CN107637858A - A kind of plant for improving water extraction and alcohol precipitation method extraction causes perfumery and extracting method and application - Google Patents
A kind of plant for improving water extraction and alcohol precipitation method extraction causes perfumery and extracting method and application Download PDFInfo
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Abstract
The present invention relates to a kind of plant for improving water extraction and alcohol precipitation method extraction to cause perfumery and extracting method and application, this method to include：Step（1）, prepare primary extraction liquid；Step（2）, prepare two level extract solution；Step（3）, prepare storing solution；The present invention more effectively extracts, has purified cause perfumery, and carry out preservative treatment, after expansion thread, thin slice use ratio are further added by delicate fragrance type cigarette leaf group, Sensory Quality of Cigarette and odor type main body sweetness note can be still kept, has the function that to lift delicate fragrance type Sensory Quality of Cigarette, highlight main body sweetness note and reach more than 12 months.
Description
Technical field
The present invention relates to a kind of plant to cause perfumery, and especially a kind of plant for improving water extraction and alcohol precipitation method extraction causes perfumery, also
It is related to extracting method and application, belongs to cigarette Titian field.
Background technology
Each tobacco enterprise in the whole nation, which all pays much attention to the Sensory Quality of Cigarette of respective brand and its odor type style and features, odor type, is
Chinese-style cigarette style important constituent element and sign.Cloud production cigarette is the Typical Representative of delicate fragrance type in Chinese-style cigarette, and fragrance is clear
It is refined elegant, there is fresh and sweet note, fragrance sensing speed is fast, and extension is strong, is to give an important factor for good fragrance is felt, jealous
Comfortably, smoke concentration is thin, and the miscellaneous gas of region is lighter, and strength softness represents type Yunnan, the tobacco leaf and its volume in Fujian to moderate
Cigarette.
FLOS CHRYSANTHEMI ALBA from Haizhou of China is the medicinal plant for having fresh and sweet note, is fit to the fresh and sweet note of delicate fragrance type cigarette main body note.
Flat-flavor：Aroma of pure is stable, and this perfume of tobacco is prominent, and fragrance sensing speed is medium, is the main body of cigarette product
Fragrance, jealous clean, smoke concentration is thin to denseer, and the miscellaneous gas of region has to larger, and it is expensive to represent type to larger for strength softness
State, Shandong, the tobacco leaf and its cigarette in northeast.
Luzhou-flavor：The dense fragrance of fragrance is heavy to overflow, and has burnt fragrant and sweet rhythm, and fragrance sensing speed is slower, long abundant, jealous comfortable,
The miscellaneous gas of region is very light extremely heavier, and strength is moderate, represents the tobacco leaf and its cigarette in type Henan, Hunan, Anhui.
Forefathers have carried out many researchs to feverfew in terms of perfuming cigarette, and Xu Chun is flat to choose mother chrysanthemum flower essential oil
(volatile oil) is core, and preparing chrysanthemum indicum essential oil microcapsules with complex coacervation is used for perfuming cigarette, and smoking result shows：When micro- glue
When capsule addition is 10~15mg/ branch, the increase of cigarette flavor amount is obvious, and excitant reduces, and pleasant impression is comfortable；Duan Binbin applications water steams
Steam distillation, Enzymatic Extraction Huai Chrysanthemi volatile oil perfuming are in cigarette；Zhang Di applications steam distillation, Simultaneous distillation-extraction, flash carry
Take, 4 kinds of extracting methods of ultrasonic assistant method carry out perfuming cigarette research to FLOS CHRYSANTHEMI ALBA from Haizhou of China volatile oil, determine ultrasonic assistant method for most
Best method；Wang Wenji have studied steam distillation, flash, cable-styled, enzyme extraction Huai Chrysanthemi volatile oil optimised process improved method,
Determine that cable-styled is the best approach；Intercalation gram of jade is divided using Simultaneous distillation extraction FLOS CHRYSANTHEMI ALBA from Haizhou of China volatile oil and with pyrolysis/GC/MS methods
Analysis identification volatile oil component.Cigarette of smokeing panel test shows：Appropriate Huai Chrysanthemi or FLOS CHRYSANTHEMI ALBA from Haizhou of China volatile oil are added in cigarette, have improve and
Modification cigarette flavor, perfume quantity and note substantially increase, mitigated the effect of excitant and miscellaneous gas.
