CN103875733A - Traditional Chinese medicine for air disinfection and preparation method thereof - Google Patents

Traditional Chinese medicine for air disinfection and preparation method thereof Download PDF

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Publication number
CN103875733A
CN103875733A CN201410128346.XA CN201410128346A CN103875733A CN 103875733 A CN103875733 A CN 103875733A CN 201410128346 A CN201410128346 A CN 201410128346A CN 103875733 A CN103875733 A CN 103875733A
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grams
chinese medicine
kuh
flowered skullcap
wrinkled giant
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CN201410128346.XA
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杨风
杨杰书
于欣
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Qingdao Central Hospital
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Qingdao Central Hospital
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Abstract

The invention discloses a traditional Chinese medicine for air disinfection. The traditional Chinese medicine is prepared from the following medicinal materials by weight: 20g of moxa leaf, 12g of cordate houttuynia, 15g of honeysuckle flower, 8g of hypericum perforatum, 5g of flavescent sophora root, 5g of scutellaria root, 8g of ageratum, 6g of eupatorium, 5g of phellodendron amurense, 6g of magnolia bark, 5g of ligustrum sinense, 8g of radix sanguisorbae and 10g of selfheal spike. A preparation method of the traditional Chinese medicine comprises the steps of weighing the medicinal materials, placing the medicinal materials in a vessel, adding water, of which the weight is 8 times that of the medicinal materials, decocting for 1.5 hours, and filtrating, so as to obtain a filtrate and filtrated residue; adding water, of which the weight is 6 times that of the filtrated residue, into the filtrated residue, decocting for 1 hour, and filtrating, so as to obtain a filtrate and filtrated residue; combining the filtrates, concentrating, drying and filling into capsule shells. Proved by clinical trials, through selecting appropriate medicinal materials and proportioning ratio thereof, the traditional Chinese medicine achieves a remarkable effect on air disinfection, is safe and is free from toxic and side effects.

