CN109461509A - Inertial base dispersion fuel pellet and preparation method thereof - Google Patents

Inertial base dispersion fuel pellet and preparation method thereof Download PDF

Info

Publication number
CN109461509A
CN109461509A CN201811152057.8A CN201811152057A CN109461509A CN 109461509 A CN109461509 A CN 109461509A CN 201811152057 A CN201811152057 A CN 201811152057A CN 109461509 A CN109461509 A CN 109461509A
Authority
CN
China
Prior art keywords
cylinder
sic
preparation
disk
base dispersion
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Granted
Application number
CN201811152057.8A
Other languages
Chinese (zh)
Other versions
CN109461509B (en
Inventor
孙茂州
马赵丹丹
高思宇
李锐
黄华伟
武海龙
刘彤
任啟森
廖业宏
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
China General Nuclear Power Corp
China Nuclear Power Technology Research Institute Co Ltd
CGN Power Co Ltd
Guangdong Nuclear Power Joint Venture Co Ltd
Institute of Materials of CAEP
Original Assignee
China General Nuclear Power Corp
China Nuclear Power Technology Research Institute Co Ltd
CGN Power Co Ltd
Guangdong Nuclear Power Joint Venture Co Ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by China General Nuclear Power Corp, China Nuclear Power Technology Research Institute Co Ltd, CGN Power Co Ltd, Guangdong Nuclear Power Joint Venture Co Ltd filed Critical China General Nuclear Power Corp
Priority to CN201811152057.8A priority Critical patent/CN109461509B/en
Publication of CN109461509A publication Critical patent/CN109461509A/en
Application granted granted Critical
Publication of CN109461509B publication Critical patent/CN109461509B/en
Active legal-status Critical Current
Anticipated expiration legal-status Critical

Links

Classifications

    • GPHYSICS
    • G21NUCLEAR PHYSICS; NUCLEAR ENGINEERING
    • G21CNUCLEAR REACTORS
    • G21C21/00Apparatus or processes specially adapted to the manufacture of reactors or parts thereof
    • G21C21/02Manufacture of fuel elements or breeder elements contained in non-active casings
    • GPHYSICS
    • G21NUCLEAR PHYSICS; NUCLEAR ENGINEERING
    • G21CNUCLEAR REACTORS
    • G21C3/00Reactor fuel elements and their assemblies; Selection of substances for use as reactor fuel elements
    • G21C3/42Selection of substances for use as reactor fuel
    • G21C3/58Solid reactor fuel Pellets made of fissile material
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E30/00Energy generation of nuclear origin
    • Y02E30/30Nuclear fission reactors

Landscapes

  • Engineering & Computer Science (AREA)
  • Physics & Mathematics (AREA)
  • Plasma & Fusion (AREA)
  • General Engineering & Computer Science (AREA)
  • High Energy & Nuclear Physics (AREA)
  • Manufacturing & Machinery (AREA)
  • Ceramic Products (AREA)

Abstract

The invention discloses a kind of inertial base dispersion fuel pellet and preparation method thereof, preparation method includes: S1, prefabricated no fuel region: SiC mixed-powder being pressed into cylinder and disk respectively and carries out pressureless sintering;S2, prefabricated fuel region: the TRISO particle with SiC clad is pressed into cylindrical body;S3, cylindrical body is packed into cylinder, places disk respectively in the opposite end of cylinder, inertial base dispersion fuel pellet is made in discharge plasma sintering;Cylindrical at inertial base dispersion fuel pellet fuel region, cylinder and disk formed inertial base dispersion fuel pellet without fuel region.Preparation method of the invention, prefabricated no fuel region, the density domination of no fuel region and the pressed density in fuel region are approached, reduce after sintering fuel region density and the density variation without fuel region in pellet, improve fuel region TRISO particle circumference structure, expand fuel region, improves the TRISO volume content of pellet entirety, further increase the comprehensive performance of inertia base fuel.

