KR20230038704A - 활성 화합물 조합물 - Google Patents
활성 화합물 조합물 Download PDFInfo
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- KR20230038704A KR20230038704A KR1020237001394A KR20237001394A KR20230038704A KR 20230038704 A KR20230038704 A KR 20230038704A KR 1020237001394 A KR1020237001394 A KR 1020237001394A KR 20237001394 A KR20237001394 A KR 20237001394A KR 20230038704 A KR20230038704 A KR 20230038704A
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- South Korea
- Prior art keywords
- aromatic
- methyl
- alkyl
- phenyl
- group
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- 150000001875 compounds Chemical class 0.000 title claims abstract description 401
- 239000000203 mixture Substances 0.000 claims abstract description 81
- 239000000417 fungicide Substances 0.000 claims abstract description 22
- 230000000855 fungicidal effect Effects 0.000 claims abstract description 14
- 241000233866 Fungi Species 0.000 claims abstract description 9
- 230000003032 phytopathogenic effect Effects 0.000 claims abstract description 4
- 125000003118 aryl group Chemical group 0.000 claims description 376
- -1 cyano, hydroxyl Chemical group 0.000 claims description 376
- 125000001424 substituent group Chemical group 0.000 claims description 291
- 125000004122 cyclic group Chemical group 0.000 claims description 171
- SNOOUWRIMMFWNE-UHFFFAOYSA-M sodium;6-[(3,4,5-trimethoxybenzoyl)amino]hexanoate Chemical compound [Na+].COC1=CC(C(=O)NCCCCCC([O-])=O)=CC(OC)=C1OC SNOOUWRIMMFWNE-UHFFFAOYSA-M 0.000 claims description 159
- 238000000034 method Methods 0.000 claims description 135
- 125000000623 heterocyclic group Chemical group 0.000 claims description 111
- 239000001257 hydrogen Substances 0.000 claims description 101
- 229910052739 hydrogen Inorganic materials 0.000 claims description 101
- 125000006552 (C3-C8) cycloalkyl group Chemical group 0.000 claims description 96
- 125000002911 monocyclic heterocycle group Chemical group 0.000 claims description 95
- 150000002431 hydrogen Chemical group 0.000 claims description 73
- 125000001931 aliphatic group Chemical group 0.000 claims description 72
- 229910052736 halogen Inorganic materials 0.000 claims description 70
- 150000002367 halogens Chemical class 0.000 claims description 70
- 125000002887 hydroxy group Chemical group [H]O* 0.000 claims description 67
- 125000000171 (C1-C6) haloalkyl group Chemical group 0.000 claims description 62
- 125000005913 (C3-C6) cycloalkyl group Chemical group 0.000 claims description 59
- 239000003112 inhibitor Substances 0.000 claims description 55
- 125000000882 C2-C6 alkenyl group Chemical group 0.000 claims description 53
- 125000001997 phenyl group Chemical group [H]C1=C([H])C([H])=C(*)C([H])=C1[H] 0.000 claims description 49
- 125000004765 (C1-C4) haloalkyl group Chemical group 0.000 claims description 46
- 125000004737 (C1-C6) haloalkoxy group Chemical group 0.000 claims description 44
- 229910052799 carbon Inorganic materials 0.000 claims description 44
- 125000002496 methyl group Chemical group [H]C([H])([H])* 0.000 claims description 41
- 150000003839 salts Chemical class 0.000 claims description 40
- 125000004432 carbon atom Chemical group C* 0.000 claims description 37
- 125000004767 (C1-C4) haloalkoxy group Chemical group 0.000 claims description 36
- 235000014113 dietary fatty acids Nutrition 0.000 claims description 36
- 239000000194 fatty acid Substances 0.000 claims description 36
- 229930195729 fatty acid Natural products 0.000 claims description 36
- 150000004665 fatty acids Chemical class 0.000 claims description 36
- 229910003849 O-Si Inorganic materials 0.000 claims description 35
- 229910003872 O—Si Inorganic materials 0.000 claims description 35
- 244000063299 Bacillus subtilis Species 0.000 claims description 33
- 235000014469 Bacillus subtilis Nutrition 0.000 claims description 33
- 125000003601 C2-C6 alkynyl group Chemical group 0.000 claims description 32
- 125000004093 cyano group Chemical group *C#N 0.000 claims description 32
- 125000006656 (C2-C4) alkenyl group Chemical group 0.000 claims description 29
- 239000011737 fluorine Substances 0.000 claims description 29
- 229910052731 fluorine Inorganic materials 0.000 claims description 29
- 125000006643 (C2-C6) haloalkenyl group Chemical group 0.000 claims description 28
- 125000005844 heterocyclyloxy group Chemical group 0.000 claims description 28
- 125000004043 oxo group Chemical group O=* 0.000 claims description 28
- 125000004454 (C1-C6) alkoxycarbonyl group Chemical group 0.000 claims description 27
- 239000003795 chemical substances by application Substances 0.000 claims description 27
- 125000000325 methylidene group Chemical group [H]C([H])=* 0.000 claims description 27
- XTDZGXBTXBEZDN-UHFFFAOYSA-N 3-(difluoromethyl)-N-(9-isopropyl-1,2,3,4-tetrahydro-1,4-methanonaphthalen-5-yl)-1-methylpyrazole-4-carboxamide Chemical compound CC(C)C1C2CCC1C1=C2C=CC=C1NC(=O)C1=CN(C)N=C1C(F)F XTDZGXBTXBEZDN-UHFFFAOYSA-N 0.000 claims description 26
- 239000005799 Isopyrazam Substances 0.000 claims description 26
- 125000003178 carboxy group Chemical group [H]OC(*)=O 0.000 claims description 24
- 239000000460 chlorine Substances 0.000 claims description 24
- 229910052801 chlorine Inorganic materials 0.000 claims description 24
- 229920006395 saturated elastomer Polymers 0.000 claims description 24
- 125000002485 formyl group Chemical group [H]C(*)=O 0.000 claims description 23
- ZAMOUSCENKQFHK-UHFFFAOYSA-N Chlorine atom Chemical compound [Cl] ZAMOUSCENKQFHK-UHFFFAOYSA-N 0.000 claims description 22
- PXGOKWXKJXAPGV-UHFFFAOYSA-N Fluorine Chemical compound FF PXGOKWXKJXAPGV-UHFFFAOYSA-N 0.000 claims description 22
- 125000004435 hydrogen atom Chemical group [H]* 0.000 claims description 22
- 125000004738 (C1-C6) alkyl sulfinyl group Chemical group 0.000 claims description 21
- 125000002950 monocyclic group Chemical group 0.000 claims description 21
- 125000004739 (C1-C6) alkylsulfonyl group Chemical group 0.000 claims description 20
- 229910052717 sulfur Inorganic materials 0.000 claims description 20
- UFHFLCQGNIYNRP-UHFFFAOYSA-N Hydrogen Chemical compound [H][H] UFHFLCQGNIYNRP-UHFFFAOYSA-N 0.000 claims description 19
- 125000006650 (C2-C4) alkynyl group Chemical group 0.000 claims description 18
- 125000004916 (C1-C6) alkylcarbonyl group Chemical group 0.000 claims description 17
- 125000004740 (C1-C6) haloalkylsulfanyl group Chemical group 0.000 claims description 17
- 125000001624 naphthyl group Chemical group 0.000 claims description 17
- 229910052760 oxygen Inorganic materials 0.000 claims description 17
- 241000194103 Bacillus pumilus Species 0.000 claims description 16
- 125000004269 oxiran-2-yl group Chemical group [H]C1([H])OC1([H])* 0.000 claims description 16
- 125000006765 (C2-C6) haloalkenyloxy group Chemical group 0.000 claims description 14
- 125000003320 C2-C6 alkenyloxy group Chemical group 0.000 claims description 14
- 239000002253 acid Substances 0.000 claims description 14
- XRECTZIEBJDKEO-UHFFFAOYSA-N flucytosine Chemical compound NC1=NC(=O)NC=C1F XRECTZIEBJDKEO-UHFFFAOYSA-N 0.000 claims description 14
- 125000004076 pyridyl group Chemical group 0.000 claims description 14
- 125000004749 (C1-C6) haloalkylsulfinyl group Chemical group 0.000 claims description 13
- 125000004741 (C1-C6) haloalkylsulfonyl group Chemical group 0.000 claims description 13
- 150000002148 esters Chemical class 0.000 claims description 13
- 238000003786 synthesis reaction Methods 0.000 claims description 13
- 241000592795 Paenibacillus sp. Species 0.000 claims description 12
- NINIDFKCEFEMDL-UHFFFAOYSA-N Sulfur Chemical compound [S] NINIDFKCEFEMDL-UHFFFAOYSA-N 0.000 claims description 12
- ZQEIXNIJLIKNTD-GFCCVEGCSA-N metalaxyl-M Chemical compound COCC(=O)N([C@H](C)C(=O)OC)C1=C(C)C=CC=C1C ZQEIXNIJLIKNTD-GFCCVEGCSA-N 0.000 claims description 12
- 125000002924 primary amino group Chemical group [H]N([H])* 0.000 claims description 12
- 239000011593 sulfur Substances 0.000 claims description 12
- JERZEQUMJNCPRJ-UHFFFAOYSA-N 2-[4-(4-chlorophenoxy)-2-(trifluoromethyl)phenyl]-1-(1H-1,2,4-triazol-1-yl)propan-2-ol Chemical compound C=1C=C(OC=2C=CC(Cl)=CC=2)C=C(C(F)(F)F)C=1C(O)(C)CN1C=NC=N1 JERZEQUMJNCPRJ-UHFFFAOYSA-N 0.000 claims description 11
- 239000000575 pesticide Substances 0.000 claims description 11
- 125000004770 (C1-C4) haloalkylsulfanyl group Chemical group 0.000 claims description 10
- 125000003161 (C1-C6) alkylene group Chemical group 0.000 claims description 10
- 125000006577 C1-C6 hydroxyalkyl group Chemical group 0.000 claims description 10
- OIPMQULDKWSNGX-UHFFFAOYSA-N bis[[ethoxy(oxo)phosphaniumyl]oxy]alumanyloxy-ethoxy-oxophosphanium Chemical compound [Al+3].CCO[P+]([O-])=O.CCO[P+]([O-])=O.CCO[P+]([O-])=O OIPMQULDKWSNGX-UHFFFAOYSA-N 0.000 claims description 10
- 125000003566 oxetanyl group Chemical group 0.000 claims description 10
- 230000035806 respiratory chain Effects 0.000 claims description 10
- 125000003396 thiol group Chemical class [H]S* 0.000 claims description 10
- LDVVMCZRFWMZSG-OLQVQODUSA-N (3ar,7as)-2-(trichloromethylsulfanyl)-3a,4,7,7a-tetrahydroisoindole-1,3-dione Chemical compound C1C=CC[C@H]2C(=O)N(SC(Cl)(Cl)Cl)C(=O)[C@H]21 LDVVMCZRFWMZSG-OLQVQODUSA-N 0.000 claims description 9
- 125000006677 (C1-C3) haloalkoxy group Chemical group 0.000 claims description 9
- PXMNMQRDXWABCY-UHFFFAOYSA-N 1-(4-chlorophenyl)-4,4-dimethyl-3-(1H-1,2,4-triazol-1-ylmethyl)pentan-3-ol Chemical compound C1=NC=NN1CC(O)(C(C)(C)C)CCC1=CC=C(Cl)C=C1 PXMNMQRDXWABCY-UHFFFAOYSA-N 0.000 claims description 9
- MNHVNIJQQRJYDH-UHFFFAOYSA-N 2-[2-(1-chlorocyclopropyl)-3-(2-chlorophenyl)-2-hydroxypropyl]-1,2-dihydro-1,2,4-triazole-3-thione Chemical compound N1=CNC(=S)N1CC(C1(Cl)CC1)(O)CC1=CC=CC=C1Cl MNHVNIJQQRJYDH-UHFFFAOYSA-N 0.000 claims description 9
- 241000223678 Aureobasidium pullulans Species 0.000 claims description 9
- 241000193744 Bacillus amyloliquefaciens Species 0.000 claims description 9
- 239000005738 Bixafen Substances 0.000 claims description 9
- 239000005745 Captan Substances 0.000 claims description 9
- 239000005760 Difenoconazole Substances 0.000 claims description 9
- 239000005781 Fludioxonil Substances 0.000 claims description 9
- 239000005783 Fluopyram Substances 0.000 claims description 9
- 239000005789 Folpet Substances 0.000 claims description 9
- 239000005802 Mancozeb Substances 0.000 claims description 9
- SQCJYCIUZGDBPJ-UHFFFAOYSA-N N'-[2-chloro-4-(2-fluorophenoxy)-5-methylphenyl]-N-ethyl-N-methylmethanimidamide Chemical compound ClC1=C(C=C(C(=C1)OC1=C(C=CC=C1)F)C)N=CN(C)CC SQCJYCIUZGDBPJ-UHFFFAOYSA-N 0.000 claims description 9
- 239000005823 Propineb Substances 0.000 claims description 9
- 239000005825 Prothioconazole Substances 0.000 claims description 9
- 239000005828 Pyrimethanil Substances 0.000 claims description 9
- 239000005831 Quinoxyfen Substances 0.000 claims description 9
- 239000005837 Spiroxamine Substances 0.000 claims description 9
- 239000005839 Tebuconazole Substances 0.000 claims description 9
- 239000005857 Trifloxystrobin Substances 0.000 claims description 9
- LDLMOOXUCMHBMZ-UHFFFAOYSA-N bixafen Chemical compound FC(F)C1=NN(C)C=C1C(=O)NC1=CC=C(F)C=C1C1=CC=C(Cl)C(Cl)=C1 LDLMOOXUCMHBMZ-UHFFFAOYSA-N 0.000 claims description 9
- 229940117949 captan Drugs 0.000 claims description 9
- 125000001559 cyclopropyl group Chemical group [H]C1([H])C([H])([H])C1([H])* 0.000 claims description 9
- BQYJATMQXGBDHF-UHFFFAOYSA-N difenoconazole Chemical compound O1C(C)COC1(C=1C(=CC(OC=2C=CC(Cl)=CC=2)=CC=1)Cl)CN1N=CN=C1 BQYJATMQXGBDHF-UHFFFAOYSA-N 0.000 claims description 9
- PYZSVQVRHDXQSL-UHFFFAOYSA-N dithianon Chemical compound S1C(C#N)=C(C#N)SC2=C1C(=O)C1=CC=CC=C1C2=O PYZSVQVRHDXQSL-UHFFFAOYSA-N 0.000 claims description 9
- MUJOIMFVNIBMKC-UHFFFAOYSA-N fludioxonil Chemical compound C=12OC(F)(F)OC2=CC=CC=1C1=CNC=C1C#N MUJOIMFVNIBMKC-UHFFFAOYSA-N 0.000 claims description 9
- KVDJTXBXMWJJEF-UHFFFAOYSA-N fluopyram Chemical compound ClC1=CC(C(F)(F)F)=CN=C1CCNC(=O)C1=CC=CC=C1C(F)(F)F KVDJTXBXMWJJEF-UHFFFAOYSA-N 0.000 claims description 9
- HKIOYBQGHSTUDB-UHFFFAOYSA-N folpet Chemical compound C1=CC=C2C(=O)N(SC(Cl)(Cl)Cl)C(=O)C2=C1 HKIOYBQGHSTUDB-UHFFFAOYSA-N 0.000 claims description 9
- WLPCAERCXQSYLQ-UHFFFAOYSA-N isotianil Chemical compound ClC1=NSC(C(=O)NC=2C(=CC=CC=2)C#N)=C1Cl WLPCAERCXQSYLQ-UHFFFAOYSA-N 0.000 claims description 9
- KKMLIVYBGSAJPM-UHFFFAOYSA-L propineb Chemical compound [Zn+2].[S-]C(=S)NC(C)CNC([S-])=S KKMLIVYBGSAJPM-UHFFFAOYSA-L 0.000 claims description 9
- ZLIBICFPKPWGIZ-UHFFFAOYSA-N pyrimethanil Chemical compound CC1=CC(C)=NC(NC=2C=CC=CC=2)=N1 ZLIBICFPKPWGIZ-UHFFFAOYSA-N 0.000 claims description 9
- WRPIRSINYZBGPK-UHFFFAOYSA-N quinoxyfen Chemical compound C1=CC(F)=CC=C1OC1=CC=NC2=CC(Cl)=CC(Cl)=C12 WRPIRSINYZBGPK-UHFFFAOYSA-N 0.000 claims description 9
- PUYXTUJWRLOUCW-UHFFFAOYSA-N spiroxamine Chemical compound O1C(CN(CC)CCC)COC11CCC(C(C)(C)C)CC1 PUYXTUJWRLOUCW-UHFFFAOYSA-N 0.000 claims description 9
- ONCZDRURRATYFI-TVJDWZFNSA-N trifloxystrobin Chemical compound CO\N=C(\C(=O)OC)C1=CC=CC=C1CO\N=C(/C)C1=CC=CC(C(F)(F)F)=C1 ONCZDRURRATYFI-TVJDWZFNSA-N 0.000 claims description 9
- 125000004769 (C1-C4) alkylsulfonyl group Chemical group 0.000 claims description 8
- PZBPKYOVPCNPJY-UHFFFAOYSA-N 1-[2-(allyloxy)-2-(2,4-dichlorophenyl)ethyl]imidazole Chemical compound ClC1=CC(Cl)=CC=C1C(OCC=C)CN1C=NC=C1 PZBPKYOVPCNPJY-UHFFFAOYSA-N 0.000 claims description 8
- 239000005764 Dithianon Substances 0.000 claims description 8
- ZHNUHDYFZUAESO-UHFFFAOYSA-N Formamide Chemical compound NC=O ZHNUHDYFZUAESO-UHFFFAOYSA-N 0.000 claims description 8