Description

A kind of Chinese medicine for air sterillization and preparation method thereof
Technical field
The present invention relates to a kind of Chinese medicine, be specifically related to a kind of Chinese medicine for air sterillization and preparation method thereof.
Background technology
Air is the important channel that pathogenic microorganisms is propagated, and it is reported and has in the world 14 kinds of infectious disease air-borne transmissions, and air sterillization is prevent disease, the important measures that prevent cross-infection, is particularly one of the important content of hospital quality management of public place.Hospital personnel density is large, the discarded object that carries disease germs in a large number, the easy contaminated environment of excreta, and floating aerial pathogenic microorganisms can be more, and patient and medical personnel are had to potential harm.At present conventional air disinfection method is chemicals, as physical methods such as the chemical methodes such as Peracetic acid, lactic acid, hydrogen peroxide, formaldehyde, 84 thimerosals, glutaraldehyde and ultraviolet ray irradiation, ozone generators.These methods can be killed pathogenic microorganisms, and fast, valid density is low, obtains good effect, but respectively has certain defect in effect, as poor in toxic, excitant, metal protection, lasting effect; Manyly itself form again pollutant, affect to some extent health, uncomfortable tenant in common's environment; When sterilization, all personnel must leave the theatre, and operating system will have safeguard procedures; After sterilization, peculiar smell can not be eliminated very soon, and long-term use meeting has the danger of accumulate poisoning etc. to human body.Still lack at present the effective Chinese traditional medicine of generally recognized as safe for air sterillization.
Summary of the invention
The present invention aims to provide a kind of Chinese medicine for air sterillization and preparation method thereof, by selecting suitable medicinal material and proportioning thereof, reach to contribute to the remarkable efficacy of air sterillization sterilization, and safe without toxic side effect.
In order to achieve the above object, the present invention is by the following technical solutions: a kind of Chinese medicine for air sterillization, is prepared from by the medicinal material of following weight proportion: 15~20 grams of tarragons, 10~12 grams of cordate houttuynias, 12~15 grams of honeysuckles, 6~8 grams of hypericum perforatums, 4~5 grams of kuh-sengs, 4~5 grams of the roots of large-flowered skullcap, 6~8 grams of wrinkled giant hyssops, 5~6 grams of eupatoriums, 4~5 grams of golden cypresses, 5~6 grams of the barks of official magnolia, 4~5 grams of ligustrum sinenses, 6~8 grams of garden burnets, 8~10 grams of selfheals.
As preferably, be prepared from by the medicinal material of following weight proportion: 20 grams of tarragons, 12 grams of cordate houttuynias, 15 grams of honeysuckles, 8 grams of hypericum perforatums, 5 grams of kuh-sengs, 5 grams of the roots of large-flowered skullcap, 8 grams of wrinkled giant hyssops, 6 grams of eupatoriums, 5 grams of golden cypresses, 6 grams of the barks of official magnolia, 5 grams of ligustrum sinenses.
As preferably, be prepared from by the medicinal material of following weight proportion: 20 grams of tarragons, 12 grams of cordate houttuynias, 15 grams of honeysuckles, 8 grams of hypericum perforatums, 5 grams of kuh-sengs, 5 grams of the roots of large-flowered skullcap, 8 grams of wrinkled giant hyssops, 6 grams of eupatoriums, 5 grams of golden cypresses, 6 grams of the barks of official magnolia, 5 grams of ligustrum sinenses, 10 grams of selfheals.
As preferably, be prepared from by the medicinal material of following weight proportion: 20 grams of tarragons, 12 grams of cordate houttuynias, 15 grams of honeysuckles, 8 grams of hypericum perforatums, 5 grams of kuh-sengs, 5 grams of the roots of large-flowered skullcap, 8 grams of wrinkled giant hyssops, 6 grams of eupatoriums, 5 grams of golden cypresses, 6 grams of the barks of official magnolia, 5 grams of ligustrum sinenses, 8 grams of garden burnets.
As preferably, be prepared from by the medicinal material of following weight proportion: 20 grams of tarragons, 12 grams of cordate houttuynias, 15 grams of honeysuckles, 8 grams of hypericum perforatums, 5 grams of kuh-sengs, 5 grams of the roots of large-flowered skullcap, 8 grams of wrinkled giant hyssops, 6 grams of eupatoriums, 5 grams of golden cypresses, 6 grams of the barks of official magnolia, 5 grams of ligustrum sinenses, 8 grams of garden burnets, 10 grams of selfheals.
A kind of preparation method of the Chinese medicine for air sterillization, comprise the steps: to take tarragon, cordate houttuynia, honeysuckle, hypericum perforatum, kuh-seng, the root of large-flowered skullcap, wrinkled giant hyssop, eupatorium, golden cypress, the bark of official magnolia, ligustrum sinense, garden burnet, selfheal, insert in container, add 8 times of water gagings, decoct 1.5 hours, filter; Filter residue adds 6 times of water gagings, decocts 1 hour, filters; Merging filtrate, concentrated, dry, incapsulate shell.
