CN107586576A - A kind of water ion activity combustion gas and its preparation method and application - Google Patents

A kind of water ion activity combustion gas and its preparation method and application Download PDF

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Publication number
CN107586576A
CN107586576A CN201610527645.XA CN201610527645A CN107586576A CN 107586576 A CN107586576 A CN 107586576A CN 201610527645 A CN201610527645 A CN 201610527645A CN 107586576 A CN107586576 A CN 107586576A
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gas
ion activity
combustion gas
water
water ion
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徐建镛
张羽瑶
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    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/36—Hydrogen production from non-carbon containing sources, e.g. by water electrolysis

Abstract

The invention belongs to novel environment friendly energy field, and in particular to a kind of water ion activity combustion gas and its preparation method and application.It by water electrolysis is vaporific hydrogen and oxygen gas mixture that the water ion activity combustion gas, which is, then is equipped with the novel gas that oil liquefied gas or natural gas are mixed to form, and compared with the combustion gas of prior art, combustion heat value and the integrated cost of water ion activity combustion gas have greater advantage；And the product after burning is mainly water, almost realizes " zero-emission ", this tackles the problem of environmental pollution of getting worse to the whole society, not less than for a big Gospel.

Description

A kind of water ion activity combustion gas and its preparation method and application
Technical field
The invention belongs to novel environment friendly energy field, and in particular to a kind of water ion activity combustion gas and preparation method thereof and should With.
Background technology
The gas class A fuel A being widely used at present, form major class on it is all relatively simple, as natural gas, oil liquefied gas, Coal gas, biogas etc., corresponding combustion heat value is all than relatively low.The combustion gas similar with the present invention, if DME manufactured gas, manufactured fuel gases are with oil or coal As raw material, alkanes mixed gas is generated, then to be equipped with dimethyl ether (DME) combustion-supporting.Although combustion heat value improves, Integrated cost is also very high.The representative formula and performance of this kind of combustion gas are shown in Table 1：
Table 1
The content of the invention
In view of the above the shortcomings that prior art, it is an object of the invention to provide a kind of water ion activity combustion gas and its Preparation method and application, it by water electrolysis is vaporific hydrogen and oxygen gas mixture that the water ion activity combustion gas, which is, then is equipped with L. P. G The novel gas that gas or natural gas are mixed to form, compared with the combustion gas of prior art, the combustion heat value of water ion activity combustion gas with Integrated cost has greater advantage；And the product after burning is mainly water, almost realizes " zero-emission ", this is tackled to the whole society The problem of environmental pollution of getting worse, not less than for a big Gospel.
In order to achieve the above objects and other related objects, first aspect present invention provides a kind of water ion activity combustion gas, main To include each component of following percent by volume：
Hydrogen 50-58%；Preferably, 52-57%；Such as：50-52%, 52-53%, 53-54%, 54-55% or 55- 57%；
Oxygen 25-29%；Preferably, 26-28%；Such as：25-26%, 26-27%, 27-28% or 28-29%；
Paraffin gas 3.4-12%；
Water vapour 9-12%, such as 9-10%, 10-11% or 11-12%.
Preferably, the paraffin gas is methane, and the percent by volume of methane is 5-12%, more preferably 6-11%, such as 5-7.88% or 7.88-12%.
Preferably, the paraffin gas includes propane and iso-butane, and the percent by volume of propane is 2.5-8%, more preferably For 3.5-6%, such as 2.5-3.56%, 3.56-4.39%, 4.39-5% or 5-8%, the percent by volume of iso-butane is 0.9- 3%, more preferably 1.2-2%, such as 0.9-1.28%, 1.28-1.58%, 1.58-1.82% or 1.82-3%.
Preferably, the water ion activity combustion gas is the vaporific hydrogen and oxygen gas mixture and oil liquefied gas obtained by water electrolysis Or natural gas mixed preparing forms.