- 229960002125 enilconazole Drugs 0.000 claims description 8
- 125000001495 ethyl group Chemical group [H]C([H])([H])C([H])([H])* 0.000 claims description 8
- 125000003718 tetrahydrofuranyl group Chemical group 0.000 claims description 8
- 125000004768 (C1-C4) alkylsulfinyl group Chemical group 0.000 claims description 7
- ZALZMUXMSIVXKA-UHFFFAOYSA-N 5-fluoro-2-[(4-fluorophenyl)methoxy]pyrimidin-4-amine Chemical compound C1=C(F)C(N)=NC(OCC=2C=CC(F)=CC=2)=N1 ZALZMUXMSIVXKA-UHFFFAOYSA-N 0.000 claims description 7
- KVUHRPLZWABERU-UHFFFAOYSA-N 5-fluoro-4-imino-3-methyl-1-(4-methylphenyl)sulfonylpyrimidin-2-one Chemical compound C1=CC(C)=CC=C1S(=O)(=O)N1C(=O)N(C)C(=N)C(F)=C1 KVUHRPLZWABERU-UHFFFAOYSA-N 0.000 claims description 7
- 125000002853 C1-C4 hydroxyalkyl group Chemical group 0.000 claims description 7
- 125000002915 carbonyl group Chemical group [*:2]C([*:1])=O 0.000 claims description 7
- ACMXQHFNODYQAT-UHFFFAOYSA-N cyflufenamid Chemical compound FC1=CC=C(C(F)(F)F)C(C(NOCC2CC2)=NC(=O)CC=2C=CC=CC=2)=C1F ACMXQHFNODYQAT-UHFFFAOYSA-N 0.000 claims description 7
- 125000001153 fluoro group Chemical group F* 0.000 claims description 7
- YTCIYOXHHQLDEI-SNVBAGLBSA-N inpyrfluxam Chemical compound C([C@H](C=12)C)C(C)(C)C2=CC=CC=1NC(=O)C1=CN(C)N=C1C(F)F YTCIYOXHHQLDEI-SNVBAGLBSA-N 0.000 claims description 7
- 125000003226 pyrazolyl group Chemical group 0.000 claims description 7
- 125000000335 thiazolyl group Chemical group 0.000 claims description 7
- 125000001544 thienyl group Chemical group 0.000 claims description 7
- JLIDBLDQVAYHNE-YKALOCIXSA-N (+)-Abscisic acid Chemical compound OC(=O)/C=C(/C)\C=C\[C@@]1(O)C(C)=CC(=O)CC1(C)C JLIDBLDQVAYHNE-YKALOCIXSA-N 0.000 claims description 6
- 125000004771 (C1-C4) haloalkylsulfinyl group Chemical group 0.000 claims description 6
- 125000006766 (C2-C6) alkynyloxy group Chemical group 0.000 claims description 6
- 125000006767 (C2-C6) haloalkynyloxy group Chemical group 0.000 claims description 6
- KRDJWAGXHSLJIL-UHFFFAOYSA-N 1-methoxy-3-methyl-1-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]urea Chemical compound CON(C(=O)NC)CC1=CC=C(C=C1)C1=NOC(=N1)C(F)(F)F KRDJWAGXHSLJIL-UHFFFAOYSA-N 0.000 claims description 6
- PFFIDZXUXFLSSR-UHFFFAOYSA-N 1-methyl-N-[2-(4-methylpentan-2-yl)-3-thienyl]-3-(trifluoromethyl)pyrazole-4-carboxamide Chemical compound S1C=CC(NC(=O)C=2C(=NN(C)C=2)C(F)(F)F)=C1C(C)CC(C)C PFFIDZXUXFLSSR-UHFFFAOYSA-N 0.000 claims description 6
- NIOPZPCMRQGZCE-WEVVVXLNSA-N 2,4-dinitro-6-(octan-2-yl)phenyl (E)-but-2-enoate Chemical compound CCCCCCC(C)C1=CC([N+]([O-])=O)=CC([N+]([O-])=O)=C1OC(=O)\C=C\C NIOPZPCMRQGZCE-WEVVVXLNSA-N 0.000 claims description 6
- SPXBEYPYQKZKGX-UHFFFAOYSA-N 2-(chloromethyl)-5-[(4-chlorophenyl)methyl]-2-methyl-1-(1,2,4-triazol-1-ylmethyl)cyclopentan-1-ol Chemical compound C1=NC=NN1CC1(O)C(C)(CCl)CCC1CC1=CC=C(Cl)C=C1 SPXBEYPYQKZKGX-UHFFFAOYSA-N 0.000 claims description 6
- PDPWCKVFIFAQIQ-UHFFFAOYSA-N 2-{2-[(2,5-dimethylphenoxy)methyl]phenyl}-2-methoxy-N-methylacetamide Chemical compound CNC(=O)C(OC)C1=CC=CC=C1COC1=CC(C)=CC=C1C PDPWCKVFIFAQIQ-UHFFFAOYSA-N 0.000 claims description 6
- XCGBHLLWJZOLEM-UHFFFAOYSA-N 3-(difluoromethyl)-N-(7-fluoro-1,1,3-trimethyl-2,3-dihydro-1H-inden-4-yl)-1-methyl-1H-pyrazole-4-carboxamide Chemical compound CC1CC(C)(C)C(C(=CC=2)F)=C1C=2NC(=O)C1=CN(C)N=C1C(F)F XCGBHLLWJZOLEM-UHFFFAOYSA-N 0.000 claims description 6
- ODJRGOYSTVDWMP-UHFFFAOYSA-N 4-(2-bromo-4-fluorophenyl)-n-(2,6-difluorophenyl)-2,5-dimethylpyrazol-3-amine Chemical compound C=1C=C(F)C=C(Br)C=1C=1C(C)=NN(C)C=1NC1=C(F)C=CC=C1F ODJRGOYSTVDWMP-UHFFFAOYSA-N 0.000 claims description 6
- LBGMYUQCXJJLIR-UHFFFAOYSA-N 4-(2-bromo-4-fluorophenyl)-n-(2-chloro-6-fluorophenyl)-2,5-dimethylpyrazol-3-amine Chemical compound C=1C=C(F)C=C(Br)C=1C=1C(C)=NN(C)C=1NC1=C(F)C=CC=C1Cl LBGMYUQCXJJLIR-UHFFFAOYSA-N 0.000 claims description 6
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- SHULZDWNYHRQNK-UHFFFAOYSA-N N-[(E)-methoxyiminomethyl]-4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzamide Chemical compound CO\N=C/NC(=O)C1=CC=C(C=C1)C1=NOC(=N1)C(F)(F)F SHULZDWNYHRQNK-UHFFFAOYSA-N 0.000 claims description 6
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- 230000009471 action Effects 0.000 claims description 6
- WFDXOXNFNRHQEC-GHRIWEEISA-N azoxystrobin Chemical compound CO\C=C(\C(=O)OC)C1=CC=CC=C1OC1=CC(OC=2C(=CC=CC=2)C#N)=NC=N1 WFDXOXNFNRHQEC-GHRIWEEISA-N 0.000 claims description 6
- 230000015572 biosynthetic process Effects 0.000 claims description 6
- LLEMOWNGBBNAJR-UHFFFAOYSA-N biphenyl-2-ol Chemical compound OC1=CC=CC=C1C1=CC=CC=C1 LLEMOWNGBBNAJR-UHFFFAOYSA-N 0.000 claims description 6
- 229940118790 boscalid Drugs 0.000 claims description 6
- WYEMLYFITZORAB-UHFFFAOYSA-N boscalid Chemical compound C1=CC(Cl)=CC=C1C1=CC=CC=C1NC(=O)C1=CC=CN=C1Cl WYEMLYFITZORAB-UHFFFAOYSA-N 0.000 claims description 6
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- 230000034303 cell budding Effects 0.000 claims description 6
- CRQQGFGUEAVUIL-UHFFFAOYSA-N chlorothalonil Chemical compound ClC1=C(Cl)C(C#N)=C(Cl)C(C#N)=C1Cl CRQQGFGUEAVUIL-UHFFFAOYSA-N 0.000 claims description 6
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- XDYYWNJGHXBYGU-UHFFFAOYSA-N N-methyl-4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzenecarbothioamide Chemical compound CNC(=S)C1=CC=C(C=C1)C1=NOC(=N1)C(F)(F)F XDYYWNJGHXBYGU-UHFFFAOYSA-N 0.000 claims description 3
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- NGUQQTZEJFXNMY-UHFFFAOYSA-N [3-[2-[1-[2-[3,5-bis(difluoromethyl)pyrazol-1-yl]acetyl]piperidin-4-yl]-1,3-thiazol-4-yl]-1,5-dihydro-2,4-benzodioxepin-6-yl] methanesulfonate Chemical compound CS(=O)(=O)OC1=CC=CC=2COC(OCC=21)C=1N=C(SC=1)C1CCN(CC1)C(CN1N=C(C=C1C(F)F)C(F)F)=O NGUQQTZEJFXNMY-UHFFFAOYSA-N 0.000 claims description 3
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- AOPCKOPZYFFEDA-UHFFFAOYSA-N nickel(2+);dinitrate;hexahydrate Chemical compound O.O.O.O.O.O.[Ni+2].[O-][N+]([O-])=O.[O-][N+]([O-])=O AOPCKOPZYFFEDA-UHFFFAOYSA-N 0.000 description 1
- BFSQJYRFLQUZKX-UHFFFAOYSA-L nickel(ii) iodide Chemical compound I[Ni]I BFSQJYRFLQUZKX-UHFFFAOYSA-L 0.000 description 1
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- 125000003538 pentan-3-yl group Chemical group [H]C([H])([H])C([H])([H])C([H])(*)C([H])([H])C([H])([H])[H] 0.000 description 1
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Classifications
-
- A—HUMAN NECESSITIES
- A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
- A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
- A01N43/00—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds
- A01N43/72—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with nitrogen atoms and oxygen or sulfur atoms as ring hetero atoms
- A01N43/88—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with nitrogen atoms and oxygen or sulfur atoms as ring hetero atoms six-membered rings with three ring hetero atoms
-
- A—HUMAN NECESSITIES
- A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
- A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
- A01N43/00—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds
- A01N43/48—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with two nitrogen atoms as the only ring hetero atoms
- A01N43/58—1,2-Diazines; Hydrogenated 1,2-diazines
-
- A—HUMAN NECESSITIES
- A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
- A01P—BIOCIDAL, PEST REPELLANT, PEST ATTRACTANT OR PLANT GROWTH REGULATORY ACTIVITY OF CHEMICAL COMPOUNDS OR PREPARATIONS
- A01P3/00—Fungicides
Landscapes
- Life Sciences & Earth Sciences (AREA)
- Environmental Sciences (AREA)
- Wood Science & Technology (AREA)
- Plant Pathology (AREA)
- Engineering & Computer Science (AREA)
- Zoology (AREA)
- Pest Control & Pesticides (AREA)
- Health & Medical Sciences (AREA)
- Dentistry (AREA)
- General Health & Medical Sciences (AREA)
- Agronomy & Crop Science (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Mycology (AREA)
- Chemical & Material Sciences (AREA)
- General Chemical & Material Sciences (AREA)
- Microbiology (AREA)
- Agricultural Chemicals And Associated Chemicals (AREA)
- Plural Heterocyclic Compounds (AREA)
- Pharmaceuticals Containing Other Organic And Inorganic Compounds (AREA)
- Heterocyclic Carbon Compounds Containing A Hetero Ring Having Nitrogen And Oxygen As The Only Ring Hetero Atoms (AREA)
- Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
Abstract
본 발명은 화합물 (A)로서 화학식 (I)의 화합물 및 화합물 (B)로서 하기 명시된 바와 같은 추가의 살진균 활성 화합물을 포함하는, 특히 살진균제 조성물 내의 활성 화합물 조합물에 관한 것이다. 또한, 본 발명은 이러한 화합물 조합물을 포함하는 조성물, 및 특히 작물 보호 및 산업적 물질의 보호에서 식물병원성 진균의 방제를 위한 생물학적 활성제로서, 및 식물 성장 조절제로서의 화합물 조합물 및 살진균제 조성물의 용도에 관한 것이다.
Description
본 발명은 화합물 (A)로서 화학식 (I)의 화합물 및 화합물 (B)로서 하기 명시된 바와 같은 추가의 살진균 활성 화합물을 포함하는, 특히 살진균제 조성물 내의 활성 화합물 조합물에 관한 것이다. 또한, 본 발명은 이러한 화합물 조합물을 포함하는 조성물, 및 특히 작물 보호 및 산업적 물질의 보호에서 식물병원성 진균의 방제를 위한 생물학적 활성제로서 및 식물 성장 조절제로서의 화합물 조합물 및 살진균제 조성물의 용도에 관한 것이다.
본 출원 전반에 걸쳐 용어 "조성물" 및 "제제"는 동의어로 사용되고, 본 발명의 화합물 조합물 및 적어도 1종의 농업상 적합한 보조제의 혼합물을 지칭한다.
화학식 (I)의 화합물은 진균에 의해 유발된 질병으로부터 식물을 보호하는 데 탁월한 수단을 제공하지만, 오늘날 작물 보호제 및 조성물에 부과되는 계속 증가하는 환경적 및 경제적 요건을 다루기 위해 이들 수단을 여전히 개선시킬 필요가 있다. 이는, 예를 들어 작용 스펙트럼, 안전성 프로파일, 선택성, 적용률, 잔류물의 형성, 및 유리한 제조 능력에 대한 개선, 및 내성과 같은 잠재적 문제를 다루기 위한 신규 조성물의 개발을 포함한다.
본 발명은 적어도 일부 측면에서 언급된 목적을 달성하는 활성 화합물 조합물 및 상기 조합물을 포함하는 조성물을 제공한다.
따라서, 본 발명은 하기를 포함하는 활성 화합물 조합물을 제공한다:
(A) 화학식 (I)의 적어도 1종의 화합물
여기서
A는 O, S, C(=O), S(=O), S(=O)2, NR1 및 CR1R2로 이루어진 군으로부터 선택되고, 여기서 R1 및 R2는 독립적으로 수소, C1-C6-알킬 및 C3-C8-시클로알킬로 이루어진 군으로부터 선택되거나, 또는 R1 및 R2는 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬 또는 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 형성하고;
m은 0, 1 또는 2이고;
T는 수소, 히드록실, C1-C6-알킬, -C(=O)Ra1, -C(=O)(ORa1), -C(=O)N(Ra2)2, -S(=O)Ra1, -S(=O)2Ra1 및 S(=O)2N(Ra2)2로 이루어진 군으로부터 선택되고,
여기서 Ra1은 C1-C6-알킬, C1-C6-할로알킬, C3-C8-시클로알킬 및 C2-C6-알케닐로 이루어진 군으로부터 선택되고,
여기서 Ra2는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬, C3-C8-시클로알킬 및 C2-C6-알케닐로 이루어진 군으로부터 선택되고;
R3 및 R4는 독립적으로 수소, 할로겐, 시아노, 히드록실, 포르밀, 카르복실, C1-C6-알킬, C1-C6-알콕시, C1-C6-알킬카르보닐, C1-C6-알콕시카르보닐, C2-C6-알케닐, C2-C6-알키닐, C3-C8-시클로알킬, 방향족 C6-C14-카르보사이클, 방향족 5- 내지 14-원 헤테로사이클, 비-방향족 3- 내지 14-원 헤테로사이클 및 -O-Si(C1-C6-알킬)3으로 이루어진 군으로부터 선택되거나, 또는 R3 및 R4는 이들이 부착되어 있는 탄소 원자와 함께, 카르보닐, 메틸리덴, C3-C8-시클로알킬 또는 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 형성하고;
R5는 수소, 히드록실, C1-C6-알킬, C1-C6-알콕시, C1-C6-알킬카르보닐옥시, C1-C6-알킬술파닐, C1-C6-알킬술피닐, C1-C6-알킬술포닐, C3-C8-시클로알킬 및 -O-Si(C1-C6-알킬)3으로 이루어진 군으로부터 선택되고;
여기서 지방족 R1, R2, R3, R4 및 R5 치환기는 할로겐, 시아노, 아미노, 니트로, 히드록실, 포르밀, 카르복실, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -O-Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 치환기로 치환될 수 있고;
여기서 시클릭 R1, R2, R3, R4 및 R5 치환기는 할로겐, 시아노, 니트로, 히드록실, 포르밀, 옥소, 메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -O-Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 치환기로 치환될 수 있고;
R3 또는 R4, 및 R5는 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬을 형성할 수 있고;
L은 직접 결합을 나타내거나, 또는 L은 카르보닐, C1-C6-알킬렌, 동일한 탄소 원자 상에서 치환기가 부착되어 있는 탄소 원자와 함께 C3-C8-시클로알킬을 형성하는 2개의 치환기에 의해 치환된 C1-C6-알킬렌, 동일한 탄소 원자 상에서 치환기가 부착되어 있는 탄소 원자와 함께 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 형성하는 2개의 치환기에 의해 치환된 C1-C6-알킬렌, C2-C6-알케닐렌, C2-C6-알키닐렌, C3-C8-시클로알킬렌, C1-C6-알킬렌-C3-C8-시클로알킬렌, C3-C8-시클로알킬렌-C1-C6-알킬렌, C1-C6-알킬렌-C3-C8-시클로알킬렌-C1-C6-알킬렌, C1-C6-알킬렌-(C=O), C(=O)-C1-C6-알킬렌, C3-C8-시클로알케닐렌, C1-C6-알킬렌-C3-C8-시클로알케닐렌, C3-C8-시클로알케닐렌-C1-C6-알킬렌, C1-C6-알킬렌-C3-C8-시클로알케닐렌-C1-C6-알킬렌, 비-방향족 3- 내지 7-원 모노시클릭 헤테로시클릴렌, -NRaL1-, -NRaL1(C=O)-, -C(=O)NRaL1-, -NRaL1S(=O)2-, -S(=O)2NRaL1-, -C(=NORaL2)-, -C(=N-N(RaL2)2) 및 -C(=NRaL2)-로 이루어진 군으로부터 선택되고;
여기서 RaL1은 수소 및 C1-C6-알킬로 이루어진 군으로부터 선택되고,
여기서 RaL2는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬, C3-C8-시클로알킬 및 C2-C6-알킬레닐로 이루어진 군으로부터 선택되고,
여기서 지방족 L 치환기는 동일하거나 상이할 수 있는 1개 이상의 LSa 치환기로 치환될 수 있고,
여기서 L 치환기의 시클릭 또는 시클릭 모이어티는 동일하거나 상이할 수 있는 1개 이상의 LSc 치환기로 치환될 수 있고,
Lsa는 할로겐, 시아노, 히드록실, 카르복실, 메틸리덴, 할로메틸리덴, C1-C6-알콕시, C1-C6-할로알콕시, C3-C8-시클로알킬, C3-C8-할로시클로알킬, C1-C6-알콕시카르보닐, -O-Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
LSc는 할로겐, 시아노, 니트로, 히드록실, 포르밀, 카르복실, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -O-Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고/거나, 2개의 LSc 치환기가 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬을 형성하고;
R6은 비-방향족 C3-C12-카르보사이클, 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클, 방향족 5- 내지 14-원 헤테로사이클, 비-방향족 C3-C12-카르보시클릴옥시, 방향족 C6-C14-카르보시클릴옥시, 방향족 5- 내지 14-원 헤테로시클릴옥시, 비-방향족 5- 내지 14-원 헤테로시클릴옥시, 비-방향족 C3-C12-카르보시클릴술파닐, 방향족 C6-C14-카르보시클릴술파닐, 방향족 5- 내지 14-원 헤테로시클릴술파닐, 비-방향족 5- 내지 14-원 헤테로시클릴술파닐, 비-방향족 C3-C12-카르보시클릴술피닐, 방향족 C6-C14-카르보시클릴술피닐, 방향족 5- 내지 14-원 헤테로시클릴술피닐, 비-방향족 5- 내지 14-원 헤테로시클릴술피닐, 비-방향족 C3-C12-카르보시클릴술포닐, 방향족 C6-C14-카르보시클릴술포닐, 방향족 5- 내지 14-원 헤테로시클릴술포닐, 비-방향족 5- 내지 14-원 헤테로시클릴술포닐, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-알콕시, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-알콕시, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-알콕시, 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-알콕시, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-할로알콕시, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-할로알콕시, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-할로알콕시, 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-할로알콕시, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-술파닐, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-술파닐, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술파닐 및 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술파닐, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-술피닐, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-술피닐, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술피닐 및 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술피닐, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-술포닐, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-술포닐, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술포닐 및 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술포닐로 이루어진 군으로부터 선택되고;
