PL399B1 - Platinum anode for the production of liquors or solids containing active oxygen - Google Patents

Platinum anode for the production of liquors or solids containing active oxygen Download PDF

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Publication number
PL399B1
PL399B1 PL399A PL39920A PL399B1 PL 399 B1 PL399 B1 PL 399B1 PL 399 A PL399 A PL 399A PL 39920 A PL39920 A PL 39920A PL 399 B1 PL399 B1 PL 399B1
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PL
Poland
Prior art keywords
active oxygen
production
containing active
liquors
solids containing
Prior art date
Application number
PL399A
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Polish (pl)
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Publication date
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Publication of PL399B1 publication Critical patent/PL399B1/en

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Przy elektrolizie pewnych roztworów wytwarza sie czynny tlen na anodzie.Tak np. przy uzyciu roztworów weglanu alkalicznego powstaje na anodzie nad¬ weglan, który pozostaje rozpuszczony.Gdy oprócz weglanu alkalicznego doda¬ ny jest jeszcze boran alkaliczny, to two¬ rzy sie wtórny nadboran, który w pew¬ nych warunkach wydziela sie jako cia¬ lo stale.Jako materjal anodowy proponowano przy tym sposobie platyne, jednak z po¬ wodu jej drozyzny i rzadkosci trzeba by¬ lo mozliwie zmniejszyc ciezar anod, t. zn. zastosowac cienkie blaszki lub siatki.Trudnosci, na jakie natrafia umocowanie blaszek lub siatek, sa nadzwyczaj wielkie, poniewaz nalezy uwzglednic mala odleg¬ losc anody od katody, w celu dobrego wyzyskania elektrycznej energji, oraz wielka gestosc pradu, w celu dobrego wyzyskania kosztownej platyny. Nie mozna dlatego celu, jak równiez dla do¬ prowadzania pradu uzywac litej platyny, albowiem urzadzenia bylyby za drogie, wskutek czego zastosowanie blaszek i sia¬ tek nie przyniosloby korzysci.Robiono rozmaite próby w celu usu¬ niecia tych trudnosci.Jednak nie mozna bylo znalezc tech¬ nicznie dobrego rozwiazania tego zada¬ nia. Tak, naprzyklad, próby spawania platyny i glinu, robione na wielka skale, wykazaly, ze miejsca ich zlaczenia ui¬ szczone sa zwolna przez elektrolity, do czego dochodzi jeszcze dzialanie ogni-wowe.platyny i glinu. Wobec tego na¬ stepuje nietylko zluznienie styku, lecz powstaja takze straty wskutek Wykrusza¬ nia sie platyny, tak, ze w ten sposób sporzadzone elektrody sa niezdatne do stalego uzytku technicznego.Obecnie stwierdzono, ze mozna roz¬ wiazac to zadanie z technicznie dobrym skutkiem, a tem samem, ze mozna wy¬ twarzac technicznie roztwory i ciala, za¬ wierajace cz)mny tlen, jezeli zastapic glin cynkiem. Przytem nie jest koniecz¬ ne spawanie platyny z metalem usztyw¬ niajacym i doprowadzajacym prad, co bylo nieodzownem przy glinie, albowiem juz po krótkim czasie, wskutek biernosci glinu, nastapiloby przerwanie pradu.Wystarczy raczej wcisnac platyne w po¬ staci siatek lub blaszek pomiedzy ramy lub sztaby z metalu usztywniajacego, azeby otrzymac trwale jednakowy styk. Rów¬ niez nie mozna bylo przewidziec, ze przy znanej wlasnosci cynku stawania sie takze biernym, nie nastapi przerwa¬ nie pradu. Z jakich powodów nie wy¬ stepuje ta biernosc cynku jest dotych¬ czas jeszcze nie wytlumaczone.Korzysci tego nowego sposobu ano¬ dowego wytwarzania roztworów lub cial, zawierajacych czynny tlen, polegaja prze- dewszystkiem na tem, ze zastosowanie tak sporzadzonych anod umozliwia rze¬ czywiscie nieprzerwalny ruch, i ze w elek¬ trolitach nie moga powstac takie ciala, któreby dzialaly katalitycznie rozkladaja- co na czynny tlen. Pominawszy to, i samo sporzadzanie i montowanie tych anod jest równiez latwiejsze, albowiem spawanie jest zbyteczne, a tem samem unika sie wszystkich z tem zwiazanych czynnosci i niedogodnosci. Dalej przez proste dopiecie zluznionych siatek lub blaszek mozna je znowu wyprezyc, co przy sztywnem polaczeniu wskutek spawania natrafia na trudnosci i powoduje wieksze przerwy ruchu, skutkiem czego caly pro¬ ces wypada niepomyslnie.Wytwarzanie roztworów nadboranu alkalicznego lub