It when water extraction and alcohol precipitation method extracts polysaccharide, can be extracted with hot water digestion or with cold water, then filter or centrifuge, carried
Take liquid；After extract solution is concentrated, ethanol is added in concentrate, its final volume fraction is reached 70% or so, using polysaccharide not
The property of ethanol is dissolved in, polysaccharide is precipitated out from extract solution, is stored at room temperature 5h；Refilter, obtain polysaccharide precipitation thing, washing
Sediment, obtain refined polysaccharide extract solution.That is plant immersion-hot water digestion or cold water extraction-separation of solid and liquid-plus ethanol reaches
70%- polysaccharide precipitations-refilter-polysaccharide precipitation thing-or water washing and precipitating-refined polysaccharide extract solution.However, traditional water extract-alcohol precipitation
Method can not accurately extract fresh and sweet fragrant plant material.
In addition, after expansion thread 5%, the use ratio of thin slice 4% are further added by delicate fragrance type cigarette leaf group, to cigarette sense organ matter
Amount and its delicate fragrance type main body note (fresh and sweet note) feature influence uncertainty be present, thus, in such a situa-tion, keep volume
Cigarette aesthetic quality and odor type main body sweetness note, turn into current technology difficult point.
The content of the invention
To solve problems of the prior art, the present invention provides a kind of fresh and sweet fragrant based on water extraction and alcohol precipitation method extraction is improved
Plant causes perfumery and the method for highlighting delicate fragrance type cigarette sweetness note.
The present invention is realized by following technical proposal：
A kind of method improved water extraction and alcohol precipitation method extraction plant and cause perfumery, comprises the following steps：
Step (1), prepare primary extraction liquid
Ground plant is soaked in water 10 minutes or so, is ultrasonically treated 0.5 ± 0.15 hour, then boil 1 ±
0.2 hour, residue is filtered, obtains primary extraction liquid；
Step (2), prepare two level extract solution
95% ethanol is added in primary extraction liquid, until the ethanol mass concentration of primary extraction liquid reaches 75% or so,
Then refrigerate, perfumery to be caused is dissolved in ethanol, filtering precipitate, obtains two level extract solution；
Step (3), prepare storing solution
After two level extract solution is concentrated into relative density 1.08-1.15, propane diols is added, until two level extract solution quality is dense
Spend for 10 ± 2%, that is, obtain causing the storing solution of perfumery containing plant.
Further, in step (1), the plant is the one or more of combination of FLOS CHRYSANTHEMI ALBA from Haizhou of China, chrysanthemum indicum and Huai Chrysanthemi.
Further, in step (1), plant mill to 40 mesh or so, ground plant is soaked in water, the quality of water
For 4 times of ground plant quality.
Further, in step (2), the time of refrigeration is 10 hours.
Further, in the volatility of the FLOS CHRYSANTHEMI ALBA from Haizhou of China and half volatile material, the cause perfumery with fresh and sweet note is：First
Base heptenone, levo-camphor, 2- borneols, farnesene, ionol, bisabolol and linoleic acid.
The plant of the present invention obtained according to the above method causes perfumery.
Above-mentioned plant of the present invention causes the application of perfumery, according to cigarette shreds mass percent, respectively with 95%
The mass concentration of ethanol dilution storing solution is 0.03 ± 0.005%, 0.05 ± 0.005%, 0.07 ± 0.005%, is then distinguished
Perfuming is in pipe tobacco.
Further, the mass ratio of ethanol and pipe tobacco is 1:100.