여기서 R6 치환기의 시클릭 또는 시클릭 모이어티는 동일하거나 상이할 수 있는 1개 이상의 R6S 치환기로 치환될 수 있고,
R6S는 할로겐, 시아노, 이소시아노, 니트로, 히드록실, 메르캅토, 펜타플루오로술파닐, 옥소, 메틸리덴, 할로메틸리덴, 포르밀, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C2-C6-알킬닐옥시, C2-C6-할로알킬닐옥시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C3-C8-시클로알킬술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C3-C8-시클로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, C3-C8-시클로알킬술포닐, C3-C8-시클로알킬, C3-C8-시클로알킬옥시, C3-C8-시클로알케닐, 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, -N(Rc)2, -O-(C=O)Rd, -C(=O)Rd, -C(=O)(ORd), -C(=O)N(Rd)2, -S(=O)2N(Rd)2, -O-Si(C1-C6-알킬)3 및 -Si(C1-C6-알킬)3으로 이루어진 군으로부터 선택되거나, 또는 2개의 R6S 치환기는 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬을 형성할 수 있고,
여기서 Rc는 독립적으로 수소, C1-C6-알킬 및 C3-C8-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 Rd는 독립적으로 수소, C1-C6-알킬 및 C1-C6-할로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 R6S, Rc 및 Rd 치환기는 시아노, 할로겐, 히드록실, C1-C6-알콕시, C1-C6-할로알콕시, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, C3-C8-시클로알킬, C3-C8-할로시클로알킬 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 치환기로 치환될 수 있고,
여기서 R6S의 시클릭 또는 시클릭 모이어티 및 시클릭 Rc 치환기는 할로겐, 시아노, 니트로, 히드록실, 포르밀, 카르복실, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C2-C6-알케닐, C3-C8-시클로알킬 및 C3-C8-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 치환기로 치환될 수 있고/거나, R6S 치환기의 시클릭 또는 시클릭 모이어티는 치환기가 부착되어 있는 탄소 원자와 함께 C3-C8-시클로알킬을 형성하는 2개의 치환기로 치환될 수 있고;
R7은 수소, 할로겐, 시아노, 이소시아노, 히드록실, 메르캅토, 니트로, 아미노, 포르밀, C1-C6-알킬, C1-C6-할로알킬, C1-C6-히드록시알킬, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알킬카르보닐, C1-C6-할로알킬카르보닐, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C2-C6-알키닐옥시, C2-C6-할로알키닐옥시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C3-C8-시클로알킬술파닐, C2-C6-알케닐술파닐, C2-C6-알키닐술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C3-C8-시클로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, C3-C8-시클로알킬술포닐, C3-C8-시클로알킬, C3-C6-시클로알케닐, 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, C3-C8-시클로알킬옥시, 방향족 C6-C14-카르보시클릴옥시, 방향족 5- 또는 6-원 모노시클릭 헤테로시클릴옥시, 비-방향족 3- 내지 7-원 모노시클릭 헤테로시클릴옥시, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, -N(Re)2, -C(=NRf)Rf, NRgC(=O)Rg, -C(=O)(ORg), -C(=O)N(Rg)2, -S(=O)2N(Rg)2 및 -S(=O)(=NRg)Rg으로 이루어진 군으로부터 선택되고,
여기서 Re는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 Rf는 독립적으로 히드록실, 아미노, 시아노, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-알킬아미노 및 디(C1-C6-알킬)아미노로 이루어진 군으로부터 선택되고,
여기서 Rg는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬 및 C3-C8-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 R7, Re, Rf 및 Rg 치환기는 동일하거나 상이할 수 있는 1개 이상의 R7Sa 치환기로 치환될 수 있고,
여기서 R7의 시클릭 또는 시클릭 모이어티, 시클릭 Re 및 시클릭 Rg 치환기는 동일하거나 상이할 수 있는 1개 이상의 R7Sc 치환기로 치환될 수 있고,
R7Sa는 시아노, 히드록실, 카르복실, C1-C6-알콕시, C1-C6-할로알콕시, C3-C8-시클로알킬, C3-C8-할로시클로알킬, C1-C6-알콕시카르보닐, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, 방향족 C6-C14-카르보사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
R7Sc는 할로겐, 시아노, 니트로, 히드록실, 포르밀, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬 C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -O-Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되거나, 또는 2개의 R7Sc 치환기는 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬을 형성하고;
R8은 수소, 할로겐, 시아노, 이소시아노, 아미노, 니트로, 히드록실, 메르캅토, 카르복실, C1-C6-알콕시카르보닐, C1-C6-알킬, C1-C6-할로알킬, C1-C6-히드록시알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C2-C6-알키닐옥시, C2-C6-할로알키닐옥시, C3-C8-시클로알킬, C3-C6-시클로알케닐, 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클, 방향족 5- 내지 14-원 헤테로사이클, C3-C8-시클로알킬옥시, 방향족 C6-C14-카르보시클릴옥시, 비-방향족 3- 내지 14-원 헤테로시클릴옥시, 방향족 5- 내지 14-원 헤테로시클릴옥시, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, -N(Rh)2, -SRi, -S(=O)Ri 및 -S(=O)2Ri로 이루어진 군으로부터 선택되고,
여기서 Rh는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, 방향족 C6-C14-카르보사이클, 방향족 5- 내지 14-원 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 Ri는 C1-C6-알킬, C1-C6-할로알킬, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, 방향족 C6-C14-카르보사이클, 방향족 5- 내지 14-원 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 지방족 R8, Rh 및 Ri 치환기는 동일하거나 상이할 수 있는 1개 이상의 R8Sa 치환기로 치환될 수 있고,
여기서 R8의 시클릭 또는 시클릭 모이어티, 시클릭 Rh 및 시클릭 Ri 치환기는 동일하거나 상이할 수 있는 1개 이상의 R8Sc 치환기로 치환될 수 있고,
R8Sa는 시아노, 아미노, 니트로, 히드록실, 포르밀, 카르복실, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시-C1-C6-알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C1-C6-알킬카르보닐, C1-C6-할로알킬카르보닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클 및 -N(Ra')2로 이루어진 군으로부터 선택되고, 여기서 Ra'는 독립적으로 수소, 포르밀, C1-C6-알킬, C1-C6-할로알킬, C3-C8-시클로알킬 및 C1-C6-알킬카르보닐로 이루어진 군으로부터 선택되고, 여기서 상기 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클 R8Sa는 동일하거나 상이할 수 있는 1개 이상의 C1-C6-알킬 치환기로 치환될 수 있고,
R8Sc는 할로겐, 시아노, 아미노, 니트로, 히드록실, 포르밀, 카르복실, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C2-C6-알케닐, C1-C6-알킬술파닐, C1-C6-알킬술피닐, C1-C6-알킬술포닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -O-Si(C1-C6-알킬)3 및 동일하거나 상이할 수 있는 1개 이상의 C1-C6-알킬 치환기로 치환될 수 있는 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되거나, 또는 2개의 R8Sc 치환기는 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬 또는 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 형성하고, 여기서 상기 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클은 동일하거나 상이할 수 있는 1개 이상의 C1-C6-알킬 치환기로 치환될 수 있고;
Q는 방향족 C6-C14-카르보사이클, 비-방향족 C3-C12-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클 및 방향족 5- 내지 14-원 헤테로사이클로 이루어진 군으로부터 선택되고, 여기서 상기 카르보사이클 또는 헤테로사이클 기 중 임의의 것은 동일하거나 상이할 수 있는 1개 이상의 QS 치환기로 치환될 수 있고,
QS는 할로겐, 시아노, 이소시아노, 니트로, 히드록실, 메르캅토, 포르밀, 카르복실, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알킬카르보닐, C1-C6-할로알킬카르보닐, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, C3-C8-시클로알킬, C3-C8-시클로알킬옥시, C3-C6-시클로알케닐, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, 방향족 C6-C14-카르보사이클, 방향족 5- 내지 14-원 헤테로사이클, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, -O-C(=O)Rj, -NRjC(=O)Rj, -C(=O)N(Rj)2, -C(=S)Rj, -C(=S)N(Rj)2, -C(=NRj)Rj 및 -C(=NORj)Rj 및 -N(Rk)2로 이루어진 군으로부터 선택되고,
여기서 Rj는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬 및 C1-C6-알콕시로 이루어진 군으로부터 선택되고,
여기서 Rk는 독립적으로 수소, 히드록실, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C2-C6-알케닐, C2-C6-할로알케닐 및 C3-C8-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 QS, Rj 및 Rk 치환기는 시아노, 아미노, 니트로, 히드록실, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 치환기로 치환될 수 있고,
여기서 QS의 시클릭 또는 시클릭 모이어티 및 시클릭 Rk 치환기는 할로겐, 시아노, 아미노, 니트로, 히드록실, 포르밀, 카르복실, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, C2-C6-알케닐 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 RQs 치환기로 치환될 수 있고, 여기서 시클릭 RQs 치환기는 치환기가 부착되어 있는 탄소 원자와 함께 C3-C8-시클로알킬을 형성하는 2개의 치환기로 치환될 수 있음,
및
(B) 하기로부터 선택된 적어도 1종의 추가의 활성 화합물
(1) 에르고스테롤 합성의 억제제,
(2) 복합체 I 또는 II에서의 호흡 사슬의 억제제,
(3) 복합체 III에서의 호흡 사슬의 억제제,
(4) 유사분열 및 세포 분열의 억제제,
(5) 다중부위 작용을 가질 수 있는 화합물,
(6) 숙주 방어를 유도할 수 있는 화합물,
(7) 아미노산 및/또는 단백질 생합성의 억제제,
(8) ATP 생산 억제제,
(9) 세포벽 합성의 억제제,
(10) 지질 및 막 합성의 억제제,
(11) 멜라닌 생합성의 억제제,
(12) 핵산 합성의 억제제,
(13) 신호 전달의 억제제,
(14) 탈커플링제로서 작용할 수 있는 화합물,
(15) 다른 살진균제,
(16) 항박테리아제,
(17) 생물학적 살진균제
(18) 지방산 또는 그의 유도체.
화합물 (A)
본 발명에 따른 활성 화합물 조합물은 화합물 (A)로서 화학식 (I)의 적어도 1종의 화합물 또는 그의 염 또는 N-옥시드를 포함한다.
바람직한 실시양태에서, 본 발명에 따른 화합물은
A가 O, S, C(=O), S(=O), S(=O)2, NR1 및 CR1R2로 이루어진 군으로부터 선택되고, 여기서 R1 및 R2는 독립적으로 수소, C1-C4-알킬 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
m이 0, 1 또는 2이고;
T는 수소 및 C1-C4-알킬로 이루어진 군으로부터 선택되고,
R3 및 R4가 독립적으로 수소, 플루오린, 염소, C1-C4-알킬, C2-C4-알케닐, C2-C4-알키닐, C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
R5가 수소, 히드록실, C1-C4-알킬, C1-C4-알콕시, C1-C4-알킬술파닐로 이루어진 군으로부터 선택되고,
여기서 지방족 R1, R2, R3, R4 및 R5 치환기는 플루오린, 염소, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬, C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 치환기로 치환될 수 있고,
여기서 시클릭 R1, R2, R3, R4 및 R5 치환기는 플루오린, 염소, 옥소, 메틸리덴, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C3-C6-시클로알킬, C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 치환기로 치환될 수 있고,
R3 또는 R4, 및 R5가 이들이 부착되어 있는 탄소 원자와 함께, C3-C6-시클로알킬을 형성할 수 있고;
L이 직접 결합을 나타내거나, 또는 L은 C1-C6-알킬렌, 동일한 탄소 원자 상에서 치환기가 부착되어 있는 탄소 원자와 함께 C3-C6-시클로알킬을 형성하는 2개의 치환기에 의해 치환된 C1-C6-알킬렌, 동일한 탄소 원자 상에서 치환기가 부착되어 있는 탄소 원자와 함께 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 형성하는 2개의 치환기에 의해 치환된 C1-C6-알킬렌으로 이루어진 군으로부터 선택되고,
여기서 지방족 L 치환기는 플루오린, 염소, 히드록실, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬 및 C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 LSa 치환기로 치환될 수 있고,
여기서 L 치환기의 시클릭 또는 시클릭 모이어티는 플루오린, 염소, 히드록실, 옥소, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C3-C6-시클로알킬 및 C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 LSc 치환기로 치환될 수 있고,
R6이 비-방향족 C3-C12-카르보사이클, 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클, 방향족 5- 내지 14-원 헤테로사이클, 비-방향족 C3-C12-카르보시클릴옥시, 방향족 C6-C14-카르보시클릴옥시, 방향족 5- 내지 14-원 헤테로시클릴옥시, 비-방향족 5- 내지 14-원 헤테로시클릴옥시, 비-방향족 C3-C12-카르보시클릴술파닐, 방향족 C6-C14-카르보시클릴술파닐, 방향족 5- 내지 14-원 헤테로시클릴술파닐 및 비-방향족 5- 내지 14-원 헤테로시클릴술파닐로 이루어진 군으로부터 선택되고,
여기서 R6 치환기의 시클릭 또는 시클릭 모이어티는 동일하거나 상이할 수 있는 1 내지 3개의 R6S 치환기로 치환될 수 있고,
R6S는 할로겐, 시아노, 니트로, 히드록실, 메르캅토, 펜타플루오로술파닐, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C3-C6-시클로알킬술파닐, C3-C6-시클로알킬, C3-C6-시클로알킬옥시, 페닐, 나프틸 방향족 5- 또는 6-원 모노시클릭 헤테로사이클, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, -C(=O)(ORd) 및 -C(=O)N(Rd)2로 이루어진 군으로부터 선택되고,
여기서 Rd는 독립적으로 수소, C1-C4-알킬 및 C1-C4-할로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 R6S, Rc 및 Rd 치환기는 플루오린, 염소, 히드록실, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬 및 C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 치환기로 치환될 수 있고, 여기서 R6S의 시클릭 또는 시클릭 모이어티 및 시클릭 Rc 치환기는 플루오린, 염소, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시 및 C1-C4-할로알콕시로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 치환기로 치환될 수 있고,
R7이 수소, 할로겐, 시아노, 히드록실, 메르캅토, C1-C4-알킬, C1-C4-할로알킬, C1-C4-히드록시알킬, C1-C4-알콕시, C1-C4-할로알콕시, C1-C4-알킬카르보닐, C1-C4-할로알킬카르보닐, C2-C4-알케닐, C2-C4-할로알케닐, C2-C4-알키닐, C2-C4-할로알키닐, C1-C4-알킬술파닐, C1-C4-할로알킬술파닐, C3-C6-시클로알킬술파닐, C1-C4-알킬술피닐, C1-C4-할로알킬술피닐, C3-C6-시클로알킬술피닐, C1-C4-알킬술포닐, C1-C4-할로알킬술포닐, C3-C6-시클로알킬술포닐, C3-C6-시클로알킬, C3-C6-시클로알케닐, 페닐, 나프틸, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, C3-C8-시클로알킬옥시, 방향족 C6-C14-카르보시클릴옥시, 방향족 5- 또는 6-원 모노시클릭 헤테로시클릴옥시, 비-방향족 3- 내지 7-원 모노시클릭 헤테로시클릴옥시, -N(Re)2, -C(=NRf)Rf, NRgC(=O)Rg, -C(=O)(ORg), -C(=O)N(Rg)2, -S(=O)2N(Rg)2 및 -S(=O)(=NRg)Rg으로 이루어진 군으로부터 선택되고,
여기서 Re는 독립적으로 수소, C1-C4-알킬, C1-C4-할로알킬, C2-C4-알케닐, C2-C4-할로알케닐, C2-C4-알키닐, C2-C4-할로알키닐, C3-C6-시클로알킬, C3-C6-할로시클로알킬로 이루어진 군으로부터 선택되고,
여기서 Rf는 독립적으로 히드록실, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시로 이루어진 군으로부터 선택되고,
여기서 Rg는 독립적으로 수소, C1-C4-알킬, C1-C4-할로알킬 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 R7, Re, Rf 및 Rg 치환기는 동일하거나 상이할 수 있는 1 내지 3개의 R7Sa 치환기로 치환될 수 있고,
여기서 R7의 시클릭 또는 시클릭 모이어티, 시클릭 Re 및 시클릭 Rg 치환기는 동일하거나 상이할 수 있는 1 내지 3개의 R7Sc 치환기로 치환될 수 있고,
R7Sa는 히드록실, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬로 이루어진 군으로부터 선택되고, R7Sc는 플루오린, 염소, 히드록실, 옥소, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
R8이 수소, 할로겐, 아미노, 히드록실, 메르캅토, C1-C4-알킬, C1-C4-할로알킬, C1-C4-히드록시알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C2-C4-할로알케닐, C2-C4-알키닐, C2-C4-할로알키닐, C2-C4-알케닐옥시, C2-C4-할로알케닐옥시, C2-C4-알키닐옥시, C2-C4-할로알키닐옥시, C3-C6-시클로알킬, C3-C6-시클로알케닐, 페닐, 나프틸, 비-방향족 3- 내지 7-원 헤테로사이클, 방향족 5- 또는 6-원 헤테로사이클, C3-C6-시클로알킬옥시, 페닐옥시, 나프틸옥시, 비-방향족 3- 내지 7-원 헤테로시클릴옥시, 방향족 5- 또는 6-원 헤테로시클릴옥시, -N(Rh)2, -SRi , -S(=O)Ri 및 -S(=O)2Ri로 이루어진 군으로부터 선택되고,
여기서 Rh는 독립적으로 수소, C1-C4-알킬, C1-C4-할로알킬, C2-C4-알케닐, C2-C4-할로알케닐, C3-C6-시클로알킬, C3-C6-할로시클로알킬, 페닐, 나프틸 방향족 5- 또는 6-원 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 Ri는 C1-C4-알킬, C1-C4-할로알킬, C2-C4-알케닐, C2-C4-할로알케닐, C2-C4-알키닐, C2-C4-할로알키닐, C3-C6-시클로알킬, C3-C6-할로시클로알킬, 페닐, 나프틸, 방향족 5- 또는 6-원 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 지방족 R8, Rh 및 Ri 치환기는 동일하거나 상이할 수 있는 1 내지 3개의 R8Sa 치환기로 치환될 수 있고,
여기서 R8의 시클릭 또는 시클릭 모이어티, 시클릭 Rh 및 시클릭 Ri 치환기는 동일하거나 상이할 수 있는 1 내지 3개의 R8Sc 치환기로 치환될 수 있고,
R8Sa는 히드록실, 카르복실, C1-C4-알콕시, C1-C4-할로알콕시, C1-C4-알콕시카르보닐, C1-C4-할로알콕시카르보닐, C3-C6-시클로알킬, C3-C6-할로시클로알킬, C1-C4-알킬술파닐, C1-C4-할로알킬술파닐, C1-C4-알킬술피닐, C1-C4-할로알킬술피닐, C1-C4-알킬술포닐, C1-C4-할로알킬술포닐, 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고, 여기서 상기 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클 R8Sa는 동일하거나 상이할 수 있는 1 또는 2개의 C1-C4-알킬 치환기로 치환될 수 있고,
R8Sc는 할로겐, 옥소, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
Q가 페닐, 나프틸, 비-방향족 C5-C10-카르보사이클, 비-방향족 5- 내지 10-원 헤테로사이클 및 방향족 5- 내지 10-원 헤테로사이클로 이루어진 군으로부터 선택되고, 여기서 상기 카르보사이클 또는 헤테로사이클 기 중 임의의 것은 동일하거나 상이할 수 있는 1 내지 3개의 QS 치환기로 치환될 수 있고,
QS는 할로겐, 시아노, 니트로, 포르밀, 카르복실, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알킬카르보닐, C1-C4-할로알킬카르보닐, C1-C4-알콕시, C1-C4-할로알콕시, C1-C4-알콕시카르보닐, C1-C4-할로알콕시카르보닐, C2-C4-알케닐, C2-C4-할로알케닐, C2-C4-알키닐, C2-C4-할로알키닐, C1-C4-알킬술파닐, C1-C4-할로알킬술파닐, C1-C4-알킬술피닐, C1-C4-할로알킬술피닐, C1-C4-알킬술포닐, C1-C4-할로알킬술포닐, C3-C6-시클로알킬, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, 페닐, 나프틸 및 방향족 5- 내지 10-원 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 지방족 QS, Rj 및 Rk 치환기는 히드록실, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬 및 C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 치환기로 치환될 수 있고, 여기서 QS의 시클릭 또는 시클릭 모이어티 및 시클릭 Rk 치환기는 플루오린, 염소, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시 및 C3-C6-시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 RQs 치환기로 치환될 수 있는 것인
화학식 (I)의 화합물이다.
