CN104122576B - Solid state nuclear track detector is utilized to measure the method and device of 218Po long-time average deposition rate - Google Patents
Solid state nuclear track detector is utilized to measure the method and device of 218Po long-time average deposition rate Download PDFInfo
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- CN104122576B CN104122576B CN201410373948.1A CN201410373948A CN104122576B CN 104122576 B CN104122576 B CN 104122576B CN 201410373948 A CN201410373948 A CN 201410373948A CN 104122576 B CN104122576 B CN 104122576B
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Abstract
One utilizes solid state nuclear track detector to measure218The method and device of Po long-time average deposition rate, during measurement, is fixed on the bottom of measurement apparatus casing and measures metope indoor in environment, and on ground or ceiling top, the measurement time is that the value of T, T is according to measuring requirement for a couple of days to hundreds of skies.After measurement process completes, take off the first solid state nuclear track detector, the second solid state nuclear track detector and the 3rd solid state nuclear track detector immediately, and it is carried out chemical etching, read the nuclear track number on the first solid state nuclear track detector, the second solid state nuclear track detector and the 3rd solid state nuclear track detector respectively, and by being calculated218The long-time average deposition rate of Po.
Description
Technical field
The present invention relates to a kind of nuclear radiation detection technology, particularly one utilizes solid state nuclear track detector to measure218Po length
The method and device of time average deposition rate.
Background technology
In air ambient, radon is the main source of natural radiation suffered by human body, inherently sees, human body is exhaled by the daughter of radon
Desorption system radiation is the major reason causing lung cancer.Radon in air has222Rn and220Rn, due to222Rn concentration is typically remote high
In220Rn concentration, environment activity is mainly monitored object and is exactly222The daughter of Rn, wherein218Po is222In Rn decay chain first
Level, has particularly important meaning.Traditional active measuring method is usually and uses filter membrane to sample the radon daughter in air,
Then being analyzed by tale or Method of Energy Spectrum Analysis obtains the concentration of Radon daughter, the method is accurately quick, but only
The data of sampling time section can be reflected, it is impossible to obtain long average data.Affect in room air218Po concentration because of
Element mainly has222The concentration of Rn, ventilation rate and218Po deposition these three parameter is so-called218In Po deposition is exactly the unit interval
In unit are body of wall, ground or roof deposition218The activity of Po.
Summary of the invention
It is an object of the invention to overcome the above-mentioned deficiency of prior art to provide one to utilize solid state nuclear track detector to survey
Amount218The method and device of Po long-time average deposition rate.
The technical scheme is that one utilizes solid state nuclear track detector to measure218Po long-time average deposition rate
Method, its concrete measuring method is as follows:
A, measurement process:
The bottom of measurement apparatus casing is fixed on and measures metope indoor in environment or ground or ceiling
On top, being provided with three solid state nuclear track detectors in the casing of measurement apparatus, three solid state nuclear track detectors are respectively first
Solid state nuclear track detector, the second solid state nuclear track detector and the 3rd solid state nuclear track detector, the first solid state nuclear track is visited
The surface area surveying device is S1, the surface area of the second solid state nuclear track detector is S2, the surface area of the 3rd solid state nuclear track detector
For S3, and meet: S1≤S2≤S3。
It is D that the surface of the second solid state nuclear track detector is coated with thickness1Primary diaphragm, the surface configuration of primary diaphragm with
The surface configuration of the second solid state nuclear track detector is the same.It is D that the surface of the 3rd solid state nuclear track detector is coated with thickness2The
Two diaphragms, the surface configuration of secondary diaphragm is as the surface configuration of the 3rd solid state nuclear track detector.The thickness of primary diaphragm
D1Thickness D less than secondary diaphragm2, primary diaphragm can stop222Rn daughter218The particle of the 6MeV that Po decay produces gets to second
On solid state nuclear track detector, secondary diaphragm can stop222Rn daughter218Po and2146MeV's and 7.69MeV that Po decay produces
Particle is got on the 3rd solid state nuclear track detector.