Compared with prior art, what the present invention possessed has the beneficial effect that：
The present invention has following advantages by improving traditional water extraction and alcohol precipitation method：
(1) ultrasound is boiled again：Ultrasonication then boils in plant cell wall (FLOS CHRYSANTHEMI ALBA from Haizhou of China etc.), efficiently isolates plant
Hydrophilic macromolecular substances (carbohydrate, globular protein, most glycosides, pectin etc.) Yu Shuizhong in thing.Ethanol is added, makes containing alcohol
Amount refrigerates 10 hours after reaching 75% extract solution quality so that macromolecular substances separate out in alcoholic solution because solubility reduces
Precipitation, and hydrophobic, micropolar organic cause perfumery is dissolved in alcohols；Plant residue is removed in filtering for the first time, second of filtering
Remove the hypostasis such as polysaccharide, produce required extract, enable Aqueous extracts primary purification；Concentrated extracting solution is to relative density 1.08-
1.15, now, concentrated extracting solution is 10% or so of original quality；(2) propane diols anti-corrosion is added：Diluted and concentrated with propane diols
Extract solution is standby to the storage of 10% mass concentration, plays good anti-corrosion, humectation effect.
Design, the combination of each step of present invention process and parameter, belong to pioneering, while qualitative 7 kinds of causes perfumery；By improving
Water extraction and alcohol precipitation method, more effectively extract, purify, anti-corrosion cause perfumery；Again by the perfuming of the feverfew storing solutions such as FLOS CHRYSANTHEMI ALBA from Haizhou of China
Concentration gradient is smoked panel test, and has filtered out optimal perfuming concentration 0.05 ± 0.005%, the anti-corrosion time or highlights main body sweetness note
Effect reaches more than 12 months；Confirm in 49 kinds of volatility of FLOS CHRYSANTHEMI ALBA from Haizhou of China and half volatile material there are 13 kinds there is unique perfume
The material of rhythm, its quality account for 11.13% (1725.83 μ g/15506.95 μ g=11.13%) of 49 kinds of material masses, 13 kinds
There are 10 kinds to be present in tobacco leaf and flue gas in material；The material of 7 kinds of fresh and sweet notes in 13 kinds of materials accounts for 13 kinds of material masses
49% (845.81/1725.83=49%).So, it is to increase expansion thread, thin slice use ratio in delicate fragrance type cigarette leaf group
Under conditions of, it is delicate fragrance type cigarette upgrading to keep Sensory Quality of Cigarette and odor type main body sweetness note to provide technical support
Titian rhythm, the fresh and sweet fragrant plant material of more accurately extraction, perfuming have been established in the technical foundation of cigarette, meanwhile, also responsive to state
Chinese herbal medicine advantage improves as the important means and direction for improving Chinese-style cigarette competitiveness in tobacco office of family.
Embodiment
It is clearly and completely described below in conjunction with the technical scheme in embodiment, it is clear that described embodiment is only
Only it is to a part of example of the present invention, rather than whole examples.Based on the embodiment in the present invention, ordinary skill people
The every other embodiment that member is obtained under the premise of creative work is not paid, belongs to the scope of protection of the invention.
1st, FLOS CHRYSANTHEMI ALBA from Haizhou of China aroma component and its note analysis
1.1 extractions cause perfumery and its analysis method
Plant aroma component mostlys come from its volatility and half volatile material, and Simultaneous distillation-extraction (SDE) is extraction
The common method of aroma component.Pass through the constituent analysis to FLOS CHRYSANTHEMI ALBA from Haizhou of China SDE2 hours/GC/MS.
In cucurbit, weigh and drink FLOS CHRYSANTHEMI ALBA from Haizhou of China 20g, add water 350mL, add internal standard substance n-heptadecane 1mL (positive 17
Alkane/dichloromethane=1/2000), in case distillation；In extraction flask, 40mL extractant dichloromethane is added；Then following step is pressed
It is rapid to carry out：1. 2h is extracted, 60 DEG C of waters bath with thermostatic control of extraction flask；2. 150 DEG C of heating mantle vapo(u)rizing temperature during extraction；3. conventionally
Moisture, concentrated extract to 1mL are separated, sample preparation, carries out gas chromatography/mass spectrometry (GC/MS) analysis.
