US2108386A - Lubricant preparation - Google Patents

Lubricant preparation Download PDF

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Publication number
US2108386A
US2108386A US49824A US4982435A US2108386A US 2108386 A US2108386 A US 2108386A US 49824 A US49824 A US 49824A US 4982435 A US4982435 A US 4982435A US 2108386 A US2108386 A US 2108386A
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US
United States
Prior art keywords
glycyl
nitrogen
oil
dihydroxybenzene
lubricant
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Lifetime
Application number
US49824A
Inventor
John M Musselman
Elliott B Mcconnell
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Standard Oil Co
Original Assignee
Standard Oil Co
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Standard Oil Co filed Critical Standard Oil Co
Priority to US49824A priority Critical patent/US2108386A/en
Application granted granted Critical
Publication of US2108386A publication Critical patent/US2108386A/en
Anticipated expiration legal-status Critical
Expired - Lifetime legal-status Critical Current

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Classifications

    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M1/00Liquid compositions essentially based on mineral lubricating oils or fatty oils; Their use as lubricants
    • C10M1/08Liquid compositions essentially based on mineral lubricating oils or fatty oils; Their use as lubricants with additives
    • CCHEMISTRY; METALLURGY
    • C10PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10MLUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M2215/00Organic non-macromolecular compounds containing nitrogen as ingredients in lubricant Compositions
    • C10M2215/02Amines, e.g. polyalkylene polyamines; Quaternary amines
    • C10M2215/06Amines, e.g. polyalkylene polyamines; Quaternary amines having amino groups bound to carbon atoms of six-membered aromatic rings
    • C10M2215/062Amines, e.g. polyalkylene polyamines; Quaternary amines having amino groups bound to carbon atoms of six-membered aromatic rings containing hydroxy groups bound to the aromatic ring

Definitions

  • Lubricating oils where subjected to high temperatures on ferrous base surfaces deteriorate quite rapidly. For emcient results therefore, lubricants obviating this have been much desired.
  • compositions of oils and certain glycyl oxy-hydrogen compounds present remarkable resistance against such deterioration and afford usage in conditions otherwise not satisfactorily met.
  • the invention comprises the features hereinafter fully described, and particularly pointed out in the claims, the following description and the contained data setting forth in detail certain illustrative embodiments of the invention, these being indicative however, of but a few of the various ways in which the principle of the invention may be employed.
  • an oil having lubricating viscosity, and a small proportion of a glycyl compound are mixed together, the latter .compound being of the general formula NR. H2NC.HzC0.R(OH)n, in which R. is a hydrocarbon radical and R(OH)n a polyhydroxy benzene in which there are at least Zhydroxyls and in 1,2 position.
  • the oil may be a petroleum oil of viscosity for instance 48 to 200 Saybolt Universal at 210 F.
  • glycyl compounds are nitrogen-alkyl glycyl polyhydroxy benzenes, nitrogen-cycloparaflin glycyl polyhydroxybenzenes, nitrogen-alkaryl glycyl polyhydroxybenzenes, nitrogen aryl glycyl polyhydroxybenzenes, and for instance nitrogen-o-tolyl-glycyl-1,2-dihydroxybenzene, nitrogen-m-cyclo-glycyl-1,2-dihydroxybenzene, nitrogen-p-isopropyl-phenyl-glycyl-1,2-
  • the glycyl derivative, as indicated, is in quite minor proportion. In general it is unnecessary to exceed 1 per cent thereof in the total'composition, and proportions as low as 0.01 per cent may be employed, depending somewhat upon the oil and the particular duty in view.
  • the glycyl com pounds in such amounts dissolve readily in the oil, and by emcient mixing to attain dissemination, the material is correspondingly prepared without recourse to complicated procedure or interference with desirable refinery practice.
  • a lubricant comprising an oil having lubricating viscosity and a small proportion of a compound of general formula NR.H2NCH2CO.R' (OH) 5 in which R is a hydrocarbon radical and R (0H) 11 a polyhydroixy benzene in which there are at least 2 hydroxyls and in 1,2 position.
  • a lubricant comprising an oil having lubricating viscosity and a small proportion of a nitrogen-alkyl-glycyl-polyhydroxybenzene in which there are at least 2 hydroxyls and in 1,2 position.
  • a lubricant comprising an oil having lubricating viscosity and a small proportion of a nitrogen cycloparaflin glycyl-polyhydroxybenzene in which there are at least 2 hydroxyls and in 1,2
  • a lubricant comprising an oil having lubrieating viscosity and a small proportion of nitrogen-benzyl-glycyl-1,2-dihydroxybenzene.