The surface of the first solid state nuclear track detector is not covered with diaphragm,220Rn daughter212The 8.78MeV that Po decay produces
Particle can get on first, second, third solid state nuclear track detector.
The measurement time is that the value of T, T is according to measuring requirement for a couple of days to hundreds of skies.
B, calculating process:
Random time t during measuring, deposited per area unit on solid state nuclear track detector222Rn daughter activity
Be changed to:
APo214(t)=ABi214(t) (4)
In formula: APo218(t)、APb214(t)、ABi214(t)、APo214T () is respectively218Po、 214Pb、214Bi、214Po is at solid
Activity on nuclear track detector;DPo218、DPb214、DBi214It is218Po、214Pb、214The deposition of Bi;λPo218、λPb214、λBi214
It is218Po、214Pb、 214The decay coefficient of Bi.
Owing in measurement apparatus, the high frame of casing blocks what chamber internal surface directly separated out220Rn and short life son
Body arrives the surface of solid core detector, only considers its long-life daughter.Deposited per area unit on solid state nuclear track detector
's220Rn long-life daughter212Pb、 212Bi、212The change of Po activity is respectively as follows: APb212(t)、ABi212(t)、APo212(t)。
After measurement process completes, take off the first solid state nuclear track detector, the second solid state nuclear track detector and immediately
Three solid state nuclear track detectors, and it is carried out chemical etching, read the first solid state nuclear track detector, the second solid core respectively
Nuclear track number on track detector and the 3rd solid state nuclear track detector.
Particle track number N on first solid state nuclear track detector1For:
η in formula1Po218、η1Po214、η1Bi212、η1Po212Represent the first solid state nuclear track detector pair respectively218Po、214Po、212Bi、212The detection efficient of the decay of Po, wherein due to218Po、 212The particle energy that Bi decay produces is close, and it detects effect
Rate is the most identical.
Particle track number N on second solid state nuclear track detector2For:
η in formula2Po214、η2Po212Represent the second solid state nuclear track detector pair respectively214Po、 212The detection of the decay of Po
Efficiency.
Particle track number N on 3rd solid state nuclear track detector3For:
η in formula3Po212Represent the 3rd solid state nuclear track detector pair212The detection efficient of the decay of Po.
According to220Rn decay chain is the most available:
APo212(t)=0.64ABi212(t) (8)
Be can get by formula (5), (6), (7), (8):
Just can be solved by formula (9)D just can be back-calculated to obtain again by formula (1)Po218I.e.218Po's is long-time flat
All depositions.
The measurement apparatus that said method uses includes casing, and casing is a lower end closed, the container of upper end open, casing
Cavity heights h be 2~8cm.Be provided with the first solid state nuclear track detector on the base plate of casing, the second solid state nuclear track is visited
Surveying device and the 3rd solid state nuclear track detector, the first solid state nuclear track detector, the second solid state nuclear track detector and the 3rd are solid
Body nuclear track detector is attached on the base plate of casing respectively by the way of bonding.The surface area of the first solid state nuclear track detector
For S1, the surface area of the second solid state nuclear track detector is S2, the surface area of the 3rd solid state nuclear track detector is S3, and meet:
S1≤S2≤S3.It is D that the surface of the second solid state nuclear track detector is coated with thickness1Primary diaphragm, the surface configuration of primary diaphragm
As the surface configuration of the second solid state nuclear track detector.It is D that the surface of the 3rd solid state nuclear track detector is coated with thickness2
Secondary diaphragm, the surface configuration of secondary diaphragm is as the surface configuration of the 3rd solid state nuclear track detector.The thickness of primary diaphragm
Degree D1Thickness D less than secondary diaphragm2。
The present invention compared with prior art has a characteristic that
Measurement apparatus, measurement process and computational methods that the present invention provides are simple, it is possible to measure218Po is the most heavy
Long-pending rate.
Below in conjunction with the drawings and specific embodiments, the detailed construction of the present invention is further described.
Accompanying drawing explanation
Accompanying drawing 1 is the structural representation of the present invention;
Accompanying drawing 2 is the A-A sectional view in accompanying drawing 1.