GC/MS analysis conditions：Chromatographic column：HP-5MS(30m×0.25mmi.d.×0.25μmd.f.)；Temperature programming：40
℃(2min)-4℃/min-250℃(10min)；Injection port：250℃；Carrier gas：He；Stigma pressure：100kPa；Split ratio：20∶1；
Sample introduction desorption time 120s；Transmission line temperature：250℃；Ion source temperature：150℃；EI energy：70eV；Scanning range：35~
350u；Internal standard：N-heptadecane；The mass spectrogram collected is retrieved using NIST1.11 versions spectrum storehouse；Using area normalization method
It is quantitative.
1.2 FLOS CHRYSANTHEMI ALBA from Haizhou of China aroma components
The main chemical compositions of FLOS CHRYSANTHEMI ALBA from Haizhou of China be FLOS CHRYSANTHEMI ALBA from Haizhou of China research important evidence, and its value of exploiting and utilizing it is important come
Source.Contained chemical composition species is various in FLOS CHRYSANTHEMI ALBA from Haizhou of China, mainly there is the compositions such as flavonoids, volatile oil, amino acid, trace element.
Pass through the constituent analysis to FLOS CHRYSANTHEMI ALBA from Haizhou of China SDE2 hours/GC/MS, substance classes such as table 5 below
The FLOS CHRYSANTHEMI ALBA from Haizhou of China SDE2 hours of table 5/GC/MS substance classes
Note：Because causing perfumery content very low, content unit is microgram (μ g)
In table in material, before content 10 kinds of materials be successively the trans pinocarveol that comes into leaves, ledol, trans-menthyl-
2,8- diene -1- alcohol, loudspeaker olefinic oxide II, pinocarvone, the ketone of 9,17- diene-ten eight, 2- nitros -2- acrylic-hexamethylene
Alkane, 1,2,3,5,6,7- hexahydro -1,1,4,8- tetramethyl-s- indenes alkene, α-curcumene, fragrant citrus olefinic oxide II；10 kinds of materials
The μ g of quality 8916.83, the μ g of total material quality 15506.95, account for 57.50%.
From the point of view of the species of 49 kinds of materials, 18 kinds of olefines；12 kinds of alcohols；9 kinds of carbonyls；3 kinds of esters；Alkanes
3 kinds；1 kind of organic acid；1 kind of alkynes；Other 2 kinds of organic matters.A few class materials are analyzed on the whole, and the olefines species of FLOS CHRYSANTHEMI ALBA from Haizhou of China is most
More, its C2~C4 alkene is gas, and C5~C18 is volatile liquid, and delicate fragrance type cigarette flavor special delivery speed is fast, adds FLOS CHRYSANTHEMI ALBA from Haizhou of China
The olefines effumability positive correlation of the delicate fragrance type cigarette of extract solution, its fragrance transmission speed and FLOS CHRYSANTHEMI ALBA from Haizhou of China；Alcohols has in itself
More or less mellowness breath；Carbonyls has more or less sweet tea rhythm in itself；Esters have more or less ester in itself
Fragrance ceases.At room temperature, the alkane containing 1~4 carbon atom is gas to alkanes；Under normal temperature, containing 5~8 carbon atoms
Alkane is liquid；Alkane containing 8~16 carbon atoms can be solid, or liquid；More than 17 carbon atoms
Normal alkane be solid, lower boiling alkane is colourless liquid, there is special odor.
In 49 kinds of volatility of FLOS CHRYSANTHEMI ALBA from Haizhou of China and half volatile material, there are 13 kinds of materials with unique note.(1) methyl heptan
Ketenes：Fragrant, the citrus sample breath with fresh green grass or young crops；(2) levo-camphor：For synthesizing efficient sweetener, irritant fragranced；
(3) 2- borneols (borneol)：Have like camphor smell, smell delicate fragrance；(4) 4- terpenols：In warm pepper is fragrant, thin soil is fragrant and
Old timber breath；(5) β-farnesene：There is the blue or green fragrant, fragrance of a flower and with face cream fragrance；(6) ionol：In irisone
Class fragrance, there are the fragrance of a flower and the banksia rose and with cream is fragrant and fruity of sweet tea；(7) cedrol (cedar wood alcohol；Cedrol)：With the banksia rose, Xin Xiang；
(8) caryophyllene oxide：With pungent perfume, the banksia rose, the cloves fragrance that citrus is fragrant, camphor is fragrant, gentle；(9) pinocarvone：It is important
Spices, spearmint type；(10) bisabolol：With happy and sweet tea, fragrance of a flower spy's domestic animal smell of uniqueness；(11) Ergol (peace
Cease fragrant acid benzyl ester)：There are faint plum, almond fragrance；(12) linoleic acid：With fruit taste；(13) n-hexyl aldehyde：In raw oil
Fat and green grass gas and apple aroma.13 kinds of materials with unique note, species account for 26.53% (13/49=of 49 kinds of materials
26.53%), 13 kinds of material masses account for 11.13% (1725.83 μ g/15506.95 μ g=of 49 kinds of material masses
11.13%).