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  • Chemical & Material Sciences (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Lubricants (AREA)

Description

Patented Feb. :15, 193
any
poration of (thin No Drag. Appiication November 1%, M235 Serial No. cases a @s. (m. W-
Lubricating oils where subjected to high temperatures on ferrous base surfaces deteriorate quite rapidly. For emcient results therefore, lubricants obviating this have been much desired. We have now found that compositions of oils and certain glycyl oxy-hydrogen compounds present remarkable resistance against such deterioration and afford usage in conditions otherwise not satisfactorily met.
To the accomplishment of the foregoing and related ends, the invention, then, comprises the features hereinafter fully described, and particularly pointed out in the claims, the following description and the contained data setting forth in detail certain illustrative embodiments of the invention, these being indicative however, of but a few of the various ways in which the principle of the invention may be employed.
In accordance with the invention, an oil having lubricating viscosity, and a small proportion of a glycyl compound are mixed together, the latter .compound being of the general formula NR. H2NC.HzC0.R(OH)n, in which R. is a hydrocarbon radical and R(OH)n a polyhydroxy benzene in which there are at least Zhydroxyls and in 1,2 position. The oil may be a petroleum oil of viscosity for instance 48 to 200 Saybolt Universal at 210 F.
Representative of the glycyl compounds are nitrogen-alkyl glycyl polyhydroxy benzenes, nitrogen-cycloparaflin glycyl polyhydroxybenzenes, nitrogen-alkaryl glycyl polyhydroxybenzenes, nitrogen aryl glycyl polyhydroxybenzenes, and for instance nitrogen-o-tolyl-glycyl-1,2-dihydroxybenzene, nitrogen-m-cyclo-glycyl-1,2-dihydroxybenzene, nitrogen-p-isopropyl-phenyl-glycyl-1,2-
dihydroxybenzene, nitrogen-me'thyi-glycyl-1,2-dihydroxybenzene, nitrogen-cyclohexyl-glycyl-1,2-
I droxybenzene, etc.
The glycyl derivative, as indicated, is in quite minor proportion. In general it is unnecessary to exceed 1 per cent thereof in the total'composition, and proportions as low as 0.01 per cent may be employed, depending somewhat upon the oil and the particular duty in view. The glycyl com pounds in such amounts dissolve readily in the oil, and by emcient mixing to attain dissemination, the material is correspondingly prepared without recourse to complicated procedure or interference with desirable refinery practice. K
As an example: With a Mid-Continent neutral lubricating stock having a viscosity of 437 sec. Saybolt Universal at 100 F., there is incorporated 0.01 per cent of nitrogen-para-tolyl-glycyl-1,2- dihydroxybenzene.
As another example: Similary with a stock having lubricating viscosity there is incorporated nitrogen-cyc1ohexyl-glycyl-1,2-dihydroxybenzene.
As another example: Similary with a stock having lubricating viscosity there is incorporated nitrogen-benzyl-glycyl-1,2-dihydroxyben2ene.
Other modes of applying the principle of the invention may be employed, change being made as regards the details described, provided the features stated in any of the following claims, or the quivalent of such, be employed.
We therefore particularly point out and distinctlyclaim as our invention:---
l. A lubricant comprising an oil having lubricating viscosity and a small proportion of a compound of general formula NR.H2NCH2CO.R' (OH) 5 in which R is a hydrocarbon radical and R (0H) 11 a polyhydroixy benzene in which there are at least 2 hydroxyls and in 1,2 position.
2. A lubricant comprising an oil having lubricating viscosity and a small proportion of a nitrogen-alkyl-glycyl-polyhydroxybenzene in which there are at least 2 hydroxyls and in 1,2 position.
3. A lubricant comprising an oil having lubricating viscosity and a small proportion of a nitrogen cycloparaflin glycyl-polyhydroxybenzene in which there are at least 2 hydroxyls and in 1,2
7. A lubricant comprising an oil having lubrieating viscosity and a small proportion of nitrogen-benzyl-glycyl-1,2-dihydroxybenzene.
'JOHN M. MUSSELMAN.
EILIO'I'I' B. MCCONNELL
US49824A 1935-11-14 1935-11-14 Lubricant preparation Expired - Lifetime US2108386A (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
US49824A US2108386A (en) 1935-11-14 1935-11-14 Lubricant preparation

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Application Number Priority Date Filing Date Title
US49824A US2108386A (en) 1935-11-14 1935-11-14 Lubricant preparation

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US2108386A true US2108386A (en) 1938-02-15

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