DE744998C - Process for the production of sintered phosphate fertilizers - Google Patents

Process for the production of sintered phosphate fertilizers

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Publication number
DE744998C
DE744998C DEK157082D DEK0157082D DE744998C DE 744998 C DE744998 C DE 744998C DE K157082 D DEK157082 D DE K157082D DE K0157082 D DEK0157082 D DE K0157082D DE 744998 C DE744998 C DE 744998C
Authority
DE
Germany
Prior art keywords
production
lime
phosphate fertilizers
sintered
coal
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
DEK157082D
Other languages
German (de)
Inventor
Dr Walter Marschner
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Kali Chemie AG
Original Assignee
Kali Chemie AG
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Kali Chemie AG filed Critical Kali Chemie AG
Priority to DEK157082D priority Critical patent/DE744998C/en
Application granted granted Critical
Publication of DE744998C publication Critical patent/DE744998C/en
Expired legal-status Critical Current

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Classifications

    • CCHEMISTRY; METALLURGY
    • C05FERTILISERS; MANUFACTURE THEREOF
    • C05BPHOSPHATIC FERTILISERS
    • C05B13/00Fertilisers produced by pyrogenic processes from phosphatic materials
    • C05B13/02Fertilisers produced by pyrogenic processes from phosphatic materials from rock phosphates

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Fertilizers (AREA)

Description

Verfahren zur Herstellung von Sinterphosphatdüngemitteln Bei einem bekannten Verfahren zur Herstellung von Sinterp4osphaten aus Rohphosphaten in Mischung mit Alkalien und Kieselsäure oder Alkalisilikaten wird das Verhältnis der Reaktionskomponenten in der Mischung derart geregelt, daß auf i Mol P.0, , etwa i Mol Alkalioxyd und solche Mengen Kalk und Kieselsäure vorhanden sind, dgß 1J3 des an die Phosphorsäure gebundenen Kalks und sonst noch etwa vorhandener Kalk bzw. Kieselsäure als Calciumorthosilikat gebunden wird, wobei Temperaturen oberhalb iooo° angewendet werden.Process for the production of sintered phosphate fertilizers At a known process for the production of sintered phosphates from rock phosphates in a mixture with alkalis and silicic acid or alkali silicates, the ratio of the reaction components regulated in the mixture in such a way that on i mole of P.0,, about i mole of alkali oxide and Lime and silicic acid are present in such quantities as 1/3 of that of phosphoric acid bound lime and any other lime or silica that may be present as calcium orthosilicate is bound, with temperatures above iooo ° are used.

Es wurde nun gefunden, daß man bei Verwenldung von mindestens 1,5, vorzugsweise 1,8 bis : Malen Soda oder Pottasche o. dgl. und darüber schon bei Temperaturen unterhalb iooo°, z. B. 85o bis 95o°, hoch citronensäurelösliche und citratlösliche Düngemittel erzielt und dabei keine Kieselsäure zuzusetzen braucht, sondern auch aus praktisch kieselsätirefreien bzw. kieselsäurearmen Rohphosphaten ohne weiteren Kieselsäurezusatz Aufschlüsse erhält, wenn man den Mischungen fein gemahlene Kohle zusetzt und sie unter Luftausschluß glüht. Läßt man die Kohle weg, so erhält man bei Verwendung von kieselsäurearmen Rohphosphaten, wie z. B. Constantine-Phosphat, Marokko-Phosphat, Murman-Konzentrat u. dgl., bei Temperaturen von 85o bis 95o° mehr oder weniger blasig geschmolzene Massen, deren Gehalt an citratlöslicher Phosphorsäure, etwa 3o bis 6o°/" verhältnismäßig gering ist, während bei Zusatz von Kohle ein Schmelzen nicht eintritt.It has now been found that when using at least 1.5, preferably 1.8 to: paint soda or potash or the like and above even at temperatures below iooo °, e.g. B. 85o to 95o °, highly citric acid-soluble and citrate-soluble Achieved fertilizers and does not need to add silica, but also from virtually silica-free or low-silica rock phosphates without any further Addition of silica gives digestions when adding finely ground coal to the mixtures clogs and it glows in the absence of air. If you leave out the coal, you get when using low-silica rock phosphates, such as. B. Constantine Phosphate, Morocco phosphate, Murman concentrate and the like, at temperatures of 85o to 95o ° more or less vesicularly molten masses, the content of which is citrate-soluble phosphoric acid, about 30 to 60 ° / "is relatively low, while with the addition of coal a melting does not occur.