In 13 kinds of materials with unique note of FLOS CHRYSANTHEMI ALBA from Haizhou of China, wherein 7 kinds of materials with fresh and sweet note, i.e. (1) methyl
Heptenone；(2) levo-camphor；(3) 2- borneols (borneol)；(5) β-farnesene；(6) ionol；(10) bisabolol；
(12) linoleic acid.The substance classes of 7 kinds of fresh and sweet notes account for 14.29% (7/49=14.29%) of 49 kinds of materials；7 kinds of sweetness
The substance classes of note account for 13 kinds of 53.85% (7/13=53.85%) with unique note material；7 kinds of fresh and sweet note things
Matter quality accounts for 13 kinds of 49% (845.81/1725.83=49%) with unique note material mass.
8 kinds of materials such as (2) (3) (6) (7) (8) (9) (12) (13) in 13 kinds of materials are present in tobacco leaf, (5) (6)
(11) 4 kinds of materials such as (12) are present in flue gas, are present in tobacco leaf and totally 10 kinds of material in flue gas, (6) coexist in (12)
In tobacco leaf and flue gas, it accounts for 13 kinds of 76.92% (10/13=76.92%) with unique note material of FLOS CHRYSANTHEMI ALBA from Haizhou of China.
In addition, in 49 kinds of materials, 8 kinds of materials of sequence number 7,8,9,14,15,44,48,49 are present in main flow flue gas in tobacco
In, sequence number 13 is present in the burley tobaccos tobacco leaf of Turkish tobaccos, and 24,37 are present in tobacco leaf, and totally 11 kinds of materials are present in cigarette
In gas and tobacco leaf, wherein 15,24,44,48 be the material with fresh and sweet note in 13 kinds of materials.
Most of material has classification smell, in the common association of the other trace materials of FLOS CHRYSANTHEMI ALBA from Haizhou of China including 49 kinds of materials
Under tune, the feature of FLOS CHRYSANTHEMI ALBA from Haizhou of China sweetness note is embodied.FLOS CHRYSANTHEMI ALBA from Haizhou of China volatility meets the main body of delicate fragrance type cigarette with half volatile material
Fresh and sweet note, therefore, Flos Chrysanthemi extract can be used to lift delicate fragrance type Sensory Quality of Cigarette and its main body sweetness note.Zhang Diyan
The main component for studying carefully FLOS CHRYSANTHEMI ALBA from Haizhou of China volatile oil is terpenes and sesquiterpene compound, mainly there is copaene, australene, α-turmeric
Alkene, beta-elemene, α-farnesene, carypohyllene, limonene etc..Point out：β-bisabolene has unique floral character smell,
Happy is fragrant and sweet；Limonene has pure and fresh and suitable citrus fragrance；Carypohyllene has the pungent fragrant and banksia rose like caryophyllus oil；Linoleic acid
There is fruit taste；Furfural has stimulation, the smell of sweet tea.Therefore, it is known that there is good fragrance containing some in FLOS CHRYSANTHEMI ALBA from Haizhou of China volatile oil
Chemical composition, can be used to develop in industries such as cigarette.
