FR2976823B1 - Dispositif d'epuration des gaz d'echappement d'un moteur thermique comprenant un support ceramique et une phase active ancree mecaniquement dans le support - Google Patents

Dispositif d'epuration des gaz d'echappement d'un moteur thermique comprenant un support ceramique et une phase active ancree mecaniquement dans le support

Info

Publication number
FR2976823B1
FR2976823B1 FR1155688A FR1155688A FR2976823B1 FR 2976823 B1 FR2976823 B1 FR 2976823B1 FR 1155688 A FR1155688 A FR 1155688A FR 1155688 A FR1155688 A FR 1155688A FR 2976823 B1 FR2976823 B1 FR 2976823B1
Authority
FR
France
Prior art keywords
support
exhaust gas
gas purifying
purifying device
active phase
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Fee Related
Application number
FR1155688A
Other languages
English (en)
French (fr)
Other versions
FR2976823A1 (fr
Inventor
Gallo Pascal Del
Fabrice Rossignol
Thierry Chartier
Raphael Faure
Sebastien Goudalle
Claire Bonhomme
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Centre National de la Recherche Scientifique CNRS
Air Liquide SA
Universite de Limoges
LAir Liquide SA pour lEtude et lExploitation des Procedes Georges Claude
Original Assignee
Centre National de la Recherche Scientifique CNRS
Air Liquide SA
Universite de Limoges
LAir Liquide SA pour lEtude et lExploitation des Procedes Georges Claude
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Priority to FR1155688A priority Critical patent/FR2976823B1/fr
Application filed by Centre National de la Recherche Scientifique CNRS, Air Liquide SA, Universite de Limoges, LAir Liquide SA pour lEtude et lExploitation des Procedes Georges Claude filed Critical Centre National de la Recherche Scientifique CNRS
Priority to CN201280031118.XA priority patent/CN103702759A/zh
Priority to BR112013033508A priority patent/BR112013033508A2/pt
Priority to EP12730415.2A priority patent/EP2723496A1/fr
Priority to PCT/EP2012/060904 priority patent/WO2013000683A1/fr
Priority to MX2013015110A priority patent/MX2013015110A/es
Priority to RU2014102340/04A priority patent/RU2014102340A/ru
Priority to US14/128,483 priority patent/US20140130482A1/en
Priority to JP2014517561A priority patent/JP2014518152A/ja
Priority to CA2838360A priority patent/CA2838360A1/fr
Priority to KR1020147001791A priority patent/KR20140082632A/ko
Publication of FR2976823A1 publication Critical patent/FR2976823A1/fr
Application granted granted Critical
Publication of FR2976823B1 publication Critical patent/FR2976823B1/fr
Expired - Fee Related legal-status Critical Current
Anticipated expiration legal-status Critical

