USH596H - Method of etching titanium diboride - Google Patents

Method of etching titanium diboride Download PDF

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Publication number
USH596H
USH596H US07/156,124 US15612488A USH596H US H596 H USH596 H US H596H US 15612488 A US15612488 A US 15612488A US H596 H USH596 H US H596H
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US
United States
Prior art keywords
mixture
gas
dry etchant
fluoride
chloride
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Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Abandoned
Application number
US07/156,124
Inventor
Linda S. Heath
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
United States Department of the Army
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United States Department of the Army
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Publication date
Application filed by United States Department of the Army filed Critical United States Department of the Army
Priority to US07/156,124 priority Critical patent/USH596H/en
Application granted granted Critical
Publication of USH596H publication Critical patent/USH596H/en
Assigned to UNITED STATES OF AMERICA, THE, AS REPRESENTED BY THE SECRETARY OF THE ARMY reassignment UNITED STATES OF AMERICA, THE, AS REPRESENTED BY THE SECRETARY OF THE ARMY ASSIGNMENT OF ASSIGNORS INTEREST. Assignors: HEATH, LINDA S.
Abandoned legal-status Critical Current

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    • CCHEMISTRY; METALLURGY
    • C04CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
    • C04BLIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
    • C04B41/00After-treatment of mortars, concrete, artificial stone or ceramics; Treatment of natural stone
    • C04B41/009After-treatment of mortars, concrete, artificial stone or ceramics; Treatment of natural stone characterised by the material treated
    • CCHEMISTRY; METALLURGY
    • C04CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
    • C04BLIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
    • C04B41/00After-treatment of mortars, concrete, artificial stone or ceramics; Treatment of natural stone
    • C04B41/80After-treatment of mortars, concrete, artificial stone or ceramics; Treatment of natural stone of only ceramics
    • C04B41/91After-treatment of mortars, concrete, artificial stone or ceramics; Treatment of natural stone of only ceramics involving the removal of part of the materials of the treated articles, e.g. etching

Definitions

  • This invention relates in general to a method of etching titanium diboride and in particular to a method of dry etching a thin film of titanium diboride that has been deposited onto a substrate and patterned using photolithography.
  • Titanium diboride has become of interest in laboratory research because of its resistance to change or degradation at high temperatures. It also shows promise in acting as a diffusion barrier to other metals.
  • the general object of this invention is to provide a method of etching titanium diboride.
  • a more particular object of this invention is to provide a method of etching a thin film of titanium diboride that has been deposited onto a substrate and patterned using photolithography.
  • a thin film of titanium diboride that has been deposited onto a substrate and patterned using photolithography is dry etched by first mounting the substrate bearing the patterned thin film on the lower electrode of pair of electrodes in the etch chamber of a commercial plasma etcher or plasma therm etcher.
  • the etch chamber is evacuated to a pressure of about 10 -6 Torr and a dry etchant as, for example, dichlorodifluoromethane (CCl 2 F 2 ) admitted at a flow rate of about 1 to 100 sccm and a pressure set at about 1 to 500 mTorr.
  • a dry etchant as, for example, dichlorodifluoromethane (CCl 2 F 2 ) admitted at a flow rate of about 1 to 100 sccm and a pressure set at about 1 to 500 mTorr.
  • An electric field is applied between the electrodes, the power level set at about 50 to 1000 watts and etching allowed to proceed for the desired time.
  • the sample is removed and the etch rate determined by measuring the etch depth and dividing by the etch time.
  • a thin film of TiB 2 is first deposited on a gallium arsenide substrate by e-beam evaporation and the substrate with thin film of TiB 2 then patterned using photolithography.
  • the substrate bearing the patterned film is then mounted on the lower electrode of a pair of electrodes in the etch chamber of a commercial plasma etcher.
  • the etch chamber with the electrodes inside is then evacuated to a pressure of about 10 -6 Torr.
  • CCl 2 F 2 is then admitted into the etch chamber at a flow rate of about 2 to 40 sccm and the pressure set at 10 to 200 mTorr.
  • An electric field is applied between the electrodes and the power level set at 150 to 400 watts.
  • the etch is allowed to proceed until the TiB 2 is completely removed in the areas exposed by the photolithography.
  • etch TiB 2 Other dry etch processes that can be used to etch TiB 2 include reactive ion beam etching (RIBE), chemically assisted ion beam etching (CAIBE), reactive ion etching (RIE), and magetron ion etching (MIE).
  • RIBE reactive ion beam etching
  • CAIBE chemically assisted ion beam etching
  • RIE reactive ion etching
  • MIE magetron ion etching