2nd, improve water alcohol method and obtain FLOS CHRYSANTHEMI ALBA from Haizhou of China cause perfumery extract solution
Embodiment 1
The method improved water extraction and alcohol precipitation method extraction FLOS CHRYSANTHEMI ALBA from Haizhou of China and cause perfumery of the present embodiment, comprises the following steps：
Step (1)：Prepare primary extraction liquid
FLOS CHRYSANTHEMI ALBA from Haizhou of China is ground to 40 mesh or so, ground FLOS CHRYSANTHEMI ALBA from Haizhou of China is soaked in the water of 4 times of FLOS CHRYSANTHEMI ALBA from Haizhou of China quality, is soaked
After 10 minutes, it is ultrasonically treated 0.35 hour, then boils 0.8 hour, filters residue, obtain primary extraction liquid.
Step (2)：Prepare two level extract solution
Ethanol is added in primary extraction liquid, until the ethanol mass concentration of primary extraction liquid reaches 75% or so, then
Refrigeration 10 hours, perfumery to be caused is dissolved in ethanol, filtering precipitate, obtains two level extract solution；
Step (3)：Prepare storing solution
After two level extract solution is concentrated into relative density 1.08, propane diols is added, until two level extract solution mass concentration is
8%, that is, obtain causing the storing solution of perfumery containing plant.
Embodiment 2
The method improved water extraction and alcohol precipitation method extraction FLOS CHRYSANTHEMI ALBA from Haizhou of China and cause perfumery of the present embodiment, comprises the following steps：
Step (1)：Prepare primary extraction liquid
FLOS CHRYSANTHEMI ALBA from Haizhou of China is ground to 40 mesh or so, ground FLOS CHRYSANTHEMI ALBA from Haizhou of China is soaked in the water of 4 times of FLOS CHRYSANTHEMI ALBA from Haizhou of China quality, is soaked
After 10 minutes, it is ultrasonically treated 0.5 hour, then boils 1 hour, filters residue, obtain primary extraction liquid；
Step (2)：Prepare two level extract solution
Ethanol is added in primary extraction liquid, until the ethanol mass concentration of primary extraction liquid reaches 75% or so, then
Refrigeration 10 hours, perfumery to be caused is dissolved in ethanol, filtering precipitate, obtains two level extract solution；
Step (3)：Prepare storing solution
After two level extract solution is concentrated into relative density 1.10, propane diols is added, until two level extract solution mass concentration is
10%, that is, obtain causing the storing solution of perfumery containing plant.
Embodiment 3
The method improved water extraction and alcohol precipitation method extraction FLOS CHRYSANTHEMI ALBA from Haizhou of China and cause perfumery of the present embodiment, comprises the following steps：
Step (1)：Prepare primary extraction liquid
FLOS CHRYSANTHEMI ALBA from Haizhou of China is ground to 40 mesh or so, ground FLOS CHRYSANTHEMI ALBA from Haizhou of China is soaked in the water of 4 times of FLOS CHRYSANTHEMI ALBA from Haizhou of China quality, is soaked
After 10 minutes, it is ultrasonically treated 0.65 hour, then boils 1.2 hours, filters residue, obtain primary extraction liquid；
Step (2)：Prepare two level extract solution
Ethanol is added in primary extraction liquid, until the ethanol mass concentration of primary extraction liquid reaches 75% or so, then
Refrigeration 10 hours, perfumery to be caused is dissolved in ethanol, filtering precipitate, obtains two level extract solution；
Step (3)：Prepare storing solution
After two level extract solution is concentrated into relative density 1.15, propane diols is added, until two level extract solution mass concentration is
12%, that is, obtain causing the storing solution of perfumery containing plant.
Embodiment 4
The storing solution of Example 1, respectively with ethanol dilution mass concentration storing solution 0.03%, 0.05%,
0.07% perfuming concentration gradient perfuming in delicate fragrance type cigarette Yuxi (soft), Hongta (1956) pipe blend in (1g ethanol：
100g pipe tobaccos).
Embodiment 5
The storing solution of Example 1, respectively with ethanol dilution mass concentration storing solution 0.045%, 0.065%,
0.075% perfuming concentration gradient, respectively perfuming in delicate fragrance type cigarette Yuxi (soft), Hongta (1956) pipe blend in
(1g ethanol：100g pipe tobaccos).
