Classifications

• • A—HUMAN NECESSITIES
  • A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
  • A01G—HORTICULTURE; CULTIVATION OF VEGETABLES, FLOWERS, RICE, FRUIT, VINES, HOPS OR SEAWEED; FORESTRY; WATERING
  • A01G7/00—Botany in general
  • A01G7/06—Treatment of growing trees or plants, e.g. for preventing decay of wood, for tingeing flowers or wood, for prolonging the life of plants
• • A—HUMAN NECESSITIES
  • A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
  • A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
  • A01N43/00—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds
  • A01N43/72—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with nitrogen atoms and oxygen or sulfur atoms as ring hetero atoms
  • A01N43/80—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with nitrogen atoms and oxygen or sulfur atoms as ring hetero atoms five-membered rings with one nitrogen atom and either one oxygen atom or one sulfur atom in positions 1,2
• • A—HUMAN NECESSITIES
  • A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
  • A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
  • A01N43/00—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds
  • A01N43/72—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with nitrogen atoms and oxygen or sulfur atoms as ring hetero atoms
  • A01N43/82—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with nitrogen atoms and oxygen or sulfur atoms as ring hetero atoms five-membered rings with three ring hetero atoms

Definitions

• the present invention relates to a plant growth regulator comprising a heterocyclic compound represented by the following general formula (I) as an active ingredient and a method for using the same, and as a cultivated plant, in particular, an increase in banana yield and leaf number, a new pseudostem
• the present invention provides a drug excellent in plant growth regulation effects such as growth promotion (hypertrophy) of a part (child strain).
• the cultivated plant belonging to the genus Basho, particularly banana is a general term for varieties of edible fruits and refers to the fruits.
• the plant includes East Asia such as China and Taiwan, Southeast Asia such as Philippines, Indonesia, Thailand and Vietnam, West Asia such as India, Brazil, Ecuador, Costa Rica, Mexico, Guatemala, Colombia, Peru and other Central and South America, Kenya, Congo, It is mainly cultivated in Africa such as Kenya and South Africa. Plantation is also cultivated throughout the year. Bananas grown and harvested in these countries are exported worldwide.
• the root part including the stem part is in the basement, and the part like a stalk that extends high above the ground part is called a fake stalk.
• a long oval leaf (leaf blade) extends greatly from the tip, and a fruit axis comes out from the tip of the pseudostem, and a whole bunch including a finger and a bunch is formed, and a banana grows in the whole bunch.
• the pseudostem parent strain
• the pseudostem is cut at about 2 m above the ground.
• a new pseudostem part (child strain) newly appearing from the underground root part is propagated in the same manner, or a new pseudostem part (child strain) is bred and propagated, and banana harvesting is repeated.
• the number of leaves is important for banana cultivation, and since there are 3 months from the last leaf extraction (before flowering) to harvest, at least 12 to 13 functional leaves during the flowering period It is necessary to leave a degree. If the number of functional leaves is insufficient, the plant is cut down during cultivation.
• the present inventors have surprisingly found that a specific fungicidal active compound having a heterocyclic structure has a plant growth regulating effect, and the compound grows healthy with the compound. As a result, the inventors have found that it is possible to increase the yield, and have further advanced research to complete the present invention.
• the present invention relates to at least the following inventions: (1) General formula (I) (Wherein A represents a nitrogen atom or C-hal (where hal represents a halogen atom), B represents a nitrogen atom, R 1 represents a halogen atom; a C 1 -C 6 alkyl group or C 3) -C 6 .R 2 showing a cycloalkyl group of the hydroxyl group; C 1 -C 6 alkoxy group; a benzyloxy group; may be the same or different, a halogen atom, a cyano group, C 1 -C 6 alkyl, C 1 A benzyloxy group having one or more substituents selected from a —C 6 haloalkyl group, a C 1 -C 6 alkoxy group or a C 1 -C 6 haloalkoxy group; a phenylamino group or the same or different , halogen atom, cyano group, C 1 -C 6
• the plant growth regulator wherein the cultivated plant is rice, wheat, corn, soybean, potato or banana.
