DE691903C - Process for producing a transparent, light protective layer on aluminum and aluminum alloys by chemical means - Google Patents

Process for producing a transparent, light protective layer on aluminum and aluminum alloys by chemical means

Info

Publication number
DE691903C
DE691903C DE1937V0034008 DEV0034008D DE691903C DE 691903 C DE691903 C DE 691903C DE 1937V0034008 DE1937V0034008 DE 1937V0034008 DE V0034008 D DEV0034008 D DE V0034008D DE 691903 C DE691903 C DE 691903C
Authority
DE
Germany
Prior art keywords
aluminum
protective layer
transparent
producing
chemical means
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
DE1937V0034008
Other languages
German (de)
Inventor
Dipl-Ing Werner Helling
Heinrich Neunzig
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Vereinigte Aluminium Werke AG
Original Assignee
Vereinigte Aluminium Werke AG
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Vereinigte Aluminium Werke AG filed Critical Vereinigte Aluminium Werke AG
Priority to DE1937V0034008 priority Critical patent/DE691903C/en
Application granted granted Critical
Publication of DE691903C publication Critical patent/DE691903C/en
Expired legal-status Critical Current

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Classifications

    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C22/00Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals
    • C23C22/05Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions
    • C23C22/60Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions using alkaline aqueous solutions with pH greater than 8
    • C23C22/66Treatment of aluminium or alloys based thereon
    • C23C22/67Treatment of aluminium or alloys based thereon with solutions containing hexavalent chromium

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  • Chemical & Material Sciences (AREA)
  • General Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Chemical Treatment Of Metals (AREA)

Description

Verfahren zur Erzeugung einer transparenten, hellen Schutzschicht auf Aluminium und Aluminiumlegierungen auf chemischem Wege Bei der Erzeugung einer oxydischen Schutzschicht auf Aluminium und Aluminiumlegierungen -in alkalischen, chromathaltigen Bädern findet zunächst eine Auflösung metallischen Aluminiums statt. Es entsteht neben Aluminat Wasserstoff, der reduzierend auf das Chromat einwirkt. Es bildet sich wasserunlösliches Chromhydroxyd, das sich in das durch Hydrolyse des Aluminats entstandene Aluminiurnhydroxyd einbaut. Dieses Chromhydroxyd färbt die entstehende Schutzschicht Hellgrau bis graugrün. Derart gefärbte Überzüge entstehen beispielsweise bei. der chemischen Oxydation des Aluminiums nach (lern modifizierten Bauer-Vogel-Verfahren (G. 1: c k e r t : »Hauszeitschrift Aluminium« a, 1931 S. 34.9). Durch fo Minuten langes Eintauchen in die 9o bis 95° C heiße MBV-Lösung, im Liter -Wasser- 6o g eines Gemisches von Natriummonochomat und Soda im Verhältnis 1,5 : 5, entsteht ein schiefergrauer Überzug. Schichten dieser 'Färbung sind bei vielen Gegenständen, bei denen man Wert darauf legt, daß die Eigenfarbe des Aluminiums erhalten bleibt, unerwünscht.Process for producing a transparent, light protective layer on aluminum and aluminum alloys by chemical means in the production of a oxidic protective layer on aluminum and aluminum alloys -in alkaline, In baths containing chromate, metallic aluminum is first dissolved. In addition to aluminate, hydrogen is produced, which has a reducing effect on the chromate. Water-insoluble chromium hydroxide is formed, which is converted into it by hydrolysis the aluminum hydroxide formed by the aluminate. This chromium hydroxide stains the resulting protective layer is light gray to gray-green. Such colored coatings are created for example at. the chemical oxidation of aluminum (learn modified Bauer-Vogel method (G. 1: c k e r t: "Hauszeitschrift Aluminum" a, 1931 p. 34.9). By immersing it in the MBV solution at 9o to 95 ° C for four minutes, in the liter -water- 6o g of a mixture of sodium monochomat and soda in the ratio 1.5: 5, a slate-gray coating is created. Layers of this' coloring are at many objects for which it is important that the natural color of the aluminum remains, undesirable.

Im Verlauf von Versuchen wurde nün festgestellt, daß schon sehr geringe Zusätze von Silicaten, z. B. Wasserglas, zu den alkalischen Chromatlösungen genügen,--um den Chromgehalt bemerkenswert herabzusetzen und farblose Schutzschichten zu erzeugen. Die nachfolgend angegebenen Werte gelten für-Schichten, die in Sodachrotnatlösungen gleicher Zusammensetzung. -mit und @ ohne Zusatz yön o,o6o/a Wasserglas hergestellt würden.In the course of experiments it was now found that very little Additions of silicates, e.g. B. water glass, suffice for the alkaline chromate solutions - to to reduce the chromium content remarkably and to produce colorless protective layers. The values given below apply to layers, those in soda soda solutions same composition. -with and @ without addition yön o, o6o / a water glass made would.

_bleche Die auf durch - i m' io walzharten Minuten langes Reinaluminium-. Eintauchen. gebildete Schichtsubstanz enthält: Wie aus der Gegenüberstellung hervorgeht, ist der Angriff der Lösung auf das Aluminium durch den Zusatz von Wasserglas igtwas abgeschwächt worden. Es ist im Verhältnis zum Aluminiumgehalt weniger Chrom einge- baut worden als in der grauen Schicht. Diese *,'atsäche deutet darauf hin, daß durch deri Ztg.sät@ von Wasserglas die Hydrolyse des zu- , clist entstehenden Natriumaluminats be- schleunigt 3vird. ._Bleche die on through - in the 'io rolling minutes long pure aluminum -. Immersion. formed layer substance contains: As can be seen from the comparison, the attack of the solution on the aluminum has been weakened somewhat by the addition of water glass. There is less chromium in relation to the aluminum content. has been built as in the gray layer. These *, 'atsache indicates that by deri Ztg.sät @ of water glass the hydrolysis of the , clist of the resulting sodium aluminate accelerates 3vird. .

