US3242423A - Resonance cells for optical pumping - Google Patents

Resonance cells for optical pumping Download PDF

Info

Publication number
US3242423A
US3242423A US250382A US25038263A US3242423A US 3242423 A US3242423 A US 3242423A US 250382 A US250382 A US 250382A US 25038263 A US25038263 A US 25038263A US 3242423 A US3242423 A US 3242423A
Authority
US
United States
Prior art keywords
bulb
vessel
metal
optical pumping
pumping
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Lifetime
Application number
US250382A
Inventor
Malnar Leon
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Thales SA
Original Assignee
Csf
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Csf filed Critical Csf
Application granted granted Critical
Publication of US3242423A publication Critical patent/US3242423A/en
Anticipated expiration legal-status Critical
Expired - Lifetime legal-status Critical Current

Links

Images

Classifications

    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N27/00Investigating or analysing materials by the use of electric, electrochemical, or magnetic means
    • G01N27/72Investigating or analysing materials by the use of electric, electrochemical, or magnetic means by investigating magnetic variables
    • G01N27/74Investigating or analysing materials by the use of electric, electrochemical, or magnetic means by investigating magnetic variables of fluids
    • GPHYSICS
    • G01MEASURING; TESTING
    • G01RMEASURING ELECTRIC VARIABLES; MEASURING MAGNETIC VARIABLES
    • G01R33/00Arrangements or instruments for measuring magnetic variables
    • G01R33/20Arrangements or instruments for measuring magnetic variables involving magnetic resonance
    • G01R33/24Arrangements or instruments for measuring magnetic variables involving magnetic resonance for measuring direction or magnitude of magnetic fields or magnetic flux
    • G01R33/26Arrangements or instruments for measuring magnetic variables involving magnetic resonance for measuring direction or magnitude of magnetic fields or magnetic flux using optical pumping
    • GPHYSICS
    • G04HOROLOGY
    • G04FTIME-INTERVAL MEASURING
    • G04F5/00Apparatus for producing preselected time intervals for use as timing standards
    • G04F5/14Apparatus for producing preselected time intervals for use as timing standards using atomic clocks