• the said plant growth regulator whose cultivated plant is a banana.
• the said usage method of the plant growth regulator whose cultivated plant is a rice, wheat, corn, soybean, potato, or a banana.
• the said usage method of the plant growth regulator whose cultivated plant is a banana.
• the said any usage method of the plant growth regulator whose heterocyclic compound represented by general formula (I) is a thiazinyl or an isotianil.
• the method for using any of the above plant growth regulators, wherein the treatment to the cultivated plant is a spraying treatment, a coating treatment, an injection treatment or a soil irrigation treatment.
• the heterocyclic compounds represented by the general formula (I) are known compounds, and the general names thiazinyl and isothianil included in the general formula (I) are known as rice blast control agents ( For example, see Patent Documents 1 and 2 and Non-Patent Document 1.) It is also known that compounds other than these two compounds can be used as various disease control agents (see, for example, Patent Documents 3 to 5). However, it is not known that these heterocyclic compounds can be used as plant growth regulators, such as increasing the yield of bananas and the number of leaves of the compound, and promoting the growth (hypertrophy) of new pseudostem parts (children). The effect is not known at all.
• the healthy growth of cultivated plants is promoted, the yield is increased, the treatment of existing pest control agents can be reduced, and the burden on the environment is reduced.
• excellent plant growth control effects such as an increase in the yield and the number of leaves (functional leaves), and further promotion of growth (hypertrophy) of the new pseudostem (child stock) are exhibited.
• plant growth regulation effects such as an increase in the yield of bananas and the number of leaves, and growth promotion (hypertrophy) of new pseudostem parts (child stocks) are particularly remarkable.
• the heterocyclic compound represented by the general formula (I), which is an active ingredient of the present invention, is a known compound, and thiazinyl and isothianyl are easily available from the market. It can be produced by the method described in (3) to (3).
• the heterocyclic compounds represented by the general formula (I) that are active ingredients of the plant growth regulator of the present invention the following are exemplified as preferred: A compound wherein A is a nitrogen atom or C—Cl; A compound in which R 1 is a halogen atom, a C 1 -C 3 alkyl group or a C 3 -C 6 cycloalkyl group; R 2 is a hydroxyl group, a C 1 -C 3 alkoxy group, a benzyloxy group having one or more substituents selected from the same or different halogen atoms on the ring, or the same or different halogen atoms , A phenylamino group having one or more substituents selected from a cyano group,
• heterocyclic compounds represented by the general formula (I) that are active ingredients of the plant growth regulator of the present invention are active ingredients of the plant growth regulator of the present invention, more preferred are those in which A is a nitrogen atom or C—Cl, and R 1 is Cl. , A C 1 -C 3 alkyl group or a C 3 -C 6 cycloalkyl group, and R 2 is a hydroxyl group, a C 1 -C 3 alkoxy group or one or more substituents which may be the same or different A benzyloxy group having Cl on the ring, or a phenylamino group having a cyano group, a C 1 -C 3 alkyl group or a C 1 -C 3 alkoxy group on the ring as one or more substituents which may be the same or different Are each exemplified.
• heterocyclic compound represented by the above general formula (I) when A is a nitrogen atom, those in which R 1 is a C 1 -C 3 alkyl group or a C 3 -C 6 cycloalkyl group are preferable, Particularly preferred are those in which R 1 is CH 3 or cC 3 H 7 .
• R 1 when A is C-hal, R 1 is preferably a halogen atom, particularly Cl. When A is C-hal, it is more particularly preferred that A is C—Cl and R 1 is Cl.
• thiazinyl and isothianyl are most preferable as the plant growth regulator of the present invention.
• thiazinyl is preferable because it is known not only to act as a plant growth regulator disclosed in the present specification but also to be effective as a disease control agent.
