CN114047101B - Optical simulation system and method for representing irregularity degree of particulate matter - Google Patents
Optical simulation system and method for representing irregularity degree of particulate matter Download PDFInfo
- Publication number
- CN114047101B CN114047101B CN202110786218.4A CN202110786218A CN114047101B CN 114047101 B CN114047101 B CN 114047101B CN 202110786218 A CN202110786218 A CN 202110786218A CN 114047101 B CN114047101 B CN 114047101B
- Authority
- CN
- China
- Prior art keywords
- scattering
- module
- light
- measurement
- particle
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Active
Links
- 238000013041 optical simulation Methods 0.000 title claims abstract description 25
- 238000000034 method Methods 0.000 title claims abstract description 15
- 239000013618 particulate matter Substances 0.000 title claims abstract description 14
- 238000005259 measurement Methods 0.000 claims abstract description 69
- 239000011159 matrix material Substances 0.000 claims abstract description 26
- 238000001514 detection method Methods 0.000 claims abstract description 19
- 230000003287 optical effect Effects 0.000 claims abstract description 15
- 238000004364 calculation method Methods 0.000 claims abstract description 8
- 239000002245 particle Substances 0.000 claims description 77
- 230000028161 membrane depolarization Effects 0.000 claims description 43
- 230000008033 biological extinction Effects 0.000 claims description 12
- 239000000443 aerosol Substances 0.000 claims description 9
- 230000001788 irregular Effects 0.000 claims description 9
- 239000012798 spherical particle Substances 0.000 claims description 7
- 238000010521 absorption reaction Methods 0.000 claims description 6
- 230000010287 polarization Effects 0.000 claims description 6
- 238000012360 testing method Methods 0.000 claims description 5
- 230000008569 process Effects 0.000 claims description 4
- 230000001133 acceleration Effects 0.000 claims description 3
- 238000004891 communication Methods 0.000 claims description 3
- 238000012937 correction Methods 0.000 claims description 3
- 230000005484 gravity Effects 0.000 claims description 3
- 238000012512 characterization method Methods 0.000 claims 1
- 238000013100 final test Methods 0.000 claims 1
- 230000007613 environmental effect Effects 0.000 abstract description 4
- 239000003344 environmental pollutant Substances 0.000 abstract description 4
- 238000012544 monitoring process Methods 0.000 abstract description 4
- 231100000719 pollutant Toxicity 0.000 abstract description 3
- 238000012821 model calculation Methods 0.000 abstract 1
- 230000009286 beneficial effect Effects 0.000 description 2
- 230000007423 decrease Effects 0.000 description 2
- 238000012986 modification Methods 0.000 description 2
- 230000004048 modification Effects 0.000 description 2
- 238000003915 air pollution Methods 0.000 description 1
- 238000010586 diagram Methods 0.000 description 1
- 230000000694 effects Effects 0.000 description 1
- 239000000126 substance Substances 0.000 description 1
- 238000002834 transmittance Methods 0.000 description 1
Images
Classifications
-
- G—PHYSICS
- G01—MEASURING; TESTING
- G01N—INVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
- G01N15/00—Investigating characteristics of particles; Investigating permeability, pore-volume or surface-area of porous materials
-
- G—PHYSICS
- G01—MEASURING; TESTING
- G01N—INVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
- G01N15/00—Investigating characteristics of particles; Investigating permeability, pore-volume or surface-area of porous materials
- G01N15/02—Investigating particle size or size distribution
- G01N15/0205—Investigating particle size or size distribution by optical means
- G01N15/0211—Investigating a scatter or diffraction pattern
-
- G—PHYSICS
- G06—COMPUTING; CALCULATING OR COUNTING
- G06F—ELECTRIC DIGITAL DATA PROCESSING
- G06F17/00—Digital computing or data processing equipment or methods, specially adapted for specific functions
- G06F17/10—Complex mathematical operations
- G06F17/16—Matrix or vector computation, e.g. matrix-matrix or matrix-vector multiplication, matrix factorization
Landscapes
- Physics & Mathematics (AREA)
- General Physics & Mathematics (AREA)
- Engineering & Computer Science (AREA)
- Chemical & Material Sciences (AREA)
- Mathematical Physics (AREA)
- Computational Mathematics (AREA)
- Mathematical Analysis (AREA)
- General Health & Medical Sciences (AREA)
- Analytical Chemistry (AREA)
- Immunology (AREA)
- Pathology (AREA)
- Life Sciences & Earth Sciences (AREA)
- Health & Medical Sciences (AREA)
- Theoretical Computer Science (AREA)
- Biochemistry (AREA)
- Mathematical Optimization (AREA)
- Dispersion Chemistry (AREA)
- Pure & Applied Mathematics (AREA)
- Data Mining & Analysis (AREA)
- Algebra (AREA)
- Databases & Information Systems (AREA)
- Software Systems (AREA)
- General Engineering & Computer Science (AREA)
- Computing Systems (AREA)
- Investigating Or Analysing Materials By Optical Means (AREA)
Abstract
The invention provides an optical simulation system and method for representing the degree of irregularity of particulate matter, which relate to the technical field of atmospheric monitoring and comprise an incident light module, a scattering measurement cavity and an intensity detection module; the incident light module, the scattering measurement cavity and the intensity detection module are coaxially arranged; the scattering measurement intracavity is provided with forward scattering light measurement module and backscattered light and moves back partial ratio measurement module, forward scattering light measurement module with backscattered light moves back partial ratio measurement module and laser emission direction and is the angle setting. The invention designs the position of the optical lens reasonably distributed through strict T-Matrix optical model calculation, and ensures higher instrument signal-to-noise ratio through repeated measurement and calculation in a laboratory. Through establishing reasonable lens group arrangement order, adopt collimating lens and condensing lens's combination, reach real-time, effectively survey the design target of environmental particulate matter irregularity degree to transmit data into remote monitoring center in real time, improved atmospheric pollutants irregularity degree detection level to a certain extent.