Description

Inertial base dispersion fuel pellet and preparation method thereof
Technical field
The present invention relates to nuclear fuel technical field more particularly to a kind of inertial base dispersion fuel pellet and its preparation sides Method.
Background technique
Nuclear fuel energy density is high, CO2Equal noxious gas emissions are few, are that solution fossil resources are in short supply and environmental pollution is serious Important means.Nuclear energy power generation is clean energy resource, nuclear energy it is with the obvious advantage, with the continuous increase of nuclear power energy ratio, nuclear energy The more aobvious protrusion in the status of power generation.However, nuclear energy is the energy generated using the fission of the heavy metal elements such as uranium, fission, which will form, to be had Certain radioactive fission product.Therefore, carrying out radiation protection and preventing radioactive product leakage is the key that Nuclear Safety, It is the premise for developing nuclear energy.A lot of nuclear activity leakage events once occurred on the road of mankind's peaceful utilization of atomic energy, especially Fukushima, Japan Nuclear Power Accident in 2011 promotes tradition UO2The accident fault-tolerant ability of-Zr alloy system fuel assembly is closed as people The focus of note.
UO2Fusing point is high, void swelling is small, but thermal conductivity is low, and it is poor to contain ability for fission gas under deep burnup.Lower thermal conductivity UO2 pellet make UO2- Zr fuel system forms biggish temperature gradient, the UO of fuel rod in the process of running2In pellet Heart temperature reaches 1500 DEG C or more.The core temperature of pellet is high, and fission gas releases that rate is big, and high temperature gradient causes pellet to produce Heat stress reduces the safety of fuel element.In addition, pellet core temperature is higher under loss of-coolant accident (LOCA) working condition, heat transfer Energy to fuel rod clad is more, and fission gas burst size is bigger, increases the risk of fuel rod clad breakage, or even draws Send out core meltdown.Therefore, advanced nuclear fuel is developed, studies high heat conductance, the fuel ball of low fission gas release rate is to mention The key of high nuclear reactor fuel element accident fault-tolerant ability.
IMDP is to use for reference high temperature gas cooled reactor fuel sphere technology, using TRISO microballoon as nuclear fuel carrier, more by TRISO microballoon It dissipates and is distributed in SiC matrix, be the important research direction of accident fault tolerant fuel pellet.In IMDP pellet, the SiC base of high heat conductance Body coats TRISO microballoon, protects the integrality of TRISO microballoon, while efficiently conducting heat.Moreover, TRISO particle and IMDP Special construction design guarantees that pellet inhibits the release of fission gas under deep burnup.The SiC matrix fusing point of IMDP fuel ball High, thermal conductivity height, TRISO microballoon fission gas release rate is low, these advantages improve the accident fault-tolerant ability of fuel element.
IMDP pellet is TRISO microballoon Dispersed precipitate in the SiC matrix of powder, and U.S.'s Oak Ridge National Laboratory uses The method of hot pressed sintering carries out hot pressed sintering after mixing TRISO particle with SiC powder, this technique is more mature, and compared to Pure UO2 pellet thermal conductivity improves, but the method has some disadvantages: that (1) compacting green compact process is difficult, especially outer layer Without fuel region, Chang Wufa combines closely with fuel region;(2) sintering temperature is high, is unfavorable for the promotion of pellet comprehensive performance.
Summary of the invention
The technical problem to be solved in the present invention is that providing a kind of inertial base disperse for improving fuel pellet comprehensive performance The preparation method of fuel pellet and inertial base dispersion fuel pellet obtained.
The technical solution adopted by the present invention to solve the technical problems is: providing a kind of inertial base dispersion fuel pellet Preparation method, comprising the following steps:
S1, prefabricated no fuel region: SiC mixed-powder is pressed into cylinder and disk respectively and carries out pressureless sintering;
S2, prefabricated fuel region: the TRISO particle with SiC clad is pressed into cylindrical body;
S3, the cylindrical body is packed into the cylinder, places the circle respectively in the opposite end of the cylinder Piece, discharge plasma sintering, is made inertial base dispersion fuel pellet;
For the cylindrical at the fuel region of the inertial base dispersion fuel pellet, the cylinder and disk form institute State inertial base dispersion fuel pellet without fuel region.
