3 Η Η m-biphenylyl •CH3 Η Η p-biphenylyl •CH3 Η Η o-tolyl •CH3 Η Η m-tolyl •CH3 Η Η p-tolyl •CH3 Η Η Ph H Η Η Η Η Η Η 1- naphtyl 2- naphthyl o-bipnenylyl H H H Η Η m-biphenylyl H Η Η p-biphenylyl H Η Η o-tolyl H Η Η m-tolyl H Η Η p-tolyl H Η Η Ph -CH3 Η Η 1-naphtyl -CH3 Η Η 2-naphthyl -CH3 Η Η o-biphenylyl -CH3. Η Η m-biphenylyl -CH3 Η Η p-biphenylyl -CH3 Η Η o-tolyl •CH3 Η Η m-tolyl •CH3 Η Η p-tolyl -CH3 Η Η Ph H Η Η 1-naphlyl H Η Η 2-naphlhyl H Η Η o-biphenylyl H Η Η m-biphenylyl H Η Η p-biphenylyl H Η Η Ph DPA Η Η 1-naphtyl DPA Η Η 2-naphthyl DPA Η Η Η Η o-biphenylyl m-biphenylyl DPA DPA Η Η p-biphenylyl DPA Η Η Ph H Η Η 1-naphtyl H Η Η Η Η 2-naphthyl o-biphenylyl H H Η Η m-biphenylyl H Η Η p-biphenylyl H Η Η Ph TPA Η Η 1-naphtyl TPA Η Η 2-naphthyl TPA Η Η o-biphenylyl TPA Η Η m-biphenylyl TPA Η Η p-biphenylyl TPA Η Η Η ΗΗ ηηηηηηηηη -C-C9-C:-CI-CI-CI-CH5-CH-CH-CH-CH-CHDPADPADPDPADPADPAHHHHH Η >ΑΑ A A A A tptptptptptphhhhhh HHH.cHH3iHH33-CH3:H3:H3:H3iH3:H3:H3;H3 (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） -93- 581751
7 A 五、發明説明（91 )
R2 R5 2-naphlhyl (2-蒂基）ob o-biphenylyl (〇·聯苯基）j-277od m-biphenyly丨（m·聯苯基） p»biphenylyl (p*脚苯基} j.284 h3c
Ri 〇6 1-naphthyl π·萘基） J-251 Ph J-252 Ph J-253 Ph J-254 Ph * J-255 Ph J-256 Ph J-257 Ph J-258 Ph J-259 1-naphthyl J-260 1-naphthyl J-261 1-naphthyl J-262 1-naphthyl J-263 1-naphthyl J-264 1-naphthyl J-265 1-naphthyl J-266 2-naphthyl J-267 2-naphthyl J-268 2-naphthyl J-269 2-naphthyl J-270 2-naphthyl J-271 2-naphthyl J-272 o-biphenylyl J-273 o-biphenylyl J-274 o-biphenylyl J-275 o-biphenylyl J-276 o-biphenylyl J-277 m-biphenylyl J-278 m-biphenylyl J-279 J-280 m-blphenylyl m-biphenylyl J-281 p-biphenylyl J-282 p-biphenylyl J-2B3 p-biphenylyl J-284 O-tolyly J-285 O-tolyly J-286 m-tolyly ηηηηηηηηηηηηηηηηηηη ηηηηηηηηηηη η ηηη η η ΗΗΗΗ ΗΗΗΗΗΗ ηηηηηηηηηηηηηηηηηη ηη Η Η Η Η Η Η Η 1 -naphthyl Η 2-naphthyl Η o-biphenylyl Η m-biphenylyl Η . p-biphenylyl Η O-tolyly Η m-tolyl Η p-tolyl Η 2-naphthyl Η d-biphenylyl Η m-biphenylyl Η p-biphenylyl Η O-tolyly Η m-tolyl Η Η p-tolyl o-biphenylyl Η m-biphenylyl Η p-biphenylyl Η O-tolyly Η m-tolyl Η p-tolyl Η m-biphenylyl Η p-biphenyJyl Η O-tolyly Η m-tolyl Η p-tolyl Η p-biphenylyl Η O-tolyly Η m-tolyl p-tolyl Η O-tolyJy Η m-tolyl Η p-tolyl Η m-tolyl Η p-tolyl Η p-tolyl ηηηηη ηηηηηηηη ηηη ηηηηηηηηηηηη ηη ηηηη ηη
Re ηηηη η ηηηηη ηηηηηηηη η ηηηηηηηηη ηη η ηηη η η (請先閲讀背面之注意事項再填寫本頁) -裝 訂 線 o-tolyl (〇*甲苯基） CH3
I I (m·甲苯基） _ -CH3 p-tolyl (p*甲苯基） 本紙伕尺度適用中國國家標準（CNS ) Α4規格（21 ΟΧ 297公釐） -94- 581751 A7 B7 五、發明説明（92 )
C0 1-naphthyl (1·系基） 2-naphthyl (2·莱基） ob o«bipheny丨yl (〇-聯苯基}
R1 r6 r7
Ra H Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph
Η H Η H Ph H Η H Ph H H Ph Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H
H H H Ph Ph H H H H H H H H H H H H H H H H H H H H Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph: Ph Ph H H H H H H Ph H Ph 1-naphthyl H 1- naphthyl 2- naphthyl H 2-naphthyl o-biphenylyl H o-biphenylyl m-biphenylyl H m-biphenylyl p-biphenylyl H p-biphenylyl H H H H H H H Ph Ph H 1-naphthyl 1- naphthyl H 2- naphthyl 2-naphthyl H o-biphenylyl o-biphenylyl H m-biphenylyl m-biphenylyl H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) Ό 3 L· 才L h 3 L ns. 土 p-biphenylyl (p·聯苯基） K-25 1-naphthyl H H H 1-naphthyl H H K-26 1-naphthyl Ph H H 1-naphthyl H H K-27 ' 1-naphthyl H H Ph 1-naphthyl H H K-28 1-naphthyl Ph H Ph 1-naphthyl H H K-29 1-naphthyl H Ph H 1-naphthyl H H K-30 1-naphthyl H H H 1-naphthyl Ph H K-31 1-naphthyl H H H 1-naphthyl H Ph K-32 1-naphthyl H H H 1-naphthyl Ph Ph K-33 1-naphthyl H H . H 1-naphthyl 1-naphthyl H Κ*34 1-naphthyl H H H 1-naphthyl H 1-naphthyl Κ-35 1-naphthyl H H H 1-naphthyl 1-naphthyl 1-naphthyl K-36 1-naphthyl H H H 1-naphthyl .2-naphthyl H Κ-37 1-naphthyl H H H 1-naphthyl' H 2-naphthyl Κ·38 1-naphthyl H H H 1-naphthyl 2-naphthyl 2-naphthyl Κ-39 1-naphthyl H H H 1-naphthyl o-biphenylyl H Κ-40 1-naphthyl H H H 1-naphthyl H o-biphenylyl Κ-41 1-naphthyl H H H 1-naphthyl o-biphenylyl o-biphenylyl Κ·42 1-naphthyl H H H 1-naphthyl m-biphenylyl H Κ-43 1-naphthyl H H H 1-naphthyl H m-biphenylyl Κ-44 1-naphthyl H H H 1-naphthyl m-biphenylyl m-biphenylyl Κ-45 1-naphthyl H H H 1-naphthyl p-biphenylyl H Κ-46 1-naphthyl H H H 1-naphthyl H p-biphenylyl Κ-47 1-naphthyl H · H H 1-naphthyl p-biphenylyl p-biphenylyl 本紙法尺度適用中國國家標準（CNS〉A4規格（210X29*7公釐） -95- 581751 A7 B7 五、發明説明（93 )
K-48 Κ-49 Κ-50 Κ-51
Re 00 1_napWhyl(i^§) 2-naphthyl (2-蒂基）ob o-biphenyly丨（〇-聯苯基） Κ-54 Κ-55 Κ-56 Κ·57 Κ·58 Κ-59 Κ-60 Κ-61 Κ-62 Κ-63 Κ-64 Κ-65 Κ-66· Κ-67 Κ·68 p-biphenylyl (ρ*聯苯基） Κ-71 Κ-72 Κ-73 Κ-74 Κ-75 Κ-76 Κ·77 Κ-7Β Κ-79 Κ-80 Κ-81 Κ·82 Κ-83 Κ-84 Κ-85 Κ-86 Κ-87 Κ-88 Κ·89 Κ-90 Κ-91 Κ·92 Κ-93 ^2 ^3 ^5 Οτ6 m-biphenylyl (m·聯苯基）κ·69 Κ-70 2-naphthy) H H H 2-naphthyl H H 2-naphthyl Ph H H 2-naphthyl H H 2-naphthyl H H Ph 2-naphthyl H H 2-naphthyl Ph H Ph 2-naphthyl H H 2-naphthyl H Ph H 2-naphthyl H H 2-naphthyl H H H 2-naphthyl Ph H 2-naphthyl H H H 2-naphthyl H Ph 2-naphthyl H H H 2-naphthyl Ph Ph 2-naphthyl H H H 2-naphthyl 1-naphthyl H 2-naphthyl H H H· 2-naphthyl H 1-naphthyl 2-naphthy) H H H 2-naphlhyl 1-naphthyl 1-naphthyl 2-naphthyl H H H 2-naphthyl 2-naphthyl H 2-naphlhyl H H H 2-naphthyl H 2-naphthyl 2-naphthyl H H H 2-naphlhyl 2-naphthyl 2-naphthyl 2-naphthyl H H H 2-naphthyl o-biphenylyl H 2-naphthyl H H H 2-naphlhyl H o-biphenylyl 2-naphthyl H H H 2-naphthyl o-biphenylyl o-biphenylyl 2-naphthyl H H H 2-naphthyl m-biphenylyl H 2-naphthyl H H H 2-naphthyl H m-biphenylyl 2-naphthyl H H H 2-naphthyl m-biphenylyl m-biphenylyl 2-naphthyl H H H 2-naphthyl p-biphenylyl H 2-naphthyl H H H 2-naphthyl H p-biphenylyl 2-naphthyl H H H 2-naphthyl p-biphenylyl p-biphenylyl o-biphenylyl H H. H o-biphenylyl H H o-biphenylyl Ph H H o-biphenylyl H H o-biphenylyl H H Ph o-biphenylyl H H o-biphenylyl Ph H Ph o-biphenylyl H H o-biphenylyl H Ph H o-biphenylyl H • H o-biphenylyl H H H o-biphenylyl Ph H o-biphenylyl H H H o-biphenylyl H Ph o-biphenylyl H H H o-biphenylyl Ph Ph o-biphenylyl H H H o-biphenylyl 1-naphthyl H o-biphenylyl H H H o-biphenylyl H 1-naphthyl o-biphenylyl H H H o-biphenylyl 1-naphthyl 1-naphthyl o-biphenylyl H H H o-biphenylyl 2-naphlhyl · H o-biphenylyl H H H o-blphenylyl H 2-naphthyl o-biphenylyl H H H o-biphenylyl 2-naphlhyl 2-naphthyl o-biphenylyl H H H o-biphenylyl o-biphenylyl H o-biphenylyl H H H o-biphenylyl H o-blphenylyl o-biphenylyl H H H o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl H H H o-biphenylyl m-biphenylyl H o-biphenylyl H H H o-biphenylyl H · m-biphenylyl o-biphenylyl H H H o-biphenylyl m-biphenylyl m-biphenylyl o-biphenylyl H H H o-biphenylyl p-biphenylyl H o-biphenylyl H H H o-biphenylyl H p-biphenylyl o-biphenylyl H H H o-biphenylyl p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CN’S ) A4規格（210X297公釐） -96 - 581751 A7 B7 五、發明説明（94 )
Ri
C0 1-naphthyl (ι·萘基） 2-naphthyl (2·荼基） K-94 K-95 K-96 K-97 K-98 K-99 K-100 K-101 K-102 K-103 K-104 K-105 K-106 K-107 K-108 K-109 K-110 K-111 K-112 K-113 K-114 K-115 K-116 / K-118 〇〇 K-119 m-biphenylyl K-120 (m-聯苯基）κ·121 K-122 p-biphenylyl Cp·聯苯基） K-123 K-124 Κ-125 Κ-126 Κ-127 Κ-128 Κ-129 Κ-130 Κ-131 Κ·132 Κ-133 Κ-134 Κ·135 Κ-136 Κ·137 Κ-138 Κ-139 m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-blphenyly! p>biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphehylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl
R hhhh^hh η ΗΗΉΗ HHHHHHHHHHH HHHH^HHHHHHHHHHHHHHH HHH R2HphHphHHHH HHHH HHHHHH.HHHHH HphHphHHHH HHHHHHHHHHHHHHH
r5 H H Ph Ph H H H H H H H H H H H H H H H H H H H H H Ph Ph H H H H H H H H H H H H H H H H H H H «6 Ry Re m-biphenylyl H H m-biphenylyl H H m-biphenylyl H H m-biphenylyl H H m-biphenylyl H H m-biphenylyl Ph H m-biphenylyl H Ph m-biphenylyl Ph Ph m-biphenylyl 1-naphthyl H m-biphenylyl H 1-naphthyl m-biphenylyl 1-naphthyl 1-naphthyl m-biphenylyl 2-naphthyl H m-biphenylyl H 2-naphthyl m-biphenylyl 2-naphthyl 2-naphthyl m-biphenylyl o-blphenylyl H m-biphenylyl H o-biphenylyl m-biphenylyl o-biphenylyl o-biphenylyl m-biphenylyl m-biphenylyl H m-biphenylyl H m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyj p-biphenylyl H m-biphenylyl H p-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl H H p-biphenylyl H H p-biphenylyJ H H p-biphenylyl H H p-biphenylyl H H p-biphenylyl Ph H p-biphenylyl H Ph p-biphenylyl Ph Ph p-biphenylyl 1-naphthyl H p-biphenylyl H 1-naphthyl p-biphenylyl 1-naphthyl 1-naphthyl p-biphenylyl 2-naphthyl H p-biphenylyl H 2-naphthyl p-blphenylyl 2-naphthyl 2-naphthyl p-biphenylyl o-biphenylyl H p-biphenylyl H o-biphenylyl p-biphenylyl o-biphenylyl o-biphenyly) p-biphenylyl m-biphenylyl H p-biphenylyl H m-biphenylyl p-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl H p-biphenylyl H p-biphenylyl p-biphenylyl p»biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 裝 訂 I I線
本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） 97 - 581751 A7 B7 五、發明説明（95 )
K-140 K-141 K-142 K-143 K-144 K-145 K-146 K-147 K-148 K-149 K-150 K-151 K-152 K-153 K-154 K-155 K-156 K-157 K-158 (1-萘基）Κ·159 〇y 請 2-naphthyl (2-莱基）K-162 Κ-163 Κ-164 〇ό 1-naphthyl o-biphenylyl (0·聯苯基) / Κ-166 〇-〇 Κ-167 m-biphenylyl Κ-168 (m·聯苯基）κ-169 〇〇- Κ-170 p-biphenylyl Κ-171 (ρ·聯苯基） H3C Κ-173 Ό Κ-174 >tolyl (〇·甲苯基）κ·175 .CH3 Γ\ Κ·176 ^\mm/ m-tolyl (m·田苯基} K-178 -〇"CH3 K-179 p-tolyl K.18〇 K-181 .K-182 K-183 K-184 K-185 Κ-1Θ6 K-1B7 K-188 K-189 K-190 Κ-165 Ri .r2 R3 Rfi R7 Re o-tolyl H H H o-tolyl H H o-tolyl Ph • H Ph o-tolyl H H o-tolyl H Ph H o-tolyl H H o-tolyl H H H o-tolyl Ph H o-tolyl H H H o-tolyl H Ph o-tolyl H H H o-tolyl 1-naphthyl H o-tolyl H H H o-tolyl H 1-naphthyl o-tolyl H H H o-tolyl 2-naphthyl H o-tolyl H H H o-tolyl H 2-naphthyl o-tolyl H H H o-tolyl o-biphenylyl H o-tolyl H H H o-tolyl H o-biphenylyl o-tolyl H H H o-tolyl m-biphenylyl H o-tolyl H H H o-tolyl H m-biphenylyl o-tolyl H H H o-tolyl p-biphenylyl H o-tolyl H H H o-tolyl H p-blphenylyl o-tolyl H H H o-tolyl o-tolyl H o-tolyl H H H o-tolyl H o-tolyl m-toly) H H H m-tolyl H H m-tolyl Ph H Ph m-tolyl H H m-tolyl H Ph H m-tolyl .H H m-tolyl H H H m-tolyl Ph H m-tolyl H H H m-tolyl H Ph m-tolyl H H H m-tolyl 1-naphthyl H m-tolyl H H H m-lolyl H 1-naphthyl m-tolyl H H H m-tolyl 2-naphlhyl H m-tolyl H H H m-tolyl H 2-naphlhyl m-tolyl H H H m-tolyl o-biphenyly] H m-tolyl H H H m-tolyl H o-biphenylyl m-tolyl H H H m-tolyl m-biphenylyl H m-tolyl H H H m-tolyl H m-biphenylyl m-tolyl H H H m-tolyl p-biphenylyl H m-tolyi H H H m-tolyl H p-biphenylyl m-tolyl H H H .m-tofyl m-toJyl H m-tolyl H H H m-tolyl H m-toiyl p-totyl H H H p-tolyl H H p-tolyl Ph H Ph p-tolyl H H p-toty) H Ph H p-tolyl H H p-tolyl H H H p-tolyl Ph H p-tolyl H H H p-toly! H Ph p-tolyl H H H p-lolyl 1-naphthyl .H p-tolyl H H H p-tolyl H 1-naphthyl p-tolyl H H H p-toly) 2-naphthyl H p-tolyf H H H p-tolyl H 2-naphihyl p-tolyl H H H p-tolyl o-biphenylyl H p-tolyl H H H p-tolyl H o-biphenylyl p-tolyl H H H p-tolyl m-biphenylyl H p-tolyl H H H p-tolyl H m-biphenylyl p-tolyl H H H p-toly! p-biphenylyl H p-tolyl H H H p-lolyl H p-biphenylyl p-tolyl H H H p-tolyl p-lolyl H p-tolyl H H H p-tolyl H p-tolyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標隼（CNS ) A4規格（210X29*7公釐） •98- 581751 A7 B7 五、發明説明（96 )
C0 1-naphthyl (i-^S) 2-naphthyl (2 ob o-biphenylyl (〇聯苯基） od m-biphenylyl (m-瞰苯基） Ri r2 K-191 Ph H K-192 1-naphtyl H K-193 2-naphthyl H K-194 K-195 o-biphenylyl m-biphenylyl .H K-196 p-biphenylyl H K-197 o-tolyl H K-198 m-tolyl H K-199 p-tolyl H K-200 Ph H K-201 1-naphtyl H K-202 2-naphthyl H K-203 o-biphenylyl H K-204 m-biphenylyl H K-205 p-biphenylyl H K-206 o-tolyl H K-207 m-tolyl H K-208 p-tolyl H K-209 Ph H K-210 K-211 K-212 1- naphtyl 2- naphthyl o-bipnenylyl H H H K-213 m-biphenylyl H K-214 p-biphenylyl H K-215 o-tolyl H K-216 m-tolyl H K-217 p-tolyl H K-218 Ph H K-219 1-naphtyl H K-220 2-naphthyl H K-221 o-biphenylyl H K-222 m-biphenylyl H K-223 p-biphenylyl H K-224 o-tolyl H· K-225 m-tolyl H R3 R6 R7
p-biphenylyl (P·鞄苯基） H3C •CH3 •CH3 •CH3 -CH3 -CH3 -CH3 •CH3 •CH3 -CH3 Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η m-tolyl (m 甲苯基） -〇ch3 p4olyl φ·田 s 基） DPA心g ΤΡΑ
K-226 K-227 Κ-228 p-tolyl Ph 1-naphtyl Η Η Η o-tolyl (〇甲苯基） ph3 K-229 K-230 2-naphlhyl o-biphenylyl H H H H K-231 m-biphenylyl H H K-232 p-biphenylyl H H K-233 Ph H H K-234 1-naphtyl H H K-235 2-naphthyl K-236 o-biphenylyl K-237 m-biphenylyl H H H H K-238 p-biphenylyl H H K-239 Ph H H K-240 1-naphlyl H H K-241 2-naphthyl H H K-242 o-biphenylyl H H K-243 m-biphenylyl H H K-244 p-biphenylyl H H K-245 Ph H H K-246 1-naphtyl H H K-247 2-naphthyl H H K-248 o-biphenylyl H H K-249 m-biphenylyl H H K-250 p-biphenylyl H H Η Η Η ΗΗ ηηηηηηη η η ηηη ηηηηη ηηηηηηηη η η η η η ηηηηηηηη ηηηη η η ηηηηηηηηηηη
Ph 1- naphtyl 2- naphlhyl o-biphenylyl m-bipheny)yl p-biphenylyl o-tolyl. m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenyiyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1-naphtyl 2-naphthyl o-biphenylyl m-bipheny(yl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Η Η Η ΗΗ Η Η Η Η 3 3 3 3 3 3 3 3 3 )Η:ΗΗ Η Η ηηηηηηηη -C-C-C-C-C-C-C.C-C卜 HJ- Η Η Η ΗΗ ΗΗΗΗΗΗΗΗ Η ΗΗΗΗ Η Η Η Η Η -CH3 •CH3 -CH3 •CH3 •CH3 •CH3 •CH3 -CH3 •CH3 Η Η Η Η Η Η DPA DPA DPA DPA DPA DPA Η Η Η Η Η Η ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ H3H3iH3H3H3H3H3H3H3H3H3H3lPAHHHH ηραιη ΗΗΗΗΗ (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X 297公釐） -99· 581751 五、發明説明（97 )
C0 1-naphthy丨（1-萊基)
2-naphthyl (2-系基)ob K-276 o-biphenylyl (〇·聯苯基)k-277 K-278 rVJ-i X-279 k-280 m-biphenylyl (m-琳苯基l K-281 厂K·282 K-283 p^biphenyly丨 苯基)K-284
H3C
Ri K-251 Ph K-252 Ph K-253 Ph K-254 Ph K-255 Ph K-256 Ph K-257 Ph K-258 Ph K-259 1-naphthyl K-260 1-naphthyl K-261 1-naphthyl K-262 1-naphthyl K-263 1-naphthyl K-264 1-naphthyl K-265 1-naphthyl K-266 2-naphthyl K-267 2-naphthyl K-268 2-naphthyl K-269 2-naphthyl K-270 2-naphthyl K-271 2-naphthyl K-272 o-biphenylyl K-273 o-biphenylyl K-274 o-biphenylyl K-275 o-biphenylyl o-biphenylyl m-rbiphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl O-tolyly K-285 OtolyJy K-286 m-tolyly R ΗΗΗΗ Η Η Η Η Η Η Η Η Η ΗΗΗΗ Η Η Η Η Η Η Η Η ΗΗ Η ΗΗ ΗΗΗΗ ΗΗ 7 7 A Β ^ ^ ΗΗΗΗ Η ηηηηηηηηηηηηηη η η η η η η ΗΗ η ΗΗ Η ΗΗΗ Η Η (請先閲讀背面之注意事項再填寫本頁) •裝· 訂 線
Rs_ Η 1-naphthyl H 2-naphthyi H o-biphenylyl H m-biphenylyl H p-biphenylyl Η O-tolyly H m-tolyl H p-tolyl H 2-naphthyl H o-biphenylyl H m-biphenylyl H p-biphenylyl H O-tolyly H m-tolyl H p-tolyl H o-biphenylyl H m-biphenylyl H p-biphenylyl H O-tolyly H m-tolyl H p-tolyl H m-biphenylyl H p-biphenylyl H O-tolyly H m-tolyl H p-tolyl H p-biphenylyl H O-tolyly H m-tolyl H p-tolyl H O-tolyly H m-tolyl H p-tolyl H m-tolyl H p-tolyl H p-t〇lyl Η Η Η Η Η Η Η ΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗ ΗΗ ΗΗΗΗ ΗΗ o-tolyl (〇·甲苯基） PH3 m-tolyl (πι-^*ϊ) ~〇"ch3 p-tolyl (p*田苯基） 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -1〇〇 - 581751 A7 B7 五、發明説明（98 )
C0 1-naphthyl (1-萘基） 2-naphthy丨（2-蔡基)
p^bipheny丨yl (p·聯苯基） 經濟部智慈財產局員工消費合作社印製 L-25 L-26 L-27 L-28 L-29 L-30 L-31 L-32 L-33 L-34 L-35 L-36 L-37 L-38 L-39 L-40 L-41 L*42 L43 L-44 L-45 L-46 L-47 r2 r3 R5 Re r7 Η H H H H H H Ph H H H Ph H H Ph .Ph H H Ph H. H Ph H H Ph Ph H H Ph Ph H Fh Ph H H Ph H Ph H Ph H H Ph H H H Ph .Ph H Ph H H H Ph H Ph Ph H H H Ph Ph Ph Ph · H H H Ph 1-naphthyl H Ph H H H Ph H 1-naphthyl Ph H H H Ph 1-naphthyl 1-naphthyl Ph H H H Ph 2-naphthyl H Ph H H H Ph H 2-naphthyl Ph H H H Ph 2-naphthyl 2-naphthyl Ph H H H Ph o-biphenylyl H Ph H H H Ph H o-biphenylyl Ph H H H Ph o-biphenylyl o-biphenylyl Ph H H H Ph m-biphenylyl H Ph H H H Ph H m-biphenylyl Ph H H H Ph m-biphenylyl m-biphenylyl Ph H H H Ph p-blphenylyl H Ph H H H Ph H p-biphenylyl Ph H H H Ph p-biphenylyl p-biphenylyl 1-naphthyl H H H 1-naphthyl H H 1-naphthyl Ph H H 1-naphthyl H H 1-naphthyl H H Ph 1-naphthyl H H 1-naphthyl Ph H Ph 1-naphthyl H H 1-naphthyl H Ph H 1-naphthyl H H 1-naphthyl H H H 1-naphthyl Ph H 1-naphthyl H H H 1-naphthyl H Ph 1-naphtfiyl H H H 1-naphthyl Ph Ph 1-naphthyl H H H 1-naphthyl 1-naphthyl H 1-naphthyl H H H 1-naphthyl H 1-naphthyl 1-naphthyl H H H 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl H H H 1-naphthyl 2-naphthyl H 1-naphthyl H H H 1-naphthyl H 2-naphthyl 1-naphthyl H H H 1-naphthyl 2-naphthyl 2-naphthyl 1-naphthyl H H H 1-naphthyl o-biphenylyl H 1-naphthyl H H H 1-naphthyl H o-biphenylyl 1-naphthyl H H H 1-naphthyl o-biphenylyl o-biphenylyl 1-naphthyl H H H 1-naphthyl m-biphenylyl H 1-naphthyl H H H 1-naphthyl H m-blphenylyl 1-naphthyl H H H 1-naphthyl m-biphenylyl m-biphenylyl 1-naphthyl H H H. 1-naphthyl p-biphenylyl H 1-naphthyl H H H 1-naphthyl H p-biphenylyl 1-naphthyl H H H 1-naphthyl p-Wphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 訂 本紙張尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） -101 - 581751 A7 B7 五、發明説明（99 )
Re 2-naphthy丨（2-蔡基）c-b 抑 o*biphenyly丨（〇>聯苯基）o-d m-biphenyly丨（m·聯苯基）l»69 經濟部智慧財產局員工消费合作社印製 C0 1-naphthyl (1-萘基） p-biphenyly丨（ρ»聯苯基） Ri r2 r3 r5 r6 R7 Re L-48 2-naphthyl H H H 2-naphthy) H H W9 2-naphthyl Ph H H 2-naphthyl H H L-50 2-naphthyl H H Ph 2-naphthyl H H L-51 · 2-naphthyl Ph H Ph 2-naphthyl H H L-52 2-naphthyl H Ph H 2-naphthyl H H b53 2-naphthyl H H H 2-naphthyl Ph H L-54 2-naphthyl H H H 2-naphthyl .H Ph L-55 2-naphlhyl H H H 2-naphlhyl Ph Ph L-56 2-naphthyl H H H 2-naphlhyl 1-naphthyl H L-57 2-naphthyl H H H 2-naphthyl H 1-naphthyl L-58 2-naphthyl H H H 2-naphthyl 1-naphthyl 1-naphthyl L-59 2-naphthyl H H H 2-naphthyl 2-naphthyl H L-60 2-naphthyl H H H 2-naphthyl H 2-naphthyl L-61 2-naphthyl H H H 2-naphthyl 2-naphthyl 2-naphthyl L-62 2-naphlhyl H H H 2-naphthyl o-biphenylyl H L-63 2-naphthyl H H H 2-naphthyl H o-biphenylyl L-64 2-naphthyl H H H 2-naphthyl o-biphenylyl o-blphenylyl L-65 2-naphthyl H H H 2-naphthyl m-biphenylyl H L-66 2-naphthyl H H H 2-naphthyl H m-biphenylyl L-67 2-naphthyl H H H 2-naphthyl m-biphenylyl m-biphenylyl L-68 2-naphthyl H H H 2-naphthyl p-biphenylyl H L-69 2-naphthyl H H H 2-naphthyl H p-biphenylyl L-70 2-naphthyl H H H 2-naphthyl p-biphenylyl p-biphenylyl L-71 o-biphenylyl H H H o-blphenylyl H H L-72 o-biphenylyl Ph H H o-biphenylyl H H L-73 o-biphenylyl H H Ph o-blphenylyl H H L-74 o-biphenylyl Ph H Ph o-biphenylyl H H L-75 o-biphenylyl H Ph H o-biphenylyl H H L-76 o-biphenylyl H H H o-biphenylyl Ph H L-77 o-biphenylyl H H H obiphenyJyl H Ph L-78 o-biphenylyl H H H o-biphenylyl Ph Ph L-79 o-biphenylyl H H H o-blphenylyl 1-naphthyl H L-80 o-biphenylyl H H H o-biphenylyl H 1-naphthyl L-81 o-blphenylyl H H H o-biphenylyl 1-naphthyl 1-naphthyl L-82 o-biphenylyl H H H o-biphenylyl 2-naphthyl H L-83 o-biphenylyl H H H o-biphenylyl H 2-naphthyl L-84 o-biphenylyl H H H o-biphenylyl 2-naphthyl 2-naphthyl L-B5 o-biphenylyl H H H o-biphenylyl o-biphenylyl H L-86 o-biphenylyl H H H o-biphenyly! H o-biphenylyl L-87 o-biphenylyl H H · H o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl H H H o-blphenylyl m-biphenylyl H L-89 o-biphenylyl H H H o-biphenylyl H m-biphenylyl L-90 o-biphenylyl H H H o-bipheny)yl m-biphenylyl m-biphenyJyl L-91 o-biphenylyl H H H o-biphenylyl p-biphenylyl H L-92 o-biphenylyl H H H o-biphenylyl H p-biphenylyl L-93 o-biphenylyl H H H o-biphenylyl p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) •訂 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -102- 581751 A7 B7 五、發明説明（100) 經濟部智慈財產局員工消費合作社印紫
Ri r2 r3 Rs r6 r7 rb · Rbr7 L-94 m-biphenylyl H H H m-biphenylyl H H c〇7 L-95 m-biphenylyl Ph H H m-biphenylyl H H L-96 m-biphenylyl H H Ph m-biphenylyl H H L-97 m-biphenylyl Ph H Ph m-biphenylyl H H L-98 m-biphenylyl H Ph H m-biphenylyl H H L-99 m-biphenylyl H H H m-biphenylyl Ph H C^R3R^6& L-IOO m-biphenylyl H H H m-biphenylyl H Ph TR^2 LTRe L-101 m-biphenylyl H H H m-blphenylyl Ph Ph TypcL L102 m-biphenylyl H H H m-biphenylyl 1-naphthyl H L-103 m-biphenylyl H H H m-biphenylyl H 1-naphthyl L-104 m-biphenylyl H H H m-biphenylyl 1-naphthyl 1-naphthyl L-105 m-biphenylyl H H H m-biphenylyl 2-naphthyl H L-1P6 m-biphenylyl H H H m-biphenylyl H 2-naphthyl L-107 m-biphenylyl H H H m-biphenylyl 2-naphthyl 2-naphthyl L-108 m-biphenylyl H H H m-biphenylyl o-blphenylyl H c0 1-naphthyl (卜蔡基） L-109 m-biphenylyl H H H m-biphenylyl H o-biphenylyl L-110 m-biphenylyl H H H m-blphenylyl o-biphenylyl o-biphenylyl L-111 m-biphenylyl H H H m-biphenylyl m-biphenylyl H 1-112 m-biphenylyl H H H m-biphenylyl H m-biphenylyl rvy L-113 m-biphenylyl H H H m-biphenylyl m-biphenylyl m-biphenylyl 2-naphthyl (2-萘基） L-114 m-biphenylyl H H H m-biphenylyl p-blphenylyl H L-115 m-biphenylyl H H H m-blphenylyl H p-biphenylyl L-116 m-biphenylyl H H H m-blphenylyl p-biphenylyl p-biphenylyl _ 雜)L-117 p-biphenylyl H H H p-biphenylyl H ..H 〇d L-118 p-biphenylyl Ph H H p-biphenylyl H H. L-119 p-biphenylyl H H Ph p-biphenylyl H 'H m-biphenyly丨（m-聯苯基） L-120 p-biphenylyl Ph H Ph p-biphenylyl H H L-121 p-biphenylyl H Ph. H p-biphenylyl H H L-122 p-biphenylyl H H H p-biphenylyl Ph H \mm/ 1—r^ p-biphenyly丨（p-聯苯基） 1 L-123 p-biphenylyl H H H p-biphenylyl H Ph L-124 p-biphenylyl H H H p-biphenylyl Ph Ph L-125 p-biphenylyl H H H p-biphenylyl 1-naphthyl H L-126 p-blphenylyl H H H p-blphenylyl H 1-naphthyl L-127 p-biphenylyl H H H p-biphenylyl 1-naphthyl 1-naphthyl L-12B p-biphenylyl H H H p-biphenylyl 2-naphthyl H L-129 p-biphenylyl H H H p-biphenylyl H 2-naphthyl L-130 p-biphenylyl H H H p-biphenylyl 2-naphthyl 2-naphthyl L-131 p-biphenylyl H H H p-biphenylyl o-biphenylyl H L-132 p-biphenylyl H H H p-biphenylyl H o-biphenylyl L-133 p-biphenylyl H H H p-biphenylyl o-biphenylyl o-biphenylyl L-134 p-biphenylyl H H H p-blphenylyl m-biphenylyl H L-135 p-biphenylyl H H H p-biphenylyl H m-biphenylyl L-136 p-biphenylyl H H H p-biphenylyl m-biphenylyl m-biphenylyl L-137 p-biphenylyl H H H p-biphenylyl p-biphenylyl H L-13B p-biphenylyl H H H p-blphenylyl · H p-biphenylyl , L-139 p-biphenylyl H H H p-biphenylyl p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁)
，1T 本紙張尺度適用中國國家標準（CNS ) Α4規格（210X297公釐） -103 - 581751 A7 B7 五、發明説明（101)
C0 卜naphthyl (I-萘基） 2-naphthyl (2·萘基) ob o-biphenylyl (〇·聯苯基） CKj m-biphenylyl (m-聯苯基)
p-biphenylyl (P-聯苯基） H3C o-tolyl (〇·甲苯基） CH3 經濟部智慧財產局員工消費合作社印髮 m-tolyj (m•甲苯基】 -〇ch3 p-tolyl (p·甲苯基） L-140 L-141 L-142 L-143 L-144 L-145 L-146 L-147 L-148 L-149 L-150 L-151 L-152 L-163 L-154 L-155 L-156 L-157 L-158 L-159 L-160 L-161 L-162 L-163 L-164 L-165 L-166 L-167 L-168 L-169 L170 L-171 L-172 L-173 L-174 L-175 L-176 L-177 L-178 L-179 L-180 L-181 L-182 L-183 L-184 L-185 L-186 L-187 L-188 L-189 L-190
Ri r2 R3 r5 Re R? Re o-tolyl H H H o-tolyl H H o-tolyl Ph H Ph o-tolyl H H o-tolyl H Ph H o-tolyl H H o-tolyl H H H o-tolyl Ph .H o-tolyl H H H o-tolyl H Ph o-tolyl H H H o-tolyl 1-naphthyl H o-tolyl H H H o-toJyJ H 1-naphthyl o-tolyl H H H o-tolyl 2-naphthyl H o-tolyl H H H o-tolyl H 2-naphthyl o-tolyl H H H o-tolyl o-biphenylyl H o-tolyl H H H o-tolyl H o-biphenylyl o-tolyl H H H o-tolyl m-biphenylyl H o-tolyl H H H o-tolyl H m-biphenylyl o-tolyl H H H o-tolyl p-blphenylyl H o-tolyl H H H o-tolyl H p-biphenyJyl o-tolyl H H H o-tolyl o-tolyl H o-tolyl H H H o-tolyl H o-tolyl m-tolyl H H H m-tolyl H H m-tolyl Ph H Ph m-tolyl H H m-tolyl H Ph H m-tolyl H H m-tolyl H H H m-tolyl Ph H m-tolyl H H H m-tolyl H Ph m-tolyl H H H m-tolyl 1-naphthyl H m-tolyl H H H m-tolyl H 1-naphthyl m-tolyl H H H m-tolyl 2-naphthyl .H m-toJy) H H H m-tolyl H 2-naphthyl m-tolyl H H H m-tolyl o-biphenylyl H m-tblyl H H H m-tolyl H o-biphenylyl m-tolyl H H H m-tolyl m-biphenylyl H m-tolyl H H H m-tolyl H m-biphenylyl m-tolyl H H H m-tolyl p-biphenylyl H m-tolyl H H H m-tolyl H p-biphenylyl m-tolyl H H H m-tolyl m-tolyl H m-tolyl H H H m-tolyl H m-tolyl p-tolyl H H H p-tolyl H H p-tolyl Ph H Ph p-tolyl H H p-toiyl H Ph H p-tolyl H H p-tolyl H H H p-tolyl Ph H p-tolyl H H H p-tolyl H Ph’ p-tolyl H H H p-tolyl 1-naphthyl H p-tolyl H H H p-tolyl H 1-naphthyl p-tolyl H H H p-tolyl 2-naphthyl H p-tolyl H H H p-tolyl H 2-naphthyl p-tolyl H H H p-tolyl o-biphenylyl H p-tolyl H H H p-tolyl H o-biphenylyl p-tolyl H H H p-tolyl m-biphenylyl H p-tolyl H H H p-tolyi H m-biphenylyl p-tolyl H H H p-tolyl p-biphenylyl H p-tolyl H H H p-tolyl H p-biphenylyl p-toJyl H H H p-tolyl p-tolyl H p-tolyl H H H p-tolyl H p-toly! (請先閲讀背面之注意事項再填寫本頁)
、1T 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） • 104 - 581751 A7 B7 五、發明説明（102)
Ri R2 R3 R5 Rfi o^w
C0 1- naphthy丨（i-萘基)ccr 2- naphthy 丨(2·莱基） ob o-biphenylyl (O聯苯基) o-d m-biphenylyl. (m-聯苯基） p-biphenylyl (p-聯苯基） o*tolyl (〇·甲苯基） CH3 經濟部智慧財產局員工消費合作社印製 L-204 L-205 L-206 L-207 L.208 L-209 L-210 L-211 L-212 L-213 L-214 L-215 L-216 L-217 L-218 L-219 L-220 L-221 L-222 L-223 L-224 L-225 L-226 L-227 L-228 L-229 L-230 L-231 L-232 L-233 L-234 L-235 L-236 L-237
Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-toiyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-blphenylyl 0- tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenyiyl
H -CH3 H -CH3 H -CH3 H -CH3 H -CH3 H -CH3 H -CH3 H -CH3 H -CH3 Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H m-toly丨⑼甲苯基） -〇ch3 prolyl (P·甲苯基） L-238 p-biphenyiyl L-239 Ph α,ο L-240 L-241 1- naphtyl 2- naphthyl D丨PA L-242 o-biphenylyl L-243 m-biphenylyl L-244 p-biphenylyl L-246 Ph L-246 1-naphtyl L-247 2-naphthyl TPA L-248 o-biphenylyl L-249 m-biphenyly! L-250 p-biphenylvl
hhhhhhh h hhhhh hhh hhh h h hhhh h h hhhhhhhhhhh H HHH HH Η Η HH HHH HHHHHHHH HHHH Η H HHHHHHHHHHH hhhhh hhhh hhhhh hhh hhhhh hhhhhhh h hhhhh hhhhhhhh hhhh h h hhhhhhhhhhh
Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-bipherryly! o-tolyl p-to)y) Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-lolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-blphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-bipherylyl p-biphenyJyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-blphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p：biphenylyl
HHHHH HH HH
h3h3h3h3h3h3h3h33 -C-C-CH?-CH-CH-CH-CH-CH
HHHHH HHHHHHH Η H HHHH hhhh
H3H3H3H3 9-cCHCH --I I (請先閲讀背面之注意事項再填寫本頁) 13133 33333 3 hhhhh,h:hh H H hhhh 9-c.c.c.c-c-c.c-c
H HHH Η H
A AAAA A p pppp p D DDDD D
H HHHHH
^A^A>A>AA A p p p p p p 丁 T 丁丁丁 T
-CH3 •CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 •CH3 -CH3 -CH3 DPA DPA DPA DPA DPA DPA H H H H H H TPA TPA TPA TPA TPA TPA H H H H H H
*1T 本紙張尺度適用中國國家標準（CNS )八私見格（210X29*7公釐） -105 - 581751 A7 B7 五、發明説明（1〇3)
C0 1-naphthyl (】-萘基）
2-naphthyl α-ΨΜ) ob o-bipJieny 丨y|r〇·聯苯基） od m-biphenyly丨 fm-聯苯基） p-biphenylyl (p·聯苯基） Ri r2 r3 Rs r6 r7 Re L-251 Ph H H H 1-naphthyl H H L-252 Ph H H H 2-naphthyl H H L-253 Ph H H H o-biphenylyl H H 卜254 Ph H H H m-biphenylyi H H L-255 Ph H H H . p-biphenylyl H H L-256 Ph H H H O-tolyly H H L-257 Ph H H H m-tolyl H H L-25B Ph H H H p-tolyl H H U259 1-naphthyl H H H 2-naphthyl H H L-260 1-naphthyl H H H o-biphenylyl H H L-261 1-naphthyl H H H m-biphenylyl H H L-262 1-naphthyl H H H . p-biphenylyl H H L-263 1-naphthyl H H H Otolyly H H L-264 1-naphthyl H H H m-tolyl H H L-265 1-naphthyl H H H p-tolyl H H L-266 2-naphthyl H H H o-biphenylyl H H L-267 2-naphthyl H H H m-biphenylyl H H L-268 2-naphthyl H H H p-biphenylyl. H H L-269 2-naphthyl H H H O-tolyly H H L-270 2-naphthyl H H H m-tolyl H H L-271 2-naphthyl H H H p-tolyl H H L-272 o-bipheny)yl H H H m-biphenylyl H H L-273 o-biphenylyl H H H p-biphenylyl H H L-274 o-biphenylyl H H H O-tolyly H H L-275 o-biphenylyl H H H m-tolyl H H L-276 o-biphenylyl H H H p-tolyl H H L-277 m-biphenylyl H H H p-biphenylyl H H L-278 m-biphenylyl H H H O-tolyly H H L-279 m-biphenylyl H H H m-tolyl H H L-280 m-biphenylyl H H H p-tolyl H H L-281 p-biphenylyl H H H O-tolyly H H L-282 p-biphenylyl H H H m-tolyl H H L-283 p-biphenylyl H H H p-tolyl H H L-284 O-tolyly H H H m-tolyl H H L-285 0-tolyly H H H p-tolyl H H L-286 m-tolyly H H H p-tolyl H H (請先閲讀背面之注意事項再填寫本頁) 訂 經濟部智慧財產局員工消費合作社印製 o-tolyl (°*年苯基） ch3 rrvtoly丨（m-甲苯基） -〇ch3 p-tolyl (p·甲苯基） 本紙張尺度適用中國國家標隼（CNS ) A4規格（210X297公釐） -106 - 581751 A7B7 五、發明説明（104) p2 R7 R R5 R4 R3
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經濟部智慈財產局員工消費合作社印製
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(請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -112- 581751 A7 B7 五、發明説明（11〇) R3R4
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od 經濟部智慈財產局員工消黃合作社印製 〇6 1-naphlhy丨（〗-萊基） 2-naphthyl (2·蔡基） ob o-biphenyly丨（°*聯苯基） p-biphenyly丨（p-聯苯基〉 Ri 0-1 Η 0-2 Ph 03 Ph 0-4 Ph 0·5 Ph 0-6 Ph 0-7 Ph 0-8 Ph 0-9 Ph 0-10 Ph 0-11 Ph 0-12 Ph 0-13 Ph 0-14 Ph 0-15 Ph 0-16 Ph 0-17 Ph 0-18 Ph 0-19 Ph 0-20 Ph 0-21 Ph 0-22 Ph 0-23 Ph 0-24 Ph 0-25 1-naphthyl 026 1-naphthyl 0-27 1-naphthyl 0-28 1-naphthyl 0-29 1-naphthyl 0-30 1-naphthyl 0-31 1-naphthyl 0-32 . 1-naphthyl 0-33 1-naphthyl 0-34 1-naphthyl 0-35 1-naphthyl 0-36 1-naphthyl 0-37 1-naphthyl 0-38 1-naphthyl 0·39 1-naphthyl 0-40 1-naphthyl 0-41 1-naphthyl 0-42 1-naphthyl 0-43 1-naphthyl 0-44 1-naphthyl 0-45 1-naphthyl 0-46 1-naphthyl 0-47 1-naphthyl ηηη^η^ηηη η η η ηηηηηηηηηηηη η η ^η^ηηη η η η η ηηηηηηηη ηηη ηηη^^ηηηη ηηη ηηηηηηηηηηηη ηη ^^ηηηη η η η η η η η η η ηηη ηηη ηηηηηηηηηηηη ηηηηηηηηηηηη ηηηηηηηηηηηη ηηηηηηηη ηηη p4 R2 R5 r7 H H H H H H Ph H H H H H H H H H H H H Ph H H H Ph H Ph Ph H 1-naphthyl H H H 1-naphthyl H 1-naphthyl 1-naphthyl H 2-naphthyl H H H 2-naphthyl H 2-naphlhyl 2-naphlhyl H o-biphenylyl H H H o-biphenylyl H o-biphenylyl obiphenylyl H m-biphenylyl H H H m-biphenylyl H m-faiphenylyl m-biphenylyl H p-biphenylyl H H H p-biphenylyl H p-biphenylyl p-biphenylyl H H H Ph H H H H H H H H H H H H Ph H H H Ph H Ph Ph H 1-naphthyl H H H 1-naphthyl H 1-naphthyl 1-naphthyl H 2-naphlhyl H H H 2-naphthyl H 2-naphthyl 2-naphthyl H o-biphenylyl H H H o-biphenylyl H o-biphenylyl o-biphenylyl H m-biphenylyl H H H m-biphenylyl H m-biphenylyl m-biphenylyl H p-biphenylyl H H H p-biphenylyl H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 訂 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -119- 581751 A7 B7 五、發明説明（117) R1
TypeO C0 1-naph丨hyl (】·萘基） 2-naphthy丨（2_萘基）ob o«biphenyly丨（〇·聯苯基） 0-4B 0-49 0-50 0-51 0-52 0·53 0-54 0-55 0-56 0-67 0-58 0-59 0-60 0-61 0-62 0-63 0-64 0-65 0-66 0-67 0-68 od m-biphenylyl (m-聯苯基）〇·69 0-70 2-naphthyl 2-naphlhyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl
Kipl!^ylyl(p·聯苯基）〇-71 °^phe_ 0-72 o-b·丨 phenylyl 經濟部智慧財產局員工消资合作社印製
0-73 o-biphenylyl H 0-74 o-biphenylyl H 0-75 o-biphenylyl H 0-76 o-biphenylyl H 0-77 o-biphenylyl h 0-78 o-biphenylyl h 0-79 o-biphenylyl h o-biphenylyl H o-biphenylyl H 0-82 〇-bipheny)yl H 0-83 o-biphenylyl H 0-84 〇-biphenylyl h 0-85 o-biphenylyl h 0-86 o-biphenylyl H 0^7 o-biphenylyl H 0-88 o-biphenylyl H 0-89 o-biphenylyl H 0-90 o-biphenyJyl H 0-91 o-biphenylyl H 0-92 o-biphenylyl H 0-93 o-biphenylyl H
HphHHHHHH'HHHHHHHHHHHHHHH Hph R3 R4 r5 Ry Re Η Η Η Η H Η Η Ph Η H Ph Ph Η Η H Ph Η Η Η H Η Ph Η Η H Η Η Η Ph H Η Η Η Η Ph Η Η Η Ph Ph Η Η Η 1-naphthyl H Η Η Η Η 1-naphthyl Η Η Η 1-naphthyl 1-naphthyl Η Η Η 2-naphthyl H Η Η Η Η 2-naphthyl Η Η Η 2-naphthyl 2-naphthyl Η Η Η. o-biphenylyl H Η Η Η Η o-biphenylyl Η Η Η o-biphenylyl o-biphenylyl Η Η Η m-biphenylyl H Η Η Η H m-biphenylyl Η Η Η m-biphenylyl m-biphenylyl Η Η Η p-biphenylyl H Η Η Η H p-biphenyJyl Η Η Η p-biphenylyl p-biphenylyl Η Η Η H H Η Η Ph H · H Ph Ph Η H H Ph Η Η H H Η Ph Η H H Η Η Η Ph H Η Η Η H Ph Η Η Η Ph Ph Η Η Η 1-naphthyl H Η Η Η H 1-naphthyl Η Η Η 1-naphthyl 1-naphthyl Η Η Η 2-naphthyl H Η Η Η H 2-naphthyl Η Η Η 2-naphthyl 2-naphthyl Η Η Η o-biphenylyl H Η Η Η H o-biphenylyl Η Η Η o-biphenylyl o-biphenylyl Η Η Η m-biphenylyl H Η Η Η H m-biphenylyl Η Η Η m-biphenylyl m-biphenylyl Η Η Η p-biphenylyl H Η Η Η H p-biphenyJyl Η Η Η p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 訂 本紙悵尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） -120- 581751
7 7 A B 五、發明説明（118)