It is highly preferred that vaporific hydrogen and oxygen gas mixture includes hydrogen, oxygen and water vapour, water vapour is with H3O+- OH- forms In the presence of.
It is highly preferred that the volume ratio of vaporific hydrogen and oxygen gas mixture and oil liquefied gas or natural gas is 87-96:4-13, enter One step is more preferably 90-94：6-10 or 88-93：7-12, such as 87-90:10-13、90-91.58：8.42-10、91.58- 92.15：7.85-8.42、92.15-95.63：4.37-7.85 or 95.63-96：4-4.37.
A kind of colourless volatile liquid that oil liquefied gas is obtained by refinery gas or natural gas pressurization cooling liquefaction, its is main Composition is propane and iso-butane.
Natural gas is the general designation for being present in the mixed gas in subsurface rock reservoir based on hydrocarbon, and its main component is Methane.
Second aspect of the present invention provides the preparation method of above-mentioned water ion activity combustion gas, comprises the following steps：
1) water electrolysis is obtained into vaporific hydrogen and oxygen gas mixture；
2) the vaporific hydrogen and oxygen gas mixture for obtaining step 1) mixes with oil liquefied gas or natural gas, that is, obtains the water Ion activity combustion gas.
Preferably, in step 1), adding water in electrolytic cell, the pH for controlling water is 7.5~9, and voltage is 350~400V, Electric current is 50-130A, and cathode product and anodic product are mixed, that is, obtain vaporific hydrogen and oxygen gas mixture.
It is highly preferred that by adding alkali into water, the pH for controlling water is 7.5~9, and even more preferably, the alkali is Sodium hydroxide or potassium hydroxide.
Preferably, the volume ratio of vaporific hydrogen and oxygen gas mixture and oil liquefied gas or natural gas is 87-96:4-13, enter one Step is more preferably 90-94：6-10 or 88-93：7-12, such as 87-90:10-13、90-91.58：8.42-10、91.58- 92.15：7.85-8.42、92.15-95.63：4.37-7.85 or 95.63-96：4-4.37.
Third aspect present invention provides the purposes of above-mentioned water ion activity combustion gas, for heating, roasting, metal smelt, hair Electricity or resident living.
As a kind of novel gas, water ion activity combustion gas has：Cost of material is low；High heating value；High flame temperature；Use Safely, conveniently；Low cost；Energy-conserving and environment-protective；The advantages that widely used, now it is described below：
1st, the energy source main matter of water ion activity combustion gas is water, and the product after burning is water vapour, substantially without dirt Contaminate thing discharge；
2nd, the combustion heat value of water ion activity combustion gas between 47-50MJ/m3 (12000 kilocalories or so)；
3rd, water ion activity combustion gas aerogenesis 1m3, only need 250ML water purification, consumption about 1.4-1.8 degree electricity；50-90L is equipped with again Natural gas, integrated cost are about 1.8-2.0 yuans, are other all kinds of combustion gas, fuel oil, the 35%-60% of coal-fired cost；
4th, water ion activity fuel gas buring flame temperature reaches as high as 1300 DEG C；And there is poecilothermia, i.e., according to different Requirement carrys out flexible modulation, and adjustable temperature scope is 900-1300 DEG C.
5th, water ion activity combustion gas in-service pipeline and source of the gas path pressure ＜ 0.09MPa-0.125MPa, belong to uncontrolled pressure Equipment container scope, it is operationally safer with respect to controlled pressure equipment；
6th, 20 times faster than gasoline of water ion activity fuel gas buring speed, can completely burned；
7th, water ion activity fuel gas buring flame stabilization, pulse free, phenomena such as fire, over-emitting black exhaust, tobacco is taken off；
8th, the combustion gas of water ion activity belongs to active gases, has combustion catalysis.It can be remixed with other combustion gas Mode accelerates catalysis burning and improves the calorific value and flame temperature of air mixture.Can be that client matches source of the gas in proportion, directly Synchronous access supply network：First, fuel gases calorific value is improved；2nd, reduce combustion gas cost and either reduce gas consumption；3rd, carbon row is reduced Put；
9th, the combustion gas of water ion activity is smaller than atmospheric density, and top and the diffusion of air are only vertically floated towards after leakage；
10th, the combustion gas of water ion activity is not in the gassing accident as other combustion gas, will not endanger the body of personnel Health；