Preferably, in step S1, the density of the cylinder and disk after pressureless sintering is respectively 60%-80%.
Preferably, in step S1, when pressureless sintering, SiC powder is covered on the cylinder and disk.
Preferably, the wall thickness of the cylinder be 3-5mm, the disk with a thickness of 2-3mm.
Preferably, the diameter of the disk is equal with the outer diameter of the cylinder;The outer diameter of the cylindrical body and the circle The internal diameter of cylinder is equal.
Preferably, in step S3, in the discharge plasma sintering, sintering temperature is 1600-2000 DEG C, sintering pressure For 10-50MPa, soaking time 5-20min.
Preferably, the preparation method is further comprising the steps of:
S0, sintering aid, SiC powder, dispersing agent are mixed, obtains finely dispersed SiC mixed slurry;
Step S1 includes:
S1.1, it takes the SiC mixed slurry to be dried, forms SiC mixed-powder;
S1.2, the SiC mixed-powder is pressed into cylinder and disk respectively;
S1.3, the cylinder and disk are sintered under the conditions of no pressure.
Preferably, step S2 includes:
S2.1, take the SiC mixed slurry and be sprayed on TRISO particle surface, it is dry after on TRISO particle shape At SiC clad;
S2.2, it the TRISO particle with SiC clad is suppressed under 20-40MPa pressure forms cylindrical body.
The present invention provides the preparation method of another inertial base dispersion fuel pellet, comprising the following steps:
S1, prefabricated no fuel region: SiC mixed-powder is pressed into cylinder and disk respectively and carries out pressureless sintering;
It is S2, the TRISO with SiC clad is particles filled in the cylinder, and by the intracorporal institute of the cylinder TRISO particle is stated to suppress to form cylindrical body;
S3, the disk is placed respectively in the opposite end of the cylinder, inertia base is made in discharge plasma sintering Body dispersion fuel pellet;
For the cylindrical at the fuel region of the inertial base dispersion fuel pellet, the cylinder and disk form institute State inertial base dispersion fuel pellet without fuel region.
Preferably, in step S1, the density of the cylinder and disk after pressureless sintering is respectively 60%-80%;
When pressureless sintering, SiC powder is covered on the cylinder and disk.
Preferably, the wall thickness of the cylinder be 3-5mm, the disk with a thickness of 2-3mm.
Preferably, in step S3, in the discharge plasma sintering, sintering temperature is 1600-2000 DEG C, sintering pressure For 10-50MPa, soaking time 5-20min.
Preferably, the preparation method is further comprising the steps of:
S0, sintering aid, SiC powder, dispersing agent are mixed, obtains finely dispersed SiC mixed slurry;
Step S1 includes:
S1.1, it takes the SiC mixed slurry to be dried, forms SiC mixed-powder;
S1.2, the SiC mixed-powder is pressed into cylinder and disk respectively;
S1.3, the cylinder and disk are sintered under the conditions of no pressure.
Preferably, step S2 includes:
S2.1, take the SiC mixed slurry and be sprayed on TRISO particle surface, it is dry after on TRISO particle shape At SiC clad;
It is S2.2, the TRISO with SiC clad is particles filled in the cylinder, it, will under 20-40MPa pressure The intracorporal TRISO particle of cylinder is suppressed to form cylindrical body.
The present invention also provides a kind of inertial base dispersion fuel pellets, using preparation method system described in any of the above embodiments ?.
Beneficial effects of the present invention: prefabricated no fuel region, the density domination of no fuel region is pressed close with fuel region Degree is close, reduces after sintering fuel region matrix density and the density variation without fuel region in inertial base dispersion fuel pellet, changes Kind fuel region TRISO (tristrutural-isotropic, abbreviation TRISO) particle circumference structure, expands combustion as far as possible Expect area, improves the TRISO volume content of pellet entirety, further increase the comprehensive performance of inertia base fuel.
Detailed description of the invention
Present invention will be further explained below with reference to the attached drawings and examples, in attached drawing:
Fig. 1 is the flow chart of the preparation method of first embodiment of the invention;
Fig. 2 is tri- perspective views of CT of pellet made from the preparation method of first embodiment of the invention;
Fig. 3 is the flow chart of the preparation method of second embodiment of the invention.
Specific embodiment
For a clearer understanding of the technical characteristics, objects and effects of the present invention, now control attached drawing is described in detail A specific embodiment of the invention.
As shown in Figure 1, the preparation method of the inertial base dispersion fuel pellet of first embodiment of the invention, it may include following Step:
S0, sintering aid, SiC powder, dispersing agent are mixed by predetermined ratio, obtains finely dispersed SiC mixing Slurry.
SiC mixed slurry obtained is used for the raw material of subsequent no fuel region and fuel region.
S1, prefabricated no fuel region: SiC mixed-powder is pressed into cylinder and disk respectively and carries out pressureless sintering.
Step S1 is further can include:
S1.1, it takes SiC mixed slurry made from step S0 to be dried, forms SiC mixed-powder.
S1.2, SiC mixed-powder is pressed into cylinder and disk respectively.
One cylinder two disk of corresponding configuration.
S1.3, cylinder and disk are sintered under the conditions of no pressure, make its densification.
In step S1, the wall thickness for suppressing the cylinder of formation can be 3-5mm, and the thickness of disk can be 2-3mm.
The density of cylinder and disk after controlling pressureless sintering is respectively 60%-80%, makes its fuel region with pellet Density it is close or identical, reduce density variation between the two.
When pressureless sintering, according to the density of desired cylinder and disk, sintering temperature is controlled, so that sintered cylinder The density of body and disk is in claimed range.
When pressureless sintering, SiC powder is covered on cylinder and disk, mainly reduces or is prevented in SiC mixed-powder The volatilization of various auxiliary agents.
S2, prefabricated fuel region: the TRISO particle with SiC clad is pressed into cylindrical body.
It is 20-40MPa by the pressure that the TRISO particle with SiC clad is pressed into cylindrical body.In cylindrical body, SiC Clad layer-forming matrix, TRISO particle disperse in the base;TRISO particle content in cylindrical body accounts for 40-60%.Cylindrical body Density be 40-50%.
Step S2 is further can include:
S2.1, SiC mixed slurry made from step S0 is taken, and SiC mixed slurry is sprayed on TRISO particle surface, done SiC clad is formed after dry on TRISO particle.
S2.2, it the TRISO particle with SiC clad is suppressed under 20-40MPa pressure forms cylindrical body.
The size of cylindrical body corresponds to cylinder, for example, the outer diameter of cylindrical body is equal with the internal diameter of cylinder or slightly smaller than justifies The internal diameter of cylinder, the height of cylindrical body and the height of cylinder are equal.
S3, cylindrical body is packed into cylinder, places disk respectively in the opposite end of cylinder, discharge plasma is burnt Inertial base dispersion fuel pellet is made in knot.
For cylindrical at the fuel region of inertial base dispersion fuel pellet, cylinder and disk form inertial base disperse combustion Expect pellet without fuel region.
Wherein, the diameter of disk and the outer diameter of cylinder are equal, and disk is in the end of cylinder by cylinder and its inside Cylindrical body covering.The outer diameter of cylindrical body and the internal diameter of cylinder are corresponding, are assemblied in cylinder so that cylindrical body can coincide.
Discharge plasma sintering carries out in graphite jig.Discharge plasma be sintered when, sintering temperature be 1600 DEG C- 2000 DEG C, sintering pressure 10MPa-50MPa, soaking time 5min-20min.After the completion of sintering, furnace cooling is obtained lazy Property matrix dispersion fuel pellet.
Due to no fuel region be it is first pre-formed, when discharge plasma is sintered, TRISO to fuel region of no fuel region Grain plays an effect of contraction, and the circumference of TRISO distribution of particles is more regular in sintered pellet.As shown in Fig. 2, its Show tri- perspective views of CT of pellet made from the present embodiment preparation method, as seen from the figure, the circumference of TRISO particle It is more regular, it is binding to TRISO particle mainly since the density of no fuel region is higher, it is therefore prevented that TRISO particle to No fuel region is mobile.
As shown in figure 3, the preparation method of the inertial base dispersion fuel pellet of second embodiment of the invention, it may include following Step:
S0, sintering aid, SiC powder, dispersing agent are mixed by predetermined ratio, obtains finely dispersed SiC mixing Slurry.
SiC mixed slurry obtained is used for the raw material of subsequent no fuel region and fuel region.
S1, prefabricated no fuel region: SiC mixed-powder is pressed into cylinder and disk respectively and carries out pressureless sintering.
Step S1 is further can include:
S1.1, it takes SiC mixed slurry made from step S0 to be dried, forms SiC mixed-powder.
S1.2, SiC mixed-powder is pressed into cylinder and disk respectively.
One cylinder two disk of corresponding configuration.
S1.3, cylinder and disk are sintered under the conditions of no pressure, make its densification.