보다 바람직한 실시양태에서, 본 발명에 따른 화합물은
A가 O, S(=O)2, NR1 및 CR1R2로 이루어진 군으로부터 선택되고, 여기서 R1 및 R2는 독립적으로 수소, C1-C4-알킬 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
m이 0, 1 또는 2이고;
T가 수소 및 C1-C4-알킬로 이루어진 군으로부터 선택되고,
R3 및 R4가 독립적으로 수소, 플루오린, 염소, C1-C4-알킬, C2-C4-알케닐, C2-C4-알키닐 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
R5가 수소, 히드록실, C1-C4-알킬 및 C1-C4-알콕시로 이루어진 군으로부터 선택되고,
L이 직접 결합을 나타내거나, 또는 L은 C1-C6-알킬렌으로 이루어진 군으로부터 선택되고,
여기서 지방족 L 치환기는 플루오린, 염소, 히드록실, C1-C4-알콕시, C1-C4-할로알콕시 및 C3-C6-시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 LSa 치환기로 치환될 수 있고,
여기서 L 치환기의 시클릭 또는 시클릭 모이어티는 플루오린, 염소, 히드록실, 옥소, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시 및 C3-C6-시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 LSc 치환기로 치환될 수 있고,
R6이 비-방향족 C5-C10-카르보사이클, 페닐, 나프틸, 비-방향족 5- 내지 10-원 헤테로사이클, 방향족 5- 내지 10-원 헤테로사이클, 비-방향족 C5-C10-카르보시클릴옥시, 페녹시, 나프틸옥시, 방향족 5- 내지 10-원 헤테로시클릴옥시, 비-방향족 5- 내지 10-원 헤테로시클릴옥시 및 페닐술파닐로 이루어진 군으로부터 선택되고,
여기서 R6 치환기의 시클릭 또는 시클릭 모이어티는 할로겐, 니트로, 히드록실, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C2-C4-알키닐, C1-C4-할로알킬술파닐, 시클로프로필, 시클로부틸, 시클로펜틸, 피리디닐, 옥세타닐 및 테트라히드로푸라닐로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 R6S 치환기로 치환될 수 있고, 여기서 시클릭 R6S 치환기는 할로겐, C1-C4-알킬, C1-C4-할로알킬 및 C1-C4-알콕시카르보닐로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 치환기로 치환될 수 있고,
R7이 수소, 할로겐, 시아노, C1-C4-알킬, C1-C4-할로알킬, C1-C4-히드록시알킬, C1-C4-알킬카르보닐, C1-C4-알콕시, C2-C4-알케닐, C2-C4-알키닐, C1-C4-알킬술파닐, C1-C4-알케닐술파닐, C1-C4-알킬술포닐, C3-C6-시클로알킬, 피리디닐, 이미다졸릴, 피라졸릴, 티아졸릴, 옥세타닐, 테트라히드로푸라닐, 피롤리디닐, -N(Re)2, -C(=NRf)Rf 및 -C(=O)N(Rg)2로 이루어진 군으로부터 선택되고,
여기서 Re는 독립적으로 수소, C1-C4-알킬 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 Rf는 독립적으로 C1-C4-알킬 및 C1-C4-알콕시로 이루어진 군으로부터 선택되고,
여기서 Rg는 독립적으로 수소, C1-C4-알킬 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 상기 지방족 R7, Re 및 Rg 치환기는 히드록실, C1-C4-알콕시 및 C3-C6-시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 R7Sa 치환기로 치환될 수 있고,
여기서 상기 시클릭 R7, Re 및 Rg 치환기는 할로겐, 히드록실, C1-C4-알킬 및 C1-C4-알콕시로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 R7Sc 치환기로 치환될 수 있고,
R8이 수소, 할로겐, 히드록실, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C2-C4-알케닐, C1-C4-알킬술파닐, C1-C4-할로알킬술파닐, C1-C4-알킬술피닐, C1-C4-알킬술포닐, C3-C6-시클로알킬, 페닐, 나프틸, 옥세타닐, 아제티디닐, 테트라히드로푸라닐, 피롤리디닐, 테트라히드로피라닐, 피페리디닐, 피페라지닐, 모르폴리닐, 푸라닐, 티에닐, 피롤릴, 피라졸릴, 티아졸릴, 이미다졸릴, 옥사졸릴, 이속사졸릴, 피리디닐, 피리미디닐, C3-C6-시클로알킬옥시 및 -N(Rh)2로 이루어진 군으로부터 선택되고,
여기서 Rh는 독립적으로 수소, C1-C4-알킬, C1-C4-할로알킬, C2-C4-알케닐, C3-C6-시클로알킬, 페닐, 옥세타닐, 아제티디닐, 피롤리디닐 및 테트라히드로푸라닐로 이루어진 군으로부터 선택되고,
여기서 본원에 개시된 바와 같은 지방족 R8 및 Rh 치환기는 히드록실, C1-C4-알콕시, C1-C4-알콕시카르보닐, C3-C6-시클로알킬, C1-C4-알킬술파닐, 옥세타닐, 아제티디닐, 피롤리디닐 및 테트라히드로푸라닐로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 R8Sa 치환기로 치환될 수 있고,
여기서 본원에 개시된 바와 같은 시클릭 R8 및 Rh 치환기는 옥소, 플루오린, 염소, 히드록실, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C3-C6-시클로알킬, 옥세타닐, 아제티디닐, 피롤리디닐 및 테트라히드로푸라닐로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 R8Sc 치환기로 치환될 수 있고,
Q가 페닐, 1,3-벤조디옥솔-5-일, 2,3-디히드로벤조푸라닐, 피리디닐, 티에닐 및 인돌-5-일로 이루어진 군으로부터 선택되고,
여기서 본원에 개시된 바와 같은 보다 바람직한 Q 기는 할로겐, 시아노, 니트로, 포르밀, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C2-C4-알키닐, C1-C4-알킬술파닐, C3-C6-시클로알킬 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 QS 치환기로 치환될 수 있고,
여기서 상기 보다 바람직한 지방족 QS 치환기는 히드록실, C1-C4-알콕시, C1-C4-할로알콕시, C1-C4-알콕시카르보닐, C1-C4-할로알콕시카르보닐 및 C3-C6-시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 치환기로 치환될 수 있는 것인
화학식 (I)의 화합물이다.
보다 더 바람직한 실시양태에서, 본 발명에 따른 화합물은
A가 O, NR1 및 CR1R2로 이루어진 군으로부터 선택되고, 여기서 R1 및 R2는 독립적으로 수소, 메틸 또는 에틸로 이루어진 군으로부터 선택되고,
m이 1이고;
T가 수소이고,
R3 및 R4가 독립적으로 수소 또는 플루오린으로 이루어진 군으로부터 선택되고,
R5가 수소이고,
L이 직접 결합을 나타내거나 또는 L이 메틸렌이고,
R6이 인다닐, 1,2,3,4-테트라히드로나프탈레닐, 페닐, 나프틸, 2,3-디히드로벤조푸라닐, 2,3-디히드로-1,4-벤조디옥시닐, 티에닐, 피리디닐, 인돌릴, 벤조푸라닐, 벤조티오페닐 또는 페녹시이고,
여기서 R6 치환기의 시클릭 또는 시클릭 모이어티는 동일하거나 상이할 수 있는 1 또는 2개의 R6S 치환기로 치환될 수 있고,
R6S는 할로겐, 시아노, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C2-C4-알키닐, C1-C4-할로알킬술파닐, C3-C5-시클로알킬, 피리디닐, 옥세타닐 및 테트라히드로푸라닐로 이루어진 군으로부터 선택되고,
R7이 할로겐, 시아노, C1-C4-알킬, C1-C4-할로알킬, C1-C4-히드록시알킬, C1-C4-알콕시, C1-C4-알킬카르보닐, C3-C6-시클로알킬, 이미다졸릴, 피라졸릴, 티아졸릴 및 피리디닐로 이루어진 군으로부터 선택되고,
여기서 지방족 R7 치환기는 히드록실, 메톡시, 에톡시 및 시클로프로필로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 R7Sa 치환기로 치환될 수 있고,
여기서 R7 치환기의 시클릭 또는 시클릭 모이어티는 플루오린, 메틸, 에틸 및 시클로프로필로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 R7Sc 치환기로 치환될 수 있고,
R8이 수소, 할로겐, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C3-C6-시클로알킬옥시 및 -N(Rh)2로 이루어진 군으로부터 선택되고,
여기서 Rh는 독립적으로 수소, C1-C4-알킬, C1-C4-할로알킬, C2-C4-알케닐, 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 R8 및 Rh 치환기는 히드록실, 메톡시 및 에톡시로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 R8Sa 치환기로 치환될 수 있고,
여기서 R8의 시클릭 또는 시클릭 모이어티 및 시클릭 Rh 치환기는 플루오린, 메틸, 에틸 및 시클로프로필로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 R8Sc 치환기로 치환될 수 있고,
Q가 페닐, 3-비시클로[4.2.0]옥타-1,3,5-트리에닐, 피라졸릴, 티아졸릴, 티에닐 및 피리디닐로 이루어진 군으로부터 선택되고,
여기서 임의의 상기 카르보사이클 또는 헤테로사이클 기는 동일하거나 상이할 수 있는 1 내지 3개의 QS 치환기로 치환될 수 있고,
QS는 할로겐, 시아노, 니트로, 포르밀, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C2-C4-알키닐, C1-C4-알킬술파닐 C3-C5-시클로알킬, 옥시라닐 및 옥세타닐로 이루어진 군으로부터 선택되는 것인
화학식 (I)의 화합물이다.
보다 더 바람직한 실시양태에서, 본 발명에 따른 화합물은
A가 O이고,
m이 1이고;
T가 수소이고,
R3 및 R4가 수소이고,
R5가 수소이고,
L이 메틸렌이고,
R6이 2,4-디메틸페닐, 2-메틸-4-브로모페닐 또는 2-클로로-4-메틸페닐이고,
R7이 메틸이고,
R8이 수소이고,
Q가 2-플루오로-3-클로로페닐, 2-플루오로-3-브로모페닐 또는 2-플루오로-3-시클로프로필페닐인
화학식 (I)의 화합물이다.
본 발명에 따른 보다 더 바람직한 화합물 조합물은 (A) (I-052) rac-3-[3-(3-시클로프로필-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-130) (5S)-3-[3-(3-시클로프로필-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2,4-디메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진, (I-300) rac-5-[(4-브로모-2-메틸페닐)메틸]-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-302) rac-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-[(2-클로로-4-메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-337) (5S)-5-[(4-브로모-2-메틸페닐)메틸]-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-338) (5R)-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2-클로로-4-메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진 및 (I-339) (5S)-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2-클로로-4-메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진으로 이루어진 군으로부터 선택된 화학식 (I)의 화합물을 포함한다.
마찬가지로 보다 더 바람직한 본 발명에 따른 화합물 조합물은 (A) (I-052) rac-3-[3-(3-시클로프로필-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-130) (5S)-3-[3-(3-시클로프로필-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2,4-디메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진, (I-300) rac-5-[(4-브로모-2-메틸페닐)메틸]-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-302) rac-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-[(2-클로로-4-메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-337) (5S)-5-[(4-브로모-2-메틸페닐)메틸]-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 및 (I-339) (5S)-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2-클로로-4-메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진으로 이루어진 군으로부터 선택된 화학식 (I)의 화합물을 포함한다.
마찬가지로 본 발명에 따른 가장 바람직한 화합물 조합물은 (A) (I-052) rac-3-[3-(3-시클로프로필-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-300) rac-5-[(4-브로모-2-메틸페닐)메틸]-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 및 (I-302) rac-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-[(2-클로로-4-메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진으로 이루어진 군으로부터 선택된 화학식 (I)의 화합물을 포함한다.
마찬가지로 가장 바람직한 본 발명에 따른 화합물 조합물은 (A) (I-130) (5S)-3-[3-(3-시클로프로필-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2,4-디메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진, (I-337) (5S)-5-[(4-브로모-2-메틸페닐)메틸]-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 및 (I-339) (5S)-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2-클로로-4-메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진으로 이루어진 군으로부터 선택된 화학식 (I)의 화합물을 포함한다.
본 발명에 따른 가장 바람직한 화합물 조합물은 (A) (I-302) rac-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-[(2-클로로-4-메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-338) (5R)-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2-클로로-4-메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진 및 (I-339) (5S)-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2-클로로-4-메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진으로 이루어진 군으로부터 선택된 화학식 (I)의 화합물을 포함한다.
본 발명에 따른 특히 바람직한 화합물 조합물은 (A) (I-339) (5S)-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2-클로로-4-메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진인 화학식 (I)의 화합물을 포함한다.
정의
본원에 사용된 용어 "할로겐"은 플루오린, 염소, 브로민 또는 아이오딘 원자를 지칭한다.
본원에 사용된 용어 "메틸리덴"은 이중 결합을 통해 탄소 원자에 연결된 CH2 기를 지칭한다.
본원에 사용된 용어 "할로메틸리덴"은 X가 할로겐인 이중 결합을 통해 탄소 원자에 연결된 CX2 기를 지칭한다.
본원에 사용된 용어 "옥소"는 이중 결합을 통해 탄소 원자 또는 황 원자에 결합된 산소 원자를 지칭한다.
본원에 사용된 용어 "포르밀"은 -CH(=O)를 지칭한다.
본원에 사용된 용어 "C1-C6-알킬"은 1, 2, 3, 4, 5 또는 6개의 탄소 원자를 갖는 포화, 분지형 또는 직쇄 탄화수소 쇄를 지칭한다. C1-C6-알킬의 예는 메틸, 에틸, 프로필 (n-프로필), 1-메틸에틸 (이소-프로필), 부틸 (n-부틸), 1-메틸프로필 (sec-부틸), 2-메틸프로필 (이소-부틸), 1,1-디메틸에틸 (tert-부틸), 펜틸, 1-메틸부틸, 2-메틸부틸, 3-메틸부틸, 2,2-디메틸프로필, 1-에틸프로필, 1,1-디메틸프로필, 1,2-디메틸프로필, 헥실, 1-메틸펜틸, 2-메틸펜틸, 3-메틸펜틸, 4-메틸펜틸, 1,1-디메틸부틸, 1,2-디메틸부틸, 1,3-디메틸부틸, 2,2-디메틸부틸, 2,3-디메틸부틸, 3,3-디메틸부틸, 1-에틸부틸, 2-에틸부틸, 1,1,2-트리메틸프로필, 1,2,2-트리메틸프로필, 1-에틸-1-메틸프로필 및 1-에틸-2-메틸프로필을 포함하나, 이에 제한되지는 않는다. 특히, 상기 탄화수소 쇄는 1, 2, 3 또는 4개의 탄소 원자 ("C1-C4-알킬"), 예를 들어 메틸, 에틸, 프로필, 이소-프로필, 부틸, sec-부틸, 이소-부틸 또는 tert-부틸을 갖는다.
본원에 사용된 용어 "C1-C6-알킬렌"은 본원에 정의된 바와 같은 2가 C1-C6-알킬 기를 지칭한다. C1-C6-알킬렌의 예는 -CH2-, -CH2-CH2-, -CH2-CH2-CH2-, -CH2-C(CH3)-CH2-, -CH2-CH2-CH2-CH2-, -CH2-C(CH3)-CH2-CH2-, -CH2-CH2-CH2-CH2-CH2- 및 -CH2-CH2-CH2-CH2-CH2-CH2-를 포함하나 이에 제한되지는 않는다.