3rd, cigarette is smoked panel test
Smoked panel test expert by 7-9 name national, provincial level cigarette, sense organ matter is carried out to cigarette made from embodiment 4 and embodiment 5
Amount and its odor type style are smoked panel test evaluation, and specific progress Sensory Quality of Cigarette and its odor type style are secretly commented.
Smoked panel test standard using smoke panel test standard, fragrance consistency profiles of national standard GB5606.4-2005 Sensory Quality of Cigarette.
In flavor type of cigarette style is smoked panel test, mainly according to the delicate fragrance type of flavor type of cigarette, flat-flavor, the main body fragrant of Luzhou-flavor
Rhythm：Fresh and sweet, this fragrant, burnt sweet tea of tobacco and its fragrance transmission speed it is fast, in, slow gradient smokes panel test to cigarette sample odor type
(secretly commenting).
Cigarette of smokeing panel test is：Yuxi (soft) control sample (YX0), cigarette shreds mass percent 0.03%, 0.05%,
0.07% different FLOS CHRYSANTHEMI ALBA from Haizhou of China storing solutions, difference perfuming cigarette Yuxi (soft) sample, sample ID YX0.03, YX0.05,
YX0.07；Hongta (1956) control sample (HT0), 0.03%, 0.05%, 0.07% difference of cigarette shreds mass percent
FLOS CHRYSANTHEMI ALBA from Haizhou of China storing solution, difference perfuming cigarette Hongta (1956) sample, sample ID HT0.03, HT0.05, HT0.07.As a result
Such as table 1 below：
The 1st cigarette sample aesthetic quality of experiment of table 1 and its smokeing panel test for odor type main body note
Note：Delicate fragrance type feature：Fragrance is elegant elegant, has fresh and sweet note, fragrance sensing speed is fast, and extension is strong.Represent
Type Yunnan, the flue-cured tobacco and its cigarette in Fujian.Score value is average mark.
It was found from being analyzed from table, all a little higher than control sample of aesthetic quality's score value of the cigarette sample of all perfumings, main body is clear
Fragrant and sweet rhythm is better than control sample；Particularly YX0.05 aesthetic quality's score value is higher than 0.46 point of control sample, HT0.05 higher than pair
In the same old way 0.43 point, fresh and sweet note is relatively best.
After 4 months, the above-mentioned cigarette sample of perfuming, carries out aesthetic quality to experiment cigarette and its odor type style is smoked panel test again
Evaluation, as a result such as table 2 below：
The 2nd cigarette sample aesthetic quality of experiment of table 2 and its smokeing panel test for odor type main body note
Note：Score value is average mark.
It was found from being analyzed from table, all a little higher than control sample of aesthetic quality's score value of cigarette is tested, main body sweetness note is better than
Control sample；Particularly YX0.05 aesthetic quality's score value is higher than 0.48 point of control sample, HT0.05 higher than the 0.44 of control sample
Point, fresh and sweet note is relatively best.
After 8 months, the above-mentioned cigarette sample of perfuming, carries out aesthetic quality to experiment cigarette and its odor type style is smoked panel test again
Evaluation, as a result such as table 3 below：
The 3rd cigarette sample aesthetic quality of experiment of table 3 and its smokeing panel test for odor type main body note
Note：Score value is average mark.
Analyzed from table, demonstrate all a little higher than control sample of aesthetic quality's score value of experiment cigarette again, it is fragrant that main body is fresh and sweet
Rhythm is better than control sample；Particularly YX0.05 aesthetic quality's score value is higher than 0.43 point of control sample, and HT0.05's is higher than control sample
0.45 point, fresh and sweet note is relatively best.
After 11 months, the above-mentioned cigarette sample of perfuming, carries out aesthetic quality to experiment cigarette and its odor type style is commented again
Evaluation is inhaled, as a result such as table 4 below：
The cigarette sample aesthetic quality of the 4th of table 4 experiment and its smokeing panel test for odor type main body note
Note：Score value is average mark.
Analyzed from table, demonstrate all a little higher than control sample of aesthetic quality's score value of experiment cigarette again, it is fragrant that main body is fresh and sweet
Rhythm is better than control sample；Particularly YX0.05 aesthetic quality's score value is higher than 0.41 point of control sample, and HT0.05's is higher than control sample
0.43 point, fresh and sweet note is relatively best.
