RU2009101923A - METHODS FOR PRODUCING A TOTAL PRODUCT WITH SELECTIVE PRODUCTION OF HYDROCARBONS - Google Patents

METHODS FOR PRODUCING A TOTAL PRODUCT WITH SELECTIVE PRODUCTION OF HYDROCARBONS Download PDF

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Publication number
RU2009101923A
RU2009101923A RU2009101923/04A RU2009101923A RU2009101923A RU 2009101923 A RU2009101923 A RU 2009101923A RU 2009101923/04 A RU2009101923/04 A RU 2009101923/04A RU 2009101923 A RU2009101923 A RU 2009101923A RU 2009101923 A RU2009101923 A RU 2009101923A
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inorganic salt
total product
carbon
alkaline earth
salt catalysts
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RU2009101923/04A
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Russian (ru)
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Томас Фэйрчайлд БРАУНСКОМБ (US)
Томас Фэйрчайлд Браунскомб
Уильям Дуглас ГИЛЛЕСПИ (US)
Уильям Дуглас ГИЛЛЕСПИ
Вейджиан МО (US)
Вейджиан МО
Эсварачандра Кумар ПАРУЧУРИ (US)
Эсварачандра Кумар ПАРУЧУРИ
Сьюзан Сикор ФРЕМ (US)
Сьюзан Сикор ФРЕМ
Чен Элизабет РАМАЧАНДРАН (US)
Чен Элизабет Рамачандран
Дейвид Уильям УОЛЛАС (US)
Дейвид Уильям УОЛЛАС
Скотт Ли ВЕЛЛИНГТОН (US)
Скотт Ли Веллингтон
Original Assignee
Шелл Интернэшнл Рисерч Маатсхаппий Б.В. (NL)
Шелл Интернэшнл Рисерч Маатсхаппий Б.В.
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Publication of RU2009101923A publication Critical patent/RU2009101923A/en

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    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G47/00—Cracking of hydrocarbon oils, in the presence of hydrogen or hydrogen- generating compounds, to obtain lower boiling fractions
    • C10G47/02—Cracking of hydrocarbon oils, in the presence of hydrogen or hydrogen- generating compounds, to obtain lower boiling fractions characterised by the catalyst used

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  • Chemical & Material Sciences (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Production Of Liquid Hydrocarbon Mixture For Refining Petroleum (AREA)
  • Catalysts (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Abstract

1. Способ получения суммарного продукта, который включает: ! контактирование сырья с источником водорода в присутствии одного или нескольких неорганических солевых катализаторов и водяного пара с целью получения суммарного продукта; и ! регулирование условий контактирования таким образом, что степень превращения сырья в углеводородные газы и жидкие углеводороды в суммарном продукте составляет между 5 и 50%, в расчете на количество молей углерода в сырье. ! 2. Способ по п.1, в котором суммарный продукт также содержит газообразные оксиды углерода, и условия контактирования регулируют таким образом, что степень превращения сырья в газообразные оксиды углерода составляет между 55 и 95% или между 80 и 95% в расчете на количество молей углерода в сырье. ! 3. Способ по п.1 или 2, в котором неорганический солевой катализатор содержит один или несколько щелочных металлов, одно или несколько соединений одного или нескольких щелочных металлов, один или несколько щелочноземельных металлов, одно или несколько соединений одного или нескольких щелочноземельных металлов или их сочетания. ! 4. Способ по по п.1 или 2, в котором, по меньшей мере, один из неорганических солевых катализаторов представляет собой смесь одного или нескольких оксидов щелочноземельных металлов. ! 5. Способ по п.1 или 2, в котором, по меньшей мере, один из неорганических солевых катализаторов представляет собой смесь одного или нескольких оксидов щелочноземельных металлов, и степень превращения сырья в газообразные и жидкие углеводороды в суммарном продукте составляет между 5 и 30%. ! 6. Способ по п.1 или 2, в котором, по меньшей мере, один из неорганических солевых кат 1. A method for obtaining a total product, which includes: ! contacting the feedstock with a hydrogen source in the presence of one or more inorganic salt catalysts and steam to obtain a net product; and ! adjusting the contacting conditions such that the degree of conversion of the feedstock into hydrocarbon gases and liquid hydrocarbons in the total product is between 5 and 50%, based on the number of moles of carbon in the feedstock. ! 2. Process according to claim 1, wherein the total product also contains gaseous carbon oxides, and the contacting conditions are controlled so that the degree of conversion of the raw material into gaseous carbon oxides is between 55 and 95%, or between 80 and 95%, based on the number of moles carbon in raw materials. ! 3. The method according to claim 1 or 2, wherein the inorganic salt catalyst comprises one or more alkali metals, one or more compounds of one or more alkali metals, one or more alkaline earth metals, one or more compounds of one or more alkaline earth metals, or combinations thereof. . ! 4. The process according to claim 1 or 2, wherein at least one of the inorganic salt catalysts is a mixture of one or more alkaline earth metal oxides. ! 5. Process according to claim 1 or 2, wherein at least one of the inorganic salt catalysts is a mixture of one or more alkaline earth metal oxides and the conversion rate of the feedstock to gaseous and liquid hydrocarbons in the total product is between 5 and 30% . ! 6. The method according to claim 1 or 2, in which at least one of the inorganic salt cat