In step S1, the wall thickness for suppressing the cylinder of formation can be 3-5mm, and the thickness of disk can be 2-3mm.
The density of cylinder and disk after controlling pressureless sintering is respectively 60%-80%, makes its fuel region with pellet Density it is close or identical, reduce density variation between the two.
When pressureless sintering, according to the density of desired cylinder and disk, sintering temperature is controlled, so that sintered cylinder The density of body and disk is in claimed range.
When pressureless sintering, SiC powder is covered on cylinder and disk, mainly reduces or is prevented in SiC mixed-powder The volatilization of various auxiliary agents.
It is S2, the TRISO with SiC clad is particles filled in cylinder, and there is SiC cladding by cylinder is intracorporal The TRISO particle of layer is suppressed to form cylindrical body.
It is 20-40MPa by the pressure that the TRISO particle with SiC clad is pressed into cylindrical body.In cylindrical body, SiC Clad layer-forming matrix, TRISO particle disperse in the base;TRISO particle content in cylindrical body accounts for 40-60%.Cylindrical body Density be 40-50%.
Step S2 is further can include:
S2.1, SiC mixed slurry made from step S0 is taken, and SiC mixed slurry is sprayed on TRISO particle surface, done SiC clad is formed after dry on TRISO particle.
It is S2.2, the TRISO with SiC clad is particles filled in cylinder, under 20-40MPa pressure, by cylinder Intracorporal TRISO particle is suppressed to form cylindrical body.
The size of cylindrical body corresponds to cylinder, for example, the outer diameter of cylindrical body is equal with the internal diameter of cylinder or slightly smaller than justifies The internal diameter of cylinder, the height of cylindrical body and the height of cylinder are equal.
S3, disk is placed respectively in the opposite end of cylinder, inertial base disperse combustion is made in discharge plasma sintering Expect pellet.
For cylindrical at the fuel region of inertial base dispersion fuel pellet, cylinder and disk form inertial base disperse combustion Expect pellet without fuel region.
Wherein, the diameter of disk and the outer diameter of cylinder are equal, and disk is in the end of cylinder by cylinder and its inside Cylindrical body covering.The outer diameter of cylindrical body and the internal diameter of cylinder are corresponding, are assemblied in cylinder so that cylindrical body can coincide.
Discharge plasma sintering carries out in graphite jig.Discharge plasma be sintered when, sintering temperature be 1600 DEG C- 2000 DEG C, sintering pressure 10MPa-50MPa, soaking time 5min-20min.After the completion of sintering, furnace cooling is obtained lazy Property matrix dispersion fuel pellet.
The present embodiment is first attached in no fuel region from fuel region material unlike above-mentioned first embodiment and is suppressed again Molding, tri- basic phases of perspective view of CT of tri- perspective views of CT and pellet made from above-mentioned first embodiment of pellet obtained Together, the circumference of TRISO particle is more regular.
Inertial base dispersion fuel pellet made from preparation method of the invention, including fuel region and without fuel region, fuel Area is in no fuel region.
Specifically, fuel region is by cylindrical at no fuel region is formed by cylinder and disk.Cylindrical body is arranged in cylinder In vivo, cylinder inner space is filled, disk is arranged on the opposite end of cylinder, and whole inertia base is formed after sintering Body dispersion fuel pellet.
To sum up, in the present invention, no fuel region first passes through sintering and carries out die-filling, sintered no fuel region with fuel region again Intensity is higher than unsintered green compact, can reduce the risk without fuel region division during die-filling.Prefabricated passes through without fuel region Sintering front and back density calculates, and can reduce fuel region and the density variation without fuel region in pellet;It is prefabricated without fuel region density compared with Height plays an effect of contraction to the TRISO particle of fuel region, and sintering process TRISO particle can be prevented mobile to no fuel region, Be conducive to the size Control of fuel region, the diameter of fuel region can be expanded, improves the TRISO volume content of pellet.In addition, in pellet The mechanical performance of pellet can be improved in raising without fuel region density.
The above description is only an embodiment of the present invention, is not intended to limit the scope of the invention, all to utilize this hair Equivalent structure or equivalent flow shift made by bright specification and accompanying drawing content is applied directly or indirectly in other relevant skills Art field, is included within the scope of the present invention.

