CN110132851A - A kind of instantaneous two-dimensional opto-acoustic wave measurement method based on the interference of femtosecond pulse - Google Patents

A kind of instantaneous two-dimensional opto-acoustic wave measurement method based on the interference of femtosecond pulse Download PDF

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CN110132851A
CN110132851A CN201910539672.2A CN201910539672A CN110132851A CN 110132851 A CN110132851 A CN 110132851A CN 201910539672 A CN201910539672 A CN 201910539672A CN 110132851 A CN110132851 A CN 110132851A
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femtosecond
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CN110132851B (en
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王婧
于连栋
陆洋
赵会宁
蒲松
孙雄鑫
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Hefei University of Technology
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    • GPHYSICS
    • G01MEASURING; TESTING
    • G01JMEASUREMENT OF INTENSITY, VELOCITY, SPECTRAL CONTENT, POLARISATION, PHASE OR PULSE CHARACTERISTICS OF INFRARED, VISIBLE OR ULTRAVIOLET LIGHT; COLORIMETRY; RADIATION PYROMETRY
    • G01J3/00Spectrometry; Spectrophotometry; Monochromators; Measuring colours
    • G01J3/28Investigating the spectrum
    • G01J3/45Interferometric spectrometry
    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N21/00Investigating or analysing materials by the use of optical means, i.e. using sub-millimetre waves, infrared, visible or ultraviolet light
    • G01N21/17Systems in which incident light is modified in accordance with the properties of the material investigated
    • G01N21/1702Systems in which incident light is modified in accordance with the properties of the material investigated with opto-acoustic detection, e.g. for gases or analysing solids

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Abstract

The invention belongs to field of optical measurements, a kind of instantaneous two-dimensional opto-acoustic wave measurement method based on the interference of femtosecond pulse is disclosed, 1) ultrafast imaging system is constructed, realizes that mode locking femto-second laser, acousto-optic pulse selector, pumping pulse, direct impulse are synchronous with cameras frame rate;It is characterized in that, 2) power amplification after femtosecond pulse frequency reducing, the mode locking femtosecond laser of high repetition frequency carries out frequency reducing, and the femtosecond pulse after frequency reducing carries out power amplification;3) photoacoustic waves induction generation module forms photoacoustic waves and filters out light ambient noise;4) it realizes that reference light and the measurement interference of light, reference light carry out high frequency modulated using Mach Zehnder interferometry method, improves interference fringe signal-to-noise ratio;5) pulse interference image is acquired within the single camera exposure time, completes instantaneous two-dimensional opto-acoustic wave measurement using Fourier transformation phase reconstruction algorithm.Using the time synchronization of camera exposure and ultrashort pulse, experiment obtains the ultrafast imaging of subpicosecond magnitude temporal resolution.

Description

A kind of instantaneous two-dimensional opto-acoustic wave measurement method based on the interference of femtosecond pulse
Technical field
The invention belongs to field of optical measurements more particularly to a kind of instantaneous two-dimensional opto-acoustic waves based on the interference of femtosecond pulse Measurement method.
Background technique
Ultrafast laser induction photoacoustic imaging can be used for the non-linear absorption and refracting characteristic research of material, inanimate object The Non-invasive detection of light spectrum image-forming and the damage of sub-surface microelectronics, photoacoustic waves are usually in tiny area with velocity of sound fast propagation, therefore, The photoacoustic waves INSTANTANEOUS OBSERVATION of the big visual field of high lateral resolution is an extremely challenging task, so far, due to lacking The limited one-dimensional piezoelectricity of spatial and temporal resolution or laser vibrometer sensing is usually used in high speed two-dimension sensor, the characterization of photoacoustic waves Device.