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0-94 0-95 0-96 0-97 0-98 0-99 0-100 0-101 0-102 0-103 0-104 1- naphthyl (i-系基〕0-105 0-106 0-107 2- naphthyl (2-萊基）0-108 v 0-109 ob = o-biphenylyl CM” (〇聯苯基）0-112 °·113 WV-/ 0-114 傘?工苯基)〇·”5 0-116 C0
m-biphenylyl H m-biphenylyl Ph m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl h m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyi H 經濟部智慧財1局員工消費合作社印製 p-blphenylyl (p-聯苯基） 0-117 0-118 0-119 0-120 0-121 0-122 0-123 0-124 0-125 0-126 0127 0-128 0-129 0-130 0-131 0-132 0-133 0-134 0-135 0-136 0-137 0-138 0-139 p-biphenylyl p-blphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl
H Ph H H H H H H H H H H H H H H H H H H H H H Η l· U. Η Η phphHHH Η ηηηηηηηηηηηηηηη Η Η Η Η Η Η ΗΗΗΗΗΗΗΗ Η Η Η H Η Ph Η H Ph Η Η H Η Η Η H Ph Η Η H Η Η Ph H Η Η Η Ph Η Η Ph Ph Η Η 1-naphlhyl H Η Η Η 1-naphthyl Η Η 1-naphthyl 1-naphthyl Η Η 2-naphthyl H Η Η Η 2-naphthyl Η Η 2-naphthyl 2-naphthyl Η Η o-biphenylyl H Η Η Η o-biphenylyl Η Η o-biphenylyl o-biphenylyl Η Η m-biphenylyl H Η Η H m-biphenylyl Η Η m-biphenylyl m-biphenylyl Η Η p-biphenylyl H Η Η H p-biphenylyl Η Η p-biphenylyl p-biphenylyl Η Η H H Η Ph H H Ph Η H H Η Η H H Ph .Η H H Η Η Ph H Η Η H Ph Η Η Ph Ph Η Η 1-naphthyl H Η Η H 1-naphthyl Η Η 1-naphthyl 1-naphthyl Η Η 2-naphthyl H Η Η H 2-naphthyl Η Η 2-naphthyl 2-naphthyl Η Η o-biphenylyl H Η Η H o-biphenylyl Η Η o-biphenylyl o-biphenylyl Η Η m-biphenylyl H Η Η H m-biphenylyl Η Η m-biphenylyl m-biphenylyl Η Η p-biphenylyl H Η Η H p-biphenylyl Η Η p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 訂 本紙張尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） -121 - 581751
A B7 五、發明説明（119)
TypcO 〇6 od· oo p-biphenylyl 經濟部智慧財產局員工消費合作社印製 1-naphthyl (1·蔡基） 2-naphthyl (2·菜基） o-b o-biphenylyl (0-聯本基） m-biphenylyl (m·聯苯基） (P·聯苯基) 〇_t〇|y| (〇·甲苯基） CH3 rrvtolyl⑻-甲苯基） -〇ch3 prolyl (p*甲苯基） Ri 0-140 o-tolyl 0-141 o-tolyl 0-142 o-tolyl 0143 o-tolyl 0-144 o-tolyl 0-145 o-tolyl 0-146 o-tolyl 0-147 o-tolyl 0-148 o-tolyl 0-149 o-tolyl 0150 o-tolyl 6-151 * o-tolyl 0-152 o-tolyl 0-153 o-tolyl 0-154 o-tolyl 0-155 o-tolyl 0-156 o-tolyl 0-157 m-tolyl 0-158 m-tolyl 0-159 m-tolyl 0-160 m-tolyl 0-161 m-tolyl 0-162 m-tolyl 0-163 m-tolyl 0-164 m-tolyl 0-165 m-tolyl 0-166 m-tolyl 0-167 m-tolyl 0-168 m-tolyl 0-169 m-tolyl 0-170 m-tolyl 0-171 m-tolyl 0-172 m-tolyl 0-173 m-tolyl 0-174 p-tolyl 0-175 p-tolyl 0-176 p-tolyl 0-177 p-tolyl 0-178 p-tolyl 0179 p-tolyl 0-180 p-tolyl 0-181 p-tolyl 0-182 p-tplyl 0-183 p-tolyl 0·1Β4 p-tolyl 0-185 p-tolyl CM 86 p-tolyl 0-187 p-tolyl 0-188 p-tolyl 0-189 p-tolyl 0-190 p-tolyl R2 Η ^ηηη ηηηηηηηηηηηηηη ηηηηηηηηηηηηηηη η^ηηηηηηηηηηηηηηη Η ^ηηη ηηηηηηηηηηηηη^ ηηηηηηηηηηηηηηη η^ηηηηηηηηηηηηηηη R41 Η HphHH ΗΗΗΗ HHHHHHHHHHphHHHHHHHHHHHHHH ΗΗ^ΗΗΗΗΗΗΗΗΗΗΗΗΗΗ Η η^ηη ηηηηηηηηηηηηηη ηηηηηηηηηηηηηηη ηη ^ηηηηηη ηηηηηηηη R8 Η Η Η Η Η Η Ph Η Η Ph 1-naphthyl Η Η 1-naphthyl 2-naphthy! Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p-biphenylyl o-tolyl Η Η o-tolyl Η Η Η Η Η Η Ph Η Η Ph 1-naphthyl Η Η 1-naphthyl 2-naphthyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p-biphenylyl m-tolyl Η Η m-tolyl Η Η Η Η Η Η Ph Η Η Ph 1-naphthyl Η Η 1-naphthyl 2-naphthyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p-biphenylyl p-tolyl Η Η p-tolyl -- (請先閲讀背面之注意事項再填寫本頁) 訂 I# 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -122 581751 經濟部智慧財產局員工消骨合作社印製 五、發明説明（120)
TypeO C0
Ri A7 Ph 1- naphtyl 2- naphthyl Β7 r2 r3 R4 Η •CH3 -CH3 Η -CH3 -CH3 Η -CH3 -CH3 Β •CH3 -CH3 -CH3 -CH3 Η •CH3 -CH3 Η -CH3 -CH3 Η -CH3 -CH3 Η •CH3 -CH3 Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η
Η HH HH HHHHHHH Η Η HHH HHHHH HHHHHHH H HHHHH HHHHHHHH HHHH Η Η HHHHHHHHHHH R7
Re
3 3 3 3 3 3 3 3 3 hhhhhhhh hhhhh Η Η H HH HHHH99-C-C-C-C-C-C-CHH HH
H H H H H H H H H H H H H H H H H •CH3 -CH3 -CH3 -CH3 -CH3 •CH3 •CH3 •CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 •CH3 -CH3 -CH3 •CH3 DPA DPA DPA DPA DPA DPA H H H · H H H TPA TPA TPA TPA TPA TPA H H H H H H 0-191 0-192 0-193 0-194 0-195 0-196 0-197 0-198 0-199 0-200 0-201 0-202 0-203 0-204 0-205 0-206 0-207 0-208 0-209 0-210 0-211 0-2 -212 0-213 0-214 0-215 ,0-216 0-217 v 0-218 〇〇 〇·219 Orbiphenylyl 0-220 (〇·聯苯基)0·221 0-222 n-biphenylyl 0-223 (m-聯苯基）0-224 0-225 1-naphthyl (1-系基) 2-naphthyl 萊基）' p-biphenylyl '27 (p·聯苯基）〇-228 h3Q 0-229 乂） 0-230 o*tolyl (〇·甲苯基）0-231 CH3 0-232 0-233 m-tolyl 0^235 ^ 0-236 -〇-CH3 0-237 p-toly丨 〇>·甲苯基）0-238 0-239 0240 0-241 0242 0-243 0-244 0-245 0-246 0-247 0-248 0-249 0-250
DPA
TPA p-biphenylyl 0- tolyl m-tolyl p-toly! Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- bipnenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2-naphthyl o-biphenylyl m-biphenylyl p-biphenylyl 0- tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-blphenytyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenyfy) m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphlhyl o-biphenylyl m-biphenylyl p-biphenylyi Ph 1- naphtyl 2- naphihyl o-biphenylyl m-biphenylyl p-biphenylyl
Η HHH H
3 3 3 Η HH .C.C-C -CH3 -CH3 -CH3 -CH3 ¥H3A A AAA A 、c Η Η Η H J» J— ppppp p -C-CH Η HH Η H D D dddd
Η Η HH Η H
—TPATPA 訂 (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -123- 581751 A7 B7 五、發明説明（121) 經濟部智慧財產局員工消贫合作社印¾ R1 r2 r3 r5 Re R7 Re P-1 H H H H H H H P-2 Ph H H H Ph H H 尽8 5? P-3 Ph Ph H H Ph H H 〇〇 P-4 Ph H H Ph Ph H H P-5 Ph Ph ft Ph Ph H H Rli>R6 P-6 Ph H Ph H Ph H H R2-O-R5 P-7 Ph H H H Ph Ph H P-8 Ph H H H Ph H Ph P-9 .Ph H H H Ph Ph Ph R5^CVR2 P-10 Ph H H H Ph 1-naphthyl H R6^>Ri P-11 Ph H H H Ph H 1-naphthyl TypeP i^VS P-12 Ph H H H Ph 1-naphthyl 1-naphthyl Vv 〇 D P-13 Ph H H H Ph 2-naphthyl H r7 r8 P-14 Ph H H H Ph H 2-naphthyl C0 P-15 Ph H H H Ph 2-naphthyl 2-naphthyl P-16 Ph H H H Ph o-biphenylyl H P-17 Ph H H H Ph H o-biphenylyl 1.-naphthy丨（1-萘基） P-18 Ph H H H Ph o-biphenylyl o-biphenylyl P-19 Ph Ή H H Ph m-biphenylyl H P-20 Ph H H H Ph H m-biphenylyl 2-naphthyl (2-萘基） P-21 Ph H H H Ph m-biphenylyl m-biphenylyl ob P-22 Ph H H H Ph p-biphenylyl H P-23 Ph H H H Ph H p-biphenylyl o-biphenylyl (〇-聯苯基） P-24 Ph H H H Ph p-biphenylyl p-biphenylyl od P-25 1-naphthyl H H H 1.naphthyl H H P-26 1-naphthyl Ph H H 1-naphthyl H H m-biphenylyl (m·聯苯基〉 P-27 1-naphthyl H H Ph 1-naphlhyl H H P-28 1-naphthyl Ph H Ph 1-naphthyl H H P-29 1-naphthyl H Ph H 1-naphthyl H H |>biphenylyl (p·聯苯基） P-30 1-naphthyl H H H 1-naphthyl Ph H P-31 1-naphthyl H H H 1-naphlhyl H Ph P-32 1-naphthyl H H H 1-naphthyl Ph Ph P-33 1-naphthyl H H H • 1-naphthyl 1-naphthyl H P-34 1-naphthyl H H H 1-naphthyl H 1-naphthyl P-35 1-naphthyl H H H 1-naphthyl 1-naphthyl 1-naphthyl P-36 1-naphthyl H H H 1-naphthyl 2-naphthyl H P-37 1-naphlhyl H H H 1-naphthyl H 2-naphthyl P-38 1-naphthyl H H H 1-naphthyl 2-naphthyl 2-naphthyl P-39 1-naphthyl H H H 1-naphthyl o-biphenylyl H P-40 1-naphthyl H H H 1-naphthyl H o-biphenylyl P-41 1-naphthyl H H H 1-naphthyl o-biphenylyl o-blphenylyl P-42 1-naphthyl H H H 1-naphthyl m-biphenylyl H P-43 1-naphthyl H H H 1-naphthyl H m-biphenylyl P-44 1-naphthyl H H H 1-naphthyl m-biphenylyl m-biphenylyl P-45 1-naphthyl H H H 1-naphthyl p-biphenylyl H P46 1-naphthyl H H H 1-naphthyl H p-biphenylyl P-47 1-naphthyl H H H 1-naphthyl p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） • 124 - 581751 A7 B7 五、發明説明（123 •Ri R2 R3 R5
Re R7
Re Ρ·48 P-49 P-50 P-51 .P-52 P-53 P-54 P-55 P-56 P-57 P-58 Ρ·59 P-60 P-61 P-62 • P-63 P-64 P-65 P-66 P-67 P-68 P-69 P-70 o*b丨phenyly丨（〇-聯苯基） P-71Pp；2 m-biphenylyi (m·聯宝基）P·74 P-75 P-76 P-77 P-78 P-79 Ρ·80 P-81 P-B2 P-83 P-84· P-85 P-86 P-87 P-88 P-89 P-90 P-91 P-92 P-93 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthy! 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyf 2-naphthyi 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-blphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl
Η H Η H H Ph H Ph Ph H Η H Η H Η H Η H H H Η H Η H Η H H H Η H H H Η H Η H Η H Η H Η H H H H H Η H H Ph Η Ph H H H H H Η H Η H Η H H H H H Η H Η H H H Η H H H Η H H H H H Η H H H Η H H H H H H H Ph Ph H 1-naphthyl 1- naphthyl H 2- naphthyl 2-naphthyl H o-biphenylyl. 0- biphenylyl H m-biphenylyl m-biphenylyl H p-biphenylyl p-blphenylyl H H H H H H Ph Ph H 1- naphthyl 1 -naphthyl H 2- naphthyl 2-naphthyl H o-biphenylyl o-biphenylyl H m-biphenylyl m-biphenylyl H p-biphenylyl p-biphenylyl
H Ph H Ph H H H H H H H H H H H H H H H H H H H H Ph H Ph H H H H H H H H H H H H H H H H H H H 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl •2-naphthyl 2-naphthy) 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenyly! o-blphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-blphenylyl H H H H H Ph H Ph 1-naphthyl H 1- naphthyl 2- naphthyl * H 2-naphthyl o-biphenylyl H 0- biphenyly! m-biphenylyl H m-biphenylyl p-biphenylyl H p-biphenylyl H H H H H Ph H Ph 1- naphthyl H 1- naphthyl 2- naphthyl H 2-naphthyl o-biphenylyl H o-biphenylyl m-biphenylyl H m-biphenylyl p-biphenylyl H p-biphenylyl (請先閲讀背面之注意事項再填寫本頁)
、1T 經濟部智慧財產局員工消費合作社印製
C0 1-naphthyl 0-^¾) 2-naphthyl (2-^S)ob p-biphenylyl (p-聯苯基）
H H 本紙張尺度適用中國國家標準（CNS ) A4規格（210><297公釐） -125- 581751 A7 B7 五、發明説明（123) 經濟部智慧財產局員工消費合作社印製 R1 r2 r3 r5 Ra R7 Rfl P-94 m-biphenylyl H H H m-biphenylyl H H P-95 m-biphenylyl Ph H H m-biphenylyl H H P-96 m-biphenylyl H H Ph m-biphenylyl H • H P-97 m-biphenylyl Ph H Ph m-biphenylyl H H • P-98 m-biphenylyl H Ph H m-biphenylyl H H Ri-Q-Rfi P-99 m-biphenylyl H H H m-biphenylyl Ph H R2-Q-R5 P-100 m-biphenylyl H H H m-biphenylyl H Ph % P-101 m-biphenylyl H H H m-biphenylyl Ph Ph P-102 m-biphenylyl H H H m-biphenylyl 1-naphthyl H P-103 m-biphenylyl H H H m-biphenylyl H 1-naphthyl R6*yy*Ri P-104 m-biphenylyl H H H m-biphenylyl 1-naphthyl 1-naphthyl TypeP (jT^) P-105 m-biphenylyl H H H m-biphenylyl 2-naphthyl H r7 r8 P-106 m-biphenylyl H H H m-biphenylyl H 2-naphthyl P-107 m-biphenylyl H H H m-biphenylyl 2-naphthyl 2-naphthyl Ρ·108 m-biphenylyl H H H m-biphenylyl o-biphenylyl H P-109 m-biphenylyl H H H m-biphenylyl H o-biphenylyl P-110 m-biphenylyl H H H m-biphenylyl o-biphenylyl o-biphenylyl P-111 m-biphenylyl H H H m-biphenyiyl m-biphenylyl H 〇6 P-112 m-biphenylyl H H H m-biphenylyl H m-blphenylyl P-113 m-biphenylyl H H H m-biphenylyl m-biphenyiyl m-biphenylyl 1-naphthyl d-^g) P-114 m-biphenylyl H H H m-biphenylyl p-biphenylyl H P-115 m-biphenylyl H H H m-biphenylyl H p-biphenylyl 〇y P-116 m-biphenylyl H H H m-blphenylyl p-biphenylyl p-biphenylyl 2-naphthyl (2-蔡基} \ F-117 p-biphenylyl H H H p-biphenylyl H H CK> o-biphenyJyl P-118 p-biphenylyl Ph H H p-biphenylyl H H P-119 p-biphenylyl .H H Ph p-biphenylyl H H (〇·聯苯基） P-120 p-biphenylyl Ph H Ph p-biphenyly! H H o-d P-121 p-biphenylyl H Ph H p-biphenylyl H H P-122 p-blphenylyl H H H p-biphenylyl Ph H m-biphenylyl (111-聯$基） r\r^K P-123 p-biphenylyl H H H p-biphenylyl H Ph P-124 p-biphenylyl H H H p-biphenylyl Ph Ph p-biphenylyl (p·聯苯基） P-125 p-biphenylyl H H H p-biphenylyl 1-naphthyl H P-126 p-biphenylyl .H H H p-biphenylyl H 1-naphthyl P-127 p-biphenylyl H H H p-biphenylyl 1-naphthyl 1-naphthyl P-128 p-biphenylyl H H H p-biphenylyl 2-naphthyl H P-129 p-biphenylyl H H H p-biphenylyl H 2-naphthyl P-130 p-biphenylyl H H H p-biphenylyl 2-naphthy! 2-naphthyl P-131 p-biphenylyl H H H p-biphenylyl o-biphenylyl H P-132 p-biphenylyl. H H H p-biphenylyl H o-biphenylyl P-133 p-biphenylyl H H H p-biphenylyl o-biphenylyl o-biphenylyl P-134 p-biphenylyl . .H H H p-biphenylyl m-biphenylyl H P-135 p-biphenylyl H H H p-biphenylyl H m-biphenylyl P-136 p-biphenylyl H H H p-biphenylyl m-biphenylyl m-biphenylyl P-137 p-biphenylyl H \ H H p-biphenylyl p-biphenylyl H P-138 p-biphenylyl H H H p-biphenylyl H p-biphenylyl P-139 p-biphenylyl H H H p-biphenylyl p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 訂 本紙張尺度適用中國國家標準（CNS ) Μ規格（210X297公釐） -126- 581751 A7 B7 五、發明説明（124)
2-naphthyl (2-萘基）Ρ·163 八《h p·164 wvy P-165 o-biphenylyl
經濟部智慧財產局員工消費合作社印製 (〇-聯苯基）卜166 」 P-167 〇〇 剛 m-biphenylyl Μ 69 (m-聯苯基）FM70 rv〇- p-171 P-172 p-biphenylyl p.173 (p·聯苯基） H3C P-174 -〇 P-175 o-tolyl (〇·甲苯基)p-176 P-177 Vr, p-178 m均1 P17Q im-甲苯基） -〇ch3 P-180 p-to!yl P-181 (p*甲苯基)p-182 P-183 P-184 P-185 P-186 P-187 P-188 P-189 P-190
Ri r2 «3 r5 Re r7 Rb o-tolyl H H H o-tolyl H H o-tolyl Ph H Ph o-tolyl H H o-tolyl H Ph H o-tolyl H H . o-tolyl .H H H o-tolyl Ph H o-tolyl H H H o-tolyl H Ph o-tolyl H H H o-tolyl 1-naphthyl H o-tolyl H H H o-tolyl H 1-naphthyl o-tolyl H H H o-tolyl 2-naphthyl H o-tolyl H H H o-tolyl H 2-naphthyl o-tolyl H H H o-tolyl o-biphenylyl H o-tolyl H H H o-tolyl H o-biphenylyl o-tolyl H H H o-tolyl m-biphenylyl H o-tolyl H H H o-tolyl H m-biphenylyl o-tolyl H H H o-tolyl p-biphenylyl H o-tolyl H H H o-tolyl H p-biphenylyl o-tolyl H H H o-tolyl o-tolyl H o-tolyl H H H o-tolyl H o-tolyl m-tolyl H H H m-tolyl H H m-tolyl Ph H Ph m-tolyl H H m-tolyl H Ph H m-tolyl H • H m-tolyl H H N m-tolyl Ph H m-lolyl H H H m-tolyl H Ph m-tolyl H H H m-tolyl 1-naphthyl H m-tolyl H H H m-tolyl H 1-naphthyl m-tolyl H H H m-tolyl 2-naphthyl H m-tolyl H H H m-tolyl H 2-naphlhyl m-tolyl H H H m-tolyl o-biphenylyl H m-tolyl H H H m-tolyl H o-biphenylyl m-tolyl H H H m-tolyl m-biphenylyl H m-tolyl H H H m-tolyl H m-biphenylyl m-tolyl H H H m-tolyl p-biphenylyl H m-tolyl H H H m-tolyi H p-biphenylyl m-tolyl H H H m-tolyl m-tolyl H m-tolyl H H H m-lolyl H m-tolyl p-tolyl H H H p-tolyl H H p-tolyl Ph H. Ph p-tolyl H H p-tolyl H Ph H p-tolyl H H p-tolyl H H H p-tolyl Ph H p-tolyl H H H p-tolyl H Ph p-tolyl H H H p-tolyl 1-naphthyl H p-t〇lyl H H H . p-tolyl H 1-naphthyl p-tolyl H H H p-tolyl 2-naphthy! H p-tolyl H H H p-tolyl H 2-naphthyl p-tolyl H H H p-tolyl o-biphenylyl H p-tolyl H H H p-tolyl. H o-biphenylyl p-tolyl H H H p-tolyl m-biphenylyl H p-tolyl H H H p-lolyl H m-biphenylyl p-tolyl H H H p-tolyl p-biphenylyl H p-tolyl H H H p-tolyl ' H p-biphenylyl p-tolyl H H H p-tolyl p-tolyl H p-tolyl H H H p-tolyl H p-tolyl (請先閲讀背面之注意事項再填寫本頁) 訂 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -127- 581751 A7 B7 五、發明説明（125) P-191 P-192 P-193 P-194 P-195 P-196 P-197 P-198 P-199 P-200 P-201 P-202 P-203 P-204 P-205 P-206 P-207 P-208 P-209 P-210 P-211 P-212 P-213 1- naphthyl P-214 (1·莱基）Ρ·215 P-216 P-217 2- naphthyl P-218 (2-萊基）p-219 ob = o-biphenylyl (〇·聯苯基）Ρ·222 γκΑ p-223 ΟΛ-/ P-224 m-biphenylyl p-225 (m·聯苯基）p 226 〇〇 P-227 p-biphenylyl P-228 (p·聯苯基）^ U r P-230 P-231 P-232 〇-tolyl⑼甲苯基）ρ·233 CH3 P-234 一^ P-235 m-tolyl (m·甲苯基d莽 -O-CHs pP^g8 p«tolyl (p·甲苯基）卜/此 P-240 A p·241 DPA P-244 P-245 P-246 P-247 P-248 P-249 P-250
R8I R7 R3 R5 R& R2I hhh hh hhhhhhh h h hhh hhhhh h hhh hh h h hh h h h hhhhhhhh hhhh h h hhhhhhhhhh h HHH ΗΗ Η
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Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphlyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph •1-naphlyl 2-naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl 0- tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphlhyl o-biphenylyl nvbiphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-bipnenylyl m-biphenylyl p-biphenylyl Ph 1- naphlyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenyiyl p-biphenylyl
Ph 1- naphty! 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthvl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphlyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphlhyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl hhhhh hhhhhhhhh hhhhhhhh hhhhhhh h hhhhh hhh hhh h h hhhh h h hhhhhhhhhH3H3H3H3H3H3H3H3H3 -C9-C-C-C-C-C9.CHHH Η H hhhhhhhhh HHH HH Η H HHHHH HHH HHH Η H HHHH Η Η hhhhhhhhhhh ----------- (請先閲讀背面之注意事項再填寫本頁) 訂 經濟部智慧財產局員工消费合作社印製
3 3 3 3 3 3 3 3 3 Hi-CH-CH-CH-CH-CH:CCHH-CHHH c6 ΗΗ hhhh.chh-ch:ch3-ch3:cchh33-ch3-ch3hhhhhohpadpadpadpadpadpa
心g TPA
Η H 彳JAA A A A A Η ΗΗΗΗΗΤΡΤΡΤΡΤΡΤΡΤΡ
TPATPATPATPATPATPAH
HHHHH 本紙張尺度適用中國國家標隼（CNS ) A4規格（210X297公釐） -128- 581751 A7 B7 五、發明説明（126)
〇5 1-naphthyl Γι-^S)
2-naphthyl (2·蔡基）ob o-biphenylyl (〇·聯苯基） o-d m-biphenylyl (m-聯苯基） 經濟部智慧財產局員工消资合作社印製
p-biphenylyl (p·聯苯基) H3C
Ri P-251 Ph P-252 Ph P-253 Ph P-254 Ph P-255 Ph P-256 Ph P-257 Ph P-258 Ph P-259 1-naphthyl P-260 1-naphthyl P-261 1-naphthyl P-262 1-naphthyl P-263 1-naphthyl P-264 1-naphthyl P-265 1-naphthyl P-266 2-naphthyl P-267 2-naphthyl P-268 2-naphthyl P-269 2-naphthyl P-270 2-naphthyl P-271 2-naphthyl P-272 〇-biphenylyl P-273 o-biphenylyl P-274 o-biphenylyl Ρ·275 o-biphenylyl P-276 o-biphenylyl P-277 m-biphenylyl m-biphenylyl P-279 m-biphenylyl P-280 m-biphenylyl P-281 p-biphenylyl P-282 p-biphenylyl P-283 p-biphenylyl P-284 O-tolyly P-285 O-tolyly P-286 m-tolyly R5 β2 Η Η Η Η ηηηηηηηηηηηηηηηηηηηηηηηη ηη Η ΗΗΗ Η Η ηηηηηηηηηηηηηηηηηηηηηηηηηηηη ΗΗ Η ΗΗΗ Η Η ΗΗΗΗ Η ΗΗΗΗΗΗΗΗΗΗΗΗΗ Η ΗΗΗΗΗΗΗΗΗ ΗΗ Η ΗΗΗ Η Η
Re 1- naphthyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl 2-naphthyl o-biphenylyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl o-biphenylyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl p-biphenylyl O-tolyly m-tolyl p-tolyl O-tolyly m-tolyl p-tolyl m-tolyl p-tolyl p-tolyl (請先閲讀背面之注意事項再填寫本頁) R HHHHH ηηηηηηηηηηηηηηηηηηηηηηη ΗΗ Η ΗΗΗ Η Η R Η Η Η Η Η ηηηηηηηηηηηηη η ηηηηηηηηη ΗΗ Η ΗΗΗ Η Η o-t〇lyl (0.甲苯基） ch3 m-tolyl (m·甲苯基） ~^>ch3 p-tolyl (p·甲苯基) 本紙張尺度適用中國國家標準（CNS ) Α4規格（210X297公釐） -129- 581751 A7 B7 五、發明説明（127)
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經濟部智慧財產局員工消费合作社印紫 Q-37 Q-38 Q-39 CMO Q-41 Q-42 CM3 Q-44 Q-45 Q-46 Q-47 Q-48 Q-49 od o-d od od od o^>c^b ob ob ob o^> ob ob
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本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） 131 - 581751 A7 B7 五、發明説明（12》 52 51 / Γ~\ /""\ f —V尽1甲2 n >R7 R7< TypcQ r2 R3 R4 R5 R6 Q-50 Q-51 Q-52 Q-53 Q-54 Q-55 Q-56 Q-57 Q-58 Q-59
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本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -132- 581751 Α7 Β7 五、發明説明（130)
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H H H H Ph H H Me H H H H Ph H H Me H H H H Ph H H (請先閱讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） •133- 581751 A7 B7 五、發明説明（131)
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HHphHHHMeHHHphHHHMeH H HHHHphHHMeHHHHphHHMeHHHHphHHMe (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -134- 581751 A7 B7 五、發明説明（13$ 經濟部智慈財產局員工消費合作社印製
146 1‘17 (請先閲讀背面之注意事項再填寫本頁)
本紙張尺度適用中國國家標準（CNS ) A4·規格（210X297公釐） -135- 581751 A7 B7 五、發明説明（13含
Re R7 od 經濟部智慧財4局員工消費合作社印製 C0 1-naphthyl (1·萘基） 2-naphthyl (2·蔡基） ob * o-Wphenylyl (〇-聯本基） p-bipheny丨yl (p-聯苯基） 只1 r2 r3 r4 Rs r7 Re R-1 Η H H H H H H R-2 Ph H H H H H H R-3 Ph Ph H H Ph H H R-4 Ph H Ph Ph H H H R-5 Ph H Ph H H H H R-6 Ph H H Ph H H H R-7 Ph H H H H Ph H R-8 Ph H H H H H Ph R-9 Ph H H H H Ph Ph R-10 Ph H H H H 1-naphthyl H R-11 Ph H H H H H 1-naphthyl R-12 Ph H H H H 1-naphthyl 1-naphthyl R-13 Ph H H H H 2-naphthyl H R-14 Ph H H H H H 2-naphthyl R-15 Ph H H H H 2-naphthyl 2-naphlhyl R-16 ·· Ph H H H H o-biphenylyl H R-17 Ph H H H H H o-biphenylyl R-18 Ph H H H H o-biphenylyl o-biphenylyl R-19 Ph H H H H m-biphenylyl H R-20 Ph H H H H H m-biphenylyl R-21 Ph H H H H m-biphenylyl m-biphenylyl R-22 Ph H H H H p-biphenylyl H R-23 Ph H H H H H p-biphenylyl R-24 Ph H •H H H p-biphenylyl p-biphenylyl R-25 1-naphthyl H H H H H H R-26 1-naphthyl Ph H H Ph H H R-27 1-naphthyl H Ph Ph H H H R-28 1-naphthyl H Ph H H H H R-29 1-naphthyl H H Ph H H H R-30 1-naphthyl H H H H Ph H R-31 1-naphthyl H H H H H Ph R-32 1-naphthyl H H H H Ph Ph R-33 1-naphthyl H H H H 1-naphthyl H R-34 1-naphthyl H H H H H 1-naphthyl R-35 1-naphthyl H H H H 1-naphthyl 1-naphthyl R-36 1-naphthyl H H H H 2-naphthyl H R-37 1-naphthyl H H H H H 2-naphihyl R-38 1-naphthyl H H H H 2-naphthyl 2-naphthyl R-39 •1-naphthyl H H H H o-biphenylyl H R-40 1-naphthyl H H H H H o-biphenylyl R-41 1-naphthyl H H H H o-biphenylyl o-biphenylyl R-42 1-naphthyl H H H H m-biphenylyl H R-43 1-naphthyl H H H H H m-biphenylyl R-44 1-naphthyl H H H H m-biphenylyl m-biphenylyl R-45 1-naphlhyI H H H . H p-biphenylyl H R-46 1-naphthyl H H H H H p-blphenylyl R-47 1-naphthyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 訂 本紙張尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） 136· 581751 A7 B7 五、發明説明（134
οό 經濟部智慈財產局員工消費合作社印製 1-naphthy丨（】·萊基） 2-naphthy丨（2·莱基） ob o-biphenylyl (〇·聯苯基〉 od m-bipheny丨yl (m-聯苯基) Ri r2 r3 r4 r7 R-48 2-naphthyl H H H H H H R-49 2-naphthyl Ph H H Ph H H R-50 2-naphthyl H Ph Ph H H H R-51 2-naphthyl H Ph H H H H R-52 2-naphthyl H H Ph H H H R-53 2-naphthyl H H H H Ph H R-64 2-naphthyl H H H H H Ph R-55 2-naphthyl H H H H Ph Ph R-56 2-naphlhyl H H H H 1-naphthyl H R-57 2-naphthyl H H H H H 1-naphthyl R-58 2-naphlhyl H H H H 1-naphthyl 1-naphthyl R-59 2naphthyt H H .H H 2-naphthyl H R-60 2-naphthy) H H H H H 2-naphthyl R-61 2-naphthyl H H H H 2-naphthyl 2-naphthyl R-62 2-naphthyl H H H H o-biphenylyl H R-63 2-naphthyl H H H H H o-biphenylyl R-64 2-naphthyl H H H Ή o-biphenylyl o-blphenylyl R-65 2-naphthyl H H H H m-biphenylyl H R-66 2-naphthyl H H H H H m-biphenylyl R-67 2-naphthyl H H H. H m-biphenylyl m-biphenylyl R-6B 2-naphthyl H H H H p-biphenylyl H R-69 2-naphthyl H H H H H p-biphenylyl R-70 2-naphthyl H H H H p-biphenylyl p-biphenylyl R-71 o-biphenylyl H H H H H H R-72 o-bipheny!yl Ph H H Ph H H R-73 o-blphenylyl H Ph Ph H H H R-74 o-biphenylyl H Ph H H H H R-75 o-biphenylyl H H Ph H H H R-76 o-biphenylyl H H H H Ph H R-77 o-biphenylyl H H H H H Ph R-78 o-biphenylyl H H H H Ph Ph R-79 o-biphenylyl H H H H 1-naphthyl H R-80 o-biphenyiyi H H H H H 1-naphthyl R-81 o-biphenylyl H H H H 1-naphthyl 1-naphthyl R-82 o-biphenylyl H H H H 2-naphthyl H R-83 o-biphenylyl H H H H H 2-naphthyl R-84 o-biphenylyl H H H H 2-naphthyl 2-naphthyl R-85 o-biphenylyl H H H H o-biphenylyl H R-86 o-biphenylyl H H H H H o-biphenylyl R-87 o-biphenylyl H H H H o-biphenylyl o-biphenylyl R-88 o-biphenylyl H H H H m-biphenylyl H R-89 o-biphenylyl • H H H H H m-biphenylyl R-90 o-biphenylyl H H H H m-biphenylyl m-biphenylyl R-91 o-biphenylyl H H H H p-biphenylyl H R-92 o-biphenylyl H H H H H p-blphenylyl R-93 o-biphenylyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) Μ規格（210X297公釐） -137- 581751 A7 B7 五、發明説明（13冷
Re Ry C0 1-naphthyl (卜蔡基） R-94 R-95 R-96 R-97 R-98 R-99 R-100 R-101 R-102 R-103 R-104 R-105 R-106 R-107 R-108 R-109 R-110 R-111 R-112 R-113 R-114 R-115 R-116 經濟部智慧財產局員工消費合作社印製 2-naphthyi (2-蔡基） ob 抑 oblphenylyl (°*聯本基）r / R-118 〇-〇 R-119 m-biphenylyl (m-聯苯基) R-121 〇〇- R-122 p-biphenylyl (p>聯苯基）R-123 R-124 R-125 R-126 R-127 R-128 R-129 R-130 R-131 R-132 R-133 R-134 R-135 R-136 R-137 R-138 R-139
Ri m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl R2HphHHHHHH hhhhhhhhhhhhhhhhhhhhh hhhh hh hhhhhh η hh % 尺4 Rs Re Η H H H H Η H Ph H H Ph Ph H H H Ph H H H H H Ph H H H H H H Ph H H H H H Ph H .H .H Ph Ph H H H 1-naphthyl H H H H H 1-naphthyl H H H 1-naphthyl 1-naphthyl H . H 、H 2-naphthyl H H H H H 2-naphthyl H H H 2-naphthyl 2-naphthyl H H H o-biphenylyl H H H H H o-biphenylyl H H H o-biphenylyl o-biphenylyl H H H m-biphenylyl H H H H H m-biphenylyl H H H m-biphenylyl m-biphenylyl H H H p-biphenylyl H H H H H p-biphenylyl H H Ή p-biphenylyl p-biphenylyl H H H H H H H Ph H H Ph Ph H H H Ph H H H H H Ph H H H H H H Ph H H H H H Ph H H H Ph Ph H H H 1-naphthyl H H H H H 1-naphthyl H H H 1-naphthyl 1-naphthyl H H H 2-naphthyl H H H H H 2-naphthyl H H H 2-naphthyl 2-naphthyl H H H o-biphenylyl H H H H H o-biphenylyl H H H o-biphenylyl o-biphenylyl H H H m-biphenylyl H H H H H m-biphenylyl H H H m-biphenylyl m-biphenylyl H H H p-biphenylyl H H H H H p-biphenylyl H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意Ϋ項再填寫本頁)
*1T 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -138- 581751
A B 五、發明説明（13冷
o-tolyl o-to)yl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl m-lolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl R4l H HphHH HHHHHHHHHHHHHHphHHHHHHHHHHHHHHHHphHHHHHHH. HHHHHHH R3l H HphHH HHHH HHHHHHH HHHphHHHHHHHHHHHHHH HH^HHHHHH HHHHHHHH Rs r7 Re Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Ph Η 1-naphthyl Η Η Η 1-naphthyl Η 2-naphthyl Η Η Η 2-naphthyl Η o-biphenylyl Η Η Η o-biphenylyl Η m-biphenylyl Η Η Η m-biphenylyl Η p-biphenylyl Η Η Η p-biphenylyl Η o-tolyl Η Η Η o-iolyl Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Ph Η 1-naphthyl Η Η Η 1-naphthyl Η 2-naphthyl Η Η Η 2-naphthyl Η o-biphenylyl Η Η Η o-biphenylyl Η m-biphenylyl Η Η Η m-biphenylyl Η p-biphenylyl Η Η Η p-biphenylyl Η m-tolyl Η Η Η m-tolyl Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Ph Η 1-naphthyl Η Η Η 1-naphthyl Η 2-naphthyl Η Η Η 2-naphthyl Η o-biphenylyl Η Η Η o-biphenylyl Η m-biphenylyl Η Η Η m-biphenylyl Η p-biphenylyl Η Η Η p-biphenylyl Η p-tolyl Η Η Η p-tolyl
Η ^HHH hhhh HHHHHHH HH^ HHHHHHH HHHHHHHH H ^ HHHHHHH HHHHHHHH R-140 R-141 R-142 R-143 R-144 R-145 R-146 R-147 R-148 R-149 R-150 R-151 R-152 R-153 R-154 R-155 R-156* R-157 R-158 R-159 R-160 R-161 R-162 R-163 R-164 R-165 R-166 R-167 R-168 R-169 R-170 R-171 R-172 R-173 R-174 R-175 R-176 R-177 R-178 R-179 R-180 R-181 R-182 R-183 R-184 R-185 R-186 R-187 R-188 R-189 R-190 經濟部智慈財產局員工消资合作社印製 (請先閲讀背面之注意事項再填寫本頁) 00 1-naphthyl (1-莱基） 2-napWhy丨（2-萘基) o-b o-biphenylyl (〇-聯茏基）od m-biphenylyl .(m-聯苯基) p-biphenylyl (p·脚苯基） o»toly丨（°·甲苯基） pH3 m·丨o丨y丨（m·甲苯基） "O"CH3 p-tolyl φ·甲苯基） 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -139- 581751 A7B7 五、發明説明（13为
Ri r4
Rs R7
ob o-biphenylyl (0-聯苯基）od m-biphenylyl (m-聯苯基）
I 經濟部智慧財產局員工消費合作社印製
TPA o N o
C0 1-naphthyl 〇 p-biphenylyl (p·聯苯基） 〇»t〇lyl (〇·甲苯基） CH3 m-lolyl (m-甲苯基） -〇CH3 p-tolyl (p·甲苯基） Cy〇 . DPA R-191 Ph H -CH3 -CH3 R-192 1-naphtyl H -CH3 -CH3 R-193 2-naphthyl H -CH3 •CH3 R-194 R-195 o-biphenylyl m-biphenyiyl H H -CH3 -CH3 -CH3 -CH3 R-196 p-biphenylyl H -CH3 -CH3 R-197 o-tolvl m-tolyl H •CH3 -CH3 R-198 H -CH3 •CH3 R-199 p-tolyl H •CH3 •CH3 R-200 Ph H H H Ε-201 1-naphtyl H H H R-202 2-naphthyl H H H R-203 o-biphenylyl H H H R-204 m-biphenylyl H H H R-205 p-biphenylyl H H H R-206 o-tolyl H H H R-207 m-tolyl H H H R-208 p-tolyl H H H R-209 Ph H H H R-210 1- naphtyl · 2- naphthyl o-bipnenylyl H H H R-211 R-212 H H H R-213 m-biphenylyl H H H R-214 p-biphenylyl H H H R-215 o-tolyl H H H R-216 R-217 m-tolyl H H H p-tolyl H H H R-218 Ph H H H R-219 1-naphtyl H H H R-220 2-naphthyl H H H R-221 o-biphenylyl H H H R-222 m-biphenylyl H H H R-223 p-biphenylyl H H H R-224 o-toJyl H H H R-225 m-tolyl H H H R-226 p-tolyl H H H R-227 Ph H H H R-228 1-naphtyl H H H R-229 2-naphthyl o-biphenylyl H H H R-230 H H H R-231 m-biphenyiyl H H H R-232 p-biphenylyl H H H R-233 Ph H H H R-234 1-naphtyl H H H R-235 R-236 2-naphthyl o-biphenylyl H H H H H H R-237 m-biphenylyl H H H R-23B p-biphenyly! H H H R-239 Ph H H H R-240 1-naphtyl H H H R-241 2-naphlhyl H H H R-242 o-biphenylyl H H H R-243 m-biphenylyl H H H R-244 p-biphenylyl .H H H R-245 Ph H H H R-246 1-naphtyl H H H R-247 2-naphthyl H H H R-248 o-biphenylyl H H H R-249 m-biphenylyl H H H R-250 p-biphenylyl H H H ηηηηηηηηηηηηηη ηηηηηηηη ηηηηηηη η ηηηηη ηηηηηηηη ηηηη η η ηηηηηηηηηηη
Η Η Η ΗΗ S Η HiHH:^:ccHH33-CH3-CH3-CH3H ΗΗ Η Η Β h:cchh33-ch3s-ch3-ch3:ch3h Η Η Η HHDPADPAgKDPADPAHHHHHHTPATPATPATPATPATPA Η Η Η ΗΗ Η Η Η Η Η Η Η 131333 333333 ^ 3 3 3 33 3 $ Α Λ Λ A Α λ X- X- Η Η hhh.chh:cchh-ch?:s:cchh:cchh.ch:cchh:s-ch-chdpadpadpadpadpadhpakhhthpatpatpatpatpathpahh Η Η Η -- (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) Α4規格（210Χ297公嫠） -140- 581751
7 A
B 五、發明説明（13θ
Ri
c6 1-naphthyl (丨·萘基） 2-naphthyi (2-^S)ob 一 o^biphenylyl (°·聯本基）Qr0 m-biphenylyl (m_聯本基） p-biphenyly丨（p*聯苯基） 經濟部智慈財產局員工消贫合作社印製 S-1 S-2 S-3 S-4 S-5 S-6 S-7 S-8 S-9 S-10 S-11 S-12 S-13 S-14 S-15 S-16 S-17 S-18 S-19 S-20 S-21 S-22 S-23 S-24 S-25 S-26 S-27 S-28 S-29 S-30 S-31 S-32 S-33 S-34 S-35 S-36 S-37 S-38 S-39 S-40 S-41 S-42 S-43 S»44 S-45 S-46 S-47 H Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphlhyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl ^ hhhhh^hhhhhhhhhhhhhhhhhh hhhh^hhhhhhh hhhhhhhhhhh R2HHphHphHHHHHHHHHHHHHHHHHHH HphHphHHHHHHHHHHHHHHHHHHH r5 Re R? Ra Η Η H H Η Ph H H Η Ph H H Ph Ph H H Ph Ph H H Η Ph H H Η Ph Ph H. Η Ph H Ph Η Ph Ph Ph Η Ph 1-naphthyl H Η Ph H 1-naphthyl Η Ph 1-naphlhyl 1-naphthyl Η Ph 2-naphthyl H Η Ph H 2-naphthyl Η Ph 2-naphthyl 2-naphthyl Η Ph o-biphenylyl H Η Ph H o-biphenylyl Η Ph o-biphenylyl o-biphenylyl Η Ph m-biphenylyl H Η Ph H m-biphenylyl Η Ph m-biphenylyl m-biphenylyl Η Ph p-biphenylyl H Η Ph H p-blphenylyl Η Ph p-biphenylyl p-biphenylyl Η 1-naphthyl H H Η 1-naphthyl H H Ph 1-naphthyl H H Ph 1-naphthyl H H Η 1-naphthyl H H Η 1-naphthyl Ph H Η 1-naphthyl H Ph Η 1-naphthyl Ph Ph Η 1-naphthyl 1-naphthyl H Η 1-naphthyl H 1-naphthyl Η 1-naphthyl 1-naphthyl 1-naphthyl Η 1-naphthyl 2-naphthyl H Η 1-naphthyl H 2-naphthyl Η 1-naphthyl 2-naphthyl 2-naphthyl Η 1-naphthyl o-biphenylyl H Η 1-naphthyl H o-biphenylyl Η 1-naphthyl o-biphenylyl o-biphenylyl Η· 1-naphthyl m-biphenylyl H Η 1-naphthyl H m-biphenylyl Η 1-naphthyl m-biphenylyl m-biphenylyl Η 1-naphthyl p-biphenylyi H Η 1-naphthyl H p-biphenylyl (請先閲讀背面之注意事項再填寫本頁)
、1T 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -141 - 581751 A7 B7 五、發明説明（13乡 只1 ^2
C0 1-naphthy丨（〗-萘基）
2-naphthy丨（2-萘基） /-V S-48 S-49 S-50 S-51 S-52 S-53 S-54 S-55 S-56 S-57 S-58 S-59 S-60 S-61 S-62 S-63 S-64 S-65 S^6 S-67 S-68 S-69 S-70 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl .2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphlhyl 2-naphthyl od 經濟部智慧財產局5貝工消资合作社印製
!>b〗phenylyl (p·聯苯基） S-71 o-biphenylyl H S-72 o-biphenylyl Ph S-73 o-biphenylyl H S-74 o-biphenylyl Ph S-75 o-biphenylyl H S-76 o-biphenylyl H S-77 o-blphenylyl H S-78 o-biphenylyl H S-79 o-biphenylyl H S-B0 o-biphenylyl H S-81 o-biphenylyl H S-82 o-biphenyly! H S-83 o-biphenylyl H S-B4 o-biphenylyl H S-85 o-biphenylyl H S-B6 o-biphenylyl H S-87 o-biphenylyl H S-88 o-biphenylyl H S-89 o-biphenylyl H S-90 o-biphenylyl H S-91 o-biphenylyl H S-92 o-biphenylyl H S-93 o-biphenylyl H
HphHphHHHH HHH hhhhhhhhhhhh r3 r5 Re H H 2-naphthyl H H 2-naphthyl H Ph 2-naphthyl H Ph 2-naphlhyl Ph H 2-naphthyl H H 2-naphlhyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyi H H 2-naphlhyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyt H H 2-naphthyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyl H H o-biphenylyl H H o-biphenylyl H Ph o-biphenylyl H Ph o-biphenylyl Ph H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl R7 Ra H Ph 1-naphthyl H 1- naphthyl 2- naphthyl H 2-naphthyl o-biphenylyl H 0- biphenylyl m-biphenylyl H m-blphenylyl p-biphenylyl H p-biphenylyl H H H H H Ph H Ph 1- naphthyl H 1- naphthyl 2- naphthyl H 2-naphlhyl o-biphenylyl H Η H o-blphenylyl 〇-biphenylyl Η H o-biphenylyl m-biphenylyl Η H o-biphenylyl h Η H o-biphenylyl m-biphenylyl Η H o-biphenylyl p-biphenylyl H H o-biphenylyl μ Η H o-biphenylyl p-biphenylyl Η Η Η Η Η Η Η Η Η Η Ph Η Ph Ph Η 1-naphthyl 1- naphthyl Η 2- naphthyl 2-naphthyl Η o-biphenylyl 0- biphenylyl H m-blphenylyl m-biphenylyl H. p-biphenylyl p-biphenylyl H H H H H H Ph Ph H 1- naphthyl 1- naphthyl H 2- naphthyl 2-naphthyl H o-biphenylyl o-biphenylyl H m-biphenylyl m-biphenylyl H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -142- 581751 A7 B7 五、發明説明（