Claims (15)

1. a kind of preparation method of inertial base dispersion fuel pellet, which comprises the following steps:
S1, prefabricated no fuel region: SiC mixed-powder is pressed into cylinder and disk respectively and carries out pressureless sintering;
S2, prefabricated fuel region: the TRISO particle with SiC clad is pressed into cylindrical body;
S3, the cylindrical body is packed into the cylinder, places the disk respectively in the opposite end of the cylinder, puts Electro-plasma sintering, is made inertial base dispersion fuel pellet;
At the fuel region of the inertial base dispersion fuel pellet, the cylinder and disk form described lazy the cylindrical Property matrix dispersion fuel pellet without fuel region.
2. the preparation method of inertial base dispersion fuel pellet according to claim 1, which is characterized in that in step S1, The density of the cylinder and disk after pressureless sintering is respectively 60%-80%.
3. the preparation method of inertial base dispersion fuel pellet according to claim 1, which is characterized in that in step S1, When pressureless sintering, SiC powder is covered on the cylinder and disk.
4. the preparation method of inertial base dispersion fuel pellet according to claim 1, which is characterized in that the cylinder Wall thickness be 3-5mm, the disk with a thickness of 2-3mm.
5. the preparation method of inertial base dispersion fuel pellet according to claim 1, which is characterized in that the disk Diameter is equal with the outer diameter of the cylinder;The outer diameter of the cylindrical body is equal with the internal diameter of the cylinder.
6. the preparation method of inertial base dispersion fuel pellet according to claim 1, which is characterized in that in step S3, In the discharge plasma sintering, sintering temperature is 1600-2000 DEG C, sintering pressure 10-50MPa, soaking time 5- 20min。
7. the preparation method of inertial base dispersion fuel pellet according to claim 1-6, which is characterized in that institute It is further comprising the steps of to state preparation method:
S0, sintering aid, SiC powder, dispersing agent are mixed, obtains finely dispersed SiC mixed slurry;
Step S1 includes:
S1.1, it takes the SiC mixed slurry to be dried, forms SiC mixed-powder;
S1.2, the SiC mixed-powder is pressed into cylinder and disk respectively;
S1.3, the cylinder and disk are sintered under the conditions of no pressure.
8. the preparation method of inertial base dispersion fuel pellet according to claim 7, which is characterized in that step S2 packet It includes:
S2.1, it takes the SiC mixed slurry and is sprayed on TRISO particle surface, formed on TRISO particle after dry SiC clad;
S2.2, it the TRISO particle with SiC clad is suppressed under 20-40 MPa pressure forms cylindrical body.
9. a kind of preparation method of inertial base dispersion fuel pellet, which comprises the following steps:
S1, prefabricated no fuel region: SiC mixed-powder is pressed into cylinder and disk respectively and carries out pressureless sintering;
It is S2, the TRISO with SiC clad is particles filled in the cylinder and the cylinder is intracorporal described TRISO particle is suppressed to form cylindrical body;
S3, the disk is placed respectively in the opposite end of the cylinder, inertial base is made more in discharge plasma sintering Dissipate fuel pellet;
At the fuel region of the inertial base dispersion fuel pellet, the cylinder and disk form described lazy the cylindrical Property matrix dispersion fuel pellet without fuel region.
10. the preparation method of inertial base dispersion fuel pellet according to claim 9, which is characterized in that in step S1, The density of the cylinder and disk after pressureless sintering is respectively 60%-80%;
When pressureless sintering, SiC powder is covered on the cylinder and disk.
11. the preparation method of inertial base dispersion fuel pellet according to claim 9, which is characterized in that the cylinder The wall thickness of body be 3-5mm, the disk with a thickness of 2-3mm.
12. the preparation method of inertial base dispersion fuel pellet according to claim 9, which is characterized in that in step S3, In the discharge plasma sintering, sintering temperature is 1600-2000 DEG C, sintering pressure 10-50MPa, soaking time 5- 20min。
13. according to the preparation method of the described in any item inertial base dispersion fuel pellets of claim 9-12, which is characterized in that The preparation method is further comprising the steps of:
S0, sintering aid, SiC powder, dispersing agent are mixed, obtains finely dispersed SiC mixed slurry;
Step S1 includes:
S1.1, it takes the SiC mixed slurry to be dried, forms SiC mixed-powder;
S1.2, the SiC mixed-powder is pressed into cylinder and disk respectively;
S1.3, the cylinder and disk are sintered under the conditions of no pressure.
14. the preparation method of inertial base dispersion fuel pellet according to claim 13, which is characterized in that step S2 packet It includes:
S2.1, it takes the SiC mixed slurry and is sprayed on TRISO particle surface, formed on TRISO particle after dry SiC clad;
It is S2.2, the TRISO with SiC clad is particles filled in the cylinder, under 20-40 MPa pressure, by institute The intracorporal TRISO particle of cylinder is stated to suppress to form cylindrical body.
15. a kind of inertial base dispersion fuel pellet, which is characterized in that using any one of claim 1-8 or claim 9- 14 described in any item preparation methods are made.
CN201811152057.8A 2018-09-29 2018-09-29 Inert matrix dispersion fuel pellet and preparation method thereof Active CN109461509B (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
CN201811152057.8A CN109461509B (en) 2018-09-29 2018-09-29 Inert matrix dispersion fuel pellet and preparation method thereof