As preferably, comprise the steps: to take tarragon, cordate houttuynia, honeysuckle, hypericum perforatum, kuh-seng, the root of large-flowered skullcap, wrinkled giant hyssop, eupatorium, golden cypress, the bark of official magnolia, ligustrum sinense, garden burnet, selfheal, insert in container, add 8 times of water gagings, decoct 1.5 hours, filter; Filter residue adds 6 times of water gagings, decocts 1 hour, filters; Merging filtrate, concentrated, dry, dry, then add appropriate dextrin and flavouring, granulate according to this area common process.
As preferably, comprise the steps: to take tarragon, cordate houttuynia, honeysuckle, hypericum perforatum, kuh-seng, the root of large-flowered skullcap, wrinkled giant hyssop, eupatorium, golden cypress, the bark of official magnolia, ligustrum sinense, garden burnet, selfheal, insert in container, add 8 times of water gagings, decoct 1.5 hours, filter; Filter residue adds 6 times of water gagings, decocts 1 hour, filters; Merging filtrate, concentrated, dry, concentrated, dry, pulverize.
The pharmacology analysis of the each Chinese medicinal ingredients of the present invention is as follows:
Tarragon [nature and flavor] is pungent, bitter, temperature; Slightly poisonous.[return through] returns liver,spleen,kidney warp.[function cures mainly] eliminating cold to stop pain, warming channel for arresting bleeding.Be used for few abdomen crymodynia, through cold uncomfortable, palace is cold infertile, spit blood, and bleeding from five sense organs or subcutaneous tissue, uterine bleeding warp is many, gestation hemorrhage.
The dry aerial parts that cordate houttuynia [source] this product is saururaceae plant houttuynia cordata.[nature and flavor] are pungent, are slightly cold.[return through] returns lung channel.[function cures mainly] is clearing heat and detoxicating, the carbuncle that disappears apocenosis, inducing diuresis for treating strangurtia.For lung carbuncle pyemesis, phlegm heat panting is coughed, hot dysentery, and heat is drenched, carbuncle sore tumefacting virus.
Honeysuckle [source] this product is the dry flower of caprifoliaceae plant honeysuckle or the flower that band is just opened.[nature and flavor] are sweet, cold.[return through] returns lung, the heart, stomach warp.[function cures mainly] is clearing heat and detoxicating, wind-heat dissipating.For the swollen furunculosis of carbuncle, larynx numbness, erysipelas, toxic-heat and blood stasis, anemopyretic cold, warm disease heating.
Hypericum perforatum [source] is herb or the whole herb with root of Garcinia maingayii hypericum perforatum.[nature and flavor] bitter; Puckery; Property is put down.[return through] Liver Channel.[function cures mainly] astringing to arrest bleeding; The logical breast of menstruation regulating; Clearing heat and detoxicating; Dampness removing.Main spitting of blood; Spit blood; Discharging fresh blood stool; Uterine bleeding; Traumatism and bleeding; Menstruation is fried and is adjusted; Breast woman agalactia; Jaundice; Have sore throat; Red eye, swell pain; Urinary tract infections; The raw sore of mouth and nose; Carbuncle furuncle poison; Burn and scald.
Kuh-seng [source] this product is the dry root of leguminous plant kuh-seng.[nature and flavor] hardship, cold.[return through] thoughts of returning home, liver, stomach, large intestine, urinary bladder channel.[function cures mainly] heat-clearing and damp-drying drug, desinsection, diuresis.For hot dysentery, have blood in stool, jaundice renal shutdown, leukorrhea with reddish discharge, swelling of vulva pruritus vulvae, eczema, wet sore, pruitus, mange leprosy; Control trichomonas vaginitis outward.
The dry root of the root of large-flowered skullcap [source] the labiate root of large-flowered skullcap.[function cures mainly] heat-clearing and damp-drying drug, purging intense heat and detonicating, hemostasis, antiabortive.For damp-warm syndrome, the heat temperature evil of vomitting uncomfortable in chest, damp and hot ruffian is full, rushes down dysentery, jaundice, and cough with lung heat, high hot polydipsia, blood-head is told nosebleed, carbuncle sore tumefacting virus, fetal irritability.
Wrinkled giant hyssop [source] is the herb of labiate Pogostemon cablin or wrinkled giant hyssop.[nature and flavor] taste is pungent; Slightly warm in nature.[return through] returns lung; Spleen; Stomach warp.[function cures mainly] dispelling summer-heat to relieve superficies syndrome; Removing dampness to restore normal functioning of the stomach.Main summertime flu; Fever and chills headache; Chest gastral cavity ruffian is vexed; Vomiting is had loose bowels; The vomiting of pregnancy; Nasosinusitis; Hand; Tinea pedis.
The dry aerial parts of eupatorium [source] feverfew eupatorium.[nature and flavor] are pungent, flat.[return through] returns spleen, stomach, lung channel.[function cures mainly] removes dampness by means of aromatics, and the appetizing of being amusing, delivers relieving summer-heat.For turbi damp obstructing in middle-JIAO, gastral cavity ruffian evils of vomitting, sweet greasy in mouth, halitosis, polysialia, summer-heat and damp table disease, alliteration is uncomfortable in chest.