본원에 사용된 용어 "C2-C6-알케닐" 또는 "알칸디일"은 2, 3, 4, 5 또는 6개의 탄소 원자를 갖고 적어도 1개의 이중 결합을 포함하는 불포화, 분지형 또는 직쇄형 탄화수소 쇄를 지칭한다. C2-C6-알케닐의 예는 에테닐 (또는 "비닐"), 프로프-2-엔-1-일 (또는 "알릴"), 프로프-1-엔-1-일, 부트-3-에닐, 부트-2-에닐, 부트-1-에닐, 펜트-4-에닐, 펜트-3-에닐, 펜트-2-에닐, 펜트-1-에닐, 헥스-5-에닐, 헥스-4-에닐, 헥스-3-에닐, 헥스-2-에닐, 헥스-1-에닐, 프로프-1-엔-2-일 (또는 "이소프로페닐"), 2-메틸프로프-2-에닐, 1-메틸프로프-2-에닐, 2-메틸프로프-1-에닐, 1-메틸프로프-1-에닐, 3-메틸부트-3-에닐, 2-메틸부트-3-에닐, 1-메틸부트-3-에닐, 3-메틸부트-2-에닐, 2-메틸부트-2-에닐, 1-메틸부트-2-에닐, 3-메틸부트-1-에닐, 2-메틸부트-1-에닐, 1-메틸부트-1-에닐, 1,1-디메틸프로프-2-에닐, 1-에틸프로프-1-에닐, 1-프로필비닐, 1-이소프로필비닐, 4-메틸펜트-4-에닐, 3-메틸펜트-4-에닐, 2-메틸펜트-4-에닐, 1-메틸펜트-4-에닐, 4-메틸펜트-3-에닐, 3-메틸펜트-3-에닐, 2-메틸펜트-3-에닐, 1-메틸펜트-3-에닐, 4-메틸펜트-2-에닐, 3-메틸펜트-2-에닐, 2-메틸펜트-2-에닐, 1-메틸펜트-2-에닐, 4-메틸펜트-1-에닐, 3-메틸펜트-1-에닐, 2-메틸펜트-1-에닐, 1-메틸펜트-1-에닐, 3-에틸부트-3-에닐, 2-에틸부트-3-에닐, 1-에틸부트-3-에닐, 3-에틸부트-2-에닐, 2-에틸부트-2-에닐, 1-에틸부트-2-에닐, 3-에틸부트-1-에닐, 2-에틸부트-1-에닐, 1-에틸부트-1-에닐, 2-프로필프로프-2-에닐, 1-프로필프로프-2-에닐, 2-이소프로필프로프-2-에닐, 1-이소프로필프로프-2-에닐, 2-프로필프로프-1-에닐, 1-프로필프로프-1-에닐, 2-이소프로필프로프-1-에닐, 1-이소프로필프로프-1-에닐, 3,3-디메틸프로프-1-에닐, 1-(1,1-디메틸에틸)에테닐, 부타-1,3-디에닐, 펜타-1,4-디에닐, 헥사-1,5-디에닐 또는 메틸헥사디에닐 기를 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "C2-C6-알케닐렌"은 본원에 정의된 바와 같은 2가 C2-C6-알케닐 기를 지칭한다. C2-C6-알케닐렌의 예는 에테닐렌, 프로페닐렌, 부테닐렌, 펜테닐렌, 헥세닐렌, 헵테닐렌, 옥테닐렌, 노네닐렌, 데세닐렌, 운데세닐렌, 도데세닐렌 등을 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "C2-C6-알키닐"은 2, 3, 4, 5 또는 6개의 탄소 원자를 갖고 적어도 1개의 삼중 결합을 포함하는 분지형 또는 직쇄형 탄화수소 쇄를 지칭한다. C2-C6-알키닐의 예는 에티닐, 프로프-1-이닐, 프로프-2-이닐 (또는 "프로파르길"), 부트-1-이닐, 부트-2-이닐, 부트-3-이닐, 펜트-1-이닐, 펜트-2-이닐, 펜트-3-이닐, 펜트-4-이닐, 헥스-1-이닐, 헥스-2-이닐, 헥스-3-이닐, 헥스-4-이닐, 헥스-5-이닐, 1-메틸프로프-2-이닐, 2-메틸부트-3-이닐, 1-메틸부트-3-이닐, 1-메틸부트-2-이닐, 3-메틸부트-1-이닐, 1-에틸프로프-2-이닐, 3-메틸펜트-4-이닐, 2-메틸펜트-4-이닐, 1-메틸펜트-4-이닐, 2-메틸펜트-3-이닐, 1-메틸펜트-3-이닐, 4-메틸펜트-2-이닐, 1-메틸펜트-2-이닐, 4-메틸펜트-1-이닐, 3-메틸펜트-1-이닐, 2-에틸부트-3-이닐, 1-에틸부트-3-이닐, 1-에틸부트-2-이닐, 1-프로필프로프-2-이닐, 1-이소프로필프로프-2-이닐, 2,2-디메틸부트-3-이닐, 1,1-디메틸부트-3-이닐, 1,1-디메틸부트-2-이닐 또는 3,3-디메틸부트-1-이닐 기를 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "C2-C6-알키닐렌"은 본원에 정의된 바와 같은 2가 C2-C6-알키닐 기를 지칭한다.
본원에 사용된 용어 "C1-C6-할로알킬"은 1개 이상의 수소 원자가 동일하거나 상이할 수 있는 1개 이상의 할로겐 원자로 대체된 상기 정의된 바와 같은 C1-C6-알킬 기를 지칭한다.
본원에 사용된 용어 "C2-C6-할로알케닐"은 1개 이상의 수소 원자가 동일하거나 상이할 수 있는 1개 이상의 할로겐 원자로 대체된 상기 정의된 바와 같은 C2-C6-알케닐 기를 지칭한다.
본원에 사용된 용어 "C2-C6-할로알키닐"은 1개 이상의 수소 원자가 동일하거나 상이할 수 있는 1개 이상의 할로겐 원자로 대체된 상기 정의된 바와 같은 C2-C6-알키닐 기를 지칭한다.
본원에 사용된 용어 "C1-C6-알콕시"는 화학식 (C1-C6-알킬)-O-의 기를 지칭하며, 여기서 용어 "C1-C6-알킬"은 본원에 정의된 바와 같다. C1-C6-알콕시의 예는 메톡시, 에톡시, n-프로폭시, 1-메틸에톡시, n-부톡시, 1-메틸프로폭시, 2-메틸프로폭시, 1,1-디메틸에톡시, n-펜톡시, 1-메틸부톡시, 2-메틸부톡시, 3-메틸부톡시, 2,2-디메틸프로폭시, 1-에틸프로폭시, 1,1-디메틸프로폭시, 1,2-디메틸프로폭시, n-헥실옥시, 1-메틸펜톡시, 2-메틸펜톡시, 3-메틸펜톡시, 4-메틸펜톡시, 1,1-디메틸부톡시, 1,2-디메틸부톡시, 1,3-디메틸부톡시, 2,2-디메틸부톡시, 2,3-디메틸부톡시, 3,3-디메틸부톡시, 1-에틸부톡시, 2-에틸부톡시, 1,1,2-트리메틸프로폭시, 1,2,2-트리메틸프로폭시, 1-에틸-1-메틸프로폭시 및 1-에틸-2-메틸프로폭시를 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "C1-C6-할로알콕시"는 1개 이상의 수소 원자가 동일하거나 상이할 수 있는 1개 이상의 할로겐 원자로 대체된 상기 정의된 바와 같은 C1-C6-알콕시 기를 지칭한다. C1-C6-할로알콕시의 예는 클로로메톡시, 브로모메톡시, 디클로로메톡시, 트리클로로메톡시, 플루오로메톡시, 디플루오로메톡시, 트리플루오로메톡시, 클로로플루오로메톡시, 디클로로플루오로메톡시, 클로로디플루오로메톡시, 1-클로로에톡시, 1-브로모에톡시, 1-플루오로에톡시, 2-플루오로에톡시, 2,2-디플루오로에톡시, 2,2,2-트리플루오로에톡시, 2-클로로-2-플루오로에톡시, 2-클로로-2,2-디플루오로에톡시, 2,2-디클로로-2-플루오로에톡시, 2,2,2-트리클로로에톡시, 펜타플루오로에톡시 및 1,1,1-트리플루오로프로프-2-옥시를 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "C1-C6-할로알콕시"는 1개 이상의 수소 원자가 동일하거나 상이할 수 있는 1개 이상의 할로겐 원자로 대체된 상기 정의된 바와 같은 C1-C6-알콕시 기를 지칭한다.
본원에 사용된 용어 "C1-C6-히드록시알킬"은 적어도 1개의 수소 원자가 히드록실 기로 대체된 상기 정의된 바와 같은 C1-C6-알킬 기를 지칭한다. C1-C6-히드록시알킬의 예는 히드록시메틸, 1-히드록시에틸, 2-히드록시에틸, 1,2-디히드록시에틸, 3-히드록시프로필, 2-히드록시프로필, 1-히드록시프로필, 1-히드록시프로판-2-일, 2-히드록시프로판-2-일, 2,3-디히드록시프로필 및 1,3-디히드록시프로판-2-일을 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "C1-C6-알킬술파닐"은 화학식 (C1-C6-알킬)-S-의 포화, 선형 또는 분지형 기를 지칭하며, 여기서 용어 "C1-C6-알킬"은 본원에 정의된 바와 같다. C1-C6-알킬술파닐의 예는 메틸술파닐, 에틸술파닐, 프로필술파닐, 이소프로필술파닐, 부틸술파닐, sec-부틸술파닐, 이소부틸술파닐, tert-부틸술파닐, 펜틸술파닐, 이소펜틸술파닐, 헥실술파닐 기를 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "C1-C6-할로알킬술파닐"은 1개 이상의 수소 원자가 동일하거나 상이할 수 있는 1개 이상의 할로겐 원자로 대체된 상기 정의된 바와 같은 C1-C6-알킬술파닐을 지칭한다.
본원에 사용된 용어 "C1-C6-알킬술피닐"은 화학식 (C1-C6-알킬)-S(=O)-의 포화, 선형 또는 분지형 기를 지칭하며, 여기서 용어 "C1-C6-알킬"은 본원에 정의된 바와 같다. C1-C6-알킬술피닐의 예는 1 내지 8개, 바람직하게는 1 내지 6개, 보다 바람직하게는 1 내지 4개의 탄소 원자를 갖는 포화, 직쇄 또는 분지형 알킬술피닐 라디칼, 예를 들어 (비제한적으로) C1-C6-알킬술피닐, 예컨대 메틸술피닐, 에틸술피닐, 프로필술피닐, 1-메틸에틸술피닐, 부틸술피닐, 1-메틸프로필술피닐, 2-메틸프로필술피닐, 1,1-디메틸에틸술피닐, 펜틸술피닐, 1-메틸부틸술피닐, 2-메틸부틸술피닐, 3-메틸부틸술피닐, 2,2-디메틸프로필술피닐, 1-에틸프로필술피닐, 1,1-디메틸프로필술피닐, 1,2-디메틸프로필술피닐, 헥실술피닐, 1-메틸펜틸술피닐, 2-메틸펜틸술피닐, 3-메틸펜틸술피닐, 4-메틸펜틸술피닐, 1,1-디메틸부틸술피닐, 1,2-디메틸부틸술피닐, 1,3-디메틸부틸술피닐, 2,2-디메틸부틸술피닐, 2,3-디메틸부틸술피닐, 3,3-디메틸부틸술피닐, 1-에틸부틸술피닐, 2-에틸부틸술피닐, 1,1,2-트리메틸프로필술피닐, 1,2,2-트리메틸프로필술피닐, 1-에틸-1-메틸프로필술피닐 및 1-에틸-2-메틸프로필술피닐을 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "C1-C6-할로알킬술피닐"은 1개 이상의 수소 원자가 동일하거나 상이할 수 있는 1개 이상의 할로겐 원자로 대체된 상기 정의된 바와 같은 C1-C6-알킬술피닐을 지칭한다.
본원에 사용된 용어 "C1-C6-알킬술포닐"은 화학식 (C1-C6-알킬)-S(=O)2-의 포화, 선형 또는 분지형 기를 지칭하며, 여기서 용어 "C1-C6-알킬"은 본원에 정의된 바와 같다. C1-C6-알킬술포닐의 예는 메틸술포닐, 에틸술포닐, 프로필술포닐, 1-메틸에틸술포닐, 부틸술포닐, 1-메틸프로필술포닐, 2-메틸프로필술포닐, 1,1-디메틸에틸술포닐, 펜틸술포닐, 1-메틸부틸술포닐, 2-메틸부틸술포닐, 3-메틸부틸술포닐, 2,2-디메틸프로필술포닐, 1-에틸프로필술포닐, 1,1-디메틸프로필술포닐, 1,2-디메틸프로필술포닐, 헥실술포닐, 1-메틸펜틸술포닐, 2-메틸펜틸술포닐, 3-메틸펜틸술포닐, 4-메틸펜틸술포닐, 1,1-디메틸부틸술포닐, 1,2-디메틸부틸술포닐, 1,3-디메틸부틸술포닐, 2,2-디메틸부틸술포닐, 2,3-디메틸부틸술포닐, 3,3-디메틸부틸술포닐, 1-에틸부틸술포닐, 2-에틸부틸술포닐, 1,1,2-트리메틸프로필술포닐, 1,2,2-트리메틸프로필술포닐, 1-에틸-1-메틸프로필술포닐 및 1-에틸-2-메틸프로필술포닐을 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "C1-C6-할로알킬술포닐"은 1개 이상의 수소 원자가 동일하거나 상이할 수 있는 1개 이상의 할로겐 원자로 대체된 상기 정의된 바와 같은 C1-C6-알킬술포닐을 지칭한다.
본원에 사용된 용어 "C1-C6-알킬카르보닐"은 화학식 (C1-C6-알킬)-C(=O)-의 포화, 선형 또는 분지형 기를 지칭하며, 여기서 용어 "C1-C6-알킬"은 본원에 정의된 바와 같다.
본원에 사용된 용어 "C1-C6-할로알킬카르보닐"은 1개 이상의 수소 원자가 동일하거나 상이할 수 있는 1개 이상의 할로겐 원자로 대체된 상기 정의된 바와 같은 C1-C6-알킬카르보닐을 지칭한다.
본원에 사용된 용어 "C1-C6-알콕시카르보닐"은 화학식 (C1-C6-알콕시)-C(=O)-의 포화, 선형 또는 분지형 기를 지칭하며, 여기서 용어 "C1-C6-알콕시"는 본원에 정의된 바와 같다.
본원에 사용된 용어 "C1-C6-할로알콕시카르보닐"은 1개 이상의 수소 원자가 동일하거나 상이할 수 있는 1개 이상의 할로겐 원자로 대체된 상기 정의된 바와 같은 C1-C6-알콕시카르보닐을 지칭한다.
본원에 사용된 용어 "C1-C6-디알킬아미노"는 본원에 정의된 바와 같은 2개의 독립적으로 선택된 C1-C6-알킬 기를 갖는 아미노 라디칼을 지칭한다. C1-C6-디알킬아미노의 예는 N,N-디메틸아미노, N,N-디에틸아미노, N,N-디이소프로필아미노, N-에틸-N-메틸아미노, N-메틸-N-n-프로필아미노, N-이소프로필-N-n-프로필아미노 및 N-tert-부틸-N-메틸아미노를 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "비-방향족 C3-C12-카르보사이클"은 3 내지 12로 다양한 모든 고리원이 탄소 원자인 비-방향족, 포화 또는 불포화, 탄화수소 고리계를 지칭한다. 고리계는 모노시클릭 또는 폴리시클릭 (융합, 스피로 또는 가교)일 수 있다. 비-방향족 C3-C12-카르보사이클은 C3-C12-시클로알킬 (모노 또는 비시클릭), C3-C12-시클로알케닐 (모노 또는 비시클릭), 모노시클릭 C3-C8-시클로알킬 (예를 들어 테트라히드로나프탈레닐, 인다닐)에 융합된 아릴 (예를 들어 페닐)을 포함하는 비시클릭 시스템, 모노시클릭 C3-C8-시클로알케닐 (예를 들어 인데닐, 디히드로나프탈레닐)에 융합된 아릴 (예를 들어 페닐)을 포함하는 비시클릭 시스템, 및 모노시클릭 C3-C8-시클로알킬 또는 모노시클릭 C3-C8-시클로알케닐에 융합된 아릴 (예를 들어 페닐)을 포함하는 비시클릭 시스템에 1개의 탄소 원자를 통해 연결된 시클로프로필을 포함하는 트리시클릭 시스템을 포함하나, 이에 제한되지는 않는다. 비-방향족 C3-C12-카르보사이클은 임의의 탄소 원자를 통해 모 분자 모이어티에 부착될 수 있다.
본원에 사용된 용어 "C3-C12-시클로알킬"은 3, 4, 5, 6, 7, 8, 9, 10, 11 또는 12개의 탄소 원자를 함유하는 포화, 1가, 모노- 또는 비시클릭 탄화수소 고리를 지칭한다. 모노시클릭 C3-C8-시클로알킬의 예는 시클로프로필, 시클로부틸, 시클로펜틸, 시클로헥실, 시클로헵틸 또는 시클로옥틸을 포함하나, 이에 제한되지는 않는다. 비시클릭 C6-C12-시클로알킬의 예는 비시클로[3.1.1]헵탄, 비시클로[2.2.1]헵탄, 비시클로[2.2.2]옥탄, 비시클로[3.2.2]노난, 비시클로[3.3.1]노난, 비시클로[4.2.0]옥틸, 옥타히드로펜탈레닐 및 비시클로[4.2.1]노난을 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "C3-C12-시클로알킬렌"은 본원에 정의된 바와 같은 2가 C3-C12-시클로알킬 기, 예컨대 시클로프로필렌, 시클로부틸렌, 시클로펜틸렌, 시클로헥실렌, 시클로헵틸렌 및 비시클로[2.2.1]헵트-2-일렌을 지칭한다.
본원에 사용된 용어 "C3-C12-시클로알케닐"은 3, 4, 5, 6, 7, 8, 9, 10, 11 또는 12개의 탄소 원자를 함유하는 불포화, 1가, 모노- 또는 비시클릭 탄화수소 고리를 지칭한다. 모노시클릭 C3-C8-시클로알케닐 기의 예는 시클로부테닐, 시클로펜테닐, 시클로헥세닐, 시클로헵테닐 및 시클로옥테닐 기를 포함하나, 이에 제한되지는 않는다. 비시클릭 C6-C12-시클로알케닐 기의 예는 비시클로[2.2.1]헵트-2-에닐 또는 비시클로[2.2.2]옥트-2-에닐을 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "C3-C12-시클로알케닐렌"은 본원에 개시된 바와 같은 2가 C3-C12-시클로알케닐을 지칭한다.
본원에 사용된 용어 "방향족 C6-C14-카르보사이클" 또는 "아릴"은 6 내지 14, 바람직하게는 6 내지 10으로 다양한 모든 고리원이 탄소 원자인 방향족 탄화수소 고리계를 지칭한다. 고리계는 모노시클릭 또는 융합된 폴리시클릭 (예를 들어 비시클릭 또는 트리시클릭)일 수 있다. 아릴의 예는 페닐, 아줄레닐 및 나프틸을 포함하나, 이에 제한되지는 않는다. 아릴은 임의의 탄소 원자를 통해 모 분자 모이어티에 부착될 수 있다. 상기 아릴 기가 1개 이상의 치환기로 치환되는 경우에, 상기 치환기(들)는 상기 아릴 고리(들) 상의 임의의 위치에 있을 수 있는 것으로 추가로 이해된다. 특히, 아릴이 페닐 기인 경우에, 상기 치환기(들)는 하나 또는 둘 다의 오르토 위치, 하나 또는 둘 다의 메타 위치, 또는 파라 위치, 또는 이들 위치의 임의의 조합을 점유할 수 있다.
본원에 사용된 용어 "비-방향족 3- 내지 14-원 헤테로사이클"은 산소, 질소 및 황으로 이루어진 군으로부터 독립적으로 선택된 1 내지 4개의 헤테로원자를 포함하는 포화 또는 불포화 비-방향족 고리계를 지칭한다. 고리계가 1개 초과의 산소 원자를 함유하는 경우에, 이들은 직접 인접하지 않는다. 비 방향족 헤테로사이클은 3- 내지 7-원 모노시클릭 비-방향족 헤테로사이클 및 6- 내지 14-원 폴리시클릭 (예를 들어 비시클릭 또는 트리시클릭) 비-방향족 헤테로사이클을 포함하나, 이에 제한되지는 않는다. 비-방향족 3- 내지 14-원 헤테로사이클은 헤테로사이클 내에 함유된 임의의 탄소 원자 또는 질소 원자를 통해 모 분자 모이어티에 연결될 수 있다.