Detailed description of the invention
One utilizes solid state nuclear track detector to measure218The method of Po long-time average deposition rate, its concrete measuring method
As follows:
A, measurement process:
The bottom of measurement apparatus casing 1 is fixed on and measures metope indoor in environment or ground or ceiling
On top, being provided with three solid state nuclear track detectors in the casing 1 of measurement apparatus, three solid state nuclear track detectors are respectively first
Solid state nuclear track detector the 2, second solid state nuclear track detector 3 and the 3rd solid state nuclear track detector 5, the first solid state nuclear track
The surface area of detector 2 is S1, the surface area of the second solid state nuclear track detector 3 is S2, the 3rd solid state nuclear track detector 5
Surface area is S3, and meet: S1≤S2≤S3。
It is D that the surface of the second solid state nuclear track detector 3 is coated with thickness1Primary diaphragm 4, the surface shape of primary diaphragm 4
The surface configuration of shape and the second solid state nuclear track detector 3 is the same.The surface of the 3rd solid state nuclear track detector 5 is coated with thickness
For D2Secondary diaphragm 6, the surface configuration of secondary diaphragm 6 is as the surface configuration of the 3rd solid state nuclear track detector 5.First film
The thickness D of sheet 41Thickness D less than secondary diaphragm 62, primary diaphragm 4 can stop222Rn daughter218The 6MeV's that Po decay produces
Particle is got on the second solid state nuclear track detector 3, and secondary diaphragm 6 can stop222Rn daughter218Po and214Po decay produces
The particle of 6MeV and 7.69MeV is got on the 3rd solid state nuclear track detector 5.
The surface of the first solid state nuclear track detector 2 is not covered with diaphragm,220Rn daughter212Po decay produces
The particle of 8.78MeV can get to first solid state nuclear track detector the 2, second solid state nuclear track detector the 3, the 3rd solid core footpath
On mark detector 5.
The measurement time is that the value of T, T is according to measuring requirement for a couple of days to hundreds of skies.
B, calculating process:
Random time t during measuring, deposited per area unit on solid state nuclear track detector222Rn daughter activity
Be changed to:
APo214(t)=ABi214(t) (4)
In formula: APo218(t)、APb214(t)、ABi214(t)、APo214T () is respectively218Po、 214Pb、214Bi、214Po is at solid
Activity on nuclear track detector;DPo218、DPb214、DBi214It is218Po、214Pb、214The deposition of Bi;λPo218、λPb214、λBi214
It is218Po、214Pb、 214The decay coefficient of Bi.
Owing in measurement apparatus, the high frame of casing 1 blocks what chamber internal surface directly separated out220Rn and short life son
Body arrives the surface of solid core detector, only considers its long-life daughter.Deposited per area unit on solid state nuclear track detector
's220Rn long-life daughter212Pb、212Bi、212The change of Po activity is respectively as follows: APb212(t)、ABi212(t)、APo212(t)。
After measurement process completes, take off first solid state nuclear track detector the 2, second solid state nuclear track detector 3 and immediately
3rd solid state nuclear track detector 5, and it is carried out chemical etching, read the first solid state nuclear track detector 2, second respectively solid
Nuclear track number on body nuclear track detector 3 and the 3rd solid state nuclear track detector 5.
Particle track number N on first solid state nuclear track detector 21For:
η in formula1Po218、η1Po214、η1Bi212、η1Po212Represent that the first solid state nuclear track detector 2 is right respectively218Po、214Po
、212Bi、212The detection efficient of the decay of Po, wherein due to218Po、212The particle energy that Bi decay produces is close, its detection
Efficiency is the most identical.
Particle track number N on second solid state nuclear track detector 32For:
η in formula2Po214、η2Po212Represent that the second solid state nuclear track detector 3 is right respectively214Po、212The detection of the decay of Po
Efficiency.
Particle track number N on 3rd solid state nuclear track detector 53For:
η in formula3Po212Represent that the 3rd solid state nuclear track detector 5 is right212The detection efficient of the decay of Po.
