US3738085A - Device for the removal of detrimental matter from exhaust gases of internal combustion engines - Google Patents
Device for the removal of detrimental matter from exhaust gases of internal combustion engines Download PDFInfo
- Publication number
- US3738085A US3738085A US00182355A US3738085DA US3738085A US 3738085 A US3738085 A US 3738085A US 00182355 A US00182355 A US 00182355A US 3738085D A US3738085D A US 3738085DA US 3738085 A US3738085 A US 3738085A
- Authority
- US
- United States
- Prior art keywords
- drum
- exhaust gases
- muffler
- detrimental
- mixing liquid
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Expired - Lifetime
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Classifications
-
- F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
- F01—MACHINES OR ENGINES IN GENERAL; ENGINE PLANTS IN GENERAL; STEAM ENGINES
- F01N—GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR MACHINES OR ENGINES IN GENERAL; GAS-FLOW SILENCERS OR EXHAUST APPARATUS FOR INTERNAL COMBUSTION ENGINES
- F01N3/00—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust
- F01N3/02—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for cooling, or for removing solid constituents of, exhaust
- F01N3/04—Exhaust or silencing apparatus having means for purifying, rendering innocuous, or otherwise treating exhaust for cooling, or for removing solid constituents of, exhaust using liquids
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
- B01D53/34—Chemical or biological purification of waste gases
- B01D53/74—General processes for purification of waste gases; Apparatus or devices specially adapted therefor
- B01D53/86—Catalytic processes
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
- B01D53/34—Chemical or biological purification of waste gases
- B01D53/92—Chemical or biological purification of waste gases of engine exhaust gases
- B01D53/922—Mixtures of carbon monoxide or hydrocarbons and nitrogen oxides
- B01D53/925—Simultaneous elimination of carbon monoxide or hydrocarbons and nitrogen oxides
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
- Y02T—CLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO TRANSPORTATION
- Y02T10/00—Road transport of goods or passengers
- Y02T10/10—Internal combustion engine [ICE] based vehicles
- Y02T10/12—Improving ICE efficiencies
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
- Y10S—TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10S55/00—Gas separation
- Y10S55/30—Exhaust treatment
Definitions
- ABSTRACT Apparatus for the removal of detrimental matter from the exhaust gases of internal combustion engines in which a cylindrical drum having a substantially tangential inlet and an aligned substantially tangential outlet is disposed in the engine exhaust pipe for imparting a whirling motion to the exhaust gases in the drum. Th'e drum has an orifice therein at the side opposite from the inlet and outlet.
- a mixing liquid is introduced into the orifice adapted to be dispersed and evaporated by the exhaust'gases entering the drum from the engine manifold'to thereby cool the drum and the exhaust gases and at the same time to form compounds between the vapor and the detrimental matters prior to passing to the muffler.
- a dehydrating device receiving the discharge of the muffler is provided for discharging substantially pure air from thedehydracting device into the atmosphere.
- the principal object of the invention is to provide in such means a mixing device which is inserted in the exhaust pipe leading from the exhaust manifold of an internal combustion engine to the usual muffler, themixing device comprising a cylindrical drum having a substantially tangential inlet and an aligned substantially tangential outlet whereby the exhaust gases in passing through said exhaust pipe towards the muffler are given a whirling motion.
- a mixing liquid from a supply tank holding a quantity of water, phosphoris acid, peroxide of barium and peroxide of hydrogen.
- the mixing liquid dropped into the drum disperses and evaporates by means of the heat of the gases exhausted from the engine. As this evaporated liquid cools down the inner part of the drum the exhaust gas which comes into the drum from the exhaust manifold is also cooled down and its volume decreases, and a low pressure condition occurs in the inner part of the drum.
- the internal combustion engine l is provided with the usual exhaustmanifold 2.
- An exhaust pipe 3 connects the rear end of the intake manifold 2 with the inlet of a muffler 4.
- a dehydrating device 5 is connected by pipe 6 from the rear end of the muffler 4 to the inlet of the dehydrating device 5, which device exhausts through pipe 7 to the atmosphere.
- a mixing device shown more particularly in FIG. 2, the same consisting of a cylindrical drum 8 having a substantially tangential inlet 9 and an aligned substantially tangential outlet 10 whereby the exhaust gases entering the mixing drum 8 will give a whirling motion within the drum 8.