C0 1-naphthyl (1·案基） S-94 S-95 S-96 S-97 S-98 S-99 S-100 S-101 S-102 S-103 S-104 S-105 S-106 S-107 S-108 S-109 S-110 S-111 S-112 S-113 S-114 S-115 S-116 2-naphthy丨（2-萘基）ob . o-biphenyly! 5.-)17 」 S-118 〇〇 ㈣ m-biphenylyl S-120 (m-聯苯基）S-121 S-122 p-biphenyly) (P·聯苯基） 經濟部智慧財產局員工消費合作社印製 S-123 S-124 S-125 S-126 S-127 S-128 S-129 S-130 S-131 S-132 S-133 S-134 S-135 S-136 S-137 S-138 S-139 R1 m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-blphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenyiyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenytyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyi p-biphenylyl QT HphHphHHHH hhhh hhhhhhhhhhh HphHphHHHH hhhh hh hhhhhhh hh Rfi Re .r7 r8 Η Η m-biphenylyl H H Η Η m-biphenylyl H H Η Ph m-biphenylyl H H Η Ph m-biphenylyl H H Ph Η m-biphenylyl H H Η Η m-biphenylyl Ph H Η Η m-biphenylyl H Ph Η Η m-biphenylyl Ph Ph Η Η m-biphenylyl 1-naphthyl H Η Η m-biphenylyl H 1-naphthyl Η Η m-biphenylyl 1-naphlhyl 1-naphthyl Η Η m-biphenyiyl 2-naphthyl H Η Η m-biphenylyl H 2-naphthyl Η Η m-bipheny)yl 2-naphthyl 2-naphthyl Η Η m-biphenylyl o-biphenylyl H Η Η m-biphenylyl H o-biphenylyl Η Η m-biphenylyl o-biphenylyl o-biphenylyl Η Η m-biphenylyl m-biphenylyl H Η Η m-biphenylyl H m-biphenyty! Η Η m-biphenylyl m-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl H Η Η m-biphenylyl H p-biphenylyl Η Η m-biphenylyl p-biphenylyl p-biphenylyl Η Η p-biphenylyl H H Η Η p-biphenylyl H H Η Ph p-biphenylyl H H Η Ph p-biphenylyl H H Ph Η p-biphenylyl H H Η Η p-biphenylyl Ph H Η Η p-biphenylyl H Ph Η Η p-biphenylyl Ph Ph Η Η p>biphenylyi 1-naphthyl H Η Η p-biphenylyl H 1-naphthyl Η Η p-biphenylyl 1-naphthyl 1-naphthyl Η Η p-biphenylyl 2-naphthyl H Η Η p-biphenylyl H 2-naphthyl Η Η p-biphenylyl 2-naphthyl 2-naphthyl Η Η p-biphenylyl o-biphenyly! H Η Η p-biphenylyl H o-biphenylyl Η Η p-biphenylyl o-biphenylyl o-biphenylyl Η Η p-biphenylyl m-biphenylyl H Η Η p-biphenylyl H m-biphenylyl Η· Η p-biphenylyl m-biphenylyl m-biphenylyl Η Η p-biphenylyl p-biphenylyi H Η Η p-biphenyfyl H p-biphenylyl Η Η p-biphenylyl p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 訂 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -143- 581751 A7 B7 五、發明説明（141)
Ri r2 r3 r5 R6 . r7 Re Η Η Η o-tolyl .H H Ph Η Ph o-tolyl H H Η Ph Η o-tolyl H H Η Η Η o-toiyl Ph H Η Η Η o-tolyl H Ph Η Η Η o-tolyl 1-naphthyl H Η Η Η o-tolyl H 1-naphthyl Η Η Η o-tolyl 2-naphthyl H Η Η Η o-iolyl H 2-naphthyl Η Η Η o-tolyl o-biphenylyl H Η Η Η o-tolyl H o-blphenylyl Η Η Η o-tolyl m-biphenylyl H Η Η Η o-tolyl H m-biphenylyl Η Η Η o-tolyl p-biphenylyl H Η Η Η o-tolyl H p-biphenylyl Η Η Η o-iolyl o-tolyl H Η Η Η o-tolyl H o-tolyl Η Η Η m-tolyl H H Ph Η Ph m-tolyl H H Η Ph Η m-tolyl H H Η Η Η m-tolyl Ph H Η Η Η m-tolyl H Ph Η Η Η m-lolyl 1-naphthyl H Η Η Η . m-tolyl H 1-naphthyl Η Η Η m-tolyl 2-naphthyl H Η Η Η m-tolyl H 2-naphthyl Η Η Η m-tolyl o-biphenylyl H Η Η Η m-tolyl H o-biphenylyl Η Η Η m-tolyl m-biphenylyl H Η Η Η m-tolyl H m-biphenylyl Η Η Η m-tolyl p-biphenylyl H Η Η Η m-tolyl H p-biphenylyl Η Η Η m-tolyl m-tolyl H Η Η Η m-tolyl H m-tolyl Η Η Η p-totyl H H Ph Η Ph p-tolyl H H Η Ph Η p-tolyl H H Η Η Η p-tolyl Ph H Η Η Η p-tolyl H Ph Η Η Η p-tolyl 1-naphthyl H Η Η Η p-t〇}yl H 1-naphthyl Η. Η Η· p-tolyl 2-naphthyl H Η Η Η p-tolyl H 2-naphthyl Η Η Η p-tolyl o-blphenylyl H Η Η Η p-tolyl • H o-biphenylyl Η Η Η p-tolyl m-biphenylyl H Η Η Η p-tolyl H m-biphenylyl Η Η Η p-tolyl p-biphenylyl H Η Η Η p-tolyl H p-biphenylyl Η Η Η p-tolyl p-tolyl H Η Η Η p-tolyl H p-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-toiyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-toiyl o-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-toiyl p-tolyl p-tolyl p-tolyl p-to^l p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl S-140 S-141 S-142 S-143 S-144 S-145 S-146 S-147 S-148 S-149 S-150 S-151 S-152 S-153 S-154 S-155 S-156 S-157 S-158 S-159 S-160 S-161 S-162 S-163 S-164 S-165 S-166 S-167 S-168 S-169 S-170 S-171 S-172 S-173 S-174 S-175 S-176 S-177 S-178 S-179 S-1B0 S-181 S-182 S-183 S-1B4 S-185 S-186 S-187 S-188 S-189 S-190 (請先閲讀背面之注意事項再填寫本頁)
*1T 經濟部智慧財產局員工消贫合作社印製 2-naphthy丨（2·萘基) ob o-biphenylyl (〇聯苯Qr0 -biphenylyl (m-聯茏基) p-biphenylyl (p·聯苯基） o»tolyl (°*甲苯基） CH3
I I (in·甲苯基） _ -ch3 ρ·ϊ5ΙγΙ (p·甲苯基） 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -144- 581751 A7 B7 五、發明説明（14含
2-naphthy丨（2-蔡基)ob o-biphenylyl (〇·聯苯基）od m-biphenylyl (m-聯苯基) p-biphenylyl CHa 經濟部智慧財產局員工消費合作社印製 ^〇CH3 p-tolyl (ρ-ψ 〇V〇
DPA
^>b TPA
Ri r2 S-191 Ph H S-192 1-naphtyl H S-193 2-naphthyl H S-194 S-195 o-biphenylyl m-biphenylyl H H S-196 p-biphenylyl H S-197 o-tolyl H S-198 m-tolyl H S-199 p-tolyl H S-200 Ph H S-201 1-naphtyl H S-202 2-naphlhyl H S-203 o-biphenylyl H S-204 m-blphenylyl H S-205 p-biphenylyl H S-206 o-tolyl H S-207 m-tolyl H S-208 p-tolyl H S-209 Ph H S-210 S-211 S-212 1- naphtyl 2- naphthyl o-bipnenylyl H H S-213 m-biphenylyl H S-214 p-biphenylyl H S-215 o-tolyl H S-216 m-tolyl H S-217 p-tolyl H S-218 Ph H S-219 1-naphtyl H S-220 2-naphthyl H S-221 o-blphenylyl H S-222 m-biphenylyl H S-223 p-biphenylyl H S-224 o-tolyl H S-225 m-tolyl H S-226 p-tolyl H S-227 Ph H S-228 1-naphtyl H S-229 2-naphthyl H S-230 o-biphenylyl H S-231 m-biphenylyl H S-232 p-biphenyiyl H S-233 Ph H S-234 1-naphlyl H S-235 2-naphthyl o-biphenylyl m-biphenylyl H S-236 S-237 H H S-238 p-biphenylyl H S-239 Ph H S-240 1-naphtyl H S-241 2-naphthyl H S-242 o-biphenylyl H S-243 m-biphenylyl H S-244 p-biphenylyl 'H S-245 Ph H S-246 1-naphtyl H S-247 2-naphthyl H S-248. o-biphenylyl H S-249 m-biphenylyl H S-250 p-biphenylyl H hhhhhhhh hhhhh h hhh hhh h hhhhh hhhhhhh hhhhh h hhhhhhhhhhhh - 333333333 ^ HHHH HHHH R 一-C-C-C99 9 999 R5 R6
Ry
R8I HHH HH hhhhhhh h h hhh hhhhh hhhhhhh h hh hhh hhhhhhhh hhhh h h hhhhhhhhhhh Ph H 1-naphtyl H 2-naphthyl H o-biphenylyl m-biphenyly! H H p-biphenylyl H o-tolyl H m-tolyl H p-tolyl H Ph -CH3 1-naphtyl -CH3 2-naphthyl -CH3 o-biphenylyl •CH3 m-biphenylyl -CH3 p-biphenylyl -CH3 o-tolyl •CH3 m-to^l -CH3 p-tolyl -CH3 Ph H 1- naphtyl 2- naphlhvl o-bipnenylyl H H H m-biphenylyl H p-biphenylyl H o-toly) H m-tolyl H p-tolyl H Ph •CH3 1-naphtyl -CH3 2-naphthyl -CH3 o-biphenylyl -CH3 m-biphenylyl. •CH3 p-biphenylyl -CH3 o-tolyl •CH3 m-tolyl -CH3 p-tolyl -CH3 Ph H 1-naphtyl H 2-naphthvl o-biphenylyl H H m-biphenylyl H p-biphenylyl H Ph . DPA 1-naphlyI DPA 2-naphthyl o-biphenylyl DPA DPA m-biphenylyl DPA p-biphenylyl DPA Ph •H 1-naphtyl H 2-naphlhyI H o-biphenylyl H m-biphenylyl H p-biphenylyl H Ph TPA 1-naphtyl TPA 2-naphlhyl TPA o-biphenylyl TPA m-biphenylyl TPA p-biphenylyl TPA A A A A A A Η HHHH htptptptptptphhhhhh HHHHH HHHHHHHH Η HHHHIH3H3H3I =H3H3H3H3H3i (請先閲讀背面之注意事項再填寫本頁) 訂 本紙張尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） -145- 581751 Α7Β7 五、發明説明（14含
C0 1-naphthyl (i-萘基） 2-naphthyl (2 ob o-biphenylyl (o-ti茏基）od m-biphenylyl (m-聯苯基)
p-biphenylyl (p·聯苯基） H3C S-251 S-252 S-253 S-254 S-255 S-256 S-257 S-258 S-259 S-260 S-261 S-262 S-263 S-264 S-265 S-266 S-267 S-268 S-269 S-270 S-271 S-272 S-273 S-274 S-275 S-276 S-277 S-278 S-279 S-280 S-281 S-282 S-283 S-2B4 S-285 S-286
Ri Ph Ph Ph Ph Ph Ph Ph Ph 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1- naphthyl 2- naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl O-tolyly O-tolyly m-iolyly R5 R2 ηηηη ηηηηηηηηηηηηηηη ηηηηηηηηη ηη η ηηη η η ηηηη ηηηηηηηηηηηηηηη ηηηηηηηηη ηη η ηηη η η Η Η Η Η Η Η Η Η Η Η Η Η Η ΗΗΗΗ Η Η Η Η Η Η Η Η ΗΗ Η ΗΗ ΗΗΗΗ Η Η R6 1- naphthyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl 2-naphthyl o-biphenylyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl o-biphenylyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl p-biphenylyl O-tolyly m-tolyl p-tolyl O-tolyly m-tolyl p-tolyl m-tolyl p-tolyl. p-tolyl R7 ρβ ηηηη η ηηηηηηηηη ηη ηηηηηηηηηηηη ηη ηηηη ηη ηηηηηηηηηηηηηηηηηηηηηηηηηηηηηη ηηηη η η ---------- (請先閲讀背面之注意事項再填寫本頁) *11 o-to丨yl (°*甲苯基） _CH3 經濟部智慧財產局員工消費合作社印製 m-tolyl (m-甲苯基） -〇ch3 (p*甲苯基） 本紙張尺度適用中國國家標準（CNS ) Α4規格（210Χ297公釐） -146- 581751 A7 B7 五、發明説明（14 經濟部智慈財1局員工消費合作社印製
Ri r2 r3 r5 Re r7 Rb T-1 Η H H H H H H T-2 Ph H H H Ph H H ί-Γ Rs T-3 Ph Ph H H Ph H H T-4 Ph H H Ph Ph H H T-5 Ph Ph H Ph Ph H H R% T-6 Ph H Ph H Ph H H T-7 Ph H H H Ph Ph H T-8 Ph H H H Ph H Ph Tvn#T \ T-9 Ph H H H Ph Ph Ph R，Κβ T-10 Ph H H H Ph 1-naphthyl H T-11 Ph H H H Ph H 1-naphthyl T-12 Ph H H H Ph 1-naphthyl 1-naphthyl T-13 Ph H H H Ph 2-naphthyl H T-14 Ph H H H Ph H 2-naphthyl οό T-15 Ph H H H .Ph 2-naphthyl 2-naphthyl T-16 Ph H H H Ph o-biphenylyl H 1-naphthyl (1-蔡基） T-17 Ph H H H Ph H o-biphenylyl T-18 Ph H H H Ph o-biphenylyl o-biphenylyl 〇y 知 T-19 Ph H H H Ph m-biphenylyl H 2-naphthyl (2-蔡基） T-20 Ph H H H Ph H m-biphenylyl T-21 Ph H H H Ph m-biphenylyl m-biphenylyl ry}^ T-22 Ph H H H Ph p-biphenylyl H Λ™Z^\_z o-biphenyly微（°·聯苯基) T-23 Ph H H H Ph H p-biphenylyl T-24 Ph H H H Ph p-biphenylyl p-biphenylyl od T-25 1-naphthyl H H H 1-naphthyl H H \mm/ \ Ψ m-biphenylyl (m-聯苯基: >T-26 1-naphthyl Ph H H 1-naphthyl H H T-27 1-naphthyl H H Ph 1-naphthyl H H oo T-28 1-naphthyl Ph H Ph 1-naphthyl H H \mmt/ p»t)iphenylyl (p·聯苯基） 了 ·29 1-naphthyl H Ph H 1-naphthyl H H T-30 1-naphthyl H H H 1-naphthyl Ph H T-31 1-naphthyl H H H 1-naphthyl H Ph Τ·32 1-naphthyl H H H 1-naphthyl Ph Ph Τ-33 1-naphthyl H H H 1-naphthyl 1-naphthyl H Τ-34 1-naphthyl H H H 1-naphthyl H 1-naphthyl Τ·35 1-naphthyl H H H 1-naphthyl 1-naphthyl 1-naphthyl Τ·36 1-naphthyl H H H 1-naphthy! 2-naphthyl H Τ·37 1-naphthyl H H H 1-naphthyl H 2-naphthyl Τ-38 1-naphthyl H H H 1-naphthyl 2-naphthyl 2-naphthyl Τ-39 1-naphthyl H H H 1-naphthyl o-biphenylyl H Τ-40 1-naphthyl H H H 1-naphthyl H o-biphenylyl Τ-41 1-naphthyl H H H 1-naphthyl o-biphenylyl o-biphenylyl Τ-42 1-naphthyl H H H 1-naphthyl m-biphenylyl H Τ43 1-naphthyl H H H 1-naphthyl H m-biphenylyl Τ-44 1-naphthyl H H H 1-naphlhyl m-biphenylyl m-biphenylyl Τ-45 1-naphthyl H H H 1-naphthyl p-biphenylyl H ΊΜ6 1-naphthyl H H H 1-naphthyl H p-biphenylyl Τ-47 1-naphthyl H H H 1-naphthyl p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -147- 581751 Α7 Β7 五、發明説明（14冷 R2 R3 R7 r8 rd
H 2-naphlhyl H 2-naphthyl Ph 2-naphthyl Ph 2-naphlhyl H 2-naphlhyl H 2-naphthyl H 2-naphthyl H 2-naphthyl 2-naphthyl H H 2-naphthyl Ph H 2-naphthyl H H 2-naphthyl Ph H 2-naphthyl H Ph 2-naphthyl H H 2-naphthyl H H 2-naphthyl * H H 2-naphthyl · H H 2-naphthyl H H 2-naphlhyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthy) H H 2-naphthyl H H 2-naphlhyl H H 2-naphthyl H H 2-naphthyl H H 2-naphthyi H H 2-naphthyl H H o-biphenylyl H H o-blphenylyl Ph H o-biphenylyl H H o-biphenylyl Ph H o-biphenylyl H Ph o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o：biphenylyl H H o-blphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o*biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H H o-biphenylyl H .H Η Η Η Η Η Η Η Η Η·Η Η Η Η Η Η Η Η Η H Η H Η H Η H Η H Ph H Η Ph Ph Ph 1-naphthyl H Η 1-naphthyl 1-naphthyl 1-naphthyl 2-naphthyl H Η 2-naphthyl 2-naphthyl 2-naphlhyl o-biphenylyl H H o-biphenylyl o-biphenylyl o-biphenylyl m-biphenylyl H H m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl H H p-biphenylyl p-biphenylyl p-biphenylyl H H H H H H H H H H Ph H H Ph Ph Ph 1-naphthyl H H 1-naphthyl 1-naphthyl 1-naphthyl 2-naphthyl H H 2-naphthyl 2-naphthyl 2-naphthyl o-biphenylyl H H o-biphenylyl o-biphenylyl o-biphenylyl m-biphenylyl H H m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl H H p-biphenylyl p-biphenylyl p-biphenyly! (請先閲讀背面之注意事項再填寫本頁) *1Τ 經濟部智慈財產局員工消費合作社印製 C0 1-naphthy丨（1-蔡基） 2-naphthyl (2-萘基） Τ·59 Τ-60 Τ-61 Τ-62 Τ-63 Τ-64 Τ-65 Τ-66 Τ-67 Τ-68 Τ·69 Τ-70 〇^> 巧 o-biphenyly丨（〇·聯苯基） y T-74 0-0 τ·75 m-biphenylyl (m_聯苯基）Τ·76 Τ-77 Τ-78 Τ-79 Τ-80 Τ·81 Τ-82 Τ-83 Τ-84 Τ-85 Τ-86 Τ-87 Τ-88 Τ·89 Τ-90 Τ·91 Τ-92 Τ·93 p-biphenylyl (ρ>聯苯基) 2-naphthyl 2-naphthyl 2-naphlhyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl o-biphenylyl o-biphenyly!
Ph o-biphenylyl Ph 〇-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-blphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl 本紙張尺度適用中國國家標準（CNS ) Α4規格（210Χ297公嫠） -148- 581751 A7 B7 五、發明説明（M冷
Ri
，R7 m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl j-100 m-biphenylyi Τ·1 〇1 m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl T-108 m-biphenylyl T-109 m-biphenylyl T-110 m-biphenylyl T-111 m-biphenylyl T-112 m-biphenylyl T-113 m-biphenylyl 了14 nvbiphenylyl T-115 m-biphenylyl T-116 m-biphenylyl T-94 T-95 T-96 T-97 T-98 T-99 T-102 T-103 T-104 丁-105 Τ·106 T-107 經濟部智慧財產局員工消費合作社印契 C0 1- naphthy丨（卜萘基）αχ 2- naphlhy丨（2-萘基）(>b 仰 o-biphenylyl (〇-聯本基）了·j π p-biphenylyl 」 T-118 P-biphenylyl t-1 19 P-biphenylyl m-b丨phenylyl (m-聯苯基)T-120 P-Wphenylyl T-121 p-biphenylyl AVV-V T-122 p-biphenylyl (p«聯苯基）Τ·123 p-biphenylyl Τ·124 P-biphenylyl T-125 P-biphenylyl T-126 p-biphenylyl T-127 p-biphenylyl T-128 p-biphenylyl T-129 p-biphenylyl T-130 p-blphenylyl T-131 p-biphenylyl T-132 p-biphenylyl T-133 p-biphenylyl T-134 p-biphenylyl T-135 p-biphenylyl T-136 p-biphenylyl T-137 p-biphenylyl T-138 p-biphenylyl T-139 p-biphenylyl
hhhh^hhhhhhhhhhhhhhhhhh hhhh^hhhhhhh hhhhhhhh hhh R2IHphHphHHHH hhhh HHHHHHHHHHHHphHphHHHH HHHHHHHHHHHHHHH R5 HHphphHHH h hhhh.hhhhhhhhhhh.HHPphHHHH hhhh hhhhhhhhhhh
Re m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-blphenylyl nvbiphenylyl m-biphenylyl m-biphenylyl m-biphenylyi m-biphenylyl m-biphenylyl nvbiphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl R?_ H H H H H Ph H Ph 1-naphthyl H 1- naphthyl 2- naphthyl H 2-naphthyl o-biphenylyl H 0- biphenylyl m-biphenylyl H m-biphenylyl p-biphenylyl H p-biphenylyl H H H H H Fh H Ph · 1- naphthyl H 1- naphthyl 2- naphthyl H 2-naphthyl o-biphenylyl H o-biphenylyl m-biphenylyl H m-biphenylyl p-biphenylyl H p-biphenylyl
Rs H H H H H H Ph Ph H 1-naphthyl 1- naphthyl H 2- naphthyl 2-naphthyl H o-biphenylyl 0- biphenylyl H m-biphenylyl m-biphenylyl H p-biphenylyl p-biphenylyl H H H H H H Ph Ph H 1- naphthyl 1- naphthyl H 2- naphthyl 2-naphthyl H o-biphenylyl o-biphenylyl H m-biphenylyl m-biphenylyl H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁)
*-IT 本紙張尺度適用中國ϋ家榡率（CNS)八4狀（210><297公董） -149- 581751 A7 B7 五、發明説明（14为 R.
C0 經濟部智慧財產局員工消費合作社印製 -〇ch3 p-tolyl 1-naphthyl π·萘基） 2-naphthy] (2·萘基） ob o-biphenylyl (〇-聯本基） m-biphenylyl im-聯苯基） p-biphenylyl (p·聯苯基） H3C o-lolyl (°·甲苯基） CH3 m-to丨yl (m.甲苯基） (p·甲苯*) Ri r2 r3 R5 Re r7 Re Τ-140 o-tolyl H H H o-tolyl H H Τ-141 o-tolyl Ph H Ph o-tolyl H H Τ-142 o-tolyl H Ph H o-tolyl H H Τ-143 o-tolyl H H H o-tolyl Ph H Τ-144 o-tolyl H H H o-tolyl H Ph Τ-145 'o-tolyl H H H o-tolyl 1-naphthyl H Τ-146 o-tolyl H H H o-tolyl H 1-naphthyl Τ-147 o-tolyl H H H o-tolyl 2-naphthyl H Τ-148 o-tolyl H H H o-tolyl H 2-naphthyl Τ-149 o-tolyl H H H o-lolyl o-biphenylyl H Τ-150 o-tolyl H H H o-tolyl H o-biphenylyl Τ-151 o-tolyl H H H o-tolyl m-biphenylyl H Τ-152 o-tolyl H .H H o-tolyl H m-biphenylyl Τ-153 o-tolyl H H H o-tolyl p-biphenylyl H Τ-154 o-tolyl H H H o-tolyl H p-biphenylyl Τ-155 o-tolyl H H H o-tolyl o-tolyl H Τ-156 o-tolyl. H H H o-tolyl H o-tolyl Τ-157 m-tolyl H H H m-tolyl H H Τ-15Β m-tolyl Ph H Ph m-tolyl H H Τ-159 m-tolyl H Ph H m-tolyl H H Τ-160 m-tolyl H H H m-tolyl Ph H Τ-161 m-tolyl H H H m-tolyl H Ph Τ-162 m-tolyl H H H m-tolyl 1-naphthyl H Τ-163 m-tolyl H H H m-tolyl H 1-naphthyl Τ-164 m-tolyl H H H m-tolyl 2-naphihyl H Τ-165 m-tolyl H H H m-tolyl H 2-naphthy! 丁-166 m-tolyl H H H m-tolyl o-biphenylyl H Τ·167 m-tolyl H H H m-tolyl H o-biphenylyl Τ-168 m-tolyl H H H m-tolyl m-biphenylyl Ή Τ-169 m-tolyl H H H m-tolyl H m-biphenylyl Τ·170 m-tolyl H H H m-tolyl p-biphenylyl H Τ-171 m-tolyl H H H m-tolyl H, p-biphenylyl Τ-172 m-tolyl H H H m-tolyl m-tolyl H Τ-173 m-tolyl H H H m-tolyl H m-tolyl Τ-174 p-tolyl H H H p-tolyl H H Τ-175 p-tolyl Ph H Ph p-tolyl H H Τ-176 p-tolyl H Ph H p-tolyl H H Τ-177 p-tolyl H H H p-tolyl Ph H Τ-178 p-tolyl H H H p-lolyl H Ph Τ-179 p-tolyl H H H p-tolyl 1-naphthyl H Τ-180 p-tolyl H H H p-tolyl H 1-naphthyl Τ-181 p-tolyl H H H p-tolyl 2-naphthyl H Τ·182 p-tolyl H H H · p-tolyl H 2-naphlhyl Τ-183 p-tolyl H H H p-tolyl o-biphenylyl H Τ-184 p-tolyl H H H p-tolyl H o-biphenylyl Τ-185 p-tolyl H H H p-toly! m-biphenylyl H Τ-186 p-tolyl H H H p-tolyl H m-biphenylyl Τ-187 p-lolyl H H H p-tolyl p-biphenylyl H 丁-188 p-tolyl H H H p-tolyl H p-biphenylyl Τ-189 p-tolyl H H H p-tolyl p-tolyl H 丁 ·190 p-tolyl H H H p-tolyl H p-tolyl (請先閲讀背面之注意事項再填寫本頁) ,ιτ 本紙張尺度適用中國國家標準（CNS ) Α4規格（210X297公釐） -150- 581751
A B7 五、發明説明（14碎 R2 r3 R5 R6 R7
Re
οό 2，naphlhyl (2·萘基）ob o-blphenylyl (〇>轵茏基）od m-biphenylyl 071-¾¾ 基） p-biphenylyl o-tolyl (〇* 甲 3 PH3 m-tolyl ㈨·弓 "〇*CH3
DPA-g TPA T-191 Ph T-192 1-naphtyl ΊΜ93 2-naphthyl 丁-194 T-195 o-biphenylyl m-biphenylyl T-196 p-biphenylyl T-197 o-tolyl T:198 m-tolyl Τ-199 p-tolyl Τ-200 Ph Τ-201 1-naphtyl Τ-202 2-naphthyl Τ-203 o-biphenylyl Τ-204 m-biphenylyl ΊΓ-205 p-blphenyJyl Τ-206 o-tolyl Τ-207 m-tolyl Τ-208 p-tolyl Τ-209 Ph Τ-210 Τ-211 Τ-212 1- naphtyl 2- naphthyl o-bipnenylyl Τ-213 m-biphenylyl Τ-214 p-biphenylyl 了-215 o-tolyl Τ-216 m-tolyl Τ·217 p-tolyl Τ-218 Ph Τ-219 1-naphtyl Τ-220 2-naphthyl Τ-221 o-biphenylyl Τ-222 m-biphenylyl Τ-223 p-biphenylyl Τ-224 o-tolyl Τ-225 m-tolyl 丁-226 p-tolyl Τ-227 Ph Τ-22Β 1-naphtyl Τ-229 2-naphthyl Τ-230 o-biphenylyl Τ-231 m-biphenylyl Τ-232 p-biphenylyl 了-233 Ph Τ-234 1-naphlyl Τ-235 2-naphtnyl Τ-236 Τ-237 o-bipnenylyl m-biphenylyl Τ-238 p-biphenylyl Τ-239 Ph Τ-240 1-naphtyl 了 ·241 2-naphthyl 了-242 o-biphenylyl 了-243 m-bipheny^l Τ-244 p-biphenylyl Τ-245 Ph Τ-246 1-naphlyl Τ-247 Τ-248 2-naphthyl o-biphenylyl Τ-249 m-biphenylyl hhh HH HHHH HHHHH HHHHHHHH HHHHHHHH HHHHH HHHHHHHH HHHH H HHHHHHHHHHHH T-250 p-biphenylyl
3 3 3 33 3 3 3 3 H2H H HH Η Η Η Η Η-Γ- -T- -Ch-CPCC.C'CP€H Η H
hhhhh hhhhh hhhhhhh h HH HHH HHHHHHH HHHHH Η HHHHHHHHHHHH HHH HH hhhhhhh h h hhh hhhhh hhhhhhhh hhhhh hhhhhhhh hhhh h h hhhhhhhhhhh
Ph 1- naphtyl 2- naphthyl o-b* m-b p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m*biphenylyl p-biphenylyl o-tolyl m-totyl p-tolyl Ph 1- naphtyl 2- naphthyl o-bipnenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-toly! m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenyiyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl obiphenylyl m-biphenylyl p-biphen>iyl Ph 1- naphlyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl -biphenylyl t-bipherylyl
Η Η Η HH Η Η Η H
H H H 33 3 3 3 3333 ,h:hhhh hhhh 99 9 9 9 99-C9 hhhh h Η Η Η Η -CH3 -CH3 -CH3 •CH3 -CH3 •CH3 •CH3 -CH3 -CH3 Η Η Η Η Η Η DPA DPA DPA DPA DPA DPA Η Η Η Η Η Η ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ
H H H H H H H H H H H H H •CH3 •CH3 -CH3 -CH3 •CH3 -CH3 -CH3 -CH3 •CH3 -CH3 •CH3 -CH3 -CH3 -CH3 •CH3 •CH3 -CH3 -CH3 DPA DPA DPA DPA DPA DPA H H H H H H TPA TPA TPA TPA TPA TPA H H H H H H (請先閲讀背面之注意事項再填寫本頁)
本紙張尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐〉 -151 - 581751 五、發明説明（14d r5 3 7 7 R A B R2
Ri 06 1-naphthy丨（i·系基） 2-naphthyl o-b o-biphenylyl (〇·财ϊ基〉 od m-biphenylyl (m-辑舌基 p»bipheny丨yl (p·聃苯基) T-251 Ph T-252 Ph T-253 Ph T-254 Ph T-255 Ph T-256 Ph T-257 Ph T-258 Ph T-259 1-naphthyl T-260 1-naphthyl T-261 1-naphthyl T-262 1-naphlhyl T-263 1-naphthyl T-264 1-naphthyl T-265 1-naphthyl T-266 2-naphthyl T-267 2-naphthyl T-268 2-naphthyl T-269 2-naphthyl T-270 2-naphthyl T-271 2-naphthyl T-272 o-biphenylyl T-273 o-biphenylyl T-274 o-biphenylyl T-275 o-biphenylyl T-276 o-biphenylyl T-277 m-biphenylyl T-278 m-biphenylyl T-279 T-280 m-biphenylyl m-biphenylyl T-281 p-biphenylyl T-282 p-biphenylyl Τ-2Θ3 p-biphenylyl T-284 O-tolyly Τ-2Θ5 O-tolyly T-286 m-tolyly HHHHH HHHHH Η Η H i H HHHHHH HHHHHH HHHHHH HHH HH Η H H HHHHH H Η Η Η Η Η Η H hhhhhh hhhhhh H HHHHH HHHHHH HHHHHH hhhhhh hhhhhh hhhhhh hhhhhh
Re 1- naphthyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl 2-naphthyl o-biphenyiyl m-biphenylyl p-biphenylyl O-tolyly m-lolyl p-tolyl o-biphenylyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl m-biphenylyl p-biphenylyl O-tolyly m-tolyl p-tolyl p-biphenylyl O-tolyly m-tolyl p-tolyl O-tolyly m-tolyl p-tolyl m-tolyl p-tolyl p-tolyl R7 hhhhh hhhhhhhhhhhhhhhhhhhhhhh hh h hhh h h hhhhhhhhhhhhhhhhhhhhhhhhhhhhhh hhhhhh ---------^-- (請先閲讀背面之注意事項再填寫本頁)
、1T o*tolyl (°*田苯基） ch3 m-tolyl -〇ch3 p-lolyl (p*田苯 5). 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -152- 581751 A7B7 五、發明説明（15d
p*biphenylyl ip·聯苯基） R1 r2 r3 Rs Re «8 υ·1 Η H H H H H H U-2 Ph H H H Ph H H U-3 Ph Ph H H Ph H H ΙΜ Ph H H Ph Ph H H U-5 Ph Ph H Ph Ph H H U-6 Ph H Ph H Ph H H U-7 Ph H H H Ph Ph H U-8 Ph H H H Ph H Ph U-9 Ph H H H Ph Ph Ph LM0 Ph H H H Ph 1-naphthyl H U-11 Ph H H H Ph H 1-naphthyl U-12 Ph H H H Ph 1-naphthyl 1-naphthyl IM3 Ph H H H Ph 2-naphthyl H U-14 Ph H H H Ph H 2-naphthyl υ-15 Ph H H H Ph 2-naphthyl 2-naphthyl U-16 Ph H H H Ph o-biphenylyl H U-17 Ph H H H Ph H o-biphenylyl U-18 Ph H H H Ph o-biphenylyl o-biphenylyl U-19 Ph H H H Ph m-biphenylyl H υ·20 Ph H H H Ph - H m-biphenylyl U-21 Ph H H H Ph m-biphenylyl m-biphenylyl U-22 Ph H H H Ph p-biphenyiyl H υ·23 Ph H H H Ph H p-biphenylyl υ·24 Ph H H H Ph p-biphenylyl p-biphenylyl U-25 1-naphthyl H H H 1-naphthyl H H U-26 1-naphthyl Ph H H 1-naphthyl H H U-27 1-naphthyl H H Ph 1-naphthyl H H U-28 1-naphthyl Ph H Ph 1-naphthyl H H U-29 1-naphlhyl H Ph H 1-naphthyl H H U-30 1-naphthyl H H H 1-naphthyl Ph H U-31 1-naphthyl H H H 1:naphthyl H Ph U-32 1-naphthyl H H H 1-naphthyl Ph Ph U-33 1-naphlhyl H H H 1-naphthyl 1-naphthyl H U-34 1-naphthyl H H H 1-naphthyl H 1-naphthyl U-35 1-naphthyl H H H 1-naphthyl 1-naphthyl 1-naphthyl U-36 1-naphthyl H H H 1-naphthyl 2-naphthyl H U-37 1-naphthyl H H H 1-naphthyl H 2-naphthyl U-38 1-naphthyl H H H 1-naphthyl 2-naphthyl 2-naphlhyl υ·39 1-naphthyl H H H 1-naphthyl o-biphenylyl H U-40 1-naphthyl H H H 1-naphthyl H o-biphenylyl U-41 1-naphthyl H H H 1-naphthyl o-biphenylyl o-biphenylyl U-42 1-naphthyl • H H H 1-naphthyl m-blphenylyl H U-43 1-naphthyl H H H 1-naphthyl H m-biphenylyl U-44 1-naphthyl H H H 1-naphthyl m-biphenylyl m-biphenylyl U-45 1-naphthyl H H H 1-naphthyl p-biphenylyl H U-46 1-naphlhvl H H H 1-naphthyl H p-biphenylyl U-47 1-naphthyl H H H 1-naphthyl p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) C0 1-naphthyl (1-萘基） 2-naphthyl (2-萘基） ob o^biphenylyl (〇-聯苯基） od * m-bipheny丨yl (m-聯本基） •153- 本紙乐尺度適用中國國家標準（CNS ) A4洗格（210X297公釐） 581751 A7 B7 五、發明説明（151)
C0 1 «naphthyl (1-蔡基）
£λ币-Τ9Π 才 i ,»7rr vl d VJV 2-naphthyl (2-萘基） o-Wphenylyl (〇·聯苯基） od m-biphenylyl (m-聯苯基） p-biphenyly丨（ρ·聯苯基） Ri r2 R3 r5 Re R7 Re LM8 2-naphthyl H H H 2-naphthyl H H LM9 2-naphthyl Ph H H 2-naphthyl H H U-50 2-naphthyl H H Ph 2-naphthyl H H U-51 2-naphthyl Ph H Ph 2-naphthyl H H U-52 2-naphthyl H Ph H 2-naphthyl H H U-53 2-naphthyl H H H 2-naphthyl Ph H U-54 2-naphthyl H H H 2-naphthyl H Ph U-55 2-naphthyl H H H 2-naphthyl Ph Ph U-56 2-naphthyl H H H 2-naphthyl 1-naphthyl H U-57 2-naphthyl H H H 2-naphthyl H 1-naphthyl U-5B 2-naphthyl H H H 2-naphthyl 1-naphthyl 1-naphthyl U-59 2-naphthyl H H H 2-naphthyl 2-naphthyl H U-60 2-naphthyl H H H 2-naphthyl H 2-naphthyl U-61 2-naphthyl H H H 2-naphthyl 2-naphthyl 2-naphthyl U-62 2-naphthyl H H H 2-naphthyl o-biphenylyl H U-63 2-naphthyl H H H 2-naphthyl H o-biphenyfyl U-64 2-naphthyl H H H 2-naphthyl o-biphenyiyl o-biphenylyl U-65 2-naphthyl H H H 2-naphthyl m-blphenylyl H U-66 2-naphlhyl H H H 2-naphthyl H m-biphenylyl U-67 2-naphthyi H H H 2-naphthyl m-bipheny)yl m-bipheriyiyl U-6B 2-naphthyl H H H 2-naphthyl p-biphenylyl H U-69 2-naphlhyl H H H 2-naphthyl H p-biphenylyl U-70 2-naphthyl H H H 2-naphthyl p-biphenylyl p-biphenylyl U-71 o-biphenylyl H H H o-biphenytyl H H U-72 o-biphenylyl Ph H H o-biphenylyl H H U-73 o-biphenylyl H H Ph o-biphenylyl H H U-74 o-biphenylyl Ph H Ph o-biphenylyl H H U-75 o-biphenylyl H Ph H o-biphenylyl .H H U-76 o-biphenylyl H H H o-biphenylyl Ph H U-77 o-biphenylyl H H H o-biphenylyl H Ph U-78 o-biphenylyl H H H o-biphenylyl Ph Ph U-79 o-biphenylyt H H H o-biphenylyl 1-naphthyl H U-B0 o-biphenylyl H H H o-biphenylyl H 1-naphlhyl U-81 o-biphenyfy! H H H o-biphenylyl 1-naphthyl 1-naphthyl υ·82 o-biphenyiyl H H H o-biphenylyl 2-naphthyi H U-83 · o-biphenylyl H H H o-biphenylyl H 2-naphthyl U-84 o-biphenytyl H H H D-biphenylyl 2-naphthyl 2-naphthyl U-85 o-biphenylyl H H H o-blphenylyl o-biphenylyl H U-86 o-biphenylyl H H H o-biphenylyl H o-biphenylyl U-87 o-biphenylyl H H H o-biphenylyl o-blphenylyl o-biphenylyl U-88 o-biphenylyl H H H o-biphenylyl m-blpheny)yl H U-89 o-bipheny}yl H H H o-biphenylyl H m-biphenylyl U-90 o-biphenylyl H H H o-biphenylyl m-biphenylyl m-biphenylyl U-91 o-biphenylyl H H H o-biphenylyl p-biphenylyl H ΙΙ·92 o-biphenylyl H H H o-biphenylyl H p-biphenylyl U-93 o-biphenylyl H H H o-biphenylyl p-biphenylyl p-biphenyfyl (請先閲讀背面之注意事項再填寫本頁) 本纸張尺度適用中國國家標準（CNS ) Α4規格（210X297公釐） -154· 581751 A7 B7 五、發明説明（152)
TypcU C0 1 «naphthyl 萘基） 2-naphthyl (2-蔡基） ob o-blphenyly丨（〇·聯苯基） Qr<S 钟 nvbiphenyly丨（m·聯苯基） p»biphenylyl (ρ·聯苯基） Ri r2 r3 Rs Re R7 Re U-94 m-biphenylyl H H H m-biphenylyl H H U-95 m-blphenylyl Ph H H m-biphenylyl H H U-96 m-biphenylyl H H Ph m-biphenylyl H H U-97 m-biphenylyl Ph H Ph m-biphenylyl H H U-98 m-blphenylyl H Ph H m-blphenylyl H H U-99 m-biphenylyl H H H m-biphenylyl Ph H U-100 m-biphenylyl H H H m-biphenylyl H Ph ύ-101 m-biphenylyl H H H m-biphenylyl Ph Ph U-102 m-biphenylyl H H H m-biphenylyl 1-naphthyl H U-103 m-biphenylyl H H H m-biphenylyl H 1-naphthyl U-104 m-biphenylyl H H H m-biphenylyl 1-naphthyl 1-naphthyl U-105 m-biphenylyl H H H m-biphenylyl 2-naphthyl H U-106 m-biphenylyl H H H m-biphenylyl H 2-naphthyl U-107 m-biphenylyl H H H m-biphenylyl 2-naphlhyl 2-naphthyl U-108 m-biphenylyl H H H m-biphenylyl o-biphenylyl H U-109 m-biphenylyl H H H m-biphenylyl H o-blphenylyl U-110 m-biphenylyl H H H m-biphenylyl o-biphenylyl o-biphenylyl U-111 m-biphenylyl H H H m-biphenylyl m-biphenylyl H U-112 m-biphenylyl H H H m-biphenylyl H m-biphenylyl U-113 m-biphenylyl H H H m-biphenylyl m-biphenylyl m-biphenylyl U-114 m-biphenylyl H H H m-biphenylyl p-biphenylyl H U-115 m-blphenylyl H H H m-biphenylyl .H p-biphenylyl U-116 m-blphenylyl H H H m-biphenylyl p-blphenylyl p-biphenylyl U-117 p-biphenyiyl H H H p-biphenylyl H H U-118 p-biphenylyl Ph H H p-blphenylyl H H U-119 p-biphenylyl H H Ph p-biphenylyl H H U-120 p-biphenylyJ Ph H Ph p-biphenylyl H H U-121 p-biphenylyl H Ph H p-blphenylyl H H U-122 p-biphenylyl H H H p-biphenylyl Ph H U-123 p-biphenylyl H H H p-biphenylyl H Ph U-124 p-blphenylyi H H H p-biphenylyl Ph Ph U-125 p-biphenylyl H H H p-biphenylyl 1-naphthyl H U-126 p-biphenylyl H H H p-biphenylyl .H 1-naphthyl U-127 p-biphenylyl H H H p-biphenylyl 1-naphthyi 1-naphthyl U-128 p-blphenylyl H H H p-biphenylyl 2-naphthyl H U-129 p-biphenylyl H H H p-biphenylyl H 2-naphthyl U-130 p-biphenylyl H H H p-biphenylyl 2-naphthyl 2-naphthyl U-131 p-biphenyfyl H H H p-biphenylyl o-biphenylyl H U-132 p-biphenylyl H H H prbiphenylyl H o-biphenylyl U-133 p-biphenylyl H H H p-blphenyJyl o-biphenylyl o-biphenylyl U-134 p-biphenylyl H H H p-blphenylyl m-biphenylyl H U-135 p-biphenylyl H H H p-biphenylyl H m-biphenylyl U-136 p-biphenylyl H H H p-biphenylyl m-biphenylyl m-biphenylyl U-137 p-biphenylyl H H H p-biphenylyl p-biphenylyl H U-138 p-biphenylyl H H H p-biphenylyl H p-biphenylyl U-139 p-biphenylyl H H H p-blphenylyl p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CN’S ) Α4規格（210X29*7公釐） -155- 581751 A7 B7 五、發明説明（153) U-140 U-141脱 = U-144 U-145 U-146 U-147 U-148 U-149 U-150 U-151 U-152 U-153 U-154 U-155 I U-156 CO U·157 U-158 U-159 U-160 U-161 U-162 r\)-\ υ·ΐ63 wvy U-164 o*biphenylyl 0-¾¾基） υ·165 / υ·166 〇-〇 U-167 m-biphenylyl >m-ife5S；U-168 U-169 〇〇- U-170 p-biphenylyl (p-b»5S) u"171 U-172 U-173 U-174 U-175 U-176 U-177 U-178 U-179 U-180 U-181 U-182 U-183 U-184 U-185 U-186 U-187 U-188 U-189 U-190
TypeU 1-naphthyl 2-naphthyl (2·菜基） % o-tolyl <°* 田苯塞） ch3 m-tolyl -〇ch3 prolyl <p·田苯基）
Ri r2 r3 R5 Re r7 Re o-tolyl H H H o-tolyl H H o-tolyl Ph H Ph o-tolyl H H o-tolyl H Ph H o-tolyl H H o-tolyl H H H o-tolyl Ph H o-tolyl H H H o-tolyl H Ph o-tolyi H H H · o-tolyl 1-naphthyl H o-tolyl H H H o-tolyl H 1-naphthyl o-toJyl H H H o-tolyl 2-naphthyl H o-tolyl H H H o-tolyl H 2-naphthyl o-tolyl H H H o-tolyl o-biphenylyl H o-tolyl H H H o-tolyl H o-biphenylyl o-tolyl H H H o-tolyl m-biphenylyl H o-tolyl H H H o-tolyl H m-biphenylyl o-tolyl H H H o-tolyl p-biphenylyl H o-tolyl H H H o-tolyi H p-biphenylyi o-tolyl H H H o-tolyl o-tolyl H o-tolyl H H H o-tolyl H o-tolyl m-tolyl H H H m-tolyl H H m-tolyl Fh H Ph m-tolyl H H m-tolyl H Ph H m-tolyl H H m-tolyl H H H m-tolyl Ph H m-tolyl H H H m-tolyl H Ph m-tolyl H H H m-tolyl 1-naphthyl H m-tolyl H H H m-tolyl H 1-naphthyl m-tolyl H H H m-tolyl 2-naphlhyl H m-tolyl H H H m-tolyl H 2-naphthyl m-tolyl H H H m-tolyl o-biphenylyl H m-tolyl H H H m-tolyl H o-biphenylyl m-tolyl H H H m-tolyl m-biphenylyl H m-toiyl H H H m-tolyl H m-biphenylyl m-tolyl H H H m-tolyl p-biphenyly! H m-tolyl H H H m-tolyl H p-biphenylyl m-tolyl H H H m-tolyl nvtolyl H m-tolyl H H H m-tolyl H nvtolyl p-toiy) •H H H p-tolyl H H p-tolyl Ph · H Ph p-tolyl H H p-tolyl H Ph H p-tolyl H H p-tolyl H H H p-tolyl Ph H p-tolyl H H H p-tolyl H Ph p-tolyl' H H H p-tolyl 1-naphthyl H p-tolyl H H H p-tolyl H 1-naphthyl p-tolyl H H H p-tolyl 2-naphthyl H p-tolyl H H H p-tolyi H 2-naphthyl p-tolyl H H H p-tolyl o-biphenylyl H p-tolyt H H H p-tolyl H o-biphenylyl p-tolyl H H H p-tolyl m-biphenylyl H p-tolyl H H H p-tolyl H m-biphenylyl p-tolyl H H H p-tolyl p-biphenylyl H p-tolyl H H H p-tolyl H p-biphenylyl p-tolyl H H H p-tolyl p-tolyl H p-tolyl H H H p-tolyl H p-iolyl (請先閲讀背面之注意事項再填寫本頁 訂 本纸法尺度適用中國國家標準（CNS ) A4洗格（210X297公釐） -156- 581751 A7 B7 五、發明説明（154)
Ri
Re .00 1-naphthyl 2-naphthyl U-191 U-192 U-193 U-194 U-195 U-196 U-197 U-198 U-199 U-200 U-201 U-202 U-203 U-204 U-205 U-206 U-207 U-208 U-209 U-210 U-211 U-212 U-213 U-214 U-215 U-216 U-217 U-218 U-219 ob o-biphenylyl (〇-聯苯基）U-220 U-221〇d 賺 m-biphenylyl (
Ph 1- naphtyl 2- naphthyl o-biphenylvl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl
DPA
TFA p-biphenylyl (p-a»5g) H3C o-tolyl 甲苯基） CH3 m-tolyl <ni-甲苯*) -〇ch3 p-tolyl U-224 o-tolyl U-225 m-tolyl U-226 p-tolyl U-227 Ph U-228 1-naphtyl U-229 2-naphthyl U-230 o-biphenylyl U-231 m-biphenylyl U-232 p-biphenylyl U-233 Ph U-234 1-naphtyl U-235 U-236 U-237 2-naphthyl o-biphenylyl m-biphenylyl U-238 p-biphenylyl U-239 Ph U-240 1-naphtyl U-241 U-242 2-naphthyl o-biphenytyl U-243 m-biphenylyl U-244 p-biphenylyl U-245 Ph U-246 1-naphlyl U-247 2-naphlhyl U-248 o-biphenylyl U-249 m-biphenylyl U-250 p-biphenylyl
HHH HH hhhhhhh h h hhh hhhhh hhhhhhh h hhhhh hhhhhhhh hhhh h h hhhhhhhhhhh 3 3 3 33 3 3 3 3 ^ η h hhh hhhhh hhhhhhh η HH HHH HHHHHHHH HHHH Η H HHHHHHHHHHH hhhhh hhhhhhhh h hhhhhhhh h hhh HH Η Η HH HHH HHHHHHHH HHHH Η H HHHHHHHHHHH
Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-bipheny!yl p-biphenylyl o-tolyl m-tolyl p-to)yl Ph 1- naphtyl 2- naphlhyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphtliyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyt p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl. o-biphenylyl m-biphenylyl p-biphenyiyl Ph 1- naphtyl 2- naphthyl o-biphenyiyl m-biphenylyl p-biphenylyl Ph · 1- naphtyl 2- naphlhyl o-biphenylyl m-bipheny^l p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl
R7I HH H HH HH HH-CH3:CCHH33-CH3-CH3-CH3-CH3:CCHH33HHHH
R8I hhhhh hhhhhhh h h hhhh
H
H H . H H -CH3 -CH3 •CH3 •CH3 •CH3 -CH3 -CH3 •CH3 •CH3 H H H H H H DPA DPA DPA DPA DPA DPA H H H H H TPA TPA TPA TPA TPA TPA
H3H3H31H3H3H3H3H3IHHHHAAA Η HHH Η Η (請先閲讀背面之注意事項再填寫本頁) 訂 線 本紙張尺度逍用中國國家標準（CNS ) A4規格（210X297公釐） -157- 581751
A Β7 五、發明説明（155)
C0 1-naphthyl (1-萘基） 2-naphlhy丨（2-萘基）ob o-biphenylyl (〇·聯苯基）od m-biphenylyl (m-聯苯基)
p-biphenylyl (P~聯苯基) H3C U-251 U-252 U-253 U-254 U-255 U-256 U-257 U-258 U-259 U-260 U-261 U-262 U-263 U-264 U-265 U-266 U-267 U-268 U-269 U-270 U-271 U-272 U-273 U-274 U-275 U-276 U-277 U-278 U-279 U-280 U-281 U-282 U-283 U-284 U-285 U-286* _Rl_ Ph Ph Ph Ph Ph Ph Ph Ph 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1- naphthyl 2- naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl o-biphenylyl o-biphenylyl o-blphenylyl o-blphenylyl o-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-bjpheny^l O-tolyly CD-tolyly m-tolyly ηηηηηηηηηηηηηηηηηηηηηηηηηηηη ΗΗ ΗΗΗΗ ΗΗ ηηηηηηηηηηηηηηηηηηη ΗΗΗΗΗΗΗΗΗ ΗΗ Η ΗΗΗ Η Η
Rb R7
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訂 o-tolyl (o·®苯基） CH, m-tolyl (τη.®苯基） ^0CH3 p-to)yl (p·® 苯基） 本紙伕尺度適用中國國家標準（CNS ) Α4規格（210Χ297公釐） -158- 581751 Α7 Β7 五、發明説明（ιθ r2 r3 R4 r5
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Η Η Η Η Η Η Η Η Η Η Η Η (請先閲讀背面之注意事項再填寫本頁) 衣· 訂 •161 - 581751 A7 B7 五、發明説明（15$ R2 R5
