PL11040B1 - Improvements in the method of obtaining synthetic ammonia. - Google Patents

Improvements in the method of obtaining synthetic ammonia. Download PDF

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Publication number
PL11040B1
PL11040B1 PL11040A PL1104028A PL11040B1 PL 11040 B1 PL11040 B1 PL 11040B1 PL 11040 A PL11040 A PL 11040A PL 1104028 A PL1104028 A PL 1104028A PL 11040 B1 PL11040 B1 PL 11040B1
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PL
Poland
Prior art keywords
gases
carbon dioxide
circulating
converter
nitrogen
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Application number
PL11040A
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Polish (pl)
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Publication date
Application filed filed Critical
Publication of PL11040B1 publication Critical patent/PL11040B1/en

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Description

Wynalazek niniejszy dotyczy synte¬ tycznego otrzymywania amonjaku z mie¬ szanin azotu z wodorem, krazacym pod cisnieniem w przetwornicy; w szczególno¬ sci zas przedmiotem wynalazku jest oczy¬ szczanie mieszanin wodoru i azotu przy wyrobie amonjaku bezwodnego. Zwykle krazace gazy po sprezeniu zawieraja je¬ szcze oprócz innych zanieczyszczen rów¬ niez i pewna ilosc pary wodnej, która dziala szkodliwie na katalizator, uzyty w przetwornicy, a przy wytwarzaniu amo¬ njaku bezwodnego wplywa ujemnie na produkt koncowy. Pod cisnieniem, prze¬ wyzszaj acem 100 atm, ilosc tej pary wod¬ nej jest oczywiscie bardzo mala, poniewaz jest ona w równowadze z krazacemi gaza¬ mi, lecz pomimo to bardzo waznem jest jej usuniecie, wykonywa sie je przewaznie zapomoca oziebiania krazacej mieszaniny, przeplókiwaniem jej bezwodnym amonja- kiem lub zapomoca innych metod.Z innych zanieczyszczen, dzialajacych szkodliwie na katalizator, nalezy wymienic dwutlenek wegla, dlatego tez swieze gazy, doprowadzane do mieszaniny, w celu za¬ stapienia utworzonego amonjaku uwalnia sie mozliwie dokladnie od dwutlenku we¬ gla, przemywajac je soda zraca albo tez stosujac w tym celu inne sposoby.Natomiast podlug niniejszego wyna¬ lazku wprowadza sie do krazacych gazów niewielkie ilosci dwutlenku wegla, przy- czem stwierdzono, ze dwutlenek weglareaguje z para wodna i z obecnym amo- njakieijp, tworzac *staly4weglan amonu we- dluf ró^ftaniaf" * * 2 NH3+C02+H20=(NHJ2 CO^ Wytworzony staly weglan amonowy mozna nastepnie usunac z krazacych ga¬ zów, przyczem jednoczesnie zabiera on ze soba inne zanieczyszczenia, jak czastki smarów i kurzu.Dwutlenek wegla najlepiej doprowa¬ dzac ze swiezemi albo dopelniajacemi ga¬ zami w odpowiednich ilosciach, po spreze¬ niu gazów ale jeszcze przed ich wejsciem do przetwornicy. Ilosc majacego byc do¬ prowadzonym dwutlenku wegla wylicza sie dokladnie odpowiednio do ilosci obecnej wody. Np. gazy pod cisnieniem 100 atm, nasycone para wodna przy 20°C, zawiera¬ ja 1 czesc objetosciowa wilgoci na 30 ty¬ siecy czesci gazu. A zatem, na kazde 30 ty¬ siecy czesci krazacego gazu wprowadza sie ze swiezemi gazami jedna czesc dwu¬ tlenku wegla, poniewaz, jak widac z po¬ wyzszego równania, do wytworzenia sta¬ lego weglanu amonowego niezbedne sa równe objetosci wody i dwutlenku, przy¬ czem w zadnym razie dwutlenek wegla nie powinien przekraczac polowy objeto¬ sci amonjaku w gazach, wchodzacych do przetwornicy.Aby uniknac zatykania rur przez wy¬ tworzony staly weglan amonowy, celowem jest zastosowanie komory lub podobnego rozszerzenia w systemie krazenia, w punk¬ cie, lezacym za wlotem gazów swiezych czyli dopelniajacych ale przed wlotem do przetwornicy. Komore te mozna napelnic pierscieniami Raschiga albo innym mate- rjalem, zatrzymujacym lub filtrujacym, któryby zatrzymywal zanieczyszczenia stale lub ciekle, nie tamujac przeplywu gazów. Stwierdzono dalej, ze osadzajace sie materjaly stale porywaja ze soba inne zanieczyszczenia stale albo ciekle, zawar¬ te w krazacych gazach. Dobrze jest zasto¬ sowac równolegle dwie takie komory albo rozszerzenia, aby umozliwic oczyszczanie jednej z nich podczas pracy drugiej. PLThe present invention relates to the synthetic preparation of ammonia from mixtures of nitrogen and hydrogen circulating under pressure in a converter; in particular, the invention relates to the purification of hydrogen and nitrogen mixtures for the production of anhydrous ammonia. Usually, the circulating gases after compression contain, apart from other impurities, also a certain amount of water vapor which is detrimental to the catalyst used in the converter and, in the production of anhydrous ammonia, negatively affects the final product. Under a pressure, exceeding 100 atm, the amount of this water vapor is of course very small, because it is in equilibrium with the circulating gases, but nevertheless it is very important to remove it, they are usually performed without cooling the circulating mixture, flushing it with anhydrous ammonia or using other methods. Other pollutants, detrimental to the catalyst, should be replaced with carbon dioxide, therefore fresh gases, fed to the mixture, in order to melt the formed ammonia, are as much as possible released from carbon dioxide by washing them with soda, or by using other methods for this purpose, while the present invention introduces small amounts of carbon dioxide into the circulating gases, and it has been found that the carbon dioxide reacts with water vapor and with the ammonia present, forming a solid carbonate of ammonium in the mixture of ammonium chloride * * 2 NH3 + CO 2 + H 2 O = (NHJ 2 CO 3). At the same time, it also collects other contaminants with it, such as particles of grease and dust. Carbon dioxide is best supplied with fresh or complementary gases in appropriate amounts, after the gases have been compressed but before they enter the converter. The amount of carbon dioxide to be fed is calculated exactly according to the amount of water present. For example, gases under a pressure of 100 atm, saturated with water vapor at 20 ° C, contain 1 part by volume of moisture per 30 thousand parts of gas. Thus, for every 30 thousand parts of circulating gas, one part of carbon dioxide is introduced with fresh gases, since, as can be seen from the equation above, equal volumes of water and dioxide are needed to produce solid ammonium carbonate, with fresh gases. However, in no case should the carbon dioxide exceed half the volume of the ammonia in the gases entering the converter. To avoid clogging of the pipes by the solid ammonium carbonate produced, it is advisable to use a chamber or similar extension in the circulation system at the point where the lying behind the inlet of fresh gases, i.e. complementary gases, but before the inlet to the converter. These chambers could be filled with Raschig rings or other retaining or filtering material that would trap solid or liquid contaminants without obstructing the flow of gases. It was further found that the depositing materials continually entrain other solid or liquid contaminants contained in the circulating gases. It is advantageous to use two such chambers or extensions in parallel to allow one of them to be purged while the other is in operation. PL