High speed camera imaging based on pulsed light reflection or transmitted light can be used to observe quick physical phenomenon, ultrashort arteries and veins The more recent application for rushing laser makes people observe picosecond even ultra-fast optical imaging faster, especially by pumping-spy Surveying experiment may be implemented photon-matter interaction observation.However, being currently available that high speed two-dimension camera is also not enough to carry out skin Second grade pump probe imaging, therefore one-dimensional photodetector is often used, the state-of-the-art photodetector response time has reached several Picosecond.Realize ultrahigh time resolution rate two-dimensional measurement, can by affixed one's name in the middle part of grid is laid out multiple photodetectors or Single photodetector is scanned on target area in order come extend it is one-dimensional detect two-dimensional imaging, but its achievable visual field is not Greatly, and imaging transverse resolution ratio is lower.Simultaneously as the light ambient noise of camera exposure time, is based on short pulse pumping-detection The contrast of imaging is lower, limits the image quality of ultra-fast dynamics, cannot achieve quantitative analysis.
Summary of the invention
The purpose of the present invention is to solve this problems, are based on the ultrafast time domain specification of femtosecond pulse, provide one kind and be based on The temporal resolution of the instantaneous two-dimensional opto-acoustic wave measurement method of femtosecond pulse interference, pulse interference scheme can achieve 250fs is only captured a pulse interference fringe image, while being filtered out using second-harmonic generation in camera each time for exposure Light amplification spontaneous radiation ambient noise, electric light phase-modulation improve striped signal-to-noise ratio, utilize Fourier transformation phase reconstruction algorithm Realize the quantitative measurment of instantaneous two-dimensional opto-acoustic wave.
For achieving the above object, the technical scheme is that
It is a kind of based on femtosecond pulse interference instantaneous two-dimensional opto-acoustic wave measurement method, include the following steps, 1) building fly Second single laser pulse interferes ultrafast imaging system, realizes mode locking femto-second laser, acousto-optic pulse selector, pumping pulse, detection Pulse is synchronous with cameras frame rate;It is characterized in that,
2) power amplification after femtosecond pulse frequency reducing, the mode locking femtosecond laser of high repetition frequency carry out frequency reducing, and to frequency reducing after Femtosecond pulse carry out power amplification;
3) photoacoustic waves induction generation module forms photoacoustic waves, filters out detection light light ambient noise using nonlinear crystal;
4) reference light is realized using Mach Zehnder interferometry method and measures the interference of light, using electrooptic modulator to reference light High frequency modulated is carried out, interference fringe signal-to-noise ratio is improved;
5) instantaneous two-dimensional opto-acoustic wave measurement, pulse interference image is only captured within the single camera exposure time, utilizes Fu In leaf transformation phase reconstruction algorithm complete instantaneous two-dimensional opto-acoustic wave measurement.
Preferably, 5) the collected pulse interference image of camera includes the phase information of photoacoustic waves.
Preferably, the femtosecond pulse interferes instantaneous two-dimensional opto-acoustic wave measuring apparatus, including mode-locked laser frequency reducing to be put Big module 1, photoacoustic waves induction generation module 26 and pulse Mach Zehnder interferometry module 27, from the mode-locked laser frequency reducing The femtosecond pulse of amplification module output is divided into pump light and detection light after frequency reducing is amplified, and the induction of pump light incidence photoacoustic waves produces Raw module photoacoustic waves pass through optical time delay after filtering out detection light light ambient noise using the second-harmonic generation of nonlinear crystal, Incident pulse Mach Zehnder interferometry module 27.
Preferably, the mode-locked laser frequency reducing amplification module 1, including mix ytterbium femtosecond mode-locked laser 2, acousto-optic pulse choosing It selects device 3, mix ytterbium laser amplifier 4, rubidium atomic clock 6 and arbitrary waveform generator 5, the rubidium atomic clock 6 exports sinusoidal signal point It is described to mix ytterbium femtosecond mode-locked laser 2 not as the reference frequency for mixing ytterbium femtosecond mode-locked laser 2 and arbitrary waveform generator 5 Femtosecond laser seed light source is exported, by photoacoustic pulse selector 3,5 output drive signal 7 of arbitrary waveform generator and camera touching Signal 8, driving signal 7 controls the working time window of acousto-optic pulse selector 3, pulse choice is carried out, using mixing ytterbium laser Amplifier 4 carries out power amplification to the femtosecond pulse after frequency reducing;Synchronizing mode-licked femto-second laser repetition rate, acousto-optic pulse choice Device, pumping pulse, direct impulse and cameras frame rate.