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TypeX Χ-4 Χ·5 Χ·6 Χ-7 Χ·8 Χ-9 Χ·10 Χ-11 Χ·121-naphthy丨（1·萘基） Χ-14 Χ·15 2^aihyl (2-萘基）Χ·16 Χ-17 Χ-18 Χ-19 'Χ-20 -」 Χ-21 〇-〇 Χ·22 m-blphenyly 丨(m-聯苯基)Χ·23 Χ·24 Χ-25 Χ-26 〇6 o-b o-biphenylyl (〇·聯苯基） p*blpheny丨y丨(ί>聯苯基) Χ·27 Χ·28 Χ-29 Χ·30 Χ-31 Χ-32 Χ33 Χ-34 Χ-35 Χ-36 Χ-37 Χ-3Θ Χ-39 Χ-40 Χ-41 Χ-42 Χ-43 Χ-44 Χ-45 Χ·46 Χ-47 Χ·1 Ri r2 r3 R4 R5 r7 Re Η H H H H H H Ph H H H H H • H Ph Ph H H Ph H H . Ph H Ph Ph H H H Ph H Ph H H H H Ph H H Ph H H H Ph H .H H H Ph H Ph H H H H H Ph Ph H H H H Ph Ph Ph H H H H 1-naphthyl H Ph H H H H H 1-naphthyl Ph H H H H 1-naphthyl 1-naphthyl Ph H H H H 2-naphthyl H Ph H H H H H 2-naphthyl Ph H H H H 2-naphthyl 2-naphthyl Ph H H H H o-biphenylyl H Ph H H H H H o-biphenylyl Ph H H H H o-biphenylyl o-biphenylyl Ph H H H H m-biphenylyl H Ph H H H H H m-biphenylyl Ph H H H H m-biphenylyl m-biphenylyl Ph H H H H p-biphenylyl H Ph H H H H H p-biphenylyl Ph H H H H p-biphenylyl p-biphenylyl 1-naphthyl · H H H H H H . 1-naphthyl Ph H H Ph H H 1-naphthyl H Ph Ph H H H 1-naphthyl H Ph H H H H 1-naphthyl H H Ph H H· H 1-naphthyl H H H H Ph H 1-naphthyl H H H H H Ph 1-naphthyl H H H H Ph Ph 1-naphthyl H H H H 1-naphthyl H 1-naphthyl H H H H H 1-naphthyl 1-naphthyl H H H H 1-naphlhyl 1-naphthyl 1-naphthyl H H H H 2-naphthyl H 1-naphthyl H H H H H 2-naphthyl 1-naphthyl H H H H 2-naphthyl 2-naphthyl 1-naphthyl H H H H o-biphenylyl H 1-naphthyl H H H H H o-biphenytyl 1-naphthyl H H H H o-biphenylyl o-biphenylyl 1-naphthyl H H H H m-biphenylyl H 1-naphthyl H H H H H m-biphenylyl 1-naphthyl H H H H m-biphenylyl m-biphenytyl 1-naphthyl H H H H p-biphenylyl H 1-naphlhyi H H H H H p-biphenylyl 1-naphthyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本纸乐尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -171 - 581751 A7 B7 五、發明説明（ 169
R3 r2 o-b o-bipheny)ylo-d m-biphenyly) C0 1-naphthyl (1-萘基） (P·聯苯基) p-biphenylyl (P~ 聯苯基) Ri r2 r3 R4 r5 r7 Re X-48 2-naphthyl H H H H H H Χ·49 2-naphthyl Ph H H Ph H H Χ-50 2-naphthyl H Ph Ph H H H Χ-51 2-naphthyl H Ph H H H H Χ-52 2-naphthyl H H Ph H H H Χ-53 2-naphthyl H H H H Ph H Χ-54 2-naphthyl H H H H H Ph Χ·55 2-naphthyl H H H H Ph Ph Χ-56 2-naphthyl H H H H 1-naphthyl H Χ-57 2-naphthyl H H H H H 1-naphthyl Χ-58 2-naphthyl H H H H i-naphthyl 1-naphthyl Χ·59 2naphthyl H H H H 2-naphthyl H Χ-60 2-naphthyl H H H H H 2-naphthyl Χ-61 2-naphthyl H H H H 2-naphthyl 2-naphthyl Χ-62 2-naphthyl H H H H o-biphenylyl H Χ-63 2-naphthyl H H H H H o-biphenylyl Χ-64 2-naphthyl H H H H o-biphenylyl o-biphenylyl Χ-65 2-naphthyl H H H H m-biphenylyl H Χ-66 2-naphthy) H H H H H m-biphenylyl Χ-67 2-naphthyl H H H H m-biphenylyl m-biphenylyl Χ-68 2-naphthyl H H H H p-biphenylyl H Χ·69 2-naphthyl H H H H H p-biphenylyJ Χ-70 2-naphthyl H H H H p-biphenylyl p-biphenylyl Χ-71 o-biphenylyl H H H H H H Χ·72 o-biphenylyl Ph H H Ph H H Χ·73 o-biphenylyl H Ph Ph H H H Χ-74 o-biphenylyl H Ph H · H H H Χ-75 o-biphenylyl H H Ph H H H Χ·76 o-biphenylyl H H H H Ph H Χ-77 o-biphenylyl H H H H H Ph Χ-78 o-biphenylyl H H H H Ph Ph Χ-79 o-biphenylyl H H H H 1-naphthyl H Χ-ΒΟ o-biphenylyl H H H H H 1-naphthyl Χ-81 o-biphenylyl H H H H 1-naphthyl 1-naphthyl Χ-82 o-biphenylyl H H H H 2-naphthyl H Χ·83 o-biphenylyl H H H H H 2-naphthyl Χ-84 o-biphenylyl H H H H 2-naphthyl 2-naphthyl Χ·85 o-biphenylyl H H H H o-biphenylyl H Χ-Β6 o-biphenylyl H H H H H o-biphenylyl Χ·87 o-biphenylyl H H H H o-biphenylyl o-biphenylyl Χ·88 o-bipheny)yl H H H H m-biphenylyi H Χ·89 o-biphenylyl H H H H H m-biphenylyl Χ·90 o-biphenylyl H H H H m-biphenylyl m-biphenylyl Χ-91 o-biphenylyl H H H H p-biphenylyl H Χ-92 o-biphenylyl H H H H H p-biphenylyl Χ·93 o-biphenylyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁)
本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -172- 581751 A7 B7 五、發明説明（ 170
Ri
〇6 1-naphthyl (1-萘基） 2-naphthyl (2-¾¾) X-94 X-95 Χ·96 Χ-97 Χ-9Θ Χ-99 Χ-100 Χ-101 Χ-102 Χ-103 Χ-104 Χ-105 Χ-106 Χ-107 Χ-108 Χ-109 Χ·110 Χ111 o»bipheny丨yl (〇·聯苯基）Χ·” 1 Χ-112 Χ-113 Χ-114 Χ-115 Χ-116 ck5 m-biphenylyl (m-聯苯基) 經濟部智慧財凌(工消骨合itfi印¾ p-biphenylyl (p·聯苯基）. X-117 Χ·118 X-119 X-120 X-121 X-122 X-123 X-124 X-125 X-126 Χ·127 Χ·128 X-129 X-130 X-131 X-132 X-133 X-134 X-135 X-136 X-137 X-138 X-139 m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p>biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenyly! p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl r2 r3 r4 r6 r7 Rb Η Η Η Η Η H Ph Η Η Ph Η H Η Ph Ph Η Η H Η Ph Η Η Η H Η Η Ph Η Η H Η Η Ή Η Ph H Η Η Η Η Η Ph Η Η Η Η Ph Ph Η Η Η Η 1-naphthyl H Η Η Η Η Η 1-naphthyl Η Η Η Η 1-naphthyl 1-naphthyl Η Η Η Η 2-naphthyl H Η Η Η Η Η 2-naphthyl Η Η Η Η 2-naphthyl 2-naphthyl Η Η Η Η o-biphenylyl H Η Η Η Η Η o-biphenylyl Η Η Η Η o-biphenylyl o-biphenylyl Η Η Η Η m-biphenylyl H Η Η Η Η H m-biphenylyl Η Η Η Η m-biphenylyl m-biphenylyl Η Η Η Η p-biphenylyl H Η Η Η Η H p-biphenylyl Η Η Η Η p-biphenylyl p-biphenylyl Η Η Η Η H H Ph Η Η Ph H H Η Ph Ph_ Η H H Η Ph Η Η H H Η Η. Ph Η H H Η Η Η Η Ph H Η Η Η Η H Ph Η Η Η Η Ph Ph Η Η Η Η 1-naphthyl H Η Η Η Η H 1-naphthyl Η Η Η Η 1-naphthyl 1-naphthyl Η Η Η Η 2-naphthyl H Η Η Η Η H 2-naphthyl Η Η Η Η 2-naphthyl 2-naphthyl Η Η Η Η o-biphenylyl H Η Η Η Η H o-biphenylyl Η Η Η Η o-biphenylyl o-biphenylyl Η Η Η Η m-biphenylyl H Η Η Η Η H m-biphenylyl Η Η Η Η m-biphenylyl m-biphenylyl Η Η Η Η p-biphenylyl H Η Η Η Η H p-biphenylyl Η Η Η Η p-biphenylyl p-biphenylyl (請先閎讀背面之注意事項再填寫本頁) 本纸乐尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） 173- 581751
A B7 五、發明説明（171) R1 R2
r3 r2 C0
Vnaphthyl (丨·系基） 2-naphthyl 〇 莕基）ob o-biphenylylod m-biphenylyl (m·取茏基) p^bipheny丨y丨（p·辑苯基） % o-tolyl (o-^s*)I nvtolyl (m-田苯基） -〇ch3 p-tolyl (p·田 3基） X-140 ,X-141 X-142 X-143 X-144 X-145 X-146 X-147 X-148 X-149 X-150 X-151 X-152 X-153 X-154 X-155 X-156 X-157 X-158 X-159 X-160 X-161 X-162 X-163 X-164· X-165 X-166 X-167 X-168 X-169 X-170 X-171 X-172 X-173 X-174 X-175 X-176 X-177 X-178 X-179· Xr180 X-181 X-182 X-183 X-184 X-185 X-186 X-187 Χ-18Θ Χ·189 X-190 o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-toiyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl p-tolyl p-tolyl p-tolyl p-to)y> p-tolyl p-tolyl p-tolyl p-to)yf p-toly! p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl
H Ph H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H H H h^hh hhhhhhhhhhhhhh hhhhhhhhhhhhhhh hh^hhhhhh hhhhhhhh Η H^HH hhhh hhhhhhh hhh hhhhhhhhhhhhhhh hh^hhhhhhhhhhhhhh R5 Η phhh hhhhhhhhhhhhh^ hhhhhhhhhhhhhhh HphHHHHHHHHHHHHH Η H «7 Re Η Η Η Η Η Η Ph Η Η Ph 1-naphthyl Η Η 1-naphthyl 2-naphthyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p-biphenylyl o-tolyl Η Η o-toiyl Η Η Η Η Η Η Ph Η Η Ph 1-naphthyl Η Η 1-naphthyl 2-naphlhyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p>biphenylyl m-tolyl Η Η m-tolyl Η Η Η Η Η Η Ph Η Η Ph 1-naphthyl Η Η 1-naphlhyl 2-naphthyl Η Η 2-naphthyl o-biphenylyl Η Η o-biphenylyl m-biphenylyl Η Η m-biphenylyl p-biphenylyl Η Η p-biphenylyl p-tolyl Η Η p-tolyi (請先閲讀背面之注意事項再填寫本頁)
本纸沬尺度適用中國國家標率（CNS ) A4*i格（210X297公釐） -174 ‘ 581751
A B7 五、發明説明（172)
TypeX R1 C0 1-naphthyl 〇 2-naphthyl (- o-b o*biphenylyl 苯基） Χ-191 Ph Χ-192 1-naphtyl Χ-193 2-naphthyl Χ-194 o-biphenylyl Χ-195 m-biphenylyl Χ-196 p-biphenylyl Χ-197 Χ-198 o-tolyl m-tolyl Χ-199 p-tolyl Χ-200 Ph Χ-201 1-naphtyl Χ-202 2-naphthyl Χ-203 o-biphenylyl Χ-204 m-biphenylyl Χ-205 p-biphenylyl Χ-206 o*tolyl Χ-207 m-tolyl Χ-208 p-tolyl Χ-209 Ph Χ-210 1-naphtyl Χ-211 Χ-212 2-naphthyl o-biphenylyl Χ-213 m-biphenyiyl Χ-214 p-biphenylyl Χ-215 Χ-216 o-tolyl m-tolyl Χ-217 p-totyi Χ-218 Ph Χ-219 1-naphtyl o-d
CyO
DPA
心g TPA CH> p»bipheny丨y丨（p·取苯基） H3C o*tolyl (〇·甲 s基） CH3 m-tolyl (m·田苯基） p-tolyl (p·田苯基） X-221 o-biphenylyl X-222 m-biphenylyl X-223 p-biphenylyJ X-224 o-tolyl X-225 nvtolyl X-226 p-tolyl X-227 Ph X-228 1-naphtyl X-229 X-230 2-naphthyl o-bipnenylyl X-231 m-biphenylyl Χ·232 p-biphenylyl X-233 Ph X-234 1-naphtyl X-235 X-236 X-237 2-naphthyl o-bipnenyiyl m-biphenylyl X-23B p-biphenylyl X-239 Ph X-240 1-naphtyi X-241 2-naphlhyl X-242 o-biphenylyl X-243 m-biphenylyl X-244 p-biphenylyl X-245 Ph X-246 1-naphtyl X-247 2-naphthyl X-248 o-biphenylyl X-249 m-biphenylyl X-250 y>-biphenylyi
R3I ^ Η H HHH HHHHH HHHH HH Η Η HHHHH HHHHHHH H HHHH H HHHHHHH^HHHH R2I HHH HH HHHHHHH Η H HHH HHHHH HHHHHHHH HHHHH HHHHHHHH HHHH Η H HHHHHHHHHHH R7 Rs R4
H3H3H3H3H3H3H3H3H3HHHHH3H3H3H3H3A A AAA A A A A A A A HHHHH HHHH9-c-c-c9-c-CH-ch-CJHH H HH HHHHH-C99 9-C99-C9HH H hhhdpdpdpdpdpdphhhhhhtptptptptptp H HH HH HHHHHHH Η Η HHHHHHHH HHHHHHH Η HH HH H HHH HHH Η Η HHHH Η Η HHHHHHHHHHH ^^hhh H H hhhhhhhh hhhhhhhh hhhh H HHHHHHHH HHHH Η H HHHHHHHHHHH rb
HHH HH HHH
H Η Η Η Η Η Η Η Η Η -CH3 •CH3 •CH3 •CH3 -CH3 -CH3 -CH3 •CH3 -CH3 •CH3 •CH3 •CH3 •CH3 •CH3 -CH3 -CH3 •CH3 •CH3 DPA DPA DPA ΏΡΑ DPA DPA Η Η Η Η Η Η 丁 ΡΑ ΊΡΑ ΤΡΑ ΤΡΑ ΤΡΑ ΤΡΑ
Η HHH Η H (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) Α4規格（210X297公釐） -175- 581751 A7 B7 五、發明説明（173)
Ri r2
C0 1-naphthyl 0·萘基） 2-naphthyl (2·蔡基）ob * o-blphenylyl (〇*聯本基）od 钟 m-biphenylyl (m-聯本基） p»biphenylyl (P-聯苯基） Χ·-1 Χ，·2 Χ，-3 Χ'-4 Χ.-5 Χ·-6 Χ··7 Χ··8 Χ*-9 Χ·-10 Χ·-11 ΧΜ2 Χ··13 Χ·-14 Χ.·15 Χ*-16 Χ·-17 Χ·-18 Χ*-19 Χ··20 , Χ··21 Χ*·22 Χ.-23 Χ'-24 Χ，-25 Χ·-26 Χ.-27 Χ··28 Χ··29 Χ，·30 Χ·-31 Χ··32 Χ·-33 Χ*·34 Χ·-35 Χ·-36 Χ.-37 Χ··38 Χ，·39 ΧΜΟ Χ'-41 Χ*-42 Χ'-43 ΧΜ4 Χ·*45 Χ*-46 Χ··47 Η Ph Ph Ph Ph Ph Ph Ph Ph Ph .Ph' Ph Ph Ph Ph Ph Ph Ph Ph Ph· Ph Ph Ph Ph 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl
H H Ph H H H H H H H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H H H H H H H H R hhh^^hhhh hhh hhhhhhhhhhhh hh ^^hhhh hhhh hhhhhhhh hhh R4 r5 r7 Re Η Η Η H Η Η Η H Η Ph Η H Ph Η Η H Η Η Η H Ph Η Η H Η Η Ph H Η Η Η Ph Η Η Ph Ph Η Η 1-naphthyl H Η Η Η 1-naphthyl Η Η 1-naphthyl 1-naphthyl Η Η 2-naphthyl H Η Η Η 2-naphthyl Η Η 2-naphthyl 2-naphthyl Η Η o-biphenylyl H Η Η Η o-biphenylyl Η Η o-biphenylyl o-biphenylyl Η Η m-biphenyiy! H Η Η H m-biphenylyl Η Η m-biphenylyl. m-biphenylyl Η Η p-biphenylyl H Η Η H p-biphenylyl Η Η p-biphenylyl p-biphenylyl Η Η H H Η Ph H H Ph Η H H Η Η H H Ph Η H H Η Η Ph H Η Η H Ph Η Η Ph Ph Η Η 1-naphthyl H Η Η H 1-naphthyl Η Η 1-naphthyl 1-naphthyl Η Η 2-naphthyl H Η Η H 2-naphthyl Η Η 2-naphthyl 2-naphthyl Η Η o-biphenylyl H Η . Η H o-biphenylyl Η Η o-biphenylyl o-bipheny!yl Η Η m-biphenylyl H Η Η H m-biphenylyl Η Η m-biphenylyl m-biphenylyl Η Η p-biphenylyl H Η η' H p-biphenylyl Η Η p-biphenylyl p-biphenylyl I 裝 訂 線 (請先閱讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -176- 581751 A7 B7 五、發明説明（1M) R7
2-naphlhyl 2-naphthyl 2-naphihyl 2-napht)iyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2naphthyi 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphlhyl 2-naphthyl 2-naphthyl 2-naphthyl
1 IiI π A n h s.\L· P
Pbipheny丨yl(p·聯苯基）X·71⑽钟卽州1 X-72 o-biphenylyl Χ·-73 o-biphenylyl X'-74 o-biphenylyl Χ·-75 o-blphenylyl χ··76 o-biphenylyl X，-77 o-biphenylyl X'-78 o-biphenylyl Χ*·79 〇.biphenyiyl x ·β0 o-biphenylyl Χ··Β1 o-biphenylyl Χ*·82 〇-biphenylyl Χ··83 o-biphenylyl X.-64 〇-biphenylyl X*-85 o-biphenylyl X'-86 o-biphenylyl X.-87 o-biphenylyl X'-88 o-biphenylyl X-89 o-biphenylyl X-90 o-biphenylyl X-91 o-biphenyiyl X'-S2 o-biphenylyl X'-93 o-biphenylyl
Ri r2 r3 FU Rs Η Η Η Η Ph Η Η Ph Η Ph Ph Η Η Ph Η Η Η Η Ph Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Ph Η Η Ph Η Ph Ph Η Η Ph Η Η Η Η Ph Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η . Η Η Η Η Η ι Η Η Η Η Η Η Η Η Η Η Η Η r7
Re
H H H H H Ph H Ph 1-naphthyl H 1- naphthyl 2- naphthyl H 2-naphthyl o-biphenylyl H H H H H H H Ph Ph H 1-naphthyl 1- naphthyl H 2- naphthyl 2-naphthyl H o-biphenylyl o-biphenylyl H m-biphenylyl m-biphenylyl H p-biphenylyl p-biphenylyl H Η H Η H Η H Η H Η H Ph H Η Ph Ph Ph 1-naphthyl H Η 1-naphthyl 1-naphthyl 1-naphthyl 2-naphthyl H Η 2-naphthyl 2-naphthyl 2-naphthyl o-biphenylyl H Η o-biphenylyl o-biphenylyl o-biphenylyl m-biphenylyl H H m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl H H p-biphenylyl p-biphenylyl p-biphenylyl I 裝 訂 線 (請先閲讀背面之注意事項再填寫本頁) 本纸張尺度適用中國國家標率（CNS ) A4说格（210X297公釐） 177- 581751 A7 B7 五、發明説明（175)
Ri
2-naphthyl (2-萘基） Χ··94 Χ.-95 Χ··96 Χ、97 Χ*-98 Χ··99 Χ·-100 Χ-101 Χ.-102 Χ.-103 Χ·-104 Χ··105 Χ··106 Χ·-107 Χ··108 Χ'«109 Χ·-110 — χ·-ι” obipherrylyJ (°·聯苯基） κ Χ'-112 7 Χ'-113 〇-〇 Χ，·114 nrvbiphenylyl Χ·-116 m-biphenylyl m-biphenylyl m*btphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-blphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-bjphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-blphenylyl m-biphenylyl p-b丨phenylyl (p·聯苯基〕
ftJR丨 L XM17 XM18 X，-119 X.-120 X.-121 X.-122 X.-123 Χ·-124 X'.125 X-126 Χ:·127 X:-128 X.-129 Χ·-130 Χ·-131 Χ·-132 Χ·-133 Χ'-134 Χ··135 Χ··136 Χ.-137 Χ··138 Χ.-139 p-biphenylyl p-blphenylyl p-biphenylyl p-biphenylyl p-biphenylyi p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenyly) p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-blphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl r2 r3 r5 «7 Re Η Η Η Η Η .H Ph Η Η Ph Η H Η Ph Ph Η Η H Η Ph Η Η Η H Η Η Ph Η Η H Η Η Η Η Ph H Η Η Η Η Η Ph Η Η Η Η Ph Ph Η Η Η Η 1-naphthyl H Η Η Η Η Η 1-naphthyl Η Η Η Η 1-naphthyl 1-naphthyl Η Η Η Η 2-naphthyl H Η Η Η Η Η 2-naphthyl Η Η Η Η 2-naphthy! 2-naphlhyl Η Η Η Η o-biphenylyl H Η Η Η· Η Η o-biphenylyl Η Η Η Η o-biphenylyl o-biphenylyl Η Η Η Η m-biphenylyl H Η Η Η Η H m-biphenylyl Η Η Η Η m-biphenylyl m-biphenylyl Η Η Η Η p-biphenylyl H Η Η Η Η H p-biphenylyl Η Η Η Η p-biphenylyl p-biphenylyl Η Η Η Η .H H Ph Η Η Ph H H Η Ph Ph Η H H Η Ph Η Η H H Η Η Ph Η H H Η Η Η Η Ph H Η Η Η Η H Ph Η Η Η Η Ph Ph Η Η Η Η 1-naphthyl H Η Η Η Η H 1-naphthyl Η Η Η Η 1-naphthyl 1-naphthyl Η Η Η Η 2-naphthyl H Η Η Η Η H 2-naphthyl Η Η Η Η 2-naphthyl 2-naphthyl Η Η Η Η o-biphenylyl H Η Η Η Η H o-biphenylyl Η Η Η Η o-biphenylyl o-biphenylyi Η Η Η Η m-biphenylyl H Η Η Η Η H m-biphenylyl Η Η Η Η m-biphenylyl m-biphenylyl Η Η Η Η p-biphenylyl H Η Η Η Η H p-biphenylyl Η Η Η Η p-biphenylyl p-biphenylyl (請先閱讀背面之注意事項再填寫本頁) -裝 訂
In ϋ n m 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公羞） 178 581751
A B7 五、發明説明（176) R2 R3
οό % »7s. 土 η
R1 1-naphthyl (丨·萃基） 2-naphlhy丨（2-菜基） ob o-biphenylyl (〇·鞞2基） <χ5 m-biphenylyl (m_琳本基） p-biphenylyl (p-W^S) o-tolyl (〇·甲苯基） CH3 m-tolyl (m·甲苯基） -〇ch3 p-tolyl (p·田苯基） Χ··140 o-tolyl Χ_·141 o-tolyl Χ_·142 o-tolyl Χ，-143 o-tolyl Χ，-144 o-tolyJ Χ-145 o-tolyl Χ.·146 o-tolyl Χ.-147 o-tolyl Χ·-148 o-tolyl Χ，·149 o-tolyl Χ，·150 o-tolyl Χ.-151 . o-tolyl Χ··152 o-tolyl Χ.-153 o-tolyl Χ··154 o-tolyl Χ.-155 o-tolyl Χ.-156 o-tolyl Χ··157 m-tolyl Χ·-158 m-tolyl Χ·-159 m-tolyl Χ·-160 m-tolyl Χ··161 m-tolyl Χ.-162 m-tolyl Χ.-163 m-tolyl Χ·-164 m-tolyl Χ.-165 m-tolyl Χ··166 m-tolyl Χ··167 m-tolyl Χ··168 m-tolyl Χ-169 m-tolyl Χ-170 m-tolyl Χ.-171 m-tolyl Χ·-172 m-tolyl Χ'-173 m-tolyl Χ··174 p-tolyl Χ·-175 p-tolyl Χ.-176 p-tolyl Χ-177 p-tolyl Χ*-178 p-tolyl Χ-179 p-tolyl Χ-180 p-tolyl Χ-181 p-tolyl Χ··182 p-lo)yl Χ·-183 p-tolyl Χ·-184 p-tolyl Χ，·185 p-tolyl Χ··186 p-tolyi Χ，·187 p-tolyl Χ··188 p-tolyl Χ··189 p-tolyl ΧΜ90 p-tolyl HphHHH HHHHHHHHHHHHHphHHHHHHHHHHHHHHH HphHHHHHHHHH.HHHH Η H R4 H h^hh hhhhhhhhhhhhhh phhhhhhhhhhhhhh hh^hhhhhhhhhhhhhh H H^HH hhhhhhhhhhhhhh ^hhhhhhhhhhhhhh hh phhhhhhhhhhhhhh R5 R7 Re H H H Ph H H H H H H Ph H H H Ph H 1-naphthyl H H H 1-naphthyl H 2-naphthyl H H H 2-naphthyl H o-biphenylyl H H H o-biphenylyl H m-bjphenylyl H H H m-biphenylyl H p-biphenylyl H H • H p-biphenylyl H o-tolyl H H H o-tolyl H H H Ph H H H H H H Ph H H H Ph H 1-naphthyl H H H 1-naphthyl H 2-naphthyl H H H 2-naphthyl H o-biphenylyl H H .H o-biphenylyl H m-biphenylyl H H H m-biphenytyl H p-biphenylyl H H H p-biphenylyl H m-tolyl H H H m-tolyl H H H Ph H H H H H H Ph H H H Ph H 1-naphthyl H H •H 1-naphthyl H 2-na()hthyl H H H 2-naphthyl H o-biphenylyl H H H o-biphenylyl H m-biphenylyl H H H m-biphenylyl H p-biphenylyl H H H p-biphenylyl H p-tolyl H H H p-tolyl (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -179、 581751 A7 B7 五、發明説明（177 )
00 ob o-biphenylyl od % -〇g
TPA 1*naphthyl(i-菜基） 2-naphthyl (〇-軟苯基） m-biphenylyl (m-辟苯基） p-biphenylyl (pJK苯基） o-tolyl (°·甲苯基） ch3 m-tolyl 甲苯基） ~〇ch3 p-tolyl α,ο D丨PA Ri R2 r3 R4 Χ，·191 Ph H -CH3 -CH3 Xf-192 1-naphtyl H -CH3 -CH3 X.-193 2-naphthyl H -CH3 -CH3 Χ，·194 o-biphenylyl m-biphenylyl H •CH3 •CH3 Χ.-195 H -CH3 •CH3 Χ·-19β p-biphenylyl H •CH3 •CH3 Χ.-197 o-tolyl m-tolyl H -CH3 -CH3 Χ，-198 H -CH3 •CH3 Χ·-199 p-tolyl H -CH3 •CH3 Χ'-200 Ph H H H Χ'-201 1-naphtyl H H H Χ-202 2-naphthyl H H H Χ.-203 o-biphenylyl H H H Χ·-204 m-biphenylyl H H H Χ.-205 p-biphenylyl H H H Χ·-206 o-tolyl H H H Χ··207 m-tolyl H H H Χ·-208 p-tolyl H H H Χ.-209 Ph H H H Χ.-210 1-naphtyI H H H Χ·-211 Χ·-212 2-naphthyi o-biphenylyl H H H H H H Χ.-213 m-biphenylyl H H H Χ'-214 p-biphenylyl H H H Χ·-215 o-tolyl H H H Χ·-216 m-tolyl H H H Χ.-217 p-tolyl H H H Χ*-218 Ph H H H Χ·-219 1-naphtyl H H H Χ'-220 2-naphthyl H H H Χ，-221 o-blphenylyl H H H Χ.·222 m-biphenylyl H H H Χ.-223 p-biphenylyl H H H Χ··224 o-toiyl H H H Χ··225 m-tolyl H H H Χ·-226 p-tolyl H H H Χ*-227 Ph H H H Χ.-228 1-naphtyl H H H Χ·-229 2-naphthyl H H H Χ.-230 o-biphenylyl .H H H Χ··231 m-biphenylyl H H H Χ.-232 p-biphenylyl* H H H Χ.-233 Ph H H H Χ··234 Χ·-235 1- naphtyl 2- naphlhyl H H H H H H Χ··236 Χ··237 o-blphenylyl nvbiphenylyl H H H H H H Χ··238 p-biphenylyl H H H Χ.-239 Ph H H H Χ'-240 1-naphtyl H H H Χ.-241 2-naphthyl H H H Χ.-242 o-biphenylyl H H H Χ，·243 m-biphenylyl H H H Χ..244 p-biphenylyl H H H Χ··245 Ph H H H Χ*-246 1-naphtyl H H H Χ··247 2-naphthyl H H H Χ.·248 o-blphenylyl H H H Χ··249 m-biphenylyl H H H Χ··250 p-biphenylyl H .H • H. R5hhhhh hhhhhh h h h hhh hhhhh h h.hh hh h h h h hh h hhhhhhhhhhhh h h hhhhhhhhhh h r7
Re
H H H H H H H H H -CH3 •CH3 •CH3 -CH3 -CH3 -CH3 •CH3 -CH3 •CH3 H H H H H H H H H -CH3 -CH3 •CH3 •CH3 -CH3 •CH3 -CH3 -CH3 -CH3 H H H H H H DPA DPA DPA DPA DPA DPA H H H H H H TPA TPA TPA TPA TPA TPA
H H H H H H H H H H H H H H H H H H -CH3 •CH3 •CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 •CH3 -CH3 •CH3 -CH3 •CH3 •CH3 DPA DPA DPA DPA DPA DPA H H H H H H TPA TPA 丁 PA TPA TPA TPA H H H H H H (請先閲讀背面之注意事項再填寫本頁) 裝. 訂 線 本紙伕尺度通用中國國家標準（CN’S ) A4規格（210X29*7公釐） -180· 581751 A7 B7 五、發明説明（178)
Y-22 〇〇 γ-23 m-biphenylyl Υ-24 至象 r^^TrA1 寸 t θ 4113 穸>乍-£.口-3^ (m•轉）Υ-25 Υ-26 Υ-27 Υ·28 Υ-29 Υ-30 Υ-31 Υ·32 Υ·33 Υ-34 Υ-35 Υ-36 Υ-37 Υ-38 Υ·39 Υ-40 Υ-41 Υ-42 Υ^3 Υ-44 Υ-45 Υ-46 Υ47 p-biphenylyl (p^aes基）
Ri r2 r3 r5 Re r7 Rb Η H H H H H H Ph H H H Ph H H Ph Ph H H Ph H H Ph H H Ph Ph H H Ph Ph H Ph Ph H H Ph H Ph H Ph H H Ph H H · H Ph Ph H Ph H H H Ph H Ph Ph H H H Ph Ph Ph Ph H H H Ph 1-naphthyl H Ph H H H Ph H 1-naphthyl Fh H H H Ph 1-naphthyl 1-naphthyl Ph H H H Ph 2-naphthyl H Ph H H H Ph H 2-naphthyl Ph H H H Ph 2-naphthyl 2-naphthyl Ph H H H Ph o-biphenylyl H Ph H H H Ph H o-biphenylyl Ph H H H Ph o-biphenylyl o-biphenylyl Ph H H H Ph m-biphenylyl H Ph H H H Ph H m-biphenylyl Ph H H H Ph m-biphenylyl m-biphenylyl Ph H H H Ph p-biphenylyl H Ph H H H Ph H p-biphenylyl Ph H H H Ph p-biphenylyl p-biphenylyl 1-naphthyl H H H 1-naphthyl H H 1-naphthyl Ph H H 1-naphthyl H H 1-naphthyl H H Ph 1-naphthyl H H 1-naphthyl Ph H Ph 1-naphthyl H H · 1-naphthyl H Ph H 1-naphthyl H H 1-naphthyl H H H 1-naphthyl Ph . H 1-naphthyl H H • H 1-naphthyl H Ph 1-naphthyl H H H 1-naphthyl Ph Ph 1-naphthyl H H H 1-naphthyl 1-naphthyl H 1-naphthyl H H H 1-naphthyl H 1-naphlhyl 1-naphthyl H H H 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl H H H 1-naphthyl 2-naphthyl H 1-naphthyl H H H 1-naphthyl H 2-naphthyl 1-naphthyl H H H 1-naphthyl 2-naphthyl 2-naphthyl 1-naphthyl· H H H 1-naphthyl o-biphenylyl H 1-naphthyl H H H 1-naphthyl H o-biphenylyl 1-naphthyl H H H 1-naphthyl o-biphenylyl o-biphenylyl 1-naphthyl H H H 1-naphthyl m-biphenylyl H 1-naphthyl H H H 1-naphthyl H m-biphenylyl 1-naphthyl H H H 1-naphlhyl m-biphenylyl m-biphenylyl 1-naphthyl H H H 1-naphthyl p-biphenylyl H 1-naphthyl H H H 1-naphthyl H p-biphenylyl 1-naphthyl H H H 1-naphthyl p-biphenylyl p-biphenylyl ^1Τ^ (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS > Α4規格（210X297公釐） -181 - 581751 A7 B7 五、發明説明（179)
R1 〇6 1-naphthyl (1-萘基） 2-naphthyl (2·菜基）ob o*blphenylyl 苯基} Υ·48 Υ·49 Υ-50 Υ·51 Υ-52 Υ-53 Υ-54 Υ-55 Υ-56 Υ-57 Υ-58 Υ-59 Υ-60 Υ-61 Υ-62 Υ·63 Υ-64 Υ-65 2-naphthyl 2>naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphlhyl 2-naphthyl 2-naphthyl 2-naphthyl od p-bipheny丨yl 苯基) Y-71 Y-72 Y-73 Y-74 Y-75 Y-76 Y-77 Y-78 Y-79 Y-BO Y-81 Υ·82 Y-83 V-84 V-85 Y-86 V-87 Y*88 V-89 V-90 Υ·91 V-92 V-93 o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-blphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl obiphenylyl o-biphenyly! o-biphenylyl o-biphenylyl Y-66 2-naphthyl Y-67 2-naphthyl Y-68 2-naphthy! m«biphenylyl (m.W 苯基〕丫《69 2-naphthy( Y-70 2-naphthyl r2 R3 Rs Re .r7 Rb Η Η Η 2-naphthyl H H Ph Η Η 2-naphthyl H H Η Η Ph 2-naphUiyI H H Ph Η Ph 2-naphthyl H H Η Ph Η 2-naphthyl H H Η Η Η 2-naphthyl Ph H Η Η Η 2-naphthyl H Ph Η Η Η 2-naphlhyl Ph Ph Η Η Η 2-naphthyl 1-naphthyl H Η Η Η 2-naphthyl H 1-naphthyl Η Η Η 2-naphthyl 1-naphthyl 1-naphthyl Η Η Η 2-naphthyl 2-naphthyl H Η Η Η 2-naphthyl H 2-naphthyl Η. Η Η 2-naphthyl 2-naphthyl 2-naphthyl Η Η Η 2-naphlhyl o-biphenylyl H Η Η Η 2-naphthyl H o-biphenylyl Η Η Η 2-naphthyl o-biphenylyl o-biphenylyl Η Η Η 2-naphthyl m-bipherrylyl H Η Η Η 2-naphthyl H m-biphenylyl Η Η Η 2-naphthyl m-biphenylyl m-biphenylyl Η Η •Η 2-naphthyl p-biphenylyl H Η Η Η 2-naphthyl H p-biphenylyl Η Η Η 2-naphlhyl p-biphenylyl p-biphenylyl Η Η Η o-biphenylyl H H Ph Η Η o-biphenylyl H H Η Η Ph o-biphenylyl H H Ph Η Ph o-biphenylyl H H Η Ph Η o-biphenylyl H H Η Η Η o-biphenylyl Ph H Η Η Η o-biphenylyl H Ph Η Η Η o-biphenylyl Ph Ph Η •Η Η o-biphenylyl 1-naphthyl H Η Η Η o-biphenylyl H 1-naphthyl Η Η Η o-biphenyiyt 1-naphthyl 1-naphthyl Η Η Η o-biphenylyl 2-naphthyl H Η Η Η o-biphenytyl H 2-naphthyl Η Η Η o-biphenylyl 2-naphthyl 2-naphthyl Η Η Η o-biphenylyl o-biphenylyl H Η Η Η o-bipheny}yi H o-biphenylyi Η Η Η o-biphenylyl o-biphenylyl o-biphenylyl Η Η • Η o-biphenylyl m-biphenylyl H Η Η Η o-biphenylyl H m-biphenylyl Η Η Η o-biphenylyl m-blphenylyl m-biphenylyl Η Η Η o-biphenylyl p-bipheny)yl H Η Η Η o-biphenylyl H p-biphenylyl Η Η Η o-biphenylyl p-biphenylyl p-blphenylyl (請先閲讀背面之注意事項再填寫本頁) 訂 本紙ifc尺度適用中S S家標準（CNS ) ( 210X297公# -182 581751 A7B7 五、發明説明（180
C0 1-naphthyl (〗·菜基） 2-naphthylob o-biphenyly丨（0*聯苯基） Qr0 m»biphenyly丨（m•脚苯基) p-bipheny|yl 苯基> £ 了\ 才 1 > η\ r_ s. 土 Ρ Υ·94 Υ-95 Υ·96 Υ·97 Υ·98 Υ·99 Υ-100 Υ-101 Υ·102 Υ-103 Υ-104 Υ-105 Υ-106 Υ-107 Υ-108 Υ-109 Υ-110 Υ-111 Υ-112 Υ-113 Υ-114 Υ-116 Υ-116 Υ-117 V-118 Υ-119 Υ-120 Υ-121 Υ-122 Υ-123 Υ-124 Υ-125 Υ-126 Υ-127 Υ-128 Υ-129 Υ-130 Υ-131 Υ-132 Υ-133 Υ-134 Υ-135 Υ-136 Υ-137 Υ-138 Υ·139
Ri m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl RSHHphphHHHH hhhhhhhhhhhhhhh hh^^hhhh hhhhhhhhhhhhhhh r3hhhh^hh h hhhh hhhhhhhhhhh hhhh^hhhhhhh hhhhhhhh hhh R2IHphHphHHHH hhhhhh hhhhhhhhh HphHphHH.HH hhhhhhhhhhhhhhh r6 r7 Re m-biphenylyl H H m-biphenylyl H H m-biphenylyl H H m-biphenylyl H H m-biphenylyl H H m-biphenylyl Ph H m-biphenylyl .H Fh m-biphenylyl Ph . Ph m-biphenylyl 1-naphthyl H m-biphenylyl H 1-naphthyl m-biphenylyl 1-naphthyl 1-naphthyl m-biphenylyl 2-naphthyl H m-biphenylyl H 2-naphthyl m-biphenylyl 2-naphlhyl 2-naphthyl m-biphenylyl o-biphenylyl H m-biphenylyl H o-biphenylyl m-biphenylyl o-biphenylyl o-biphenylyl m-biphenylyl m-biphenylyl H m-biphenylyl H m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl H m-biphenylyl H p-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p>biphenyly] H H p-biphenylyl H H p-biphenylyl H H p-biphenylyl H H p-biphenylyl H H p-biphenylyl Ph H p-biphenylyl H Ph p-biphenylyl Ph Ph p-biphenylyl 1-naphthyl H p-biphenylyl H 1-naphihyI p-biphenylyl 1-naphthyl 1-naphthyl p-biphenylyl 2-naphthyl H p-biphenylyl H 2-naphthyl p-biphenylyl 2-naphthyl 2-naphthyl p-biphenyjyl o-biphenylyl H . p-biphenylyl H o-biphenylyl p-biphenylyl o-biphenylyl o-biphenylyl p-biphenylyl m-biphenylyl H p-biphenylyl H m-biphenylyl p-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl H p-biphenylyl H p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl ---------^------IT------線 (請先閲讀背面之注意事項再填寫本頁) 本紙朱尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） 581751 A7 B7 五、發明説明（181 )
Ri R2 R3 R5
00 Ί-naphthy丨（丨·萊基） 2«naphthyl (2·萘基）ob o-biphenylyl (〇·聯苯基） Οτό m-biphenylyl (m·聯苯基) p-biphenylyl (p·聯苯基) o-tolyl 甲苯基） wch3 m-tolyl (m·田苯基） -〇ch3 p-tolyl (p*田苯基） Y-140 Y-141 Y-142 Y-143 Y-144 Y-145 Y-146 Y-147 Y-148 Y-149 Y-150 Y-161 Y-152 Y-153 Y-154 Y-155 Y-156 Y-157 Y-158 Y-159 Y-160 Y-161 Y-162 Y-163 Y-164 Y-165 Y-166 Y-167 Y-168 Y-169 Y-170 Y-171 Y-172 Y-173 Y-174 Y-175 Y-176 Y-177 Y-178 Y-179 Y-1B0 Y-181 Υ-1Θ2 Y-183 Y-184 Y-185 Y-186 Y-187 Y-18B Y-189 Y-190 o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-lolyl
Η H Ph H H Ph Η H Η H Η H Η H Η H H . H Η H Η H Η H Η H Η H Η H Η H Η H Η H Ph H H Ph Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H Η H
H Ph H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H r6 R7 Re o-tolyl H H o-tolyl H H o-tolyl H H o-tolyl Ph H o-tolyl H Ph o-tolyl 1-naphthyl H o-tolyl H 1-naphthyl o-tolyl 2-naphthyl H o-tolyl H 2-naphthyl o-tolyl o-biphenylyl H o-tolyl H o-biphenylyl o-tolyl m-biphenylyl H o-tolyl. H m-biphenylyl o-tolyl p-biphenylyl H o-tolyl H p-biphenylyl o-tolyl o-tolyl H o-tolyl H o-tolyl m-tolyl H H m-tolyl H H m-tolyl H H m-tolyl Ph H m-tolyl H Ph m-tolyl 1-naphthyl H m-tolyl H 1-naphthyl m-tolyl •2-naphthyl H m-tolyl H 2-naphthyl m-tolyl o-biphenylyl H m-tolyl H o-biphenytyl m-tolyl m-biphenylyl H m-tolyl H m-biphenylyl m-tolyl p-biphenylyl H m-tolyl H H H H p-biphenylyl m-tolyl H H H m-tolyl m-tolyl H m-tolyl H H H m-tolyl H m-tolyl p-tolyi H H H p-toiyl H H p-tolyl Ph H Ph p-tofyl H H p-tolyl H Ph H p-tolyl H H p-tolyl H H H p-tofyl Ph H p-tolyl H H H p-tolyl H Ph p-tolyl H H H p-tolyl 1-naphthyl H p-tolyl H H H p-tolyl H 1-naphlhyl p-tolyl H H H p-toiyl 2-naphthyl H p-tolyl H H H p-tolyl H 2-naphthyl p-tofyl H H H p-lofyl o-biphenylyl H p-tolyl H H H p-tolyl H o-biphenylyl p-tolyl H H H p-tolyl m-biphenylyl H p-tolyl H H H p-tolyl H m-biphenylyl p-tolyl H H H p-tolyl p-biphenylyl H p-tolyl H H H p-tolyl H p-biphenylyl p-tolyl H H H p-tolyl p-tolyl H p-tolyl H H H p-tolyl H p-tolyl 本紙伕尺度適用中國囷家橾準（CNS ) A4規格（210X297公釐） -184- (請先閲讀背面之注意事項再填寫本頁) 581751 A7 B7 五、發明説明（182 )
Ri -c L· y-191 Y-192 Y-193 Y-194 Y-195 Y-196 Y-197 Y-198 Y-199 Y-200 Y-201 Y-202 Y-203 Y-204 Y-205 Y-206 Y-207 Y-208 Y-209 Y-210 Y-211 Y-212 1- naphthyl (l-系基）γ·213 Y-214 CCX V-215 2- naphthyl (2·萘基） , Y-218 〇-〇 ⑽ o-biphenylyl Y-220 (〇聯苯基） /-W-< Y-222 Y-223 Y-224 Y-225 u. K ,, Y-226 p-biphenylyl yJ2l7 (p"眯苯基）Y-228 H3C y-229 -(3 Y*230 〇-tolyl (〇·田苯基> Y-231 CU. Y-232 Y-233 Y-234 m-tolyl (m•甲苯基）γ·235 厂、 Y-236 Y-237 p-tolyl γ-238 Y-239 Y-240 Υ-241 V-242 Υ-243 Υ-244 Υ-245 Υ-246 Υ-247 Υ-248 Υ-249 Υ-250
C0 m-biphenylyl (m·聯苯基) 〇V〇
DPA
丁 PA
Ph 1- naphtyl 2- naphthyl o-biphenylyl m-blphenylyl p-biphenyiyl 0- tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl 0- tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-bipnenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-blphenylyl Ph 1- naphtyl 2- naphthyl o-biphenyiy) m-biphenylyl p-biphenylyl
R2hhh HH hhhhhhh η h hhh hhhhh hhhhhh η h HH HH Η HHHHHHHHHHHHH HHHHHHHHHHHH R7
Re_
•CH3 -CH3 -CH3 -CH3 •CH3 -CH3 -CH3 -CH3 -CH3 H H H H H
Η Η Η HHHHH HHHHHHH Η HHHHH HHHHHHHHHHHHHHHHHHHHHHHHH H HH HH hhhhhhh h h hhh hhhhh hhhhhhh h hhhhh hhhhhhhh hhhh h h hhhhhhhhhhh
Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenyly) p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p>bipheny!yl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyi o-tolyl m-tolyl p-tolyl Ph 1*naphlyl 2-naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-bipherylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph ' 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl
Η Η H HH Η Η Η H
H3H3H3 -CH-CH.CH
Η Η Η HH Η Η Η Η Η Η H •CH3 Η •CH3 Η -CH3 Η -CH3 Η -CH3 Η -CH3 Η Η -CH3 Η -CH3 Η -CH3 Η •CH3 Η -CH3 Η •CH3 Η -CH3 Η -CH3 Η •CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 •CH3 -CH3 -CH3 -CH3 -CH3 -CH3 •CH3 •CH3 Η DPA Η DPA Η DPA DPA Η DPA Η DPA DPA Η DFA Η DPA Η DPA Η DPA DPA Η Η ΤΡΑ Η ΤΡΑ Η ΤΡΑ Η ΤΡΑ Η ΤΡΑ Η ΤΡΑ ΤΡΑ Η ΤΡΑ Η ΤΡΑ Η ΤΡΑ Η ΤΡΑ Η ΤΡΑ Η (請先閲讀背面之注意事項再填寫本頁) -裝. 訂 線 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -185· 581751
A B7 五 、發明説明（^ ) Y-251 Υ-252 Υ-253 Υ-254 Υ-255 Υ-256 Υ·257 Υ-258 Υ·259 Υ·260 Υ-261 Υ-262 Υ-263 Υ-264 Υ-265 Υ-266 Υ-267 ρΛ γ·268 Υ-269 ’ — Υ-270 Υ-271 Υ-272 Υ-273 Υ-274 γ"275 _ Υ-276 o-biphenyly丨（〇·聯苯基)γ·277 Υ-278 r\-ri γ-279 Υ-280. >Υ-281 Υ-282 Υ-283 p-biphenyly丨(ρ*聯苯基）γ-2Β4 Υ-285 Υ-286
RO
Ri Ph Ph Ph Ph Ph Ph Ph Ph 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1-naphthyl 1- naphthyl 2- naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl o-biphenylyl o-biphenylyl o-biphenylyl o-biphenylyl o-blphenylyl nvbiphenylyl m-biphenylyl m-biphenylyl m-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl O-tolyly O-tolyly m-tolyly R5 R6
H HHHH hhhhhhhhhhhhhhhhhhhhhhhh hh hhhh hh Η 1-naphthyl Η 2-naphthyl Η o-biphenylyl Η m-biphenylyl Η p-biphenylyl Η O-tolyly Η m-tolyl Η p-tolyl Η 2-naphlhyl Η o-biphenylyl Η m-biphenylyl Η p-biphenylyl Η O-tolyly Η m-tolyl Η p-tolyl Η o-biphenylyl Η m-biphenylyl Η p-biphenylyl Η O-tolyly Η m-tolyl Η p-tolyl Η .m-biphenylyl Η p-biphenylyl Η O-tolyly Η m-tolyl Η p-tolyl Η p-biphenylyl Η O-toiyly Η m-tolyl Η p-tolyl Η O-tolyly Η m-tolyl Η p-tolyl Η m-tolyl Η p-tolyl Η p-tolyl hhhhhhhhhhhhhhhhhhhhhhhhhhhhhh hhhh hh (請先聞讀背面之注意事項再填寫本頁)
*1T 經濟部皙慧^^^貞工消免合作社印货 1-naphthyl (1-蔡基） 2«naphthyl (2-萘基） nvbiphenylylOn·聯笨基)，
H3C 〇.t〇|y| (°·*苯基） •ch3 m-tolyl 如·Φ 苯基） ^〇ch3 p-tolyl (ρ-φ**) hhhhhhhh hhhh hhhh
H 本纸法尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -186- 581751 A7 B7 五、發明説明（
Q? CZR3 yp2 T R
R3
Rs R6 經濟部智慧时/itllra:工消費合作Ti印誕 2-1z-2z-3z-4z-5z-6z-7z-8z-9z-1(sz-12z-13z-14z-15z-16z-17z-1lζ-1ίζ-2(ζ.2ζ-2ζ-2ζ-2ζ-2 0 12 3 4 2-2^14-2 h h h h h h h p p p p p p p phph phphphphphphphph (請先閲讀背面之注意事項再填寫本頁)
多这这这这 phph
Μ Η Η H
PhH H HMeH H
H
HphphH HMeH H HphH H HMe
H
phH Η HMH H
MeHHHHphHHMe 訂 本纸乐尺度適用中國國家標準（CNS ) A4说格（210X297公釐） -187 - 581751 Α7 Β7 經濟部智慧財產局員工消費合作Ti印¾ (請先閲讀背面之注意事項再填寫本頁)
五、發明説明（189
R7 Z-43
Η Η Ph Ph Η Η Me Η Η Η Ph Ph Η Η Me Η Η Η Ph Ph Η Η Me Η Η Ph Η Η Η Me Η Η Η Ph Η Η Η Me Η Η Η Ph Η Η Η Me
Η 本紙法尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -188- 581751 A7 B7 五、發明説明（18弓
TypeZ Z-50 Z-51 Z-52 Z-53 Z-54 Z-55 Z-56 Z-57 Z-58 Z-59 CCT06
經濟部智慧財凌局員工消骨合作社印¾ Z-63 Z-64 Ζ·65 Z-66 Z-67 Z-68 Z-69 Z-70 Z-71 Z-72 Z-73 Z-74 Ζ·75
H H H H H H H H H H
Ph Ph Ph Ph Ph
H H H H H H H H H H H H H H H H H H H H H H H H H (請先閲讀背面之注意事項再填寫本頁)
、1T 本纸張尺度適用中國國家標準（CNS ) A4規格（210X 297公釐） -189- 581751 A7 B7 五、發明説明（18分
經濟部智慈財凌^肖工消費合作社印焚 (請先閲讀背面之注意事項再填寫本頁)
Ri Z-76 H3Ch〇- z·77 h3c〇 Z-78 H3C〇 z·79 h3o〇
H Ph H H H Me H H
z-81 H3C-0- z*82 H3C-0 2*83 H3C-〇- Z-84 h3c-〇 H Z-85 H3C-O Ph Z-86 h3c-<^ H Z-87 h3c^3 H Z-88 h3c<5 H Z-89 h3c<5 Me Z-90 h3c-<^ H Z-91 h3c-<^ H 2-92 H3C-t> H Z-93 H3C-t) Ph Z-94 HaC-t) H Z-96 H3C-b H Z-96 H3C^> H Z-97 n3c-b Me Z-98 H3C-t) H Z-99 HaC-t) H
H H Ph Ph H H Me H H H Ph Ph H H Me H H H Ph Ph H H Me H H H Ph H H H Me H H H Ph H H H Me H H H Ph H H H Me r6 H h3c-〇~ Ph H3C-O H H3C-O H H3C-O H H3C-O Μβ H3C-O H h3c-〇-h h3o〇- H H3C-<j Ph h3〇5 n H3C H H3C- h3c- h3c-
H H H H Ph H H Me H H H H Ph H
H H3C-O H H Me H n3c-b H Ph H3C-b H
H
H H3C- h3c- h3c- h3o H3C-H H3C^>
H H Ph H H 本纸永尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -190- 581751 A7 B7 五、發明説明（1㈣ R2
Ri
Η Ph Η Η Η Me H 108 109 111 112 113 114 115 116 117 經濟部智^財產苟肖工消費合作社印製 】21 122 123 op H op Pb op H op H op H<>p M< <>P H op H op H op Ph op H op h op h op M op ^ op h R.1 H H Ph Ph H H Me H H H Ph Ph H H Me 1¾ H H Ph H H H Me H H H Ph H H H Me R5
Rfi R?