Definitions

  • RESONANCE CELLS FOR OPTICAL PUMPING Filed Jan. 9, 1963 United States Patent 3 242 423 RESGNANCE CELLS F0 R OPTICAL PUMPING Lon Malnar, Paris, France, assignor to C.S.F.Compagnie gnrale de tlgraphie Sans Fil, a corporation of The present invention relates to resonance cells for optical pumping.
  • Such cells may be used in many applications, for example in certain magnetometers. They may comprise a glass or Pyrex vessel containing an alkali metal, such as cesium or rubidium, and saturated vapour of this metal and, in a magnetometer, the vapour is subjected to the action of a uniform magnetic field.
  • the saturated vapour is at a low pressure and the mean free path of the atom is greater than the dimensions of the vessel.
  • the vapour atoms are subjected to a large number of impacts against the wall, resulting in the destruction of the favourable orientation due to optical pumping.
  • a rare gas such as argon
  • the walls of the vessel may be coated with a layer of parafiin or silicone against which the atoms may be rebound without changing their orientation.
  • This layer has to be very thin, so as to maintain the transparency of the vessel to the light from the optical pump and this makes it difficult to coat certain portions of the vessel, for example the pumping stem, with the protecting layer.
  • the collision of the atoms of the gaseous metal against the solid metal also contributes to change the orientation of these atoms.
  • the metal in solid state is contained in a portion of the cell building up a bulb formed in the wall of the cell and communicating with the latter through a bent portion.
  • This bulb is, for example, arranged to be in symmetrical relationship to the pumping stem, with respect to the axis of symmetry of the body of the cell.
  • FIGS. 1 and 2 show, very diagrammatically, various embodiments of a vessel for resonance cells according to the invention.
  • Vessel 1 is provided with a pumping stem 2 for evacuating vessel 1 and introducing rare gas therein.
  • a bulb 3, integral with vessel 1, is arranged for receiving metal 4 in solid state.
  • bulb 3 and the pumping stem 2 are positioned symmetrically with respect to the axis of vessel 1.
  • bulb 3 communicates with vessel 1 through a bent por- 3,242,423 Patented Mar. 22, 1966 tion 6 so that the metal in solid state 4 does not directly face the body of vessel 1.
  • the pumping stem 2 has also a bent portion 7 similar to that of bulb 3.
  • the arrangement shown in FIGS. 1 and 2 makes it possible to avoid the disorientation of the atoms of the vaporized metal through collision with the solid metal 4, while a substantial amount of the latter can be placed in bulb 3.
  • the body of vessel 1 may be spherically shaped, which reduces the impacts of atoms against the walls.
  • the number of these impacts is, as known, proportional to the surface of the body, whereas, for a given pressure, the number of the atoms is proportional to the volume of the body.
  • the ratio of the volume to the inner surface is a maximum; it follows that the coefiicient of disorientation through impacts against the walls is a minimum when vessel 1 has a spherical shape.
  • the magnetic field applied may be, for example, perpendicular to the axis of the cell.
  • the cell may then assume any desired position around an axis perpendicular to the magnetic field, without this resulting in any particular trouble as to the space required.
  • the described vessels are of course made of a material transparent to the light of the pump. They can contain a large amount of metal in solid state.
  • a resonance cell for optical pumping systems comprising in combination: a vacuum tight vessel having walls and including a main body, a bulb having a bent portion, formed in one of said walls and communicating with said body, and a pumping stem; and an alkali metal in said bulb and saturated vapour of this metal filling said vessel, whereby metal in the solid state in said bulb does not directly face said body.
  • a resonance cell for optical pumping systems comprising in combination: a vacuum tight vessel, having walls and an axis of symmetry, and including a main body, a bulb having a bent portion formed in one of said walls and communicating with said body, and a bent pumping stern; an alkali metal in said bulb and saturated vapour of this metal filling said vessel; said stern and said bulb being arranged symmetrically with respect to said axis, whereby metal in the solid state in said bulb does not directly face said body.
  • a resonance cell for optical pumping systems comprising in combination: a vacuum tight rotational vessel having a lateral wall and including a main body, a bulb having a bent portion, formed in said wall and communicating with said body, and a pumping stern; an alkali metal in said bulb and saturated vapour of this metal filling said vessel, whereby metal in the solid state in said bulb does not directly face said body.

Landscapes

  • Physics & Mathematics (AREA)
  • General Physics & Mathematics (AREA)
  • Chemical & Material Sciences (AREA)
  • General Health & Medical Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Analytical Chemistry (AREA)
  • Biochemistry (AREA)
  • Electrochemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Immunology (AREA)
  • Pathology (AREA)
  • Condensed Matter Physics & Semiconductors (AREA)
  • Discharge Lamps And Accessories Thereof (AREA)
  • Optical Measuring Cells (AREA)