- the compound of the vapor and carbon monoxide, sulphurous acid gas, lead, hydrogenchloride, nitrogenoxide, carbon, dust, etc., which is discharged out of the outlet 10 is dehydrated and separated by means of passing from muffler 4 through the dehydrating device 5 in which calcium carbonate etc. is contained, and which device 5 is connected with the rear end of the muffler 4, and the pure air remaining in the dehydrating device 6 is discharged into the open air or atmosphere.
- Each of the devices i.e., the mixing device 8 of the exhaust pipe 3 which is characterized by its capacity of forming the compound of the detrimental matters in the exhaust-gas and the vapor into which the mixing liquid is transformed by the heat from the exhaust-gas which enters the drum 8, and the dehydrating device 5 of the detachable container which contains the dehydrator in which the chief ingredient is calcium, together form novel means for removal of detrimental matter contained in the exhaust gas of internal combustion engines.
- Apparatus for the removal of detrimental matter from the exhaust gases of internal combustion engines having an exhaust manifold, and an exhaust pipe extending from said manifold, comprising a cylindrical drum having a substantially tangential inlet and outlet disposed in the exhaust pipe for imparting a whirling motion to said exhaust gases in said drum; said drum having an orifice therein; means for introducing a mixing liquid into said orifice which will be dispersed and evaporated by the exhaust gases entering from said manifold to thereby cool the drum and the exhaust gases and at the same time to form compounds between 1 3.
- said detrimental matters comprising carbon monoxide, sulphurous acid gas, lead, hydrogenchloride, nitrogenoxide, carbon, and dust which are melted into the evaporated mixing liquid and form compounds with said vapor.
- Apparatus for the removal of detrimental matter from the exhaust gases of internal combustion engines having an exhaust manifold, a muffler, and an exhaust pipe connecting said manifold and muffler, comprising a cylindrical drum having a substantially tangential inlet and an aligned substantially tangential outlet disposed in the exhaust pipe for imparting a whirling motion to said exhaust gases in said drum; said drum having an orifice therein at the side opposite from said inlet and outlet; means for introducing a mixing liquid into said orifice which will be dispersed and evaporated by the exhaust gases entering from said manifold to thereby cool the drum and the exhaust gases and at the same time to form compounds between said vapor and said detrimental matters prior to passing to the muffler; and a dehydrating device receiving the discharge of the muffler for discharging substantially pure air from the dehydrating device into the atmosphere.
- said mixing liquid comprising water, phosphoric acid, peroxide of barium and peroxide of hydrogen.
- said detrimental matters comprising carbon monoxide, sulphurous acid gas, lead, hydrogenchloride, nitrogenoxide, carbon, and dust which are melted into the evaporated mixing liquid and form compounds with said vapor.
- said dehydrating chamber containing calcium carbonate.
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- Engineering & Computer Science (AREA)
- Chemical & Material Sciences (AREA)
- Environmental & Geological Engineering (AREA)
- Analytical Chemistry (AREA)
- Biomedical Technology (AREA)
- Health & Medical Sciences (AREA)
- Combustion & Propulsion (AREA)
- General Chemical & Material Sciences (AREA)
- Oil, Petroleum & Natural Gas (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Mechanical Engineering (AREA)
- General Engineering & Computer Science (AREA)
- Treating Waste Gases (AREA)
- Exhaust Gas After Treatment (AREA)
Abstract
Apparatus for the removal of detrimental matter from the exhaust gases of internal combustion engines in which a cylindrical drum having a substantially tangential inlet and an aligned substantially tangential outlet is disposed in the engine exhaust pipe for imparting a whirling motion to the exhaust gases in the drum. The drum has an orifice therein at the side opposite from the inlet and outlet. A mixing liquid is introduced into the orifice adapted to be dispersed and evaporated by the exhaust gases entering the drum from the engine manifold to thereby cool the drum and the exhaust gases and at the same time to form compounds between the vapor and the detrimental matters prior to passing to the muffler. A dehydrating device receiving the discharge of the muffler is provided for discharging substantially pure air from thedehydracting device into the atmosphere.