Pli
Ph
Me
Ph
Me
HHHHphHHMeHHHHphHHMeH Η H HphHΗMe HphHHHMeHHHphHHHMeHHHphHHHMeH H (請先閲讀背面之注意事項再填寫本頁) 本纸法尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -191 - 581751 A7 B7 五、發明説明（18令
Ri R2
Ra
Rr,
Re R?
Typ«Z
w« «* Ri n, 125 126 127 128 129 130 131 132 133 134 135 136 137 138 139
Ph
Me H H Ph Ph H H Me H H H Ph Ph H H M« H H Ph H H H Me H H H Ph H H H Me H HjC-
(請先閲讀背面之注意事項再填寫本頁)
Me
Ph 142
Ph
Ph 經濟部智慧財凌笱員工^費合作社印紫 143 145 本纸伕尺度適用中國國家標窣（CNS ) A4規格（210X297公釐）
Ph
Me
Me
Me
Me -192· 581751 A7 B7 五、發明説明（190)
Ri Ra R3 Rs R? R8 1 H H H H H H H 2 Ph H H H. H H H χχ, JO-t； 3 Ph Ph H H Ph H H «4 J 4 PIi H Ph Ph H .H H 5 Ph H Ph H H H H rV, 6 Ph H H Ph H H H ^ F 7 Ph H H H H Ph H TypeAAA 8 Ph H H H H H Ph 9 Ph H H H H Ph Ph 10 Ph H H H H 1-naphthyl H C0 11 Ph H H H H H 1-naphthyJ 12 Ph . H H H H 1-naphthyl 1-naphthyl 1-naphthyl (1-蔡基） 13 Ph H H H H 2-naphthyl H 14 Ph H H H H H 2-naphthyl αχ 15 Ph H H H H 2-naphthyl 2-naphthyi 2-naphthyl (2-蔡基） 16 Ph H H H H o-biphenylyl H 17 Ph H H H H H o-biphenylyl 〇-〇 18 Ph H H H H o-biphenylyl o-biphenylyl o-biphenyjyl (〇·聯苯基） 19 Ph H H H H m-biphenylyl H 20 Ph H H H H H m-biphenylyl 21 Ph H H H H m-biphenylyl m-biphenylyl ΟΌ 22 Ph H H H H p-biphenylyl H m-bipheny!yl (m-聯苯基) 23 Ph H H H H H p-biphenylyl 24 Ph H H H H p-blphenylyl p-biphcny)yJ p~biphenylyl (P~ 聯苯基） 25 1-naphthyl H H H H H H 26 1-naphthyl Ph H H Ph H H 27 1-naphthyl H Ph Ph H H H 28 1-naphthyl H Ph H H H H 29 1-naphthyl H H Ph H H H 30 1-naphthyl H H H H Ph H 31 1-naphthyl H H H H H Ph 32 1-naphthyl H H H H Ph Ph 33 1-naphthyl H H H H 1-naphthyl H 34 1-naphthyl H H H H H 1-naphthyi 35 1-naphthyl H H H H 1-naphthyl 1-naphthyl 36 1-naphthy! H H H H 2-naphthyl H 37 1-naphthyi H H H H H 2-naphthyl 38 1-naphthyl H H H H 2-naphthyl 2-naphthyl 39 1-naphthyl H H H H o-biphenylyl H 40 1-naphthyi H .H H H H o-biphenylyl 41 1-naphthyJ H H H H o-biphenylyl o-biphenylyl 42 1-naphthyl H H H H m-biphenylyl H 43 1-naphthyi H H H H H i m-biphenylyl 44 1-naphthyl H H H H m-biphenylyl m-biphenylyl 45 1-naphthyl H H H H p-biphenylyl H 1-naphthyl H H H H H p-biphenylyl 47 1-naphthyl H H H H p-biphenylyl p-biphenylyJ (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） · 193 _ 581751 A7B7 五、發明説明（191 )
TypcAAA C0 1-naphthyl (1-萘基） 2-naphthyl (2-蔡基） o-b 仲 o~Wphenylyl (°* 聯本基） p»blphenylyl ({>聯苯基） Ri R2 R3 Rs R? R8 48 2-naphthyl H H H H H H 49 2-naphthyl Ph H H Ph H H 50 2-naphthyl H Ph Ph H H H 51 2-naphthyl H Ph H H H H 52 2-naphthyl H H Ph H H H 53 2-naphthyl H H H H Fh H 54 2-naphthyl H H H H H Ph 55 2-naphthyl H H H H Ph Ph 56 2-naphthyl H H H H 1-naphthyl H 57 2-naphthyl H H H H H 1-naphthyl 58 2-naphthyJ H H H H 1-naphthyl 】-naphthyl 59 2naphthyl H H H H 2-naphthyl H 60 2-naphthyl H H H H H 2-naphthyl 61 2-naphthyl H H H H 2-naphthyJ 2-naphthyJ 62 2-naphthyl H H H H o-biphenylyJ H 63 2-naphthyl H H H H H o-biphenylyl 64 2-naphthyl H H H H o-biphenylyl o-biphenylyl 65 2-naphthyl H H H H m-biphenylyl H 66 2-naphthyl H H H H H m-biphenyiyl 67 2-naphthyl H H H H m-biphenylyl m-biphenyiyl 68 2-naphthyl H H H H p-blphenylyl H 69 2-naphthyl H H H H H p-biphenylyl 70 2-naphthyl H H H H p-blphenylyl p-biphenylyl 71 o-blphenylyl H H H H H H 72 o-biphenylyl Ph H H Ph H H 73 a-blphenylyl H Ph Ph H H H 74 o-blphenylyl H Ph H H H H 75 o-biphenylyl H H Ph H H H 76 o-biphenyJyl H H H H Ph H 77 o-biphenylyi H H H H H Ph 78 o-biphcnylyl H H H H Ph Ph 79 o-biphenylyl H H H H 1-naphthyl H 80 o-biphcnyJyl H H H H H 1-naphthyl 81 o-biphenylyl H H H H 】-naphthyl 1-naphthyl 82 o-biphenylyl H H H H 2-naphthyi H 83 o-biphenylyl H H H H H 2-naphthyl 84 o-biphenylyl H H H H 2-naphthyl 2-naphthyl 85 o-blphenylyl H H H H o-biphenylyi H 86 o-biphenylyl H H H H H o-biphenylyl 87 o-biphenylyl H H H H o-biphenylyl o-biphenylyl 88 o-biphenylyl H H H H m-biphenyiyl H 89 o-biphenylyl H H H H H m-biphenylyl 90 o-biphenylyl H H H H m-biphenyJyl ; m-biphenylyl 91 o-biphenylyl H H H H p-biphenylyl H 92 o-biphenyJyJ H H H H H p-blphenylyl 93 o-biphenylyi H H H H p-biphenylyl p-biphenyjyl 111111 訂— — 1111 線(請先閲讀背面之注意事項再填寫本頁) 本紙沬尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -194- 581751 A7 B7 五、發明説明（192)
Ri R2
116 p-b丨pheny丨yl (P·聯苯基） m-bipheny!yl m-biphenylyl m-biphenylyl m-biphenyJyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl m-biphenylyl 117 118 119 120 121 122 123 124 125 126 127 128 129 130 131 132 133 134 135 136 137 138 139
H Ph H H H H H H H H H m-biphenylyl H m-biphenylyl H m-blphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl h m-biphenylyl H m-blphenylyl H m-blphenylyl H m-biphenylyl H m-biphenylyl H p-biphenylyl H p-biphenylyl Ph p-biphenylyl H p-blphcnylyi H p-biphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyl H p-blphenyW H p-blphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyl H p-blphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyi H p-biphenylyl H R3 R4 Rs R? Re Η Η Η Η H Η Η Ph Η H Ph Ph Η Η H Ph Η Η Η H Η Ph Η Η H Η Η Η Ph H Η Η Η Η Ph Η Η Η Ph Ph Η Η Η 1-naphthyl H Η Η Η Η 1-naphthyl Η Η Η 1-naphthyJ 1-naphthyl Η Η Η 2-naphthyl H Η Η Η Η 2-naphthyl Η Η Η 2-naDhthyl 2-naphthyl Η Η Η o-biphenylyl H Η Η Η Η o-biphenylyl Η Η Η o-biphenylyl o-biphenylyl Η Η Η m-biphenylyl H Η Η Η H m-biphenylyl Η Η Η m-biphenylyl m-biphenylyl Η Η Η p-biphenylyl H Η Η Η H p-biphenylyl Η Η Η p-biphenylyl p-biphenylyl Η Η Η H H Η Η Ph H H Ph Ph Η H H Ph Η Η H H Η Ph Η H H Η Η Η Ph H Η Η Η H Ph Η Η Η Ph Ph Η Η Η 1-naphthyl H Η Η Η H 1-naphthyi Η Η Η 卜 naphthyl 1-naphthyl Η Η Η 2-naphthyl H Η Η Η H 2-naphthyl Η Η Η 2-naphthyl 2-naphthyl Η Η Η o-biphenylyl H Η Η Η H o-biphenylyl Η Η Η o-biphenylyl o-biphenylyl Η Η Η m-biphenylyl H Η Η Η H m-biphenylyl Η Η Η m-biphenylyJ m-biphenylyl Η Η Η p-biphenylyl H Η Η Η H p-biphenylyl Η Η Η p-biphenylyl p-bipheny»yl (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4说格（210X297公釐） -195- 581751 A7 B7 五、發明説明（193) 140 141 142 143 144 145 146 147 148 149 150 151 152 153 154 155C0 Ι-naphthyl (丨·蔡基）158 159 CCX 160 2-naphthyl (2·案基）161 162〇-b o-blphenylyl (〇·賺苯基）165
TypeAAA
o-toly] i £ a m-toly丨（m·田苯基） p-to丨yl (p·田苯基） 174 175 176 177 178 179 180 181 182 183 184 185 1S6 187 188 189 190
Ri R2 R3 R/i Rs R? Re o-tolyl H H H H H H o-tolyl Ph H H Ph H H o-tolyl H Ph Ph H H H o-tolyi H H H H Ph H o-tolyl H H H H H Ph o-tolyi H H H H 1-naphthyl H o~toJyl H H H H H 1-naphthyl o-tolyi H H H H 2-naphthyl H o-tolyl H H H H H 2-naphthyl o-tolyl H H H H o-biphenylyi H o-tolyJ H H H H H o-blphenyJyl o-tolyJ H H H H m-biphenylyl H o-tolyl H H H H H m-biphenylyl o-tolyl H H H H p-biphenylyJ H o-tolyl H H H H H p-biphenylyl o-tolyl H H H H o-tolyl H o-toly] H H H H H o-tolyl m-tolyl H H H H H H m-toJyl Ph H H Ph H H m-tolyl H Ph Ph H H H m-tolyJ H H H H Ph H m-tolyl H H H H H Ph m-tolyl H H H H 1-naphthyJ H m-tolyl H H H H H 1-naphthyl m-tolyl H H H H 2-naphthyl H m-toiyl H H H H H 2-naphthyl m-tolyl H H H H o-biphenylyl H m-tolyl H H H H H o-biphenylyl m-tolyl H H H H m-biphenylyl H m-tolyl H H H H H m-blphenyJyl m-tolyl H H H H p-biphenylyl H m-tolyl H H H H H p-biphenyjyl m-tdyl H H H H m-tolyJ H m-tolyJ H H H H H m-tolyl p-toJyl H H H H H H p-tolyl Ph H H Ph H H p-tolyl H Ph Ph H H H p-tolyl H H H H Ph H p-tolyl H H H H H Ph p-tolyl H H H H 1-naphthyl H p-tolyl H H H H H 1-naphthyl p-tolyl H H H H 2-naphthyi H P-tolyl H H H H H 2-naphthyi p-tolyl H H H H o-blphenyly] H p-tolyl H H H H H o-biphenylyl p-tolyl H H H H m-biphenylyl H p-tolyl H H H H Η π i-biphenylyl p-tolyl H H H H p-biphenylyl H p-tolyl H H H H H p-biphenylyl p-tolyl H H H H p-tolyl H p-toiyl H H H H H p-tolyl (請先閱讀背面之注意事項再填寫本頁) 訂 線 本紙永尺度適用中國國家標準（CNS〉A4規格（210X297公釐） -196- 581751
A B7 五、發明説明（194)Ri R2 ¾ ¾ r5 R? ¾
TypeAAA οό m-biphenylyl 223 (m-脚苯基）224 225
l-naphthyl (丨·系基） ob o-biphenylyl (〇·脚苯基） 191 Ph 192 1-naphtyl 193 2~naphthyl 194 o-biphenyJy) 195 m-biphenylyl 196 p-blphenylyl 197 o-tolyi 198 m-tolyJ 199 p-tolyl 200 Ph 201 1-naphtyJ 202 2-naphthyl 203 o-blphenylyl 204 m-biphenylyl 205 p-blphenylyl 206 o-toiyl 207 m-tolyl 208 p-tolyl 209 Ph 210 1-naphtyl 211 2-naphthyl 212 o-blphenylyl 213 m-biphenylyl 214 p-biphenylyl 215 o-tolyl 216 m-tolyl 217 p-tolyl 218 Ph 219 1-naphtyl 220 2-naphthyl 221 o-biphenylyl 222 m-biphenylyl HHHHH HHHHHHH Η Η HHHHHHHH HHHHHH Η HHH p-biphenylyl o-tolyl m-tolyl
H H H t aNo
DPA ό
TPA p-biphenylyl CP·聃苯基) o-tolyl (°·甲苯基） m-tolyl (m·甲苯基） p-tolyl (p·田苯 S) 226 P-tolyl 227 Ph 228 1-naphtyl 229 2-naphthyl 230 o-biphenylyl 231 m-blphenyly] 232 p-biphenylyl 233 234 Ph 1-naphtyl 235 2-naphthyl 236 o-biphenylyl 237 m-biphenyiyl 238 p-biphenylyl 239 Ph 240 1-naphtyl 241 2-naphthyl 242 o-biphenylyl 243 m-biphenylyl 244 p-biphenylyl 245 Ph 246 1-naphtyl 247 2-naphthyi 248 o-biphenylyl 249 m-biphenylyl 250 p-biphenylyj HHHHHHHHHHHHH hhhhhhhhhhhh
Η3Η3Η3Η3Η34343-ί3·ί3 HHHHH HHHHHHHH HHHHH HHHHHH HHHHHH HHHHHHHHHHHHH hhhhhhhh HHHHHHH H HHHHH HHHHHHHHHHHHHHHHHHHHHHHHH ^s^^shhhhhhhhhhhhh h HHHHH HHHHHHHHHHH-
HHHHH HHHHHH Η Η H H H H H H H H H H -CH3 -CH3 -CH3 -CH3 -CH3
ψ-chi-CH-CHHHrcH Η HHH H:H:H:H:H:H:H,:H: -CV V v-c hhhhh£dp/dp/dp/dp/
H HHHHH TP>TpiiTP/TP/TP/TP/ ηηηηηηηηηηηηηηηηηηη3η3η3η3η3η3η3η3η3η3η3η3η3η3η3^3η3·13λαλααα^ ^ i i i vvv-cvvv-chvv-ch-ch-ch-ch-ch-ch-ch-chdpdpdpdpdpdpahhhhhhtpatpatpatpatpatpahhhhhh (請先閲讀背面之注意事項再填寫本頁 本纸乐尺度適用中國國家標準（CNS ) A4洗格（210X297公釐） -197- 581751 A7 B7 五、發明説明（195)
Ri Ri Ra R4 Rs R? Re R, R, 1 Η H H H H H H 2 Fh H H H H H H 3 Ph Ph H H Ph H H ^ y 4 Ph H Ph Ph H H H 5 Ph H Ph H H H H «•-CrV 6 Ph H H Ph H H H R， B. 7 Ph H H H H Ph H TypeBBB 8 Ph H H H H H Ph 9 Ph H H H H Ph Fh 10 Ph H H H H 1-naphthyl H C0 11 Ph H H H H H 1-naphthyl 12 Ph H H H H 1-naphthyl 1-naphthyl 1-naphthyl (1-蔡基） 13 Ph H H H H 2-naphthyl H 14 Ph H H H H H 2-naphthyl ccr 15 Ph H H H H 2-naphthyJ 2-naphthyl 2-naphthyl (2-萘基） 16 Ph H H H H o-biphenylyl H 17 Ph H H H H H o-biphenylyl ry^) 18 Ph H H H H o-biphenylyl o-blphenylyl o-biphenylyl (〇«聯苯基） 19 Ph H H H H m-biphenylyJ H 20 Ph H H H H H m-blphenylyl 21 Ph H H H H m-biphenylyl m-biphenylyl oo 22 Ph H H H H p-biphenylyl H m-biphenylyl (m-聯苯基) 23 Ph H H H H H p-biphenylyl 24 Ph H H H H p-bipheny]y] p-biphenylyl p-biphenylyl (p·聯苯基） 25 1-naphthyl H H H H H H 26 1-naphthyl Ph H H Ph H H 27 1-naphthjd H Ph Ph H H H 28 1-naphthyl H Ph H H H H 29 1-naphthyl H H Ph H H H 30 1-naphthyl H H H H Ph H 31 1-naphthyl H H H H H Ph 32 1-naphthyl H H H H Ph Ph 33 1-naphthyl H H H H 1-naphthyl H 34 1-naphthyl H H H H H 1-naphthyi 35 1-naphthyl H H H H 1-naphthyl 1-naphthyl 36 1-naphthyl H H H H 2-naphthyl H 37 1-naphthyl H H H H H 2-naphthyi 38 1-naphthyl H H H H 2-naphthyl 2-naphthyi 39 1-naphthyl H H H H o-biphenylyl H 40 1-naphthyl H H H H H o-biphenylyi 41 1-naphthyl H H H H o-blphenylyl o-blphenylyl 42 1-naphthyl H H H H m-biphenylyi H 43 1-naphthyl H H H H H m-biphenylyl 44 1-naphthyl H H H H m-biphenyJyl m-biphenyW 45 1-naphthyl H H H H p-blphenyly] H 46 卜 naphthyl H H H H H p-biphenylyi 47 1-naphthyl H H H H p-blphenylyl p-blphenylyl 裝 訂 線 (請先閲讀背面之注意事項再填寫本頁) 本紙法尺度適用中國國家標準（CNS ) A4規格（210X 297公釐） -198- 581751 A7 B7 五、發明説明（196)
Ri R2 R3 R4 Rs R? Re 48 2-naphthyl H H H H H H 0 i 49 2-naphthyl Ph H H Ph H H rV 50 2-naphthyl H Ph Ph H H H 51 2-naphthyl H Ph H H H H w R, 52 2-naphthyl H H Ph H H H 53 2-naphthyl H H H H Ph H TypeDDD 54 2-naphthyl H . H H H H Ph 55 2-naphthyl H H H H Ph Ph 56 2-naphthyl H H H H l-naphthyl H c6 57 2-naphthyl H H H H H 1-naphthyJ 58 2-naphthyl H H H H l-naphthyl l-naphthyl l-naphthyl (1-蔡基） 59 2naphthyl H H H H 2-naphthyl H 60 2-naphthyl H H H H H 2-naphthyl 〇y 61 2-naphthyl H H H H 2-naphthyl 2-naphthyi 2-naphthyi (2-蔡基） 62 2-naphthyl H H H H o-biphenylyl H 63 2-naphthyl H H H H H o-biphenylyl 64 2-naphthyl H H H H o-blphenyiyl o-blphenylyl o-blphenylyl (〇·聯苯基） 65 2-naphthyl H H H H m-biphenylyl H 66 2-naphthyl H H H H H m-biphenylyl 67 2-naphthyl H H H H m-biphenylyl m-biphenylyl <y〇 68 2-naphthyl H H H H p-biphenylyl H m-biphenylyl (m-聯苯基) 69 2-naphthyl H H H H H p-blphenvlyl γ\^γ\ 70 2-naphthyl H H H H p-biphenylyl p-biphenylyl p-biphenylyl (P·聯苯基） 71 o-biphenylyl H H H H H H 72 o-biphenylyl Ph H H Ph H H 73 o-blphenylyl H Ph Ph H H H 74 o-biphenylyl H Ph H H H H 75 o-biphenylyl H H Ph H H H 76 o-biphenylyl H H H H Ph H 77 o-biphenylyi H H H H H Ph 78 o-biphenylyl H H H H Ph Ph 79 o-biphenylyl H H H H l-naphthyl H 80 o-biphenylyi H H H H H l-naphthyl 81 o-biphenylyl H H H H l-naphthyl l-naphthyl 82 o-biphenyiyl H H H H 2-naphthyi H S3 o-biphenylyl H H H H H 2-naphthyl 84 o-biphenylyl H H H H 2-naphthyl 2-naphthyl 85 o-blphenylyl H H H H o-biphenylyl H 86 o-biphenylyl H H H H H o-biphenylyl 87 o-biphenylyl H H H H o-biphenylyl o-biphenylyl 88 o-blphenylyl H H H H m-biphenyly] H 89 o-blphenylyl H H H H H m-biphenylyl 90 o-biphenylyl H H H H m-biphenylyl m-biphenylyl 91 o-biphenylyl H H H H p-blphenyly] H 92 o-biphenylyi H H H H H p-biphenylyl 93 o-biphenylyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁
訂 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） •199· 581751 A7B7 五、發明説明（197)
Ri
TypeBBD 94 95 96 97 98 99 100 101 102οό :3 1- naphthyl (1·荼基）105οσ ；〇°： 2- na如hyi (2·莱基）ι〇8 ν 109 〇〇 110 o-biphenylyl 111 (〇·聯苯基）112od ：；：m-biphenylyl (m·聯苯基） 115 116 經濟部智慧財4局8工消黃合作社印繁 p-b丨pheny丨yl (P·聯苯基） 117 118 119 120 121 122 123 124 125 126 127 128 129 130 131 132 133 134 135 136 137 138 139 p-biphenylyl p-blphenylyl p-biph€nyiyl p-biphenylyl p-biphenylyl p-biphenytyl R2 R3 Ri Κΰ R? Re Η Η Η Η Η H Ph Η Η Ph Η H Η Ph Ph Η Η H Η Ph Η Η Η H Η Η Ph Η Η H Η Η Η Η Ph H Η Η Η Η Η Ph Η Η Η Η Ph Ph Η Η Η Η 1-naphthyl H Η Η Η Η Η 1-naphthyl Η Η Η Η 1-naphthy] 1-naphthy] Η Η Η Η 2-naphthyl H Η Η Η Η Η 2-naphthyl Η Η Η Η 2-naphthyl 2-naphthyl Η Η Η Η o-biphenylyl H Η Η Η Η Η o-biphenylyl Η Η Η Η o-biphenylyl o-biphenyiyl Η Η Η Η m-biphenylyl H Η Η Η Η H m-blphenyly) Η Η Η Η m-biphenylyl m-biphenytyl Η Η Η Η p~biphenylyl H Η Η Η Η H p-biphenylyl Η Η Η Η p-biphenylyl p-biphenyJyl Η Η Η Η H H Ph Η Η Ph H H Η Ph Ph Η H H Η Ph Η Η H H Η Η Ph Η H H Η Η Η Η Ph H Η Η Η Η H Ph Η Η Η Η Ph Ph Η Η Η Η 1-naphthyl H Η Η Η Η H 1-naphthyl Η Η Η Η 1-naphthyl 1-naphthyl Η Η Η Η 2-naphthyl H Η Η Η Η H 2-naphthyl Η Η Η Η 2-naphthyl 2-naphthyl Η Η Η Η o-biphenylyl H Η Η Η Η H o-biphcnylyi Η Η Η Η o-biphenylyl o-biphenyJyl Η Η Η Η m-blphenyjyl H Η Η Η Η H m-bipheny)yl Η Η Η Η m-biphenylyl m-biphenylyl Η Η Η Η p-biphenylyl H Η Η Η Η H p-biphenylyl Η Η Η Η p-biphenylyl p-biphenylvl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -200- 581751 A7 B7 五、發明説明（198)
TypeBBB 00 ob o-biphenylyl (〇-聯苯基）Cnd m-biphenylyi (m·聯苯基）
L P o-toly丨（〇*甲苯基） ni_tolyl (m-田苯基） ~〇"CHs p-tolyl (P* 甲苯 Ϊ) Ri R2 1¾ R/i Rs R? Re 140 o-tolyl H H H H H H 141 o-tolyl Ph H H Ph H H \42 o-tolyl H Ph Ph H H H 143 o-tolyl H H H H Ph H 144 o-tolyl H H H H H Ph 145 o-tolyl H H H H 1-naphthyl H 146 o-tolyl H H H H H 1-naphthyl 147 o-tolyl H H H H 2-naphthyl H 148 o-tolyl H H H H H 2-naphthyl 149 o-tolyl H H H H o-biphenylyl H 150 o-tolyl H H H H H o-biphenylyl 151 o-tolyl H H H H m-biphenylyl H 152 o-tolyl H H H H H m-blphenylyl 153 o-tolyl H H H H p-blphenylyl H 154 o-tolyl H H H H H p-biphenylyl 155 o-tolyl H H H H o-tolyl H 156 o-tolyl H H H H H o-tolyl 157 m-tolyl H H H H H H 158 m-tolyl Ph H H Ph H H 159 m-tolyl H Ph Ph H H H 160 m-toJyl H H H H Ph H 161 m-tolyl H H H H H Ph 162 m-tolyl H H H H 1-naphthyl H 163 m-toJyl H H H H H 1-naphthyl 164 m-tolyl H H H H 2-naphthyl H 165 m-tolyl H H H H H 2-naphthyl 166 m-tolyl H H H H o-biphenylyl H 167 m-tolyl H H H H H o-biphenylyl 166 m-tolyl H H H H m-blphenylyl H 169 m-tolyl H H H H H m-biphenylyl 170 m-tolyl H H H H p-biphenylyl H 171 m-tolyl H H H H H p-biphenylyl 172 m-tolyl H H H H m-tolyl H 173 m-tolyl H H H H H m-tolyl 174 p-tolyl H H H H H H 175 p-tolyl Ph H H Ph H H 176 p-tolyl H Ph Ph H H H 177 p-tolyl H H H H Ph H 178 p-tolyl H H H H H Ph 179 p-tolyl H H H H 1-naphthyl H 180 p-tolyl H H H H H 1-naphthyl 181 p-tolyl H H H H 2-naphthyl H 182 p-tolyl H H H H H 2-naphthyl 183 p-tolyj H H H H o-biphenylyl H 184 p-toly) H H H H H o-biphenylyl 185 p-tolyl H H H . H m-biphenylyl H 186 p-tolyl H H H H H m-biphenylyl 187 p-tolyl H H H H p-biphenylyl H 188 p-tolyl H H H H H p-biphenylyl 189 p-tolyl H H H H p-tolyi H 190 p-tolyl H H H H H p-tolyl (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -201 - 581751 A7 B7 五、發明説明（199)
Rt
TypeBBB
222 o-biphenylyl 220 (〇>聯苯基）221 m-biphenylyl 223 (m-聯苯基）224 225
Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenyly] p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-blphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-blphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-blphenylyl o-tolyl m-tolyl p-biphenylyl (P·賺苯基） 226 227 228 p-tolyl Ph 1-naphtyl 229 2-naphthyl 230 o-biphenylyl o-tolyl (〇*甲苯基） 231 m-biphenylyl yCHs 232 p-biphenylyl -ηΛ 233 Ph m-tolyl im·甲苯基） 234 1-naphtyl 235 2-naphthyl 236 o-biphenylyl 237 m-biphenylyl p-tolyl少甲苯基） 238 p-biphenylyl αΝο 1 239 Ph 240 241 1- naphtyl 2- naphthyl DPA 242 o-biphenylyl 243 m-biphenylyl 244 p-biphenylyl 245 246 Ph 1-naphtyl 247 2-naphthyl TPA 248 o-biphenylyl 249 m-biphenylyl 250 p-biphenylyl R2ΗΗΗΗΗ ηηηηηηη η η ηηηηηηηη ηηηηηη η η ηη ηη η ηηηηηηηηηηηηη ηηηηηηηηηηηη R3 R/i Rg R7 R8 CHCHCHCHCHCHCHCHHHHH Η ΗΗΗΗΗΗΗΗ ηηηηηηη Η ΗΗΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗ -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 Η Η Η Η Η ΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗΗ Η ΗΗΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗ ηηηηηηηηηηηηηη ηηηηηηηη ηηηηηηη η ηηηηη ηηηηηηηηηηηηηηηηηηηηηηηηη 13133 3 ΗΗΗΗΗΗΗΗΗ^^^^ ηηηηη ηηηηηηη η -CH3 Η 3 3 3 3 ΗΗ'Η-Η-ΗΗΗΗ -Ο-Ο-Ο-ΟΡΛΡΗ ΗΗΗ蓮
H -CH3 H -CH3 H -CH3 H -CH3 H -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 - CH3 -CH3 -CH3 -CH3 -CH3 H DPA H DPA H DPA H DPA H DPA
hdpadpadpadpadpadpah H s Η HTPATPATPATPATPATPA dpahhhhhhtpatpatpatpatpatpahhhhhh (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -202 581751 A7 B7 五、發明説明（200) iL L! t* »1 fa :r- »7 u' - - K4 tr t p Jtf R) R2 1¾ R4 Rs R? 1¾ 1 H H H H H H H 2 Ph H H H H H H 3 Ph Ph H H Ph H W 4 Ph H Ph Ph H H H h-oAV 5 Ph H Ph H H H H r,^x^xr, 6 Ph H H Ph H H H ^ Ri k 7 Ph H H H H Ph H TypeCCC 8 Ph H H H H H Ph 9 Ph H H H H Ph Ph 10 Ph H H H H l-naphthyl H c6 11 Ph H H H H H 1-naphthyJ 12 Ph H H H H l-naphthyl l-naphthyl l-naphthyl (1-蔡基） 13 Ph H H H H 2-naphthyl H 14 Ph H H H H H 2-naphthy] ca 15 Ph H H H H 2-naphthyl 2-naphthyJ 2_naphthyl (2-萘基） 16 Ph H H H H o-biphenylyl H 17 Ph H H H H H o-biphenylyl r\^h> 16 Ph H H H H o-biphenylyl o-biphenylyl \e/\—/ o-biphenylyl (〇>聯苯基） 19 Ph H H H H m-blphenyjyi H 20 Ph H H H H H m-biphenylyl 21 Ph H H H H m-blphenylyl m-biphenylyl CMD 22 Ph H H H H p-blphenylyl H m-biphenylyl (m-聯苯基） 23 Ph H H H H H p-biphenylyl /~V-TV 24 Ph H H H H p-biphenylyl p-biphenylyl W\_/ p~blphenyiyl (p~聯苯基） 25 l-naphthyl H H H H H H 26 l-naphthyl Ph H H Ph H H 27 l-naphthyl H Ph Ph H H H 28 l-naphthyl H Ph H H H H 29 l-naphthyl H H Ph H H H 30 l-naphthyl H H H H Ph H 31 l-naphthyl H H H H H Ph 32 l-naphthyl H H H H Ph Ph 33 l-naphthyl H H H H l-naphthyl H 34 l-naphthyl H H H H H l-naphthyl 35 1-naphthyl H H H H l-naphthyl l-naphthyl 36 l-naphthyl H H H H 2-naphthyl H 37 1-naphthyJ H H H H H 2-naphthy] 38 l-naphthyl H H H H 2-naphthyJ 2-naphthyl 39 l-naphthyl H H H H o-biphenylyl H 40 l-naphthyl H H H H H o-biphenylyl 41 1-naphthyl H H H H o-biphenylyl o-biphenylyi 42 l-naphthyl H H H H m-biphenylyl H 43 l-naphthyl H H H H H m-biphenylyl 44 l-naphthyl H H H H m-biphenylyl m-biphenylyl 45 l-naphthyl H H H H p-biphenylyl H 46 l-naphthyl H H H H H p-biphenylyj 47 l-naphthyl H H H H p-bipheny!yl p-biphenylyl ---------装------1T------0 (請先閲讀背面之注意事項再填寫本頁) 本纸張尺度適用中國國家標準（CNS ) A4規格（21〇X297公釐） -203- 581751 A7 B7 五、發明説明（2〇1)
Ri R2 R3 R4 Rs R? 1¾ R, R, ^CVfi· 48 2-naphthyl H H H H H H Λ： 49 2-naphthyl Ph H H Ph H H 50 2-naphthyl H Ph Ph H H H 51 2-naphthyl H Ph H H H H ^-<>V 52 2-naphthyl H H Ph H H H R, «a 53 2-naphthyi H H H H Ph H TypeCCC 54 2-naphthyl H H H H H Ph 55 2-naphthyl H H H H Ph Ph 56 2-naphthyl H H H H 1-naphthyl H c6 57 2-naphthyl H H H H H 1-naphthyl 58 2-naphthyl H H H H 1-naphthyl 1-naphtliyl 1-naphthyl (1-蔡基） 59 2naphthyl H H H H 2-naphthyl H 60 2-naphthyl H H H H H 2-naphtliyl CO 61 2-naphthyl H H H H 2-naphthyl 2-naphthyl 2-naphthyl (2-萘基） 62 2-naphthyl H H H H o-biphenylyl H 63 2-naphthyl H H H H H o-blphenyM <>h> 64 2-naphthyl H H H H o-biphenylyl o-biphenylyl o-biphenylyl (〇聯苯基） 65 2-naphthyl H H H H m-biphenylyl H 66 2-naphthyl H H H H H m-biphenylyi 67 2-naphthyl H H H H m-biphenylyl m-biphenylyl 68 2-naphthyl H H H H p-blphenylyl H m-Wphenylyl (m-聯苯基) 69 2-naphthyl H H H H H p-biphenylyl rvrv 70 2-naphthyl H H H H p~biphenyjyl p-blphenylyl /vy p-blphenylyl (p«聯苯基) 71 o-biphenylyl H H H H H H 72 o-biphenylyl Ph H H Ph H H 73 o-biphenylyl H Ph Ph H H H 74 o-biphenylyl H Ph H H H H 75 o-biphenylyl H H Ph H H H 76 o-biphenylyl H H H H Ph H 77 o-biphenylyl H H H H H Ph 78 o-biphenylyl H H H H Ph Ph 79 o-biphenylyl H H H H 1-naphthyl H 80 o-biphenylyl H H H H H 1-naphthyJ 81 o-biphenylyl H H H H 1-naphthyl 1-naphthyl 82 o-biphenylyl H H H H 2-naphthyl H 83 o-biphenylyl H . H H H H 2-naphthyi 84 o-biphenylyl H H H H 2-naphthyl 2-naphthyl 85 o-biphcnylyl H H H H o-biphenylyl H 86 o-biphenylyl H H H H H o-biphenylyl 87 o-biphenylyl H H H H o-biphenylyl o-biphenylyl 88 o-biphenyjyl H H H H m-biphenylyi H 89 o-biphenylyl H H H H H m-biphenylyl 90 o-biphenylyl H H H H m-biphenylyl ] m-biphenylyl 91 o-biphenylyl H H H H p-blphenylyl H 92 o-biphenyiy] H H H H H p-biphenylyl 93 o-biphcnylyl H H H H p-biphenylyl p-biphenylyi ---------^------1T------^ (請先閲讀背面之注意事項再填寫本頁) 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -204 - 581751 A7B7 五、發明説明（202)
Ri R2
v 109 〇〇 110 o-biphenylyl 111 (〇·聯苯基）112 od π1! m-biphenylyl (m-聯本基) 115 116 p-b丨phenylyl (P-聯苯基） 117 118 119 120 121 122 123 124 125 126 127 128 129 130 131 132 133 134 135 136 137 138 139
m-biphenylyl H m-biphenylyl Ph m~bipheny]y] H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl h m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H m-biphenylyl H p-biphenylyl H p-biphenylyl Ph p-biphenylyl H p-biphenylyl H p-blphenylyl H p-biphenylyl H p-blphenylyl H p-blphenylyl h p-biphenylyl H p-biphenylyl H p-biphenylyl H p-blphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyl H p-blphenylyl H p-biphenylyl H p-blphenylyl H p-biphenylyl H p-biphenylyl H p-biphenylyl H R3 & R5 R? Re Η Η Η Η H Η Η Ph Η H Ph Ph Η Η H Ph Η Η Η H Η Ph Η Η H Η Η Η Ph H Η Η Η Η Ph Η Η Η Ph Ph Η Η Η 1-naphthyl H Η Η Η Η 1-naphthyl Η Η Η 1-naphthyl 1-naphthyl Η Η Η 2-naphthyl H Η Η Η Η 2-naphthyl Η Η Η 2-naphthyl 2-naphthyl Η Η Η o-blphenylyl H Η Η Η Η o-biphenyJyl Η Η Η o-biphenylyl o-biphenylyl Η Η Η m-biphenylyl H Η Η Η H m-biphenyJy) Η Η Η m-biphenylyl m-biphenylyl Η Η Η p-biphenylyl H Η Η Η H p-blphenylyi Η Η Η p-biphenylyl p-biphenylyl Η Η Η H H Η Η Ph H H Ph Ph Η H H Ph Η Η H H Η Ph Η H H Η Η Η Ph H Η Η Η H Ph Η Η Η Ph Ph Η Η Η 1-naphthyl H Η Η Η H 1-naphthyl Η Η Η 1-naphthyl 1-naphthy] Η Η Η 2-naphthyl H Η Η Η H 2-naphthyl Η Η Η 2-naphthyl 2-naphthyl Η Η Η o-biphenyJyl H Η Η Η H o-biphenyJyd Η Η Η o-blphenylyl o-blphenylyl Η Η Η m-biphenyiyl H Η Η Η H m-biphenylyl Η Η Η m-biphcnyjyl m-blphenylyl Η Η Η p-biphenylyJ H Η Η Η H p-blphenylyi Η Η Η p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -205- 581751 A7 B7 五、發明説明（203)
Ri
141 142 143 144 145 146 147 148 149 150 151 152 153
p-blphenyJyl (P«聯苯基）172 173 o-toly丨（〇·甲苯基） m-tdyl (m-甲苯基） p-tolyl (p* 甲苯基） 174 175 176 177 178 179 180 181 182 183 184 185 186 187 188 189 190 o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-toJyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-toiyl m-tolyl m-tolyl m-tolyl m-toiyl m-tolyl m-tolyj m-tolyl m-tolyl m-tolyl m-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-toJyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-toiyl p-tolyl p-tolyJ p-tolyl p-tolyl R2 R3 Ra Rs R? Re Η Η Η Η Η Η Ph Η Η Ph Η Η Η Ph Ph Η Η Η Η ' Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Η 1-naphthyl Η Η Η Η Η Η 1-naphthyJ Η Η Η Η 2-naphthyl Η Η Η Η Η Η 2-naphthyl Η Η Η Η o-biphenylyl Η Η Η Η Η Η o-biphenylyl Η Η Η Η m-biphenylyl Η Η Η Η Η Η m-biphenylyl Η Η Η Η p-biphenylyl Η Η Η Η Η Η p-biphenylyl Η Η Η Η o-tolyl Η Η Η Η Η Η o-toly] Η Η Η Η Η Η Ph Η Η Ph Η Η Η Ph Ph Η Η Η Η Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Η 1-naphthyl Η Η Η Η Η Η 1-naphthyl Η Η Η Η 2-naphthyl Η Η Η Η Η Η 2-naphthyl Η Η Η Η o-biphenylyl Η Η Η Η Η Η o-biphenylyl Η Η Η Η m-biphenylyl Η Η Η Η Η Η m-biphenylyl Η Η · Η Η p-biphenylyl Η Η Η Η Η Η p-biphenylyl Η Η Η Η m-tolyl Η Η Η Η Η Η m-tolyl Η Η Η Η Η Η Ph Η Η Ph Η Η Η Ph Ph Η Η Η Η Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Η 1-naphthyl Η Η Η Η Η Η 1-naphthyl Η Η Η Η 2-naphthyl Η Η Η Η Η Η 2-naphthyl Η Η Η Η o-biphenylyl Η Η Η Η Η Η o-biphenylyl Η Η Η Η m-biphenylyl Η Η Η Η Η Η m-biphenylyl Η Η Η Η p-blphenylyl Η Η Η Η Η Η ] p-biphenylyl Η Η Η Η p-tolyl Η Η Η Η Η Η p-tolyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -206- 581751 Α7 Β7 五、發明説明（204)
Rl
191 192 193 194 195 196 197 198 199 200 201 202 203 204 205 206 207 208 209 210 211 212 213 214 215 216 217 218 219 220 221 222 m-biphenylyl 223 (m-聯苯基）224 225 C0 1-naphUiyl (】·萘基) 2-naphthyl (2·萘基) ob o-biphenylyl (〇·聯苯基)od p-biphenylyl (P·聯苯基) o^to丨yl (〇·甲苯基） m-tolyl (m·甲苯基） p-tolyl <p*田苯基） aNj〇
DPA
TPA 226 227 228 229 230 231 232 233 234 235 236 237 238 239 240 241 242 243 244 245 246 247 248 249 250
Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenyiyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyJ m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-blphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenyiyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl R2ΗΗΗΗΗ ΗΗΗΗΗΗΗ Η Η ΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗ Η Η Η Η ΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗ R3 Η/1 R7
Re -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 Η Η Η Η Η Η Η Η Η Η ΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗΗ Η ΗΗΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗΗ Η ΗΗΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗ ΗΗΗΗΗ ΗΗΗΗΗΗ Η Η Η ΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗ Η Η Η Η ΗΗ Η ΗΗΗΗΗΗΗΗΗΗΗΗ Η Η ΗΗΗΗΗΗΗΗΗΗΗ
Η Η Η HH
13133 Η Η S-CH-CH-CH -CH3 -CH3 -CH3 -CH3 i3133 3 3 -CH-CHH Η Η Η Η Η Η h.chh-ch-ch Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η -CH3 -CH3 -CH3 -CH3 (請先閲讀背面之注意事項再填寫本頁) Η -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 •CH3
Η3Η3 V V
-C -CH3HH Η Η Η HDPADPADPADPADPADPAH Η Η Η Η ΗΤΡΑΤΡΑΤΡΑΤΡΑΤΡΑΤΡΑ :CH3-CH3HDPADPADPADPADPADPAH ΗΗΗΗ ΗΤΡΑΤΡΑΤΡΑΤΡΛΤΡΑΤΗΗ Η Η 本紙伕尺度適用中國國家標準（CNS ) A4M ( 210X297公釐） 207- 581751 A7 B7 五、發明説明（205) ^vur^rAl'ti^alL^: Ατ.·>乍4-p^
Rl R2 R3 Rs R? Re -〇-r· 1 Η H H H H H H λ3~°7 2 Ph H H H H H H 6 3 Ph Ph H H Ph H H X 〕R 4 Ph H Ph Ph H H H 5 Ph H Ph H H H H 6 Ph H H Ph H H H Ri 1 B« 7 Ph H H H H Ph H TypcDDD 8 Ph H H H H H Ph 9 Ph H H H H Ph Ph 10 Ph H H H H 1-naphthyl H 〇6 11 Ph H H H H H 1-naphthyl 12 Ph H H H H 1-naphthyl 1-naphthyl 1-naphthyl (1-萘基） 13 Ph H H H H 2-naphthyJ H 14 Ph H H H H H 2-naphthyl ccr 15 Ph H H H H 2-naphthyl 2-naphthyl 2-naphthyl (2·蔡基） 16 Ph H H H H o-biphenylyl H 17 Ph H H H H H o-biphenylyl 18 Ph H H H H o-biphenylyl o-biphenylyl \-Tvy o-blphenyJyl (0-聯苯基） 19 Ph H H H H m-blphenylyl H 20 Ph H H H H H m-biphenylyl 21 Ph H H H H m-biphenylyl m-biphenylyl 〇〇 22 Ph H H H H p-blphenylyl H m-Wphenylyl (m·聯苯基） 23 Ph H H H H H p-biphenylyl 24 Ph H H H H p-blphenylyi p-biphenylyJ p~blphenyly】(P~ 聯苯基） 25 1-naphthyl H H H H H H 26 1-naphthyl Ph H H Ph H H 27 1-naphthyl H Ph Ph H H H 28 1-naphthyl H Ph H H H H 29 1-naphthyl H H Ph H H .H 30 1-naphthyl H H H H Ph H 31 1-naphthyl H H H H H Ph 32 1-naphthyl H H H H Ph Ph 33 1-naphthyl H H H H 1-naphthyl H 34 1-naphthyl H H H H H 1-naphthyl 35 1-naphthyl H H H H 1-naphthyl 1-naphthyl 36 1-naphthyl H H H H 2-naphthyl H 37 1-naphthyl H H H H H 2-naphthyl 38 1-naphthyl H H H H 2-naphthyl 2-naphthyl 39 1-naphthyi H H H H o-biphenylyl H 40 1-naphthyl H H H H H o-biphenylyl 41 1-naphthyl H H H H o-biphenylyl o-biphenylyl 42 1-naphthyl H H H H m-biphenylyl H 43 1-naphthyl H H H H H m-blphenylyl 44 1-naphthyl H H H H m-blphenylyl m-biphenylyl 45 1-naphthyl H H H H p-biphenylyl H 46 1-naphthyl H H H H H p-biphenylyl 47 1-naphthyi H H H H p-blphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -208- 581751 A7 B7 五、發明説明（ 206)
TypeDDD od C0 1-naphthyl (1-蔡基） 2-naphthyl (2·蔡基） ob o~biphenyiyl (〇-聯苯基） Ri R2 Rj R4 Rs R? Re 48 2-naphthyl H H H 0 H H H 49 2-naphthyJ Ph H H Ph H H 50 2-naphthyl H Ph Ph H H H 51 2-naphthyl H Ph H H H H 52 2-naphthyl H H Ph H H H 53 2-naphthyl H H H H Ph H 54 2-naphthyl H H H H H Ph 55 2-naphthyl H H H H Ph Ph 56 2-naphthyl H H H H 1-naphthyl H 57 2-naphthyJ H H H H H 1-naphthyl 58 2-naphthyl H H H H 1-naphthyl 1-naphthyl 59 2naphthyl H H H H 2-naphthyl H 60 2-naphthyl H H H H H 2-naphthyl 61 2-naphthyl H H H H 2-naphthyl 2-naphthyl 62 2-naphthyl H H H H o-blphenylyl H 63 2-naphthyl H H H H H o-biphenylyi 64 2-naphthyl H H H H o-biphenylyl o-biphenylyl 65 2-naphthyl H H H H m-blphenylyl H 66 2-naphthyl H H H H H m-biphenylyl 67 2-naphthyl H H H H m-biphenylyl m-biphenylyl 68 2-naphthyl H H H H p-biphenylyl H 69 2-naphthyl H H H H H p-biphenylyl 70 2-naphthyl H H H H p-biphenylyl p-biphenylyl 71 o-blphenylyl H H H H H H 72 o-biphenylyl Ph H H Ph H H 73 o-biphenylyl H Ph Ph H H H 74 o-biphenylyl H Ph H H H H 75 o-biphenylyl H H Ph H H H 76 o-blphenylyl H H H H Ph H 77 o-biphenylyl H H H H H Ph 78 o-biphenylyl H H H H Ph Ph 79 o-biphenylyl H H H H 1-naphthyl H 80 o-blphenylyl H H H H H 1-naphthyl 81 o-blirfienylyl H H H H 1-naphthyl 1-naphthyl 82 o-biphenylyl H H H H 2-naphthyl H 83 o-biphenylyl H H H H H 2-naphthyl 84 o-biphenylyl H H H H 2-naphthyl 2-naphthyl 85 o-blphenylyl H H H H o-biphenylyl H 86 o-biphenylyi H H H H H o-biphenylyi 87 o-biphenylyi H H H H o-biphenylyl o-biphenyly! 88 o-biphenyly) H H H H m-biphenylyl H 89 o-biphenylyl H H H H H m-biphenylyl 90 o-biphenylyl H H H H m-biphenylyl m-biphenylyi 91 o-biphenylyl H H H H p-biphenylyl H 92 o-biphenyly】 H H H H H p-biphenylyl 93 o-biphenylyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -209- 581751 A7B7 五、發明説明（2〇7)
TypcDDD C0 ob o-blphenylyl (0,od £耷r巧 Ar>t*£;p^ -biphenyly] (m-聯苯基) Rl R2 R3 Rs R? Re 94 m-biphenylyl H H H H H H 95 m-biphenylyl Ph H H Ph H H 96 m-biphenylyl H Ph Ph H H H 97 m-biphenylyl H Ph H H H H 98 m-biphenylyl H H Ph H H H 99 m-blphenyJyl H H H H Ph H 100 m-biphenylyl H H H H H Ph 101 m-biphenylyl H H H H Ph Ph 102 m-biphenylyl H H H H 1-naphthyl H 103 m-blphenylyl H H H H H 1-naphthyl 104 m-biphenylyl H H H H 1-naphthyl 1-naphthyl 105 m-biphenylyl H H H H 2-naphthyl H 106 m-biphenylyl H H H H H 2-naphthyl 107 m-biphenylyl H H H H 2-naphthyl 2-naphthyl 108 m-biphenylyl H H H H o-biphenylyl H 109 m-biphenylyl H H H H H o-biphenylyl 110 m-biphenylyl H H H H o-biphenylyl o-blphenylyl 111 m-biphenylyl H H H H m-biphenylyl H 112 m-biphenylyl H H H H H m-biphenylyl 113 m-biphenylyl H H H H m-biphenyjyl m-blphenylyl 114 m-biphenylyl H H H H p-biphenylyl H )115 m-biphenylyl H H H H H p-biphenyiyl 116 m-biphenylyl H H H H p-biphenyjyl p-biphenylyl 基） 117 p-biphenylyl H H H H H H 118 p-biphenylyl Ph H H Ph H H 119 p-biphenylyl H Ph Ph H H H 120 p-biphenylyl H Ph H H H H 121 p-biphenylyl H H Ph H H H 122 p-biphenylyl H H H H Ph H . 123 p-biphenylyl H H H H H Ph 124 p-blphenylyl H H H H Ph Ph 125 p-biphenylyl H H H H 1-naphthyl H 126 p-biphenylyl H H H H H 1-naphthyl 127 p-biphenyJyl H H H H 1-naphthyl 1-naphthyl 128 p-biphenylyl H H H H 2-naphthyl H 129 p-biphenylyl H H H H H 2-naphthyl 130 p-biphenylyl H H H H 2-naphthyl 2-naphthyl 131 jx-biphenylyl H H H H o-biphenylyl H 132 p-biphenylyl H H H H H o-biphenylyl 133 p-biphenylyl H H H H o-biphenylyl o-biphenylyl 134 p-biphenylyl H H H H m-blphenylyl H 135 p-biphenylyl H H H H H m-biphenyjyl 136 p-biphenylyl H H H H m-biphenylyl m-biphenylyl 137 p-biphenylyl H H H H p-biphenylyl H 138 p-biphenylyl H H H H H p-biphenylyJ 139 p-biphenylyl H H H H p-biphenylyl p-biphenylyj (請先閱讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -210- 581751 A7 B7 五、發明説明（208)
140 141 142 143 144 145
TypcDDD
o-tolyl (°·甲苯蕞） lyylylylylylylyl RIl-totolto]to]tolto]toltol 0-o-o-o-o-o-o-cr m-tolyl (m·甲苯基） p-tdyl介甲χ基）
£ P 174 175 176 177 178 179 180 181 182 183 184 185 186 187 188 189 190 R2 R3 1¾ Rs R? Re Η Η Η Η η Η Ph Η Η Ph Η Η Η Ph Ph Η Η Η Η Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Η 1-naphthyl Η Η Η Η Η Η 1-naphthyl Η Η Η Η 2-naphthyl Η Η Η Η Η Η 2-naphthyl Η Η Η Η o-biphenylyl Η Η Η Η Η Η o-biphenylyl Η Η Η Η m-biphenylyl Η Η Η Η Η Η m-biphenylyl Η Η Η Η p-biphenylyl Η Η Η Η Η Η p-biphenylyl Η Η Η Η o-tolyl Η Η Η Η Η Η o-tolyl Η Η Η Η Η Η Ph Η Η Ph Η Η Η Ph Ph Η Η Η Η Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Η 1-naphthyl Η Η Η Η Η Η 1-naphthyl Η Η Η Η 2-naphthyl Η Η Η Η Η Η 2-naphthyl Η Η Η Η o-biphenylyl Η Η Η Η Η Η o-biphenyJyi Η Η Η Η m-biphenylyl Η Η Η Η Η Η m-biphenylyl Η Η Η Η p-biphenylyl Η Η Η Η Η Η p-biphenylyl Η Η Η Η m-tolyl Η Η Η Η Η Η m-tolyl Η Η Η Η Η Η Ph Η Η Ph Η Η Η Ph Ph Η Η Η Η Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Η 1-naphthyl Η Η Η Η Η Η 1-naphthyl Η Η Η Η 2-naphthyl Η Η Η Η Η Η 2-naphthyl Η Η Η Η o-biphenylyl Η Η Η Η Η Η o-biphenylyl Η Η Η Η m-biphenylyl Η Η Η Η Η Η m-biphenylyl Η Η Η Η p-biphenylyl Η Η Η Η Η Η p-biplienyly! Η Η Η Η p-tolyi Η Η Η Η Η Η p-tolyl (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） .1 581751 A7B7 五、發明説明（209) R|
R3 R4 κ·ΗΗΗΗΗ ηηηηηηη η η ΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗ Η Η ΗΗ ΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗ R7
Ral ηηηηη ηηηηηηη η η ηηηη H3CH3H3H3 -CY-C-C Ι3Ι3[3[33 3333 ΗΗΗΗΗ -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 Η Η Η Η Η Η Η Η Η Η
Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenyJyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenyjyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphcnylyl p-biphenylyl ΗΗΗΗΗ ΗΗΗΗΗΗΗ Η Η ΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗΗ Η ΗΗΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗ 191 192 193 194 195 196 197 198 199 200 201 202 203 204 205 206 207 208 209 210 211 212 213 214 215 216 217 218 219 220 221 222 223 224 225 226 227 228 229 230 231 232 233 234 235 236 237 238 (請先閲讀背面之注意事項再填寫本頁) 色 乔.？Λ1 寸 ι η57ήηή at^^ml^^.