According to220Rn decay chain is the most available:
APo212(t)=0.64ABi212(t) (8)
Be can get by formula (5), (6), (7), (8):
Just can be solved by formula (9)D just can be back-calculated to obtain again by formula (1)Po218I.e.218Po's is long-time flat
All depositions.
The measurement apparatus that said method uses includes that casing 1, casing 1 are a lower end closed, the container of upper end open, case
The cavity heights h of body 1 is 2~8cm.The base plate of casing 1 is provided with first solid state nuclear track detector the 2, second solid core footpath
Mark detector 3 and the 3rd solid state nuclear track detector 5, first solid state nuclear track detector the 2, second solid state nuclear track detector 3
It is attached on the base plate of casing 1 by the way of bonding respectively with the 3rd solid state nuclear track detector 5.First solid state nuclear track detection
The surface area of device 2 is S1, the surface area of the second solid state nuclear track detector 3 is S2, the surface of the 3rd solid state nuclear track detector 5
Amass as S3, and meet: S1≤S2≤S3.It is D that the surface of the second solid state nuclear track detector 3 is coated with thickness1Primary diaphragm 4, the
The surface configuration of one diaphragm 4 is as the surface configuration of the second solid state nuclear track detector 3.3rd solid state nuclear track detector 5
To be coated with thickness be D on surface2The table of secondary diaphragm 6, the surface configuration of secondary diaphragm 6 and the 3rd solid state nuclear track detector 5
Face shape is the same.The thickness D of primary diaphragm 41Thickness D less than secondary diaphragm 62。
Claims (3)
1. one kind utilizes solid state nuclear track detector to measure218The method of Po long-time average deposition rate, is characterized in that: it is concrete
Measuring method is as follows:
A, measurement process:
The bottom of measurement apparatus casing is fixed on and measures on metope indoor in environment or ground or ceiling top,
Being provided with three solid state nuclear track detectors in the casing of measurement apparatus, three solid state nuclear track detectors are respectively the first solid core
Track detector, the second solid state nuclear track detector and the 3rd solid state nuclear track detector, the first solid state nuclear track detector
Surface area is S1, the surface area of the second solid state nuclear track detector is S2, the surface area of the 3rd solid state nuclear track detector is S3,
And meet: S1≤S2≤S3;
It is D that the surface of the second solid state nuclear track detector is coated with thickness1Primary diaphragm, the surface configuration of primary diaphragm and second
The surface configuration of solid state nuclear track detector is the same, and it is D that the surface of the 3rd solid state nuclear track detector is coated with thickness2Second film
Sheet, the surface configuration of secondary diaphragm as the surface configuration of the 3rd solid state nuclear track detector, the thickness D of primary diaphragm1Little
Thickness D in secondary diaphragm2, primary diaphragm can stop222Rn daughter218It is solid that the particle of the 6MeV that Po decay produces gets to second
On body nuclear track detector, secondary diaphragm can stop222Rn daughter218Po and214The grain of 6MeV and 7.69MeV that Po decay produces
Son is got on the 3rd solid state nuclear track detector;
The surface of the first solid state nuclear track detector is not covered with diaphragm,220Rn daughter212The grain of the 8.78MeV that Po decay produces
Son can be got on first, second, third solid state nuclear track detector;
The measurement time is that the value of T, T is according to measuring requirement for a couple of days to hundreds of skies;
B, calculating process:
Random time t during measuring, deposited per area unit on solid state nuclear track detector222The change of Rn daughter activity
Turn to:
APo214(t)=ABi214(t) (4)
In formula: APo218(t)、APb214(t)、ABi214(t)、APo214T () is respectively218Po、214Pb、214Bi、214Po is in solid core footpath
Activity on mark detector;DPo218、DPb214、DBi214It is218Po、214Pb、214The deposition of Bi;λPo218、λPb214、λBi214It is218Po、214Pb、214The decay coefficient of Bi;
Owing in measurement apparatus, the high frame of casing blocks what chamber internal surface directly separated out220Rn and short life daughter arrive