Description
llnited States Patet 1 Nishinomiya 1 3,738,085 1 June 12, 1973 [76] Inventor: Tomekichi Nishinomiya, 1-11-2,
. Niijuku, Katsushika-ku, Tokyo,
Japan [22] Filed: Sept. 21 1971 [21] Appl. No.: 182,355
[30] Foreign Application Priority Data June 29, 1971 Japan 46/47417 [56] References Cited UNITED STATES PATENTS 1,048,111 12/1912 Tobey 261/79 A 1,080,208 12/1913 Gardner 55/DIG. 30
2,789,032 4/1957 Bayley et al. 55/DlG. 30 2,935,840 5/1960 Schoppe 261/79 A Primary ExaminerDennis E. Talbert, Jr. Attorney- Arthur E. Dowell, Jr. and Arthur E. Dowell, I11 1 [57] ABSTRACT Apparatus for the removal of detrimental matter from the exhaust gases of internal combustion engines in which a cylindrical drum having a substantially tangential inlet and an aligned substantially tangential outlet is disposed in the engine exhaust pipe for imparting a whirling motion to the exhaust gases in the drum. Th'e drum has an orifice therein at the side opposite from the inlet and outlet. A mixing liquid is introduced into the orifice adapted to be dispersed and evaporated by the exhaust'gases entering the drum from the engine manifold'to thereby cool the drum and the exhaust gases and at the same time to form compounds between the vapor and the detrimental matters prior to passing to the muffler. A dehydrating device receiving the discharge of the muffler is provided for discharging substantially pure air from thedehydracting device into the atmosphere.
8 Claims, 2 Drawing Figures PAIIENIED m w;
FIG. 2
I Q INVENTOR V M lid) BY AW DESCRIPTION OF INVENTION This invention relates to novel means for the removal of detrimental matter from the exhaust gases of internal combustion engines.
The principal object of the invention is to provide in such means a mixing device which is inserted in the exhaust pipe leading from the exhaust manifold of an internal combustion engine to the usual muffler, themixing device comprising a cylindrical drum having a substantially tangential inlet and an aligned substantially tangential outlet whereby the exhaust gases in passing through said exhaust pipe towards the muffler are given a whirling motion.
Into the drum of said mixing device is dropped a mixing liquid from a supply tank holding a quantity of water, phosphoris acid, peroxide of barium and peroxide of hydrogen. The mixing liquid dropped into the drum, disperses and evaporates by means of the heat of the gases exhausted from the engine. As this evaporated liquid cools down the inner part of the drum the exhaust gas which comes into the drum from the exhaust manifold is also cooled down and its volume decreases, and a low pressure condition occurs in the inner part of the drum. At the same time carbon monoxide, sulphurous acid gas, lead, hydrogenchloride, nitrogenoxide, carbon, dust, etc., are melted into the above mentioned evaporated mixed liquid, mingled into a compound with the vapor, and discharged from the exhaust gas outlet. The compound of the vapor and carbon monoxide, sulphurous acid gas, lead, hydrogenchloride, nitrogenoxide, carbon, dust, etc., which is discharged out of the outlet of the mixing device is dehydrated and separated by means of passing same beyond the muffler and through a dehydrating device in which calcium carbonate, etc., is contained, and which is connected to the rear end of the muffler, and the substantially pure air remained is discharged into the open air.
I will explain the invention with reference to the accompanying drawing, which illustrates one practical embodiment thereof, to enable others familiar with the art to adopt and use the same; and will summarize in the exhaust pipe between the manifold and muffler.
As shown in FIG. 2, the internal combustion engine l is provided with the usual exhaustmanifold 2. An exhaust pipe 3 connects the rear end of the intake manifold 2 with the inlet of a muffler 4. A dehydrating device 5 is connected by pipe 6 from the rear end of the muffler 4 to the inlet of the dehydrating device 5, which device exhausts through pipe 7 to the atmosphere.
In the pipe 3 is a mixing device shown more particularly in FIG. 2, the same consisting of a cylindrical drum 8 having a substantially tangential inlet 9 and an aligned substantially tangential outlet 10 whereby the exhaust gases entering the mixing drum 8 will give a whirling motion within the drum 8.
Extending laterally into the drum 8 at the side remote from the inlet 9 and outlet 10 is an orifice 8a (FIG. 1) receiving the end of a pipe 11 (FIG. 2) extending from a tank 12, which tank 12 holds a quantity of mixing liquid consisting of water, phosphoric acid, peroxide of barium and peroxide of hydrogen which is dropped from the pipe 11 into the drum 8.
In operation, when the engine 1 is in operation the mixing liquid from the tank 12 is dropped into the drum 8 and is dispersed and evaporates by means of the heat of the gas exhausted from the engine 1. As this evaporated mixing liquid cools down the inner walls of the drum 8, the exhaust gas which is whirling within the drum 8 and which comes into contact with the walls of the drum 8 is also cooled down, and its volume decreases, and a low pressure condition occurs in the inner part of the drum 8. At the same time carbon monoxide, sulphurous acid gas, lead, hydrogenchloride nishowing means for introducing the mixing liquid into trogenoxide, carbon, dust, etc., are melted into the above mentioned evaporated mixing liquid, mingled into a compound with the vapor and discharged from the exhaust gas outlet 10. The compound of the vapor and carbon monoxide, sulphurous acid gas, lead, hydrogenchloride, nitrogenoxide, carbon, dust, etc., which is discharged out of the outlet 10 is dehydrated and separated by means of passing from muffler 4 through the dehydrating device 5 in which calcium carbonate etc. is contained, and which device 5 is connected with the rear end of the muffler 4, and the pure air remaining in the dehydrating device 6 is discharged into the open air or atmosphere.