TypcDDD C0 l-naphthyl Ο莱基) 2-naphthyl (2-萘基)ob o-biphenylyl (〇·聯苯基)od -biphenylyl (m·聯苯基） p-biphenylyl (p·聯苯基) 〇-tolyl (〇甲苯基） m-tolyl (m·甲苯基） p-tolyl (p·田χ基） Q <Qb< 90123 4 5 6 7 8 9 ο 3 4 4 4 4 4 4 4 4 4 4 5 22222 2 22222 2 ΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗ Η Η ΗΗΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗΗ Η ΗΗΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗ Η -CH3 Η -CH3 Η -CH3 Η -CH3 Η -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 Η DPA Η DPA Η DPA Η DPA Η DPA Η DPA DPA Η DPA Η DPA Η DPA Η DPA Η DPA Η τρατρλτρατρατρατραη ΗΗΗ Η Η ηηηηηητρατρατρατρατρατρα 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -212 - 581751 A7 B7 五、發明説明（21〇)
Rl R2 Γ<3 R4 Rs R? 1¾ 1 Η H H H H H H Λτ 2 Ph H H H H H H 3 Ph Ph H H Ph H H 4 Ph H Ph Ph H H H 5 Ph H Ph H H H H 6 Ph H H Ph H H H 1 7 Ph H H H H Ph H Type££E 8 Ph H H H H H Ph 9 Ph H H H H Ph Ph 10 Ph H H H H l-naphthyl H C0 11 Ph H H H H H 1-naphthyJ 12 Ph H H H H l-naphthyl l-naphthyl l-naphthyl (1·萘基） 13 Ph H H H H 2-naphthyl H 14 Ph H H H H H 2-naphthyJ ca 15 Ph H H H H 2-naphthyl 2-naphthyl 2-naphthyl (2-蔡基） 16 Ph H H H H o-biphenylyl H 17 Ph H H H H H o-biphenylyl /^v-H 18 Ph H H H H o-blphenylyl o-biphenylyl o-biphenylyl (〇·聯苯基） 19 Ph H H H H m-blphenylyl H 20 Ph .H H H H H m-biphenylyl 21 Ph H H H H m-biphenylyl m-biphenylyl oo 22 Ph H H H H p-biphenylyl H m-blphenylyl (m-聯苯基) 23 Ph H H H H H p-biphenylyl 24 Ph H H H H p-biphenyjyl p-biphenylyl p-biphenylyl 々聯苯基） 25 l-naphthyl H H H H H H 26 l-naphthyl Ph H H Ph H H 27 l-naphthyl H Ph Ph H H H 28 l-naphthyl H Ph H H H H 29 l-naphthyl H H Ph H H H 30 l-naphthyl H H H H Ph H 31 l-naphthyl H H H H H Ph 32 1-naphthyl H H H H Ph Ph 33 l-naphthyl H H H H l-naphthyl H 34 1-naphthyl H H H H H l-naphthyl 35 l-naphthyl H H H H l-naphthyl l-naphthyl 36 l-naphthyl H H H H 2-naphthyl H 37 l-naphthyl H H H H H 2-naphthyl 38 l-naphthyl H H H H 2-naphthyl 2-naphthyl 39 l-naphthyl H H H H o-biphenyjy] H 40 l-naphthyl H H H H H o-biphenylyl 41 l-naphthyl H H H H o-blphenyJyl o-biphenylyl 42 l-naphthyl H H H H m-blphenylyl H 43 l-naphthyl H H H H H m-biphenylyl 44 l-naphthyl H H H H m-biphenyJyl m-biphenylyl 45 l-naphthyl H H H H p-biphenylyl H 46 l-naphthyl H H H H H p-biphenylyl 47 l-naphthyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） _213 - 581751 A7 B7 五、發明説明（211) «2 R, Ri 1¾ R3 R4 Rs R? Re 48 2-naphthyl H H H H H H 0 49 2-naphthyl Ph H H Ph H H >τ 50 2-naphthyl H Ph Ph H H H rV 51 2-naphthyl H Ph H H H H ^-ο^ν 52 2-naphthyl H H Ph H H H Η1 53 2-naphthyl H H H H Ph H TypeEEE 54 2-naphthyl H H H H H Ph 55 2-naphthyl H H H H Ph Ph 56 2-naphthyl H H H H 1-naphthyl H C0 57 2-naphthyl H H H H H 1-naphthyl 58 2-naphthyl H H H H 1-naphthyl 1-naphtha 卜naphthyl (1-萘基） 59 2naphthyl H H H H 2-naphthyJ H 60 2-naphthyl H H H H H 2-naphthyl ccr 61 2-naphthyl H H H H 2-naphthyl 2-naphthyl 2-naphthyl (2-蔡基） 62 2-naphthyl H H H H o-biphenylyl H 63 2-naphthyl H H H H H o-biphenylyl O-K 64 2-naphthyl H H H H o-biphenylyl o-biphenylyl \—/ λ_/ o-biphenylyl (o聯苯基） 65 2-naphthyl H H H H m-biphenyjyl H 66 2-naphthyl H H H H H m-biphenylyl 67 2-naphthyl H H H H m-biphenylyl m-biphenylyl o~o 68 2-naphthyl H H H H p-biphenyiyl H m-biphenylyl (m-聯本基) 69 2-naphthyl H H H H H p-biphenyly] /"VTV* 70 2-naphthyJ H H H H p-biphenyly] p-biphenyJyl wvy p-biphenylyl (I>聯苯基） 71 o-biphenylyl H H H H H H 72 o-biphenylyl Ph H H Ph H H 73 o-biphenylyl H Ph Ph H H H 74 o-biphenylyl H Ph H H H H 75 o-biphenylyl H H Ph H H H 76 o-biphenylyl H H H H Ph H 77 o-biphenylyl H H H H H Ph 78 σ-blphenylyl H H H H Ph Ph 79 o-biphenylyl H H H H 1-naphthyl H 80 o-biphenylyl H H H H H 1-naphthyl 81 o-biphenylyl H H H H 1-naphthyl 1-naphthyl 82 o-biphenylyl H H H H 2-naphthyl H 83 o-biphenylyl H H H H H 2-naphthyl 84 o-biphenylyl H H H H 2-naphthyl 2-naphthyl 85 o-biphenylyl H H H H σ-blphenylyJ H 86 o-biphenylyl H H H H H o-biphenylyl 87 o-biphenylyl H H H H o-biphenylyl o-biphenylyl 88 o-blphenylyl H H H H m-biphenylyl H 89 o-biphenylyl H H H H H m-biphenylyl 90 o-biphenylyl H H H H m-biphenylyl ; m-biphenylyl 91 o-blphenylyl H H H H p-biphenylyl H 92 o-biphenylyl H H H H H p-biphenylyl 93 o-biphenylyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X 297公釐） -214- 581751 A7 B7 五、發明説明（212) b ?， X—V Ri R2 Ra Ri Rr, R? Rfi 94 m-biphenylyl H H H H H H χτ^-^ 95 m-biphenylyl Ph H H Ph H H C00 96 m-biphenyiyl H Ph Ph H H H η* 97 m-biphenylyl H Ph H H H H 98 m-biphenylyl H H Ph H H H 99 m-biphenylyl H H H H Ph H R1 100 m-biphenylyl H H H H H Ph TypeEEE 101 m-biphenylyl H H H H Ph Ph 102 m-biphenylyl H H H H 1-naphthyl H C0 103 m-biphenylyl H H H H H 1-naphthyl 104 m-biphenylyJ H H H H 1-naphthyl 1-naphthyl l-naphthyl (1-萊基） 105 m-biphenylyl H H H H 2-naphthyl H 106 m-biphenylyl H H H H H 2-naphthyl OC> 107 m-blphenylyl H H H H 2-naphthyl 2-naphthyl 2-naphthyl (2-萊基) 108 m-biphenylyl H H H H o-biphenylyl H ob 109 m-blphenylyl H H H H H o-biphenylyl 110 m-biphenylyl H H H H o-biphenylyl o-biphenylyl o-biphenylyl 111 m-biphenylyl H H H H m-biphenylyl H (〇·聯苯基）112 m-biphenylyl H H H H H m-biphenylyl od m-blphenylyl (m-聯苯基) 113 m-blphenyJyl H H H H m-biphenylyl m-blphenylyl 114 m-biphenylyl H H H H p-biphenylyl H 115 m-biphenylyl H H H H H p-biphenylyl 116 m-bipheny]yl H H H H p-biphenyjyl p-biphenylyl p~biphenylyl (P·聯苯基） 117 p-biphenylyl H H H H H H 118 p-blphenylyl Ph H H Ph H H 119 p-biphenylyl H Ph Ph H H H 120 p-blphenylyl H Ph H H H H 121 p-biphenylyl H H Ph H H H 122 p-biphenylyl H H H H Ph H 123 p-biphenylyl H H H H H Ph 124 p-biphenylyl H H H H Ph Ph 125 p-biphenylyl H H H H 1-naphthyl H 126 p-biphenylyl H H H H H 1-naphthyl 127 p-biphenylyl H H H H 1-naphthyl 1-naphthyl 128 p-biphenylyl H H H H 2-naphthyl H 129 p-biphenylyl H H H H H 2-naphthyl 130 p-biphenylyl H H H H 2-naphthyl 2-naphthyl 131 p-blphenyly! H H H H o-biphenylyl H 132 p-biphenylyl H H H H H o-biphenylyl 133 p-biphenylyl H H H H o-biphenylyl o-biphenylyl 134 p-biphenylyl H H H H m-biphenylyi H 135 p~blphenyly] H H H H H m-biphenylyl 136 p-biphenylyj H H H H m-biphenylyl m-biphenylyl 137 p-biphenylyl H H H H p-bipheny]y] H 138 p-biphenylyl H H H H H p-biphenylyl 139 p-biphenylyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -215 - 581751 A7 B7 五、發明説明（213)
TypeEEE C0 2-naphthyl (2-莱基） ob o-biphenylyl (〇·聯苯基） od m-blphenylyl p-blphenyJyl (p·聯苯基） crto丨yl (〇·甲苯基） m-tolyl <nv田苯基） -〇-ch> p-tolyl 田苯塞） Ri R2 R3 1¾ Rs R? Re 140 o-tolyl H H H H H H 141 o-tolyl Ph H H Ph H H 142 o-tolyl H Ph Ph H H H 143 o-tolyl H H H H Ph H 144 o-tolyl H H H H H Ph 145 o-tolyl H H H H 1-naphthyl H 146 o-tolyl H H H H H 1-naphthyl 147 o-tolyl H H H H 2-naphthyl H 148 o-tolyl H H H H H 2-naphthyl 149 o-tolyl H H H H o-biphenylyl H 150 o-tolyl H H H H H o-biphenylyl 151 o-tolyl H H H H m-biphenylyl H 152 o-tolyl H H H H H m-biphenyiyl 153 o-tolyJ H H H H p-biphenylyl H 154 o-tolyl H H H H H p-biphenylyl 155 o-tolyl H H H H o-tolyl H 156 o-tolyl H H H H H o-tolyJ 157 m-tolyl H H H H H H 158 m-tolyl Ph H H Ph H H 159 m-tolyl H Ph Ph H H H 160 m-tolyJ H H H H Ph H 161 m-tolyl H H H H H Ph 162 m-tolyl H H H H 1-naphthyl H 163 m-tolyl H H H H H 1-naphthyl 164 m-toly] H H H H 2-naphthyl H 165 m-tolyl H H H H H 2-naphthyl 166 m-tolyl H H H H o-biphenylyl H 167 m-tolyl H H H H H o-biphenylyl 168 m-tolyl H H H H m-biphenylyl H 169 m-tolyl H H H H H m-biphenylyl 170 m-tolyl H H H H p-biphenylyl H 171 m-tolyl H H H H H p-biphenylyl 172 m-tolyl H H H H m-tolyl H 173 m-tolyJ H H H H H m-tolyl 174 p-tolyl H H H H H H 175 p-tolyl Ph H H Ph H H 176 p-tolyl H Ph Ph H H H 177 p-tolyl H H H H Ph H 178 p-tolyl H H H H H Ph 179 p-tolyl H H H H 1-naphthyl H 180 P-tolyl H H H H H 1-naphthyl 181 p-tolyl H H H H 2-naphthyl H 182 p-tolyl H H H H H 2-naphthyl 183 p-tolyl H H H H o-biphenylyl H 184 p-tolyi H H H H H o-blphenylyl 185 p-toiyi H H H H m-biphenylyl H 1S6 p-toJy] H H H H H m-biphenylyl 187 p-tolyi H H H H p-biphenylyl H 188 p-tolyl H H H H H p-biphenylyl 189 p-tolyl H H H H p-tolyl H 190 p-tolyl H H H H H p-iolyl (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4说格（210X297公釐） -216- 581751
7 7 A B 五、發明説明（214)
Ri R2 ¾
Rd rs R7
191 192 193 194 195 196 197 198 199 200 201 202 203 204 205 206 207 208 209 210 211 212 卜naphthyl (l·萘基） 213 ca 2；: 2-naphthyl (2-萘基）216 217 v 218 <>0 219 220 221 od 222 m-biphenylyl 223 (m·聯苯基）224 225 226 227 H,c 228 ^ W 229 230 o-toly] (〇甲苯基）231 _^CH, 232 233 234 235 236 237 238 239 240 241 242 243 244 245 246 247 248 249 250
TypeEEE οό o-blphenylyl (〇·聯苯基） p-biphenylyl Ο聯苯基） m-toly】（m·甲苯基） -O-chj p-to丨yl少田茏基）αΝο
DPA 0
TPA
Ph 1- naphtyl 2- naphthyl 0- biphenyly] m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- blphenylyl m-blphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-blphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-biphenylyi p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyJ p-biphenylyl Ph 1- naphtyJ 2- naphthyl o-biphenyly] m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-blphenylyl p-bipheny]yj HHHHH hhhhhhh η h hhhhhhhh hhhh
HH Η H HH HHH HHHHHHHHHHHHH H
H3hi3H3H3hl3啦-I3-I3-I3 HHHHHH HH HHHHHHH Η HH HHH HHHHHHHHHHH
HHHHHHHHHHH
HH HHHHHHHHHHHH ^^^^^hhhhhhhhhhhhh hhhhhhhh hhhhh hhhhhh hhhhhh hhhhhhhhhhhhh hhhhh hhhhhh h h h hhhhhhhh hhhhhhh η hhhhh hhhhhhh hhhhh η h hhhhhhhhhhh hxhhx HHHH:S-CH3:S33:HHHH HHHHH-CH3:HH33:CH33»CH3-CH3r3HHHHHHDPADPADPADPADPAT hhhhhtpa^tpa=
ReΗ Η Η HH Η Η Η Η Η Η Η Η Η Η Η Η Η -CH3 - CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 ? :dpadpadpadpathhhh ητρλτρλτρλτρλτρατραηηηηηη (請先閲讀背面之注意事項再填寫本頁) 裝.
、1T 線 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -217- 581751 A7 B7 五、發明説明（215)
Ri R2 R3 Ri Rs R? Re FU R 1 Η H H H H H H -X\ 2 Ph H H H H H H γ 3 Ph Ph H H Ph H H /-V ] 4 Ph H Ph Ph H H H ώΒ‘ 5 Ph H Ph H H H H 6 Ph H H Fh H H H 7 Ph H H H H Ph H TypeLLL 8 Ph H H H H H Ph 9 Ph H H H H Ph Ph 10 Ph H H H H 1-naphthyl H o6 11 Ph H H H H H 1-naphthyl 12 Ph H H H H 1-naphthyl 1-naphtliyl 1-naphthyl (1·蔡基） 13 Ph H H H H 2-naphthyl H 14 Ph H H H H H 2-naphthyl ccr 15 Ph H H H H 2-naphthyl 2-naphthyl 2-naphthyI (2-萘基） 16 Ph H H H H o-biphenylyl H 17 Ph H H H H H o-biphenylyl 18 Ph H H H H o-biphenyiyl o-biphenylyl o-biphenylyl (o-聯苯基） 19 Ph H H H H m-biphenylyl H 20 Ph H H H H H m-biphenylyl 21 Ph H H H H m-biphenylyl m-biphenylyl Ολ3 22 Ph H H H H p-blphenylyl H m-biphenyJyl (m-聯苯基) 23 Ph H H H H H p-blphenylyl 24 Ph H H H H p-biphenylyi p-biphenylyl p-biphenylyl (P~聯苯基） 25 1-naphthyl H H H . H H H 26 1-naphthyl Ph H H Ph H H 27 1-naphthyl H Ph Ph H H H 28 1-naphthyl H Ph H H H H 29 1-naphthyl H H Ph H H H 30 1-naphthyl H H H H Ph H 31 1-naphthyl H H H H H Ph 32 1-naphthyl H H H H Ph Ph 33 1-naphthyl H H H H 1-naphthyJ H 34 1-naphthyl H H H H H 1-naphthyl 35 1-naphthyl H H H H 1-naphthyl 1-naphthyl 36 1-naphthyl H H H H 2-naphthyl H 37 1-naphthyJ H H H H H 2-naphthyJ 33 1-naphthyl H H H H 2-naphthyl 2-naphthyl 39 1-naphthyl H H H H o-biphenylyl H 40 1-naphthyl H H H H H o-biphenylyl 41 1-naphthyl H H H H o-biphenylyl o-biphenyiyl 42 1-naphthyl H H H H m-biphenylyl H 43 1-naphthyl H H H H H m-biphenylyl 44 1-naphthyl H H H H m-biphenylyl m-biphenylyl 45 1-naphthyl H H H H p-biphenylyl H 46 1-naphthyl H H H H H p-biphenylyl 47 1-naphthyl H H H H p-biphenylyl p-biphenyh/l (請先閲讀背面之注意事項再填寫本頁) -裝. 訂 線 本紙浪尺度適用中國國家標準（CNS ) Α4規格（210X29*7公釐） -218- 581751 A7B7 五、發明説明（216)
p»biphenylyl (p·聯苯基） Ri 1¾ R3 R/i Rs R? Re 48 2-naphthyl H H H H H H 49 2-naphthyl Ph H H Ph H H 50 2-naphthyl H Ph Ph H H H 51 2-naphthyl H Ph H H H H 52 2-naphthyl H H Ph H H H 53 2 - naphthyl H H H H Ph H 54 2-naphthyl H H H H H Ph 55 2 - naphthyl H H H H Ph Ph 56 2-naphthyl H H H H 1-naphthyl H 57 2-naphthyl H H H H H 1-naphthyl 58 2-naphthyl H H H H 1-naphthyl 1-naphthyl 59 2naphthyl H H H H 2-naphthyl H 60 2-naphthyl H H H H H 2-naphthyl 61 2-naphthyl H H H H 2-naphthyl 2-naphthyl 62 2-naphthyl H H H H o-biphenylyl H 63 2-naphthyl H H H H H o-biphenylyl 64 2-naphthyl H H H H o-biphenylyl o-biphenylyl 65 2-naphthyl H H H H m-blphenylyl H 66 2-naphthyl H H H H H m-biphenylyl 67 2-naphthyl H H H H m-biphenylyl m-blphenylyl 68 2-naphthyl H H H H p-blphenylyl H 69 2-naphthyl H H H H H p-biphenylyl 70 2-naphthyl H H H H p-biphenylyl p-blphenylyl 71 o-biphenylyl H H H H H H 72 o-blphenylyl Ph H H Ph H H 73 o-blphenylyl H Ph Ph H H H 74 o-biphenylyl H Ph H H H H 75 o-biphenylyl H H Ph H H H 76 o-blphenylyl H H H H Ph H 77 o-biphenylyl H H H H H Ph 78 o-biphenylyl H H H H Ph Ph 79 o-blphenylyl H H H H 1-naphthyl H 80 o-biphenylyl H H H H H 1-naphthyl 81 o-biphenylyl H H H H l-napMhyJ 1-naphthyl 82 o-biphenylyl H H H H 2-naphthyl H 83 o-blphenylyJ H H H H H 2-naphthyl 84 o-biphenyM H H H H 2-naphthyi 2-naphthyl 85 o-blphcnylyl H H H H o-biphenylyl H 86 o-biphenylyl H H H H H o-blphenylyl 87 o-biphenylyl H H H H o-biphenylyl o-biphenylyl 88 o-bipheny)yl H H H H m-biphenylyl H 89 o-blphenyJyl H H H H H m-biphenylyl 90 o-biphenylyl H H H H m-biphenylyl m-biphenylyl 91 o-biphenylyl H H H H p-biphenylyj H 92 o-biphenylyl H H H H H p-biphenylyl 93 o-biphenylyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁)
TypeLLL 〇6 l-naphthyl (1·蔡基） 2-naphthyl (2-蔡基） ob * o-blphenylyl (〇聯苯基） od * m-b丨pheny丨yl (m-聯本基）69 -219- 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） 581751 A7B7 五、發明説明（217 )
Ri R2 R4
Rg R?
Ra
TypeLLL 94 95 96 97 98 99 100 101 102 rrS 103 104 1- naphthy] (1-萊基）105 οσ ：〇°； 2- naphthyl Ο萘基）i〇8 v 109 〇〇 110 o-biphenylyl 1 工1 (〇聯苯基）112 orf m-biphenylyl (m·聯苯基) 115 116 p»blphenylyl (p-聯苯基） 117 118 119 120 121 122 123 124 125 126 127 128 129 130 131 132 133 134 135 136 137 138 139 L·a
m-biphenyiyl Η Η H m-biphenylyl Ph Η H m-biphenylyl H Ph Ph m-biphenylyl H Ph H m-biphenylyl Η H Ph m-biphenylyl Η Η H m-biphenylyl Η Η H m-biphenylyl Η Η H m-biphenylyl Η Η H m-blphenylyl Η Η H m-biphenylyl Η Η H m-biphenylyl Η Η H m-biphenylyl Η Η H m-biphenylyl Η Η H m-blphenylyl Η Η H m-biphenylyJ Η Η H m-blphenylyl Η Η H m-biphenylyl Η Η H m-biphenylyl Η Η H m-biphenylyl Η Η H m-biphenylyl Η Η H m-biphenylyl Η Η H m-biphenyJyl Η Η H p-biphenylyl Η Η H p-biphenylyl Ph Η H p-blphenylyJ H Ph Ph p-blphenylyl H Ph H p-biphenylyl Η H Ph p-biphenylyl Η Η H p-biphenylyl Η Η H p-btphenylyl Η Η H p-biphenylyl Η Η H p-biphenyJvl Η Η H p-biphenylyl Η Η H p-biphenylyl Η Η H p-biphenylyl Η Η H p-biphenylyl Η Η H p-blphenylyl Η Η H p-biphenylyl Η Η H p-biphenylyl Η Η H p-biphenylyl Η Η H p-biphenyJyl Η Η H p-biphenyJyl Η Η H p-biphenyiyl Η Η H p-biphenylyl Η Η H p-biphenylyl Η Η H H H Η H Η H Η H H Ph Η H H Ph H 1-naphthyl Η H H 1-naphthyl H 2-naphthyl Η H H 2-naphthyl H o-biphenylyl Η H H o-biphenylyl H m-biphenylyl Η H H m-biphenylyl H p-biphenylyl Η H H p-biphenylyl H Ph
H Ph H H H H H H H H H H H Ph H Ph H 1-naphthyl Η H H 1-naphthyl H 2-naphthyl Η H H 2-naphthyl H o-biphenylyl H o-biphenyiyl m-biphenylyl H m-biphenylyJ p-biphenylyl H p-biphenylyl H H H H H H Ph Ph H 1-naphthyl 1- naphthyl H 2- naphthyl 2-naphthyl H o-biphenylyl 0- biphenylyl H m-biphenylyl m-biphenylyl H p-biphenylyl p-bipheny]yl H H H H H H Ph Ph H 1- naphthyl 1 - naphthyl H 2- naphthyl 2-naphthyl H o-biphenylyl o-biphenyJyl H m-biphenylyl m-biphenylyl H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -220- 581751 A7B7 五、發明説明（218 )
Ri R2 R：i R/i
TypeLLL 141 142 143 144 145 146 147 148 149 150 151 152 153 154 155 156 157 158 159 160 161 162 163 164 165
Rs R? Re Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Ph Η 1-naphthyl Η Η Η 1-naphthyl Η 2-naphthyl Η Η Η 2-naphthyl Η o-biphenylyl Η Η Η o-biphenylyl Η m-biphenylyl Η Η Η m-biphenylyl Η p-biphenylyl Η Η Η p-biphenylyl Η o-tolyl Η Η Η o-tolyl Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Ph Η 1-naphthyl Η Η Η 1-naphthyl Η 2-naphthyl Η Η Η 2-naphthyl Η o-biphenylyl Η Η Η o-biphenylyl Η m-biphenylyl Η Η Η m-biphenylyl Η p-blphenylyl Η Η Η p-biphenylyl Η m-toiyl Η Η Η m-toly] Η Η Η Ph Η Η Η Η Η Η Ph Η Η Η Ph Η 1-naphthyl Η Η Η 1-naphthyl Η 2-naphthyl Η Η Η 2-naphthyl Η o-biphenylyl Η Η Η o-biphenylyl Η m-biphenylyl Η Η Η m-biphenylyl Η p-biphenylyl Η Η Η p-biphenylyl Η p-tolyl Η Η Η p-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyi o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl o-tolyl m-tolyl m-tolyl m-tolyl m-tolyJ m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-toiyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl p-toiy] p-tolyi p-tolyl p-to)yl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl
H H Ph H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H
H Ph H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H H
H H Ph H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H H H Ph H H H H H H H H H H H H H H (請先閲讀背面之注意事項再填寫本頁) L· i C0 1- naphthyl (丨-萘基）οσ 2- napiUhyl (2·萘基）ob o-biphenylyl (〇·聯苯基） 」 166 〇-〇 167 m-biphenylyl 168 (m-聯苯基）169 170 171 172 p-biphenylyl 0>聯苯基）% o-tolyl 甲苯基） m-tolyl •田苯基） ~〇"CHs p-tolyl <]>*甲茏基） 173 174 175 176 177 178 179 180 181 182 183 184 185 186 187 188 189 190 本紙法尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -221 - 581751 A7B7 五、發明説明（219 )
Ri R2
TypeLLL 191 192 193 194 195 196 197 198 199 200 201 202 203 204 205 206 207 208 209 210 211 212 1- naphthyl (1.莱基） 213οα nt 2- naphthyl (2-萘基）216 217 v 218 〇-v> 219 o-blphenylyl 220 (〇·聯苯基）221 od ξ m-blphenylyl (m-聯苯基）224 225 C0 226 227 p-blphenylyl (P·聯苯基）咖 Η,ε\_. 229 230 crtolyl (°*甲茏基）231 232 233 234 235 —237 p-tolyl (p·田苯基> m**tolyl (m·甲茏基）
CXOP
DPA -O' t>
TPA 238 239 240 241 242 243 244 245 246 247 248 249 250
Ph 1- naphtyl 2- naphthyl 0- biphenylyl m-blphenylyl p-blphenylyl o-toJyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl crblphenylyl m-biphenylyl p-biphenylyl o-toly] m-toJyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenyJyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tdyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl ΗΗΗΗΗ ηηηηηηη η η ηηηηηηηη ηηηηηη η η ηη ηη η ηηηηηηηηηηηηη η ΗΗΗΗΗΗΗΗΗΗ Η ^ ΗΗΗΗΗΗΗΗ ΗΗΗΗΗΗΗ Η ΗΗΗΗΗ ΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗΗ ι«131313133333 R31 η ηηηηηηηη ηηηηηηη η η η ηηη ηηηηηηηηηηηηη ηηηηηηηηηηηη r5 R7 ηηηηη ηηηηηηη η η ηηηηηηηη ηηηηηηη η ηηηηη ηηηηηηηηηηηηηηηηηηηηηηηηη ΗΗΗΗΗ HHHH-CH3SHH3:-CH3-CH3PHHHH hhhxh:h33:hh33-ch3::h3hhhhhhdpadpadpadpadpadpahhhhhhtpatpatpatpatpatpa RSηηηηη ηηηηηηη η η ηη
Η Η -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 DPA DPA DPA DPA DPA DPA H H H H H H ΤΡΛ ΤΡΛ ΤΡΛ TPA ΤΡΛ TPA H H H H H H (請先閱讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4坑格（210>< 29*7公* ) -222 581751 A7 B7 五、發明説明（220 )
TypcMMM
EL 土 P C0 1-naphthyl (1 -萘基） 2-naphthyl (2-萘基） ob 一 o-b丨phenylyl (〇聯本基） p-blphenylyl (p« 聯苯基） R] R2 R3 Hi 1¾ R? 1¾ 1 Η H H H H H H 2 Ph H H H H H H 3 Ph Ph H H Ph H H 4 Ph H Ph Ph H H H 5 Ph H Ph H H H H 6 Ph H H Ph H H H 7 Ph H H H H Ph H 8 Ph H H H H H Ph 9 Ph H H H H Ph Ph 10 Ph H H H H 1-naphthyl H 11 Ph H H H H H 1-naphthyl 12 Ph H H H H 1-naphthyl 卜 naphthyl 13 Ph H H H H 2-naphthyl H 14 Ph H H H H H 2-naphthyl 15 Ph H H H H 2-naphthyl 2-naphthyl 16 Ph H H H H o-biphenylyj H 17 Ph H H H H H o-biphenylyl 18 Ph H H H H o-biphenylyl o-biphenylyl 19 Ph H H H H m-biphenylyl H 20 Ph H H H H H m-biphenylyl 21 Ph H H H H m-biphenyJyl m-biphenylyl 22 Ph H H H H p-biphenylyl H 23 Ph H H H H H p-biphenylyl 24 Ph H H H H p-biphenylyl p-blphenylyl 25 1-naphthyl H H H H H H 26 1-naphthyl Ph H H Ph H H 27 1-naphthyl H Ph Ph H H H 28 1-naphthyl H Ph H H H H 29 1-naphthyl H H Ph H H H 30 1-naphthyl H H H H Ph H 31 1-naphthyl H H H H H Ph 32 1-naphthyl H H H H Ph Ph 33 1-naphthyl H H H H 1-naphthyl H 34 1-naphthyl H H H H H 1-naphthyl 35 1-naphthyl H H H H 1-naphthyl 1-naphthyl 36 1-naphthyl H H H H 2-naphthyJ H 37 1-naphthyl H H H H H 2-naphthyl 38 1-naphthyl H H H H 2-naphthyl 2-naphthyl 39 1-naphthyl H H H H o-biphenyJyl H 40 1-naphthyl H H H H H o-biphenylyl 41 1-naphthyl H H H H o-biphenylyl o-biplienylyi 42 1-naphthyl H H H H m-biphenylyl H 43 1-naphthyl H H H H H m-biphenylyl 44 1-naphlhy] H H H H m-biphenylyl m-biphenylyl 45 1-naphthyJ H H H H p-biphenylyJ H 46 1-naphthyl H H H H H p-biphenylyl 47 1-naphthyl H H H H p-biphenylyl p-biphenylyi (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -223- 581751 A7 B7 五、發明説明（221 ) 一£.斧芦？^1才1，73、11巧^^乍土卞^
Ri R2 R3 Rl Ks R? Rh 48 2-naphthyl H H H H H H Y Rs 49 2-naphthyl Ph H H Ph H H 50 2-naphthyl H Ph Ph H H H 51 2-naphthyl H Ph H H H H 52 2-naphthyl H H Ph H H H TypeMMM 53 2-naphthyl H H H H Ph H 54 2-naphthyl H H H H H Ph 55 2-naphthyl H H H H Ph Ph 56 2-naphthyl H H H H 1-naphthyl H οό 1-naphthy丨（1-蔡基） 57 2-naphthyl H H H H H 1-naphthyl 58 2-naphthyl H H H H 1-naphthyl 1-naphthyl 59 2naphthyl H H H H 2-naphthyl H 60 2-naphthyl H H H H H 2-naphthyl CCX 61 2-naphthyl H H H H 2-naphthyl 2-naphthyl 2-naphthyl (2-蔡基） 62 2-naphthyl H H H H crbiphenylyl H 63 2-naphthyl H H H H H o-biphenylyl ob * o-biphenylyl (〇·聯苯基） 64 2-naphthyl H H H H o-blphenylyl o-blphenylyl 65 2-naphthyl H H H H m-biphenylyl H 66 2-naphthyl H H H H H m-biphenylyl od … 67 2-naphthyl H H H H m-biphenylyl m-blphenylyJ 68 2-naphthyl H H H H p-blphenylyl H m-biphenylyl (m_聯本基） 69 2-naphthyJ H H H H H p-biphenylyl 70 2-naphthyl H H H H p-biphenylyl p-biphenylyl p-bipheny】yl (p«聯苯基） 71 o-biphenylyl H H H H H H 72 o-blphenylyl Ph H H Ph H H 73 o-blphenylyl H Ph Ph H H H 74 o-biphenylyl H Ph H H H H 75 o-biphenylyl H H Ph H H H 76 o-biphenylyl H H H H Ph H 77 o-blphcnylyl H H H H H Ph 78 o-biphenylyl H H H H Ph Ph 79 o-blphenylyl H H H H 1-naphthyl H 80 o-biphenyiyl H H H H H 1-naphthyl 81 o-biphenylyl H H H H 1-naphthyJ 1-naphthyl 82 o-biphenylyl H H H H 2-naphthyl H 83 o-biphenylyl H H H H H 2-naphthyl 84 o-blphenylyi H H H H 2-naphthyl 2-naphthyl 85 o-blphenylyl H H H H o-biphenyiyj H 86 o-biphenylyl H H H H H o-biphcny)yl 87 o-biphenylyl H H H H o-biphenylyl o-blphenylyl 88 o-Wphenylyl H H H H m-biphenylyl H 89 o-biphenylyl H H H H H m-blphenylyi 90 o-biphenylyl H H H H m-biphenylyl m-biphenylyl 91 o-biphenylyl H H H H p-biphenylyl H 92 o-biphenylyl H H H H H p-biphenylyl 93 o-biphenylyl H H H H p-biphenylyl p-biphenylyl 訂 線 (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4洗格（210X297公釐） -224- 581751 A7 B7 五、發明説明（222 )
TypcMMM 00 o-b α-biphenylyl (〇·聯苯基） o-d n-biphenylyl (m·聯苯基) Rl R2 R3 Iti Rs R? He 94 m-biphenylyl H H H H H H 95 m-biphenylyl Ph H H Ph H H 96 m-biphenylyl H Ph Ph H H H 97 m-biphenyiyl H Ph H H H H 98 m-biphenylyl H H Ph H H H 99 m-biphenylyl H H H H Ph H 100 m-blpheny]yl H H H H H Ph 101 m-biphenylyl H H H H Ph Ph 102 m-biphenylyl H H H H 1-naphthyl H 103 m-biphenylyl H H H H H 1-naphthyl 104 m-biphenylyl H H H H 1-naphthyl 1-naphthyl 105 m-biphenylyl H H H H 2-naphthyl H 106 m-biphenylyl H H H H H 2-naphthyl 107 m-biphenylyl H H H H 2-naphthyl 2-naphthyl 108 m-biphenylyl H H H H o-blphenylyl H 109 m-biphenylyl H H H H H o-biphenylyl 110 m-biphenylyl H H H H o-blphenylyl o-biphenylyl 111 m-biphenylyl H H H H m-biphenylyl H 112 m-biphenylyl H H H H H m-biphenylyl 113 m-biphenylyl H H H H m-blphenylyl m-blphenyJyl 114 m-biphenylyl H H H H D-biphenylyl H 115 m-biphenylyl H H H H H p-biphenylyJ 116 m-biphenylyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) Λϋκι ρ Γ H 才 3、Γ!气 Λ .T 土 CLyJv 117 p-biphenylyl H H H H H H 118 p-biphenylyl Ph H H Ph H H 119 p-biphenylyl H Ph Ph H H H 120 p-blphenyiyl H Ph H H H H 121 p-biphenylyl H H Ph H H H 122 p-biphenylyl H H H H Ph H 123 p-biphenylyl H H H H H Ph 124 p-biphenylyl H H H H Ph Ph 125 p-biphenylyl H H H H 1-naphthyl H 126 p-biphenylyl H H H H H 1-naphthyl 127 p-biphenylyl H H H H 1-naphthyl 1-naphthyl 128 p-biphenylyl H H H H 2-naphthyl H 129 p-biphenylyl H H H H H 2-naphthyl 130 p-biphenyly] H H H H 2-naphthyl 2-naphthyl 131 p-biphenylyl H H H H o-biphenylyl H 132 p-biphenylyl H H H H H o-blphenylyl 133 p-biphenylyJ H H H H o-biphenylyl o-biphenylyl 134 p-biphenylyl H H H H m-biphenylyl H 135 p-biphenyiyl H H H H H m-biphenylyl 136 p-biphenylyl H H H H m-blphenylyl m-biphenylyl 137 p-biphenylyl H H H H p-biphenylyl H 138 p-biphenylyl H H H H H p-biphenylyl 本紙張尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） -225- 581751 A7 B7 五、發明説明（223 )
TypeMMM c6 爱氧r^rrA15i4-7nirx.3 Ar->乍 1 卞货 ob o-biphenylyl (〇·聯苯基) o-d m-blphenylyl (m·聯苯基） o-to】y丨（°·甲苯基） m-tolyl <m•甲苯基） p-toly丨（P·田苯基） Rj R2 R3 R4 R5 R? 1¾ 140 crtolyl H H H H H H 141 o-tolyl Ph H H Ph H H 142 o-tolyl H Ph Ph H H H 143 o-tolyl H W H H Ph H 144 o-tolyl H H H H H Ph 145 o-tolyl H H H H 1-naphthyl H 146 o-tolyl H H H H H 1-naphthyl 147 o-tolyl H H H H 2-naphthyJ H 148 o-tolyl H H H H H 2-naphthyl 149 o-tolyl H H H H o-biphenylyi H 150 o-tolyl H H H H H o-biphenylyl 151 o-tolyl H H H H m-biphenylyl H 152 o-tolyl H H H H H m-biphenylyl 153 o-tolyl H H H H p-biphenylyl H 154 o-toJyl H H H H H p-biphenylyl 155 o-tolyl H H H H o-tolyl H 156 o-tolyl H H H H H o-tolyl 157 m-tolyl H H H H H H 158 m-tolyl Ph H H Ph H H 159 m-tolyl H Ph Ph H H H 160 m-tolyl H H H H Ph H 161 m-tolyl H H H H H Ph 162 m-tolyl H H H H 1-naphthyl H 163 m-tolyl H H H H H 1-naphthyl 164 m-tolyl H H H H 2-naphthyl H >165 m-tolyl H H H H H 2-naphthyl 166 m-tolyl H H H H o-biphenylyl H 167 m-tolyl H H H H H o-blphenylyl 168 m-tolyl H H H H m-biphenylyl H 169 m-tolyl H H H H H m-biphenylyl 170 m-tolyl H H H H p-blphenylyl H )m m-tolyl H H H H H p-biphenylyl 172 m-tolyl H H H H m-tolyl H 173 m-tolyl H H H H H m-tolyl 174 p-tolyl H H H H H H 175 p-tolyl Ph H H Ph H H 176 p-tolyl H Ph Ph H H H 177 p-tolyl H H H H Ph H 178 p-toJy] H H H H H Ph 179 p-tolyl H H H H 1-naphthyl H 180 p-toiyl H H H H H 1-naphthyl 181 p-tolyl H H H H 2-naphthyl H 182 p-tolyl H H H H H 2-naphthyl 183 p-tolyl H H H H o-biphenylyl H 184 p-tolyl H H H H H o-biphenylyl 185 p-tolyl H H H H m-biphenylyl H 186 p-tolyl H H H H H m-biphenylyl 187 p-tolyi H H H H p-biphenylyl H 188 p-tolyl H H H H H p-biphenylyl 189 p-toiyl H H H H p-tolyl H 190 p-tolyl H H H H H p-tolyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） -226- 581751 A7 B7 五、發明説明（224 )
Ri R2
Rn
Rs r7
TypeMMM 191 192 193 194 195 19β 197 198 199 200 201 202 203 204 205 206 207 208 209 210 211 212 213 214 215 216 217 218 219 220 221 222 n-biphenylyl 223 (m-聯苯基） 225 C0 1-naphthyl 莱基) 2-naphthyl (2·萘基）ob o-biphenylyl (O聯苯基) p-biphenylyl (P·聯苯基) o-to丨yl (〇·甲苯基） έ夸l^rAl 才 1^411巧^^乍1卞^
m-tolyl (m·甲苯基） p>tolyl (p·甲苯基）CXjO
DPA -o t>
TPA 226 227 228 229 230 231 232 233 23A 235 236 237 238 239 240 241 242 243 244 245 246 247 248 249 250
Ph 1- naphtyl 2- naphthyl 0- blphenylyl m-biphenylyl p-biphenylyl o-toly] m-toJyl p-tolyl Ph 1- naphtyl 2- naphthyl o-blphenylyl m-biphenylyl p-biphenyJyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-blphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-blphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl
HHHHH hhhhhhh Η H HHHHHHHH HHHHHH Η H HH HHH HHHHHHHHHHHHH HHHHHHHHHHHH
a:ccHH:^3p:s33^HHHHH HHHHHHHH HHHHHHH H HHHHH HHHHHHHHHHHHH HHHHHHHHHHHH -i3333I33333 HHHHHHHHHH HHHHHH Η H HHHHH HHHHHHHHHHHH H HHHHHHHHHHHH hhhhh hhhhhh h h h hhhhhhhh hh
HHHHH H HHHHH HHHHHHHHHHHH Η Η HHHHHHHHHH H hhhhh hhhh:s33:ch33:hh33pthh hhhh h-ch3:ch;:chh33p: hhhhh hdpadpadpadpadpadpahhhhhhtpatpatpatpatpatpa ¾hhhhh hhhhhhhh h hh Η Η -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3
-CH3:-CH3:DPADPAiDPATΗ HHH ΗΤΡΑΤΡΑΤΡΛΤΡΑΤΡΑΤΡΑΗ Η Η Η Η H (請先閲讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -227- 581751 A7 B7 五、發明説明（225 )
TypeNNN od η 土 Ρ C0 1-naphthyl (卜蔡基） 2-naphthyl (2-萘基） ob * o-Wphenylyl (〇-聯本基） p-biphenylyl (P* 聯苯基） Rl Rz 1¾ Rii R? 1¾ 1 Η H H H H H H 2 Ph H H H H H H 3 Ph Ph H H Ph H H 4 Ph H Ph Ph H H H 5 Ph H Ph H H H H 6 Ph H H Ph H H H 7 Ph H H H H Ph H 8 Ph H H H H H Ph 9 Ph H H H H Ph Ph 10 Ph H H H H 1-naphthyl H 11 Ph H H H H H 1-naphthyl 12 Ph H H H H 1-naphthyl 1-naphtliyJ 13 Ph H H H H 2-naphthyl H 14 Ph H H H H H 2-naphthyl 15 Ph H H H H 2-naphthyl 2-naphthyl 16 Ph H H H H o-biphenylyl H 17 Ph H H H H H o-biphenylyl 18 Ph H H H H o-biphenylyl o-biphenylyl 19 Ph H H H H m-biphenylyl H 20 Ph H H H H H m-biphenylyl 21 Ph H H H H m-biphenylyl m-biphenylyl 22 Ph H H H H p-blphenylyl H 23 Ph H • H H H H j>-biphenylyl 24 Ph H H H H p-biphenylyl p-biphenylyl 25 1-naphthyl H H H H H H 26 1-naphthyl Ph H H Ph H H 27 1-naphthyl H Ph Ph H H H 28 1-naphthyl H Ph H H H H 29 1-naphthyl H H Ph H H H 30 1-naphthyl H H H H Ph H 31 1-naphthyl H H H H H Ph 32 1-naphthyl H H H H Ph Ph 33 1-naphthyl H H H H 1-naphthyl H 34 1-naphthyl H H H H H 1-naphthyl 35 1-naphthyl H H H H 1-naphthyl 1-naphthyl 36 1-naphthyl H H H H 2-naphthyl H 37 1-naphthyl H H H H H 2-naphthyl 38 1-naphthyl H H H H 2-naphthyl 2-naphthyl 39 1-naphthyl H H H H o-blphenyly] H 40 1-naphthyl H H H H H o-biphenylyl 41 1-naphthyl H H H H o-biphenylyl o-biphenylyl 42 1-naphthyl H H H H m-biphenylyl H 43 1-naphthyl H H H H H m-biphenylyl 44 1-naphthyl H H H H m-biphenylyJ m-biphenylyl 45 1-naphthyl H H H H p-biphenylyl H 46 1-naphthyl H H H H H p-biphen3flyl 47 1-naphthyl H H H H p-biphenylyl p-biphenyJyl 裝 訂 線 (請先閲讀背面之注意事項再填寫本頁) 本纸張尺度適用中國國家標隼（CN’S ) A4«l格（210X29*7公釐） -228- 581751 A7 B7 五、發明説明（226 )
TypeNNN od C0 1-naphthyl (1-萘基） 2-naphthyl (2-蔡基） ob 抑 o-biphenylyl (〇«聯苯基） p-Wpheny】yl (]>聯苯基） Ri R2 Rl R4 R5 R? 1¾ 48 2-naphthyl H H H H H H 49 2-naphthyl Ph H H Ph H H 50 2-naphthyl H Ph Ph H H H 51 2-naphthyl H Ph H H H H 52 2-naphthyl H H Ph H H H 53 2-naphthyl H H H H Ph H 54 2-naphthyl H H H H H Ph 55 2-naphthyl H H H H Ph Ph 56 2-naphthyl H H H H 1-naphthyl H 57 2-naphthyl H H H H H 1-naphthy) 58 2-naphthyl H H H H 卜 naphthyl 1-naphthyl 59 2naphthyl H H H H 2-naphthyl H 60 2-naphthyl H H H H H 2-naphthyl 61 2-naphthyl H H H H 2-naphthyl 2-naphthyl 62 2-naphthyl H H H H o-blphenylyl H 63 2-naphthyl H H H H H o-biphenylyl 64 2-naphthyl H H H H o-blphenylyl o-biphenylyl 65 2-naphthyl H H H H m-biphenylyl H 66 2-naphthyl H H H H H m-biphenylyl 67 2-naphthyl H H H H m-biphenylyl m-biphenylyl 68 2-naphthyl H H H H p-biphenylyl H 69 2-naphthyl H H H H H p-biphenylyl 70 2-naphthyl H H H H p-biphenylyl p-biphenylyl 71 o-biphenylyl H H H H H H 72 o-biphenylyl Ph H H Ph H H 73 o-blphenylyl H Ph Ph H H H 74 o-biphenylyl H Ph H H H H 75 o-biphenylyl H H Ph H H H 76 o-blphenylyl H H H H Ph H 77 o-blpheny]yJ H H H H H Ph 78 o-biphenylyl H H H H Ph Ph 79 o-biphenylyl H H H H 1-naphthyl H 80 o-biphenylyl H H H H H 1-naphthyl 81 o-biphenylyl H H H H 1-naphthyl 1-naphthyl 82 o-biphenylyl H H H H 2-naphthyJ H 83 o-biphenylyl H H H H H 2-naphthyl 84 o-biphenyjy] H H H H 2-naphthyl 2-naphthyl 85 o-biphenylyl H H H H o-biphenylyl H 86 o-biphenylyl H H H H H o-bipheriyjyl 87 o-biphenylyl H .H H H o-biphenylyl o-biphenylyl 88 o-biphenylyl H H H H m-biphenylyl H 89 o-biphenylyl H H H H H m-biphenylyl 90 o-biphenylyl H H H H m-blphenylyl m-biDhenylyl 91 o-biphenylyl H H H H p-biphenylyl H 92 o-biphenylyl H H H H H p-biphenvly] 93 o-biphenylyl H H H H p-biphenylyl p-biphenylyl (請先閱讀背面之注意事項再填寫本頁) 本紙伕尺度適用中國國家標準（CNS ) A4洗格（210X297公釐） -229- 581751 A7B7 五、發明説明（227 )
Ri
TypeNNN 94 95 96 97 98 99 100 101 102 rrS 103 104卜naphthyl (1-萘基）i〇5ca : 2-naphthyl (2-萘基）i〇8 v 109 0-0 110 o-biphenylyl 111 (〇·聯苯基）112od ；；Im-biphenylyl (m-聯苯基) 115 116
土 P p-biphenylyl (P*聯苯基） 117 118 119 120 121 122 123 124 125 126 127 128 129 130 131 132 133 134 135 136 137 138 139 p-blphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenyJyl p-biphenylyl p-biphenylyl p-biphenylyl p-blphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-biphenylyl p-bipheny)yl p-biphenylyl p-biphenylyl p-biphenylyl m-biphenylyl R2 1¾ R-i R5 Η Η Η Η Ph Η Η Ph Η Ph Ph Η Η Ph Η Η Η Η Ph Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η. Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Ph Η Η Ph Η Ph Ph Η Η Ph Η Η Η Η Ph Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η Η R?
