JP2016114011A - Exhaust emission control device - Google Patents

Exhaust emission control device Download PDF

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JP2016114011A
JP2016114011A JP2014255124A JP2014255124A JP2016114011A JP 2016114011 A JP2016114011 A JP 2016114011A JP 2014255124 A JP2014255124 A JP 2014255124A JP 2014255124 A JP2014255124 A JP 2014255124A JP 2016114011 A JP2016114011 A JP 2016114011A
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exhaust gas
reduction catalyst
catalyst
upstream side
selective reduction
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JP6500422B2 (en
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幸博 川島
Yukihiro Kawashima
幸博 川島
嘉久 植田
Yoshihisa Ueda
嘉久 植田
祥平 小椋
Shohei Ogura
祥平 小椋
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Isuzu Motors Ltd
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    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02A—TECHNOLOGIES FOR ADAPTATION TO CLIMATE CHANGE
    • Y02A50/00—TECHNOLOGIES FOR ADAPTATION TO CLIMATE CHANGE in human health protection, e.g. against extreme weather
    • Y02A50/20—Air quality improvement or preservation, e.g. vehicle emission control or emission reduction by using catalytic converters
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02T—CLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO TRANSPORTATION
    • Y02T10/00—Road transport of goods or passengers
    • Y02T10/10—Internal combustion engine [ICE] based vehicles
    • Y02T10/12—Improving ICE efficiencies

Abstract

PROBLEM TO BE SOLVED: To provide an exhaust emission control device including an oxidation catalyst, a PM collection filter and a selection reduction type catalyst, and capable of being arranged near a Diesel engine.SOLUTION: In an exhaust passage 1 of a Diesel engine, a storage container 2 and a casing 3 are interposed in order from an upstream side; in the storage container 2, a first DOC 6 and an SCR filter 7 comprising a PM collection filter to which a selective reduction type catalyst is applied are disposed separately from each other in order from the upstream side; in a flow passage of exhaust gas G between the first DOC 6 and the SCR filter 7, a urea water injector 9 is installed; and in the casing 3, an SCR 10 and a second DOC 11 are arranged in order from the upstream side.SELECTED DRAWING: Figure 1

Description

本発明は排ガス浄化装置に関し、更に詳しくは、酸化触媒、ＰＭ捕集フィルター及び選択還元型触媒を備えるとともに、ディーゼルエンジンに対する近接配置を可能にした排ガス浄化装置に関する。   The present invention relates to an exhaust gas purification device, and more particularly to an exhaust gas purification device that includes an oxidation catalyst, a PM trapping filter, and a selective reduction catalyst, and that can be disposed close to a diesel engine.

大型車のディーゼルエンジンに係るポスト新長期規制（ＰＮＬＴ）を達成するために、酸化触媒（ＤＯＣ）、酸化機能を有するＰＭ捕集フィルター（ＣＳＦ）、選択還元型触媒（ＳＣＲ）及びアンモニアスリップＤＯＣを備えた排ガス浄化装置が採用されている（例えば、特許文献１を参照）。しかし、次期ＰＮＬＴやＥｕｒｏ６排出ガス規制では、排ガス規制が強化されるとともに、重量車排出ガス試験法（ＷＨＤＣ）が採用されるため、排ガス浄化装置の更なる改良が必要となっている。   In order to achieve post-new long-term regulations (PNLT) for diesel engines of large vehicles, oxidation catalyst (DOC), PM collection filter (CSF) with oxidation function, selective reduction catalyst (SCR) and ammonia slip DOC An exhaust gas purification apparatus provided is employed (see, for example, Patent Document 1). However, in the next PNLT and Euro6 exhaust gas regulations, exhaust gas regulations will be strengthened and the heavy vehicle exhaust gas test method (WHDC) will be adopted, so further improvement of the exhaust gas purification device is required.