Each of the devices, i.e., the mixing device 8 of the exhaust pipe 3 which is characterized by its capacity of forming the compound of the detrimental matters in the exhaust-gas and the vapor into which the mixing liquid is transformed by the heat from the exhaust-gas which enters the drum 8, and the dehydrating device 5 of the detachable container which contains the dehydrator in which the chief ingredient is calcium, together form novel means for removal of detrimental matter contained in the exhaust gas of internal combustion engines.
I claim:
1. Apparatus for the removal of detrimental matter from the exhaust gases of internal combustion engines having an exhaust manifold, and an exhaust pipe extending from said manifold, comprising a cylindrical drum having a substantially tangential inlet and outlet disposed in the exhaust pipe for imparting a whirling motion to said exhaust gases in said drum; said drum having an orifice therein; means for introducing a mixing liquid into said orifice which will be dispersed and evaporated by the exhaust gases entering from said manifold to thereby cool the drum and the exhaust gases and at the same time to form compounds between 1 3. In apparatus as set forth in claim 1, said detrimental matters comprising carbon monoxide, sulphurous acid gas, lead, hydrogenchloride, nitrogenoxide, carbon, and dust which are melted into the evaporated mixing liquid and form compounds with said vapor.
4. In apparatus as set forth in claim 1, said dehydrating chamber containing calcium carbonate.
5. Apparatus for the removal of detrimental matter from the exhaust gases of internal combustion engines having an exhaust manifold, a muffler, and an exhaust pipe connecting said manifold and muffler, comprising a cylindrical drum having a substantially tangential inlet and an aligned substantially tangential outlet disposed in the exhaust pipe for imparting a whirling motion to said exhaust gases in said drum; said drum having an orifice therein at the side opposite from said inlet and outlet; means for introducing a mixing liquid into said orifice which will be dispersed and evaporated by the exhaust gases entering from said manifold to thereby cool the drum and the exhaust gases and at the same time to form compounds between said vapor and said detrimental matters prior to passing to the muffler; and a dehydrating device receiving the discharge of the muffler for discharging substantially pure air from the dehydrating device into the atmosphere.
6. In apparatus as set forth in claim 5, said mixing liquid comprising water, phosphoric acid, peroxide of barium and peroxide of hydrogen.
7. In apparatus as set forth in claim 5, said detrimental matters comprising carbon monoxide, sulphurous acid gas, lead, hydrogenchloride, nitrogenoxide, carbon, and dust which are melted into the evaporated mixing liquid and form compounds with said vapor.
8. In apparatus as set forth in claim 5, said dehydrating chamber containing calcium carbonate.
Claims (7)
- 2. In apparatus as set forth in claim 1, said mixing liquid comprising water, phosphoric acid, peroxide of barium and peroxide of hydrogen.
- 3. In apparatus as set forth in claim 1, said detrimental matters comprising carbon monoxide, sulphurous acid gas, lead, hydrogenchloride, nitrogenoxide, carbon, and dust which are melted into the evaporated mixing liquid and form compounds with said vapor.
- 4. In apparatus as set forth in claim 1, said dehydrating chamber containing calcium carbonate.
- 5. Apparatus for the removal of detrimental matter from the exhaust gases of internal combustion engines having an exhaust manifold, a muffler, and an exhaust pipe connecting said manifold and muffler, comprising a cylindrical drum having a substantially tangential inlet and an aligned substantially tangential outlet disposed in the exhaust pipe for imparting a whirling motion to said exhaust gases in said drum; said drum having an orifice therein at the side opposite from said inlet and outlet; means for introducing a mixing liquid into said orifice which will be dispersed and evaporated by the exhaust gases entering from said manifold to thereby cool the drum and the exhaust gases and at the same time to form compounds between said vapor and said detrimental matters prior to passing to the muffler; and a dehydrating device receiving the discharge of the muffler for discharging substantially pure air from the dehydrating device into the atmosphere.
