LV15540A -
Method for the determination of pharmaceutical compounds in untreated and treated effluents by high-resolution mass spectrometry
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Method for the determination of pharmaceutical compounds in untreated and treated effluents by high-resolution mass spectrometry
Pārtikas Drošības, Dzīvnieku Veselības Un Vides Zinātniskais Institūts 'bior'
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Other Investigation Or Analysis Of Materials By Electrical Means
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Abstract
Izgudrojums attiecas uz analītisko ķīmiju, konkrēti uz vides piesārņojuma noteikšanas metodēm, un var tikt izmantots selektīvai divdesmit astoņu farmaceitisko savienojumu kvantitatīvā satura noteikšanai, kā arī farmaceitisko savienojumu sastopamāko metabolītu (<200 savienojumi) kvalitatīvai identificēšanai neattīrītos un attīrītos municipālajos netekūdeņos, pielietojot augstefektīvo šķidruma hromatogrāfiju pozitīvas un negatīvas jonizācijas režīmā, kombinētu ar ultra augstas izšķirtspējas Furjē transformāciju jonu ciklotrona rezonanses masspektrometrijas detektoru pilno masspektru detektēšanas režīmā. Paraugu sagatavošanu veic ar dispersīvo metodi, ekstrakcijai lietojot ūdens un acetonitrila maisījumu (tilpuma attiecība 50:50) un magnija sulfāta/nātrija hlorīda maisījumu (attiecība 4:1), bet ekstrakta tālākai apstrādei lietojot acetonu un paraugu rekonstruēšanu analīzei veicot ūdens/metanola maisījumā (tilpumattiecība 8:2) ar 0,1% skudrskābi. Paņēmiens nodrošina ātru un efektīvu paraugu sagatavošanu gan bāzisku, gan skābu savienojumu analīzei, pielietojot instrumentālo metodi ar uzlabotu jutību un precizitāti tiešai farmaceitisko vielu noteikšanai un rektrospektīvam zāļu atliekvielu skrīningam notekūdeņu paraugos.The invention relates to analytical chemistry, in particular to methods for the determination of environmental contamination, and can be used for the selective quantification of twenty-eight pharmaceutical compounds and for the qualitative identification of the most common metabolites of pharmaceutical compounds (<200 compounds) in untreated and purified municipal wastewater. and a negative ionization mode combined with an ultra high resolution Fourier transform ion cyclotron resonance mass spectrometry detector in full mass detection mode. Samples are prepared by the dispersive method, using a mixture of water and acetonitrile (50:50 by volume) and a mixture of magnesium sulphate / sodium chloride (4: 1 by volume) for extraction, and further processing of the extract using acetone and reconstruction of the samples in water / methanol for analysis ( volume ratio 8: 2) with 0.1% formic acid. The method provides fast and efficient sample preparation for the analysis of both basic and acidic compounds, using an instrumental method with improved sensitivity and accuracy for direct detection of pharmaceutical substances and spectroscopic screening of drug residues in wastewater samples.
LVP-19-29A2019-05-302019-05-30
Method for the determination of pharmaceutical compounds in untreated and treated effluents by high-resolution mass spectrometry
LV15540A
(en)
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