CS238467B1 - A method of precipitating sulfate ions from wastewater by adding wastewater from the production of aluminumbenzene-containing ethylbenzene, at a dose corresponding to 0.045-0.36g Al 2+ + 2g per g with concomitant addition of dissolved salt in a dose of 0.2g to 1g. 66 g 2 + 2 - Ca per 1 g 30. The method is suitable for treatment of industrial waters, wastewater and mine water treatment, water finishing in water supply. - Google Patents

A method of precipitating sulfate ions from wastewater by adding wastewater from the production of aluminumbenzene-containing ethylbenzene, at a dose corresponding to 0.045-0.36g Al 2+ + 2g per g with concomitant addition of dissolved salt in a dose of 0.2g to 1g. 66 g 2 + 2 - Ca per 1 g 30. The method is suitable for treatment of industrial waters, wastewater and mine water treatment, water finishing in water supply. Download PDF

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Publication number
CS238467B1
CS238467B1 CS646183A CS646183A CS238467B1 CS 238467 B1 CS238467 B1 CS 238467B1 CS 646183 A CS646183 A CS 646183A CS 646183 A CS646183 A CS 646183A CS 238467 B1 CS238467 B1 CS 238467B1
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Czechoslovakia
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wastewater
per
water
treatment
dose
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CS646183A
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Czech (cs)
Inventor
Jaroslav Jonas
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Jaroslav Jonas
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Priority to CS646183A priority Critical patent/CS238467B1/en
Priority to CS842562A priority patent/CS253313B1/en
Publication of CS238467B1 publication Critical patent/CS238467B1/en

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Abstract

Předmětem vynálezu je příprava sodné soli (E)-3-(hydroxymethylen)-dihydro- -2(3H)-furanonu. Sodná sůl (E)-3-(hydroxymethylen)dihydro-2(3H)-furanonu se podle vynálezu připravuje tak, že se sodná sůl 3-(hydroxymethylen)dihydro-2(3H)-furanonu, rozpustí ve vodě nebo dimethylsulfoxidu nebo dimethylformamidu a rozpouštědlo se odstraní odpařením nebo zeotropní destilaci.The subject of the invention is the preparation of the sodium salt of (E)-3-(hydroxymethylene)-dihydro-2(3H)-furanone. The sodium salt of (E)-3-(hydroxymethylene)dihydro-2(3H)-furanone is prepared according to the invention by dissolving the sodium salt of 3-(hydroxymethylene)dihydro-2(3H)-furanone in water or dimethyl sulfoxide or dimethylformamide and removing the solvent by evaporation or zeotropic distillation.

Description

Předmět vynálezu se týkX^pr/pravy sodné soli (E)-3 -(hydroxymethylen)dihydro-2(3H)-furanonu.The present invention relates to the preparation of (E) -3- (hydroxymethylene) dihydro-2 (3H) -furanone sodium salt.

Sodná sůl 3-(hydroxymethylen)dihydro-2(3H)-furanonu,připravená poprvé Korteni a Machleidtem (Ber.Deut.Chem.Ges.88, 1684 (1955)), je reaktivní nukleofilní činidlo, jehož četné reakce jsou popsány v literatuře. Vzhledem k nevyjasněné konfiguraci této soli vznikají při jejich reakcích obvykle směsi (E) a (Z)-isomerů,kde poměr isomerů ve směsi není dobře reprodukovatelný.3- (hydroxymethylene) dihydro-2 (3H) -furanone sodium, first prepared by Korteni and Machleidt (Ber.Deut.Chem.Ges.88, 1684 (1955)), is a reactive nucleophilic reagent whose numerous reactions are described in the literature . Due to the unclear configuration of this salt, their reactions usually result in mixtures of (E) and (Z) -isomers where the ratio of isomers in the mixture is not well reproducible.

Nyní bylo zjištěno (Jonas J.: Coll.Czech. Chem. Coramun.- v tisku), že sodná sůl 3-{hydroxymethylen)dihydro-2(3H)-furanonu existuje v roztocích pouze ve formě (E)-isomeru a tuto formu lze z roztoků kvantitativně vyisolovat. Sodná sůl (E)-3-(hydroxymethylen)dihydro-2(3H)-furanonu byla charakterisovány C NMR spektry v pevné fázi a IR spektry v nujolu.It has now been found (Jonas J .: Coll.Czech. Chem. Coramun.- in press) that 3- (hydroxymethylene) dihydro-2 (3H) -furanone sodium exists in solutions only in the form of the (E) -isomer and this the form can be quantitatively isolated from the solutions. The (E) -3- (hydroxymethylene) dihydro-2 (3H) -furanone sodium salt was characterized by solid state C NMR and nujol IR spectra.

-2238 467-2238 467

Podle vynálezu byla nalezena příprava čisté sodné soli (E)-3-(hydroxymethylen)dihydro-2(3H)-furanonu vzorce I,According to the invention, the preparation of pure (E) -3- (hydroxymethylene) dihydro-2 (3H) -furanone sodium salt of formula I has been found,

ON aON a

I která umožňuje použít k nukleofilním reakcím konfiguračně čistou sloučeninu I a dovoluje připravit čisté deriváty (E)-3-(hydroxymethylen)dihydro-2(3H)-furanonu, na př, sulfonáty neb?» karboxyláty. Sloučeninu vzorce I lze připravit rozpuštěním sodné soli 3-(hydroxymethylen)dihydro-2(3H)-furanonu na př. ve vodě nebo v dimethylsulfoxidu nebo v dimethyKormamidu a odstraněním rozpouštědla oddestilováním nebo azeotropním oddestilováním.I which allows the use of a configurationally pure compound I for nucleophilic reactions and allows the preparation of pure (E) -3- (hydroxymethylene) dihydro-2 (3H) -furanone derivatives, for example sulfonates or carboxylates. The compound of formula (I) may be prepared by dissolving 3- (hydroxymethylene) dihydro-2 (3H) -furanone sodium salt, for example, in water or dimethylsulfoxide or dimethylformamide and removing the solvent by distillation or azeotropic distillation.