11st, the alternative coal of water ion activity combustion gas of the invention, natural gas, oil liquefied gas, electric power, heavy oil, diesel oil, Alcohol-based fuel equal energy source, it is widely used in the every field such as heating, roasting, metal smelt, generating, resident living.
Embodiment
Instantiation is set forth below the present invention is expanded on further, it should be appreciated that instantiation is not intended to limit the present invention's Protection domain.
The vaporific hydrogen and oxygen gas mixtures of embodiment 1-12 obtain water ion activity with oil liquefied gas or natural gas mixed preparing Combustion gas
The preparation of vaporific hydrogen and oxygen gas mixture：
Raw material：Pure water and sodium hydroxide；
Condition：PH=7.5~9, voltage are 350~400V, and this embodiment takes 380V, electric current 50-130A, this embodiment Take 130A；
Pure water is added in electrolytic cell and is electrolysed, is 7.5~9 by adding sodium hydroxide to control pH, negative electrode is produced Thing and anodic product mixing obtain vaporific hydrogen and oxygen gas mixture, due to containing water vapour (H in hydrogen and oxygen gas mixture3O+— OH-), therefore in vaporific.
By the above-mentioned vaporific hydrogen and oxygen gas mixture and oil liquefied gas or natural gas being prepared according to following distribution scheme Mixed preparing is carried out, is shown in Table 2：
The distribution scheme of table 2
Vaporific hydrogen and oxygen gas mixture obtains the test of water ion activity combustion gas with oil liquefied gas or natural gas mixed preparing Parameter
● using the distribution scheme of embodiment 2, the test parameter of its water ion activity combustion gas is shown in Table 3, and composition is shown in Table 4, combustion Burn thing composition and be shown in Table 5.
The test parameter of the water ion activity combustion gas of table 3
The composition of the water ion activity combustion gas of table 4
Sequence number Component title Content/% CAS registration numbers Remarks
1 Propane 5.05 74-98-6
2 Ethane 0.11 74-84-0
3 Ethene 0.16 74-85-1
4 Propylene 0.32 115-07-1
5 Iso-butane 1.82 75-28-5
6 Normal butane 0.60 106-97-8
7 N-butene 0.16 106-98-9
8 Isobutene 0.23 115-11-7
9 Maleic 0.01 ---
10 N-pentene 0.01 109-67-1
11 Anti- amylene 0.44 646-04-8
12 Isopentane 0.02 78-78-4
13 Butadiene --- 106-99-0 Do not detect
14 Carbon monoxide (CO) --- 630-08-0 Do not detect
15 Carbon dioxide (CO2) --- 124-38-9 Do not detect
16 Nitric oxide (NO) 0.01 10102-43-9
17 Nitrogen dioxide (NO2) --- 10102-44-0 Do not detect
18 Other alkane derivatives 0.81 ---
19 Oxygen (O2) 27.08 7782-44-7 Main Ingredients and Appearance
20 Hydrogen (H2) 54.17 1333-74-0 Main Ingredients and Appearance
21 Water vapour 9
It is total 100.00
The water ion activity fuel gas buring thing composition of table 5
Sequence number Component title Content/% CAS registration numbers Remarks
1 Oxygen (O2) 1.81 7782-44-7 Adulterated in air
2 Nitrogen (N2) 4.26 7727-37-9 Adulterated in air
3 Carbon monoxide (CO) 0.000021 630-08-0
4 Carbon dioxide (CO2) 3.25 124-38-9
5 Nitric oxide (NO) --- 10102-43-9
6 Nitrogen dioxide (NO2) 0.000004 10102-44-0
7 Alkane micromolecular 0.09 Burn insufficient product
8 H2O (gas) 90.59 7732-18-5 Main Ingredients and Appearance
It is total 100.00
● using the distribution scheme of embodiment 4, the test parameter of its water ion activity combustion gas is shown in Table 6, and composition is shown in Table 7, combustion Burn thing composition and be shown in Table 8.
The test parameter of the water ion activity combustion gas of table 6
Flash-point -26℃ Critical pressure 4.11MPa
Fusing point <-80℃ Saturated vapor 120.1KPa(50℃)
Boiling point <-80℃ Relative steam density 1.342g/L
Critical-temperature 295℃ Combustion heat value 49.33MJ/Nm3
The composition of the water ion activity combustion gas of table 7
The water ion activity fuel gas buring thing composition of table 8
Sequence number Component title Content/% CAS registration numbers Remarks
1 Oxygen (O2) 1.72 7782-44-7 Adulterated in air
2 Nitrogen (N2) 4.21 7727-37-9 Adulterated in air
3 Carbon monoxide (CO) 0.000021 630-08-0
4 Carbon dioxide (CO2) 3.04 124-38-9
5 Nitric oxide (NO) --- 10102-43-9
6 Nitrogen dioxide (NO2) 0.000004 10102-44-0
7 Alkane micromolecular 0.07 Burn insufficient product
8 H2O (gas) 91.03 7732-18-5 Main Ingredients and Appearance
It is total 100.00
