PL8909B1 - A method of recovering phosphorus and its hydrogen compounds in the form of phosphoric acid or phosphates. - Google Patents

A method of recovering phosphorus and its hydrogen compounds in the form of phosphoric acid or phosphates. Download PDF

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Publication number
PL8909B1
PL8909B1 PL8909A PL890927A PL8909B1 PL 8909 B1 PL8909 B1 PL 8909B1 PL 8909 A PL8909 A PL 8909A PL 890927 A PL890927 A PL 890927A PL 8909 B1 PL8909 B1 PL 8909B1
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PL
Poland
Prior art keywords
phosphorus
phosphoric acid
hydrogen compounds
tower
phosphates
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Application number
PL8909A
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Polish (pl)
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Publication of PL8909B1 publication Critical patent/PL8909B1/en

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Description

Wynalazek niniejszy dotyczy sposobu odzyskiwania fosforu lub jego zwiazków wodorowych w postaci kwasu fosforowego lub fosforanów i daje sie stosowac we wszelkich zakladach przemyslowych pro¬ dukujacych fosfor lub jego zwiazki wodo¬ rowe.Sposób ten polega na tern, ze fosfor spala sie powietrzem, a wytworzony bez¬ wodnik kwasu fosforowego nawadnia sie, przyczem cieplo wywiazane podczas spa¬ lania fosforu uzywa sie do stezania otrzy¬ manych roztworów kwasu fosforowego.Zasada sposobu oraz urzadzenia sluza¬ ce do jego przeprowadzania nie sa bynaj¬ mniej nowe, a istota wynalazku polega je¬ dynie na polaczeniu znanych juz urzadzen i na sposobie ich dzialania, co umozliwia calkowite odzyskanie fosforu i jego zwiaz¬ ków wodorowych w postaci stezonego kwa¬ su fosforowego lub fosforanów.Na zalaczonym rysunku przedstawiony jest przyklad wykonania niniejszego wy¬ nalazku.Fosfor spala sie w komorach 1 zaopa¬ trzonych w dajace sie regulowac otwory doprowadzajace powietrze. Temperatura gazów spalinowych wychodzacych z tych komór wynosi od 900° do 1100°C, zaleznie od ilosci powietrza, wprowadzonego do ko-mór/ przyczem cieplo spalania sluzy do podniesienia normalnej temperatury azo¬ tu i pozostalego tlenu do najwyzszej tem¬ peratury.Gazy powstale wskutek spalenia fosfo¬ ru wprowadza sie do dolnej czesci wiezy Gaillardla 2, gdzie wchodza one w zetknie¬ cie z roztworem kwasu fosforowego, który ma Byc stezony. Kwas ten o stezeniu 20° lub 22° Be wytryskuje ze zbiornika 3 do szczytu wiezy 2, w której opada w postaci bardzo drobnych kropelek.Wskutek zetkniecia sie wspomnianych gazów z roztworem nastepuje wymiana ciepla, a roztwór kwasu fosforowego kon¬ centruje sie tak, ze rurka 4 odplywa z dol¬ nej czesci wiezy 2 kwas fosforowy o ste¬ zeniu 50°Be.Gazy wznoszace sie w wiezy 2 zawiera¬ ja pare wodna, która nawadnia bezwod¬ nik kwasu fosforowego^ który wraca na¬ stepnie do wiezy 2 w postaci roztworów kwasu fosforowego o stezeniu 20° lub 22°Be.Gazy uchodzace z wiezy 2, o tempera¬ turze od 200° do 280°C, wchodza do pod¬ grzewacza 5, skladajacego sie z szeregu rurek zanurzonych w roztworze kwasu fo¬ sforowego, doplywajacego z komór kokso¬ wych 6.W aparacie tym nastepuje pierwsze stezanie kwasu, które podnosi sie od 17° do 20° i od 20° do 22° Be, poczem kwas ten wprowadza sie do wiezy Gaillard'a.Aby uniknac skroplenia pary wodnej, za¬ wartej w gazach, nalezy baczyc na to, aby temperatura roztworu kwasu wprowadza¬ nego do wiezy nie spadla ponizej 100° lub 120°C.Po przejsciu przez podgrzewacz gazy dostaja sie do komór 6, zawierajacych koks.Bezwodnik kwasu fosforowego w obecno¬ sci pary wodnej nawadnia sie, dajac kwas fosforowy, który gromadzi sie na dnie ko¬ mór 6, skad odplywa rurka 7.Podczas nawadniania bezwodnika fo¬ sforowego wywiazuja sie znaczne ilosci ciepla, wskutek czego moze zachodzic po¬ trzeba ochladzania komór 6, co przepro¬ wadza sie przez wtryskiwanie i do nich wody. W tym wypadku woda rozciencza kwas fosforowy, utworzony w komorach 6, i otrzymuje sie roztwór tego kwasu o stezeniu od 17° do 20°Be i o temperatu¬ rze od 50° do 70°C.Pozostala pare wodna lub azot i inne gazy odciaga sie przewodem 8 zapomoca odpowiednich dmuchaw i wprowadza do komina.Sposób niniejszy odznacza sie tern, ze uzywa sie jednej i tej samej ilosci wody, a mianowicie wprowadza sie ja do