Preferably, photoacoustic waves induce generation module 26, including beam splitter prism 9, pump light 10 and microcobjective 11, dichroic Mirror 12, amplified pulsed light are divided into two bundles by beam splitter prism 9, and respectively as pump light 10 and detection light 14, pump light passes through It is focused by microcobjective 11, photoacoustic waves is generated by the incident acetone soln 15 of dichroscope 12.
Preferably, pulse Mach Zehnder interferometry module, including barium metaborate nonlinear crystal 13, delay optical path 16, Bandpass optical filtering device 18, Amici prism 2 23, reflecting mirror 21, electrooptic modulator 20, acetone soln 22, is shown Amici prism 1 Speck mirror 24 and CMOS camera 25 detect light after barium metaborate nonlinear crystal 13 filters out light ambient noise, pass through delay Optical path 16 is reflected into reflecting mirror 17, filters the prism 1 that is split through bandpass optical filtering device 18 and is divided into reference light and measurement light, ginseng It examines light to be reflected after electrooptic modulator 20 is modulated and improves interference fringe signal-to-noise ratio by reflecting mirror 21, passes sequentially through no pumping After the acetone soln 22 of photoinduction, the reflection of Amici prism 2 23 and microcobjective 24, incident CMOS camera 25;It is filtered using band light passing Wave device chooses visible light wave range laser, and the interference image of single pulse is only captured in the single exposure time of CMOS camera.
Compared with prior art, the beneficial effects of the present invention are:
This method of the present invention realizes instantaneous two-dimensional opto-acoustic wave measurement using general camera for the first time.Ultrafast pulse interferometer It is the effective tool of high contrast, ultrafast two-dimensional optical imaging.Utilize camera each time for exposure (1ms) and ultrashort pulse The time synchronization of (0.25ps), experiment obtain the ultrafast imaging of subpicosecond magnitude temporal resolution.With existing Pulse Imageing phase Than nonlinear second harmonic filtering restrained effectively the amplified spontaneous emission in pulse, improve interference fringe signal-to-noise ratio.It is logical It crosses pump probe experiment quantitative measurment 60.8MHz photoacoustic waves to propagate in a liquid, demonstrates two-dimentional ultrahigh speed interference imaging energy Power, this method demonstrate the feasibility of measurement result in acetone soln.It is expected to provide for different photon matter interactions A kind of cost-effective novel ultrafast imaging method.
Detailed description of the invention
The drawings herein are incorporated into the specification and forms part of this specification, and shows and meets implementation of the invention Example, and be used to explain the principle of the present invention together with specification.
Fig. 1 is the structure chart for the instantaneous two-dimensional opto-acoustic wave measurement method interfered the present invention is based on femtosecond pulse.
Fig. 2 is the noise interference that has powerful connections for the instantaneous two-dimensional opto-acoustic wave measurement method interfered the present invention is based on femtosecond pulse Figure.
Fig. 3 is interfering without ambient noise for the instantaneous two-dimensional opto-acoustic wave measurement method interfered the present invention is based on femtosecond pulse Figure.
Fig. 4 is the induced with laser photoacoustic waves for the instantaneous two-dimensional opto-acoustic wave measurement method interfered the present invention is based on femtosecond pulse Without ambient noise interference pattern.
Fig. 5 is the 10ns delay phase weight for the instantaneous two-dimensional opto-acoustic wave measurement method interfered the present invention is based on femtosecond pulse Composition.
Fig. 6 is the 30ns delay phase weight for the instantaneous two-dimensional opto-acoustic wave measurement method interfered the present invention is based on femtosecond pulse Composition.
Specific embodiment
Below in conjunction with attached drawing, technical scheme in the embodiment of the invention is clearly and completely described.