Description
Technical Field
The invention relates to the technical field of atmospheric environment real-time monitoring, in particular to an optical simulation system and method for representing the irregularity degree of particulate matters.
Background
At present, the monitoring on air pollution particles mainly focuses on properties such as concentration, chemical components and the like. The real-time monitoring of the depolarization property of the single particulate matter is less, the irregularity degree of the environmental particulate matter is difficult to detect, and the judgment and judgment of the environmental pollutants are inaccurate. At present, related commercial instruments are lacked, and instruments and equipment for representing the irregularity degree of particles at present have great deviation on finally obtained data due to the lack of scientific guidance for selecting the detection angle of scattered light. Therefore, the angle of the incident laser line deviation is adjusted according to the particle characteristics with different regularity in the current urgent need, the optimal incident angle and position are determined according to the information such as the focal length of the lens system, and then the light intensity information of different vibration directions in the backscattering laser of the particles is obtained by the high-light-transmittance optical splitter, so that the precise calibration work of the lens system and the laser is carried out.
Disclosure of Invention
The invention aims to provide an optical simulation system and method for representing the irregularity degree of particulate matters, so as to solve the problems in the prior art.
In order to achieve the purpose, the technical scheme adopted by the invention is as follows:
an optical simulation system for representing the irregularity degree of particulate matter comprises an incident light module, a scattering measurement cavity and an intensity detection module; the incident light module, the scattering measurement cavity and the intensity detection module are coaxially arranged;
the scattering measurement intracavity is provided with forward scattering light measurement module and backscattered light and moves back partial ratio measurement module, forward scattering light measurement module with backscattered light moves back partial ratio measurement module and laser emission direction and is the angle setting.
Preferably, the arrangement direction of the forward scattering light measurement module forms an included angle of 45 degrees with the laser emission direction;
the setting direction of the backward scattering light depolarization ratio measuring module and the laser emission direction form an included angle of 135 degrees.
Preferably, an aerosol particle beam inlet is further arranged in the scatterometry cavity, and the inlet is arranged between the forward scattered light measurement module and the backward scattered light depolarization ratio measurement module and is used for placing an aerosol particle beam to be measured into the scatterometry cavity.
Preferably, the optical simulation system further comprises a data acquisition processor, a remote monitoring center and a power module, wherein the power module is respectively connected with the incident light module, the forward scattering light measuring module, the backward scattering light depolarization ratio measuring module and the laser intensity detecting module, and the data acquisition processor is respectively connected with the forward scattering light measuring module, the backward scattering light depolarization ratio measuring module and the laser intensity detecting module;
the remote monitoring center is in communication with the data acquisition processor.
Preferably, the forward scattering light measuring module is connected with the data acquisition processor through a deconcentrator, and the backward scattering light depolarization ratio measuring module is connected with the laser intensity detecting module.
Preferably, the forward scattering light measurement module comprises two sets of symmetrically arranged forward scattering measurement optical paths, each measurement optical path comprises a lens group and a photomultiplier, and the lens groups and the photomultiplier are sequentially arranged to measure the intensity of forward scattering light caused by particles.
Preferably, the backscattered light depolarization ratio measuring module comprises a backscattered light measuring light path which is symmetrically arranged, the backscattered light measuring light path comprises a first plano-convex lens, a second plano-convex lens, a third plano-convex lens, a polarized light splitter, a first photomultiplier and a second photomultiplier, the first plano-convex lens, the polarized light splitter, the second plano-convex lens and the first photomultiplier are sequentially arranged, the third plano-convex lens is arranged between the second photomultiplier and the polarized light splitter, and the two groups of photomultipliers are arranged along the vertical direction.
