SE412658B - SET IN CEMENT BEDDING ACID OR BORATE-RADIOACTIVE WASTE - Google Patents

SET IN CEMENT BEDDING ACID OR BORATE-RADIOACTIVE WASTE

Info

Publication number
SE412658B
SE412658B SE7707770A SE7707770A SE412658B SE 412658 B SE412658 B SE 412658B SE 7707770 A SE7707770 A SE 7707770A SE 7707770 A SE7707770 A SE 7707770A SE 412658 B SE412658 B SE 412658B
Authority
SE
Sweden
Prior art keywords
cement
radioactive waste
weight
borate
parts
Prior art date
Application number
SE7707770A
Other languages
Swedish (sv)
Other versions
SE7707770L (en
Inventor
H Christensen
Original Assignee
Asea Atom Ab
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Asea Atom Ab filed Critical Asea Atom Ab
Priority to SE7707770A priority Critical patent/SE412658B/en
Priority to CH616078A priority patent/CH638922A5/en
Priority to DE2827030A priority patent/DE2827030C2/en
Priority to FI781993A priority patent/FI66095C/en
Priority to JP8082178A priority patent/JPS5434000A/en
Publication of SE7707770L publication Critical patent/SE7707770L/en
Publication of SE412658B publication Critical patent/SE412658B/en

Links

Classifications

    • GPHYSICS
    • G21NUCLEAR PHYSICS; NUCLEAR ENGINEERING
    • G21FPROTECTION AGAINST X-RADIATION, GAMMA RADIATION, CORPUSCULAR RADIATION OR PARTICLE BOMBARDMENT; TREATING RADIOACTIVELY CONTAMINATED MATERIAL; DECONTAMINATION ARRANGEMENTS THEREFOR
    • G21F9/00Treating radioactively contaminated material; Decontamination arrangements therefor
    • G21F9/28Treating solids
    • G21F9/30Processing
    • G21F9/301Processing by fixation in stable solid media
    • G21F9/302Processing by fixation in stable solid media in an inorganic matrix
    • G21F9/304Cement or cement-like matrix
    • CCHEMISTRY; METALLURGY
    • C04CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
    • C04BLIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
    • C04B28/00Compositions of mortars, concrete or artificial stone, containing inorganic binders or the reaction product of an inorganic and an organic binder, e.g. polycarboxylate cements
    • C04B28/02Compositions of mortars, concrete or artificial stone, containing inorganic binders or the reaction product of an inorganic and an organic binder, e.g. polycarboxylate cements containing hydraulic cements other than calcium sulfates
    • GPHYSICS
    • G21NUCLEAR PHYSICS; NUCLEAR ENGINEERING
    • G21FPROTECTION AGAINST X-RADIATION, GAMMA RADIATION, CORPUSCULAR RADIATION OR PARTICLE BOMBARDMENT; TREATING RADIOACTIVELY CONTAMINATED MATERIAL; DECONTAMINATION ARRANGEMENTS THEREFOR
    • G21F9/00Treating radioactively contaminated material; Decontamination arrangements therefor
    • G21F9/04Treating liquids
    • G21F9/06Processing
    • G21F9/16Processing by fixation in stable solid media
    • G21F9/162Processing by fixation in stable solid media in an inorganic matrix, e.g. clays, zeolites
    • G21F9/165Cement or cement-like matrix
    • CCHEMISTRY; METALLURGY
    • C04CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
    • C04BLIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
    • C04B2111/00Mortars, concrete or artificial stone or mixtures to prepare them, characterised by specific function, property or use
    • C04B2111/00474Uses not provided for elsewhere in C04B2111/00
    • C04B2111/00767Uses not provided for elsewhere in C04B2111/00 for waste stabilisation purposes
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02WCLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO WASTEWATER TREATMENT OR WASTE MANAGEMENT
    • Y02W30/00Technologies for solid waste management
    • Y02W30/50Reuse, recycling or recovery technologies
    • Y02W30/91Use of waste materials as fillers for mortars or concrete

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Inorganic Chemistry (AREA)
  • General Engineering & Computer Science (AREA)
  • Ceramic Engineering (AREA)
  • Physics & Mathematics (AREA)
  • High Energy & Nuclear Physics (AREA)
  • Materials Engineering (AREA)
  • Structural Engineering (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Processing Of Solid Wastes (AREA)
  • Curing Cements, Concrete, And Artificial Stone (AREA)

Description

15 25 1707770-9 2 med synnerligen god hâllfasthet. Enligt uppfinningen åstadkommas detta genom att avfallet före blandningen med cementen behandlas med ett ämne, som neutra- lieerar den retarderande verkan, som borsyra och borater har på. cementens stelnsnde. 170 25707770-9 2 with extremely good strength. According to the invention, this is achieved by treating the waste before mixing with the cement with a substance which neutralises the retarding effect of boric acid and borates. cement setting.