- 6. In apparatus as set forth in claim 5, said mixing liquid comprising water, phosphoric acid, peroxide of barium and peroxide of hydrogen.
- 7. In apparatus as set forth in claim 5, said detrimental matters comprising carbon monoxide, sulphurous acid gas, lead, hydrogenchloride, nitrogenoxide, carbon, and dust which are melted into the evaporated mixing liquid and form compounds with said vapor.
- 8. In apparatus as set forth in claim 5, said dehydrating chamber containing calcium carbonate.
Applications Claiming Priority (1)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
JP4741771 | 1971-06-29 |
Publications (1)
Publication Number | Publication Date |
---|---|
US3738085A true US3738085A (en) | 1973-06-12 |
Family
ID=12774562
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
US00182355A Expired - Lifetime US3738085A (en) | 1971-06-29 | 1971-09-21 | Device for the removal of detrimental matter from exhaust gases of internal combustion engines |
Country Status (3)
Country | Link |
---|---|
US (1) | US3738085A (en) |
FR (1) | FR2177670A1 (en) |
GB (1) | GB1361315A (en) |
Cited By (5)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US4074975A (en) * | 1973-05-07 | 1978-02-21 | Nissan Motor Company, Limited | Combination exhaust-gas cleaner and muffler for an automobile engine |
US4670233A (en) * | 1984-10-04 | 1987-06-02 | Filterwerk Mann & Hummel Gmbh | Method of removing soot which has been trapped in an exhaust gas filter of an internal combustion engine |
US5175998A (en) * | 1989-11-22 | 1993-01-05 | Leonid Simuni | Exhaust system |
US5367876A (en) * | 1992-04-02 | 1994-11-29 | Harper, Iii; Raymond F. | Apparatus for controlling of automotive exhaust emissions by treatment of exhausting gases traveling through an automotive exhaust conduit |
DE19515649A1 (en) * | 1995-04-28 | 1995-10-05 | Wilhelm Dr Ing Wiederhold | High efficiency combined impact- and electrostatic filter |
Citations (4)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US1048111A (en) * | 1912-08-15 | 1912-12-24 | William L Tobey | Muffling device. |
US1080208A (en) * | 1912-10-28 | 1913-12-02 | George W Gardner | Cleaner for engine-cylinders. |
US2789032A (en) * | 1953-06-05 | 1957-04-16 | United States Borax Chem | Method for scrubbing exhaust gases from diesel engines |
US2935840A (en) * | 1953-02-26 | 1960-05-10 | Metallbau Semler Gmbh | Fluid mixing chamber |
-
1971
- 1971-09-21 US US00182355A patent/US3738085A/en not_active Expired - Lifetime
-
1972
- 1972-05-02 GB GB2034872A patent/GB1361315A/en not_active Expired
- 1972-06-16 FR FR7221715A patent/FR2177670A1/fr not_active Withdrawn
Patent Citations (4)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US1048111A (en) * | 1912-08-15 | 1912-12-24 | William L Tobey | Muffling device. |
US1080208A (en) * | 1912-10-28 | 1913-12-02 | George W Gardner | Cleaner for engine-cylinders. |
US2935840A (en) * | 1953-02-26 | 1960-05-10 | Metallbau Semler Gmbh | Fluid mixing chamber |
US2789032A (en) * | 1953-06-05 | 1957-04-16 | United States Borax Chem | Method for scrubbing exhaust gases from diesel engines |
Cited By (5)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US4074975A (en) * | 1973-05-07 | 1978-02-21 | Nissan Motor Company, Limited | Combination exhaust-gas cleaner and muffler for an automobile engine |
US4670233A (en) * | 1984-10-04 | 1987-06-02 | Filterwerk Mann & Hummel Gmbh | Method of removing soot which has been trapped in an exhaust gas filter of an internal combustion engine |
US5175998A (en) * | 1989-11-22 | 1993-01-05 | Leonid Simuni | Exhaust system |
US5367876A (en) * | 1992-04-02 | 1994-11-29 | Harper, Iii; Raymond F. | Apparatus for controlling of automotive exhaust emissions by treatment of exhausting gases traveling through an automotive exhaust conduit |
DE19515649A1 (en) * | 1995-04-28 | 1995-10-05 | Wilhelm Dr Ing Wiederhold | High efficiency combined impact- and electrostatic filter |
Also Published As
Publication number | Publication date |
---|---|
FR2177670A1 (en) | 1973-11-09 |
GB1361315A (en) | 1974-07-24 |
DE2147685B2 (en) | 1976-12-23 |
DE2147685A1 (en) | 1973-01-18 |
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