Another object of the present invention is to provide an optical simulation method for characterizing the irregularity degree of particles, which is characterized by comprising the following steps:
s1, the incident light module emits laser, enters the measurement cavity module, and is intersected with the aerosol particle beam in the measurement cavity module to generate scattering;
s2, allowing the scattered forward scattered light to enter a forward scattered light measuring module for light intensity measurement, allowing the backward scattered light to enter a backward scattered light depolarization ratio measuring module, calculating a depolarization ratio, and representing the irregular degree of the particle shape;
and S3, the data acquisition processor acquires the test results of the forward scattering light measurement module and the backward scattering light depolarization ratio measurement module and transmits the results to a remote control center.
Preferably, the specific calculation process in step S2 is as follows:
s21, according to the key parameter of particle swarm scattering, namely Stokes scattering matrix, considering a small volume element dvThe inner particle group, each randomly oriented and rotationally symmetric, is capable of independent scattering, and has optical properties such as extinction cross section (C) averaged with all the individual particlesext) Scattering cross section (C)sca) And dimensionless Stokes scattering matrix representation, namely:
where Θ is the scattering angle, i.e. the angle between the incident light and the scattered beam; assuming the Stokes vector I of the incident lightincAnd Stokes vector I of scattered lightscaAre both defined relative to the scattering plane (the plane defined by the incident and scattered light), the total scattered light intensity IscaCan be expressed as:
wherein n is0Is the density of the particles, R is the small volume element dvDistance to a viewpoint; the Stokes vector I is defined as a (4 × 1) column function containing four Stokes parameters I, Q, U and V:
of these 8 parameters, 8 are non-zero, and 6 of these 8 parameters are independent parameters, and there is a special relationship between these 6 parameters at scattering angles of 0 and π, as follows:
a2(0)=a3(0),a2(π)=-a3(π),
b1(0)=b2(0)=b1(π)=b2(π)=0,
a4(π)=a1(π)-2a2(π)
f in Stokes scattering matrix11I.e. a1(Θ), a well-known phase function in particle scattering optics, satisfies the following equation:
the parameter g is the symmetry factor of the phase function, positive for forward-scattering particles, negative for backward-scattering particles, 0 for forward-backward symmetric particles of the phase function:
the average absorption cross-section of each particle is defined as the difference between the extinction cross-section and the scattering cross-section,
Cabs=Cext-Csca
for a small volume element, the single scattering albedo is defined as the ratio of the scattering cross-section to the extinction cross-section:
ω=Csca/Cext
s22, solving key parameters in the Stokes matrix by adopting a T-matrix:
considering the case where a planar electromagnetic wave is scattered by a non-spherical particle, the incident field E isincAnd a scattered field EscaUsing spherical vector functions M, respectivelymnAnd NmnUnfolding into the following steps:
wherein R is the radius of the outer spherical surface of the scattering particles; g is gravity acceleration; k is a correction coefficient and has no specific meaning; m and n are the arguments of the spherical function.
In the formula, the scattered wave coefficient pmnAnd QmnCoefficient of incident wave amnAnd bmnLinear correlation, which can be expressed as:
written in matrix form as follows:
a is obtained by solving T matrixmnAnd bmnAnd further calculating the extinction cross section, the scattering cross section, the absorption cross section and the single scattering albedo of the non-spherical particle swarm as follows:
Cabs=Cett-Cxa
the invention has the beneficial effects that:
the optical simulation system is reasonable in structure, the detection angles of 45 degrees in the forward direction and 135 degrees in the backward direction are selected by utilizing the T-maxtrix theory for calculation, the linear relation between the scattering light intensity and the depolarization ratio and the particle size of the particles is observed to be more obvious, and therefore the particle size and the morphology of the particles can be more accurately estimated. Through establishing the combination of reasonable collimating lens and condensing lens, reach the purpose of effectively surveying the irregular degree of environmental particulate matter to transmit data in real time to the remote monitoring center, effectively improved the detection level of atmospheric pollutants physicochemical property.
Drawings
Fig. 1 is a schematic diagram of a basic principle of an optical simulation system in embodiment 1 of the present invention;
FIG. 2 is a schematic view of an external configuration of an optical simulation system in embodiment 1 of the present invention;
FIG. 3 is a graph of the calculated grain depolarization ratio as a function of its aspect ratio and scattering light angle based on a T-matrix optical model according to the present invention;
FIG. 4 is a graph of particle depolarization ratio versus particle aspect ratio at 135 deg. for different complex refractive indices calculated based on the T-matrix optical model of the present invention. (ii) a
Detailed Description
In order to make the objects, technical solutions and advantages of the present invention more apparent, the present invention is further described in detail below with reference to the accompanying drawings. It should be understood that the detailed description and specific examples, while indicating the invention, are intended for purposes of illustration only and are not intended to limit the scope of the invention.