Zur Erzielung eines weitgehend citratlcisliehen Düngemittels von etwa 94. bis ioo°;" genügt es im allgemeinen, der Mischung etwa io bis 15 Teile Braunkohlenstaub zuzusetzen. Es können jedoch auch größere lengen Kohle beigemischt werden.To achieve a largely citrate fertilizer of about 94 to 100%, it is generally sufficient to add about 10 to 15 parts of pulverized lignite to the mixture to add. However, larger quantities of coal can also be added.

Beim Arbeiten in Drehrohröfen unter direkter Beheizung mit Feuerbasen muß ebenfalls darauf geachtet werden, dar die Gasatmosphäre keine oxydierenden Wirkungen ausübt. Man läßt das Düngemittel zweckmäßig in einer neutralen oder reduzierenden Atmosphäre abkühlen. Es ist zwar schon bekannt, Roliphospliz;te mit i bis 2 Molen _@lhalisulfat aufzuschließen. wob °i der verwendeten Mischung auch hohle zugesetzt tvird. Die Kohle dient hier aber zur Reduktion des Alkalisulfates zu _@ll;ali:ulnil. _iußerdem liegt die erforderliche Temperatur über iooo° C. Beispiel Zoo Teile fein gemahlenes Constantine-Plio -;; - tlrl @f phat (mit 29,4--1/0 P.0,-, 48,14'/, Ca 0 i,oi°io SiO.) werden mit 9o,98 Teilen Soda von q6"5/, entsprechend z Holen 1; a=CO auf 1 Mol P.05, inn.igst gemischt und bei 85o° C unter Luftabschluß geglüht. Die Masse war blasig geschmolzen und enthielt 2.76°/o Phosphorsäure. wovon 3o°4 citrat- löslich waren. Werden die gleichen Ausgangs- stoffe mit 12,5 Teilen Braunkohlenstaub auf ioo Teile Constantine-Phosphat vermischt und bei 90o° C unter Luftabschluß geglüht, so ist das Glühprodukt nicht geschmolzen, sondern gesintert und enthält 24,32°/a Phosphorsäure, TVOVon 97.7°!o citraföslich sind. When working in rotary kilns under direct heating with firebases, care must also be taken that the gas atmosphere does not have any oxidizing effects. The fertilizer is expediently allowed to cool in a neutral or reducing atmosphere. It is already known, Roliphospliz; te to be digested with 1 to 2 moles of lhalisulphate. where the mixture used is also hollow added tvird. The coal is used here for Reduction of the alkali sulfate to _ @ ll; ali: ulnil. The required temperature is also there over iooo ° C. example Zoo parts finely ground Constantine-Plio - ;; - tlrl @f phat (with 29.4--1 / 0 P.0, -, 48.14 '/, Ca 0 i, oi ° io SiO.) are mixed with 9o.98 parts of soda from q6 "5 /, corresponding to z fetch 1; a = CO to 1 mole of P.05, intimately mixed and with Annealed at 85o ° C in the absence of air. the The mass had melted and contained blisters 2.76% phosphoric acid. of which 3o ° 4 citrate were soluble. Are the same starting substances with 12.5 parts of lignite dust ioo parts of constantine phosphate mixed and Annealed at 90o ° C in the absence of air, so is the glow product is not melted, but rather sintered and contains 24.32% phosphoric acid, TVO of 97.7 °! O are citra-soluble.

Claims (1)