● using the distribution scheme of embodiment 6, the test parameter of its water ion activity combustion gas is shown in Table 9, and composition is shown in Table 10, combustion Burn thing composition and be shown in Table 11.
The test parameter of the water ion activity combustion gas of table 9
Flash-point -28℃ Critical pressure 3.96MPa
Fusing point <-80℃ Saturated vapor 118.7KPa(50℃)
Boiling point <-80℃ Relative steam density 1.321g/L
Critical-temperature 292℃ Combustion heat value 45.62MJ/Nm3
The composition of the water ion activity combustion gas of table 10
The water ion activity fuel gas buring thing composition of table 11
Sequence number Component title Content/% CAS registration numbers Remarks
1 Oxygen (O2) 1.65 7782-44-7 Adulterated in air
2 Nitrogen (N2) 4.15 7727-37-9 Adulterated in air
3 Carbon monoxide (CO) 0.000021 630-08-0
4 Carbon dioxide (CO2) 2.82 124-38-9
5 Nitric oxide (NO) --- 10102-43-9
6 Nitrogen dioxide (NO2) 0.000004 10102-44-0
7 Alkane micromolecular 0.06 Burn insufficient product
8 H2O (gas) 91.33 7732-18-5 Main Ingredients and Appearance
It is total 100.00
● using the distribution scheme of embodiment 7, the test parameter of its water ion activity combustion gas is shown in Table 12, and composition is shown in Table 13, Comburant composition is shown in Table 14.
The test parameter of the water ion activity combustion gas of table 12
Flash-point -26℃ Critical pressure 4.06MPa
Fusing point <-80℃ Saturated vapor 120.3KPa(50℃)
Boiling point <-80℃ Relative steam density 1.351g/L
Critical-temperature 297℃ Combustion heat value 45.12MJ/Nm3
The composition of the water ion activity combustion gas of table 13
The water ion activity fuel gas buring thing composition of table 14
Sequence number Component title Content/% CAS registration numbers Remarks
1 Oxygen (O2) 1.86 7782-44-7 Adulterated in air
2 Nitrogen (N2) 4.39 7727-37-9 Adulterated in air
3 Carbon monoxide (CO) 0.000028 630-08-0
4 Carbon dioxide (CO2) 3.44 124-38-9
5 Nitric oxide (NO) --- 10102-43-9
6 Nitrogen dioxide (NO2) 0.000005 10102-44-0
7 Alkane micromolecular 0.06 Burn insufficient product
8 H2O (gas) 90.25 7732-18-5 Main Ingredients and Appearance
It is total 100.00
● using the distribution scheme of embodiment 9, the test parameter of its water ion activity combustion gas is shown in Table 15, and composition is shown in Table 16, Comburant composition is shown in Table 17.
The test parameter of the water ion activity combustion gas of table 15
Flash-point -26℃ Critical pressure 3.96MPa
Fusing point <-80℃ Saturated vapor 119..3KPa(50℃)
Boiling point <-80℃ Relative steam density 1.344g/L
Critical-temperature 297℃ Combustion heat value 48.77MJ/Nm3
The composition of the water ion activity combustion gas of table 16
Sequence number Component title Content/% CAS registration numbers Remarks
1 Methane 7.88 74-82-8
2 Ethane 0.19 74-84-0
3 Iso-butane 0.11 75-28-5
4 Normal butane 0.04 106-97-8
5 Hydrogen sulfide (H2S) 0.07 7783-06-4
6 Nitrogen (N2) 0.05 7727-37-9
7 Carbon monoxide (CO) --- 630-08-0 Do not detect
8 Carbon dioxide (CO2) 0.01 124-38-9
9 Nitric oxide (NO) 0.01 10102-43-9
10 Nitrogen dioxide (NO2) --- 10102-44-0 Do not detect
11 Other alkane derivatives 0.07 ---
12 Oxygen (O2) 26.85 7782-44-7 Main Ingredients and Appearance
13 Hydrogen (H2) 53.72 1333-74-0 Main Ingredients and Appearance
14 Water vapour 11
It is total 100.00
The water ion activity fuel gas buring thing composition of table 17
● using the distribution scheme of embodiment 12, the test parameter of its water ion activity combustion gas is shown in Table 18, and composition is shown in Table 19, Comburant composition is shown in Table 20.
The test parameter of the water ion activity combustion gas of table 18
Flash-point -25℃ Critical pressure 3.95MPa
Fusing point <-80℃ Saturated vapor 118..4KPa(50℃)
Boiling point <-80℃ Relative steam density 1.337g/L
Critical-temperature 296℃ Combustion heat value 45.47MJ/Nm3
The composition of the water ion activity combustion gas of table 19
The water ion activity fuel gas buring thing composition of table 20
Sequence number Component title Content/% CAS registration numbers Remarks
1 Oxygen (O2) 1.77 7782-44-7 Adulterated in air
2 Nitrogen (N2) 4.02 7727-37-9 Adulterated in air
3 Carbon monoxide (CO) 0.000027 630-08-0
4 Carbon dioxide (CO2) 2.38 124-38-9
5 Nitric oxide (NO) --- 10102-43-9
6 Nitrogen dioxide (NO2) 0.000005 10102-44-0
7 Alkane micromolecular 0.05 Burn insufficient product
8 H2O (gas) 91.78 7732-18-5 Main Ingredients and Appearance
It is total 100.00