小型車のディーゼルエンジンでは、排ガス浄化装置をエンジンに近接させることで、触媒反応温度のより高い条件での排ガスの浄化が可能である。これに対して大型車では、前輪が２軸であるなどのレイアウトの制約があるので、排ガス浄化装置をエンジンに近接させることは困難であった。そのため、排ガス浄化装置の各触媒を大型化せざるを得ず、製造コストの増加を招いてしまうという問題があった。   In a diesel engine of a small car, exhaust gas can be purified under a higher catalyst reaction temperature by placing an exhaust gas purification device close to the engine. On the other hand, in a large vehicle, there are restrictions on the layout such as the front wheels having two axles, so it is difficult to bring the exhaust gas purification device close to the engine. Therefore, each catalyst of the exhaust gas purification apparatus has to be increased in size, resulting in an increase in manufacturing cost.

特開２０１４−００５７３５号公報JP 2014-005735 A

本発明の目的は、酸化触媒、ＰＭ捕集フィルター及び選択還元型触媒を備えるとともに、ディーゼルエンジンに近接して配置することを可能にした排ガス浄化装置を提供することにある。   An object of the present invention is to provide an exhaust gas purification apparatus that includes an oxidation catalyst, a PM collection filter, and a selective reduction catalyst, and that can be disposed close to a diesel engine.

上記の目的を達成する本発明の排ガス浄化装置は、ディーゼルエンジンの排ガスが流れる排気通路に介設された排ガス浄化装置であって、前記排気通路に、格納容器及びケーシングを上流側から順に介設し、前記格納容器内に、第１酸化触媒又はＮＯｘ吸蔵還元触媒と、選択還元型触媒が塗布されたＰＭ捕集フィルタとを、上流側から順に離間して配設するとともに、前記第１酸化触媒又はＮＯｘ吸蔵還元触媒と前記選択還元型触媒が塗布されたＰＭ捕集フィルタとの間の前記排ガスの流路に尿素水インジェクタを設置し、前記ケーシング内に、選択還元型触媒及び第２酸化触媒を上流側から順に配置したことを特徴とするものである。   An exhaust gas purifying apparatus of the present invention that achieves the above object is an exhaust gas purifying apparatus interposed in an exhaust passage through which exhaust gas from a diesel engine flows, and a storage container and a casing are provided in the exhaust passage sequentially from the upstream side. In the containment vessel, a first oxidation catalyst or NOx occlusion reduction catalyst, and a PM collection filter coated with a selective reduction catalyst are arranged sequentially apart from the upstream side, and the first oxidation catalyst is disposed. A urea water injector is installed in the exhaust gas flow path between the catalyst or the NOx occlusion reduction catalyst and the PM collection filter coated with the selective reduction catalyst, and the selective reduction catalyst and the second oxidation are provided in the casing. The catalyst is arranged in order from the upstream side.

本発明の排ガス浄化装置によれば、従来の排ガス浄化装置におけるＤＯＣ、ＣＳＦ及びＳＣＲによる浄化機能を、格納容器内にコンパクトに集約できるので、排ガス浄化装置を小型化してディーゼルエンジンに近接して配置することができる。   According to the exhaust gas purifying apparatus of the present invention, the purification function by DOC, CSF and SCR in the conventional exhaust gas purifying apparatus can be compactly integrated in the containment vessel, so the exhaust gas purifying apparatus is downsized and arranged close to the diesel engine. can do.

本発明の実施形態からなる排ガス浄化装置の構成図である。It is a block diagram of the exhaust gas purification apparatus which consists of embodiment of this invention. 排ガスの撹拌手段の例を示す斜視図である。It is a perspective view which shows the example of the stirring means of waste gas. 排ガスの撹拌手段の他の例を示す斜視図である。It is a perspective view which shows the other example of the stirring means of waste gas.

以下に、本発明の実施の形態について、図面を参照して説明する。図１は、本発明の実施形態からなる排ガス浄化装置を示す。なお、図中の矢印は、気体の流れる方向を示す。   Embodiments of the present invention will be described below with reference to the drawings. FIG. 1 shows an exhaust gas purification apparatus according to an embodiment of the present invention. In addition, the arrow in a figure shows the direction through which gas flows.

この排ガス浄化装置は、車両に搭載されたディーゼルエンジン（図示せず）の排ガスＧが流れる排気通路１に、上流側から順に介設された箱形の格納容器２及び円筒形のケーシング３とを備えている。なお、排ガス浄化装置は、ターボチャージャー４の下流側に介設されている。   The exhaust gas purifying apparatus includes a box-shaped containment vessel 2 and a cylindrical casing 3 that are interposed in order from an upstream side in an exhaust passage 1 through which exhaust gas G of a diesel engine (not shown) mounted on a vehicle flows. I have. The exhaust gas purification device is interposed downstream of the turbocharger 4.