nadweglanu it.d., da sie przeprowadzic przy pomocy tych anod we wskazany sposób w trwalym ruchu bez wzrastania napiecia. PLIn the electrolysis of certain solutions, active oxygen is produced at the anode. For example, with alkaline carbonate solutions, percarbonate is formed at the anode, which remains dissolved. When alkaline borate is added in addition to alkali carbonate, secondary perborate is formed. which under certain conditions is released as a solid. Platinum has been proposed as an anode material in this process, but due to its expensive and rarity, it was possible to reduce the weight of the anodes, i.e. Use thin lamellae or meshes. The difficulties faced by the attachment of the lamellae or meshes are extremely great, because the small distance from the anode to the cathode must be taken into account for good electrical energy recovery, and a high current density in order to exploit the expensive platinum well. It is therefore impossible to use solid platinum for the purpose and also for the electric connection, since the equipment would be too expensive and the use of lamellae and mesh would not be of benefit. Various attempts were made to remedy these difficulties. However, no one could find a technically good solution to this task. Thus, for example, large-scale trials of platinum and aluminum welding have shown that their junctions are slowly cleared by electrolytes, in addition to the fusing action of platinum and aluminum. Thus, not only the contact loosening occurs, but also losses due to chipping of the platinum, so that the electrodes prepared in this way are incapable of permanent technical use. It has now been found that this task can be solved with technically good results, and at the same time that it is possible to produce technically solutions and bodies, containing some oxygen, if the aluminum is replaced with zinc. Moreover, it is not necessary to weld platinum with the metal that provides the stiffening and current, which was indispensable for clay, because after a short time, due to the passivity of aluminum, the current would be interrupted. Rather, it is enough to press the platinum in the form of nets or plates between the frames. or bars of stiffening metal in order to obtain a permanently uniform contact. It was also impossible to predict that, given the known property of zinc, by becoming also passive, the current would not be interrupted. For what reasons this passivity of zinc does not work, it has yet to be explained. The advantages of this new method of anodic preparation of solutions or bodies containing active oxygen consist mainly in the fact that the use of anodes prepared in this way makes it possible uninterrupted movement, and that no body can be formed in the electrolytes that would act catalytically to decompose active oxygen. Aside from this, the fabrication and assembly of these anodes is also easier, as welding is unnecessary and thus avoids all the associated steps and inconvenience. Then, by simply tightening the loosened meshes or lamellae, they can be distorted again, which in the case of a rigid connection due to welding causes difficulties and causes greater breaks in motion, as a result of which the whole process is unsuccessful. carry out with these anodes as indicated in a permanent motion without increasing the voltage. PL

Claims (1)

1. Zastrzezenie patentów e. '" Anoda platynowa do wytwarzania lu¬ gów i cial stalych, zawierajacych czynny tlen, tem znamienna, ze jako metal do¬ prowadzajacy prad i usztywniajacy uzyty jest cynk. ZAkl 6KAF.KDZIAHSKICH W WARSZAWIL PL1. Patents are reserved e. '"Platinum anode for the production of chunks and solids containing active oxygen, characterized by the fact that zinc is used as the metal for supplying electricity and stiffening. ZAkl 6KAF.KDZIAHSKI W WARSZAWIL PL
PL399A 1920-06-23 Platinum anode for the production of liquors or solids containing active oxygen PL399B1 (en)

Publications (1)

Publication Number Publication Date
PL399B1 true PL399B1 (en) 1924-07-30

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