Description

March 22, 1966 MALNAR 3,242,423
RESONANCE CELLS FOR OPTICAL PUMPING Filed Jan. 9, 1963 United States Patent 3 242 423 RESGNANCE CELLS F0 R OPTICAL PUMPING Lon Malnar, Paris, France, assignor to C.S.F.Compagnie gnrale de tlgraphie Sans Fil, a corporation of The present invention relates to resonance cells for optical pumping. Such cells may be used in many applications, for example in certain magnetometers. They may comprise a glass or Pyrex vessel containing an alkali metal, such as cesium or rubidium, and saturated vapour of this metal and, in a magnetometer, the vapour is subjected to the action of a uniform magnetic field.
Under the action of an optical pump the population of excited atoms, the magnetic moment of which is parallel to the magnetic field applied, increases.
However, known cells of this type have a major drawback.
The saturated vapour is at a low pressure and the mean free path of the atom is greater than the dimensions of the vessel. The vapour atoms are subjected to a large number of impacts against the wall, resulting in the destruction of the favourable orientation due to optical pumping.
To eliminate this drawback, a rare gas, such as argon, may be introduced into the vessel at a pressure higher than that of the vapour, or else the walls of the vessel may be coated with a layer of parafiin or silicone against which the atoms may be rebound without changing their orientation.
This layer has to be very thin, so as to maintain the transparency of the vessel to the light from the optical pump and this makes it difficult to coat certain portions of the vessel, for example the pumping stem, with the protecting layer.
In addition, the collision of the atoms of the gaseous metal against the solid metal also contributes to change the orientation of these atoms.
It is an object of the invention to provide a resonant cell for optical pumping, which does not present those drawbacks.
According to a feature of the invention, the metal in solid state is contained in a portion of the cell building up a bulb formed in the wall of the cell and communicating with the latter through a bent portion. This bulb is, for example, arranged to be in symmetrical relationship to the pumping stem, with respect to the axis of symmetry of the body of the cell.
The invention will be best understood from the following description and appended drawing, wherein:
FIGS. 1 and 2 show, very diagrammatically, various embodiments of a vessel for resonance cells according to the invention.
The same reference numerals designate the same elements throughout all the figures.
Vessel 1 is provided with a pumping stem 2 for evacuating vessel 1 and introducing rare gas therein. A bulb 3, integral with vessel 1, is arranged for receiving metal 4 in solid state.
Referring to FIGS. 1 and 2, it may be seen that bulb 3 and the pumping stem 2 are positioned symmetrically with respect to the axis of vessel 1. In these figures, bulb 3 communicates with vessel 1 through a bent por- 3,242,423 Patented Mar. 22, 1966 tion 6 so that the metal in solid state 4 does not directly face the body of vessel 1.
In FIG. 2, the pumping stem 2 has also a bent portion 7 similar to that of bulb 3. The arrangement shown in FIGS. 1 and 2 makes it possible to avoid the disorientation of the atoms of the vaporized metal through collision with the solid metal 4, while a substantial amount of the latter can be placed in bulb 3.
The body of vessel 1 may be spherically shaped, which reduces the impacts of atoms against the walls. The number of these impacts is, as known, proportional to the surface of the body, whereas, for a given pressure, the number of the atoms is proportional to the volume of the body. In a sphere the ratio of the volume to the inner surface is a maximum; it follows that the coefiicient of disorientation through impacts against the walls is a minimum when vessel 1 has a spherical shape.
- The magnetic field applied may be, for example, perpendicular to the axis of the cell. The cell may then assume any desired position around an axis perpendicular to the magnetic field, without this resulting in any particular trouble as to the space required.
The described vessels are of course made of a material transparent to the light of the pump. They can contain a large amount of metal in solid state.
Of course, the invention is not limited to the embodiments shown which are given solely by way of example.
What is claimed is:
1. A resonance cell for optical pumping systems comprising in combination: a vacuum tight vessel having walls and including a main body, a bulb having a bent portion, formed in one of said walls and communicating with said body, and a pumping stem; and an alkali metal in said bulb and saturated vapour of this metal filling said vessel, whereby metal in the solid state in said bulb does not directly face said body.
2. A resonance cell for optical pumping systems comprising in combination: a vacuum tight vessel, having walls and an axis of symmetry, and including a main body, a bulb having a bent portion formed in one of said walls and communicating with said body, and a bent pumping stern; an alkali metal in said bulb and saturated vapour of this metal filling said vessel; said stern and said bulb being arranged symmetrically with respect to said axis, whereby metal in the solid state in said bulb does not directly face said body.
3. A resonance cell for optical pumping systems comprising in combination: a vacuum tight rotational vessel having a lateral wall and including a main body, a bulb having a bent portion, formed in said wall and communicating with said body, and a pumping stern; an alkali metal in said bulb and saturated vapour of this metal filling said vessel, whereby metal in the solid state in said bulb does not directly face said body.
References Cited by the Examiner UNITED STATES PATENTS 2,884,524 4/1959 Dicke 324-0.5 3,038,126 6/1962 Robinson 3240.5
FOREIGN PATENTS 1,215,432 11/1959 France.
875,242 8/ 1961 Great Britain.
(Other references on following page) 3 OTHER REFERENCES Carpenter et al.: Physical Review, vol. 46, October 1934, pp. 607 to 612.
De Zafra: American Journal of Physics, vol. 28, No. 7, October 1960, pp. 646 to 654 incl.
Franzen: Physical Review, vol. 115, No. 4, Aug. 15, 1949, pages 850 to 856 inclusive.
Kastler: The Ann Arbor Conference on Optical PumpingUniversity of Michigan, Ann Arbor, Michigan, June 1959, pp. 71-73 principally relied on.
4 Novick: Ann Arbor Conference on Optical Pumping, pages 11 to 16 relied on.
Ritter et 211.: Royal Society of London, Proceedings, vol. 238, N0. 1215, Jan. 29, 1957, pp. 473 to 488 (pp. 477479 principally relied on).
CHESTER L. JUSTUS, Primary Examiner.
MAYNARD R. WILBUR, Examiner.