Närmare bestämt avser den föreliggande uppfinningen ett sätt att i cement bädda in borsyra- eller borathaltigt radioaktivt avfall, varvid avfallet blandas med cement och blandningen bringas att stelna i en behållare, t e: en betongkokill, som kännetecknas av att det radioaktiva avfallet före bland- ningen med cementen behandlas med ett ämne 'som med borsyran respektiveboratet ger en 'i vatten svårlöslig eller komplexbunden förening. och består av kalcium- klorid eller annan, jordalkalimetallhalogenid, av kaliumfluorid eller annan galkalimetallfluorid såsom natrizmfluorid eller av en flervärd organisk hydroxyl- förening såsom polyvinylalkohol och mannit. Bland flervärda organiska hydroxyl- föreningar föredragee specielltsådana med fler än tre hydroxylgrupper. liamet tillsättes företrädesvis i fast form, om det radioaktiva avfallet, såsom är normalt för jonbytarmassor och indunstarkoncentrat, är vattenhaltigt.More particularly, the present invention relates to a method of embedding boric acid or borate-containing radioactive waste in cement, wherein the waste is mixed with cement and the mixture is made to solidify in a container, te: a concrete mold, which is characterized in that the radioactive waste before mixing with the cement is treated with a substance 'which with the boric acid and the borate, respectively, gives a' water-insoluble or complex-bound compound. and consists of calcium chloride or other, alkaline earth metal halide, of potassium fluoride or other alkaline earth metal fluoride such as sodium fluoride or of a polyhydric organic hydroxyl compound such as polyvinyl alcohol and mannit. Among polyhydric organic hydroxyl compounds, those with more than three hydroxyl groups are especially preferred. The laminate is preferably added in solid form if the radioactive waste, as is normal for ion exchange compositions and evaporator concentrates, is aqueous.

Den tillsatta. mängden av ämnet uppgår lämpligen till minut en med borsyrs- eller boratmängden ungefär stökiometrisk mängd. överskott på upp till i varje fall 25 9š har ingen negativ inverkan.The appointed. the amount of the substance suitably amounts to minute one with the amount of boric oxygen or borate approximately stoichiometric. surplus of up to at least 25 9š has no negative impact.

Av de nämnda ämnena ger jordalkalimetallklorider vid behandlingen av det bor- syra- eller borathaltiga radioaktiva avfallet svår-lösliga borater, alkalimetall- fluorider ger svårlösliga alkalimetallfluoborater och de fler-värda hydroxyl- föreningarna ger didiolkomplexer.Of the substances mentioned, alkaline earth metal chlorides in the treatment of the boric acid or borate-containing radioactive waste give sparingly soluble borates, alkali metal fluorides give sparingly soluble alkali metal fluoroborates and the polyhydric hydroxyl compounds give didiol complexes.

Före blandningen av det med ämnet behandlade radioaktiva avfallet med cement justeras pE-värdet vid användningen av jordalkalimetallklorider till omlnfing 11 och i övriga fall till omkring 8 eller däröver.Prior to mixing the radioactive waste treated with the substance with cement, the pE value in the use of alkaline earth metal chlorides is adjusted to around 11 and in other cases to about 8 or more.

I blandningen av radioaktivt avfall och cement inkorporeras lämpligen på. känt sätt ett vattsntätande medel, som hindrar vattentransport inom det stelnsde cementblocket. Exempel på. sådana medel är vattenglas, polymera material med förmåga att blockera vatteninträngzzing till det radioaktiva avfallet samt metalltvålar av högre fettsyror. längden vattentätande medel uppgår lämpligen till 1-20 viktsdelar per 100 viktsdelar cement. 10 15 25 '7707770-9 Uppfinningen skall beslmivas ytterligare i nedanstående exempel.The mixture of radioactive waste and cement is suitably incorporated on. known method a waterproofing agent which prevents water transport within the solidified cement block. Examples of. such agents are water glass, polymeric materials capable of blocking water penetration into the radioactive waste, and metal soaps of higher fatty acids. the length of waterproofing agent suitably amounts to 1-20 parts by weight per 100 parts by weight of cement. The invention will be further elucidated in the following examples.

Ehcemgl 1.Ehcemgl 1.