Golden cypress [source] this product is the dry bark of rutaceae wampee.[nature and flavor] hardship, cold.[return through] returns kidney, urinary bladder channel.[function cures mainly] heat-clearing and damp-drying drug, purging intense heat is except steaming, detoxification sore treatment.For damp-heat dysentery, jaundice, under band, heat is drenched, beriberi, and impotence { is warded off }, hectic fever due to yin labor heat, night sweat, seminal emission, sore swollen toxin, eczema itch.
Dry dry hide, Gen Pi and the branch skin of the bark of official magnolia [source] the Magnoliacea plant bark of official magnolia or Magnolia bilola.The dissolving phlegm of [function cures mainly] eliminating dampness, lower gas is except full.For humidity hysteresis wound, gastral cavity ruffian is vomited and diarrhoea, stagnation of QI due to dyspepsia, and abdominal distention constipation, phlegm and retained fluid is breathed with cough.
Ligustrum sinense [source] Oleaceae Ligustrum plant ligustrum sinense, is used as medicine with leaf.Can adopt the whole year, dries or using fresh herb.[function cures mainly] is clearing heat and detoxicating, restraining and sterilizing bacteria, swelling and pain relieving, putrefaction-removing granulation-promoting.For acute icteric catarrhal jaundice, dysentery, cough with lung heat; Traumatic injury is controlled in external application, wound infection, burn and scald.The surgical infection diseases such as sore swollen toxin.
Garden burnet [source] this product is the dry root of rosaceous plant garden burnet.[nature and flavor] are bitter, acid, puckery, are slightly cold.[function cures mainly] cooling blood and hemostasis, removing toxic substances sore.Be used for having blood in stool, hemorrhoid blood, bloody flux, uterine bleeding, scald, carbuncle sore tumefacting virus.
Selfheal [source] this product is the dry fruit ear of labiate selfheal.[nature and flavor] are pungent, bitter, cold.[return through] returns liver, gallbladder channel.[function cures mainly] relieves inflammation or internal heat, improving eyesight, dissipating bind, detumescence.For red eye, swell pain, order pearl nyctalgia, has a headache dizzy, scrofula, and goiter and tumor, acute mastitis swells and ache; Thyroid gland enlargement, scrofula, the proliferation of mammary gland, hypertension.
Below in conjunction with clinical trial data declaration beneficial effect of the present invention:
Adopt the air sterillization of the present invention for direct rooming-in.Indoor clump count before and after sterilization is compared, result shows, after the present invention sterilizes, indoor clump count all reaches hospital hygienics standard (≤200cfu/m3), and has aromatic odor, non-stimulated to puerpera and neonate, be applicable to the sleeping air sterillization that has patients room.
Embodiment
In order to understand better and to implement the present invention, further illustrate the present invention below in conjunction with specific embodiment.
Embodiment 1
Take: 20 grams of tarragons, 12 grams of cordate houttuynias, 15 grams of honeysuckles, 8 grams of hypericum perforatums, 5 grams of kuh-sengs, 5 grams of the roots of large-flowered skullcap, 8 grams of wrinkled giant hyssops, 6 grams of eupatoriums, 5 grams of golden cypresses, 6 grams of the barks of official magnolia, 5 grams of ligustrum sinenses, 8 grams of garden burnets, 10 grams of selfheals, insert in container, add 8 times of water gagings, decoct 1.5 hours, filter; Filter residue adds 6 times of water gagings, decocts 1 hour, filters; Merge filtrate twice, concentrated.
For air sterillization.
Embodiment 2
Take: 20 grams of tarragons, 12 grams of cordate houttuynias, 15 grams of honeysuckles, 8 grams of hypericum perforatums, 5 grams of kuh-sengs, 5 grams of the roots of large-flowered skullcap, 8 grams of wrinkled giant hyssops, 6 grams of eupatoriums, 5 grams of golden cypresses, 6 grams of the barks of official magnolia, 5 grams of ligustrum sinenses, 8 grams of garden burnets, 10 grams of selfheals, insert in container, decoct 1.5 hours, filter; Filter residue adds 6 times of water gagings, decocts 1 hour, filters; Filter residue adds 2 times of water gagings, decocts 1 hour, filters; Merge three times filtrate, concentrated.
For air sterillization.
Embodiment 3
Take: 20 grams of tarragons, 12 grams of cordate houttuynias, 15 grams of honeysuckles, 8 grams of hypericum perforatums, 5 grams of kuh-sengs, 5 grams of the roots of large-flowered skullcap, 8 grams of wrinkled giant hyssops, 6 grams of eupatoriums, 5 grams of golden cypresses, 6 grams of the barks of official magnolia, 5 grams of ligustrum sinenses, 8 grams of garden burnets, 10 grams of selfheals, insert in container, add 8 times of water gagings, decoct 1.5 hours, filter; Filter residue adds 6 times of water gagings, decocts 1 hour, filters; Merge filtrate twice, concentrated.
For air sterillization.
Obviously, the above embodiment of the present invention is only for example of the present invention is clearly described, and is not the restriction to embodiments of the present invention.For those of ordinary skill in the field, can also make other changes in different forms on the basis of the above description.Here cannot give exhaustive to all embodiments.Everyly belong to apparent variation or the still row in protection scope of the present invention of variation that technical scheme of the present invention extends out.