Claims (1)

1. A RESONANCE CELL FOR OPTICAL PUMPING SYSTEMS COMPRISING IN COMBINATION; A VACUUM TIGHT VESSEL HAVING WALLS AND INCLUDING A MAIN BODY, A BULB HAVING A BENT PORTION, FORMED IN ONE OF SAID WALLS AND COMMUNICATING WITH SAID BODY, AND A PUMPING STEM; AND AN ALKALI METAL IN SAID BULB AND SATURATED VAPOUR OF THIS METAL FILLING SAID VESSEL, WHEREBY METAL IN THE SOLID STATE IN SAID BULB DOES NOT DIRECTLY FACE SAID BODY.
US250382A 1962-01-10 1963-01-09 Resonance cells for optical pumping Expired - Lifetime US3242423A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
FR884376A FR1318738A (en) 1962-01-10 1962-01-10 Optical pumping resonance cell enhancements

Publications (1)

Publication Number Publication Date
US3242423A true US3242423A (en) 1966-03-22

Family

ID=8770212

Family Applications (1)

Application Number Title Priority Date Filing Date
US250382A Expired - Lifetime US3242423A (en) 1962-01-10 1963-01-09 Resonance cells for optical pumping

Country Status (4)

Country Link
US (1) US3242423A (en)
DE (1) DE1295082B (en)
FR (1) FR1318738A (en)
GB (1) GB1036002A (en)

Cited By (8)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3418565A (en) * 1965-07-22 1968-12-24 Csf Optical resonance cells
US3510758A (en) * 1967-11-14 1970-05-05 Varian Associates Atomic resonance gas cell having an evacuated double end wall structure
US3536993A (en) * 1967-10-18 1970-10-27 Csf Optical resonance cells
US3629697A (en) * 1968-12-12 1971-12-21 Agencie Nationale De Valorisat Paramagnetic resonance and optical pumping magnetometer in the near zero magnetic field-range
US3675067A (en) * 1968-02-02 1972-07-04 Csf Optical resonance cell with means for regulating internal vapor pressure
US4405905A (en) * 1980-01-11 1983-09-20 Oscilloquartz S.A. Atomic frequency standard having microwave loop around absorption cell
US4596962A (en) * 1983-11-03 1986-06-24 Duke University Evacuated, wall-coated, sealed, alkali atom cell for an atomic frequency standard
US5256995A (en) * 1992-07-17 1993-10-26 Ball Corporation Low helium permeability atomic frequency standard cell and method for forming same

Families Citing this family (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US6295834B1 (en) * 1999-06-30 2001-10-02 Medi-Physics, Inc. NMR polarization monitoring coils, hyperpolarizers with same, and methods for determining the polarization level of accumulated hyperpolarized noble gases during production

Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2884524A (en) * 1955-08-01 1959-04-28 Robert H Dicke Method and system employing photon absorption by a microwave resonant medium
FR1215432A (en) * 1957-12-10 1960-04-19 Int Standard Electric Corp Improvements to micrometric oscillations production devices
GB875242A (en) * 1958-02-21 1961-08-16 Varian Associates Atomic stabilized frequency source
US3038126A (en) * 1960-11-22 1962-06-05 Space Technology Lab Inc Tuning arrangement utilizing optical pumping