格納容器２は断熱材５に覆われており、その内部には、第１酸化触媒（第１ＤＯＣ）６と、選択還元型触媒である物質が塗布されたＰＭ捕集フィルタ（以下、「ＳＣＲフィルタ」という。）７とが、上流側から順に離間して配設されている。具体的には、第１ＤＯＣ６とＳＣＲフィルタ７とは、平行に又はＬ字に配置されるとともに、接続通路８により接続されている。   The containment vessel 2 is covered with a heat insulating material 5, and a PM collection filter (hereinafter referred to as “SCR filter”) in which a first oxidation catalyst (first DOC) 6 and a material that is a selective reduction catalyst are applied. 7) are spaced apart from the upstream side in order. Specifically, the first DOC 6 and the SCR filter 7 are arranged in parallel or in an L shape and are connected by a connection passage 8.

また、格納容器２の出口の向きは、ＳＣＲフィルタ７の出口の向きと逆方向になっている。更に、格納容器２には、接続通路８内に尿素水を供給する尿素水インジェクタ９が設置されている。   Further, the direction of the outlet of the storage container 2 is opposite to the direction of the outlet of the SCR filter 7. Further, the storage container 2 is provided with a urea water injector 9 for supplying urea water into the connection passage 8.

ケーシング３内には、選択還元型触媒（ＳＣＲ）１０及び第２酸化触媒（第２ＤＯＣ）１１が、上流側から順に直列に配置されている。   In the casing 3, a selective reduction catalyst (SCR) 10 and a second oxidation catalyst (second DOC) 11 are arranged in series in order from the upstream side.

上記の第１ＤＯＣ６及び第２ＤＯＣ１１は、排ガスＧの混合機能を有する構造に成形した金属製の担持体に、ロジウム、酸化セリウム、白金、酸化アルミニウム等を担持して形成される。ＳＣＲフィルタ１０は、多孔質セラミック製のハニカムのチャンネル（セル）の入口と出口を交互に目封じしたモノリスハニカム型のウオールフローフィルタに、ゼオライト触媒などを塗布して形成される。ＳＣＲ１０は、コージェライトや酸化アルミニウムや酸化チタン等で形成されるハニカム構造等の担体に、ゼオライト触媒などを担持して形成される。   Said 1st DOC6 and 2nd DOC11 are formed by carrying | supporting rhodium, a cerium oxide, platinum, aluminum oxide etc. on the metal support body shape | molded in the structure which has the mixing function of the waste gas G. FIG. The SCR filter 10 is formed by applying a zeolite catalyst or the like to a monolith honeycomb wall flow filter in which inlets and outlets of a porous ceramic honeycomb channel (cell) are alternately plugged. The SCR 10 is formed by supporting a zeolite catalyst or the like on a carrier such as a honeycomb structure formed of cordierite, aluminum oxide, titanium oxide or the like.

この排ガス浄化装置においては、ターボチャージャー４から排気通路１を通じて格納容器２内に流入した排ガスＧは、第１ＤＯＣ６において一酸化炭素（ＣＯ）、炭化水素（ＨＣ）及び粒子状物質（ＰＭ）に含まれる未燃焼物質（ＳＯＦ）が酸化除去された後に、尿素水インジェクタ９から噴射された尿素水が加水分解して生成したアンモニア（ＮＨ3）とともにＳＣＲフィルタ７へ流入する。そして、ＳＣＲフィルタ７においてＮＨ3による還元反応によりＮＯｘが浄化されるとともにＰＭが除去された後に格納容器２から放出される。 In this exhaust gas purification apparatus, the exhaust gas G flowing into the containment vessel 2 from the turbocharger 4 through the exhaust passage 1 is included in carbon monoxide (CO), hydrocarbon (HC), and particulate matter (PM) in the first DOC 6. After the unburned material (SOF) is oxidized and removed, urea water injected from the urea water injector 9 flows into the SCR filter 7 together with ammonia (NH 3 ) generated by hydrolysis. In the SCR filter 7, NOx is purified by a reduction reaction with NH 3 and PM is removed and then released from the storage container 2.