Ra H H H H H Ph H Ph 1-naphthyl H 1- naphthyl 2- naphthyl H 2-naphthyl o-biphenylyl H o-biphenylyl m-biphenylyl H m-biphenylyl p-biphenylyl H p-biphenylyl H H H H H H Ph Ph H 1-naphthyl 1- naphthyJ H 2- naphthyl 2-naphthyl H o-biphenylyl o-biphenylyl H m-biphenylyl m-biphenylyl H D-biphenylyl p-biphenyJyl Η H Η H Η H Η H Η H Ph H Η Ph Ph Ph 1-naphthyl H Η 1-naphthyl 1-naphthyl 1-naphthyl 2-naphthyl H Η 2-naphthyl 2-naphthyl 2-naphthyl o-blphenylyj H Η o-biphenylyl o-biphenylyl o-biphenylyl m-biphenylyl H H m-blphenylyl m-biphenylyl m-blphenylyl p-biphenylyl H H p-biphenylyl p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（21〇X297公釐） -230 581751 A7B7 五、發明説明（228)
TypeNNN00 1-naphthyl (1-萊基） 2-naphthy】（2-萘基）ob a-blphenylyl (〇·聯苯基） od m-biphenylyl 1¾ R/1 Rr) R? Rfi Η Η Η Η Η Η Η Ph Η Η Ph Ph Η Η Η Η Η Η Ph Η Η Η Η Η Ph Η Η Η 1-naphthyl Η Η Η Η Η 1-naphthyl Η Η Η 2-naphthyl Η Η Η Η Η 2-naphthyl Η Η Η o-biphenylyl Η Η Η Η Η o-biphenylyl Η Η Η m-biphenylyl Η Η Η Η Η m-biphenyJyl Η Η Η p-biphenylyi Η Η Η Η Η p-biphenylyl Η Η Η o-tolyl Η Η Η Η Η o-tolyl Η Η Η Η Η Η Η Ph Η Η Ph Ph Η Η Η Η Η Η Ph Η Η Η Η Η Ph Η Η Η 1-naphthyl Η Η Η Η Η 1-naphthyl Η Η Η 2-naphthyl Η Η Η Η Η 2-naphthyl Η Η Η o-biphenylyl Η Η Η Η Η o-biphenyiyl Η Η Η m-biphenylyl Η Η Η Η Η m-biphenylyl Η Η Η p-biphenylyl Η Η Η Η Η p-bipheny]yl Η Η Η m-tolyi Η Η Η Η Η m-tolyl Η Η Η Η Η Η Η Ph Η Η Ph Ph Η Η Η Η Η Η Ph Η Η Η Η Η Ph Η Η Η 1-naphthyl Η Η Η Η Η 1 一 naphthyl Η Η Η 2-naphthyl Η Η Η Η Η 2-naphthyl Η Η Η o-biphenylyl Η Η Η Η Η o-biphenylyl Η Η Η m-biphenylyi Η Η Η Η Η m-biphenylyl Η Η Η p-biphenyiyl Η Η Η Η Η p-hiphenylvl Η Η Η p-tolyl Η Η Η Η Η p-tolyl
R2HphHHH HHHHHHHHHHHHHphHHHHHHHHHHHHHHH HphHHHHHHHHHHHHHHH
Ri 140 o-tolyl 141 o-tolyl 142 o-tolyl 143 o-toJyl 144 o-tolyl 145 o-tolyl 146 o-tolyl 147 o-tolyl 148 o-tolyl 149 o-tolyl 150 〇-tolyl 151 o-tolyl 152 o-tolyl 153 °"toIyl 154 o-toiyl 155 o-tolyl 156 O-tolyl 157 m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl m-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl p-tolyl 158 159 160 161 162 163 164 165 166 167 168 (m·聯苯基）Mg p-blphenylyl (P·聃苯基) o-tolyl (〇*甲2基） m-t〇lyl (m-甲苯基） p-tolyl Φ·甲苯基） 170 171 172 173 174 175 176 177 178 179 180 181 182 183 184 185 186 187 188 189 190 本紙張尺度適用中國國家標準（CNS ) A4現格（210X297公釐） -231 - (請先閱讀背面之注意事項再填寫本頁) 581751 A7 B7 五、發明説明（229)
Ri
191 192 193 194 195 196 197 198 199 200 201 202 203 204 205 206 207 208 209 210 211 212 1- naphthyl (1-萘基） 213ca 22；: 2- naphthyl (2-系基）216 217 V 218CKD 219 o-blphenylyl 220 (〇·聯苯基）221 224 225
TypeNNN C0 m-biphenylyl (m·聯苯基) F L· 226 227 (p·聃苯基）228 H*C>-X 229 -〇 230 o-tolyl (°·甲苯基）231 232 233 m-tolyl (m•甲 5基） 236 237 238 239 240 241 242 243 244 245 246 247 248 249 250 p-biphenylyl
p-tolyl 甲苯I
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TPA
Ph 1- naphtyl 2- naphthyl o~biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-blphenylyl m-biphenylyJ p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-blphenylyl p-biphenylyl o-tolyl m-tolyl p-tolyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphcnylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-biphenylyl m-biphenylyl p-biphenylyl Ph 1- naphtyl 2- naphthyl o-blphenylyl m-biphenylyl p-biphenylyJ
R2hhhhh HHHHHHHH h HHHHHHHH hhhhhh η h hh hhh hhhhhhhhhhhhh HHHHHHHHHHHH
Ra R/i -
-CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 Η H Η H Η H Η H Η H
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R7H Η Η Η Η Η Η Η H : : :-CH3:CH33H Η Η Η Η Η Η H H-CH3r3: ::H3H Η Η Η H HDPADPADPADPADPADPAH Η Η Η Η HTPATPATPATPATPATPA R.,HHHHH HHHHHHH HHHHHHHHHH HHHHHHH H HHHHH HHHHHHHHHHHH HHHHHHHHHHHHH RKhhhhh hhhhhhh h h hh
Η Η -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 -CH3 DPA DPA DPA DPA DPA DPA H H H H H H ΤΡΛ TPA TPA TPA TPA TPA H H H H H H (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -232- 9 581751 A7 B7 五、發明説明（230
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RI R2 R3 1¾
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HphH Η 泰紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -236- 581751 A7 B7 五、發明説明（234)
R6 R?
經濟部智慧財/1局員工消黃合作社印製
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經濟部智您財凌局員工消費合作社印製
HphHHHMeHHHphHHHMeHHHph Η Η Η Η Η HHphHHHMeHHHphΗ Η Η HHphphHHMeHHHphphH Η Η Η HphH Η Η Η Η HphphH Η
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RI
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Hphphphphphphphph Η Η e Μ Η Η Η Η HHHHHphHHMeHHHHphHHMeΗ Η Η ΗphΗ Η (請先閱讀背面之注意事項再填寫本頁) 訂 本纸張尺度適用中國國家標準（CNS ) A4規^ ( 210X 297公釐） -239- 581751 A7 B7 五、發明説明（^了)
本纸乐尺度適用中國國家標準（CNS ) A4規格（210X 297公釐） -240· 581751 A7 B7 R1
Re R7 Η Η 經濟部智慧財凌局S(工消费合作社印製
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r3 r* TypeSSS
Ri R2 R3 1¾ R7 經濟部智慧財凌局員工消費合作社印災 76 77 78 79 80 81 82 83 84 85 86 87 88 89 90 91 92 93 94 96 96 97 98 99 h,c- H^C- HjC- HjC- HjC- HjC- HjC— MjC^
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R6 R? 經濟部智慧財凌局員工消费合作社印製 1 1 1 12 2 1 X 1 111 2223 100101102103104105106107108109110111112113114115
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Ri R2 R3 1¾ R5 R?
Re
TypeTTT C0 1-naphthyl (l-蔡基） 2-naphthyl (2-蔡基）o-b o-biphenylyl (〇聯苯基）gk5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 H Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph Ph
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H 1-naphthyl M Η h 1-naphthyl H 1-naphthyl 1-naphthyJ H 2-naphthyl H Η H 2-naphthyl H 2-naphthyl 2-naphthy] H 〇-blpheny]yl H Η h o-biphenylyl H 〇-biphenylyl 〇-bipheny]yl H m-biphenyly] H 20 Ph H H H H H m-biphenylyl 21 Ph H H H H m-biphenylyJ m-blpheny]yl 22 Ph H H H H p-biphenylyl H (m-聯苯基）23 Ph H H H H H p-bipheny]yJ 24 Ph H .H H H p-biphenyjyl p-biphenylyl (P-聯苯基）^ 1-naphthyl H H H H H H 26 1-naphthyl Ph H H Ph H H 27 1-naphthyl H Ph Ph H H H 28 1-naphthyl H Ph H H H H 29 1-naphthyl H H Ph H H H 30 1-naphthyl H H H H Ph H 31 1-naphthyi H H H H H Ph 32 1-naphthyl H H H H Ph Hi 33 1-naphthyl H H H H 1-naphthyl H 34 1-naphthyl H H H H H 1-naphthyi 35 1-naphthyl H H H H 1-naphthyl 1-naphthyl 36 1-naphthyl H H H H 2-naphthyl H 37 卜 naphthyl H H H H H 2-naphthyl 38 1-naphthyl H H H H 2-naphthyl 2-naphthyJ 39 1-naphthyl H H H H o-blphenyly] H 40 1-naphthyl H H H H H o-bIpheny}y] 41 1-naphthyl H H H H o-biphenyiyl o-biphenylyl 42 】-naphthyJ H H H H nvbiphenylyl H 43 1-naphthyl H H H H H m-bipheny^J 44 1-naphthyl H H H H m-biphenyly] m-biphenylyl 45 1-naphthyl H H H H p-biphenylyl H 46 1-naphthyl H H H H H p-biphenylyl 47 1-naphthyl H H H H p-biphenylyl p-biphcrn：/lyl 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -245- (請先閲讀背面之注意事項再填寫本頁) .裝·
、1T 線 581751 A7 B7 五、發明説明（243)
Ri R2 R3 R5 R?
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TypeTTT g4 55 56 57 58 59 60 61 62 63 64 65 66 〇r6 l m-Wphenylyl (m-聯苯基）69 70 OO p-biphenylyl (P"聯苯基）71 72 73 74 75 76 77 78 79 80 81 82 83 84 85 86 87 88 89 90 91 92 93 C0 1-naphthyl (1-蔡基） 2-naphthyl (2-萘基） ob 许 o-biphenylyl (〇*聯苯基） 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyJ 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyl 2-naphthyJ 2-naphthyl
H Ph H H H H H H H H H H H H H H H _ H H H H H H o-biphenylyl H o-biphenylyl Ph o-blphenylyl h o-biphenylyl H o-biphenylyl h o-biphenylyl h o-biphenyjyl h o-biphenylyl o-blphenylyl h o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl h σ-blphenylyl o-biphenylyl o-blphenylyl H o-blphenylyl h o-biphenyjyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl H o-biphenylyl h
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H H Ph H Ph H H H H H H H H H H H H H H H H H H H H Ph H Ph H H H H H H H H H H H H H H H H H H Η Η H Ph Η H Η Η H Η Η H Η Η H H Ph H Η H Ph H Ph Pli H 1-naphthyl H Η h !-naphthyl H 1-naphthyl 1-naphthyl H 2-naphthyl H Η H 2-naphtIiyl H 2-naphthyl 2-naphthyl H o-biphenylyl H Η H o-biphenylyl H o-biphenylyl 〇-bipheny]yl H m-biphenylyi H Η H m-biphenyJyl H m-biphenylyl m-biphenylyl H p-biphenylyl H Η H p-blphenylyl H P-biphenylyl p-biphenyly] H Ph H H Η H Η H Η H H Ph Η H H Ph H 1-naphthyl H 1- naphthyl 2- naphthyl H 2-naphthyl o-biphenylyl
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H H H H H H Ph Ph H 1-naphthyl 1- naphthyl H 2- naphthyl 2-naphthyi H H o-blphenylyl o-biphenylyl o-biphenyjyl m-biphenylyl h H m-biphenylyl m-biphenyly] m-biphenylyl p-biphenylyJ H H p-bipher.ylyl p-biphenylyl p-biphenylyl (請先閱讀背面之注意事項再填寫本頁) 本紙沬尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -246- 581751 A7B7 113 114 115 116 Rj R2 Ri R/i Rs R? m-biphenylyl H H H H H H m-biphenylyl Ph H H Ph H H m-biphenylyl H Ph Ph H H H m-biphenylyl H Ph H H H H m-biphenylyl H H Ph H H H m-biphenylyl H H H H Ph H m-biphenylyl H H H H H Ph m-biphenylyl H H H H Ph Ph m-biphenylyl H H H H 1-naphthyl H m-biphenylyl H H H H H 1-naphthyl m-biphenylyl H H H H I-naphthyl 1-naphthyl m-biphenylyl H H H H 2-naphthyl H m-biphenylyl H H H H H 2-naphthyl m-biphenylyl H H H H 2-naphthyl 2-naphthyl m-biphenylyl H H H H o-blphenylv] H m-biphenylyJ H H H H H o-biphenylyl m-biphenyjyl H H H H o-biphenylyl o-biphenylyi m-biphenylyl H H H H m-biphenylyl H m-biphenylyl H H H H H m-biphenyJyl m-biphenylyl H H H H m-biphenylyl m-biphenyjyl m-biphenylyl H H H H p-biphenylyl H m-biphenylyl H H H H H p-biphenylyl m-biphenylyl H H H H p-blphenylyl p-biphenylyl p-biphenylyl H H H H H H p-biphenylyl Ph H H Ph H H p-biphenylyl H Ph Ph H H H p-biphenylyl H Ph H H H H p-biphenylyl H H Ph H H H p-biphenyJyl H H H H Ph H p-blphenylyi H H H H H Ph p-biphenylyl H H H H Ph Ph p-biphenylyl H H H H 1-naphthyl H p-biphenylyl H H H H H 1-naphthyl p-biphenylyl H H H H 1-naphthyl 1-naphthyJ p-biphenylyl H H H H 2-naphthyl H p-biphenylyl H H H H H 2-naphthyl p-biphenylyl H H H H 2-naphthyl 2-naphthyl p-biphenylyl H H H H o-biphenylyl H p-biphenylyl H H H H H o-biphenylvi p-biphenylyl H H H H o-biphenylyl o-bipheny^l p-biphenylyl H H H H m-biphenylyl H p-biphenylyl H H H H H 】 m-biphenylyJ p-biphenylyl H H H H m-biphenylyl m-biphenylyl p-biphenylyl H H H H p-biphenylyl H p-biphenyly] H H H H H p-biphenylyl p-biphcnylyl H H H H p-biphenylyl p-biphenylyl (請先閲讀背面之注意事項再填寫本頁)
R3 TypeTTT 五、發明説明（244 ) 94 95 96 r2 97 98 99 100 101 102 trS 103 104 1- naphthyl (丨-萘基） οσ ；〇°： 2- naphthyl (2-萘基）ι〇8 ν 109 〇〇 110 o-blphenyiyl 111 (〇聯苯基）112 m-biphenylyl (m·聯苯基) p-b丨phenylyl (p·聯苯基） 117 118 119 120 121 122 123 124 125 126 127 128 129 130 131 132 133 134 135 136 137 138 139 本紙伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -247- 581751 A7 B7 五、發明説明（245)
148 149 150 151 152 153 154 155 00 - 1- naphthyl (1-萘基） 159 (XX 160 2- naphthyl (2-萘基） 162 〇^> ;s o-b 丨 phenylyl (〇·聯苯基） 165 」 166 〇-〇 167 m-biphenylyl 168 (m-聯苯基）169 O〇- 17〇 p-biphenylyl 171 (P·聯苯基）172 173
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7 7 A B 五、發明説明（ 246)
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裝 ； 訂 ^ 線 (請先閲讀背面之注意事項再填寫本頁) 本纸永尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -257- 581751 A7 B7 五、發明説明（25θ
經濟部智慧財/i局a(工消費合作社印¾
(請先閲讀背面之注意事項再填寫本頁) 裝· 線 本紙張尺度適用中國國家標準（CNS ) Α4規格（210Χ 297公釐） -258- 581751 A7 B7 五、發明説明（25会 本發明之化合物，具有作爲有機電致發光元件材料之 極佳特性。特別是作爲摻雜劑使用時，可發出色座標中， χ = 0·05 至 0.20，y = 0.02 至 0.30，特 別是 χ = 0 · 1 至 0 · 20，y = 0 · 05 至 0 · 20 所 示之近乎純藍色之發光色。 本發明之化合物具有極佳之安定性，於蒸鍍、塗佈等 有機電致發光元件之製造步驟中亦顯示出安定特性，製造 後即使經過長期後亦可維持安定之特性。 本發明之化合物用於有機電致發光元件使用時，其可 作爲主體材料，或作爲摻雜劑使用，特別是作爲摻雜劑使 用時，可得到上記般優良發光色與發光效率。本發明之化 合物，因兼具有電子注入輸送性、正孔注入性、或輸送性 等任一性質，故可作爲電子材料、或可作爲正孔注入，或 輸送材料等使用。 於決定有機電致發光元件之主體材料與摻雜劑之組合 內容時，需考慮下述各點內容。 (1 )應考慮以構造式進行組合。即，化合物之構造 亦會影響發光特性。 (2 )摻雜劑（發光材料）之離子化位差，以與主體 材料之離子化位差相等，或較其爲小爲佳。摻雜劑於發光 時係具有正孔捕集器之機能，而使摻雜劑容易產生單項激 勵子。又，此時，主體之單項激勵子將容易與基底狀態之 摻雜劑進行能量交換，而可提高發光效率。 (3 )摻雜劑（發光材料）之半波氧化電位，以與主 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公簸） I I I —裝 訂 —— — — —線 (請先閲讀背面之注意事項再填寫本頁) -259- 581751 A7 B7 五、發明説明（25> 體材料之半波氧化電位相等，或較其爲小爲佳。摻雜劑於 發光時係具有正孔捕集器之機能，而使摻雜劑容易產生單 項激勵子。又，此時，主體之單項激勵子將容易與基底狀 態之摻雜劑進行能量交換，而可提高發光效率。 使用本發明化合物作爲發光層時，可作爲主體材料或 作爲摻雜劑使用，特別是以作爲藍色發光用摻雜劑使用爲 最佳。本發明之化合物作爲摻雜劑使用時，主體材料以使 用蒽系材料爲佳。又，將電子輸送性材料與正孔輸送性材 料之混合材料以作爲主體之混合層使用亦爲佳。發光層， 可含有本發明化合物以外之其他複數化合物，將前述含有 複數種類化合物之發光層，或將複數種類發光層層合時， 可得到具有複數之波峰波長，或廣泛發光波長之發光層或 元件。 本發明化合物作爲主體材料使用時，摻雜劑可使用各 種有機電致發光用螢光物質。其中又以下記實施例所使用 之并四苯系之紅熒烯衍生物或二苯基并四苯衍生物、驼系 紅色螢光材料、并五苯系紅色螢光材料、苯乙烯基衍生物 系材料等爲佳。 本發明之化合物用於正孔注入輸送層時，其可作爲正 孔輸送性材料、或作爲發光材料使用亦可。作爲正孔輸送 性材料使用時，摻雜劑可使用上記所列舉之物質。 本發明之化合物用於電子注入輸送層使用時，其可作 爲電子輸送性材料，或作爲發光材料使用皆可。作爲電子 輸送性材料使用時，摻雜劑可使用上記所列舉之物質。又 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐> " ~ •260· (請先閲讀背面之注意事項再填寫本頁) -裝· 訂 線 581751 A7 ______B7 五、發明説明（25令 〇 (請先閲讀背面之注意事項再填寫本頁) (7)具有較高玻璃移轉溫度（Tg)，故可製得具 有優良高溫保存性之元件。 上記所述含有主體來要與摻雜劑之發光層，係具有正 孔與電子之注入機能、輸送機能、正孔與電子再鍵結而形 成激勵子之機能。發光層除本發明之化合物以外，尙包含 比較對電子爲中性之化合物，故可以將電子與正孔容易且 可平衡地注入、輸送。 主體材料，可單獨使用或將2種以上混合使用皆可。 2種以上使用時之混合比例可爲任意之比例。本發明之化 合物作爲主體材料時，於發光層中以含有8 0至9 9 . 9 質量％爲佳，又以90至99·9質量％ ，以95.0至 99·5質量％爲更佳。 發光層之厚度，可爲相當於分子層一層之厚度至有機 化合物層之膜厚度之間爲佳。具體而言例如1至8 5 11 m ，又以5至6 0 nm、特別是5至5 0 nm爲佳。 绶濟部替.¾时1馬8X消費合作社印災 又’混合層之形成方法，以使用不同蒸鍍來源以蒸發 方式進行共蒸鍍之方法爲佳，蒸氣壓（蒸發溫度）爲相同 程度或非常近似之情形中，可使其先於蒸鍍槽中混合再進 行蒸鍍。混合層以化合物間可以均勻混合之方式爲佳，依 各種狀況之不同，亦可使化合物以島狀形式存在。發光層 一般而言係將有機螢光物質以蒸鍍方式、或將其分散於樹 脂粘合劑中再以塗覆之方式形成發光層所需要之厚度。 ϋ張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） " 一 -262- 581751 A7 B7 五、發明説明（26〇) (蒽系化合物） 本發明之元件中較適合使用之主體材料之一， 式（5 )所示之苯基蒽衍生物。 本發明之元件，較佳以式（5 )、更佳爲式（ )、式（5-2)所示蒽系衍生物爲較適合作爲主 使用，其可抑制與摻雜劑之相互作用，而使摻雜劑 強之發光。又，此蒽系衍生物，因具有優良之耐熱 久性，故可製得長壽命之元件。 此電致發光元件，於保持元件之色純度、及最 之摻雜濃度時，可爲1質量％左右，於2至3%質 時亦僅減少1成之比例的情形下，即可得到充分實 用之元件。 / …(5) 例如下 5 - 1 體材料 得到較 性、 耐 大功率 用旦耐 (請先閱讀背面之注意事項再填寫本頁」 -裝 A101 十 式（5 )中’ Αιοι係爲單苯基蒽基或二苯基蒽基 其可爲相同或不同。L爲氫、單鍵或二價之連結基 1或2之整數。 η舄 上記式（5)、較佳爲下記式（5 一丄） 式 線 經濟部智慧財產局資工消費合作社印製 )所示化合物 本纸伕尺度適用中國國家標率（CNS ) Α4規格（210X297公釐） -263 581751 A7 B7 經濟部智慧財4局S工消費合作社印^
(Mi)q1 五、發明説明（261) (5-1)
(M4)q4 上記化合物之蒸鍍膜爲安定之非晶質狀態，故薄膜之 膜物性良好，可發出均勻且無斑紋之發光。又，大氣下可 維持一年以上之安定性而不致產生結晶化。 式（5 )之內容中，A1()1各自爲單苯基蒽基或二苯 基蒽基，其可爲相同或不同。η爲1或2之整數^ A 10 1所示之單苯基蒽基或二苯基蒽基，可爲未取代 或有取代基之基皆可，具有取代基時，其取代基可爲烷基 、芳基、烷氧基、芳氧基、胺基等，此些取代基可再被取 代基所取代。此些取代基將於後詳述。此些取代基之取代 基位置並未有特別之限定，並無須爲Μ環’其以爲與;g胃 鍵結之苯基爲佳。 本纸張尺度適用中國國家標準（CNS)A4規格（210X297公釐） (請先閲讀背面之注意事項再填寫本頁)
-264 581751 A7 ___B7 五、發明説明（262) 又，蒽環中與苯基鍵結之位置爲蒽環之9位、1 0位 爲佳。 (請先閱讀背面之注意事項再填寫本頁) 式（5 - 1 )中，L爲氫、單鍵或二價之基，L爲二 價之基時，例如可夾有伸烷基或伸芳基爲佳。前述伸芳基 之內容將於後詳述。 式（5 )所示之苯基蒽衍生物中，以式（5 - 1 )、 式（5 - 2)所示者爲佳。對式（5 - 1)說明時，式（ 5)中，Mi、M2各自爲烷基、環烷基、芳基、烷氧基、 芳氧基、胺基或雜環基等。 Μ:、M2所示之烷基，例如爲可具有直鏈或支鏈之基 ，又以碳數1至1 0，特別是1至4之經取代或未取代之 烷基爲佳。特別是碳數1至4之未取代之烷基爲更佳，具 體而言，例如甲基、乙基、（n —、i 一）丙基、（η -、i —、s —、t 一）丁基等。
Mi、M2所示之環烷基，例如環己基、環戊基等。
Mi、M2所示之芳基，以碳數6至20者爲佳，又可 具有苯基、甲苯基等取代基。具體而言，例如（〇 一、m 經濟部智慧財凌局員工消費合作社印¾ -、p -）甲苯基、芘基、萘基、蒽基、聯苯基、苯基蒽 基、甲苯基蒽基等。 Μ !、Μ 2所示之烯基，例如總碳數6至5 0者爲佳， 其可爲未取代者或具有取代基者皆可，又以具有取代基者 爲更佳。此時之取代基，例如苯基等芳基爲佳。具體而言 ’例如三苯基乙烯基、三甲苯基乙烯基、三聯苯基乙烯基 等。 . 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -265- 581751 A 7 B7 五、發明説明（263) (請先閲讀背面之注意事項再填寫本頁)
Mi、M2所示之烷氧基，其烷基部分之碳數以1至6 者爲佳，具體而言，例如甲氧基、乙氧基等。烷氧基可再 被取代亦可。
Mi、M2所示之芳氧基，例如苯氧基等。 M i、Μ 2所示之胺基，例如未取代或具有取代基者皆 可，又以具有取代基者爲佳，此時之取代基例如烷基（甲 基、乙基等）、芳基（苯基等）等。具體而言，例如二乙 基胺基、二苯基胺基、二（m -甲苯基）胺基等。 M i、Μ 2所示之雜環基，例如聯二吡啶、嘧啶基、D奎 啉基、吡啶基、噻嗯基、呋喃基、氧雜二唑基等，其又可 具有甲基、苯基等取代基。 式（5 - 1)中，Ql與q2其各自表示1至5的整 數，特別是以0或1爲佳。Μ :與Μ 2各以爲烷基、芳基、 烯基、烷氧基、芳氧基、胺基爲佳。 經濟部智您財產局資工消費合作社印^ 式（5 — 1 )中，Mi、Μ2可爲相同或不同，Mi、 M2可各自以複數形式存在，Mi間、M2間各自可爲相同 或不同，Mi間或M2間可鍵結形成苯環等環，又以形成環 之情形爲佳。 式C5 - 1)中，Li爲氫、單鍵或伸芳基，Li所示 之伸方基以無取代者爲佳’具體而言，例如伸苯基、伸聯 苯基、伸蒽基等一般之伸芳基外，尙包含2個或2個以上 芬芳基所直接連結者。L!例如單鍵、p -伸苯基、4， 4 ’ -伸聯苯基等爲佳。 L i所示之伸芳基，例如2個或2個以上伸芳基之伸院 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -266- 581751 A7 _B7___ 五、發明説明（264) 基、其可夾有—◦一、一 S —或一 NR —等進行連結者亦 可。其中，R爲烷基或芳基，烷基例如甲基、乙基等，芳 基例如苯基等，其中又以芳基爲佳，除上記之苯基外，可 爲A1()1，或苯基受A1Q1取代者亦可。 又，伸烷基例如伸甲基、伸乙基等爲佳。其中伸芳基 之具體例係如下所示。 ---------批衣----r--IT------^ (請先閱讀背面之注意事項再填寫本頁) 經濟部智慧財凌苟肖工消費合作社印製 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -267- 581751 A7 B7 五、發明説明（26冷
—<Q>-ch2h(Q>— —<^^CH2 一 CH2h(^ ~Qn香 (請先閲讀背面之注意事項再填寫本頁) 裝. 經濟部智楚財凌局員工消費合作社印复
*1T 線 本紙張尺度適用中國國家標準（CNS ) Α4規格（210X297公釐） -268- 581751 A7 B7 五、發明説明（266) 其次，將對式（5 — 2)進行說明。式（5一2)中 ，M3與M4係與式（5 - 1)中之及，q3與 Q4係與式（5 — 1)中之Ql與Q2及，l2係與式（5 一 1 )之L 1分別爲同義’較佳之例示亦爲相同。 式（5 — 2)中，m3與M4可爲相同或不同，m3|^ Μ4各爲多數存在時，M3間、Μ4間各自可爲相同或不同 ，Μ 3間或Μ 4間可鍵結形成苯環等環，又以形成環之情形 爲佳。 式（5 - 1 )、式（5 - 2 )所示化合物例如以下之 例示，本發明並不僅限定於此些化合物。又，化4 1、化 4 3、化4 5、化4 7、化4 9、化5 1、化5 3、化 5 6係爲一般式，化4 2、化4 4、化4 6、化4 8、化 50、化52、化54、化55、化57等，各自對應之 具體例係以Mil〜Ml6、Μ21〜Μ25或Μ31〜Μ35、 Μ 4 1〜Μ 4 5之組合表示。 (請先閲讀背面之注意事項再填寫本頁) 經濟部智您財是局員工消費合作社印^ 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -269 - 581751 A7 B7 五、發明説明（267)
I I I I n I扣衣 ： 訂 (請先閲讀背面之注意事項再填寫本頁) 線 經濟部智葸財凌局肖工消費合作社印絜 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -270- 581751 A7 B7 五、發明説明（26鲂 經濟部智慧財/i局員工消贲合作社印災
化合物 No. Μη m12 m13 M14 m15 m21 M22 M23 M24 m25 Μ Η H H H H H H H H H 1-2 ch3 H H H H ch3 . H H H H 1-3 H H H H t.C4H9 H H H H Ι·4 〇CH3 H H H H och3 H H H H 1-5 OPh H H H H OPh H H H H 1-6 N(C2H5)2 H H H H N(C2H5)2 H H H H 1-7 N(Ph)2 H H H H N(Ph)2 H H H H 1*8 Ph H H H H Ph H H H H 1-9 O-CHa H H H H O~CH3 H H H H MO H ch3 H H H H ch3 H H H 1-11 H ch3 H ch3 H H ch3 H ch3 H M2 H H ch3 H H H H ch3 H H 1-13 H ch3 H H ch3 H ch3 H H ch3 1-14 H H H H H H H H H 1-15 H H H H H H H H Ι·16 H Ph H H H H Ph H H H Ι·17 H \ 尸h H Ph H H H \ Ph H Ph II H 1.18 /C=C、 Ph Ph H H H H /C==Cv Ph Ph H H H H Ι·19 n-C^Hg H H H H n-C4H9 H H H H 1-20 H H H H Oh〇 H H H H 1-21 H H ΌΌ H H H H H H Ι·22 H H H H H H H H Ι·23 H H op H H H H q-o H H 1-24 H H Ph H Ph H H Ph H Ph 1-25 H H Ph Ph H H H Ph Ph H (請先閲讀背面之注意事項再填寫本頁) 本纸乐尺度適用中國國家標準（CNS ) A4規格（210X297公嫠） -271- 581751 A7 B7 五、發明説明（26身 經濟部智慧財/i局肖工消費合作社印製
(請先閱讀背面之注意事項再填寫本頁) 裝----Ί--訂------線
本紙乐尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -272- 581751 A7 B7 五、發明説明（270)
化合物 No. Μη m12 m13 M14 m15 M21 M22 m23 M24 m25 II· 1 Η H H H H H H H H H II-2 ch3 H H H H ch3 H H H H II-3 t-C4H9 H H H H H H H H ΙΙ·4 och3 H H H H 〇ch3 H H H H ΙΙ-5 OPh H H H H OPh H H H H ΙΙ·6 N(C2H5)2 H H H H N(C2H5)2 H H H H ΙΙ·7 N(Ph)2 H H H H N(Ph)2 H H H H ΙΙ·8 Ph H H H H Ph H H H H ΙΙ·9 -〇-ch3 H H H H -〇-ch3 H H H H ΙΜΟ H ch3 H H H H ch3 H H H ΙΙ-11 H H ch3 H H H ch3 ch3 H H ΙΜ2 H H ch3 ch3 H H H ch3 ch3 H ΙΜ3 H H ch3 H ch3 H ch3 ch3 H ch3 ΙΜ4 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ΙΜ5 t-C^Hg H H H H H H H H H ΙΜ6 oo H H H H H H H H ΙΙ·17 H Ph H H H H Ph H H H ΙΜ8 H H Ph H H H H Ph H H ΙΜ9 H H OO H H H H H H ΙΙ-20 ΟτΏ H H H H ~OhO H H H H 11-21 qo H H H H ΟζΟι H H H H ΙΙ-22 H H H H H H H H ΙΙ·23 H H Ph H Ph H H Ph H Ph ΙΙ·24 H H Ph Ph H H H Ph Ph H (請先閲讀背面之注意事項再填寫本頁) -裝· 訂 經濟部智慧財/1局_工^贪合作社印^ 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） •273- 581751 A7 B7 五、發明説明（271) 經濟部智慈財產局員工消费合作社印製
(請先閲讀背面之注意事項再填寫本頁) 裝----r--訂------線
本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -274- 581751 A7 B7 五、發明説明（27勿 蛵濟部智慧財凌局員工消黄合作社印¾
化合物 No. Mu m12 M】3 Mh m15 M21 M22 M23 M24 m25 ΙΙΙ·1 Η H H H H H H H H H 111-2 ch3 H H H H ch3 H H H H ΙΙΙ-3 t-C4Hg H H H H t-C^jHg H H H H ΙΙΙ-4 och3 H H H H och3 H H H H ΙΙΙ·5 OPh H H H H OPh H H H H ΙΙΙ·6 N(C2H5)2 H H H H N(C2H6)2 H H H H ΙΙΙ·7 N(Ph)2 H H H H N(Ph)2 H H H H ΙΙΙ·8 Ph H H H H Ph H H H H ΙΙΙ-9 -〇^ch3 H H H H ~O~CH3 H H H H ΙΙΜΟ H ch3 H H H H ch3 H H H ΠΙ-11 H H ch3 H H H H ch3 H H ΙΙΙ·12 H H ch3 ch3 H H H ch3 ch3 H ΙΙΙ-13 H H ch3 H ch3 H H ch3 H ch3 ΙΙΜ4 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ΙΙΙ·15 H Ph H H H H Ph H H H III· 16 H H Ph H H H H Ph H H ΙΙΜ7 H H H H OrQ H H H H III· 18 t-C4H9 H H H H H H H H H ΙΙΜ9 -o H H H H H H H H ΙΙΙ-20 N-N H H H H N~N H H H H ΙΙΙ-21 -^Vch3 H H H H -Q^ch3 H H H H ΙΙΙ-22 Cpo H H H H 090 H H H H ΙΙΙ-23 ΌΌ II H H H H H H H ΙΙΙ-24 H H H H H H -〇hQ H H ΙΙΙ·25 H H H H H H H H ΙΙΙ-26 H H H H H H H H ΙΙΙ-27 H H Ph H Ph H H Ph H Ph ΙΙΙ-28 H H Ph Ph H H H Ph Ph H (請先閲讀背面之注意事項再填寫本頁) 本紙永尺度適用中國國家標準（CNS ) A4規格（210X 297公釐） -275- 581751 A7 _B7 五、發明説明（27$ 蛵濟部智M?財/i局資工消費合作社印¾
(請先閱讀背面之注意事項再填寫本頁) 裝· —線 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -276- 581751 A7 B7 五、發明説明（27今 經濟部智您財4局：®工消费合作社印¾
化合物 No. Μπ m12 m13 M14 m15 m21 M22 M23 m24 m25 IV· 1 Η H H H H H H H H H IV-2 ch3 H H H H ch3 H H H H IV-3 t-C^Hg H H H H t-C4H9 H H H H IV-4 och3 H H H H och3 H H H H ΐν·5 OPh H H H H OPh H H H H IV-6 N(C2H5)2 H H H H N(C2H5)2 H H H H ΐν·7 N(Ph)2 H H H H N(Ph)2 H H H H IV-8 Ph H H H H Ph H H H H IV-9 -〇-ch3 H H H H -〇-ch3 H H H H IV· 10 H ch3 H H H H ch3 H H H IV· 11 H H ch3 H H H H ch3 H H IV-12 H H ch3 ch3 H H H ch3 ch3 H IV-13 H H ch3 H ch3 H H ch3 H ch3 IV-14 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 IV-15 H H H H H H H H H H IV-16 H H Ph H H H H Ph H H IV· 17 oo H H H H 〇〇 H H H H IV-18 t*C4H9 H H H H H H H H H IV-19 -o H H H H o H H H H IV-20 N-N 人 >>Ph 0 H H H H N-N 々Ph H H H H IV-21 OO H H H H H H H H IV-22 H H H H H H H H IV-23 H H H H H H H H IV-24 H H ΟζΡ H H H H H H IV-25 H H Ph H Ph H H Ph H Ph IV-26 H H Ph Ph H H H Ph Ph H (請先閱讀背面之注意事項再填寫本頁) -裝- 訂 線 本紙永尺度適用中國國家標隼（CNS ) A4規格（210X297公釐） -277- 581751 A7 B7 五、發明説明（2巧
(請先閱讀背面之注意事項再填寫本頁)
經濟部智慧財凌局員工消費合作社印製 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -278- 581751 A7 B7 五、發明説明（27$ 經濟部智慈財凌局g(工消費合作社印災
化合物 No. μ31 m32 m33 m34 m35 m41 m43 m44 m45 ν·ι Η H H H H H H H H H V-2 ch3 H H II H ch3 H H H H V-3 t*C4Hg H H H H t-C4H9 H H H H V-4 och3 H H H H och3 H H H H V-5 OPh H H H H OPh H H H H V-6 N(C2H5)2 H H H H N(C2H5)2 H H H H V-7 N(Ph)2 H H H H N(Ph)2 H H H H V-8 Ph H H H H Ph H H H H V-9 -〇-ch3 H H H H H H H H ν·ιο H ch3 H H H H ch3 H H H V-ll H H ch3 H H H H ch3 H H V-12 H H ch3 ch3 H H H ch3 ch3 H V-13 H H ch3 H ch3 H H ch3 H ch3 ν·14 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 V-15 H Ph H H H H Ph H H H V-16 H H Ph H H H Ή Ph H H V-17 H H H H OrO H H H H V-18 t-C^Hg H H H H t-C4H9 H H H H V-19 cpo H H H H OpO H H H H V-20 〇9 H H H H 〇9 H H H H V-21 -o N-N H H H H N-N H H H H V-22 -4, >-Ph 0 H H H H H H H H V-23 -4^Vch3 H H H H H H H H V.24 H H H H oo H H H H V-25 H H <y〇 H H H H H H V-26 ΟζΟ H H H H q-o H H H H V-27 H H qO H H H H qo H H V-28 H H Ph H Ph H H Ph H Ph V.29 H H Ph Ph H H H Ph Ph H (請先閱讀背面之注意事項再填寫本頁) -裝- 訂 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -279- 581751 A7 B7 五、發明説明（27》 M31
(請先閲讀背面之注意事項再填寫本頁) 經濟部智您財凌局員工消費合作社印製 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -280- 581751
A B 五、發明説明（27$ 經濟部智慧財/i局肖工消费合作社印¾ 化合物 No. m31 M32 M33 M34 M35 M41 M42 M43 M44 M 45 VI-1 Η Η Η Η Η Η H H H H VI-2 ch3 Η Η Η Η ch3 H H H H VI-3 t-C^Hg Η Η Η Η H H H H VI-4 OCH3 Η Η Η Η OCH3 H H H H VI-5 OPh Η Η Η Η OPh H H H H VI-6 N(C2H5)2 Η Η Η Η N(C2H5)2 H H H H VI-7 N(Ph)2 Η Η Η Η N(Ph)2 H H H H VI-8 Ph Η Η Η Η Ph H H H H VI-9 O-ch3 Η Η Η Η O~CH3 H H H H VI-10 H ch3 Η Η Η H ch3 H H H VI-11 H Η ch3 Η Η H H ch3 H H V1-12 H Η ch3 ch3 Η H H ch3 ch3 H VI-13 H Η ch3 Η ch3 H H ch3 H ch3 VI-14 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 ch3 VI-15 H Ph Η Η Η H Ph H H H VI-16 H Η Ph Η Η H H Ph H H VI-17 Η Η Η Η H H H H VI-18 t-C4Hg Η Η Η Η H H H H H VI-19 OP Η Η Η Η O9O H H H H VI-20 09 Η Η Η Η H H H H V1-21 Ph οφ λ—\ Η Η Η Η H H H H H VI-22 Η Η Η Η ch3 H H H H V1-23 -ο Η Η Η Η H H H H VI-24 N一 N Η Η Η Η N-N 々Ph H H H H VI-25 Η Η Ph Η Ph H H Ph H Ph VI-26 Η Η Ph Ph Η H H Ph Ph H VI-27 Η Η Η Η H H H H VI-28 Η Η Η Η H H H H (請先閱讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X 297公釐） -281 - 581751 A7 B7 五、發明説明（27今 m3
(請先閲讀背面之注意事項再填寫本頁) 經濟部智慧財凌局資工消費合作社印製 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -282- 581751 A7 B7 五、發明説明（2的 短濟部智慈財4^7資工消費合作社印^