As shown in figures 1 to 6, a kind of instantaneous two-dimensional opto-acoustic wave measurement method based on the interference of femtosecond pulse, including walk as follows Suddenly, 1) building femtosecond laser pulse interferes ultrafast imaging system, reduces the repetition rate of femtosecond pulse, realizes that mode locking femtosecond swashs Light device, acousto-optic pulse selector, pumping pulse, direct impulse are synchronous with cameras frame rate;
2) frequency reducing is carried out using mode locking femtosecond laser of the acousto-optic pulse selector to high repetition frequency, and utilizes and mixes ytterbium laser Amplifier carries out power amplification to the femtosecond pulse after frequency reducing;
3) high power femtosecond pulse is divided into two beams, respectively as pump light and detection light, pump light incidence fluid sample, light Sound wave induces generation module to form photoacoustic waves, filters out detection light light ambient noise using the second-harmonic generation of nonlinear crystal;
4) reference light is realized using Mach Zehnder interferometry method and measures the interference of light, using electrooptic modulator to reference light High frequency modulated is carried out, interference fringe signal-to-noise ratio is improved;
5) instantaneous two-dimensional opto-acoustic wave measurement, using rubidium atomic clock synchronizing mode-licked femto-second laser repetition rate, acousto-optic pulse Selector driving signal and cameras frame rate, using the flight time of optical path delay synchronous pump light and detection light, in single phase The interference image of acquisition capture pulse in the machine time for exposure realizes instantaneous two-dimentional light using Fourier transformation phase reconstruction algorithm Acoustic measurement.
Preferably, 5) the collected pulse interference image of camera includes the phase information of photoacoustic waves.Become using Fourier It changes phase reconstruction algorithm photoacoustic waves are reconstructed, realizes the instantaneous two-dimensional opto-acoustic wave measurement of every width interference pattern, specific algorithm are as follows: The interference strength of point (x, y) can be expressed as I (x, y)=a (x, y)+b (x, y) cos [+2 π f of φ (x, y) in two-dimensional surface0X], A (x, y) and b (x, y) is background light intensity and fringe contrast, f respectively0It is acquired for striped carrier frequency using Fourier transformation Phase (x, y)=tan-1{ Im [c (x, y)]/Re [c (x, y)] }, whereinThen meter is utilized The phase of obtained each pixel reconstructs instantaneous two-dimensional surface photoacoustic waves, temporal resolution 250fs.
Preferably, the femtosecond pulse interferes instantaneous two-dimensional opto-acoustic wave measuring apparatus, including mode-locked laser frequency reducing to be put Big module 1, photoacoustic waves induction generation module 26 and pulse Mach Zehnder interferometry module 27, from the mode-locked laser frequency reducing The femtosecond pulse of amplification module output is divided into pump light and detection two beam of light, pump light incidence sample optoacoustic after frequency reducing is amplified Wave induces generation module to form photoacoustic waves, using the second-harmonic generation of nonlinear crystal, after filtering out detection light light ambient noise By optical time delay, incident pulse Mach Zehnder interferometry module 27;Using rubidium atomic clock as reference frequency, using any Waveform generator generates acousto-optic pulse selector driving signal 7 and camera trigger signal 8, and synchronizing mode-licked femto-second laser repeats frequency Rate, acousto-optic pulse selector, pumping pulse, direct impulse and cameras frame rate, camera, which captures, carries instantaneous two-dimensional opto-acoustic wave Phase information obtains interference fringe, realizes instantaneous two-dimensional opto-acoustic wave measurement using Fourier transformation phase reconstruction algorithm.
As shown in Figure 2 and Figure 3, fringe contrast is increased to 1 from 0.33 using barium metaborate nonlinear crystal by this method.
As shown in figure 3, being interfered using pulse, CMOS camera captures the instantaneous two-dimensional opto-acoustic wave phase information of carrying and must do Relate to striped.
The pulse interference light intensity is represented byWherein τ reference arm The optical time delay between measurement arm, IoFor average intensity,Measurement arm phase caused by photoacoustic waves is generated for pumping photoinduction Delay, γ (τ) are interference contrast function.
As shown in Figure 5,6, the present invention is reconstructed two-dimensional opto-acoustic wave phase, realizes the measurement of instantaneous two-dimensional opto-acoustic wave.