ディーゼルエンジンが、エンジン回転数が高くかつ高負荷となる運転領域にあるときは、格納容器２から放出された排ガスＧ中にＮＯｘが残存するおそれがあるが、その残存するＮＯｘは、ＳＣＲ１０においてＮＨ3による還元反応により浄化される。なお、還元反応において消費されなかったＮＨ3は、第２ＤＯＣ１１において酸化・分解される。 When the diesel engine is in an operating region where the engine speed is high and the load is high, NOx may remain in the exhaust gas G released from the containment vessel 2, but the remaining NOx is converted into NH in the SCR 10. Purified by the reduction reaction by 3 . Note that NH 3 that has not been consumed in the reduction reaction is oxidized and decomposed in the second DOC 11.

このように排ガス浄化装置を構成することで、従来の排ガス浄化装置におけるＤＯＣ、ＣＳＦ及びＳＣＲによる浄化機能を、格納容器２内にコンパクトに集約できるので、排ガス浄化装置を小型化してディーゼルエンジンに近接して配置することができるのである。   By configuring the exhaust gas purification device in this way, the purification function by the DOC, CSF and SCR in the conventional exhaust gas purification device can be compactly integrated in the containment vessel 2, so the exhaust gas purification device is downsized and close to the diesel engine Can be arranged.

また、選択還元型触媒である物質の総容量の削減が可能となるため、排ガス浄化装置の製造コストを低減することができる。   In addition, since the total capacity of the substance that is the selective reduction catalyst can be reduced, the manufacturing cost of the exhaust gas purification device can be reduced.

更には、ＳＣＲフィルタ７から排出された排ガスＧの一部が、断熱材５に覆われている格納容器２の内壁面１２と接続通路２との間に滞留して、自身の有する熱（廃熱）により第１ＤＯＣ６及びＳＣＲフィルタ７を加温するので、触媒反応温度を高温に維持して浄化性能を向上することができる。   Furthermore, a part of the exhaust gas G discharged from the SCR filter 7 stays between the inner wall surface 12 of the storage container 2 covered with the heat insulating material 5 and the connection passage 2, and heat (waste) Since the first DOC 6 and the SCR filter 7 are heated by heat), the catalytic reaction temperature can be maintained at a high temperature and the purification performance can be improved.

上記の排ガス浄化装置においては、第１ＤＯＣ６とＳＣＲフィルタ７との間の接続通路２内であって尿素水インジェクタ９の下流側に、排ガスＧの撹拌手段１３を設置することが望ましい。この撹拌手段１３としては、金属プレート１４に切り込み１５を互い違いに入れて軸方向へ折り曲げたミキサー板１６（図２を参照）や、金属プレート１４に適当な間隔で貫通孔１７を形成したバッフル板１８（図３を参照）などが好ましく例示される。   In the exhaust gas purifying apparatus described above, it is desirable to install the agitation means 13 for the exhaust gas G in the connection passage 2 between the first DOC 6 and the SCR filter 7 and downstream of the urea water injector 9. As the stirring means 13, a mixer plate 16 (see FIG. 2) in which notches 15 are alternately inserted into the metal plate 14 and bent in the axial direction, or a baffle plate in which through holes 17 are formed in the metal plate 14 at appropriate intervals. 18 (see FIG. 3) is preferably exemplified.

このように撹拌手段１３を設置することで、尿素水インジェクタ９から噴射された尿素水を高温の排ガスＧと撹拌させて十分に気化させることができる。   By installing the stirring means 13 in this way, the urea water injected from the urea water injector 9 can be stirred with the high-temperature exhaust gas G and sufficiently vaporized.

また、上記の排ガス浄化装置においては、格納容器２内の第１ＤＯＣ６をＮＯｘ吸蔵還元触媒（ＬＮＴ）に置き換えるようにしても良い。そのようにすることで、ディーゼルエンジンが、排ガスＧの温度が低くかつ高負荷となる運転領域において、車両からのＮＯｘの排出を効果的に低減することができる。   In the exhaust gas purification apparatus, the first DOC 6 in the containment vessel 2 may be replaced with a NOx storage reduction catalyst (LNT). By doing so, the diesel engine can effectively reduce NOx emission from the vehicle in an operation region where the temperature of the exhaust gas G is low and the load is high.