Example 1
An optical simulation system for representing the irregularity degree of particulate matter comprises an incident light module, a scattering measurement cavity and an intensity detection module; the incident light module, the scattering measurement cavity and the intensity detection module are coaxially arranged;
the scattering measurement intracavity is provided with forward scattering light measurement module and backscattered light and moves back partial ratio measurement module, forward scattering light measurement module with backscattered light moves back partial ratio measurement module and laser emission direction and is the angle setting.
In the embodiment, the arrangement direction of the forward scattering light measurement module forms an included angle of 45 degrees with the laser emission direction;
the setting direction of the backward scattering light depolarization ratio measuring module and the laser emission direction form an included angle of 135 degrees.
And an aerosol particle beam inlet is also arranged in the scattering measurement cavity, and the inlet is arranged between the forward scattering light measurement module and the backward scattering light depolarization ratio measurement module and is used for placing an aerosol particle beam to be measured into the scattering measurement cavity.
The optical simulation system in this embodiment further includes a data acquisition processor, a remote monitoring center, and a power module, where the power module is connected to the incident light module, the forward scattered light measurement module, the backward scattered light depolarization ratio measurement module, and the laser intensity detection module, respectively, and the data acquisition processor is connected to the forward scattered light measurement module, the backward scattered light depolarization ratio measurement module, and the laser intensity detection module, respectively;
the remote monitoring center is in communication with the data acquisition processor.
The device is connected with the forward scattering light measuring module, the backward scattering light depolarization ratio measuring module and the laser intensity detecting module through a data acquisition processor and a deconcentrator.
The forward scattering light measurement module in this embodiment includes two sets of forward scattering measurement optical paths that the symmetry set up, the measurement optical path includes a lens group and photomultiplier, lens group and photomultiplier set up in order, measure the forward scattering light intensity that is aroused by the particulate matter.
The backscatter depolarization ratio measuring module in this embodiment includes the backscatter measurement light path that the symmetry set up, the backscatter measurement light path includes first plano-convex lens, second plano-convex lens, third plano-convex lens, polarisation beam splitter, first photomultiplier and second photomultiplier, first plano-convex lens the polarisation beam splitter the second plano-convex lens with first photomultiplier sets up in order, the third plano-convex lens sets up the second photomultiplier with between the polarisation beam splitter, and two sets of photomultiplier sets up along the vertical direction.
Example 2
The embodiment provides an optical simulation method for characterizing the irregularity degree of particulate matter, which adopts the optical simulation system described in embodiment 1, and includes the following steps:
s1, the incident light module emits laser, enters the measurement cavity module, and is intersected with the aerosol particle beam in the measurement cavity module to generate scattering;
s2, allowing the scattered forward scattered light to enter a forward scattered light measuring module for light intensity measurement, allowing the backward scattered light to enter a backward scattered light depolarization ratio measuring module, calculating a depolarization ratio, and representing the irregular degree of the particle shape;
and S3, the data acquisition processor acquires the test results of the forward scattering light measurement module and the backward scattering light depolarization ratio measurement module and transmits the results to a remote control center.
In this embodiment, the specific calculation process in step S2 is as follows:
the specific calculation process in step S2 is as follows:
s21, according to the key parameter of particle swarm scattering, namely Stokes scattering matrix, considering a small volume element dvThe inner particle group, each randomly oriented and rotationally symmetric, is capable of independent scattering, and has optical properties such as extinction cross section (C) averaged with all the individual particlesext) Scattering cross section (C)sca) And dimensionless Stokes scattering matrix representation, namely:
where Θ is the scattering angle, i.e. the angle between the incident light and the scattered beam; assuming the Stokes vector I of the incident lightincAnd Stokes vector I of scattered lightscaAre both defined relative to the scattering plane (the plane defined by the incident and scattered light), the total scattered light intensity IscaCan be expressed as:
wherein n is0Is the density of the particles, R is the small volume element dvDistance to a viewpoint; the Stokes vector I is defined as a (4 × 1) column function containing four Stokes parameters I, Q, U and V:
of these 8 parameters, 8 are non-zero, and 6 of these 8 parameters are independent parameters, and there is a special relationship between these 6 parameters at scattering angles of 0 and π, as follows:
a2(0)=a3(0),a2(π)=-a3(π),
b1(0)=b2(0)=b1(π)=b2(π)=0,
a4(π)=a1(π)-2a2(π)
f in Stokes scattering matrix11I.e. a1(Θ), a well-known phase function in particle scattering optics, satisfies the following equation:
the parameter g is the symmetry factor of the phase function, positive for forward-scattering particles, negative for backward-scattering particles, 0 for forward-backward symmetric particles of the phase function:
the average absorption cross-section of each particle is defined as the difference between the extinction cross-section and the scattering cross-section,
Cabs=Cext-Csca
for a small volume element, the single scattering albedo is defined as the ratio of the scattering cross-section to the extinction cross-section:
ω=Csca/Cext
solving key parameters in the Stokes matrix by adopting a T-matrix:
considering the case where a planar electromagnetic wave is scattered by a non-spherical particle, the incident field E isincAnd a scattered field EscaUsing spherical vector functions M, respectivelymnAnd NmnUnfolding into the following steps:
wherein R is the radius of the outer spherical surface of the scattering particles; g is gravity acceleration; k is a correction coefficient and has no specific meaning; m and n are the arguments of the spherical function.