Generally, FLOS CHRYSANTHEMI ALBA from Haizhou of China is the medicinal plant for having fresh and sweet note, is fit to the sweetness of delicate fragrance type cigarette main body note
Note.In cigarette sample is tested, aesthetic quality's score value is：
YX0.05>YX0.03>YX0.07>Control sample；HT0.05>HT0.03>HT0.07>Control sample.
The degree of delicate fragrance type cigarette main body sweetness note is：
YX0.05>YX0.03>YX0.07>Control sample；HT0.05>HT0.03>HT0.07>Control sample.
Optimal perfuming concentration is：0.05%.
The Flos Chrysanthemi extract with fresh and sweet note that application enhancements water alcohol method obtains, perfuming have sweetness in delicate fragrance type
In the cigarette shreds of note, it is exactly on the basis of inherently there is the delicate fragrance type cigarette of fresh and sweet note, further lifts cigarette
Fresh and sweet note so that cigarette flavor qualitative change obtain more preferably, jealous have more fresh and sweet note.
Above content is to combine the further description that specific preferred embodiment is done to the present invention, is easy to this skill
Art those skilled in the art is understood that and using the present invention, it is impossible to assert that the specific implementation of the present invention is confined to these and said
It is bright.For those skilled in the art, without departing from the inventive concept of the premise, it can also make
Some simple deductions and replacement, without by performing creative labour.Therefore, those skilled in the art's taking off according to the present invention
Show, the improvement made to the present invention all should be within protection scope of the present invention.
Claims (8)
- A kind of 1. method improved water extraction and alcohol precipitation method extraction plant and cause perfumery, it is characterised in that：Comprise the following steps：Step（1）, prepare primary extraction liquidGround plant is soaked in water 10 minutes or so, is ultrasonically treated 0.5 ± 0.15 hour, it is small then to boil 1 ± 0.2 When, residue is filtered, obtains primary extraction liquid；Step（2）, prepare two level extract solutionEthanol is added in primary extraction liquid, until the ethanol mass concentration of primary extraction liquid reaches 75% or so, is then refrigerated, Perfumery to be caused is dissolved in ethanol, filtering precipitate, obtains two level extract solution；Step（3）, prepare storing solutionAfter two level extract solution is concentrated into relative density 1.08-1.15, propane diols is added, until two level extract solution mass concentration is 10 ± 2%, that is, obtain causing the storing solution of perfumery containing plant.
- 2. the method according to claim 1 improved water extraction and alcohol precipitation method extraction plant and cause perfumery, it is characterised in that：Step （1）In, the plant is the one or more of combination of FLOS CHRYSANTHEMI ALBA from Haizhou of China, chrysanthemum indicum and Huai Chrysanthemi.
- 3. the method according to claim 1 improved water extraction and alcohol precipitation method extraction plant and cause perfumery, it is characterised in that：Step （1）In, plant mill to 40 mesh or so, ground plant is soaked in water, and the quality of water is the 4 of ground plant quality Times.
- 4. the method according to claim 1 improved water extraction and alcohol precipitation method extraction plant and cause perfumery, it is characterised in that：Step （2）In, the time of refrigeration is 10 hours.
- 5. the method according to claim 2 improved water extraction and alcohol precipitation method extraction plant and cause perfumery, it is characterised in that：The Hangzhoupro In the volatility and half volatile material of feverfew, the cause perfumery with fresh and sweet note is：Methyl heptenone, levo-camphor, 2- thatches Alcohol, farnesene, ionol, bisabolol and linoleic acid.
- 6. the plant obtained according to claim 1-5 method causes perfumery.
- 7. plant according to claim 6 causes the application of perfumery, it is characterised in that：According to cigarette shreds mass percent, Respectively using the mass concentration of 95% ethanol dilution storing solution as 0.03 ± 0.005%, 0.05 ± 0.005%, 0.07 ± 0.005%, so Perfuming is distinguished afterwards in pipe tobacco.
- 8. plant according to claim 7 causes the application of perfumery, it is characterised in that：The mass ratio of ethanol and pipe tobacco is 1: 100。
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