PATENTANSPRUCH --erfahren zur Herstellung von Sinterpliosphatdüngemitteln durch Glühen von G,nnischen von Roliphospliaten mit Soda, Pottasche cnd dergleichen oz@-di'sclien Alkalien in :Mengen von mehr als i Mol Alkaliolvd auf i llol P=O,; hei Tempe- raturen unterhalb iooo°, dadurch gekenn- zeichnet, daßl mindestens i,5 vorzugsweise 1,8 bis 2 Mole und darüber Alkalioxyd auf .i iNlol P:*O; verwendet «-erden', ferner der'-.@ti-fschliiß ohne oder in Gegenwart gerie,ei.@Iengen Kieselsäure vollzogen iyxtd, als sich zur Bindung von 1/3 des an Phosphorsäure gebundenen Kalks und des noch in anderer Form vorliegenden Kalks als Calciumorthosilikat errechnet, und die Erhitzung unter Ausschluß oxydierender Wirkungen und unter Zusatz von Reduk- tionskohle erfnlgt.
Zur Abgrenzung des Anmeldungsgegenstandes vom Stand der Technik sind im Erteilungsverfahren folgende Druckschriften in Betracht gezogen worden: deutsche Patentschriften . . . , \r.600 269, 507 925 französische Patentschritt 816 693; Angewandte Chemie. 51. Talirgang, 1938, S. 197 his 2 03.
PATENT CLAIM - Experienced in the production of sintered phosphate fertilizers by annealing G, niches of Roliphospliaten with soda, Potash cnd like oz @ -di'sclien Alkalis in: amounts of more than 1 mole Alkali metal on i llol P = O ,; hot tempe- temperatures below iooo °, which means that draws thatl at least 1.5 preferably 1.8 to 2 moles and above alkali oxide on .i iNlol P: * O; uses "-erden", furthermore der '-. @ ti-fschliiß without or in the present gerie, ei. @ Iengen Silicic acid completed iyxtd when deciding to bind 1/3 of the to Phosphoric acid bound lime and des lime present in another form calculated as calcium orthosilicate, and the Heating to the exclusion of oxidizing agents Effects and with the addition of reducing tion coal succeeded.
To distinguish the subject of the application from the state of the art, the following publications were considered in the granting procedure: German patents. . . , \ r. 600 269, 507 925 French patent step 816 693; Applied Chemistry. 51st Talirgang, 1938, P. 197 to 2 03.
DEK157082D 1940-03-16 1940-03-16 Process for the production of sintered phosphate fertilizers Expired DE744998C (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
DEK157082D DE744998C (en) 1940-03-16 1940-03-16 Process for the production of sintered phosphate fertilizers

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Application Number Priority Date Filing Date Title
DEK157082D DE744998C (en) 1940-03-16 1940-03-16 Process for the production of sintered phosphate fertilizers

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DE744998C true DE744998C (en) 1944-02-22

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Cited By (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE942928C (en) * 1954-05-12 1956-05-09 Dessau Gaerungschemie Process for processing Melssian mash
DE1018075B (en) * 1955-08-03 1957-10-24 Walter Hildebrand Process for the production of ammonium citrate-soluble sintered phosphate fertilizers
DE1266768B (en) * 1966-04-21 1968-04-25 Kali Chemie Ag Process for the preparation of potassium gluehphosphate fertilizers
DE1294979B (en) * 1966-11-16 1969-05-14 Kali Chemie Ag Process for the production of gluehphosphate fertilizers
FR2382416A1 (en) * 1977-03-02 1978-09-29 Kali Chemie Ag PROCESS FOR THE PRODUCTION OF PHOSPHATE FERTILIZERS

Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE507925C (en) * 1924-06-23 1930-09-22 Kali Chemie Akt Ges Manufacture of fertilizers
DE600269C (en) * 1927-11-22 1934-09-21 Anton Messerschmitt Dr Process for the preparation of citrate-soluble calcium alkali metal phosphates
FR816693A (en) * 1936-01-24 1937-08-13 Metallgesellschaft Ag Process for preparing a double alkaline and alkaline earth fertilizer

Patent Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE507925C (en) * 1924-06-23 1930-09-22 Kali Chemie Akt Ges Manufacture of fertilizers
DE600269C (en) * 1927-11-22 1934-09-21 Anton Messerschmitt Dr Process for the preparation of citrate-soluble calcium alkali metal phosphates
FR816693A (en) * 1936-01-24 1937-08-13 Metallgesellschaft Ag Process for preparing a double alkaline and alkaline earth fertilizer

Cited By (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE942928C (en) * 1954-05-12 1956-05-09 Dessau Gaerungschemie Process for processing Melssian mash
DE1018075B (en) * 1955-08-03 1957-10-24 Walter Hildebrand Process for the production of ammonium citrate-soluble sintered phosphate fertilizers
DE1266768B (en) * 1966-04-21 1968-04-25 Kali Chemie Ag Process for the preparation of potassium gluehphosphate fertilizers
DE1294979B (en) * 1966-11-16 1969-05-14 Kali Chemie Ag Process for the production of gluehphosphate fertilizers
FR2382416A1 (en) * 1977-03-02 1978-09-29 Kali Chemie Ag PROCESS FOR THE PRODUCTION OF PHOSPHATE FERTILIZERS

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