１ 排気通路
２ 格納容器
３ ケーシング
６ 第１ＤＯＣ
７ ＳＣＲフィルタ
８ 接続通路
９ 尿素水インジェクタ
１０ ＳＣＲ
１１ 第２ＤＯＣ
１３ 撹拌手段 1 exhaust passage 2 containment vessel 3 casing 6 first DOC
7 SCR filter 8 Connection passage 9 Urea water injector 10 SCR
11 Second DOC
13 Stirring means

Claims (4)

ディーゼルエンジンの排ガスが流れる排気通路に介設された排ガス浄化装置であって、
前記排気通路に、格納容器及びケーシングを上流側から順に介設し、
前記格納容器内に、第１酸化触媒又はＮＯｘ吸蔵還元触媒と、選択還元型触媒が塗布されたＰＭ捕集フィルタとを、上流側から順に離間して配設するとともに、前記第１酸化触媒又はＮＯｘ吸蔵還元触媒と前記選択還元型触媒が塗布されたＰＭ捕集フィルタとの間の前記排ガスの流路に尿素水インジェクタを設置し、
前記ケーシング内に、選択還元型触媒及び第２酸化触媒を上流側から順に配置したことを特徴とする排ガス浄化装置。 An exhaust gas purification device interposed in an exhaust passage through which exhaust gas from a diesel engine flows,
In the exhaust passage, a containment vessel and a casing are interposed in order from the upstream side,
In the containment vessel, a first oxidation catalyst or NOx occlusion reduction catalyst and a PM collection filter coated with a selective reduction catalyst are sequentially spaced from the upstream side, and the first oxidation catalyst or A urea water injector is installed in the exhaust gas flow path between the NOx storage reduction catalyst and the PM collection filter coated with the selective reduction catalyst,
An exhaust gas purifying apparatus, wherein a selective reduction catalyst and a second oxidation catalyst are arranged in order from the upstream side in the casing. 前記第１酸化触媒又はＮＯｘ吸蔵還元触媒と、前記選択還元型触媒が塗布されたＰＭ捕集フィルタとを平行に、又はＬ字に配置した請求項１に記載の排ガス浄化装置。   The exhaust gas purification apparatus according to claim 1, wherein the first oxidation catalyst or NOx storage reduction catalyst and the PM collection filter coated with the selective reduction catalyst are arranged in parallel or in an L shape. 前記第１酸化触媒又はＮＯｘ吸蔵還元触媒と、前記選択還元型触媒が塗布されたＰＭ捕集フィルタとの間の前記排ガスの流路に、前記排ガスの撹拌手段を設置した請求項１又は２に記載の排ガス浄化装置。   The exhaust gas stirring means is installed in a flow path of the exhaust gas between the first oxidation catalyst or NOx occlusion reduction catalyst and the PM collection filter coated with the selective reduction catalyst. The exhaust gas purification apparatus as described. 前記ディーゼルエンジンが、前記排気通路にタービンが介設されたターボチャージャーを備えるとともに、前記格納容器を前記タービンの下流側の前記排気通路に介設した請求項１〜３のいずれか１項に記載の排ガス浄化装置。   The diesel engine includes a turbocharger in which a turbine is interposed in the exhaust passage, and the containment vessel is interposed in the exhaust passage on the downstream side of the turbine. Exhaust gas purification equipment.
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Cited By (3)

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JP2018062932A (en) * 2016-10-11 2018-04-19 現代自動車株式会社Ｈｙｕｎｄａｉ Ｍｏｔｏｒ Ｃｏｍｐａｎｙ Heat insulation structure for vehicular catalytic converter
KR20180096089A (en) * 2017-02-20 2018-08-29 현대자동차주식회사 Device for reducing nitrogen oxide of diesel engine
JP2021025482A (en) * 2019-08-07 2021-02-22 日新工業株式会社 Exhaust emission control device, flow path formation member, and cylindrical member

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