Die durch: das neue Verfahren erhaltenen Schutzschichten weisen einen hohen Widerstand . gegen chemische und atmosphärische Einflüsse auf: In der nachfolgenden Aufstellung sind einige Ergebnisse von Korrosionsversuchen wiedergegeben. In die Versuche wurden zum Vergleich Bleche einbezogen, die nach dem MBV=Verfahren behandelt worden waren Gewichts- - Werkstoff Zeitdauer Verlust Oberflächenbehandlung Korrosionsmittel . in glms Reinal 99,5 ..... 14 Tage 1,08 keine oxydische Kochsalz- 9g,5 0,41 MBV=Behandlung lösung 30/a NaCl - -99,5 ..... - ' 0,07 farblose Schutzschicht x0/0 B202. Reinal 99,5 ...... 14 Tage- 84 keine Carbidschlarnm 99,5.'.... 5,8 MBV-Behandlung - 99,5 ....:. o,g farblose Schutzschicht Reinal 99,5 ..... 2 Monate ' 0,46 keine Wasserdampf 4ö° C _ 99,5 ..... 0 -- MBV-Behandlung im Kühlturm :. 99,5 ..... o farblose Schutzschicht Duralumin weich 14 Tage 2,9o walzblank oxydische Kochsalz- desgl. 0,07 farblose Schutzschicht lösung Duralumin weich x4 Tage 90,5 walzblank Carbidschlamm desgl. . 0,92 farblose Schutzschicht ' Nach den bisherigen Versuchen ist das Verfahren am wirtschaftlichsten, wenn man das 'gleiche Verhältnis von Soda : Natriummonochromat wählt wie bei der MBV-Behandlung. Ausführungsbeispiel 6o g eines Salzgemisches von 5 Teilen Soda und 1,5 Teilen Natriummonochromat werden in i 1 Wasser gelöst: Die Lösung wird auf 95 bis ioo° C erhitzt und mit o,o6 g Wasserglas, NaQ Si. 05. -J-- HZ O, versetzt. Der Aluminiumgegenstand wird 8 bis to Minuten lang eingetaucht und anschließend-15 Minuten lang in aa/oiger Wassetglaslösung ausgekocht.The protective layers obtained by: the new process have a high resistance. against chemical and atmospheric influences on: The following list shows some results of corrosion tests. For comparison, the tests included metal sheets that had been treated according to the MBV method Weight - Material Duration Loss Surface treatment Corrosion agent . in glms Reinal 99.5 ..... 14 days 1.08 no oxidic salt 9g, 5 0.41 MBV = treatment solution 30 / a NaCl - -99.5 ..... - ' 0.07 colorless protective layer x0 / 0 B202. Reinal 99.5 ...... 14 days- 84 no carbide slips 99.5 .'.... 5.8 MBV treatment - 99.5 ....:. o, g colorless protective layer Reinal 99.5 ..... 2 months' 0.46 no water vapor 40 ° C _ 99.5 ..... 0 - MBV treatment in the cooling tower :. 99.5 ..... o colorless protective layer Duralumin soft 14 days 2.9o brightly rolled oxidic table salt the same. 0.07 colorless protective layer solution Duralumin soft x4 days 90.5 bright-rolled carbide slurry the same. 0.92 colorless protective layer ' According to previous attempts, the process is most economical if one chooses the same ratio of soda: sodium monochromate as in the MBV treatment. Embodiment 60 g of a salt mixture of 5 parts of soda and 1.5 parts of sodium monochromate are dissolved in 1 liter of water: The solution is heated to 95 to 100 ° C. and 0.06 g of water glass, NaQ Si. 05. -J-- HZ O, offset. The aluminum object is immersed for 8 to 10 minutes and then boiled for 15 minutes in a / o water glass solution.

Claims (1)

PATENTANSPRUCH: Verfahren zur Erzeugung einer transparenten, hellen Schutzschicht auf Aluminium und Aluminiumlegierungen auf rein chemischem Wege in alkalischen, chromathaltigen Lösungen; dadurch gekennzeichnet, daß diesen Lösungen Wasserglas oder andere Silicate in Mengen bis zu 2 g11 zugesetzt werden.PATENT CLAIM: Process for producing a transparent, bright Protective layer on aluminum and aluminum alloys in a purely chemical way alkaline, chromate-containing solutions; characterized in that these solutions Water glass or other silicates can be added in amounts up to 2 g11.
DE1937V0034008 1937-07-13 1937-07-13 Process for producing a transparent, light protective layer on aluminum and aluminum alloys by chemical means Expired DE691903C (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
DE1937V0034008 DE691903C (en) 1937-07-13 1937-07-13 Process for producing a transparent, light protective layer on aluminum and aluminum alloys by chemical means

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DE1937V0034008 DE691903C (en) 1937-07-13 1937-07-13 Process for producing a transparent, light protective layer on aluminum and aluminum alloys by chemical means

Publications (1)

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DE691903C true DE691903C (en) 1940-06-07

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Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE745043C (en) * 1941-04-25 1944-02-24 Vaw Ver Aluminium Werke Ag Process for the production of enamel-like protective layers on aluminum and its alloys

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE745043C (en) * 1941-04-25 1944-02-24 Vaw Ver Aluminium Werke Ag Process for the production of enamel-like protective layers on aluminum and its alloys

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