In the formula, the scattered wave coefficient pmnAnd QmnCoefficient of incident wave amnAnd bmnLinear correlation, which can be expressed as:
written in matrix form as follows:
after the T matrix is solved, parameters such as an extinction cross section, a scattering cross section, an absorption cross section, a single scattering albedo and the like of the non-spherical particles can be calculated, so that the irregular degree of the particle morphology is represented;
Cabs=Cett-Cxa
the irregular particles are detected by the system and the method, irregular parameters are obtained through T-maxtrix theoretical calculation, and the results are shown in fig. 3 and fig. 4, wherein in fig. 3, the depolarization ratio (delta) of the scattered light of the particles is obtained when infrared light (1024nm) irradiates the particles with different shapes at different scattering angles. Obviously, although the polarization degree of each particle is different, the distribution of the patterns is approximately similar, and the depolarization ratio (delta) is almost 0 within the scattering angle of 0 DEG to 90 DEG, taking the scattering result of 10 mu m particles as an example; in the range of 90 degrees to 180 degrees, the depolarization ratio increases and then decreases along with the increase of the irregularity of the particles, and the aspect ratio (lambda) when the depolarization ratio (delta) reaches the peak value decreases along with the increase of the scattering angle, which is more obvious for large particles (the particle size is more than 2.5 mu m). From this, we conclude that: the depolarization ratio (delta) shows great difference when different particle shapes exist, the scattering polarization characteristic of single non-spherical particles is not eliminated by the random effect of particle groups, and therefore, the particle scattering polarization distribution is influenced by the shapes of the particles and can be used as a detection index of the particle morphology in atmospheric detection.
Fig. 4 is a graph of a relationship between a particle depolarization ratio and a particle aspect ratio at 135 ° when different complex refractive indexes are calculated based on a T-matrix optical model, where the abscissa in the graph is the depolarization ratio and the ordinate is an irregular parameter — the particle aspect ratio, and according to the graph, only the detected depolarization ratio value at a forward scattering angle of 45 ° is substituted, and the corresponding aspect ratio is found to obtain the degree of irregularity of the particles.
By adopting the technical scheme disclosed by the invention, the following beneficial effects are obtained:
the optical simulation system is reasonable in structure, the detection angles of 45 degrees in the forward direction and 135 degrees in the backward direction are selected by utilizing the T-maxtrix theory for calculation, the linear relation between the scattering light intensity and the depolarization ratio and the particle size of the particles is observed to be more obvious, and therefore the particle size and the morphology of the particles can be more accurately estimated. Through establishing the combination of reasonable collimating lens and condensing lens, reach the purpose of effectively surveying the irregular degree of environmental particulate matter to transmit data in real time to the remote monitoring center, effectively improved the detection level of atmospheric pollutants physicochemical property.
The foregoing is only a preferred embodiment of the present invention, and it should be noted that, for those skilled in the art, various modifications and improvements can be made without departing from the principle of the present invention, and such modifications and improvements should also be considered within the scope of the present invention.