Claims (10)

1. a kind of water ion activity combustion gas, it is characterised in that mainly include each component of following percent by volume：
Hydrogen 50-58%；
Oxygen 25-29%；
Paraffin gas 3.4-12%；
Water vapour 9-12%.
2. water ion activity combustion gas as claimed in claim 1, it is characterised in that the paraffin gas is methane, the body of methane Product percentage is 5-12%.
3. water ion activity combustion gas as claimed in claim 1, it is characterised in that the paraffin gas includes propane and isobutyl Alkane, the percent by volume of propane is 2.5-8%, and the percent by volume of iso-butane is 0.9-3%.
4. water ion activity combustion gas as claimed in claim 1, it is characterised in that the water ion activity combustion gas is by water electrolysis Obtained vaporific hydrogen and oxygen gas mixture and oil liquefied gas or natural gas mixed preparing forms.
5. water ion activity combustion gas as claimed in claim 4, it is characterised in that vaporific hydrogen and oxygen gas mixture includes hydrogen, oxygen Gas and water vapour.
6. water ion activity combustion gas as claimed in claim 4, it is characterised in that vaporific hydrogen and oxygen gas mixture and oil liquefied gas Or the volume ratio of natural gas is 87-96:4-13.
7. the preparation method of the water ion activity combustion gas as described in any one of claim 1 to 6, it is characterised in that including as follows Step：
1) water electrolysis is obtained into vaporific hydrogen and oxygen gas mixture；
2) the vaporific hydrogen and oxygen gas mixture for obtaining step 1) mixes with oil liquefied gas or natural gas, that is, obtains the water ion Active combustion gas.
8. the preparation method of water ion activity combustion gas as claimed in claim 7, it is characterised in that in step 1), add water to In electrolytic cell, the pH for controlling water is 7.5-9, voltage 350-400V, electric current 50-130A, by cathode product and anodic product Mixing, that is, obtain vaporific hydrogen and oxygen gas mixture.
9. the preparation method of water ion activity combustion gas as claimed in claim 7, it is characterised in that vaporific hydrogen and oxygen gas mixture with The volume ratio of oil liquefied gas or natural gas is 87-96:4-13.
10. described water ion activity combustion gas as described in any one of claim 1 to 6 be used for heating, roasting, metal smelt, Generating or resident living.
CN201610527645.XA 2016-07-06 2016-07-06 A kind of water ion activity combustion gas and its preparation method and application Pending CN107586576A (en)

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Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN101498456A (en) * 2008-02-01 2009-08-05 佐藤利五郎 Apparatus for generating electrolytic gas composite fuel, and method for generating this fuel
CN101935565A (en) * 2009-06-29 2011-01-05 北京奥润泰克教育科技有限责任公司 Low-carbon gas fuel and preparation method thereof
CN202203980U (en) * 2011-08-29 2012-04-25 张维萍 Energy-saving combustion device adopting combustion method of water electrolysis oxyhydrogen and fuel blending
KR101532508B1 (en) * 2014-01-27 2015-06-29 충남대학교산학협력단 a mixture fuel of water electrolysis gas and the water vapor, and this mixture blended fossil fuel, and the combustion method with these

Patent Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN101498456A (en) * 2008-02-01 2009-08-05 佐藤利五郎 Apparatus for generating electrolytic gas composite fuel, and method for generating this fuel
CN101935565A (en) * 2009-06-29 2011-01-05 北京奥润泰克教育科技有限责任公司 Low-carbon gas fuel and preparation method thereof
CN202203980U (en) * 2011-08-29 2012-04-25 张维萍 Energy-saving combustion device adopting combustion method of water electrolysis oxyhydrogen and fuel blending
KR101532508B1 (en) * 2014-01-27 2015-06-29 충남대학교산학협력단 a mixture fuel of water electrolysis gas and the water vapor, and this mixture blended fossil fuel, and the combustion method with these

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