En jonbytarmassa av styrendivinvlbensentyp innehållande en blandning av korn med sulfonsyregwnipper och korn med kvartära amoniumgrxzpper, 'vilken an- vänts i primärloretsen i en tryckvattenreaktor och därvid absorberat box-syra. och natriumborater så att halten av dessa räknat som borsyra uppgår till 12 viktsprooent och dessutom radioaktiva ämnen, innehåller 35 viktsprooent torr- substans och 65 viktsprocent vatten. Till 1000 viktsdelar av denna jonbytar- massa sättas 125 viktsdelar pulverformig kaloiumklorid. Efter blandning av komponenterna nöjes pil-värdet till omkring.11 genom tillsats av natriumhydroxid.A styrene-divinylbenzene-type ion exchange mass containing a mixture of granules with sulfonic acid groups and grains with quaternary ammonium groups, which is used in the primary chlorine etch in a pressurized water reactor and thereby absorbed box acid. and sodium borates so that their content, calculated as boric acid, amounts to 12% by weight and, in addition, radioactive substances, contain 35% by weight of dry matter and 65% by weight of water. To 1000 parts by weight of this ion exchange mass is added 125 parts by weight of powdered potassium chloride. After mixing the components, the arrow value is satisfied to about 11 by the addition of sodium hydroxide.

Den så. erhållna. blandningen som omfattar omkring 1125 viktsdelar blandas med. 1600 viktsdelar cement och vidare med 32 viktsdeler vattenglas bestående ev lika delar silikat och vatten som vattentätande tillsats till oementen. Efter något dygn är massan stelnad och förblir sedan intakt. ' ggyel 2 1000 viktsdelar av en Jonbytarmassa av same slag som i Exempel 1 försättes med 460 viktsdelar kaïlitmfluoridpulver, varvid pH-värdet blir omkring 8. Efter blandning av komponenterna tillsättes till den erhållna blandningen 1300 vikte- delar cement och videre 26 viktsdelar av ett vattentätande medium bestående av sin: er (ingenjören-inse Per mgvalz, sverige). Liksom 1 föregående fall erhålles en stelnad produkt som är intakt. hångel 2 1000 viktsdelar av en jonbytarmassa av same slag som i Exempel 1 försättes med 820 viktsdslar mannit i pulverform. pil-värdet justeras med natriumbydroxid till 8. Blandningelx, som omfattar omkring 1820 viktsdelar blandas med 1000 viktsdslar cement och vidare med 20 viktsdelar vattenglas bestående av lika delar siliket och vatten. Liksom i föregående fall erhålles en stelnad produkt som är intakt.It saw. obtained. the mixture comprising about 1125 parts by weight is mixed with. 1600 parts by weight of cement and further with 32 parts by weight of water glass consisting of possibly equal parts of silicate and water as a waterproofing additive to the elements. After a few days, the mass solidifies and then remains intact. ggyel 2 1000 parts by weight of an ion exchange mass of the same kind as in Example 1 is added with 460 parts by weight of potassium fluoride powder, the pH value being about 8. After mixing the components, 1300 parts by weight of cement and a further 26 parts by weight of a waterproofing are added to the resulting mixture. medium consisting of sin: er (engineer-inse Per mgvalz, sweden). As in the previous case, a solidified product is obtained which is intact. hångel 2 1000 parts by weight of an ion exchange mass of the same kind as in Example 1 is added with 820 parts by weight of mannit in powder form. The arrow value is adjusted with sodium hydroxide to 8. Mixture elx, which comprises about 1820 parts by weight, is mixed with 1000 parts by weight of cement and further with 20 parts by weight of water glass consisting of equal parts of silica and water. As in the previous case, a solidified product is obtained which is intact.

Claims (1)

1. ?'7:Û'?770-9 \ ' 4 FATENTICHAV 'sätt att 1 cement baaaa m borsyæa- ene» beraflnmgc radioaktivt avfall. varvid. avfallet blandas med. cement och blandniflšeä bring-as att etelna i en behållaxe, t ex en betongkokill, k ä n n e t e c k n a t därav, att det radioaktiva avfallet före blanäningen med cementen behandlas med ett ämne sem med borsyran respektive boratet ger en i vatten svårlöslig eller komplexbunden förening och består av kalciumklqrid eller annan Jordalkalimetallhalogenid, av kaliumfluorid eller annan alkalimetallfluorid eller av en flervärâ organisk hyärcxylförening, t ex polyvinylalkohol eller mannit. _ ANFÜRDA PUBLIKATIONER: Sverige patentansökan 890/7?1.? '7: Û'? 770-9 \ '4 FATENTICHAV' way that 1 cement baaaa m borsyæa- ene »carry fl nmgc radioactive waste. whereby. the waste is mixed with. cement and mixtures are brought to etelna in a retaining shaft, for example a concrete mold, characterized in that the radioactive waste before mixing with the cement is treated with a substance which with the boric acid and borate gives a water-insoluble or complex-bound compound and consists of calcium chloride or other alkaline earth metal halide, of potassium fluoride or other alkali metal fluoride or of a polyhydric organic hydroxyl compound, for example polyvinyl alcohol or mannit. _ CALLED PUBLICATIONS: Sweden patent application 890/7?
SE7707770A 1977-07-05 1977-07-05 SET IN CEMENT BEDDING ACID OR BORATE-RADIOACTIVE WASTE SE412658B (en)