Claims (15)

1. Способ получения суммарного продукта, который включает:1. The method of obtaining the total product, which includes: контактирование сырья с источником водорода в присутствии одного или нескольких неорганических солевых катализаторов и водяного пара с целью получения суммарного продукта; иcontacting the feed with a hydrogen source in the presence of one or more inorganic salt catalysts and water vapor in order to obtain a total product; and регулирование условий контактирования таким образом, что степень превращения сырья в углеводородные газы и жидкие углеводороды в суммарном продукте составляет между 5 и 50%, в расчете на количество молей углерода в сырье.regulation of the contact conditions in such a way that the degree of conversion of the feed into hydrocarbon gases and liquid hydrocarbons in the total product is between 5 and 50%, based on the number of moles of carbon in the feed. 2. Способ по п.1, в котором суммарный продукт также содержит газообразные оксиды углерода, и условия контактирования регулируют таким образом, что степень превращения сырья в газообразные оксиды углерода составляет между 55 и 95% или между 80 и 95% в расчете на количество молей углерода в сырье.2. The method according to claim 1, in which the total product also contains gaseous carbon oxides, and the contacting conditions are controlled so that the degree of conversion of the feed to gaseous carbon oxides is between 55 and 95% or between 80 and 95% based on the number of moles carbon in raw materials. 3. Способ по п.1 или 2, в котором неорганический солевой катализатор содержит один или несколько щелочных металлов, одно или несколько соединений одного или нескольких щелочных металлов, один или несколько щелочноземельных металлов, одно или несколько соединений одного или нескольких щелочноземельных металлов или их сочетания.3. The method according to claim 1 or 2, in which the inorganic salt catalyst contains one or more alkali metals, one or more compounds of one or more alkali metals, one or more alkaline earth metals, one or more compounds of one or more alkaline earth metals, or a combination thereof . 4. Способ по по п.1 или 2, в котором, по меньшей мере, один из неорганических солевых катализаторов представляет собой смесь одного или нескольких оксидов щелочноземельных металлов.4. The method according to claim 1 or 2, in which at least one of the inorganic salt catalysts is a mixture of one or more oxides of alkaline earth metals. 5. Способ по п.1 или 2, в котором, по меньшей мере, один из неорганических солевых катализаторов представляет собой смесь одного или нескольких оксидов щелочноземельных металлов, и степень превращения сырья в газообразные и жидкие углеводороды в суммарном продукте составляет между 5 и 30%.5. The method according to claim 1 or 2, in which at least one of the inorganic salt catalysts is a mixture of one or more oxides of alkaline earth metals, and the degree of conversion of the feed into gaseous and liquid hydrocarbons in the total product is between 5 and 30% . 6. Способ по п.1 или 2, в котором, по меньшей мере, один из неорганических солевых катализаторов представляет собой оксид кальция.6. The method according to claim 1 or 2, in which at least one of the inorganic salt catalysts is calcium oxide. 7. Способ по п.1 или 2, в котором, по меньшей мере, один из неорганических солевых катализаторов представляет собой оксид магния.7. The method according to claim 1 or 2, in which at least one of the inorganic salt catalysts is magnesium oxide. 8. Способ по п.7, в котором степень превращения сырья в газообразные и жидкие углеводороды составляет не более чем 20%.8. The method according to claim 7, in which the degree of conversion of raw materials into gaseous and liquid hydrocarbons is not more than 20%. 