본원에 사용된 용어 "비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클"은 산소, 질소 및 황으로 이루어진 군으로부터 독립적으로 선택된 1, 2 또는 3개의 헤테로원자를 함유하는 3-, 4-, 5-, 6- 또는 7-원 모노시클릭 고리계를 지칭하며, 여기서 고리계는 포화 또는 불포화이지만 방향족은 아니다. 예를 들어, 헤테로사이클은 1 내지 3개의 질소 원자, 또는 1 또는 2개의 산소 원자, 또는 1 또는 2개의 황 원자, 또는 1 내지 3개의 질소 원자 및 1개의 산소 원자, 또는 1 내지 3개의 질소 원자 및 1개의 황 원자 또는 1개의 황 원자 및 1개의 산소 원자를 포함할 수 있다. 포화 비-방향족 헤테로사이클의 예는 3-원 고리 예컨대 옥시라닐, 아지리디닐, 4-원 고리 예컨대 아제티디닐, 옥세타닐, 티에타닐, 5-원 고리 예컨대 테트라히드로푸라닐, 1,3-디옥솔라닐, 테트라히드로티에닐, 피롤리디닐, 피라졸리디닐, 이미다졸리디닐, 트리아졸리디닐, 이속사졸리디닐, 옥사졸리디닐, 옥사디아졸리디닐, 티아졸리디닐, 이소티아졸리디닐, 티아디아졸리디닐, 6-원 고리 예컨대 피페리디닐, 헥사히드로피리다지닐, 헥사히드로피리미디닐, 피페라지닐, 트리아지나닐, 헥사히드로트리아지닐, 테트라히드로피라닐, 디옥사닐, 테트라히드로티오피라닐, 디티아닐, 모르폴리닐, 1,2-옥사지나닐, 옥사티아닐, 티오모르폴리닐 또는 7-원 고리 예컨대 옥세파닐, 아제파닐, 1,4-디아제파닐 및 1,4-옥사제파닐을 포함하나, 이에 제한되지는 않는다. 불포화 비-방향족 헤테로시클릴의 예는 5-원 고리, 예컨대 디히드로푸라닐, 1,3-디옥솔릴, 디히드로티에닐, 피롤리닐, 디히드로이미다졸릴, 디히드로피라졸릴, 이속사졸리닐, 디히드로옥사졸릴, 디히드로티아졸릴 또는 6-원 고리 예컨대 피라닐, 티오피라닐, 티아지닐 및 티아디아지닐을 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "비-방향족 6- 내지 14-원 폴리시클릭 헤테로사이클"은 산소, 질소 및 황으로 이루어진 군으로부터 독립적으로 선택된 1, 2 또는 3개의 헤테로원자를 함유하는 6-, 7-, 8-, 9-, 10-, 11-, 12-, 13- 또는 14-원 폴리시클릭 (예를 들어 비시클릭 또는 트리시클릭) 고리계를 지칭하며, 여기서 고리계는 포화 또는 불포화이지만 방향족은 아니다. 비-방향족 비시클릭 헤테로사이클은 모노시클릭 C3-C8-시클로알킬, 모노시클릭 C3-C8-시클로알케닐 또는 모노시클릭 비-방향족 헤테로사이클에 융합된 본원에 정의된 바와 같은 모노시클릭 헤테로아릴로 이루어질 수 있거나, 또는 아릴 (예를 들어 페닐), 모노시클릭 C3-C8-시클로알킬, 모노시클릭 C3-C8-시클로알케닐 또는 모노시클릭 비-방향족 헤테로사이클에 융합된 모노시클릭 비-방향족 헤테로사이클로 이루어질 수 있다. 질소 원자를 포함하는 2개의 모노시클릭 헤테로사이클 (방향족 또는 비-방향족)이 융합되는 경우에, 질소 원자는 브리지헤드에 존재할 수 있다 (예를 들어 4,5,6,7-테트라히드로피라졸로[1,5-a]피리디닐, 5,6,7,8-테트라히드로-[1,2,4]트리아졸로[1,5-a]피리디닐, 5,6,7,8-테트라히드로이미다조[1,2-a]피리디닐). 비-방향족 트리시클릭 헤테로사이클은 1개의 공통 원자를 통해 비-방향족 비시클릭 헤테로사이클에 연결된 모노시클릭 시클로알킬로 이루어질 수 있다.
본원에 사용된 용어 "비-방향족 3- 내지 7-원 모노시클릭 헤테로시클릴렌"은 본원에 개시된 바와 같은 2가 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 지칭한다.
본원에 사용된 용어 "방향족 5- 내지 14-원 헤테로사이클" 또는 "헤테로아릴"은 산소, 질소 및 황으로 이루어진 군으로부터 독립적으로 선택된 1 내지 4개의 헤테로원자를 포함하는 방향족 고리계를 지칭한다. 고리계가 1개 초과의 산소 원자를 함유하는 경우에, 이들은 직접 인접하지 않는다. 방향족 헤테로사이클은 방향족 5- 또는 6-원 모노시클릭 헤테로사이클 및 6- 내지 14-원 폴리시클릭 (예를 들어 비시클릭 또는 트리시클릭) 방향족 헤테로사이클을 포함한다. 5- 내지 14-원 방향족 헤테로사이클은 헤테로사이클 내에 함유된 임의의 탄소 원자 또는 질소 원자를 통해 모 분자 모이어티에 연결될 수 있다.
본원에 사용된 용어 "방향족 5- 또는 6-원 모노시클릭 헤테로사이클" 또는 "모노시클릭 헤테로아릴"은 산소, 질소 및 황으로 이루어진 군으로부터 독립적으로 선택된 1, 2, 3 또는 4개의 헤테로원자를 함유하는 5- 또는 6-원 모노시클릭 고리계를 지칭한다. 5-원 모노시클릭 헤테로아릴의 예는 푸릴 (푸라닐), 티에닐, 피롤릴, 피라졸릴, 이미다졸릴, 트리아졸릴, 테트라졸릴, 이속사졸릴, 옥사졸릴, 옥사디아졸릴, 옥사트리아졸릴, 이소티아졸릴, 티아졸릴, 티아디아졸릴 및 티아트리아졸릴을 포함하나, 이에 제한되지는 않는다. 6-원 모노시클릭 헤테로아릴의 예는 피리디닐, 피리다지닐, 피리미디닐, 피라지닐, 트리아지닐, 테트라지닐을 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "6- 내지 14-원 폴리시클릭 방향족 헤테로사이클" 또는 "폴리시클릭 헤테로아릴"은 산소, 질소 및 황으로 이루어진 군으로부터 독립적으로 선택된 1, 2 또는 3개의 헤테로원자를 함유하는 6-, 7-, 8-, 9-, 10-, 11-,12-, 13- 또는 14-원 폴리시클릭 (예를 들어 비시클릭 또는 트리시클릭) 고리계를 지칭한다. 방향족 비시클릭 헤테로사이클은 아릴 (예를 들어 페닐) 또는 모노시클릭 헤테로아릴에 융합된 본원에 정의된 바와 같은 모노시클릭 헤테로아릴로 이루어질 수 있다. 비시클릭 방향족 헤테로사이클의 예는 9-원 고리, 예컨대 인돌릴, 인돌리지닐, 이소인돌릴, 벤즈이미다졸릴, 이미다조피리디닐, 인다졸릴, 벤조트리아졸릴, 퓨리닐, 벤조푸라닐, 벤조티오페닐, 벤조티아졸릴, 벤족사졸릴 및 벤즈이속사졸릴 또는 10-원 고리, 예컨대 퀴놀리닐, 이소퀴놀리닐, 신놀리닐, 퀴나졸리닐, 퀴녹살리닐, 프탈라지닐, 나프티리디닐, 프테리디날 및 벤조디옥시닐을 포함하나, 이에 제한되지는 않는다. 2개의 융합된 5- 또는 6-원 모노시클릭 방향족 헤테로사이클을 포함하는 9- 또는 10-원 방향족 비시클릭 헤테로사이클에서, 질소 원자는 브리지헤드에 존재할 수 있다 (예를 들어 이미다조[1,2-a]피리디닐,[1,2,4]트리아졸로[4,3-a]피리디닐, 이미다조[1,2-a]피리디닐, 이미다조[2,1-b]옥사졸릴, 푸로[2,3-d]이속사졸릴). 트리시클릭 방향족 헤테로사이클의 예는 카르바졸릴, 아크리디닐 및 페나지닐을 포함하나, 이에 제한되지는 않는다.
본원에 사용된 용어 "비-방향족 C3-C12-카르보시클릴옥시", "C3-C8-시클로알킬옥시", "방향족 C6-C14-카르보시클릴옥시", "방향족 5- 내지 14-원 헤테로시클릴옥시", "비-방향족 5- 내지 14-원 헤테로시클릴옥시"는 R이 각각 본원에 정의된 바와 같은 비-방향족 C3-C12-카르보시클릴, C3-C8-시클로알킬, 방향족 C6-C14-카르보시클릴, 방향족 5- 내지 14-원 헤테로시클릴 또는 비-방향족 5- 내지 14-원 헤테로시클릴 기인 화학식 -O-R의 기를 지정한다.
본원에 사용된 바와 같이, 기가 "치환된" 것으로 언급되는 경우에, 기는 1개 이상의 치환기로 치환될 수 있다. 표현 "1개 이상의 치환기"는 안정성 및 화학적 실행가능성의 조건이 충족되는 한, 이용가능한 결합 부위의 수에 기초하여 가능한 치환기의 1 내지 최대 수의 범위인 치환기의 수를 지칭한다.
본원에 사용된 용어 "이탈기"는 치환 또는 제거 반응에서 화합물로부터 대체되는 기, 예를 들어 할로겐 원자, 트리플루오로메탄술포네이트 ("트리플레이트") 기, 알콕시, 메탄술포네이트, p-톨루엔술포네이트 등을 의미하는 것으로 이해되어야 한다.
가변기 A, Q, L, m, T, R1, R2, R3, R4, R5, R6, R7, R8을 지칭하는 경우에 용어 "본원에 기재된 바와 같은"은 가변기의 광범위한 정의 뿐만 아니라 존재하는 경우에 바람직한, 보다 바람직한 및 보다 더 바람직한 정의를 참조로 포함한다.
자연 법칙에 반하는 조합으로부터 생성된 화합물은 본원에 포괄되지 않으며, 따라서 관련 기술분야의 통상의 기술자는 그의 전문 지식에 기초하여 배제할 것이다. 예를 들어, 3개 이상의 인접한 산소 원자를 갖는 고리 구조는 제외된다.
화학식 (I)의 화합물은 적합하게는 그의 유리 형태, 염 형태, N-옥시드 형태 또는 용매화물 형태 (예를 들어, 수화물)일 수 있다.
치환기의 성질에 따라, 화학식 (I)의 화합물은 상이한 입체이성질체의 형태로 존재할 수 있다. 이들 입체이성질체는, 예를 들어 거울상이성질체, 부분입체이성질체, 회전장애이성질체 또는 기하 이성질체이다. 따라서, 본 발명은 순수한 입체이성질체 및 이들 이성질체의 임의의 혼합물 둘 다를 포괄한다. 화합물이 2종 이상의 호변이성질체 형태로 평형으로 존재할 수 있는 경우에, 하나의 호변이성질체 설명에 의한 화합물에 대한 언급은 모든 호변이성질체 형태를 포함하는 것으로 간주되어야 한다.
본 발명의 임의의 화합물은 또한 화합물 내의 이중 결합의 수에 따라 1개 이상의 기하 이성질체 형태로 존재할 수 있다. 이중 결합 또는 고리에 대한 치환기의 성질에 의한 기하 이성질체는 시스 (= Z-) 또는 트랜스 (= E-) 형태로 존재할 수 있다. 따라서, 본 발명은 동등하게 모든 비율의 모든 기하 이성질체 및 모든 가능한 혼합물에 관한 것이다.
치환기의 성질에 따라, 화학식 (I)의 화합물은 유리 화합물 및/또는 그의 염, 예컨대 농약 활성 염의 형태로 존재할 수 있다.
농약 활성 염은 무기 및 유기 산의 산 부가염 뿐만 아니라 통상의 염기의 염을 포함한다. 무기 산의 예는 할로겐화수소산, 예컨대 플루오린화수소, 염화수소, 브로민화수소 및 아이오딘화수소, 황산, 인산 및 질산, 및 산성 염, 예컨대 중황산나트륨 및 중황산칼륨이다. 유용한 유기 산은, 예를 들어 포름산, 탄산 및 알칸산 예컨대 아세트산, 트리플루오로아세트산, 트리클로로아세트산 및 프로피온산, 및 또한 글리콜산, 티오시안산, 락트산, 숙신산, 시트르산, 벤조산, 신남산, 옥살산, 6 내지 20개의 탄소 원자를 갖는 포화 또는 단일- 또는 이중불포화 지방산, 알킬황산 모노에스테르, 알킬술폰산 (1 내지 20개의 탄소 원자를 갖는 직쇄 또는 분지형 알킬 라디칼을 갖는 술폰산), 아릴술폰산 또는 아릴디술폰산 (1 또는 2개의 술폰산 기를 보유하는 방향족 라디칼, 예컨대 페닐 및 나프틸), 알킬포스폰산 (1 내지 20개의 탄소 원자를 갖는 직쇄 또는 분지형 알킬 라디칼을 갖는 포스폰산), 아릴포스폰산 또는 아릴디포스폰산 (1 또는 2개의 포스폰산 라디칼을 보유하는 방향족 라디칼, 예컨대 페닐 및 나프틸)을 포함하며, 여기서 알킬 및 아릴 라디칼은 추가의 치환기, 예를 들어 p-톨루엔술폰산, 살리실산, p-아미노살리실산, 2-페녹시벤조산, 2-아세톡시벤조산 등을 포함한다.
본 발명의 화합물 또는 그의 염의 용매화물은 화합물과 용매의 화학량론적 조성이다.
본 발명의 화합물은 다중 결정질 및/또는 무정형 형태로 존재할 수 있다. 결정질 형태는 비용매화 결정질 형태, 용매화물 및 수화물을 포함한다.
표현 "지방족 R1, R2, R3, R4 및 R5 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 R1 및 R2의 치환기는 C1-C6-알킬을 나타낸다.
표현 "지방족 R1, R2, R3, R4 및 R5 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 R3 및 R4 치환기는 C1-C6-알킬, C1-C6-알콕시, C1-C6-알콕시카르보닐 및 -Si(C1-C6-알킬)3의 C1-C6-알킬 모이어티를 나타낸다.
표현 "지방족 R1, R2, R3, R4 및 R5 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 R5 치환기는 C1-C6-알킬, C1-C6-알콕시, C1-C6-알킬술파닐, C1-C6-알킬술피닐, C1-C6-알킬술포닐 및 -O-Si(C1-C6-알킬)3의 C1-C6-알킬 모이어티를 나타낸다.
표현 "지방족 L 치환기는 1개 이상의 LSa 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 L 치환기는 C1-C6-알킬렌, C2-C6-알케닐렌, C2-C6-알키닐렌, 및 C1-C6-알킬렌-C3-C8-시클로알킬렌, C3-C8-시클로알킬렌-C1-C6-알킬렌, C1-C6-알킬렌-C3-C8-시클로알킬렌-C1-C6-알킬렌, C1-C6-알킬렌-(C=O)-, C1-C6-알킬렌-C3-C8-시클로알케닐렌, C3-C8-시클로알케닐렌-C1-C6-알킬렌, C1-C6-알킬렌-C3-C8-시클로알케닐렌-C1-C6-알킬렌의 C1-C6-알킬렌 모이어티를 나타낸다.
표현 "지방족 R6S, Rc 및 Rd 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 R6S 치환기는 C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, 및 -Si(C1-C6-알킬)3 및 -O-Si(C1-C6-알킬)3의 C1-C6-알킬 모이어티를 나타낸다.
표현 "지방족 R6S, Rc 및 Rd 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 Rc 치환기는 C1-C6-알킬을 나타낸다.
표현 "지방족 R6S, Rc 및 Rd 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 Rd 치환기는 C1-C6-알킬 및 C1-C6-할로알킬을 나타낸다.
표현 "지방족 R7, Re, Rf 및 Rg 치환기는 1개 이상의 R7Sa 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 R7 치환기는 C1-C6-알킬, C1-C6-할로알킬, C1-C6-히드록시알킬, C1-C6-알킬카르보닐, C1-C6-할로알킬카르보닐, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C2-C6-알키닐옥시, C2-C6-할로알키닐옥시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, 및 -Si(C1-C6-알킬)3 및 -O-Si(C1-C6-알킬)3의 C1-C6-알킬 모이어티를 나타낸다.
표현 "지방족 R7, Re, Rf 및 Rg 치환기는 1개 이상의 R7Sa 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 Re 치환기는 C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐 및 C2-C6-할로알키닐을 나타낸다.
표현 "지방족 R7, Re, Rf 및 Rg 치환기는 1개 이상의 R7Sa 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 Rf 치환기는 C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, 및 C1-C6-알킬아미노 및 디(C1-C6-알킬)아미노의 C1-C6-알킬 모이어티를 나타낸다.
표현 "지방족 R7, Re, Rf 및 Rg 치환기는 1개 이상의 R7Sa 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 Rg 치환기는 C1-C6-알킬 및 C1-C6-할로알킬을 지정한다.
표현 "지방족 R8, Rh 및 Ri 치환기는 1개 이상의 R8Sa 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 R8 치환기는 C1-C6-알킬, C1-C6-할로알킬, C1-C6-히드록시알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C2-C6-알키닐옥시, C2-C6-할로알키닐옥시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, 및 -Si(C1-C6-알킬)3 및 -O-Si(C1-C6-알킬)3의 C1-C6-알킬 모이어티를 나타낸다.
표현 "지방족 R8, Rh 및 Ri 치환기는 1개 이상의 R8Sa 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 Rh 치환기는 C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐 및 C2-C6-할로알키닐을 나타낸다.
표현 "지방족 R8, Rh 및 Ri 치환기는 1개 이상의 R8Sa 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 Ri 치환기는 C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐 및 C2-C6-할로알키닐을 나타낸다.
표현 "지방족 QS, Rj 및 Rk 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 QS 치환기는 C1-C6-알킬, C1-C6-할로알킬, C1-C6-알킬카르보닐, C1-C6-할로알킬카르보닐, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, 및 -Si(C1-C6-알킬)3 및 -O-Si(C1-C6-알킬)3의 C1-C6-알킬 모이어티를 나타낸다.
표현 "지방족 QS, Rj 및 Rk 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 Rj 치환기는 C1-C6-알킬, C1-C6-할로알킬 및 C1-C6-알콕시를 나타낸다.
표현 "지방족 QS, Rj 및 Rk 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 지방족 Rk 치환기는 C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C2-C6-알케닐 및 C2-C6-할로알케닐을 나타낸다.
표현 "시클릭 R1, R2, R3, R4 및 R5 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 R1, R2 및 R5 치환기는 C3-C8-시클로알킬을 나타낸다.