• Thiazinyl is, for example, various diseases in seed treatment and seed treatment, such as rice yellow dwarf disease, rice seedling blight, rice idiot disease, rice blast disease, rice blast, rice sesame leaf disease, rice browning , Rice red rice, Rice rice mildew, Rice blight bacterial disease, Rice leaf sheath browning disease, Rice brown streak disease, Rice seedling blight disease, Rice white leaf blight, Wheat snow rot (Brown), Wheat snow rot Disease (red), wheat snow rot (large fungus nuclei), snow rot (black small particles), snow rot (brown small particles), wheat red mold, ergot disease, wheat blight, wheat strain rot, sharp eyespot, wheat powdery mildew, wheat blight, wheat red rust, wheat black rust, wheat yellow rust, wheat eye spot, wheat leaf blight, wheat yellow, wheat streak, wheat naked scab, Wheat scab, wheat to smut, potato powdery scab, potato scab, potato / toma Plague,
• Thiazinyl is also a pear-like fruit fire such as cucumber spotted bacterial disease, rice brown streak disease, rice seedling bacterial disease, tea red burning disease, citrus ulcer disease, cabbage black rot, peach perforated bacterial disease, apple and pear Wound disease, soft rot, kidney wilt bacterial disease, root carcinoma disease, citrus stabon disease, tomato ulcer disease, citrus greening disease, rice wilt bacterial disease, rice leaf sheath browning disease, solanaceae blight, rice white leaf It has also been found to be effective against bacterial diseases such as blight, grape / apple blacklot disease, soft rot, and grape head carcinoma.
• thiazinyl has white crotch, ume powdery mildew, peach / ume black streak, oyster circle leaf fall, oyster anthracnose disease, oyster leaf blight, oyster horn leaf fall, oyster black leaf disease, loquat anthracnose, It is also known to be effective for mango anthracnose, banana sigatoka disease, banana panama disease, root cancer and the like.
• the plant growth regulating effect or the plant growth regulating action means an increase in the number of leaves of plants (crop), plant height elongation, stem enlargement, root generation and / or activation of growth (promoting rooting, amount of elongation).
• Increase in planting or early rooting increase in plant vitality, decrease in leaf dryness, increase in plant salt tolerance, drought resistance and low temperature resistance, fruit coloration, cereals, fruits and potatoes And the like, and the increase in sugar content of fruits and potatoes, etc., which in turn leads to improved crop quality and / or increased yield.
• the plant growth regulation effect or plant growth regulation effect in banana leads to an increase in the yield of banana fruit by increasing the number of leaves (functional leaves) or promoting the growth (hypertrophy) of the new false stem (child stock). It is.
• the preparation can be used as it is.
• the heterocyclic compound (active ingredient compound) represented by the general formula (I) is mixed and dissolved in an appropriate inert carrier together with a surfactant and, if necessary, an auxiliary agent in an appropriate ratio.
• turbidity agent flowable agent
• a milk suspension agent an emulsion
• a liquid agent a wettable powder, a granular wettable powder, a granule, a powder agent, a tablet, a jumbo agent, or a pack agent.
• the inert carrier that can be used in the present invention may be either solid or liquid.
• materials that can be used as a solid inert carrier include vegetable powders (for example, soybean flour, cereal flour, and wood flour). , Bark powder, sawdust, tobacco stem powder, walnut shell powder, bran, fiber powder, residues after extraction of plant extracts), synthetic polymers such as ground synthetic resin, clays (eg kaolin, bentonite, acid clay) Etc.), talc (for example, talc, pyrophyllite, etc.), silica (for example, diatomaceous earth, silica sand, mica, white carbon (hydrous finely divided silicon, hydrous silicic acid, synthetic highly dispersed silicic acid, with calcium silicate as the main component depending on the product) Some).
• Activated carbon natural minerals (eg, sulfur powder, pumice, attapulgite, zeolite, etc.), calcined diatomaceous earth, brick ground, fly Sand, plastic carrier, etc.
• inorganic mineral powders such as calcium carbonate and calcium phosphate
• chemical fertilizers such as ammonium sulfate, phosphate, nitrate, urea, and ammonium chloride, compost, etc.
• Materials that can be used as a liquid inert carrier in the present invention include those having solvent ability, and those capable of dispersing an active ingredient compound with the aid of an auxiliary agent without having solvent ability.