9. Способ по п.1 или 2, в котором, по меньшей мере, один из неорганических солевых катализаторов представляет собой смесь одного или нескольких карбонатов щелочных металлов.9. The method according to claim 1 or 2, in which at least one of the inorganic salt catalysts is a mixture of one or more alkali metal carbonates. 10. Способ по п.1 или 2, в котором, по меньшей мере, один из неорганических солевых катализаторов представляет собой смесь одного или нескольких карбонатов щелочных металлов и одного или нескольких оксидов щелочноземельных металлов.10. The method according to claim 1 or 2, in which at least one of the inorganic salt catalysts is a mixture of one or more alkali metal carbonates and one or more alkaline earth metal oxides. 11. Способ по п.1, в котором, по меньшей мере, один из неорганических солевых катализаторов является нанесенным, причем носитель включает известняк, углерод, кокс, нелетучий древесный уголь, активированный углерод, зольную пыль, доломит, глину, TiO2 ZrO2, алюмосиликат, отработанный катализатор гидрогенизационной переработки, металлы и/или соединения металлов, извлеченные из смеси суммарный продукт/сырье, один или несколько металлов из групп 5-10 Периодической таблицы элементов, одно или несколько соединений одного или нескольких металлов из групп 5-10 Периодической таблицы элементов, или их сочетания.11. The method according to claim 1, in which at least one of the inorganic salt catalysts is deposited, and the carrier includes limestone, carbon, coke, non-volatile charcoal, activated carbon, fly ash, dolomite, clay, TiO 2 ZrO 2 , aluminosilicate, spent catalyst for hydrogenation processing, metals and / or metal compounds extracted from the mixture total product / raw materials, one or more metals from groups 5-10 of the Periodic table of elements, one or more compounds of one or more metals from pp 5-10 of the Periodic table of the elements, or combinations thereof. 12. Способ по п.1 или 2, дополнительно включающий варьирование весового отношения водяного пара к сырью с целью изменения соотношения монооксида углерода к диоксиду углерода.12. The method according to claim 1 or 2, further comprising varying the weight ratio of water vapor to raw materials in order to change the ratio of carbon monoxide to carbon dioxide. 13. Способ по п.1 или 2, дополнительно включающий варьирование весового отношения водяного пара к сырью с целью изменения соотношения газообразных углеводородов к неочищенному продукту.13. The method according to claim 1 or 2, further comprising varying the weight ratio of water vapor to raw materials in order to change the ratio of gaseous hydrocarbons to the crude product. 14. Способ по п.1 или 2, дополнительно включающий варьирование скорости потока водяного пара, чтобы изменить соотношение газообразных углеводородов к неочищенному продукту.14. The method according to claim 1 or 2, further comprising varying the flow rate of water vapor to change the ratio of gaseous hydrocarbons to the crude product. 15. Способ по п.1 или 2, дополнительно включающий варьирование скорости потока водяного пара и скорости потока сырья, чтобы изменить соотношение газообразных углеводородов к неочищенному продукту. 15. The method according to claim 1 or 2, further comprising varying the flow rate of water vapor and the flow rate of the feed to change the ratio of gaseous hydrocarbons to the crude product.
RU2009101923/04A 2006-06-22 2007-06-20 METHODS FOR PRODUCING A TOTAL PRODUCT WITH SELECTIVE PRODUCTION OF HYDROCARBONS RU2009101923A (en)

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