표현 "시클릭 R1, R2, R3, R4 및 R5 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 R3 및 R4 치환기는 C3-C8-시클로알킬, 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클 및 방향족 5- 내지 14-원 헤테로사이클을 나타낸다.
표현 "L 치환기의 시클릭 또는 시클릭 모이어티는 1개 이상의 LSc 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 L 치환기는 C3-C8-시클로알킬렌, C3-C8-시클로알케닐렌 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로시클릴렌을 나타낸다.
표현 "L 치환기의 시클릭 또는 시클릭 모이어티는 1개 이상의 LSc 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 L 치환기는 C1-C6-알킬렌-C3-C8-시클로알킬렌, C3-C8-시클로알킬렌-C1-C6-알킬렌, C1-C6-알킬렌-C3-C8-시클로알킬렌-C1-C6-알킬렌의 C3-C8-시클로알킬렌 모이어티 및 C1-C6-알킬렌-C3-C8-시클로알케닐렌, C3-C8-시클로알케닐렌-C1-C6-알킬렌 및 C1-C6-알킬렌-C3-C8-시클로알케닐렌-C1-C6-알킬렌의 C3-C8-시클로알케닐렌 모이어티를 나타낸다.
표현 "R6 치환기의 시클릭, 또는 시클릭 모이어티는 1개 이상의 R6S 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 R6 치환기는 비-방향족 C3-C12-카르보사이클, 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클 및 방향족 5- 내지 14-원 헤테로사이클을 나타낸다.
표현 "R6 치환기의 시클릭, 또는 시클릭 모이어티는 1개 이상의 R6S 치환기로 치환될 수 있다"에서 본원에 사용된 바와 같은 R6 치환기의 시클릭 모이어티는 비-방향족 C3-C12-카르보시클릴옥시의 비-방향족 C3-C12-카르보사이클, 방향족 C6-C14-카르보시클릴옥시의 방향족 C6-C14-카르보사이클, 방향족 5- 내지 14-원 헤테로시클릴옥시의 방향족 5- 내지 14-원 헤테로사이클, 비-방향족 5- 내지 14-원 헤테로시클릴옥시의 비-방향족 5- 내지 14-원 헤테로사이클, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-알콕시의 비-방향족 C3-C12-카르보사이클, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-알콕시의 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-알콕시의 비-방향족 3- 내지 14-원 헤테로사이클, 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-알콕시의 방향족 5- 내지 14-원 헤테로사이클, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-할로알콕시의 비-방향족 C3-C12-카르보사이클, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-할로알콕시의 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-할로알콕시의 비-방향족 3- 내지 14-원 헤테로사이클 및 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-할로알콕시의 방향족 5- 내지 14-원 헤테로사이클을 나타낸다.
표현 "시클릭 R6S 및 Rc 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 R6S 치환기는 C3-C8-시클로알킬, C3-C8-시클로알케닐, 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 나타낸다.
표현 "R6S의 시클릭 또는 시클릭 모이어티 및 시클릭 Rc 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 R6S 치환기의 시클릭 모이어티는 C3-C8-시클로알킬옥시의 C3-C8-시클로알킬을 나타낸다.
표현 "R6S의 시클릭 또는 시클릭 모이어티 및 시클릭 Rc 치환기는 1개 이상의 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 Rc 치환기는 C3-C8-시클로알킬을 나타낸다.
표현 "시클릭 R7, Re 및 Rg 치환기는 1개 이상의 R7Sc 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 R7 치환기는 C3-C8-시클로알킬, C3-C6-시클로알케닐, 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 나타낸다.
표현 "R7의 시클릭 또는 시클릭 모이어티, 시클릭 Re 및 시클릭 Rg 치환기는 1개 이상의 R7Sc 치환기로 치환될 수 있다"에서 본원에 사용된 R7 치환기의 시클릭 모이어티는 C3-C8-시클로알킬옥시의 C3-C8-시클로알킬, 방향족 C6-C14-카르보시클릴옥시의 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로시클릴옥시의 방향족 5- 또는 6-원 모노시클릭 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로시클릴옥시의 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 나타낸다.
표현 "시클릭 R7, Re 및 Rg 치환기는 1개 이상의 R7Sc 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 Re 치환기는 C3-C8-시클로알킬, C3-C8-할로시클로알킬, 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 나타낸다.
표현 "시클릭 R7, Re 및 Rg 치환기는 1개 이상의 R7Sc 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 Rg 치환기"는 C3-C8-시클로알킬을 나타낸다.
표현 "여기서 시클릭 R8, Rh 및 Ri 치환기는 1개 이상의 R8Sc 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 R8 치환기는 C3-C8-시클로알킬, C3-C6-시클로알케닐, 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클 및 방향족 5- 내지 14-원 헤테로사이클을 나타낸다.
표현 "R8의 시클릭 또는 시클릭 모이어티, 시클릭 Rh 및 시클릭 Ri 치환기는 1개 이상의 R8Sc 치환기로 치환될 수 있다"에서 본원에 사용된 R8 치환기의 시클릭 모이어티는 C3-C8-시클로알킬옥시의 C3-C8-시클로알킬, 방향족 C6-C14-카르보시클릴옥시의 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로시클릴옥시의 비-방향족 3- 내지 14-원 헤테로사이클 및 방향족 5- 내지 14-원 헤테로시클릴옥시의 방향족 5- 내지 14-원 헤테로사이클을 나타낸다.
표현 "여기서 R8의 시클릭 또는 시클릭 모이어티, 시클릭 Rh 및 시클릭 Ri 치환기는 1개 이상의 R8Sc 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 Rh 치환기는 C3-C8-시클로알킬, C3-C8-할로시클로알킬, 방향족 C6-C14-카르보사이클, 방향족 5- 내지 14-원 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 나타낸다.
표현 "여기서 시클릭 R8, Rh 및 Ri 치환기는 1개 이상의 R8Sc 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 Ri 치환기는 C3-C8-시클로알킬, C3-C8-할로시클로알킬, 방향족 C6-C14-카르보사이클, 방향족 5- 내지 14-원 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 나타낸다.
표현 "QS의 시클릭 또는 시클릭 모이어티 및 시클릭 Rk 치환기는 1개 이상의 RQs 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 QS 치환기는 C3-C8-시클로알킬, C3-C6-시클로알케닐, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클 및 방향족 5- 내지 14-원 헤테로사이클을 나타낸다.
표현 "QS의 시클릭 또는 시클릭 모이어티 및 시클릭 Rk 치환기는 1개 이상의 RQs 치환기로 치환될 수 있다"에서 본원에 사용된 QS 치환기의 시클릭 모이어티는 C3-C8-시클로알킬옥시의 C3-C8-시클로알킬을 나타낸다.
표현 "시클릭 QS 및 Rk 치환기는 1개 이상의 RQs 치환기로 치환될 수 있다"에서 본원에 사용된 시클릭 Rk 치환기는 C3-C8-시클로알킬을 나타낸다.
화학식 (I)의 화합물 및 중간체의 제조 방법
본 발명은 화학식 (I)의 화합물 및 그의 중간체의 제조 방법에 관한 것이다. 달리 나타내지 않는 한, 라디칼 A, Q, T, L, R1, R2, R3, R4, R5, R6, R7, R8, m은 화학식 (I)의 화합물에 대해 상기 주어진 의미를 갖는다. 이들 정의는 화학식 (I)의 최종 생성물 뿐만 아니라 모든 중간체에도 적용된다.
화학식 (I-a) - (I-f)의 화합물은 화학식 (I)의 다양한 하위세트이다. 화학식 (I-a-1) - (I-a-7)의 화합물은 화학식 (I-a)의 다양한 하위세트이다. 화학식 (I-a) - (I-f) 및 (I-a-1) - (I-a-7)에 대한 모든 치환기는 달리 나타내지 않는 한 화학식 (I)에 대해 상기 정의된 바와 같다.
화학식 (I)의 화합물은 공지된 방법과 유사하게 다양한 경로에 의해 제조될 수 있다 (예를 들어 및 그의 참고문헌 참조). 적합한 방법의 비제한적 예가 본원에 기재되어 있다.
화학식 (I)의 화합물은 방법 A 내지 I를 수행함으로써 직접 수득할 수 있거나, 또는 본원에 기재된 방법에 따라 제조된 화학식 (I)의 또 다른 화합물의 전환 또는 유도체화에 의해 수득할 수 있다. 예를 들어, 화학식 (I)의 화합물은 화학식 (I)의 출발 화합물의 1개 이상의 치환기를 다른 치환기로 대체함으로써 화학식 (I)의 또 다른 화합물로 전환시킬 수 있다. 이러한 전환 또는 유도체화의 비제한적 예는 하기 기재된다 (방법 J 내지 L).
본원에 기재된 방법은 고려되는 반응에 통상적인 1종 이상의 불활성 유기 용매를 사용하여 적합하게 수행할 수 있다. 적합한 불활성 유기 용매는 지방족, 지환족 또는 방향족 탄화수소 (예를 들어 석유 에테르, 펜탄, 헥산, 헵탄, 시클로헥산, 메틸시클로헥산, 리그로인, 벤젠, 톨루엔, 크실렌 또는 데칼린), 할로겐화 지방족, 지환족 또는 방향족 탄화수소 (예를 들어 클로로벤젠, 디클로로벤젠, 디클로로메탄, 클로로포름, 사염화탄소, 1,2-디클로로에탄 또는 트리클로로에탄), 에테르 (예를 들어 디에틸 에테르, 디이소프로필 에테르, 메틸 t-부틸 에테르, 메틸 t-아밀 에테르, 디옥산, 테트라히드로푸란, 2-메틸테트라히드로푸란, 1,2-디메톡시에탄, 1,2-디에톡시에탄 또는 아니솔), 케톤 (예를 들어 아세톤, 메틸 에틸 케톤, 메틸 이소프로필 케톤 및 메틸 이소부틸 케톤), 에스테르 (예를 들어 메틸 아세테이트, 에틸 아세테이트 또는 부틸 아세테이트), 알콜 (예를 들어 메탄올, 에탄올, 프로판올, 이소-프로판올, 부탄올, tert-부탄올), 니트릴 (예를 들어 아세토니트릴, 프로피오니트릴, n- 또는 i-부티로니트릴 또는 벤조니트릴), 아미드 (예를 들어 N,N-디메틸포름아미드, N,N-디메틸아세트아미드, N-메틸포름아닐리드, N-메틸피롤리돈 또는 헥사메틸인산 트리아미드), 술폭시드 (예를 들어 디메틸 술폭시드) 또는 술폰 (예를 들어 술폴란), 우레아 (예를 들어 1,3-디메틸-3,4,5,6-테트라히드로-2(1H)-피리미디논) 또는 그의 임의의 혼합물로부터 선택될 수 있다.
본원에 기재된 일부 방법은 이러한 반응에 통상적인 1종 이상의 무기 또는 유기 염기를 필요로 하거나 또는 임의로 사용하여 수행할 수 있다. 적합한 무기 및 유기 염기의 예는 알칼리 토금속 또는 알칼리 금속 탄산염 (예를 들어 탄산나트륨, 탄산칼륨, 중탄산칼륨, 중탄산나트륨 또는 탄산세슘), 알칼리 금속 수소화물 (예를 들어 수소화나트륨), 알칼리 토금속 또는 알칼리 금속 수산화물 (예를 들어 수산화나트륨, 수산화칼슘, 수산화칼륨 또는 다른 수산화암모늄 유도체), 알칼리 토금속, 알칼리 금속 또는 플루오린화암모늄 (예를 들어 플루오린화칼륨, 플루오린화세슘 또는 테트라부틸암모늄 플루오라이드), 알칼리 금속 또는 알칼리 토금속 아세테이트 (예를 들어 아세트산나트륨, 아세트산리튬, 아세트산칼륨 또는 아세트산칼슘), 알칼리 금속 알콜레이트 (예를 들어 포타슘 tert-부톡시드 또는 소듐 tert-부톡시드), 알칼리 금속 포스페이트 (예를 들어 트리-포타슘 포스페이트), 3급 아민 (예를 들어 트리메틸아민, 트리에틸아민, 트리부틸아민, N,N-디메틸아닐린, N,N-디시클로헥실메틸아민, N,N-디이소프로필에틸아민, N-메틸피페리딘, N,N-디메틸아미노피리딘, 디아자비시클로옥탄 (DABCO), 디아자비시클로노넨 (DBN), 디아자비시클로운데센 (DBU), 퀴누클리딘, 3-아세톡시퀴누클리딘, 구아니딘 또는 방향족 염기 (예를 들어 피리딘, 피콜린, 루티딘 또는 콜리딘)를 포함하나, 이에 제한되지는 않는다.
본원에 기재된 방법 중 일부는 임의로 전이 금속 촉매, 예컨대 금속 (예를 들어 구리 또는 팔라듐) 염 또는 착물의 존재 하에, 적절한 경우에 리간드의 존재 하에 수행할 수 있다.
적합한 구리 염 또는 착물 및 그의 수화물은 구리 금속, 아이오딘화구리(I), 염화구리(I), 브로민화구리(I), 염화구리(II), 브로민화구리(II), 산화구리(II), 산화구리(I), 아세트산구리(II), 아세트산구리(I), 구리(I) 티오펜-2-카르복실레이트, 시안화구리(I), 황산구리(II), 구리(II) 비스(2,2,6,6-테트라메틸-3,5-헵탄디오네이트), 구리(II) 트리플루오로메탄술포네이트, 테트라키스(아세토니트릴)구리(I) 헥사플루오로포스페이트, 테트라키스(아세토니트릴)-구리(I) 테트라플루오로보레이트를 포함하나, 이에 제한되지는 않는다.
구리 염 및 리간드 또는 염, 예컨대 에틸렌디아민, N,N-디메틸에틸렌디아민, N,N'-디메틸에틸렌디아민, rac-트랜스-1,2-디아미노시클로헥산, rac-트랜스-N,N'-디메틸시클로헥산-1,2-디아민, 1,1'-비나프틸-2,2'-디아민, N,N,N',N'-테트라메틸에틸렌디아민, 프롤린, N,N-디메틸글리신, 퀴놀린-8-올, 피리딘, 2-아미노피리딘, 4-(디메틸아미노)피리딘, 2,2'-비피리딜, 2,6-디(2-피리딜)피리딘, 2-피콜린산, 2-(디메틸아미노메틸)-3-히드록시피리딘, 1,10-페난트롤린, 3,4,7,8-테트라메틸-1,10-페난트롤린, 2,9-디메틸-1,10-페난트롤린, 4,7-디메톡시-1,10-페난트롤린, N,N'-비스[(E)-피리딘-2-일메틸리덴]시클로헥산-1,2-디아민, N-[(E)-페닐메틸리덴], N-[(E)-페닐메틸리덴]-시클로헥산아민, 1,1,1-트리스(히드록시메틸)에탄, n-부틸이미다졸, 에틸렌 글리콜, 2,2,6,6-테트라메틸헵탄-3,5-디온, 2-(2,2-디메틸프로파노일)시클로헥사논, 아세틸아세톤, 디벤조일메탄, 2-(2-메틸프로파노일)시클로헥사논, 비페닐-2-일(디-tert-부틸)포스판, 에틸렌비스-(디페닐포스핀), N,N-디에틸살리실아미드, 2-히드록시벤즈알데히드 옥심, 옥소[(2,4,6-트리메틸페닐)아미노]아세트산 또는 1H-피롤-2-카르복실산의 반응에 대한 개별 첨가에 의해 반응 혼합물에서 적합한 구리 착물을 계내 생성하는 것이 또한 가능하다.
적합한 팔라듐 염 또는 착물은 염화팔라듐, 아세트산팔라듐, 테트라키스(트리페닐포스핀)팔라듐(0), 비스(디벤질리덴아세톤)팔라듐(0), 트리스(디벤질리덴아세톤)디팔라듐(0), 비스(트리페닐포스핀)팔라듐(II) 디클로라이드, [1,1'-비스(디페닐포스피노)페로센]디클로로팔라듐(II), 비스(신나밀)디클로로디팔라듐(II), 비스(알릴)-디클로로디팔라듐(II) 또는 [1,1'-비스(디-tert-부틸포스피노)페로센]디클로로팔라듐(II)을 포함하나, 이에 제한되지는 않는다.
팔라듐 염 및 리간드 또는 염, 예컨대 트리에틸포스핀, 트리-tert-부틸포스핀, 트리-tert-부틸포스포늄 테트라플루오로보레이트, 트리시클로헥실포스핀, 2-(디시클로헥실포스피노)비페닐, 2-(디-tert-부틸포스피노)비페닐, 2-(디시클로헥실포스피노)-2'-(N,N-디메틸아미노)비페닐, 2-(tert-부틸포스피노)-2'-(N,N-디메틸아미노)비페닐, 2-디-tert-부틸포스피노-2',4',6'-트리이소프로필비페닐, 2-디시클로헥실포스피노-2',4',6'-트리이소프로필비페닐, 2-디시클로헥실포스피노-2,6'-디메톡시비페닐, 2-디시클로헥실포스피노-2',6'-디이소프로폭시비페닐, 트리페닐-포스핀, 트리스-(o-톨릴)포스핀, 소듐 3-(디페닐포스피노)벤젠술포네이트, 트리스-(2-메톡시-페닐)포스핀, 2,2'-비스(디페닐포스피노)-1,1'-비나프틸, 1,4-비스(디페닐포스피노)부탄, 1,2-비스(디페닐포스피노)에탄, 1,4-비스(디시클로헥실포스피노)부탄, 1,2-비스(디시클로헥실포스피노)-에탄, 2-(디시클로헥실포스피노)-2'-(N,N-디메틸아미노)-비페닐, 1,1'-비스(디페닐포스피노)-페로센, (R)-(-)-1-[(S)-2-디페닐포스피노)페로세닐]에틸디시클로헥실포스핀, 트리스-(2,4-tert-부틸-페닐)포스파이트, 디(1-아다만틸)-2-모르폴리노페닐포스핀 또는 1,3-비스(2,4,6-트리메틸페닐)이미다졸륨 클로라이드의 반응에 대한 개별 첨가에 의해 반응 혼합물에서 팔라듐 착물을 생성하는 것이 또한 가능하다.
적절한 촉매 및/또는 리간드는 상업적 카탈로그, 예컨대 문헌 ["Metal Catalysts for Organic Synthesis" by Strem Chemicals] 또는 리뷰 (문헌 [Chemical Society Reviews (2014), 43, 3525, Coordination Chemistry Reviews (2004), 248, 2337] 및 그의 참고문헌)로부터 선택될 수 있다.
본원에 기재된 방법 중 일부는 문헌에 보고된 방법에 따라 금속-광산화환원 촉매작용에 의해 수행할 수 있다 (Nature chemistry review, (2017) 0052 and references therein; Science (2016) 352, 6291, 1304; Org. Lett. 2016, 18, 4012, J. Org. Chem 2016, 81, 6898; J. Am. Chem. Soc. 2016, 138, 12715, J. Am. Chem. Soc. 2016, 138, 13862; J. Am. Chem. Soc. 2016, 138, 8034; J. Org. Chem. 2016, 81, 12525, J. Org. Chem. 2015, 80, 7642). 이어서, 상기 방법은 광증감제, 예컨대 Ir 및 Ru 착물 또는 유기 염료, 및 금속 촉매 예컨대 Ni 착물의 존재 하에 수행한다. 반응은 리간드의 존재 하에 및 적절한 경우에 염기의 존재 하에 청색 또는 백색 광의 조사 하에 수행할 수 있다.