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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Ceramic Engineering (AREA)
  • Materials Engineering (AREA)
  • Structural Engineering (AREA)
  • Organic Chemistry (AREA)
  • Drying Of Semiconductors (AREA)

Abstract

A thin film of titanium diboride that has been deposited onto a substrate d patterned using photolithography is dry etched in a commercial plasma etcher with either a chloride, or a mixture of a chloride gas with oxygen, or a mixture of a chloride gas with nitrogen, or a mixture of a chloride gas with a noble gas, or a fluoride gas, or a mixture of a fluoride gas with oxygen, or a mixture of a fluoride gas with nitrogen, or a mixture of a fluoride gas with a noble gas.

Description

The invention described herein may be manufactured, used, and licensed by or for the Government for governmental purposes without the payment to me of any royalty thereon.
This invention relates in general to a method of etching titanium diboride and in particular to a method of dry etching a thin film of titanium diboride that has been deposited onto a substrate and patterned using photolithography.
BACKGROUND OF THE INVENTION
Titanium diboride has become of interest in laboratory research because of its resistance to change or degradation at high temperatures. It also shows promise in acting as a diffusion barrier to other metals.
One of the difficulties involved with working with titanium diboride is that because of its resistance to attack, it is difficult to pattern. In fact, no wet etches have been available to carry out such patterning.
SUMMARY OF THE INVENTION
The general object of this invention is to provide a method of etching titanium diboride. A more particular object of this invention is to provide a method of etching a thin film of titanium diboride that has been deposited onto a substrate and patterned using photolithography.
It has now been found that the aforementioned objects can be attained by etching titanium diboride with a dry etch.
More particularly, according to the invention, a thin film of titanium diboride that has been deposited onto a substrate and patterned using photolithography is dry etched by first mounting the substrate bearing the patterned thin film on the lower electrode of pair of electrodes in the etch chamber of a commercial plasma etcher or plasma therm etcher. The etch chamber is evacuated to a pressure of about 10-6 Torr and a dry etchant as, for example, dichlorodifluoromethane (CCl2 F2) admitted at a flow rate of about 1 to 100 sccm and a pressure set at about 1 to 500 mTorr. An electric field is applied between the electrodes, the power level set at about 50 to 1000 watts and etching allowed to proceed for the desired time.
Other dry etchants that will etch TiB2 include a chloride gas, a mixture of a chloride gas with oxygen, a mixture of a chloride gas with nitrogen, a mixture of a chloride gas with a noble gas, a fluoride gas, a mixture of a fluoride gas with nitrogen, a mixture of a fluoride gas with oxygen, and a mixture of a fluoride gas with a noble gas.
After the dry etch, the sample is removed and the etch rate determined by measuring the etch depth and dividing by the etch time.
By adjusting the process parameters, one is able to attain etch rates of 5 to 800 Å/min for TiB2. This is useful for patterning TiB2 as a diffusion barrier or a Schottky contact to semiconductors.
DESCRIPTION OF THE PREFERRED EMBODIMENT
A thin film of TiB2 is first deposited on a gallium arsenide substrate by e-beam evaporation and the substrate with thin film of TiB2 then patterned using photolithography.
The substrate bearing the patterned film is then mounted on the lower electrode of a pair of electrodes in the etch chamber of a commercial plasma etcher. The etch chamber with the electrodes inside is then evacuated to a pressure of about 10-6 Torr. CCl2 F2 is then admitted into the etch chamber at a flow rate of about 2 to 40 sccm and the pressure set at 10 to 200 mTorr. An electric field is applied between the electrodes and the power level set at 150 to 400 watts. The etch is allowed to proceed until the TiB2 is completely removed in the areas exposed by the photolithography.
Other dry etch processes that can be used to etch TiB2 include reactive ion beam etching (RIBE), chemically assisted ion beam etching (CAIBE), reactive ion etching (RIE), and magetron ion etching (MIE).
I wish it to be understood that I do not desire to be limited to the exact details as described for obvious modifications will occur to a person skilled in the art.