szczytu wiezy Gaillard'a w postaci roztworu kwa¬ su fosforowego o stezeniu 17°—20°Be, któ¬ ry wychodzi nastepnie z komór koksowych 6 w tern samem stezeniu.Woda wprowadzona do komór kokso¬ wych 6, celem ich ochlodzenia, sluzy do wyrównywania strat wspomnianej ilosci wody, której nadmiar usuwa sie z urza¬ dzenia w postaci pary. Przeprowadzajac sposób niniejszy, nalezy zapobiegac skra¬ planiu sie pary wodnej przed nawodnie¬ niem tlenowych zwiazków fosforu. PL PLThe present invention relates to a method of recovering phosphorus or its hydrogen compounds in the form of phosphoric acid or phosphates and is applicable to all industrial plants producing phosphorus or its hydrocarbons. The method consists in the fact that phosphorus is burned with air and produced without Phosphoric acid hydride is hydrated, while the heat generated during phosphorus combustion is used to concentrate the obtained phosphoric acid solutions. The principle of the method and the equipment used to carry it out are not at all new, and the essence of the invention lies solely in the combination of the devices already known and their mode of operation, which makes it possible to completely recover phosphorus and its hydrogen compounds in the form of concentrated phosphoric acid or phosphates. An example of the present invention is shown in the attached figure. Phosphorus is burnt in the chambers provided with adjustable air vents. The temperature of the flue gases leaving these chambers ranges from 900 ° to 1100 ° C, depending on the amount of air introduced into the chambers, while the combustion heat serves to raise the normal temperature of nitrogen and residual oxygen to the highest temperature. the phosphorus burns are introduced into the lower part of the Gaillardl tower 2 where they come into contact with the phosphoric acid solution to be concentrated. This acid, having a concentration of 20 ° or 22 ° Be, is sprayed from the tank 3 to the top of the tower 2, where it falls down in the form of very fine droplets. As the gases come into contact with the solution, heat exchange takes place, and the phosphoric acid solution concentrates so that tube 4 drains from the lower part of tower 2 phosphoric acid at 50 ° C. The gases rising in tower 2 contain water vapor which irrigates phosphoric acid anhydride which returns to tower 2 in the form of phosphoric acid solutions at a concentration of 20 ° or 22 ° C. Gases escaping from the tower 2, at a temperature of 200 ° to 280 ° C, enter the heater 5, consisting of a series of tubes immersed in a phosphoric acid solution, The first concentration of acid takes place in this apparatus, which rises from 17 ° to 20 ° and from 20 ° to 22 ° Be, then this acid is introduced into the Gaillard tower. To avoid condensation of water vapor contained in gases, care should be taken that the temperature of the solution is acidic When the gas passes through the preheater, it enters the chambers 6 containing the coke. Phosphoric acid anhydride in the presence of water vapor is hydrated to give phosphoric acid, which accumulates on the The bottom of the chambers 6, from where the tube 7 flows. When the phosphoric anhydride is irrigated, a considerable amount of heat is generated, which may result in the need for cooling the chambers 6 by spraying water into them. In this case, water dilutes the phosphoric acid formed in the chambers 6, and a solution of this acid is obtained with a concentration of 17 to 20 ° Be and a temperature of 50 to 70 ° C. The remaining water vapor or nitrogen and other gases are sucked off by means of appropriate blowers and introduced into the chimney. The present method is characterized by the fact that one and the same amount of water is used, namely, it is introduced to the top of the Gaillard tower in the form of a phosphoric acid solution of 17 ° -20 20 Be, which then emerges from the coke chambers 6 at the same concentration. The water introduced into the coke chambers 6 for cooling, serves to compensate for the loss of the aforementioned amount of water, the excess of which is removed from the device in the form of steam. In carrying out the present method, it is necessary to prevent condensation of the water vapor from hydrating the phosphorus oxygenates. PL PL