PříkladExample

Sodná sůl 3-(hydroxymethylen)dihydro-2 (3H)-furanonu byla rozpuštěna ve vodě nebo ▼ dimethylsulfoxidu nebo v dimethylformaraidu. Vzniklý roztok sodné soli (E)-3-(hydroxymethylen)dihydro-2(3H)-furanonu lze přímo použít k reakcím nebo sloučeninu vzorce I vyisolovat v pevném stavu odpařením rozpouštědla za atmosferického nebo sníženého tlaku nebo azeotropní destilací. Sodná sůl (E)-3-(hydroxymethylen)dihydro-2(3H)-furanonu vykazuje signály C při NUň v pevném stavu při 180.9, 175^7, 92,2, 25,1 a 64,8 ppm vzhledem k tetramethylsilanu jako vnitřnímu standardu.The sodium salt of 3- (hydroxymethylene) dihydro-2 (3H) -furanone was dissolved in water or dimethylsulfoxide or dimethylformaraid. The resulting (E) -3- (hydroxymethylene) dihydro-2 (3H) -furanone sodium salt solution can be directly used for the reactions or the compound of formula I can be isolated in the solid state by evaporation of the solvent under atmospheric or reduced pressure or by azeotropic distillation. The (E) -3- (hydroxymethylene) dihydro-2 (3H) -furanone sodium salt shows solid state C signals at 180.9, 175-7, 92.2, 25.1 and 64.8 ppm relative to tetramethylsilane as internal standard.

Claims (1)

Ρ δ £ D M Ě T VYNÁLEZUΡ δ £ D MEASURE OF THE INVENTION 238 467238 467 Způsob přípravy sodné soli (E)-3-(hydroxymethylen)dihydro 2(3H)-furanonu vzorce I vyznačený tím, že se sodná sůl 3-(hydroxymethylen)dihydro 2 (3H)-furanonu rozpustí ve vodě nebo dimethylsulfoxidu nebo dimethylformamidu a rozpouštědlo se odstraní odpařením nebo azeotropní destilací.A process for the preparation of (E) -3- (hydroxymethylene) dihydro 2 (3H) -furanone sodium salt of formula I, characterized in that the sodium salt of 3- (hydroxymethylene) dihydro 2 (3H) -furanone is dissolved in water or dimethylsulfoxide or dimethylformamide and a solvent. are removed by evaporation or azeotropic distillation.
CS646183A 1983-09-05 1983-09-05 A method of precipitating sulfate ions from wastewater by adding wastewater from the production of aluminumbenzene-containing ethylbenzene, at a dose corresponding to 0.045-0.36g Al 2+ + 2g per g with concomitant addition of dissolved salt in a dose of 0.2g to 1g. 66 g 2 + 2 - Ca per 1 g 30. The method is suitable for treatment of industrial waters, wastewater and mine water treatment, water finishing in water supply. CS238467B1 (en)

Priority Applications (2)

Application Number Priority Date Filing Date Title
CS646183A CS238467B1 (en) 1983-09-05 1983-09-05 A method of precipitating sulfate ions from wastewater by adding wastewater from the production of aluminumbenzene-containing ethylbenzene, at a dose corresponding to 0.045-0.36g Al 2+ + 2g per g with concomitant addition of dissolved salt in a dose of 0.2g to 1g. 66 g 2 + 2 - Ca per 1 g 30. The method is suitable for treatment of industrial waters, wastewater and mine water treatment, water finishing in water supply.
CS842562A CS253313B1 (en) 1983-09-05 1984-04-03 Process for preparing (Z) -3- (hydroxymethylene) -dihydro-2 (3H) -furanone sodium salt

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CS646183A CS238467B1 (en) 1983-09-05 1983-09-05 A method of precipitating sulfate ions from wastewater by adding wastewater from the production of aluminumbenzene-containing ethylbenzene, at a dose corresponding to 0.045-0.36g Al 2+ + 2g per g with concomitant addition of dissolved salt in a dose of 0.2g to 1g. 66 g 2 + 2 - Ca per 1 g 30. The method is suitable for treatment of industrial waters, wastewater and mine water treatment, water finishing in water supply.

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CS238467B1 true CS238467B1 (en) 1985-11-13

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CS646183A CS238467B1 (en) 1983-09-05 1983-09-05 A method of precipitating sulfate ions from wastewater by adding wastewater from the production of aluminumbenzene-containing ethylbenzene, at a dose corresponding to 0.045-0.36g Al 2+ + 2g per g with concomitant addition of dissolved salt in a dose of 0.2g to 1g. 66 g 2 + 2 - Ca per 1 g 30. The method is suitable for treatment of industrial waters, wastewater and mine water treatment, water finishing in water supply.
CS842562A CS253313B1 (en) 1983-09-05 1984-04-03 Process for preparing (Z) -3- (hydroxymethylene) -dihydro-2 (3H) -furanone sodium salt

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CS842562A CS253313B1 (en) 1983-09-05 1984-04-03 Process for preparing (Z) -3- (hydroxymethylene) -dihydro-2 (3H) -furanone sodium salt

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