Claims (7)
1. An optical simulation system for representing the irregularity degree of particulate matter is characterized by comprising an incident light module, a scattering measurement cavity, an intensity detection module, a data acquisition processor, a remote monitoring center and a power module; the incident light module, the scattering measurement cavity and the intensity detection module are coaxially arranged;
a forward scattering light measuring module and a backward scattering light depolarization ratio measuring module are arranged in the scattering measuring cavity, and the forward scattering light measuring module and the backward scattering light depolarization ratio measuring module are arranged at an angle with the laser emission direction;
the power supply module is respectively connected with the incident light module, the forward scattered light measuring module, the backward scattered light depolarization ratio measuring module and the laser intensity detecting module, and the data acquisition processor is respectively connected with the forward scattered light measuring module, the backward scattered light depolarization ratio measuring module and the laser intensity detecting module;
the remote monitoring center is in communication connection with the data acquisition processor;
the method for performing optical simulation of the particle irregularity characterization by using the optical simulation system comprises the following steps:
s1, the incident light module emits laser, enters the measurement cavity module, and is intersected with the aerosol particle beam in the measurement cavity module to generate scattering;
s2, enabling the forward scattered light after scattering to enter a forward scattered light measuring module, measuring the light intensity by the forward scattered light measuring module, enabling the backward scattered light to enter a backward scattered light depolarization ratio measuring module, calculating a depolarization ratio, and representing the irregular degree of the particle morphology;
s3, the data acquisition processor acquires the test results of the forward scattering light measurement module test and the backward scattering light depolarization ratio measurement module, and transmits the test results to a remote control center;
the specific calculation process in step S2 is as follows:
s21, according to the key parameter of particle swarm scattering, namely Stokes scattering matrix, considering a small volume element dvThe inner particle group, each of which is randomly oriented and rotationally symmetric, is capable of independent scattering, and the optical properties of which can be averaged by the extinction cross section C of all the individual particle groupsextScattering cross section CscaAnd dimensionless Stokes scattering matrix representation, namely:
where Θ is the scattering angle, i.e. the angle between the incident light and the scattered beam, assuming the Stokes vector I of the incident lightincAnd Stokes vector I of scattered lightscaAre all defined relative to the scattering plane, the total scattered light intensity IscaExpressed as:
wherein n is0Is the particle density and R is the small volume element dvThe Stokes vector I is defined as a 4 × 1 column function, including four Stokes parameters I, Q, U, and V:
of these 8 parameters, 8 are non-zero, and 6 of these 8 parameters are independent parameters, and there is a special relationship between these 6 parameters at scattering angles of 0 and π, as follows:
a2(0)=a3(0),a2(π)=-a3(π),
b1(0)=b2(0)=b1(π)=b2(π)=0,
a4(π)=a1(π)-2a2(π).
f in Stokes scattering matrix11I.e. a1(Θ), a well-known phase function in particle scattering optics, satisfies the following equation:
the parameter g is the symmetry factor of the phase function, positive for forward-scattering particles, negative for backward-scattering particles, 0 for forward-backward symmetric particles of the phase function:
the average absorption cross-section of each particle is defined as the difference between the extinction cross-section and the scattering cross-section,
Cabs=Cext-Csca
for a small volume element, the single scattering albedo is defined as the ratio of the scattering cross-section to the extinction cross-section:
ω=Csca/Cext
s22, calculating the T-matrix solving method of the key parameters in the Stokes matrix by adopting the T-matrix solving method:
considering the case where a planar electromagnetic wave is scattered by a non-spherical particle, the incident field (E) isinc) And a scattered field (E)sca) Using spherical vector functions M, respectivelymnAnd NmnUnfolding into the following steps:
wherein R is the radius of the outer spherical surface of the scattering particles; g is gravity acceleration; k is a correction coefficient and has no specific meaning; m and n are independent variables of the spherical function;
in the formula (1), the scattered wave coefficient pmnAnd QmnCoefficient of incident wave amnAnd bmnLinear correlation, which can be expressed as:
written in matrix form as follows:
a is obtained by solving T matrixmnAnd bmnAnd further calculating the extinction cross section, the scattering cross section, the absorption cross section and the single scattering albedo of the non-spherical particle swarm as follows:
Cabs=Cett-Cxa
2. the optical simulation system of claim 1, wherein the forward scattering light measurement module is disposed at an angle of 45 ° to the laser emission direction;
the setting direction of the backward scattering light depolarization ratio measuring module and the laser emission direction form an included angle of 135 degrees.
3. The optical simulation system of claim 1, wherein an aerosol particle beam inlet is further disposed in the scatterometry cavity, the inlet being disposed intermediate the forward scattered light measurement module and the backscattered light depolarization measurement module for introducing an aerosol particle beam to be measured into the scatterometry cavity.
4. The optical simulation system of claim 2, wherein the forward scattered light measurement module, the backward scattered light depolarization ratio measurement module and the laser intensity detection module are connected through a splitter by a data acquisition processor.
5. The optical simulation system of claim 1, wherein the forward scattering light measurement module comprises two symmetrically arranged sets of forward scattering measurement paths, the measurement paths comprising a lens set and a photomultiplier tube, the lens set and the photomultiplier tube being arranged in series to measure the intensity of forward scattering light caused by particulate matter.