• the following carriers may be selected as typical examples, and these may be used alone or in the form of a mixture of two or more: for example, water, alcohols (eg, methanol, ethanol, isopropyl alcohol, butanol) , Ethylene glycol, etc.), ketones (eg, acetone, methyl ethyl ketone, methyl isobutyl ketone, diisobutyl ketone, cyclohexanone, etc.), ethers (eg, ethyl ether, dioxane, cellosolve, dipropyl ether, tetrahydrofuran, etc.), aliphatic hydrocarbons (Eg kerosene, mineral oil, etc.) Aromatic hydrocarbons (eg, benzene,
• adjuvants can be used according to the purpose, and may be used alone or in combination of two or more. In the present invention, it is possible to use no adjuvant.
• Surfactants can be used for the purpose of emulsifying, dispersing, solubilizing and / or wetting the active ingredient compound, for example, polyoxyethylene alkyl ether, polyoxyethylene alkyl aryl ether, polyoxyethylene higher fatty acid ester, polyoxyethylene Illustrative surfactants such as ethylene resin acid ester, polyoxyethylene sorbitan monolaurate, polyoxyethylene sorbitan monooleate, alkylaryl sulfonate, naphthalene sulfonic acid condensate, lignin sulfonate or higher alcohol sulfate be able to.
• adjuvants As other adjuvants, the following typical adjuvants can be mentioned, and these adjuvants are used depending on the purpose, and may be used alone or in combination with two or more kinds of adjuvants. Although it is good, it is possible not to use any adjuvant in the present invention.
• Surfactants can be used for the purpose of emulsifying, dispersing, solubilizing and / or wetting of the active ingredient compound, such as polyoxyethylene alkyl ether, polyoxyethylene alkyl aryl ether, polyoxyethylene higher fatty acid ester, polyoxyethylene.
• Examples include surfactants such as resin acid esters, polyoxyethylene sorbitan monolaurate, polyoxyethylene sorbitan monooleate, alkylaryl sulfonates, naphthalene sulfonic acid condensates, lignin sulfonates, and higher alcohol sulfates. it can.
• auxiliary agents such as naphthalenesulfonic acid condensate and condensed phosphate can be used.
• an auxiliary agent such as silicone oil can be used.
• the blending ratio of the active ingredient compound in 100 parts by mass of the plant growth regulator of the present invention can be adjusted as necessary and is not particularly limited, but it may be appropriately selected from the range of usually 0.1 to 50 parts by mass. Preferably, it may be appropriately selected from the range of 1 to 50 parts by mass.
• the cultivated plant in which the plant growth regulator of the present invention can be used is not particularly limited.
• cereals for example, rice, barley, wheat, rye, oats, corn, potato, etc.
• beans for example, Soybeans, red beans, broad beans, peas, peanuts, etc.
• fruit trees and fruits eg, apples, citrus fruits, pears, grapes, peaches, plums, cherry peaches, walnuts, almonds, bananas, strawberries, etc.
• vegetables eg, Cabbage, tomato, spinach, broccoli, lettuce, onion, leek, bell pepper, etc.
• root vegetables eg, carrot, potato, sweet potato, radish, lotus root, turnip, etc.
• processing crops eg, cotton, hemp, mulberry, Mitsumata, rapeseed, beet, hop, sugar cane, sugar beet, olive, gum, coffee, tobacco, tea, etc.
• moss eg, pumpkin, Cucumbers, watermelons
• Rice, wheat, corn, soybeans or potatoes are important for food production, and fruit trees and fruits are important from the viewpoint of economic value in certain regions. East Asia, Southeast Asia, West Asia, Latin America, Africa Bananas are also important in and the use of the present invention in these cultivated plants is preferred.
• Glycaceae plants include Gros Michel, Cavendish, Dwarf Cavendish, and Dwarf Chinese. Enano, Catura, Giant Cavendish, Gran Enano, Grande Nine, Williams Hybrid, Valerie Vals Poyo, Lacatan, Monte Ku Strike (Monte cristo), can be exemplified boat Rondo (Bout rond), etc., but is not limited thereto.