Family Cites Families (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE553701C (en) * 1932-06-29 Karl Edmund Hermann Pressler Melting nozzle for vacuum vessels with a liquid bottom body
US1854912A (en) * 1930-01-18 1932-04-19 Ne Arga Corp Lamp starting device
NL39334C (en) * 1932-07-01
FR1250157A (en) * 1959-03-03 1961-01-06 Varian Associates Electrode-less discharge lamp

Patent Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2884524A (en) * 1955-08-01 1959-04-28 Robert H Dicke Method and system employing photon absorption by a microwave resonant medium
FR1215432A (en) * 1957-12-10 1960-04-19 Int Standard Electric Corp Improvements to micrometric oscillations production devices
GB875242A (en) * 1958-02-21 1961-08-16 Varian Associates Atomic stabilized frequency source
US3038126A (en) * 1960-11-22 1962-06-05 Space Technology Lab Inc Tuning arrangement utilizing optical pumping

Cited By (8)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3418565A (en) * 1965-07-22 1968-12-24 Csf Optical resonance cells
US3536993A (en) * 1967-10-18 1970-10-27 Csf Optical resonance cells
US3510758A (en) * 1967-11-14 1970-05-05 Varian Associates Atomic resonance gas cell having an evacuated double end wall structure
US3675067A (en) * 1968-02-02 1972-07-04 Csf Optical resonance cell with means for regulating internal vapor pressure
US3629697A (en) * 1968-12-12 1971-12-21 Agencie Nationale De Valorisat Paramagnetic resonance and optical pumping magnetometer in the near zero magnetic field-range
US4405905A (en) * 1980-01-11 1983-09-20 Oscilloquartz S.A. Atomic frequency standard having microwave loop around absorption cell
US4596962A (en) * 1983-11-03 1986-06-24 Duke University Evacuated, wall-coated, sealed, alkali atom cell for an atomic frequency standard
US5256995A (en) * 1992-07-17 1993-10-26 Ball Corporation Low helium permeability atomic frequency standard cell and method for forming same

Also Published As

Publication number Publication date
DE1295082B (en) 1969-05-14
GB1036002A (en) 1966-07-13
FR1318738A (en) 1963-02-22

Similar Documents

Publication Publication Date Title
US3242423A (en) Resonance cells for optical pumping
Miyake Fermi liquid theory of dilute submonolayer 3He on thin 4He II film: Dimer bound state and Cooper pairs
Török et al. Radial and vertical epicyclic frequencies of Keplerian motion in the field of Kerr naked singularities-Comparison with the black hole case and possible instability of naked-singularity accretion discs
US5371591A (en) Triaxial split-gain ring laser gyroscope
GB1477028A (en) Cryostat
Western et al. Linear polarization of astronomical masers by anisotropic pumping and its enhancement due to geometry
Hoyle et al. On the formation of elliptical galaxies
Schearer Ion polarization via Penning collisions with optically pumped metastable helium
DeBenedetti et al. The three-photon annihilation of positrons and electrons
US3577069A (en) Optical resonance cells containing an alloy of an alkali metal with another metal
US3566125A (en) Radiation excited light source
Kogan et al. Texture in layers of hydgoren isotopes condensed on a cooled substrate
GB964201A (en) Luminescent lamps
US3328633A (en) Molecular beam tube
Scheiman A review of monoethanolamine chemistry
US3153204A (en) Laser assembly
Pottasch Bright rims in diffuse nebulae
US3267360A (en) Optical absorption monitoring of aligned alkali atoms
Shaw et al. Cyclotron Resonance in Zinc
Carlqvist et al. Manifestations of electric currents in interstellar molecular clouds
GB953074A (en) Improvements in cold-cathode tubes
Ertmer et al. Cooled atomic beams for frequency standards
US3789253A (en) Crucible for vaporizing chemically active elements method of manufacturing the same and ion source including said crucible
US3536993A (en) Optical resonance cells
Morrissey et al. Intrinsic fragment spins generated in the reactions of 20Ne with 197Au and 238U at 12.6 MeV/nucleon