Claims (4)

Zastrzezenia patentowe. 1. Sposób otrzymywania amon jaku z mieszaniny azotu z wodorem, krazacej pod cisnieniem w przetwornicy, znamienny tern, ze do krazacych gazów wprowadza sie male ilosci dwutlenku wegla w celu wytworzenia stalego weglanu amonowego, który wraz z innemi zanieczyszczeniami u- suwa sie z tych gazów przed ich wejsciem do przetwornicy.Patent claims. 1. The method of obtaining ammonium yak from a mixture of nitrogen and hydrogen, circulating under pressure in a converter, characterized by the fact that small amounts of carbon dioxide are introduced into the circulating gases in order to produce solid ammonium carbonate which, along with other impurities, is used from these gases before they enter the inverter. 2. Sposób wedlug zastrz. 1, znamien¬ ny tern, ze dwutlenek wegla doprowadza sie z gazami swiezemi lub dopelniajacemi w okreslonych zgóry ilosciach do gazów krazacych po ich sprezeniu ale przed wej¬ sciem do przetwornicy.2. The method according to claim The characteristic of claim 1 is that the carbon dioxide is fed with fresh or complementary gases in predetermined amounts to the circulating gases after they have been compressed but before they enter the converter. 3. Sposób wedlug zastrz. 1 i 2, zna¬ mienny tern, ze krazace gazy po dodaniu do nich dwutlenku wegla, przeprowadza sie przez komore albo podobne rozszerze¬ nie systemu krazenia, w której to komorze usuwa sie staly weglan amonowy bez ta¬ mowania przeplywu gazów.3. The method according to p. 1 and 2, the significant point in which the circulating gases, upon addition of carbon dioxide thereto, are passed through a chamber or similar expansion of the circulatory system in which the solid ammonium carbonate is removed without obstructing the flow of gases. 4. Sposób wedlug zastrz. 3, znamien¬ ny tern, ze stosuje sie dwie równolegle ko¬ mory, z których jedna mozna oczyszczac podczas pracy drugiej. Nitrogen Engineering Corporati on. Zastepca: M. Brokman, rzecznik patentowy. Druk L. Boguslawskiego, Warszawa. PL4. The method according to p. 3, the characteristic of using two chambers in parallel, one of which can be cleaned while the other is in operation. Nitrogen Engineering Corporati on. Deputy: M. Brokman, patent attorney. Print by L. Boguslawski, Warsaw. PL
PL11040A 1928-04-02 Improvements in the method of obtaining synthetic ammonia. PL11040B1 (en)

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PL11040B1 true PL11040B1 (en) 1929-10-31

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