6. The optical simulation system of claim 1, wherein the backscattered light depolarization ratio measurement module comprises a symmetrically arranged backscatter measurement optical path, the backscatter measurement optical path comprising a first plano-convex lens, a second plano-convex lens, a third plano-convex lens, a polarization beam splitter, a first photomultiplier tube, and a second photomultiplier tube, the first plano-convex lens, the polarization beam splitter, the second plano-convex lens, and the first photomultiplier tube being arranged in sequence, the third plano-convex lens being arranged between the second photomultiplier tube and the polarization beam splitter, and both sets of photomultiplier tubes being arranged in a vertical direction.
7. The optical simulation system of claim 1, wherein the final test result in step S3 is a depolarization ratio at a forward scattering angle of 45 °.
Priority Applications (1)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
CN202110786218.4A CN114047101B (en) | 2021-07-12 | 2021-07-12 | Optical simulation system and method for representing irregularity degree of particulate matter |
Applications Claiming Priority (1)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
CN202110786218.4A CN114047101B (en) | 2021-07-12 | 2021-07-12 | Optical simulation system and method for representing irregularity degree of particulate matter |
Publications (2)
Publication Number | Publication Date |
---|---|
CN114047101A CN114047101A (en) | 2022-02-15 |
CN114047101B true CN114047101B (en) | 2022-06-10 |
Family
ID=80204498
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
CN202110786218.4A Active CN114047101B (en) | 2021-07-12 | 2021-07-12 | Optical simulation system and method for representing irregularity degree of particulate matter |
Country Status (1)
Country | Link |
---|---|
CN (1) | CN114047101B (en) |
Citations (9)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
CN101566551A (en) * | 2008-04-25 | 2009-10-28 | 宇星科技发展(深圳)有限公司 | Backscattering smoke analyzer |
EP2243420A1 (en) * | 2009-04-24 | 2010-10-27 | Schmidt-Erfurth, Ursula | Method for determining exudates in the retina |
CN103278440A (en) * | 2013-05-14 | 2013-09-04 | 桂林优利特医疗电子有限公司 | Cell scattered light multi-position detecting method as well as cell analyzer |
CN103714646A (en) * | 2013-12-18 | 2014-04-09 | 公安部第三研究所 | Optical-polarization pressure-type intrusion alarm floor |
CN107478617A (en) * | 2017-09-04 | 2017-12-15 | 中国计量大学 | Long-range underground water multi-parameter online test method and measurement apparatus |
AU2017203205B1 (en) * | 2017-05-12 | 2018-08-02 | Australian National University | Frequency conversion of electromagnetic radiation |
CN109061668A (en) * | 2018-06-25 | 2018-12-21 | 南京信息工程大学 | A kind of more visual field polarization lidar detection systems and the method for detecting ice cloud |
CN109491038A (en) * | 2017-09-12 | 2019-03-19 | 北京维天信气象设备有限公司 | A kind of the focal length self-checking device and method of optical system of laser ceilometer |
CN113029342A (en) * | 2021-04-02 | 2021-06-25 | 西北工业大学 | Bidirectional reflection theory-based simulation method for polarized light reflected by underwater target |
Family Cites Families (7)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US8125648B2 (en) * | 2006-06-05 | 2012-02-28 | Board Of Regents, The University Of Texas System | Polarization-sensitive spectral interferometry |
CN101435761A (en) * | 2008-12-18 | 2009-05-20 | 任中京 | Sample pool for testing graininess of granule |
US8736826B2 (en) * | 2012-01-20 | 2014-05-27 | Norscan Instruments Ltd. | Monitoring for disturbance of optical fiber |
CN207248733U (en) * | 2017-09-04 | 2018-04-17 | 杭州职业技术学院 | A kind of underground water multi-parameter on-line measuring device |
CN208334194U (en) * | 2018-06-15 | 2019-01-04 | 北京华科仪科技股份有限公司 | A kind of light channel structure measuring high range turbidity |
CN110907316A (en) * | 2019-12-16 | 2020-03-24 | 中国科学院大气物理研究所 | Light path system for single particle forward and backward scattering and depolarization ratio measurement |
CN112782121B (en) * | 2020-12-25 | 2023-09-19 | 中国科学院合肥物质科学研究院 | Multi-angle optical particle counting and refractive index online measuring device and method |
-
2021
- 2021-07-12 CN CN202110786218.4A patent/CN114047101B/en active Active
Patent Citations (9)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
CN101566551A (en) * | 2008-04-25 | 2009-10-28 | 宇星科技发展(深圳)有限公司 | Backscattering smoke analyzer |
EP2243420A1 (en) * | 2009-04-24 | 2010-10-27 | Schmidt-Erfurth, Ursula | Method for determining exudates in the retina |