化合物 No. m31 M32 m33 M3, m35 MA1 m,2 m43 Mi4 m45 VIM H H H H H H H H H H VII-2 ch3 H H H H ch3 H H H H VII-3 t*C4H9 H H H H t-C^Hg H H H H VII-4 och3 H H H H och3 H H H H VH-5 OPh H H H H OPh H H H H VII-6 N(C2H5)2 H H H H n(c2h5)2 H H H H VH-7 N(Ph)2 H H H H N(Ph)2 H H H H νΐΙ·8 Ph H H H H Ph H H H H VII-9 〇^ch3 H H H H ~hO^CH3 H H H H VII-IO H H ch3 ch3 H H H ch3 CI-I3 H VIM1 H H ch3 H ch3 H H ch3 H CH； VU-12 H ch3 丨H H H H ch3 H H H .13 H H ch3 H H H H ch3 H H VII-14 ch3 ch2 丨ch3 ch3 ch3 ch3 ch3 ch3 ch3 CH； VIM5 H H Ph H Ph H H Ph H Ph VH-16 H H Ph Ph H H H Ph Ph H VH-17 H H -O^Qh H H H -〇hQ H H YII-18 H H q-o H H H H H H (請先閲讀背面之注意事項再填寫本頁) 木紙張尺度適用中國國家標準（CNS ) A4規格（210X 297公釐） -283- 581751 A7 B7 五、發明説明（28)1 化合物 No. M31
M32 M33 M34 M35 M41 M42 M43 M44 M4S VII· 19 VII-20 VII-21
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VII-22 t-C4H9 H H H H H H H H H VII.23 "ΟΌ H H H H OQ H H H H VII-24 H H H H 〇 H H H H VII-25 N-N ΛλρΐΊ H H H H N-N 人>-Ph H H H H VII-26 ~^Vch3 H H H H —C^-CH3 H H H H \ \ 尸h VII-27 C=C / \ H H H H C=C / 、 H H H H Ph Ph Ph Ph VH-28 n-C4Hg H H H H n-C^Hg H H H H VII-29 H H 0CH3 H H H H 0CH3 H H
VII-30 H R32 L· R33 縮合環 H H H R42 R43 縮合々ytv環 H H VII-31 知 12 H H H H H H H H VII-32 hO^O H H H H H H H H H h〇hQ Η H H VII-33 H vii-34 VII-35 VH-36 YII-37
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H 〇〇 Η H Η Η Η H Η Η H H Ph H Ph H Ph Ph H (請先閲讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公漦） -284- 581751 A7 B7 五、發明説明（28会
經濟部智慧財凌笱資工消費合作社印製
化合物 No. Μη=Μ21 M12=M22 M13=M23 M14=M24 M15=M25 νιΐΓ-ι Η H H H H VIir-2 ch3 H H H H VIir-3 Η ch3 H H H νΐΙΓ·4 Η H ch3 H H νΐΙΓ-5 Ph H ch3 ch3 H νΐΙΓ-6 Η Ph H H H νΐΙΓ·7 Η H Ph H H νΐΙΓ-8 Η H Ph Ph H νΐΙΓ-9 Η H Ph H Ph viir-io Η H H H VIIM1 H H H H νΐΠ，·12 Η H 〇〇 H H νΐΙΓ-13 H H H H VHM4 N(Ph)2 H H H H νΊΙΓ-15 N(C2H5)2 H H H H νΐΙΓ-16 och3 H H H H VIII，· 17 Oph H H H H νΐΙΓ·18 H H H H ΥΙΙΓ·19 H H H H 請 閱 讀 背 冬
S 事 項 再 填 ί裝 頁 訂 線丨 本纸張尺度適用中國國家標準（CNS ) Α4規格（210X297公釐） -285- 581751 A7 B7 五、發明説明（2的 經濟部智慧財凌局員工消費合作社印製
(請先閱讀背面之注意事項再填寫本頁) 裝 ^ 訂 線
本紙張尺度適用中國國家標準（CNS ) A4規格（210X29*7公釐） -286- 581751 A7 B7 五、發明説明（28令 經濟部智慧財凌笱員工消費合作社印裂
批衣 „ 訂 線 (請先閱讀背面之注意事項再填寫本頁) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -287- 581751 A7 B7 五、發明説明（28今 IX -
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經濟部智慧財凌局g(工消費合作社印1i
(請先閱讀背面之注意事項再填寫本頁)
本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -288- 581751 經濟部智您財產局資工消贲合作社印製 A7 B7 五、發明説明（2β6)
本發明所使用之苯基蒽衍生物，係可以 (1 )鹵化二苯基蒽化合物係使用，與 Ni (cod)2〔cod:l，5 —環辛二烯〕偶合，或 將二鹵化芳基經格麗雅化形成N i C 1 2 ( d p p e )[ dppe:二苯基膦酸乙烷〕、NiCl2(dppp)〔 d ρ ρ p :二苯基膦酸丙烷〕等N i錯合物進行緊偶合之 方法； (2 )蒽醌、苯醌、蒽酮或聯二蒽酮與格麗雅化之芳 基或鋰化芳基反應與還原以產生緊偶合之方法； 等而製得。 依此方法所製得之化合物，可經由元素分析、質量分 析、紅外線吸收光譜、1 Η或1 3 C核磁共振光譜予以測定 〇 苯基蒽衍生物，係具有4 0 0至2 0 0 0左右，更佳 爲400至1000左右之分子量，具有200至500 t之高融點，並顯示出8 0至2 5 0 t、更佳爲1 0 0至 本纸乐尺度適用中國國家標率（CNS ) A4規格（210X297公釐） (請先閱讀背面之注意事項再填寫本頁)
-289- 581751 A7 ___B7_ 五、發明説明（287) 2 50°C、最佳爲1 30至250 °C、特佳爲1 50至 2 5 0 °C之玻璃移轉溫度（T g )。因此，以一般之真空 蒸鍍等方法可形成透明且於室溫以上亦呈現出安定之非晶 質狀態的平滑且良好之膜，此外，亦可長期間維持此良好 之膜狀態。 苯基蒽衍生物，因係爲比較趨近中性之化合物，故用 於發光層時會產生良好之效果。又，於考慮組合後之發光 層、電子注入層或正孔注入輸入層之載體移動度或載體密 度（係受離子化位能-電子親和力所決定）中，可對膜厚 度進行控制，進而可自由地設計再鍵結領域-發光領域， 而可對發光色之設計、因兩電極之繞射效果所產生之發光 亮度、發光光譜進行控制，或對發光空間之分布進行控制 (有機電致發光元件） 使用本發明化合物所製得之電致發光元件之構成例， 例如於基板上由依序設置正孔注入電極、正孔注入-輸送 層、發光與電子注入輸送層、電子注入電極等所構成。又 ，必要時於電子注入電極上可再設置補助電極或封閉層。 本發明之有機電致發光元件，並不僅限定於上記例示 ，其可具有各種構成內容，例如單獨設置發光層，並於此 發光層與電子注入電極間夾有電子注入輸送層之構造等。 又，必要時，可將正孔注入-輸送層與發光層混合亦可。 發光層之厚度、正孔注入輸送層之厚度與電子注入輸 本纸伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） ---------批衣----Ί--1T------^ (請先閲讀背面之注意事項再填寫本頁) -290· 581751 A7 B7 五、發明説明（2册） 送層之厚度並未有特別之限定，係依形成方法之不同而有 所改變，一般爲5至500nm左右，又以10至300 n m之範圍爲更佳。 正孔注入輸送層之厚度與電子注入輸送層之厚度，依 再鍵結-發光區域之設計，使其達與發光層相同厚度或 1/1 0至1 0倍左右亦可。若將正孔或電子之各注入層 與輸送層予以區分時，輸送層以1 nm以上爲佳。此時， 注入層、輸送層厚度之上限，一般而言，注入層爲5 0 0 nm左右，輸送層則爲5 0 0 nm左右。於此膜厚下，注 入輸送層若分爲2層時亦爲相同。 正孔注入層，係具有可使正孔注入電極容易地注入正 孔之機能、可將正孔安定地輸送之機能與妨礙電子之機能 ，電子注入輸送層係爲具有可由電子注入電極容易地注入 電子之機能、使電子安定地輸送之機能與妨礙正孔之機能 者，上述之各層可增大或封閉注入發光層之正孔或電子， 使再鍵結區域達最適當化，而改善發光效率。 又，正孔注入輸送層，例如本發明之化合物以外，亦 可使用特開昭6 3 - 2 9 5 6 9 5號公報、特開平2 -1 9 1 6 9 4號公報、特開平3 - 79 2號公報、特開平 5 - 23468 1號公報、特開平5 - 239455號公 報、特開平5 — 2 9 9 1 7 4號公報、特開平7 — 126225號公報、特開平7 - 126226號公報、 特開昭平8 — 1 00172號公報、EP0650955 A 1等所記載之各種有機化合物等。例如，四芳基聯苯胺 木纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） ---------裝-- (請先閱讀背面之注意事項再填寫本頁) 訂 線 經*部智^財^^7肖工消^合作社印% -291 - 經濟部智毯財/4苟資工消费合作社印製 581751 A7 B7 五、發明説明（心/\ 化合物（三芳基二胺至三苯基二胺：TPD)、芳香族三 級胺、腙、咔唑、三唑、咪唑、具有胺基之氧雜二唑衍生 物、聚噻吩等。此些化合物可將2種以上合倂使用，並用 時可與其他層層合，或混合皆可。 正孔注入輸送層分設爲正孔注入層與正孔輸送層時， 可由正孔注入輸送層之化合物中選擇較佳組合使用。此情 形中，以由正孔注入電極（I T 0等）側開始依離子化位 能較小之化合物層的順序依序層合較佳。又，正孔注入電 極表面以使用薄膜性良好之化合物爲佳。此層合順序，與 將正孔注入輸送層設計爲2層以上者爲相同。依此層合順 序，可降低驅動電壓，而防止泄電流或暗色斑點之發生或 生成。又，元件化時，即使用於蒸鎪之1至1 0 nm左右 之膜，亦可形成均勻且不會產生砂孔，故正孔注入層之離 子化位能較小，即使使用可視部分可吸收之化合物，亦可 防止發光色之色調變化或降低因再吸收所造成之效率降低 。正孔注入輸送層，可以與發光層相同般，以蒸鍍上記化 合物之方式形成。 又，電子注入輸送層，除本發明之化合物以外，尙可 使用三（8 -喹啉醇酯）鋁（A 1 Q3)等8 —喹啉醇或其 衍生物作爲配位基之有機金屬化合物等喹啉衍生物、氧雜 二唑衍生物、驼、芘、鸣喔啉、菲繞啉衍生物等含氮雜芳 香環族、二苯基醌衍生物、硝基取代芴衍生物等。電子注 入輸送層可兼具發光層者亦可，此時，以使用本發明之發 光層爲佳。電子注入層之形成方式可與發光層相同般使用 本紙張尺度適用中國國家標準（CNS ) A4洗格（210X297公釐） I I 批衣 訂 I I I I線 (請先閲讀背面之注意事項再填寫本頁) -292 - 581751 A7 _B7 _ __ 五、發明説明（巧'):. 蒸鍍方式製得。 電子注入輸送層將電子注入層與電子輸入層分別層合 時，可由電子注入輸送層之化合物中選擇較佳組合使用。 此情形中，以由電子注入電極（I T〇等）側開始依電子 親合力之値較大之化合物的順序依序層合較佳。此層合順 序，與將電子注入輸送層設計爲2層以上者爲相同。 正孔注入輸送層、發光層與電子注入輸送層之形成， 以使用可形成均質薄膜之真空蒸鍍法爲佳。使用真空蒸鍍 法時，可製得非晶質狀態或結晶粒徑爲0 · 1 // m以下之 均質薄膜。結晶粒徑超過0 · 1 /zm時，會產生不均勻之 發光，故而必須提高元件之驅動電壓，近而造成正孔之注 入效率顯著降低。 真空蒸鍍之條件並未有特別之限定，一般以 1 〇_4P a以下之真空度、蒸鍍速度爲〇 · 〇 1至1 nm /s e c左右爲佳。又，以於真空中連續形成各層者爲佳 。於真空中連續成型時，可防止各層之界面間吸附不純物 質，而可得到較高之性能。又，因可降低元件之驅動電壓 ，故可抑制暗色斑點之成長、生成。 使用蒸空蒸鍍法形成前述各層之情形中，其1層中含 有複數個化合物時，以對放置有各化合物之各個槽以分別 控制溫度方式進行共蒸鍍爲佳。
電子注入電極，較佳係由功函數爲4 e V以下之金屬 、合金或金屬間化合物所構成。功函數超過4 e V時，會 降低電子注入效率，進而降低發光效率。功函數爲4 e V 本纸伕尺度適用中國國家標準（CNS ) A4洗格（210X29*7公釐> ： -293 - I I I I I I I 訂— II !線 (請先閲讀背面之注意事項再填寫本頁) 581751 A7 __B7 五、發明説明（291) (請先閱讀背面之注意事項再填寫本頁) 以下之電子注入電極_的構成金屬，例如可爲L i 、Na 、K等鹼金屬，Mg、Ca、Sr、Ba等鹼土類金屬， La、Ce 等稀土類金屬或，A1 、i n、Ag、Sn、 Z η、Z r等。構成功函數4 e V以下之膜得構成合金例 如 Ag-Mg(Ag:〇.l 至 50at%) 、A1 —
Li (Li :〇·〇1 至 12at%)、In— Mg(
Mg : 50 至 8〇at% ) 、A1—Ca (Ca : 0 · 01至20a t% )等。其可單獨、或將2種以上組 合方式使用皆可’其2種以上組合之混合筆可爲任意之比 例。又，可將鹼金屬、鹼土類金屬、稀土類金屬之氧化物 或鹵化物形成薄膜，作爲鋁等之支撐電極（輔助電極、配 線電極等）亦可。 此電子注入電極可以蒸鍍法或濺鍍法等予以形成。 前述電子注入電極之厚度，只要具有可充分進行電子 注入之厚度皆可，即0 · 1 nm以上即可。又，其上限値 並未有特別之限定，一般之膜厚以0 . 1至5 0 0 nm左 右即可。 經濟部智慧財凌局肖工消費合作社印焚 正孔注入電極，較佳爲可使發光之光透過8 0%以上 之材料與厚度予以決定爲佳。具體而言，以氧化物透明導 電薄膜爲佳，例如錫摻雜氧化銦（I T〇）、鋅摻雜氧化 銦（IZO)、氧化銦（In2〇3)、氧化錫（Sn〇2 )與氧化鋅（Z nO )中任一者爲主成分皆可。前述氧化 物之化學量組成內容可有些許偏差亦可。對I n2〇3而言 ，Sn〇2之混合比以1至20質量％爲佳，又以5至1 2 本紙乐尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -294- 581751 A7 _________B7 _ 五、發明説明（292) 質量％爲更佳。對I η 2 〇 3而言，Z n 〇 2之混合比以 1 2至3 2質量％爲佳。 (請先閱讀背面之注意事項再填寫本頁) 正孔注入電極，其發光波長區域，一般爲3 5 0至 8 0 0 nm，特別是對各發光之光透過率爲8 〇%以上， 特別是9 0 %以上爲佳。一般，發光之亮光係透過正孔注 入電極而取出，故其透過率過低時，由發光層產生之亮光 本身會產生衰減，而會有未能得到發光元件所必須的亮度 之傾向。一般而言，取出亮光之發光側只要爲8 0 %以上 即可。 正孔注入電極之厚度，只要具有可充分進行正孔注入 之厚度即可，一般爲5 0至5 0 0 nm，又以5 0至 3 0 0 n m之範圍爲佳。又，其上限並未有任何限定，但 過厚時會有容易剝離之疑慮。厚度過薄時，於製造時容易 產生膜強度或正孔輸送力、電阻値等問題。 蛵濟部智慧財凌局員工消費合作社印¾ 將正孔注入電極成膜之方法例如可使用濺鎪法。濺鍍 法例如可使用R F電源以進行高周波濺鍍法等，但就考慮 成膜時正孔注入電極之膜物性的容易控制性或，成膜面之 平滑度等情形時，以使用D C濺鍍法爲佳。 又，必要時亦可形成保護膜。保護膜可使用S i Ox 等無機材料、鐵氟隆（登記商標）等有機材料予以成型。 保護膜可爲明或不透明者，保護膜之厚度一般爲5 0至 1 2 0 0 nm左右。保護膜除前記反應性濺鍍法外，例如 可使用一般之濺鏟法、蒸鍍法等予以成型皆可。 此外，爲防止元件之有機層或電極氧化，一般以於元 本纸伕尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -295- 581751 A7 ______B7_ 五、發明説明（293) (請先閱讀背面之注意事項再填寫本頁) 件上設置封鎖層爲佳。封鎖層，例如可使用防止濕氣侵入 而以使用市售低吸濕性光硬化黏著劑、環氧系黏著劑、聚 矽氧系黏著劑、交聯乙烯-乙酸乙酯共聚合物黏著劑薄片 等黏著劑樹脂層，將玻璃板等封鎖板黏著密封。玻璃板以 外亦可使用金屬板、塑膠板等。 基板材料，例如具有由基板側取出發光之亮光時，可 使用玻璃或石英、樹脂等透明或半透明之材料。又，基板 上可再含有包含色彩過濾膜或螢光性物質之色彩變換膜、 或使用電介質反射膜對發光色進行控制亦可。又，前記逆 層合中，基板可爲透明或不透明者，爲不透明時可使用陶 瓷等材料。 彩色過濾膜例如可使用用於液晶顯示器等彩色過濾膜 即可’只要其可配合有機電致發光所發出之亮光而可調整 彩色之特性，而使取出之效率-色彩純度最適當化即可。 又，有機電致發光元件材料或螢光變換層若使用可切 斷光吸收之短波長以外之光的彩色過濾膜時，可提高元件 之耐光性、顯示之色差對比等。 經濟部智慧財凌局資工消費合作钍印災 又，亦可使用介電體多層膜等光學薄膜以替代彩色過 濾膜。 本發明之有機電致發光元件，例如圖1所示般，係具 有於基板1上依序層合正孔注入電極（陽極）2、正孔注 入輸送層3、發光層4、電子注入輸送層5、電子注入電 極（陰極）6等構成者。又，與此層合順序相反之構成亦 可，或省略正孔注入輸送層3、電子注入輸送層5，或間 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） — 一 " -296- 581751 A7 B7 五、發明説明（294) 用發光層4亦可。其可配合所需要之元件機能而對構成層 作最適當之調整。 (請先閱讀背面之注意事項再填寫本頁) 本發明之有機電致發光元件一般係作爲直流驅動型、 脈衝驅動型之電致發光元件使用，但亦可作爲交流驅動使 用。附加電壓，一般爲2至3 0V左右。 實施例 以下，將說明本發明之具體實施例與比較例，以對本 發明作更詳盡之說明。 (合成例1 ) 3-溴一7， 12二苯基并ik]熒蒽之合成 經濟部智慧財/i^gi消費合作社印¾ 將5g (18 . 5mmo 1)之二苯基異苯并呋喃與 4 · 3g (18 · 5mmo 1)之5 —溴厄萘置於甲苯中 ，於迴流溫度下攪拌2 4小時。將溶媒以減壓餾除後，使 其溶解於5 0 0 m 1乙酸中。於其中，再加入4 0%之溴 酸水溶液5 0 c m 3，並於8 0 °C下加熱1小時。冷卻至室 溫後，將沉澱物濾除，將甲苯、己烷之混合溶媒作爲萃取 溶媒並以矽膠柱狀色層分析法精製，得黃色3 -溴- 7， 12二苯基并〔k〕熒蒽7g。 (合成例2 ) 1 2二苯基并〔k ]熒蒽基—3 -硼酸之合成 將2 · 5g之3 -溴一 7，12二苯基并〔k〕熒蒽 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -297- 581751 A7 _B7________ 五、發明説明（295) (請先閲讀背面之注意事項再填寫本頁) 溶解於5 0 cm3之THF中，冷卻至一 4 0°C。於其中加 入庚基鋰之己烷溶液（1 · 5mo 1/1) 50cm3後反 應2小時。於其中再加入硼酸三乙酯1 · 5 g後反應1小 時。回復至室溫後，加入5 N之鹽酸水溶液1 5 cm3後， 以碳酸氫鈉中和。將T H F餾除後’將固型物濾除。過濾 物以蒸餾水洗淨後，以再沉澱方式精製’得2 g之硼酸。 (合成例3 ) 例示化合物A - 2之合成 將先前製得之硼酸2g (4 · 5mmo 1 )與p 一二 溴基苯0 · 33g (1 · 4mmo 1)溶解於50cm3之 二甲氧基乙烷中，並加熱至8 0°C。於其中加入蒸餾水 5 0 cm3與碳酸鈉1 0 g。再投入四—三苯基膦鋇（〇) 0 · 2 g 〇 經3小時沉澱後，回收目的物。精製方法係使用矽膠 柱狀色層分析法精製，得黃色結晶1 g。 所得化合物係使用質譜分析光譜、紅外線吸收光譜、 蛵濟部智慧財/i局員工消費合作社印製
N M R進行測定。 質譜分析光譜 m / e = 紅外線吸收光譜 圖 3 N M R 圖 4 坡璃移轉溫度 2 5 1 °C 883 (M+1) + 圖 2 (合成例4 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -298- 581751 A7 B7 五、發明説明（296) 例{示仆:合物V — 2之合成 (請先閲讀背面之注意事項再填寫本頁) 將先前製得之硼酸2g(4·5mmo1)與雙一p 一二溴基三苯基胺〇·56g(1·4mmo1)溶解於 5 0 cm3之二甲氧基乙烷中，並加熱至8 0°C。於其中加 入蒸餾水5 0 cm3與碳酸鈉1 〇 g。再投入四一三苯基膦 鋇（0 ) 0 · 2 g。 經3小時沉澱後，回收目的物。精製方法係使用矽膠 柱狀色層分析法精製，得黃色結晶1 g。 所得化合物係使用質譜分析光譜、紅外線吸收光譜、 N M R進行測定。 質譜分析光譜 m/e=1050(M+l)+ 例示化合物Z - 2之合成 於5 0 cm3之二甲苯中，將先前製得之3 -溴—7， 12二苯基并〔k〕熒蒽2g (4 · lmmo 1)與苯胺 0 · 13g (1 · 4mmo 1)溶解於其中’並加入三— 經濟部智慧財凌苟替工消費合作社印焚 二苄叉酮鋇（0) 0 · 2g與三一 t— 丁基膦0 · 5 cm3 後，於1 3 0 °C下反應1 2小時。 將沉澱後之目的物回收’以矽膠柱狀色層分析法精製 ，得黃色結晶1 g。 所得化合物係使用質譜分析光譜、紅外線吸收光譜、 N M R進行測定。 質譜分析光譜 m/e=898(M+l)+ 衣纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -299- 581751 A7 B7 五、發明説明（297) (實施例1 ) (請先閲讀背面之注意事項再填寫本頁) 於玻璃基板上，使用R F濺鍍法將I T 0透明電極薄 膜以1 0 0 nm厚度成膜。隨後於附有此I TO透明電極 之玻璃基板，使用中性洗劑、丙酮、乙醇等進行超音波洗 淨處理，將其由煮沸之乙醇中取出，使其乾燥。透明電極 表面以UV/Ο 3洗淨後，固定於真空蒸鎪裝置之基板座上 ，並將槽內減壓至lx 1 〇_4P a以下。 隨後於保持減壓狀態下，將具有下記構造之N，N ’ —二苯基一 N，N， 一雙〔N -（4 一甲基苯基）一 N — 苯基一（4一胺基苯基）〕一1，1’ —聯苯基一4， 4’ 一二胺以蒸鍍速度0.111111/86〇:蒸鍍1〇〇 n m厚度之膜，作爲正孔注入層。
經濟部智楚財產局3(工消黃合作社印焚 隨後，將下記構造之N，N，NT ，N，—四（m -聯苯基）—1 ，1’ 一聯苯基—4，4， 一二胺以蒸鍍速 度0 · 1 nm/s e c蒸鍍1 〇nm厚度之膜，作爲正孔 輸送層。 ^纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） ' -300- 581751 A7 B7 五、發明説明（298)
隨後，於保持減壓下，將下記構造之蒽系主體材料與 ，本發明化合物（A — 2 )之摻雜劑，於質量比9 8 : 2 之比例下，以全體蒸鍍速度爲0 . 1 n m/ s e c蒸鍍 4 0 nm之厚度，以作爲發光層。 (請先閱讀背面之注意事項再填寫本頁)
經濟部智慧財/4笱2:工消費合作社印製 隨後，於保持減壓狀態下，將三（8 -羥基喹啉）銘 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -301 - 581751 A7 _______B7_ 五、發明説明Gfp. (A 1 Q3)以蒸鍍速度ο · i nm/s e c蒸鍍厚度1 5 n m之膜，以作爲電子注入輸送層。 (請先閱讀背面之注意事項再填寫本頁) 其次，將L i F以蒸鍍速度〇 · 1 n m / s e c蒸鍍 0 · 5nm之厚度，作爲電子注入電極，保護電極則使用 A 1蒸鍍1 〇 〇 n m，最後使用玻璃予以封鎖而製得有機 電致發光元件。 對此有機電致發光元件施加直流電壓，初期爲1 〇 mA/cm2之電流密度，驅動電壓爲8·6V，確認出其 具有7 3 0 c d/m2以上之發光。此時之波峰波長爲 450nm，色度座標（x，y) = (〇. 15， 0 · 1 1)。此元件，於流有l〇mA/cm2之一定電流 ，並連續驅動結果，其初期之亮度爲7 3 0 c d/m 2以上 ，亮度半衰期爲5 0 0小時以上。因此，亮度c d X半衰 期時間h爲36 5000。圖5即爲發光光譜。 (實施例2 ) 經濟部智慧財產局❺工消贲合作社印災 於實施例1中，將Ν，Ν·—二苯基一 Ν，Ν’ -雙 〔Ν - (4 -甲基苯基）一 Ν -苯基—（4 一胺基苯基） 〕一1，1’ 一聯苯基一4，4’ 一二胺以蒸鍍速度 〇· 1 nm/s e c蒸鍍50nm厚度之膜，作爲正孔注 入層。 隨後，將N，N，N， ，N’ 一四（m —聯苯基）一 1 ，1’ —聯苯基—4，4’ —二胺作爲主體材料與，本 發明化合物（A - 2 )之摻雜劑，於質量比9 8 : 2之比 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） ^ -302 - 581751 A7 B7 五、發明説明 例下，以全體蒸鍍速度爲0 · 1 nm/s e c下蒸鍍40 n m之厚度，以作爲正孔輸送層兼發光層。 (請先閲讀背面之注意事項再填寫本頁) 隨後，於保持減壓狀態下，將三（8 -羥基喹啉）鋁 (A 1 Q3)以蒸鍍速度〇 · 1 nm/s e c蒸鍍厚度40 n m之膜，以作爲電子注入輸送層。 其次，將L i F以蒸鍍速度〇 . 1 nm/s e c蒸鍍 0 · 3 nm之厚度，作爲電子注入電極，保護電極則使用 A 1蒸鍍2 0 0 n m，最後使用玻璃予以封鎖而製得有機 電致發光元件。 對此有機電致發光元件施加直流電壓，初期爲1 0 m A / c m 2之電流密度，驅動電壓爲7 · 9 V，確認出其 具有7 8 0 c d/m2以上之發光。此時之波峰波長爲 45〇nm，色度座標（X，y) = (〇 . 15， 0 · 1 1 )。此元件，於流有1 0 m A / c m 2之一定電流 ，並連續驅動結果，其初期之亮度爲7 8 0 c d/m 2以上 ，壳度半哀期爲4 0 0小時以上。 經濟部智慧財4^吕：工消費合作社印^ (實施例3 ) 於實施例1中，將Ν，Ν· -二苯基一 Ν，Ν’ 一雙 〔N — C 4 —甲基苯基）一 Ν —苯基—（4 一胺基苯基） 〕—1，1’ 一聯苯基—4，4’ —二胺以蒸鍍速度 0 · lnm/sec蒸鍍50nm厚度之膜，作爲正孔注 入層。 隨後，將N，N，N’ ，N’ 一四（m-聯苯基）— 本紙張尺度適用中國國家標準（CNS〉八4規格（210X29*7公釐） -303 - 581751 A 7 ____B7_ 五、發明説明（3〇1) 1’1’ 一聯苯基一4，4’ —二胺以蒸鍍速度0.1 nm/s e ◦蒸鍍2 0 nm厚度之膜，作爲正孔輸送層。 (請先閱讀背面之注意事項再填寫本頁} _後，於保持減壓下，將實施例1之本發明化合物（ A — 2 )作爲主體材料，與具有下記構造之并四苯系化合 物之摻雜劑，於質量比9 8 : 2之比例下，以全體蒸鍍速 度爲〇 · 1 nm/s e c下蒸鍍40nm之厚度以作爲發 光層。
經濟部智慧財凌局肖工消費合作社印紫 隨後，於保持減壓狀態下，將三（8 -羥基喹啉）鋁 (A 1 q3)以蒸鍍速度〇 · 1 nm/s e c蒸鍍厚度30 n m之膜，以作爲電子注入輸送層。 其次，將L i F以蒸鍍速度〇 . 1 n m / s e c蒸鍍 0 · 3 n m之厚度，作爲電子注入電極，保護電極則使用 A 1蒸鍍1 5 0 n m，最後使用坡璃予以封鎖而製得有機 電致發光元件。 對所製得之有機電致發光元件施加直流電壓，初期爲 1 0 m A / c m 2之電流密度，驅動電壓爲6 · 3 V，確認 本紙張尺度適用中國國家標準（CN’S ) A4規格（210X297公釐） -304- 581751 A7 B7 五、發明説明（302) 出其具有9 0 〇 c d/m2以上之發光。此時之波峰波長爲 560nm，色度座標（x，y) = (〇 . 45， (請先閱讀背面之注意事項再填寫本頁) 〇 · 55)。此元件，於流有lOmA/cm2之一定電流 ’並連續驅動結果，其初期之亮度爲9 0 0 c d/m2以上 ，亮度半衰期爲3 0 0 0小時以上。 (實施例4 ) 於實施例3中，除發光層之摻雜劑使用具有下記構造 之并四苯系化合物替代以外，其他皆依實施例3相同方法 製得有機電致發光元件。
經濟部智慧財/i^Jg(工消費合作社印製 對所製得之有機電致發光元件施加直流電壓，初期爲 10mA/cm2之電流密度，驅動電壓爲6 · 3V，確認 出其具有9 1 0 c d/m2以上之發光。此時之波峰波長爲 本紙伕尺度適用中國國家標準（CN’S ) A4規格（210X29*7公釐） -305- 581751 經濟部智慧財4^轉工消費合作社印製
A7 B7 五、發明説明（303) 560nm，色度座標（X，y) = (〇 . 45， 0 · 55)。此元件，於流有10mA/Cm2之〜定電流 ，並連續驅動結果，其初期之亮度爲9 1 〇 c d / 〇 hl μ ’ ΓΠ 以上 ，亮度半衰期爲3 0 0 0小時以上。 (實施例5 ) 於實施例3中，除發光層之摻雜劑使用具有T q ^ 之化合物替代以外，其他皆依實施例3相同方丨去_ # @ 電致發光元件。 對所製得之有機電致發光元件施加直流電壓，初_ m 1 0 m A / c m 2之電流密度，驅動電壓爲6 · 5 V，確認 出其具有7 5 0 c d/m2以上之發光。此時之波峰波長爲 580nm，色度座標（X，y) = (0 . 52， 0.48)。此元件，於流有l〇mA/cm2之〜定電流 ，並連續驅動結果，其初期之亮度爲了 5 0 c d/m2以上 ，亮度半衰期爲3 0 0 0小時以上。 本紙張尺度適用中國國家標準（CNS〉A4規格（210X 297公釐） 衣----；----IT------ (請先閱讀背面之注意事項再填寫本頁) •306- 581751 A7 B7 五、發明説明（3〇4) C實施例6 ) (請先閱讀背面之注意事項再填寫本頁} 於實施例3中，除發光層之摻雜劑使用下記構造之化 合物替代以外’其他皆依實施例3相同方法製得有機電致 發光元件。
對所製得之有機電致發光元件施加直流電壓，初期爲 1 〇 m A / c m 2之電流密度，驅動電壓爲6 · 6 v，確認 出其具有1 1 〇 〇 c d/m2以上之發光。此時之波峰波長 爲 515nm，色度座標（X，y) = (〇 · 30， 經濟部智慧財產苟肖工消費合作社印製 〇·65)。此元件，於流有l〇mA/cm2之一定電流 ，並連續驅動結果，其初期之亮度爲1 1 〇 〇 c d/m2以 上’亮度半衰期爲3 0 0 〇小時以上。 (實施例7 ) 於實施例3中，除摻雜劑使用下記構造之化合物替代 以外’其他皆依實施例3相同方法製得有機電致發光元件 本紙乐尺度適用中國國家標準（（：^5)八4規格（210/ 297公釐） -307- 581751 A7 B7 五、發明説明（305)
(請先閲讀背面之注意事項再填寫本頁) 對所製得之有機電致發光元件施加直流電壓，初期爲 1 0mA/cm2之電流密度，驅動電壓爲6 · 5V，確認 出其具有5 5 0 c d/m2以上之發光。此時之波峰波長爲 6 10nm，色度座標（X，y) = (〇 · 65， 0 · 3 5 )。此元件，於流有1 0 m A / c m 2之一定電流 ’並連續驅動結果，其初期之亮度爲5 5 0 c d/m2以上 ，亮度半衰期爲5 0 0 0小時以上。 (實施例8 ) 經濟部智慈財凌局貝工消費合作钍印^ 於實施例1中，將Ν，Ν’ 一二苯基一 Ν，Ν，—雙 〔Ν — (4 —甲基苯基）—Ν —苯基一（4 —胺基苯基） 〕一1，1’ 一聯苯基—4，4，一二胺以蒸鍍速度 〇· 1 nm/s e c蒸鍍50nm厚度之膜，作爲正孔注 入層。 隨後，將N’N，N， ，N，—四（m —聯苯基）— 1，1’ —聯苯基—4，4’ 一二胺以蒸鍍速度〇.1 nm/s e c蒸鍍2 0 nm厚度之膜，作爲第1正孔輸送 f^· 0 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） •308- 581751 A7 B7 五、發明説明（306) 隨後，於保持減壓下，將實施例1之本發明化合物（ A— 2)以蒸鍍速度0 . 1 nm/s e c蒸鍍1 〇nm之 厚度，作爲第2正孔輸送層。 隨後，將具有下記構造之化合物作爲主體材料，
以具有下記構造之化合物作爲摻雜劑，於質量比9 8 :2之比例下，以全體蒸鍍速度爲〇 · 1 n m / s e c下 蒸鍍4 0 nm之厚度以作爲發光層。 (請先閲讀背面之注意事項再填寫本頁) 經濟部智慧財/|^7資工消費合作钍印製
隨後，於保持減壓狀態下，將三（8 -羥基喹啉）鋁 (A1Q3)以蒸鍍速度〇 · lnm/sec蒸鍍厚度 3 0 nm之膜，以作爲電子注入輸送層。 其次，將L i F以蒸鍍速度〇 · 1 nm/s e c蒸鍍 0 · 3 n m之厚度，作爲電子注入電極，保護電極則使用 訂 L·, 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -309- 581751 A7 ____B7 五、發明説明（3〇7) A 1蒸鍍1 5 0 n m，最後使用玻璃予以封鎖而製得有機 電致發光元件。 (請先閱讀背面之注意事項再填寫本頁) 對所製得之有機電致發光元件施加直流電壓，初期爲 1 OmA/cm2之電流密度，驅動電壓爲6 . 〇v，確認 出其具有8 2 0 c d/m2以上之發光。此時之波峰波長爲 556nm，色度座標（X，y) = (〇 . 45， 0.55) ° (實施例9 ) 於實施例1中，將Ν，Ν’ 一二苯基—Ν，Ν，—雙 〔Ν — (4 -甲基苯基）一 Ν —苯基一（4-胺基苯基） 〕一1，1’ —聯苯基—4，4’ -二胺以蒸鍍速度 0 · 1 nm/s e c蒸鍍90nm厚度之膜，作爲正孔注 入層。 隨後，將N，N，N’ ，N’ —四（m —聯苯基）一 1，1’ —聯苯基—4，4’ —二胺以蒸鍍速度0·1 nm/s e c蒸鍍1 〇 nm厚度之膜，作爲正孔輸送層。 經濟部智慧財/1场3(工消費合作社印災 隨後，於保持減壓下，將本發明之化合物（A - 2 ) 以蒸鍍速度0 · 1 nm/s e c蒸鍍1 Onm之厚度，作 爲第2正孔輸送層。 隨後，將實施例8之化合物作爲主體材料，將本發明 之化合物（A - 2 )作爲摻雜劑，於質量比9 8 : 2之比 例下，以全體蒸鍍速度爲0 . 1 nm/s e c下蒸鍍40 n m之厚度以作爲發光層。 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -310· 581751 A7 B7 五、發明説明（308) (請先閱讀背面之注意事項再填寫本頁) 隨後，於保持減壓狀態下，將三（8 -羥基D奎啉）絕 (A1 Q3)以蒸鍍速度〇 · Inm/ s e c蒸鍍厚度 1 5 nm之膜，以作爲電子注入輸送層。 其次，將L i F以蒸鍍速度〇 · 1 nrn/s e c蒸鍍 〇 . 5 nm之厚度，作爲電子注入電極，保護電極則使用 A 1蒸鍍1 0 0 n m，最後使用玻璃予以封鎖而製得有機 電致發光元件。 對所製得之有機電致發光元件施加直流電壓，初期爲 10mA/cm2之電流密度，驅動電壓爲8 · 0V，確認 出其具有7 0 0 c d/m2以上之發光。此時之波峰波長爲 450nm，色度座標（X，y) = (0 · 15， 0.11)。 此元件，於流有1 0 m A / c m 2之一定電流，並連續 驅動結果，其初期之亮度爲7 0 0 c d /m 2以上，亮度半 衰期爲1 0 0 0小時以上。 C實施例1 0 ) 經濟部智慧財4局員工消費合作社印災 於實施例1中，將Ν，Ν’ —二苯基—Ν，Ν，—雙 〔Ν — (4 —甲基苯基）一 Ν -苯基—（4 一胺基苯基） 〕一1，1，—聯苯基一4，4’ 一二胺以蒸鍍速度 0 · 1 n m / s e c蒸鍍1 0 n m厚度之膜，作爲正孔注 入層。 隨後，將Ν，Ν，Ν· ，Ν’ 一四（m —聯苯基）— 1，1，—聯苯基—4，4’ 一二胺以蒸鍍速度〇 . 1 本纸張尺度適用中國國家標準（CNS ) A4規格（210X 297公釐） -311 - 581751 A7 B7 經濟部智慧財/t^7員工消費合作社印¾ 五、發明説明（31〇) (實施例1 1 ) 於實施例1中，除發光層之慘雜劑使用下記構造（ τ y P e B B B - 9 )之化合物替代以外，其他皆依， 施例1相同方法製得有機電致發光元件。
對此有機電致發光元件施加直流電壓，初期爲1 〇 m A / c m 2之電流密度’驅動電壓爲8 · 6 v，確認出其 具有8 0 0 c d/m2以上之發光。此時之波峰波長爲 452nm，色度座標（X，y) = (〇 . 15， 0.11)。 此元件，於流有1 OmA/cm2之一定電流，並連續 驅動結果，其初期之亮度爲8 〇 〇 c d /m 2以上，亮度半 衰期爲1 2 0 0小時以上。因此，亮度c d X半衰期時間 爲960000。圖6爲發光之光譜。 (實施例1 2 ) 於實施例1中，除發光層之摻雜劑使用下記構造（ Tvpe V - 2 )之化合物替代以外，其他皆依實施例 本紙張尺度適用中國國家標準（CNS ) A4規格（210X 297公釐） --------0^----r--IT------· (請先閱讀背面之注意事項再填寫本頁) -313- 581751 A7 B7
五、發明説明（311) 1相同方法製得有機電致發光元件 Q
對此有機電致發光元件施加直流電壓’初期爲1 0 mA/cm2之電流密度，驅動電壓爲8 · 6V，確認出其 具有9 0 0 c d/m2以上之發光。此時之波峰波長爲 473nm，色度座標（X，y) = (0 · 14， 0.27) ° 此元件，於流有5 0 m A / c m 2之一定電流，並連續 驅動結果，其初期之売度爲4 5 0 0 c d / in2以上，亮度 半衰期爲5 0 0小時以上。因此，亮度c dx半衰期時間 爲22500000。圖7爲發光之光譜。 衣-- (請先閲讀背面之注意事項再填寫本頁) 、-卩 經濟部智慧財凌局：^工消費合作钍印災 (實施例1 3 ) 於實施例1中，除發光層之摻雜劑使用下& Type Z — 2 )之化合物替代以外，其 1相同方法製得有機電致發光元件。 他皆依實施例
-314- 581751 A7 B7 五、發明説明（312) (請先閱讀背面之注意事項再填寫本頁) 對此有機電致發光元件施加直流電壓，初期爲1 〇 mA/cm2之電流密度，驅動電壓爲8 _ 6V，確認出其 具有1 1 0 0 c d/m2以上之發光。此時之波峰波長爲 518nm，色度座標（X，y) = (〇 . 28， 0.61) ° 此元件，於流有5 0 m A / c m 2之一定電流，並連續 驅動結果，其初期之亮度爲5 5 0 0 c d/m2以上，亮度 半衰期爲5 0 0小時以上。因此，亮度c d X半衰期時間 爲27500000。圖8爲發光之光譜。 (比較例1 ) 於實施例1中，除發光層不使用摻雜劑摻雜以外，其 他皆依實施例1相同方法製得有機電致發光元件。 對此有機電致發光元件施加直流電壓，初期爲1 0 m A / c m 2之電流密度，驅動電壓爲6 · 5 V，確認出其 爲1 8 0 0 c d/m2以下之發光。此時之波峰波長爲 440nm，色度座標（x，y) = (〇· 16， 經濟部智慧財產笱資工消費合作社印製 0.07)。此元件，於流有1 0 m A / c m 2之一定電流 ，並連續驅動結果，其初期之亮度爲1 8 0 c d/m2，亮 度半衰期爲2 5 0小時以下。因此，亮度c d X半衰期時 間爲4 5 0 0。基於此實驗，實施例1之元件較比較例1 之元件具有4倍以上之發光亮度，且在同一發光亮度下具 有8倍以上之壽命。 本紙張尺度適用中國國家標率（CNS ) A4規格（210X29*7公釐） -315· 581751 經濟部智慧財凌局貨工消費合作社印紫 A7 B7 五、發明説明（313) C比較例2 ) 於實施例i中’除發光層之摻雜劑使用下記構造之化 合物替代以外，其他皆依實施例1相同方法製得有機電致 發光元件。
對此有機電致發光元件施加直流電壓，初期爲1 〇 mA/cm2之電流密度，驅動電壓爲6 . 6V，確認出其 具有7 0 0 c d/m2之發光。此時之波峰波長爲4 6 5 11!11，色度座標（\，7) = (〇.2〇，〇.2〇·)， 且具有由藍色偏向長波長側之發光色。此元件，於流有 1 OmA / cm2之一定電流，並連續驅動結果，其初期之 売度爲7 0 0 c d/m2，売度半孩期爲5 0 〇小時。 (比較例3 ) 於實施例1中，除發光層之摻雜劑使用下記構造之化 合物替代以外，其他皆依實施例1相同方法製得有機電致 發光元件。 本紙張尺度適用中國國家標準（CNS ) A4規格（210x 297公廣） .0^----r--1T------·· (請先閱讀背面之注意事項再填寫本頁) -316- 581751 A7 ________ B7 五、發明説明（314)
(請先閱讀背面之注意事項再填寫本頁) 對此有機電致發光元件施加直流電壓，初期爲1 〇 mA/cm2之電流密度，驅動電壓爲6 · 5V，確認出其 具有1 8 0 c d/m2之發光。此時之波峰波長爲4 4 〇 11111，色度座標（\，7) = (〇.16，〇.〇7)。 此元件，於流有1 〇 m A / c m 2之一定電流，並連續驅動 結果’其初期之亮度爲1 8 0 c d/m2，亮度半衰期爲 2 5 0小時。 【發明之效果】 經濟部智慧財/i^7s工消費合作社印焚 基於以上發明之說明，本發明係提供一種具有充分亮 度之發光’特別是可得到長波長之亮光，具有優良之色彩 純度’特別是用於彩色顯示器時可得到充分之色彩純度， 且具有良好發光性能，並經長期使用亦具有優良耐久性之 有機電致發光元件用化合物，及有機電致發光元件。 本纸張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） -317-

Claims (1)

  1. 581751 ABCD 六、申請專利範圍 第9 1 1 08294號專利申請案 中文申請專利範圍修正本 民國92年7月4日修正 1、一種有機電致發光元件用化合物，其係具有下式 (1)所示之基本骨架； Χη-γ …（1) 〔式（1 )中，X爲下記式（2 )所示化合物，其可 爲相同或不同；Υ爲單鍵或爲經取代或未取代之芳基、或 由雜環基所形成之連結基，但Υ於R 7與R 7、R 8與R. 8或 R 7與R 8位置之組合中進行鍵結時，不含單鍵鍵結，ια爲 2或3之整數〕 (請先閲讀背面之注意事項再填寫本頁) ·?·%>’
    Ra R? 經濟部智慧財產局員工消費合作社印製 合物 X 〔式（2)中，Ri至R8與a至d爲氫、院基、可具有取 代基之芳基、可具有取代基之烯丙基、可具有取代基之雜 環基、胺基、或可具有取代基之芳基胺基之任一者]。 2、如申請專利範圍第1項之有機電致發光元件用化 其中，前記Y係由下記化合物所選出之任一種； 本紙張尺度適用中國國家標準（CNS ) A4規格（210X：297公釐） 581751 Α8 Β8 C8 D8 申μ專利範圍
    .Ν. 經濟部智慧財產局員工消費合作社印製 3、如申請專利範圍第1 項 之 有 機 電 致 發 光 元 件 用 化 合物 ，其中，ΓΙ爲2。 合物 4、如申請專利範圍第1 項 之 有 機 電 致 發 光 元 件 用 化 ’其係作爲摻雜劑。 合物 5、如申請專利範圍第1 項 之 有 機 電 致 發 光 元 件 用 化 ’其係爲電子輸送材料。 6、如申請專利範圍第1 項 之 有 機 電 致 發 光 元 件 用 化 合物 ’其係爲正孔注入或輸送材料。 7、如申請專利範圍第1 項 之 有 機 電 致 發 光 元 件 用 化 合物，其係具有下記式 所示基本骨架； ci di
    R丨4 R丨3 (3a) 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） _ 2 _ (請先閲讀背面之注意事項再填寫本頁)
    581751 A8 B8 C8 D8 &、申請專利範圍 〔式（3a)中，1^至1^7與31至31、Rh至 R】7與a 2至（12爲氫、烷基、可具有取代基之芳基、可具 有取代基之烯丙基、可具有取代基之雜環基、胺基、或可 胃有取代基之芳基胺基之任一者，Y爲取代或未取代之伸 苯基、伸聯苯基、并四苯基、茈、芘、菲、噻吩、吡啶、 卩比嗪、三嗉、胺、三芳基胺、吡咯衍生物、噻唑、噻二唑 、菲繞啉、喹啉、喹喔啉中任一所形成之連結基〕。 8、如申請專利範圍第1項之有機電致發光元件用化 合物，其係具有下記式（3 b )所示基本骨架； n r> h ai Rs R) (3b) (請先閱讀背面之注意事項再填寫本頁)
    訂 〔式（3b)中，尺1至尺8與31至（1 R 經濟部智慧財產局員工消費合作社印製 R 與 至d 2爲氫、烷基 至 、可具有取代基之芳基、可具 有取代基之烯丙基、可具有取代基之雜環基、胺g、 或可 具有取代基之芳基胺基之任一者，Y爲單鍵、取代^ $ 代之芳基、或由雜環所形成之連結基，但Y於R 7 _ R R 8與R 8或R 7與R 8位置之組合中進行鍵結時，$ $ 鍵結〕。 單鍵 本紙張尺度適用中國國家標準（CNS ) A4規格（210 X 297公釐） -3 - 581751 A8 B8 C8 D8 六、申請專利範圍 9、如申I靑專利範S桌1項之有機電致發光元件用化 合物，其係具有下記式（3 c )所示基本骨架；
    〔式（3c)中，1^至1^8 與 31至01、1^1至 Rl8與a 2至d 2爲氫、烷基、可具有取代基之芳基、可具 有取代基之烯丙基、可具有取代基之雜環基、胺基、^ $ 具有取代基之芳基胺基之任一者，Y爲單鍵、取代 代之芳基、或由雜環所形成之連結基，但Y於R 7與R 7、 R 8與R 8或R 7與R 8位置之組合中進行鍵結時，不含單鍵 鍵結〕。 1 〇、如申請專利範圍第1項之有機電致發光元件 化合物，其係具有下記式（A )所不基本骨架；
    〔式（A)中，R]至R7與尺“至尺^爲氫、院基 (請先閱讀背面之注意事項再填寫本頁}
    經濟部智慧財產局員工消費合作社印製 本紙張尺度適用中國國家標準（CNS ) A4規格（21〇X：297公釐） -4
    、'申請專利範圍 耳又代或未取代之芳基、或雜環基〕。 1 1 、如申請專利範圍第1項之有機電致發光元件用 t Θ % ’其係具有下記式（B )所示基本骨架；
    R5 R 、取代 化合物 式（B)中，Ri至尺7與1111至R 或未取代之芳基、或雜環基〕。 2、如申請專利範圍第1項之有機電致發光元件用 ’其係具有下記式（E )所示基本骨架； 爲氫、烷基 (請先閲讀背面之注意事項再填寫本頁) 55 ri R2H(_)-R5 R3 R4 RJ4^13 r15/)-r12>Rn (E) 訂 、取代 化合物 經濟部智慧財產局員工消費合作社印製 Rl7R18 式（E)中，！^1至1^8與1^1】至1^】8爲氫、院基 或未取代之芳基、或雜環基〕。 3、如申請專利範圍第1項之有機電致發光元件用 ’其係具有下記式（H)所示基本骨架；
    、取代或未取代之芳基、或雜環基〕。 1 4、如申請專利範圍第1項之有機電致發光元件用 ^國家標準（CNS)八4雜（21()><297公董） 581751 A8 B8 C8 D8 ^'中請專利範圍 t &物，其係具有下記式（χ )所示基本骨架；
    (X) 〔式（X)中，尺1至118與Rh至R '耳5代或未取代之芳基、或雜環基〕。 爲氫、烷基 1 5、如申請專利範圍第1項之有機電致發光元件用 &合*物’其係具有下記式（Z )所示基本骨架；
    14 (Z) 至R 1 7爲氫、烷基 '取代或未取代之芳基、或雜環基〕。 1 6、如申請專利範圍第1項之有機電致發光元件用 化合物，其係具有下記式（A A A，）所示基本骨架； (請先聞讀背面之注意事項再填寫本頁) 經濟部智慧財產局員工消費合作社印製
    (MA·) 〔式（AAA，）中，Ri 至 Rs、與 Rii 至 Ri8 爲 氫、烷基、可具有取代基之芳基、可具有取代基之烯丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 本紙張尺度適用中國國家標準（CNS )八4規格（2丨0><297公釐） -6 - 581751 A8 B8 C8 D8 六、申請專利範圍 基之任一者〕。 1 7、如申請專利範圍第1項之有機電致發光元件用 化合物’其係具有下記式（B B B ’ ）所示基本骨架；
    (B巳巳’） (請先閲讀背面之注意事項再填寫本頁) 、與R 1 1至R 1 8爲 氫 '烷基 '可具有取代基之芳基、可具有取代基之烯丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 基之任一者〕。 1 8、如申請專利範圍第1項之有機電致發光元件用 化合物，其係具有下記式（C C C ’ ）所示基本骨架； 經濟部智慧財產局員工消費合作社印製
    與R 1 1至R 1 8爲 氫、烷基、可具有取代基之芳基、可具有取代基之烯丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 基之任一者〕。 1 9、如申請專利範圍第1項之有機電致發光元件用 化合物，其係具有下記式（D D D ’ ）所示基本骨架； 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） 581751
    經濟部智慧財產局員工消費合作社印製 A8 B8 C8 D8 申請專利範圍 (DDD·) 〔式（DDD，）中，1^至1^8、與只^至只"爲 氫、院基、可具有取代基之芳基、可具有取代基之嫌丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 基之任一者〕。 . 2 0、如申請專利範圍第1項之有機電致發光元件用 化合物，其係具有下記式（EEE’ ）所示基本骨架； (EEF) 〔式（EEE’ ）中，1^至118、與Rh至Rh爲 氫、烷基、可具有取代基之芳基、可具有取代基之烯丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 基之任一者〕。 2 1 、如申請專利範圍第1項之有機電致發光元件用 化合物’其係具有下記式（R R R ’ ）所示基本骨架； 本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） · 8 (請先閱讀背面之注意事項再填寫本頁)
    581751 A8 B8 C8 D8 六、申請專利範圍 經濟部智慧財產局員工消費合作社印製 _ R,16 ^15 (RRR·) 〔式（RRR’ ）中，尺1至尺7、與尺11至1117爲 氫、烷基、可具有取代基之芳基、可具有取代基之烯丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 基之任一者〕。 2 2、如申請專利範圍第1項之有機電致發光元件用 化合物，其係具有下記式（SSS’ ）所示基本骨架；. 〔式（SSS，）中，111至117、與爲 氫、烷基、可具有取代基之芳基、可具有取代基之烯丙基 、可具有取代基之雜環基、胺基、可具有取代基之芳基胺 基之任一者〕。 2 3、一種有機電致發光元件，其係於一對電極間至 少含有1種或2種以上與發光機能有關之有機層，其中至 少1層有機層係含有1種或2種以上申請專利範圍第1項 之有機電致發光元件用化合物。 2 4、如申請專利範圍第2 3項之有機電致發光元件 ’其中’除前記有機電致發光元件用化合物外，尙含有1 種或2種以上蒽系化合物。 2 5、如申請專利範圍第2 4項之有機電致發光元件
    本紙張尺度適用中國國家標準（CNS ) A4規格（210X297公釐） (請先閲讀背面之注意事項再填寫本頁) 581751 A8 B8 C8 ___D8 々、申請專利範圍 ，其中，前記葱系衍生物係作爲發光層之主體材料。 2 6、如申請專利範圍第2 3項之有機電致發光元件 ，其中，前記有機電致發光元件用化合物係以摻雜劑形式 含有。 2 7、如申請專利範圍第2 3項之有機電致發光元件 ，其中’前記有機電致發光元件用化合物係包含於發光層 中〇 2 8、如申請專利範圍第2 3項之有機電致發光元件 ，其中，前記有機電致發光元件用化合物係包含於電子輸 送層中。 2 9、如申請專利範圍第2 3項之有機電致發光元件 ，其中，前記有機電致發光元件用化合物係包含於正孔注 入輸送層中。 3 0、如申請專利範圍第2 3項之有機電致發光元件 ，其係具有由2種以上發光材料所形成之2種以上發光極 大波長者。 (請先閲讀背面之注意事項再填寫本頁) 經濟部智慧財產局員工消費合作社印製 本紙張尺度適用中國國家橾準（CNS ) A4規格（210X297公釐） -1〇 -
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EP1719748A2 (en) 2006-11-08
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