Priority Applications (5)

Application Number Priority Date Filing Date Title
SE7707770A SE412658B (en) 1977-07-05 1977-07-05 SET IN CEMENT BEDDING ACID OR BORATE-RADIOACTIVE WASTE
CH616078A CH638922A5 (en) 1977-07-05 1978-06-06 Method for embedding in cement radioactive waste containing boric acid or borate
DE2827030A DE2827030C2 (en) 1977-07-05 1978-06-20 Method for embedding radioactive waste containing boric acid or borate in cement
FI781993A FI66095C (en) 1977-07-05 1978-06-21 SAETT ATT I CEMENT BAEDDA IN BORSYRA ELLER BORATHALTIGT RADIOACTIVE AVFALL
JP8082178A JPS5434000A (en) 1977-07-05 1978-07-03 Method of sealing up radioactive waste containing boric acid or borate in cement

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
SE7707770A SE412658B (en) 1977-07-05 1977-07-05 SET IN CEMENT BEDDING ACID OR BORATE-RADIOACTIVE WASTE

Publications (2)

Publication Number Publication Date
SE7707770L SE7707770L (en) 1979-01-06
SE412658B true SE412658B (en) 1980-03-10

Family

ID=20331786

Family Applications (1)

Application Number Title Priority Date Filing Date
SE7707770A SE412658B (en) 1977-07-05 1977-07-05 SET IN CEMENT BEDDING ACID OR BORATE-RADIOACTIVE WASTE

Country Status (5)

Country Link
JP (1) JPS5434000A (en)
CH (1) CH638922A5 (en)
DE (1) DE2827030C2 (en)
FI (1) FI66095C (en)
SE (1) SE412658B (en)

Families Citing this family (10)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4416810A (en) * 1981-07-30 1983-11-22 Noakes John E Disposal of radioactive aromatic liquid wastes
US4504317A (en) * 1983-03-07 1985-03-12 Westinghouse Electric Corp. Encapsulation of boric acid slurries
US4620947A (en) * 1983-10-17 1986-11-04 Chem-Nuclear Systems, Inc. Solidification of aqueous radioactive waste using insoluble compounds of magnesium oxide
FR2565851B1 (en) * 1984-06-14 1994-02-11 Innovations Meca Alimentaires MECHANICAL SEPARATION HEAD, ESPECIALLY FOR THE TREATMENT OF CRUSHED CARCASES AND MACHINE EQUIPPED THEREWITH
JPS6118898A (en) * 1984-07-06 1986-01-27 株式会社日立製作所 Radioactive waste solidified body and manufacture thereof
JPS61239197A (en) * 1985-04-17 1986-10-24 ウエスチングハウス エレクトリック コ−ポレ−ション Radioacitve waste containing fixed cesium and fixing method thereof
US5143653A (en) * 1987-05-15 1992-09-01 Societe Anonyme: Societe Generale Pour Les Techniques Nouvelles-Sgn Process for immobilizing radioactive ion exchange resins by a hydraulic binder
FR2615315B1 (en) * 1987-05-15 1989-08-25 Sgn Soc Gen Tech Nouvelle METHOD FOR IMMOBILIZING RESINS EXCHANGING RADIOACTIVE IONS BY A HYDRAULIC BINDER
FR3080112B1 (en) * 2018-04-17 2020-05-01 Onet Technologies Cn PROCESS FOR CONDITIONING BORATE WASTE BY CEMENT
FI129112B (en) * 2018-12-16 2021-07-15 Fortum Power & Heat Oy Method for treating and solidifying liquid waste

Family Cites Families (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE2553569C2 (en) * 1975-11-28 1985-09-12 Kernforschungszentrum Karlsruhe Gmbh, 7500 Karlsruhe Process for the solidification of radioactive aqueous waste materials by spray calcination and subsequent embedding in a matrix made of glass or glass ceramic
DE2603116C2 (en) * 1976-01-28 1983-01-27 Nukem Gmbh, 6450 Hanau Process for the solidification of radioactive borate-containing aqueous solutions and suspensions

Also Published As

Publication number Publication date
DE2827030C2 (en) 1984-01-26
FI66095C (en) 1984-08-10
SE7707770L (en) 1979-01-06
FI66095B (en) 1984-04-30
JPS5434000A (en) 1979-03-13
CH638922A5 (en) 1983-10-14
DE2827030A1 (en) 1979-01-11
FI781993A7 (en) 1979-01-06
JPS6333118B2 (en) 1988-07-04

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