Reach the surface of solid core detector, only consider its long-life daughter, deposited per area unit on solid state nuclear track detector220Rn long-life daughter212Pb、212Bi、212The change of Po activity is respectively as follows: APb212(t)、ABi212(t)、APo212(t);
After measurement process completes, take off the first solid state nuclear track detector, the second solid state nuclear track detector and the 3rd immediately solid
Body nuclear track detector, and it is carried out chemical etching, read the first solid state nuclear track detector, the second solid state nuclear track respectively
Nuclear track number on detector and the 3rd solid state nuclear track detector;
Particle track number N on first solid state nuclear track detector1For:
η in formula1Po218、η1Po214、η1Bi212、η1Po212Represent the first solid state nuclear track detector pair respectively218Po、214Po、212Bi
、212The detection efficient of the decay of Po, wherein due to218Po、212The particle energy that Bi decay produces is close, and its detection efficient is also
Identical;
Particle track number N on second solid state nuclear track detector2For:
η in formula2Po214、η2Po212Represent the second solid state nuclear track detector pair respectively214Po、212The detection efficient of the decay of Po;
Particle track number N on 3rd solid state nuclear track detector3For:
η in formula3Po212Represent the 3rd solid state nuclear track detector pair212The detection efficient of the decay of Po;
According to220Rn decay chain is the most available:
APo212(t)=0.64ABi212(t)(8)
Be can get by formula (5), (6), (7), (8):
Just can be solved by formula (9)D just can be back-calculated to obtain again by formula (1)Po218I.e.218The long-time average deposition of Po
Rate.
One the most according to claim 1 utilizes solid state nuclear track detector to measure218The side of Po long-time average deposition rate
Method, is characterized in that: described measurement apparatus includes casing, and casing is a lower end closed, the container of upper end open, at casing
Base plate is provided with the first solid state nuclear track detector, the second solid state nuclear track detector and the 3rd solid state nuclear track detector, the
One solid state nuclear track detector, the second solid state nuclear track detector and the 3rd solid state nuclear track detector are respectively by the side of bonding
Formula is attached on the base plate of casing;It is D that the surface of the second solid state nuclear track detector is coated with thickness1Primary diaphragm, the 3rd solid
It is D that the surface of nuclear track detector is coated with thickness2Secondary diaphragm.
One the most according to claim 2 utilizes solid state nuclear track detector to measure218The side of Po long-time average deposition rate
Method, is characterized in that: the cavity heights h of casing is 2~8cm.
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CN107144871B (en) * | 2017-05-08 | 2019-05-14 | 北京市化工职业病防治院 | Utilize the method for the track morphology of optical microscope inspection solid state nuclear track detector |
CN109307881B (en) * | 2018-11-27 | 2023-06-16 | 衡阳师范学院 | Measurement of 222 Rn、 220 Device and method for eliminating temperature and humidity effect during Rn average concentration |
CN111551979B (en) * | 2020-05-27 | 2022-06-03 | 北京市化工职业病防治院 | Solid nuclear track-based radioactive radon and thorium emanator concentration detection method |
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CN102830418A (en) * | 2012-08-30 | 2012-12-19 | 衡阳师范学院 | Method for open-loop measurement of radon exhalation rate by utilizing total count of 218Po and 214Po |
CN102830417A (en) * | 2012-08-30 | 2012-12-19 | 衡阳师范学院 | Method for closed-loop measurement of radon exhalation rate by utilizing total count of 218Po and 214Po |
CN102830128A (en) * | 2012-08-30 | 2012-12-19 | 衡阳师范学院 | Method for measuring 222Rn (radon) and 220Rn daughters in air by means of alpha energy disperse spectroscopy |
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CN102830418A (en) * | 2012-08-30 | 2012-12-19 | 衡阳师范学院 | Method for open-loop measurement of radon exhalation rate by utilizing total count of 218Po and 214Po |
CN102830417A (en) * | 2012-08-30 | 2012-12-19 | 衡阳师范学院 | Method for closed-loop measurement of radon exhalation rate by utilizing total count of 218Po and 214Po |
CN102830128A (en) * | 2012-08-30 | 2012-12-19 | 衡阳师范学院 | Method for measuring 222Rn (radon) and 220Rn daughters in air by means of alpha energy disperse spectroscopy |
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