• bananas including Giant Cavendish, Dwarf Cavendish, Cavendish, Plantain, Red Banana, Apple Banana, Monkey Banana, Island Banana, etc. that are generally cultivated for food.
• herbicide resistance genes insecticidal pest resistance genes, anti-pathogenic substance production genes, oil component modification and amino acid content enhancement traits are useful for cultivated plants in which the plant growth regulator of the present invention can be used.
• the same plant that is a genetically modified organism (GMO) that has undergone gene conversion is also included.
• the method of use or the method of regulating the growth of cultivated plants can be expressed as it is, or appropriately diluted with water, etc.
• a desired plant growth regulating action can be expressed.
• an excellent plant growth regulating action can be expressed by spraying or coating the stems and leaves and leaf sheaths, injecting them with a syringe or the like, and irrigating the surrounding soil.
• the number of bananas cultivated per hectare (ha) is about 1500 to 2000, and the processing amount is the blending ratio of active ingredients, meteorological conditions, formulation form, treatment time, treatment method However, it varies depending on the processing place and the like and is not particularly limited.
• Suspension is a frequently used dosage form. In the case of this agent, 1 to 10 L (chemical solution) per hectare is applied to the target plant or the surrounding soil where the target plant is growing in the spraying or irrigation treatment.
• the amount of the active ingredient is preferably in the range of 300 g to 3000 g / ha).
• the medicinal solution diluted to a predetermined concentration is appropriately selected from the range of 0.2 ml to 10 ml per plant (depending on the concentration of the medicinal solution, specific gravity, etc., but the amount of active ingredient is preferably in the range of 40 mg to 800 mg).
• the amount of drug used can be reduced, and unlike the case of spraying, the user is not exposed to the chemical solution (in the case of general spraying), and uses the plant growth regulator of the present invention more safely. It is something that can be done.
• agricultural or horticultural fungicides or agricultural and horticultural use Insecticides can be used simultaneously.
• the typical compound of this agricultural and horticultural fungicide or agricultural and horticultural insecticide is illustrated below, the said agricultural and horticultural fungicide or agricultural and horticultural insecticide is not limited to these.
• Agricultural and horticultural fungicides include, for example, isoprothiolane, tricyclazole, azoxystrobin, pyracrostrobin, propiconazole, copper-ol-8, and organic copper-ol.
• Methinostrobin carpropamide, fthalide, kasugamycin, pyroquilon, probenazole, cibenzol-S-methyl-S-methyl-S-methyl-S-methyl lutolanil, mepronil, furamethpyr, pencyclone, thifluzamide, validamycin, diclomezine, dimimzine.
• Hexaconazole, difenoconazole, bittertanol
• Examples of agricultural and horticultural insecticides include benfuracarb, carbosulfan, PHC (propoxur), furatiocarb, mesomyl, NAC (carbaryl), bendiocarb (bendiocarb) analycarb), imidacloprid, nitenpyram, acetamiprid, thiamethoxam, dithiophthinothin, dithotefurone (Diazinon), trichlorfon (trichlorfon), fenthion (fenthion), acephate (acephate),
• Cyromazine (cyromazine), Rufenyuron (lufenuron), tebufenozide (tebufenozide), methoxyfenozide (methoxyfenozide), chromafenozide (chromafenozide), oxamyl (oxamyl), pyraclofos (pyraclofos), fosthiazate (fosthiazate), fenpyroximate (fenpyroximate), fipronil (fipronil), Endosulfan, endaldehyde, metadealdehyde, emamectin benzoate, spinosad, chlorfenapyr, indoxacarb (indo) Mixed with Oxacarb) or the like can be used.