CN103278440A (en) * | 2013-05-14 | 2013-09-04 | 桂林优利特医疗电子有限公司 | Cell scattered light multi-position detecting method as well as cell analyzer |
CN103714646A (en) * | 2013-12-18 | 2014-04-09 | 公安部第三研究所 | Optical-polarization pressure-type intrusion alarm floor |
AU2017203205B1 (en) * | 2017-05-12 | 2018-08-02 | Australian National University | Frequency conversion of electromagnetic radiation |
CN107478617A (en) * | 2017-09-04 | 2017-12-15 | 中国计量大学 | Long-range underground water multi-parameter online test method and measurement apparatus |
CN109491038A (en) * | 2017-09-12 | 2019-03-19 | 北京维天信气象设备有限公司 | A kind of the focal length self-checking device and method of optical system of laser ceilometer |
CN109061668A (en) * | 2018-06-25 | 2018-12-21 | 南京信息工程大学 | A kind of more visual field polarization lidar detection systems and the method for detecting ice cloud |
CN113029342A (en) * | 2021-04-02 | 2021-06-25 | 西北工业大学 | Bidirectional reflection theory-based simulation method for polarized light reflected by underwater target |
Non-Patent Citations (3)
Title |
---|
Solutions of navier-stokes equation with coriolis force;Lee Sunggeun 等;《ADVANCE IN MATHEMATICAL PHYSICS》;20170907;第2017卷;1-10 * |
可见光波段非球形沙尘气溶胶散射和辐射特性的理论模拟;冯倩 等;《大气与环境光学学报》;20150210;第10卷(第1期);1-10 * |
煤粉燃烧中碳黑颗粒的辐射特性计算研究;童世唯;《中国优秀硕士学位论文全文数据库》;20140715(第7期);B017-11 * |
Also Published As
Publication number | Publication date |
---|---|
CN114047101A (en) | 2022-02-15 |
Similar Documents
Publication | Publication Date | Title |
---|---|---|
Nakayama et al. | Characterization of a three wavelength photoacoustic soot spectrometer (PASS-3) and a photoacoustic extinctiometer (PAX) | |
CN103454203B (en) | Real-time online measurement system and method of particle size and chemical components of atmospheric particulate | |
Sakai et al. | Backscattering linear depolarization ratio measurements of mineral, sea-salt, and ammonium sulfate particles simulated in a laboratory chamber | |
CN102636459B (en) | Forward scattering and transmission combined visibility measuring instrument and measuring method thereof | |
CN106295505A (en) | State estimating system during pavement usage | |
CN106018193A (en) | Light scattering measurement system and method for particulate matters | |
Nakagawa et al. | Design and characterization of a novel single-particle polar nephelometer | |
Wang et al. | A light-scattering study of the scattering matrix elements of Arizona Road Dust | |
Arends et al. | Comparison of techniques for measurements of fog liquid water content | |
CN105044039B (en) | A kind of method according to laser radar data automatic inversion horizontal visibility | |
Deng et al. | Dual-wavelength optical sensor for measuring the surface area concentration and the volume concentration of aerosols | |
US20180059023A1 (en) | Lidar instrument and method of operation | |
CN105092444B (en) | The measuring method of concentrations of nanoparticles and geometric feature Joint Distribution | |
US20150116709A1 (en) | Sensor and method for turbidity measurement | |
CN114047101B (en) | Optical simulation system and method for representing irregularity degree of particulate matter | |
KR20170116805A (en) | Method for retrieving aerosol height using Raman scattering property of atmospheric molecules based on sunlight measurement in multi-angle | |
Mulholland et al. | Radiometric model of the transmission cell-reciprocal nephelometer | |
CN218584995U (en) | Laser divergence angle and pointing stability measuring device for atmospheric pollution detection | |
CN207730938U (en) | A kind of movable type aerosol LIDAR network data quality control system | |
Ding et al. | A method of simultaneously measuring particle shape parameter and aerodynamic size | |
US10950108B2 (en) | Characterization of aerosols | |
CN108844870A (en) | PM based on optical fiber structure10And PM2.5Detection instrument device and system | |
Ji et al. | Calculation and Analysis on Scattering Characteristics of Non-Spherical Particles of Haze | |
Wang et al. | Correlation analysis on light scattering intensity distribution and mass concentration of atmospheric particles in different polarization states | |
Guo et al. | Laser backscattering of multi-scaled large particles based on superimposed scattering |
Legal Events
Date | Code | Title | Description |
---|---|---|---|
PB01 | Publication | ||
PB01 | Publication | ||
SE01 | Entry into force of request for substantive examination | ||
SE01 | Entry into force of request for substantive examination | ||
GR01 | Patent grant | ||
GR01 | Patent grant |