Claims (8)

1. the Chinese medicine for air sterillization, it is characterized in that, be prepared from by the medicinal material of following weight proportion: 15~20 grams of tarragons, 10~12 grams of cordate houttuynias, 12~15 grams of honeysuckles, 6~8 grams of hypericum perforatums, 4~5 grams of kuh-sengs, 4~5 grams of the roots of large-flowered skullcap, 6~8 grams of wrinkled giant hyssops, 5~6 grams of eupatoriums, 4~5 grams of golden cypresses, 5~6 grams of the barks of official magnolia, 4~5 grams of ligustrum sinenses, 6~8 grams of garden burnets, 8~10 grams of selfheals.
2. a kind of Chinese medicine for air sterillization according to claim 1, it is characterized in that, be prepared from by the medicinal material of following weight proportion: 20 grams of tarragons, 12 grams of cordate houttuynias, 15 grams of honeysuckles, 8 grams of hypericum perforatums, 5 grams of kuh-sengs, 5 grams of the roots of large-flowered skullcap, 8 grams of wrinkled giant hyssops, 6 grams of eupatoriums, 5 grams of golden cypresses, 6 grams of the barks of official magnolia, 5 grams of ligustrum sinenses.
3. a kind of Chinese medicine for air sterillization according to claim 1, it is characterized in that, be prepared from by the medicinal material of following weight proportion: 20 grams of tarragons, 12 grams of cordate houttuynias, 15 grams of honeysuckles, 8 grams of hypericum perforatums, 5 grams of kuh-sengs, 5 grams of the roots of large-flowered skullcap, 8 grams of wrinkled giant hyssops, 6 grams of eupatoriums, 5 grams of golden cypresses, 6 grams of the barks of official magnolia, 5 grams of ligustrum sinenses, 10 grams of selfheals.
4. a kind of Chinese medicine for air sterillization according to claim 1, it is characterized in that, be prepared from by the medicinal material of following weight proportion: 20 grams of tarragons, 12 grams of cordate houttuynias, 15 grams of honeysuckles, 8 grams of hypericum perforatums, 5 grams of kuh-sengs, 5 grams of the roots of large-flowered skullcap, 8 grams of wrinkled giant hyssops, 6 grams of eupatoriums, 5 grams of golden cypresses, 6 grams of the barks of official magnolia, 5 grams of ligustrum sinenses, 8 grams of garden burnets.
5. a kind of Chinese medicine for air sterillization according to claim 1, it is characterized in that, be prepared from by the medicinal material of following weight proportion: 20 grams of tarragons, 12 grams of cordate houttuynias, 15 grams of honeysuckles, 8 grams of hypericum perforatums, 5 grams of kuh-sengs, 5 grams of the roots of large-flowered skullcap, 8 grams of wrinkled giant hyssops, 6 grams of eupatoriums, 5 grams of golden cypresses, 6 grams of the barks of official magnolia, 5 grams of ligustrum sinenses, 8 grams of garden burnets, 10 grams of selfheals.
6. the preparation method for the Chinese medicine of air sterillization, it is characterized in that, comprise the steps: to take tarragon, cordate houttuynia, honeysuckle, hypericum perforatum, kuh-seng, the root of large-flowered skullcap, wrinkled giant hyssop, eupatorium, golden cypress, the bark of official magnolia, ligustrum sinense, garden burnet, selfheal, insert in container, add 8 times of water gagings, decoct 1.5 hours, filter; Filter residue adds 6 times of water gagings, decocts 1 hour, filters; Merging filtrate, concentrated, dry, incapsulate shell.
7. the preparation method of a kind of Chinese medicine for air sterillization according to claim 6, it is characterized in that, comprise the steps: to take tarragon, cordate houttuynia, honeysuckle, hypericum perforatum, kuh-seng, the root of large-flowered skullcap, wrinkled giant hyssop, eupatorium, golden cypress, the bark of official magnolia, ligustrum sinense, garden burnet, selfheal, insert in container, add 8 times of water gagings, decoct 1.5 hours, filter; Filter residue adds 6 times of water gagings, decocts 1 hour, filters; Merging filtrate, concentrated, dry, dry, then add appropriate dextrin and flavouring, granulate according to this area common process.
8. the preparation method of a kind of Chinese medicine for air sterillization according to claim 6, it is characterized in that, comprise the steps: to take tarragon, cordate houttuynia, honeysuckle, hypericum perforatum, kuh-seng, the root of large-flowered skullcap, wrinkled giant hyssop, eupatorium, golden cypress, the bark of official magnolia, ligustrum sinense, garden burnet, selfheal, insert in container, add 8 times of water gagings, decoct 1.5 hours, filter; Filter residue adds 6 times of water gagings, decocts 1 hour, filters; Merging filtrate, concentrated, dry, concentrated, dry, pulverize.
CN201410128346.XA 2014-04-01 2014-04-01 Traditional Chinese medicine for air disinfection and preparation method thereof Pending CN103875733A (en)