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Classifications

    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
    • B01D53/34—Chemical or biological purification of waste gases
    • B01D53/92—Chemical or biological purification of waste gases of engine exhaust gases
    • B01D53/94—Chemical or biological purification of waste gases of engine exhaust gases by catalytic processes
    • B01D53/9445—Simultaneously removing carbon monoxide, hydrocarbons or nitrogen oxides making use of three-way catalysts [TWC] or four-way-catalysts [FWC]
    • B01D53/945—Simultaneously removing carbon monoxide, hydrocarbons or nitrogen oxides making use of three-way catalysts [TWC] or four-way-catalysts [FWC] characterised by a specific catalyst
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
    • F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
    • F01N3/00—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust
    • F01N3/08—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous
    • F01N3/10—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust
    • F01N3/18—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust characterised by methods of operation; Control
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J35/00—Catalysts, in general, characterised by their form or physical properties
    • B01J35/50—Catalysts, in general, characterised by their form or physical properties characterised by their shape or configuration
    • B01J35/51—Spheres
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J21/00—Catalysts comprising the elements, oxides, or hydroxides of magnesium, boron, aluminium, carbon, silicon, titanium, zirconium, or hafnium
    • B01J21/005—Spinels
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/005—Spinels
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/38—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of noble metals
    • B01J23/54—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of noble metals combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36
    • B01J23/56—Platinum group metals
    • B01J23/63—Platinum group metals with rare earths or actinides
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/70—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper
    • B01J23/76—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36
    • B01J23/83—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36 with rare earths or actinides
    • B—PERFORMING OPERATIONS; TRANSPORTING
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    • B01J35/30—Catalysts, in general, characterised by their form or physical properties characterised by their physical properties
    • B01J35/391—Physical properties of the active metal ingredient
    • B01J35/393—Metal or metal oxide crystallite size
    • B—PERFORMING OPERATIONS; TRANSPORTING
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    • B01J35/00—Catalysts, in general, characterised by their form or physical properties
    • B01J35/60—Catalysts, in general, characterised by their form or physical properties characterised by their surface properties or porosity
    • B—PERFORMING OPERATIONS; TRANSPORTING
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    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/0009—Use of binding agents; Moulding; Pressing; Powdering; Granulating; Addition of materials ameliorating the mechanical properties of the product catalyst
    • B01J37/0027—Powdering
    • B01J37/0045—Drying a slurry, e.g. spray drying
    • B—PERFORMING OPERATIONS; TRANSPORTING
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    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/0215—Coating
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
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    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/024—Multiple impregnation or coating
    • B01J37/0242—Coating followed by impregnation
    • C—CHEMISTRY; METALLURGY
    • C04—CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
    • C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
    • C04B38/00—Porous mortars, concrete, artificial stone or ceramic ware; Preparation thereof
    • C04B38/06—Porous mortars, concrete, artificial stone or ceramic ware; Preparation thereof by burning-out added substances by burning natural expanding materials or by sublimating or melting out added substances
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
    • F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
    • F01N3/00—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust
    • F01N3/08—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous
    • F01N3/10—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust
    • F01N3/24—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust characterised by constructional aspects of converting apparatus
    • F01N3/28—Construction of catalytic reactors
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
    • F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
    • F01N3/00—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust
    • F01N3/08—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous
    • F01N3/10—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust
    • F01N3/24—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust characterised by constructional aspects of converting apparatus
    • F01N3/28—Construction of catalytic reactors
    • F01N3/2803—Construction of catalytic reactors characterised by structure, by material or by manufacturing of catalyst support
    • F01N3/2825—Ceramics
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
    • F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
    • F01N3/00—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust
    • F01N3/08—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous
    • F01N3/10—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust
    • F01N3/24—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for rendering innocuous by thermal or catalytic conversion of noxious components of exhaust characterised by constructional aspects of converting apparatus
    • F01N3/28—Construction of catalytic reactors
    • F01N3/2803—Construction of catalytic reactors characterised by structure, by material or by manufacturing of catalyst support
    • F01N3/2832—Construction of catalytic reactors characterised by structure, by material or by manufacturing of catalyst support granular, e.g. pellets
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
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    • B01D2255/10—Noble metals or compounds thereof
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    • B01D2255/92—Dimensions
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    • B01D2258/012—Diesel engines and lean burn gasoline engines
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    • C—CHEMISTRY; METALLURGY
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    • C04B—LIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
    • C04B2111/00—Mortars, concrete or artificial stone or mixtures to prepare them, characterised by specific function, property or use
    • C04B2111/00474—Uses not provided for elsewhere in C04B2111/00
    • C04B2111/0081—Uses not provided for elsewhere in C04B2111/00 as catalysts or catalyst carriers
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02A—TECHNOLOGIES FOR ADAPTATION TO CLIMATE CHANGE
    • Y02A50/00—TECHNOLOGIES FOR ADAPTATION TO CLIMATE CHANGE in human health protection, e.g. against extreme weather
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    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Materials Engineering (AREA)
  • Organic Chemistry (AREA)
  • Combustion & Propulsion (AREA)
  • Health & Medical Sciences (AREA)
  • Ceramic Engineering (AREA)
  • Toxicology (AREA)
  • Mechanical Engineering (AREA)
  • General Engineering & Computer Science (AREA)
  • Analytical Chemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Environmental & Geological Engineering (AREA)
  • Biomedical Technology (AREA)
  • Structural Engineering (AREA)
  • Catalysts (AREA)
FR1155688A 2011-06-27 2011-06-27 Dispositif d'epuration des gaz d'echappement d'un moteur thermique comprenant un support ceramique et une phase active ancree mecaniquement dans le support Expired - Fee Related FR2976823B1 (fr)

Priority Applications (11)