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CN201811152057.8A CN109461509B (en) 2018-09-29 2018-09-29 Inert matrix dispersion fuel pellet and preparation method thereof

Publications (2)

Publication Number Publication Date
CN109461509A true CN109461509A (en) 2019-03-12
CN109461509B CN109461509B (en) 2020-11-10

Family

ID=65607257

Family Applications (1)

Application Number Title Priority Date Filing Date
CN201811152057.8A Active CN109461509B (en) 2018-09-29 2018-09-29 Inert matrix dispersion fuel pellet and preparation method thereof

Country Status (1)

Country Link
CN (1) CN109461509B (en)

Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN110223789A (en) * 2019-05-07 2019-09-10 中广核研究院有限公司 Manufacturing method, inertia base dispersion fuel pellet and the integrated fuel stick and its manufacturing method of high uranium density coated fuel particles
CN111933310A (en) * 2020-06-09 2020-11-13 上海核工程研究设计院有限公司 High-thermal-conductivity uranium dioxide single crystal composite fuel pellet and preparation method thereof
CN113012832A (en) * 2019-12-20 2021-06-22 中核北方核燃料元件有限公司 UO2Composite UN-UO2Method for producing fuel pellets
WO2022241733A1 (en) * 2021-05-20 2022-11-24 中广核研究院有限公司 High-entropy ceramic inert matrix dispersion fuel pellet and preparation method therefor

Citations (11)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2006284489A (en) * 2005-04-04 2006-10-19 Nuclear Fuel Ind Ltd Manufacturing method of coated fuel particle for high-temperature gas-cooled reactors
CN102770921A (en) * 2009-12-04 2012-11-07 原子能与替代能源委员会 Nuclear fuel rod and method for manufacturing pellets for such a fuel rod
CN103466568A (en) * 2013-09-09 2013-12-25 中国原子能科学研究院 Preparation method of uranium nitride fuel powder and pellet
CN104628395A (en) * 2013-11-07 2015-05-20 中国科学院宁波材料技术与工程研究所 Production method of nuclear fuel clad element
CN104671766A (en) * 2015-03-10 2015-06-03 桂林电子科技大学 High-temperature piezoelectric and dielectric energy storage lead-free ceramic and preparation method thereof
CN106448749A (en) * 2016-09-23 2017-02-22 中广核研究院有限公司 Fuel pellet and preparation method thereof
CN106904984A (en) * 2017-02-27 2017-06-30 中国核动力研究设计院 A kind of SiC short fiber composite materials and compound cladding tubes and preparation method thereof
CN106971764A (en) * 2017-04-13 2017-07-21 中国工程物理研究院材料研究所 A kind of quick preparation technology of inertia base dispersion fuel pellet
CN106981318A (en) * 2017-04-13 2017-07-25 中国工程物理研究院材料研究所 A kind of inertia base disperse pellet fuel and its production and use
US20170287575A1 (en) * 2016-03-29 2017-10-05 Ultra Safe Nuclear Corporation Fully ceramic microencapsulated fuel fabricated with burnable poison as sintering aid
CN107500767A (en) * 2017-08-21 2017-12-22 中广核研究院有限公司 Uranium carbide pellet and preparation method thereof, fuel rod

Patent Citations (11)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2006284489A (en) * 2005-04-04 2006-10-19 Nuclear Fuel Ind Ltd Manufacturing method of coated fuel particle for high-temperature gas-cooled reactors
CN102770921A (en) * 2009-12-04 2012-11-07 原子能与替代能源委员会 Nuclear fuel rod and method for manufacturing pellets for such a fuel rod
CN103466568A (en) * 2013-09-09 2013-12-25 中国原子能科学研究院 Preparation method of uranium nitride fuel powder and pellet
CN104628395A (en) * 2013-11-07 2015-05-20 中国科学院宁波材料技术与工程研究所 Production method of nuclear fuel clad element
CN104671766A (en) * 2015-03-10 2015-06-03 桂林电子科技大学 High-temperature piezoelectric and dielectric energy storage lead-free ceramic and preparation method thereof
US20170287575A1 (en) * 2016-03-29 2017-10-05 Ultra Safe Nuclear Corporation Fully ceramic microencapsulated fuel fabricated with burnable poison as sintering aid
CN106448749A (en) * 2016-09-23 2017-02-22 中广核研究院有限公司 Fuel pellet and preparation method thereof
CN106904984A (en) * 2017-02-27 2017-06-30 中国核动力研究设计院 A kind of SiC short fiber composite materials and compound cladding tubes and preparation method thereof
CN106971764A (en) * 2017-04-13 2017-07-21 中国工程物理研究院材料研究所 A kind of quick preparation technology of inertia base dispersion fuel pellet
CN106981318A (en) * 2017-04-13 2017-07-25 中国工程物理研究院材料研究所 A kind of inertia base disperse pellet fuel and its production and use
CN107500767A (en) * 2017-08-21 2017-12-22 中广核研究院有限公司 Uranium carbide pellet and preparation method thereof, fuel rod

Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN110223789A (en) * 2019-05-07 2019-09-10 中广核研究院有限公司 Manufacturing method, inertia base dispersion fuel pellet and the integrated fuel stick and its manufacturing method of high uranium density coated fuel particles
CN113012832A (en) * 2019-12-20 2021-06-22 中核北方核燃料元件有限公司 UO2Composite UN-UO2Method for producing fuel pellets
CN111933310A (en) * 2020-06-09 2020-11-13 上海核工程研究设计院有限公司 High-thermal-conductivity uranium dioxide single crystal composite fuel pellet and preparation method thereof
WO2022241733A1 (en) * 2021-05-20 2022-11-24 中广核研究院有限公司 High-entropy ceramic inert matrix dispersion fuel pellet and preparation method therefor

Also Published As

Publication number Publication date
CN109461509B (en) 2020-11-10

Similar Documents

Publication Publication Date Title
CN109461509A (en) Inertial base dispersion fuel pellet and preparation method thereof
KR101793896B1 (en) Fully ceramic nuclear fuel and related methods
JP7113828B2 (en) Sintered nuclear fuel pellets, fuel rods, nuclear fuel assemblies, and methods of making sintered nuclear fuel pellets
US10475543B2 (en) Dispersion ceramic micro-encapsulated (DCM) nuclear fuel and related methods
US20230112687A1 (en) Integrated in-vessel neutron shield
CN108335760B (en) Preparation method of high-uranium-loading-capacity dispersed fuel pellet
CN108885907B (en) Full ceramic micro-encapsulated fuel prepared by taking burnable poison as sintering aid
CN106782681B (en) Three cold type fuel rod and fuel assembly
CN103214231B (en) For improvement performance oxide ceramics core body and the preparation method of thermal reactor
KR20180121788A (en) SiC and graphite matrix TRISO-containing process for rapid treatment of pebble fuel
CN107093468A (en) A kind of ZrC inertia base disperse pellet nuclear fuel and its preparation method and purposes
CN108806804A (en) Fibre-reinforced fuel pellets of SiC and preparation method thereof
CN108039210A (en) Fuel pellet and its manufacture method
CN114068043A (en) Particulate dense fuel element
CN107967950A (en) The manufacture method and fuel pellet of fuel pellet
JP2004309453A (en) Nuclear fuel sinter containing tungsten metal mesh and its manufacturing method
CN108182979A (en) Adulterate the fuel pellet and its manufacturing method of boron carbide
JPH01232289A (en) Fuel element and fuel assembly
CA1100302A (en) High performance nuclear fuel element
CN111710443B (en) Diamond composite nuclear fuel pellet and preparation method thereof
JP2860615B2 (en) Fuel assembly for plutonium firing
CN116313173A (en) Particle coated dispersion fuel and fuel pellets
JP2024503914A (en) heat bridge
Tournier et al. Performance analysis of coated 238 PuO 2 fuel particles compact for radioisotope heater units
CN118352102A (en) Solid moderator material arrangement form for miniaturized design of liquid metal cooling reactor

Legal Events

Date Code Title Description
PB01 Publication
PB01 Publication
SE01 Entry into force of request for substantive examination
SE01 Entry into force of request for substantive examination
TA01 Transfer of patent application right

Effective date of registration: 20200619

Address after: 518031 Guangdong province Futian District Shangbu Road West of the city of Shenzhen Shenzhen science and technology building 15 layer (1502-1504, 1506)

Applicant after: CHINA NUCLEAR POWER TECHNOLOGY RESEARCH INSTITUTE Co.,Ltd.

Applicant after: GUANGDONG NUCLEAR POWER JOINT VENTURE

Applicant after: Institute of Materials, China Academy of Engineering Physics

Applicant after: CHINA GENERAL NUCLEAR POWER Corp.

Applicant after: CGN POWER Co.,Ltd.

Address before: 518031 Guangdong province Futian District Shangbu Road West of the city of Shenzhen Shenzhen science and technology building 15 layer (1502-1504, 1506)

Applicant before: CHINA NUCLEAR POWER TECHNOLOGY RESEARCH INSTITUTE Co.,Ltd.

Applicant before: GUANGDONG NUCLEAR POWER JOINT VENTURE

Applicant before: CHINA GENERAL NUCLEAR POWER Corp.

Applicant before: CGN POWER Co.,Ltd.

TA01 Transfer of patent application right
GR01 Patent grant
GR01 Patent grant