The mode-locked laser frequency reducing amplification module 1, including mix ytterbium femtosecond mode-locked laser 2, acousto-optic pulse selector 3, Ytterbium laser amplifier 4, rubidium atomic clock 6 and arbitrary waveform generator 5, camera trigger signal 8 are mixed, what the rubidium atomic clock 6 exported 10MHz sinusoidal signal provides frequency respectively as the reference frequency for mixing ytterbium femtosecond mode-locked laser 2 and arbitrary waveform generator 5 Benchmark, the ytterbium femtosecond mode-locked laser 2 of mixing export the femtosecond laser seed light source that repetition rate is 100MHz, pass through optoacoustic arteries and veins Selector 3,5 output drive signal 7 of arbitrary waveform generator and camera trigger signal 8 are rushed, driving signal 7 controls acousto-optic pulse choosing The working time window of device 3 is selected, pulse choice is carried out, reduces repetition rate, is flown using ytterbium laser amplifier 4 is mixed to after frequency reducing Pulse per second (PPS) carries out power amplification.Synchronizing mode-licked femto-second laser repetition rate, acousto-optic pulse selector, pumping pulse, detection arteries and veins Punching and cameras frame rate.
Preferably, photoacoustic waves induce module 26, including beam splitter prism 9, pump light 10 and microcobjective 11, dichroscope 12, amplified pulsed light is divided into two bundles by beam splitter prism 9, respectively as pump light 10 and detection light 14, pump light by by Microcobjective 11 focuses, generates photoacoustic waves by the incident acetone soln 15 of dichroscope 12.It is poly- to pump light using microcobjective Coke, by acetone soln incident after dichroscope, induction generates photoacoustic waves.Light is detected to filter by barium metaborate nonlinear crystal 13 After light ambient noise, pass through the optical path 16 that is delayed, incident pulse Mach Zehnder interferometry module 27.
The transforming function transformation function of the electric field energy E of above-mentioned detection light t at any time can be expressed asIts Middle voIndicate that frequency of light wave, I (t) indicate the light wave envelope intensity for meeting Gaussian Profile, herein the half peak height width (pulse of light intensity Width) it is 250fs.
Preferably, pulse Mach Zehnder interferometry module, including barium metaborate nonlinear crystal 13, delay optical path 16, Bandpass optical filtering device 18, Amici prism 2 23, reflecting mirror 21, electrooptic modulator 20, acetone soln 22, is shown Amici prism 1 Speck mirror 24 and CMOS camera 25 detect light after barium metaborate nonlinear crystal 13 filters out light ambient noise, pass through delay Optical path 16 is reflected into reflecting mirror 17, filters the prism 1 that is split through bandpass optical filtering device 18 and is divided into reference light and measurement light, ginseng It examines light to be reflected after electrooptic modulator 20 is modulated and improves interference fringe signal-to-noise ratio by reflecting mirror 21, passes sequentially through no pumping After the acetone soln 22 of photoinduction, the reflection of Amici prism 2 23 and microcobjective 24, incident CMOS camera 25;It measures light and passes through two To after Look mirror reflection, the acetone soln 15 of pumping photoinduction, after Amici prism and microcobjective, incident CMOS phase are passed sequentially through Machine changes measurement light and reference light optical path difference by adjusting the optical path that is delayed;Visible light wave range is chosen using bandpass optical filtering device to swash Light only captures the interference image of single pulse in the single exposure time of CMOS camera.Using nonlinear crystal to filter out detection Light ambient noise realizes pump light using delay optical path and detects the time synchronization of light, utilizes bandpass optical filtering device Selection Center Wavelength is the visible light wave range laser of 532nm, is modulated using electrooptic modulator to reference light, and interference fringe noise is improved Than only capturing the interference image of single pulse in the single exposure time of CMOS camera.
Embodiments described above is only a part of the embodiment of the present invention, instead of all the embodiments.Based on this Embodiment in invention, every other reality obtained by those of ordinary skill in the art without making creative efforts Example is applied, shall fall within the protection scope of the present invention.

Claims (6)

1. a kind of instantaneous two-dimensional opto-acoustic wave measurement method based on the interference of femtosecond pulse, includes the following steps, 1) building femtosecond Single laser pulse interferes ultrafast imaging system, realizes mode locking femto-second laser, acousto-optic pulse selector, pumping pulse, detection arteries and veins It rushes synchronous with cameras frame rate;It is characterized in that,
2) the mode locking femtosecond laser of power amplification after femtosecond pulse frequency reducing, high repetition frequency carries out frequency reducing, the femtosecond arteries and veins after frequency reducing Rush in row power amplification;
3) photoacoustic waves induction generation module forms photoacoustic waves, filters out detection light light ambient noise using nonlinear crystal;
4) reference light is realized using Mach Zehnder interferometry method and measures the interference of light, reference light is carried out using electrooptic modulator High frequency modulated improves interference fringe signal-to-noise ratio;
5) pulse interference image is acquired within the single camera exposure time, completes wink using Fourier transformation phase reconstruction algorithm When two-dimensional opto-acoustic wave measurement.