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Cited By (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN105432689A (en) * 2016-01-27 2016-03-30 时启梅 Traditional Chinese medicine disinfectant and preparation method thereof
CN106106556A (en) * 2016-07-26 2016-11-16 柳州市明达鸽业养殖专业合作社 Dovecote disinfectant that stone qi Columba livia is special and preparation method thereof
CN106165704A (en) * 2016-07-26 2016-11-30 柳州市明达鸽业养殖专业合作社 Dovecote disinfectant special for U.S. Wang Ge and preparation method thereof
CN106900781A (en) * 2017-03-02 2017-06-30 湖北灵参中药科技有限公司 Antibacterial bacteriostatic liquid prepared by a kind of vegetable Chinese herbal medicine
CN106982866A (en) * 2017-04-07 2017-07-28 安徽中煦环保新材料科技有限公司 A kind of high-efficiency environment friendly air cleaning repair process material and preparation method thereof

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Publication number Priority date Publication date Assignee Title
CN1140544A (en) * 1996-06-20 1997-01-22 高福兴 Producing process for green disinfectant
CN1535754A (en) * 2003-04-04 2004-10-13 苏继挺 Antimicrobial filter and its preparation method
CN103495053A (en) * 2013-09-25 2014-01-08 合肥智上农业开发有限公司 Disinfectant with lavender fragrance
CN103583609A (en) * 2013-11-20 2014-02-19 平阴县中医医院 Air disinfectant

Patent Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN1140544A (en) * 1996-06-20 1997-01-22 高福兴 Producing process for green disinfectant
CN1535754A (en) * 2003-04-04 2004-10-13 苏继挺 Antimicrobial filter and its preparation method
CN103495053A (en) * 2013-09-25 2014-01-08 合肥智上农业开发有限公司 Disinfectant with lavender fragrance
CN103583609A (en) * 2013-11-20 2014-02-19 平阴县中医医院 Air disinfectant

Cited By (6)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN105432689A (en) * 2016-01-27 2016-03-30 时启梅 Traditional Chinese medicine disinfectant and preparation method thereof
CN106106556A (en) * 2016-07-26 2016-11-16 柳州市明达鸽业养殖专业合作社 Dovecote disinfectant that stone qi Columba livia is special and preparation method thereof
CN106165704A (en) * 2016-07-26 2016-11-30 柳州市明达鸽业养殖专业合作社 Dovecote disinfectant special for U.S. Wang Ge and preparation method thereof
CN106900781A (en) * 2017-03-02 2017-06-30 湖北灵参中药科技有限公司 Antibacterial bacteriostatic liquid prepared by a kind of vegetable Chinese herbal medicine
CN106900781B (en) * 2017-03-02 2019-06-04 湖北灵参中药科技有限公司 A kind of antibacterial bacteriostatic liquid of vegetable Chinese herbal medicine preparation
CN106982866A (en) * 2017-04-07 2017-07-28 安徽中煦环保新材料科技有限公司 A kind of high-efficiency environment friendly air cleaning repair process material and preparation method thereof

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Application publication date: 20140625