• Test Example 1 Increase test of number of functional leaves in banana (injection process)
• a drug solution prepared by diluting the drug (active ingredient: Compound No. 1) of the pharmaceutical formulation of Formulation Example 5 with water 5 times in an amount of 10 ml per strain (600 mg as the active ingredient amount) in the pseudostem part of the banana child stock or the parent strain was injected into a place about 1 m above the ground using a 10 ml syringe. From the 11th day after the drug treatment, the total number of functional leaves per plant (healthy leaves functioning) was calculated, and thereafter, every week, the same calculation was made for 7 weeks (1 ward, 4 systems). In addition, the number of functional leaves in the parent pseudostem-treated section indicates the number of functional leaves of child pseudostem that comes from the same root. The results are shown in Table 2.
• Test Example 2 Plant growth control effect on parent strain by parent strain treatment (injection treatment) A drug solution prepared by diluting the drug (active ingredient: Compound No. 1) of the pharmaceutical formulation of Formulation Example 5 with water to 10 times the amount of 10 ml (600 mg as the active ingredient amount) per strain in the pseudostem part of the parent strain It inject
• chlorothalonil 72% flowable at a dose of 1 L / ha and 100 L / ha sprayed water about every week from 10 days to 125 days after treatment in all test plots
• the foliage spraying process is performed at The results are shown in Table 3.
• Test Example 3 Plant growth control effect by spraying or irrigation treatment
• the drug (active ingredient: Compound No. 1) of the formulation of Formulation Example 5 is sprayed on the foliage part or in the stock soil in an amount of 3 L per 1 ha (effective ingredient quantity: 900 g) Irrigated.
• After treatment with chemicals we measured and calculated functional leaves per plant (healthy leaves), plant height, pseudostem diameter, plant height of offspring, and banana yield (specifically 80 stations) System).
• chlorotalonyl 72% flowable agent at a dose of 1 L / ha and a sprayed water amount of 100 L / ha every week from 7 days to 122 days after treatment in all test plots.
• the foliage spraying process is performed at The results are shown in Table 4.
• Test Example 4 Effect of plant growth control on parent plants by treatment with various drugs (injection treatment)
• a preparation prepared according to Formulation Example 5 or Formulation Example 5 active ingredient: Compound No. 1, Compound No. 7, and Compound No. 12
• the amount of 10 ml per strain is injected into a portion about 1 m above the ground using a syringe, and the plant height and pseudostem diameter of the offspring are measured about every 2 weeks from the 17th day after the drug treatment.
• the average value was calculated (1 ward 20 continuous system).
• chlorothalonil 72% flowable agent at a dose of 1 L / ha and a sprayed water amount of 100 L / ha every week after 7 days of treatment in all test plots The spraying process is performed.
• the treatment group for the compounds represented by the general formula (I) of the present invention (Compound No. 1, Compound No. 7 and Compound No. 12) is the pseudostem of the parent strain.
• the plant height and the pseudostem diameter of the banana seedlings were significantly increased by injecting into the part. That is, it was further clarified that the plant growth regulator of the present invention has an excellent plant growth promoting effect.
• the healthy growth of cultivated plants is promoted, the yield is increased, the treatment of existing pest control agents can be reduced, and the burden on the environment is reduced. This is especially true for bananas. Therefore, the present invention greatly contributes to the development of agriculture and related industries.

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• Life Sciences & Earth Sciences (AREA)
• Environmental Sciences (AREA)
• Wood Science & Technology (AREA)
• Engineering & Computer Science (AREA)
• Health & Medical Sciences (AREA)
• Biodiversity & Conservation Biology (AREA)
• Dentistry (AREA)
• General Health & Medical Sciences (AREA)
• Pest Control & Pesticides (AREA)
• Zoology (AREA)
• Agronomy & Crop Science (AREA)
• Plant Pathology (AREA)
• Ecology (AREA)
• Forests & Forestry (AREA)
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• Agricultural Chemicals And Associated Chemicals (AREA)
• Plural Heterocyclic Compounds (AREA)
• Cultivation Of Plants (AREA)
• Nitrogen And Oxygen Or Sulfur-Condensed Heterocyclic Ring Systems (AREA)

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• 2011
  • 2011-01-12 JP JP2011003603A patent/JP2014088322A/ja not_active Withdrawn
• 2012
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