Claims (2)

1. Zastrzezenia patentowe. 1. Sposób odzyskiwania fosforu i je¬ go zwiazków wodorowych w postaci kwa¬ su fosforowego lub fosforanów, znamienny tern, ze gazy otrzymane przez spalanie fo¬ sforu wprowadza sie do dolnej czesci wie¬ zy Gaillard'a, gdzie wchodza w zetkniecie z roztworem kwasu fosforowego, który ste¬ zaja, przyczem roztwór ten ulega jeszcze pierwszej koncentracji w podgrzewaczu, wskutek zetkniecia sie ze strumieniem ga¬ zów, przechodzacych ze wspomnianej wie¬ zy do komór koksowych, w których nawad¬ nia sie bezwodnik kwasu fosforowego, da¬ jac kwas fosforowy. 1. Patent claims. 1. A method of recovering phosphorus and its hydrogen compounds in the form of phosphoric acid or phosphates, characterized by the fact that the gases obtained by burning phosphorus are introduced into the lower part of the Gaillard tower, where they come into contact with an acid solution which concentrates, while this solution is still first concentrated in the heater, as a result of contact with the stream of gases passing from the said tower to the coking chambers in which phosphoric anhydride is irrigated, giving acid phosphoric. 2. Sposób wedlug zastrz. 1, znamienny — 2 —tern, ze cieplo, wywiazane podczas spala¬ nia fosforu i jego zwiazków wodorowych sluzy do stezania otrzymanych roztworów kwasu fosforowego, przyczem woda odpa rowujaca z tych roztworów zuzywa sie po¬ nownie do nawodniania tlenowych zwiaz¬ ków fosforu, a ilosc wody krazacej utrzy¬ muje sie stala, przez regulowanie ilosci wody wprowadzanej do komór koksowych, celem ich chlodzenia, Urbain Corporation. Zastepca: Inz. S. Pawlikowski, rzecznik patentowy.Do opisu patentowego Nr 8909. Druk L. Boguslawskiego, Warszawa. B!E. PL PL2. The method according to claim 1, characterized by the fact that the heat generated during the combustion of phosphorus and its hydrogen compounds serves to concentrate the obtained phosphoric acid solutions, while the water evaporating from these solutions is used again to hydrate the oxygen compounds of phosphorus, and the amount of circulating water is kept constant by regulating the amount of water introduced into the coking chambers for cooling them, Urbain Corporation. Deputy: Inz. S. Pawlikowski, patent attorney. To the patent description No. 8909. Print by L. Boguslawski, Warsaw. B! E. PL PL
PL8909A 1927-04-20 A method of recovering phosphorus and its hydrogen compounds in the form of phosphoric acid or phosphates. PL8909B1 (en)

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