Application Number Priority Date Filing Date Title
FR1155688A FR2976823B1 (fr) 2011-06-27 2011-06-27 Dispositif d'epuration des gaz d'echappement d'un moteur thermique comprenant un support ceramique et une phase active ancree mecaniquement dans le support
JP2014517561A JP2014518152A (ja) 2011-06-27 2012-06-08 セラミック担体、及び担体において機械的に固定された活性相を含む、熱機関からの排ガスを浄化するためのデバイス
EP12730415.2A EP2723496A1 (fr) 2011-06-27 2012-06-08 Dispositif d'épuration des gaz d'échappement d'un moteur thermique comprenant un support céramique et une phase active ancrée mécaniquement dans le support
PCT/EP2012/060904 WO2013000683A1 (fr) 2011-06-27 2012-06-08 Dispositif d'épuration des gaz d'échappement d'un moteur thermique comprenant un support céramique et une phase active ancrée mécaniquement dans le support
MX2013015110A MX2013015110A (es) 2011-06-27 2012-06-08 Dispositivo para la purificacion de gases de escape de un motor de combustion termica que comprende un portador ceramico y una fase activa mecanicamente anclada en el portador.
RU2014102340/04A RU2014102340A (ru) 2011-06-27 2012-06-08 Устройство для очистки выхлопных газов теплового двигателя, содержащее керамический носитель и активную фазу, механически закрепленную в носителе
CN201280031118.XA CN103702759A (zh) 2011-06-27 2012-06-08 用于净化来自热机的废气的装置，其包含陶瓷载体和机械锚定在载体中的活性相
BR112013033508A BR112013033508A2 (pt) 2011-06-27 2012-06-08 dispositivo de purificação de gases de escape de um motor de combustão, compreendendo um suporte cerâmico e uma fase ativa acoplada mecanicamente ao suporte
CA2838360A CA2838360A1 (fr) 2011-06-27 2012-06-08 Dispositif d'epuration des gaz d'echappement d'un moteur thermique comprenant un support ceramique et une phase active ancree mecaniquement dans le support
KR1020147001791A KR20140082632A (ko) 2011-06-27 2012-06-08 세라믹 담체, 및 상기 담체에 기계적으로 고정된 활성 상을 포함하는, 열기관으로부터의 배기 가스의 정화를 위한 장치
US14/128,483 US20140130482A1 (en) 2011-06-27 2012-06-08 Device for the Purification of Exhaust Gases from a Heat Engine, Comprising a Ceramic Carrier and an Active Phase Mechanically Anchored in the Carrier

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FR1155688A FR2976823B1 (fr) 2011-06-27 2011-06-27 Dispositif d'epuration des gaz d'echappement d'un moteur thermique comprenant un support ceramique et une phase active ancree mecaniquement dans le support

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FR2991713A1 (fr) * 2012-06-11 2013-12-13 Air Liquide Dispositif d'epuration des gaz d'echappement d'un moteur thermique comprenant un support ceramique fractionne a l'echelle nanometrique
FR3009973B1 (fr) * 2013-08-30 2023-06-09 Air Liquide Materiau de pre-revetement d’un substrat metallique d’un materiau catalytique a base de ceramique
KR102016751B1 (ko) * 2017-12-14 2019-10-14 한국에너지기술연구원 다양한 오염물질을 함유한 반도체 제조 공정 배기가스 내 질소 산화물(NOx) 및 아산화질소(N2O)의 촉매 제거 방법
EP4365590A2 (en) 2019-03-20 2024-05-08 Juntendo Educational Foundation Agent targeting double-membrane organelle dna

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ATE326558T1 (de) * 2001-08-30 2006-06-15 Aktina Ltd Verfahren zur herstellung poröser keramik-metall verbundwerkstoffe und dadurch erhaltene verbundwerkstoffe
ATE539814T1 (de) * 2006-11-08 2012-01-15 Air Liquide Verfahren zur herstellung einesträgerkatalysators
FR2991713A1 (fr) * 2012-06-11 2013-12-13 Air Liquide Dispositif d'epuration des gaz d'echappement d'un moteur thermique comprenant un support ceramique fractionne a l'echelle nanometrique

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KR20140082632A (ko) 2014-07-02
CN103702759A (zh) 2014-04-02
JP2014518152A (ja) 2014-07-28
EP2723496A1 (fr) 2014-04-30
FR2976823A1 (fr) 2012-12-28
CA2838360A1 (fr) 2013-01-03
WO2013000683A1 (fr) 2013-01-03
BR112013033508A2 (pt) 2017-01-24
US20140130482A1 (en) 2014-05-15
RU2014102340A (ru) 2015-08-10
MX2013015110A (es) 2014-04-14

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