Claims (11)

What is claimed is:
1. Method of etching a thin film of titanium diboride that has been deposited onto a substrate and patterned using photolithography, said method including the steps of:
(A) mounting a substrate bearing a patterned thin film of titanium diboride on a lower electrode of a pair of electrodes in an etch chamber of a plasma therm etcher,
(B) evacuating the etch chamber to a pressure of about 10-6 Torr,
(C) admitting a dry etchant to the etch chamber at a flow rate of about 1 to 100 sccm and a pressure set at about 1 to 500 mTorr,
(D) applying an electric field between the pair or electrodes and setting the power level at about 50 to 1000 watts, and
(E) allowing the etch to proceed for a preselected time.
2. Method according to claim 1 wherein the dry etchant is selected from the group consisting of a chloride gas, a mixture of a chloride gas with oxygen, a mixture of chloride gas with nitrogen, a mixture of a chloride gas with noble gas, a fluoride gas, a mixture of a fluoride gas with oxygen, a mixture of a fluoride gas with nitrogen, and a mixture of a fluoride gas with a noble gas.
3. Method according to claim 2 wherein the dry etchant is a chloride gas.
4. Method according to claim 3 wherein the dry etchant is dichlorodifluoromethane.
5. Method according to claim 2 wherein the dry etchant is a mixture of chloride gas with oxygen.
6. Method according to claim 2 wherein the dry etchant is a mixture of chloride gas with nitrogen.
7. Method according to claim 2 wherein the dry etchant is a mixture of a chloride gas with a noble gas.
8. Method according to claim 2 wherein the dry etchant is a fluoride gas.
9. Method according to claim 2 wherein the dry etchant is a mixture of a fluoride gas with oxygen.
10. Method according to claim 2 wherein the dry etchant is a mixture of a fluoride gas with nitrogen.
11. Method according to claim 2 wherein the dry etchant is a mixture of a fluoride gas with a noble gas.
US07/156,124 1988-02-16 1988-02-16 Method of etching titanium diboride Abandoned USH596H (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
US07/156,124 USH596H (en) 1988-02-16 1988-02-16 Method of etching titanium diboride

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US07/156,124 USH596H (en) 1988-02-16 1988-02-16 Method of etching titanium diboride

Publications (1)

Publication Number Publication Date
USH596H true USH596H (en) 1989-03-07

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Citations (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4203800A (en) 1977-12-30 1980-05-20 International Business Machines Corporation Reactive ion etching process for metals
US4229247A (en) 1978-12-26 1980-10-21 International Business Machines Corporation Glow discharge etching process for chromium
US4440841A (en) 1981-02-28 1984-04-03 Dai Nippon Insatsu Kabushiki Kaisha Photomask and photomask blank
US4473436A (en) 1982-05-05 1984-09-25 Siemens Aktiengesellschaft Method of producing structures from double layers of metal silicide and polysilicon on integrated circuit substrates by RIE utilizing SF6 and Cl2
US4635343A (en) 1983-03-14 1987-01-13 Fujitsu Limited Method of manufacturing GaAs semiconductor device
US4647339A (en) 1984-05-23 1987-03-03 British Telecommunications Production of semiconductor devices
US4668335A (en) 1985-08-30 1987-05-26 Advanced Micro Devices, Inc. Anti-corrosion treatment for patterning of metallic layers
US4680086A (en) 1986-03-20 1987-07-14 Motorola, Inc. Dry etching of multi-layer structures
US4734157A (en) 1985-08-27 1988-03-29 International Business Machines Corporation Selective and anisotropic dry etching

Patent Citations (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4203800A (en) 1977-12-30 1980-05-20 International Business Machines Corporation Reactive ion etching process for metals
US4229247A (en) 1978-12-26 1980-10-21 International Business Machines Corporation Glow discharge etching process for chromium
US4440841A (en) 1981-02-28 1984-04-03 Dai Nippon Insatsu Kabushiki Kaisha Photomask and photomask blank
US4473436A (en) 1982-05-05 1984-09-25 Siemens Aktiengesellschaft Method of producing structures from double layers of metal silicide and polysilicon on integrated circuit substrates by RIE utilizing SF6 and Cl2
US4635343A (en) 1983-03-14 1987-01-13 Fujitsu Limited Method of manufacturing GaAs semiconductor device
US4647339A (en) 1984-05-23 1987-03-03 British Telecommunications Production of semiconductor devices
US4734157A (en) 1985-08-27 1988-03-29 International Business Machines Corporation Selective and anisotropic dry etching
US4668335A (en) 1985-08-30 1987-05-26 Advanced Micro Devices, Inc. Anti-corrosion treatment for patterning of metallic layers
US4680086A (en) 1986-03-20 1987-07-14 Motorola, Inc. Dry etching of multi-layer structures

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Owner name: UNITED STATES OF AMERICA, THE, AS REPRESENTED BY T

Free format text: ASSIGNMENT OF ASSIGNORS INTEREST.;ASSIGNOR:HEATH, LINDA S.;REEL/FRAME:005044/0906

Effective date: 19880209