2. the instantaneous two-dimensional opto-acoustic wave measurement method according to claim 1 based on the interference of femtosecond pulse, it is characterised in that: 5) the collected pulse interference image of camera includes the phase information of photoacoustic waves.
3. the instantaneous two-dimensional opto-acoustic wave measurement method according to claim 1 based on the interference of femtosecond pulse, it is characterised in that: The femtosecond pulse interferes instantaneous two-dimensional opto-acoustic wave measuring apparatus, including mode-locked laser frequency reducing amplification module (1), photoacoustic waves Generation module (26) and pulse Mach Zehnder interferometry module (27) are induced, amplifies mould from the mode locking femto-second laser frequency reducing The seed femtosecond pulse of block output is divided into pump light and detection light after frequency reducing is amplified, and the induction of pump light incidence photoacoustic waves generates Module (26) forms photoacoustic waves;Using the second-harmonic generation of nonlinear crystal, pass through light after filtering out detection light light ambient noise Learn delay, incident pulse Mach Zehnder interferometry module (27).
4. the instantaneous two-dimensional opto-acoustic wave measurement method according to claim 3 based on the interference of femtosecond pulse, it is characterised in that: The mode-locked laser frequency reducing amplification module (1), including mix ytterbium femtosecond mode-locked laser (2), acousto-optic pulse selector (3), mix Ytterbium laser amplifier (4), rubidium atomic clock (6) and arbitrary waveform generator (5) and camera trigger signal (8), the rubidium atomic clock (6) output sinusoidal signal is respectively as the reference frequency for mixing ytterbium femtosecond mode-locked laser (2) and arbitrary waveform generator (5), institute It states and mixes ytterbium femtosecond mode-locked laser (2) output femtosecond laser seed light source, pass through acousto-optic pulse selector (3), random waveform hair Raw device (5) output drive signal (7), driving signal (7) control the working time window of acousto-optic pulse selector (3), carry out arteries and veins Punching selection carries out power amplification to the femtosecond pulse after frequency reducing using ytterbium laser amplifier (4) is mixed;Synchronizing mode-licked femto-second laser Repetition rate, acousto-optic pulse selector, pumping pulse, direct impulse and cameras frame rate.
5. the instantaneous two-dimensional opto-acoustic wave measurement method according to claim 3 based on the interference of femtosecond pulse, it is characterised in that: Photoacoustic waves induce generation module (26), including beam splitter prism (9), pump light (10) and microcobjective (11), dichroscope (12), Amplified pulsed light is divided into two bundles by beam splitter prism (9), and respectively as pump light (10) and detection light (14), pump light passes through It is focused by microcobjective (11), photoacoustic waves is generated by dichroscope (12) incident acetone soln (15).
6. the instantaneous two-dimensional opto-acoustic wave measurement method according to claim 3 based on the interference of femtosecond pulse, it is characterised in that: Pulse Mach Zehnder interferometry module, including barium metaborate nonlinear crystal (13), delay optical path (16), bandpass optical filtering device (18), Amici prism (19), Amici prism two (23), reflecting mirror (21), electrooptic modulator (20), microcobjective (24) and CMOS Camera (25) detects light after barium metaborate nonlinear crystal (13) filters out light ambient noise, anti-by delay optical path (16) Reflecting mirror (17) are mapped to, the prism one (19) that is split is filtered through bandpass optical filtering device (18) and is divided into reference light and measurement light, reference Light is reflected after electrooptic modulator (20) is modulated and improves interference fringe signal-to-noise ratio by reflecting mirror (21), passes sequentially through no pump Behind the acetone soln (22) of Pu photoinduction, Amici prism two (23) reflection and microcobjective (24), incident CMOS camera (25).
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