적합한 광증감제는 Ir(III) 광촉매 예컨대 [Ir(dFCF3ppy)2(bpy)]PF6 (dFCF3ppy = 2-(2,4-디플루오로페닐)-5-트리플루오로메틸피리딘, bpy = 2,2'-비피리딘), [Ir(dFCF3ppy)2(dtbbpy)]PF6 (dtbbpy = 4,4'-디-tert-부틸-2,2'-비피리딘), Ir(ppy)2(dtbbpy)PF6 (ppy = 2-페닐피리딘), Ir(ppy)2(bpy)PF6, Ir(dFppy)3PF6 (dFCF3ppy = 2-(2,4-디플루오로페닐)피리딘), fac-Ir(ppy)3, (Ir[diF(5-Me)ppy]2(테트라MePhen)PF6 (diF(5-Me)ppy = 2-(2,4-디플루오로페닐)-5-메틸피리딘, 테트라MePhen = 3,4,7,8-테트라메틸-1,10-페난트롤린), Ru(II) 광촉매 예컨대 Ru(bpy)3Cl2 또는 Ru(bpy)3(PF6)2 또는 유기 염료 예컨대 9-메시틸-10-아크리디늄 퍼클로레이트 또는 테트라플루오로보레이트, 또는 2,4,5,6-테트라-9H-카르바졸-9-일-1,3-벤젠디카르보니트릴, 9-플루오레논 및 9,10-페난트렌퀴논을 포함하나, 이에 제한되지는 않는다.
적합한 니켈 촉매는 비스(1,5-시클로옥타디엔)니켈 (0), 염화니켈(II), 브로민화니켈(II), 무수 또는 수화물 형태 하의 또는 디메톡시에탄 착물로서의 아이오딘화니켈(II), 니켈(II) 아세틸아세토네이트, 질산니켈(II) 6수화물을 포함하나, 이에 제한되지는 않는다. 이들 니켈 촉매는 비피리딘 리간드, 예컨대 2,2'-비피리딘, 4,4'-디-tert-부틸-2,2'-비피리딘, 4,4'-디메톡시-2,2'-비피리딘, 4,4'-디메틸-2,2'-비피리딘 또는 페난트롤린, 예컨대 1,10-페난트롤린, 4,7-디메틸-1,10-페난트롤린, 4,7-디메톡시-1,10-페난트롤린 또는 디아민, 예컨대 N,N,N',N'-테트라메틸에틸렌디아민 또는 디온, 예컨대 테트라메틸헵탄디온과 조합하여 사용될 수 있다.
본원에 기재된 방법은 -105℃ 내지 250℃, 바람직하게는 -78℃ 내지 185℃ 범위의 온도에서 수행할 수 있다.
반응 시간은 반응의 규모 및 반응 온도의 함수로서 달라지지만, 일반적으로 수분 내지 48시간이다.
본원에 기재된 방법은 일반적으로 표준 압력 하에 수행한다. 그러나, 승압 또는 감압 하에 작업하는 것이 또한 가능하다.
본원에 기재된 방법은 임의로 표준 또는 승압 하에 마이크로웨이브 조사 하에 수행할 수 있다.
본원에 기재된 방법에서, 출발 물질은 일반적으로 대략 등몰량으로 사용된다. 그러나, 출발 물질 중 하나를 비교적 과량으로 사용하는 것이 또한 가능하다.
화학식 (I)의 화합물의 제조 방법
방법 A
화학식 (I-a-1)의 화합물 (즉 A가 O이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물)은 하기 단계를 포함하는, 반응식 1에 나타낸 바와 같은 방법에 의해 제조할 수 있다:
- W가 수소인 경우에, 화학식 (4)의 화합물을 임의로 염기의 존재 하에 탈수제로 처리하여 화학식 (I-a-1)의 화합물을 직접 수득하는 단계;
- W가 아미노보호기인 경우에, 화학식 (4)의 화합물을 임의로 염기의 존재 하에 탈수제로 처리한 다음, 탈보호 단계를 수행하여 화학식 (I-a-1)의 화합물을 수득하는 단계.
화학식 (I-a-1)의 화합물은 화학식 (4)의 화합물을 임의로 염기의 존재 하에 탈수제, 예컨대 POCl3, P2O5 또는 트리플산 무수물로 처리함으로써 수득할 수 있다. 옥사디아진 고리를 형성하는 이러한 방법은 공지되어 있고, 문헌 (J. Med. Chem. 2017, 60, 2383-2400)에 기재되어 있다. 반응은 임의의 통상적인 불활성 유기 용매 중에서 수행될 수 있다. 임의로 할로겐화된 지방족, 지환족 또는 방향족 탄화수소, 예컨대 석유 에테르, 헥산, 헵탄, 시클로헥산, 메틸시클로헥산, 벤젠, 톨루엔, 크실렌 또는 데칼린; 클로로벤젠, 디클로로벤젠, 디클로로메탄, 클로로포름, 사염화탄소, 디클로르에탄 또는 트리클로르에탄; 에테르, 예컨대 디이소프로필 에테르, 메틸 t-부틸 에테르, 메틸 t-아밀 에테르, 디옥산, 테트라히드로푸란, 1,2-디메톡시에탄, 1,2-디에톡시에탄 또는 아니솔; 니트릴, 예컨대 아세토니트릴, 프로피오니트릴, n- 또는 i-부티로니트릴 또는 벤조니트릴; 알콜, 예컨대 에탄올 또는 이소프로판올을 사용하는 것이 바람직하다.
W가 아미노 보호기를 나타내는 경우에, 단계 3은 문헌 (Greene's Protective Groups in organic Synthesis; Peter G. M. Wuts; Wiley; Fifth Edition; 2014; 895-1194)에 기재된 반응 조건을 사용하는 추가의 탈보호 단계로 이어진다. 예를 들어 tert-부톡시카르보닐 기는 산성 매질 예컨대 염산 또는 트리플루오로아세트산 중에서 제거할 수 있다.
화학식 (4)의 화합물은 하기에 의해 수득할 수 있다:
- 화학식 (1)의 화합물을 화학식 (2)의 아민 또는 그의 염 중 하나와 반응시켜 화학식 (3)의 화합물을 수득하는 단계;
- 화합물 (3)의 프탈이미드 기를 제거하여 화학식 (4)의 화합물을 수득하는 단계.
프탈이미드 기를 제거하기 위한 반응 조건은 널리 공지되어 있고, 문헌 (Greene's Protective Groups in organic Synthesis; Peter G. M. Wuts; Wiley; Fifth Edition; 2014; 1012-1014)에 보고되어 있다.
화학식 (1)의 화합물은 본원에 기재된 1개 이상의 방법에 의해 제조할 수 있다 (방법 N, O 및 P 참조).
화학식 (2)의 아민은 본원에 기재된 방법 S에 의해 제조할 수 있다.
U1이 히드록실 기인 화학식 (1)의 화합물은 문헌 (예를 들어 문헌 [Tetrahedron 2005, 61, 10827-10852])에 기재된 방법에 의해 축합 시약의 존재 하에 화학식 (2)의 아민과 반응할 수 있다. 적합한 축합 시약의 예는 할로겐화 시약 (예를 들어 포스겐, 삼브로민화인, 삼염화인, 오염화인, 삼염화인, 옥살릴 클로라이드 또는 티오닐 클로라이드), 탈수 시약 (예를 들어 에틸 클로로포르메이트, 메틸 클로로포르메이트, 이소프로필 클로로포르메이트, 이소부틸 클로로포르메이트 또는 메탄술포닐 클로라이드), 카르보디이미드 (예를 들어 N,N'-디시클로헥실카르보디이미드 (DCC)) 또는 다른 통상의 축합 (또는 펩티드 커플링) 시약 (예를 들어 오산화인, 폴리인산, 비스(2-옥소-3-옥사졸리디닐)포스핀산 클로라이드, 1-[비스(디메틸아미노)메틸렌]-1H-1,2,3-트리아졸로[4,5-b]피리디늄 3-옥시드 헥사플루오로포스페이트 (HATU), N,N'-카르보닐-디이미다졸, 2-에톡시-N-에톡시카르보닐-1,2-디히드로퀴놀린 (EEDQ), 트리페닐포스핀/테트라클로로-메탄, 4-(4,6-디메톡시[1.3.5]-트리아진-2-일)-4-메틸모르폴리늄 클로라이드 수화물, 브로모-트리피롤리디노포스포늄헥사플루오로포스페이트 또는 프로판포스폰산 무수물 (T3P)을 포함하나, 이에 제한되지는 않는다.
U1이 할로겐 원자인 화학식 (1)의 화합물은 널리 공지된 방법에 의해 산 스캐빈저의 존재 하에 화학식 (2)의 아민과 반응할 수 있다. 적합한 산 스캐빈저는 본원에 기재된 바와 같은 임의의 무기 및 유기 염기를 포함하며, 이는 이러한 반응에 통상적이다. 알칼리 금속 탄산염, 알칼리 토금속 아세트산염, 3급 아민 또는 방향족 염기가 바람직하다.
U1이 C1-C6-알콕시 기인 화학식 (1)의 화합물은 임의로 루이스 산, 예컨대 트리메틸알루미늄의 존재 하에 과량의 화학식 (2)의 아민과 반응시킬 수 있다.
방법 B
화학식 (I-a-1)의 화합물 (즉 A가 O이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물)은 반응식 2에 나타낸 바와 같이, 화학식 (7)의 화합물을 염기 (예를 들어 유기 또는 무기 염기)의 존재 하에 및 임의로 적합한 구리 염 또는 착물의 존재 하에 화학식 (8)의 화합물과 반응시키는 단계를 포함하는 방법에 의해 제조할 수 있다.
화학식 (7)의 화합물은 방법 A에 대해 본원에 기재된 것과 동일한 조건에서 하기에 의해 제조할 수 있다:
- 화학식 (5)의 화합물을 화학식 (2)의 아민 또는 그의 염 중 하나와 반응시켜 화학식 (6a)의 화합물을 수득하는 단계;
- 화합물 (6a)의 프탈이미드 기를 제거하여 화학식 (6b)의 화합물을 수득하는 단계;
- W가 수소인 경우에, 화학식 (6b)의 화합물을 임의로 염기의 존재 하에 탈수제로 처리하여 화학식 (7)의 화합물을 직접 수득하는 단계;
- W가 아미노보호기인 경우에, 화학식 (6b)의 화합물을 임의로 염기의 존재 하에 탈수제로 처리한 다음, 탈보호 단계를 수행하여 화학식 (7)의 화합물을 수득하는 단계.
화학식 (7)의 화합물과 화학식 (8)의 화합물의 반응은 전이 금속 촉매 예컨대 구리 염 또는 착물의 존재 하에, 및 적절한 경우에 본원에 기재된 바와 같은 리간드의 존재 하에 수행할 수 있다.
화학식 (5)의 화합물은 상업적으로 입수가능하거나, 또는 본원에 기재된 방법 Q에 의해 제조할 수 있다.
화학식 (8)의 화합물은 상업적으로 입수가능하거나, 또는 널리 공지된 방법에 따라 화학식 (8)의 또 다른 화합물의 전환 또는 유도체화에 의해 수득할 수 있다.
방법 C
화학식 (I-a-1)의 화합물 (즉 A가 O이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물)은 산성 조건 하에 환원제를 화학식 (12)의 화합물에 첨가하여 화학식 (I-a-1)의 화합물을 수득하는 단계를 포함하는, 반응식 3에 나타낸 바와 같은 방법에 의해 제조할 수 있다:
화학식 (12)의 화합물을 환원제, 예컨대 소듐 시아노보로히드라이드의 존재 하에 산성 조건 하에 고리화시켜 화학식 (I-a-1)의 화합물을 수득할 수 있다. 이러한 방법론으로 옥사디아진 고리를 형성하는 반응 조건은 공지되어 있으며, 문헌 (Heterocycles 2016, 92, 2166-2200)에 기재되어 있다.
화학식 (12)의 화합물은 염기의 존재 하에 화학식 (10)의 화합물을 화학식 (11)의 화합물과 반응시킴으로써 수득할 수 있다. 적합한 염기는 문헌 (Heterocycles 2016, 92, 2166-2200)에 기재된 바와 같이 알칼리 금속 수소화물 예컨대 수소화나트륨, 알칼리 금속 탄산염 예컨대 탄산칼륨, 알칼리 금속 수산화물 예컨대 수산화칼륨, 또는 포스파젠 염기 예컨대 BEMP일 수 있다.
화학식 (10)의 화합물은 화학식 (9)의 화합물을 히드록실아민 또는 그의 염 중 하나와 반응시킴으로써 수득할 수 있다. 이러한 변환을 수행하기 위한 반응 조건은 공지되어 있고, 문헌 (WO2010138600)에 보고되었다.
화학식 (9)의 화합물은 본원에 기재된 방법 R에 의해 제조할 수 있다.
화학식 (11)의 화합물은 상업적으로 입수가능하거나 또는 문헌 (Eur. J. Med. Chem. 2014, 84, 302, Eur. J. Med. Chem. 2015, 100, 18-23, WO2017031325)에 기재된 방법에 의해 제조할 수 있다.
방법 D
화학식 (I-a-1)의 화합물 (즉 A가 O이고, T가 수소이고, L이 직접 결합이고, m이 1 또는 2인 화학식 (I)의 화합물)은 반응식 4에 나타낸 바와 같이 하기 단계를 포함하는 방법에 의해 제조할 수 있다:
- 화학식 (13)의 화합물을 산화 조건 하에 두어 화합물 (14)를 수득하는 단계;
- R6-H (15)가 방향족 C6-C14-카르보사이클, 비-방향족 C7-C14-카르보사이클, 비-방향족 7- 내지 14-원 헤테로사이클 또는 방향족 5- 내지 14-원 헤테로사이클인 경우에, 화학식 (14)의 화합물을 산성 조건 하에 화학식 (15)의 화합물로 처리하여 화학식 (I-a-1)의 화합물을 형성하는 단계;
- R6-H (15)가 알콜 (R6'-O)-H 또는 티올 (R6'-S)-H 유도체인 경우, 화학식 (14)의 화합물을 할로겐화 시약 예컨대 SOCl2 및 화학식 (15)의 화합물로 처리하여 R6이 옥시, 알콕시, 또는 티올 기를 나타내는 화학식 (I-a-1)의 화합물을 형성하는 단계.
화학식 (14)의 화합물은 산성 조건 하에 방향족 C6-C14-카르보사이클, 비-방향족 C7-C14-카르보사이클, 비-방향족 7- 내지 14-원 헤테로사이클 또는 방향족 5- 내지 14-원 헤테로사이클 (R6-H)과 반응시켜 화학식 (I-a-1)의 화합물을 수득할 수 있다. 이러한 방법론으로 옥사디아진 고리를 형성하는 반응 조건은 공지되어 있으며, 문헌 (WO2017031325)에 기재되어 있다.
화학식 (14)의 화합물은 산화 조건 하에, 예를 들어 삼산화오스뮴 및 과아이오딘산나트륨의 존재 하에 화학식 (13)의 화합물로부터 수득할 수 있다.
화학식 (13)의 화합물은 본원에 기재된 방법 R에 의해 제조할 수 있다.
방법 E
화학식 (I-a-1)의 화합물 (즉 A가 O이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물)은 반응식 5에 나타낸 바와 같이 하기 단계를 포함하는 방법에 의해 제조할 수 있다:
- 화학식 (18)의 화합물을 화학식 (19)의 화합물 또는 그의 염 중 하나와 반응시켜 화학식 (20)의 화합물을 수득하는 단계;
- E1이 히드록실인 경우에, 미츠노부 반응 조건을 사용하여 화학식 (20)의 화합물을 화학식 (I-a-1)의 화합물로 전환시키는 단계,
- E1이 할로겐인 경우에, 염기의 존재 하에 화학식 (20)의 화합물을 화학식 (I-a-1)의 화합물로 전환시키는 단계.
화학식 (19-a, E1 = 히드록실)의 아미노알콜은 상업적으로 입수가능하거나 또는 문헌 (Molecules, 9 (6), 405-426; 2004; WO2017203474)에 기재된 방법에 의해 제조가능할 수 있다. 화학식 (19-b, E1 = 할로겐)의 화합물 또는 그의 염 중 하나는 널리 공지된 방법에 의해 상응하는 아미노알콜로부터 수득할 수 있다.
E1이 히드록실인 경우에, 화학식 (20)의 화합물은 관련 기술분야의 통상의 기술자에게 공지된 전형적 미츠노부 반응 조건을 사용하여 방법의 단계 4에 의해 화학식 (I-a-1)의 화합물로 전환시킬 수 있다 (문헌 [Strategic Applications of Named Reactions in Organic Synthesis; Laszlo Kuerti, Barbara Czako; Elsevier; 2005; 294-295] 및 그 안의 참고문헌).
E1이 할로겐인 경우에, 화학식 (20)의 화합물은 방법의 단계 4에 의해 본원에 언급된 바와 같은 염기의 존재 하에 화학식 (I-a-1)의 화합물로 전환시킬 수 있다.
W가 아미노 보호기를 나타내는 경우에, 단계 4에 이어서 문헌 (Greene's Protective Groups in organic Synthesis; Peter G. M. Wuts; Wiley; Fifth Edition; 2014; 895-1194)에 기재된 반응 조건을 사용하는 추가의 탈보호 단계를 수행하여 화학식 (I-a-1)의 화합물을 수득한다.
화학식 (18)의 화합물을 염기 예컨대 트리에틸아민의 존재 하에 화학식 (19)의 화합물 또는 그의 염 중 하나로 처리하여 화학식 (20)의 화합물을 형성할 수 있다.
화학식 (18)의 화합물은 화학식 (17)의 옥심을 방법의 단계 2에 의해 할로겐화 시약 예컨대 NCS로 처리함으로써 수득할 수 있다. 이러한 변환을 수행하기 위한 반응 조건은 문헌 (WO2013173672; RSC Advances 2015, 5, 58587-58594)에 보고되었다.
화학식 (17)의 옥심은 임의로 염기의 존재 하에, 히드록실아민 또는 그의 염 중 1종의 존재 하에 단계 1에 의해 화학식 (16)의 알데히드로부터 수득할 수 있다. 이러한 변환은 공지되어 있고, 문헌 (Tetrahedron 2000, 56, 1057-1064; ChemMedChem 2013, 8, 1210-1223)에 보고되었다.
화학식 (16)의 알데히드는 관련 기술분야의 통상의 기술자에게 널리 공지된 방법에 따라, 예를 들어 웨인렙 아미드 전구체를 DIBAL-H로 처리함으로써 (WO2016045591), 또는 에스테르 전구체를 1급 알콜로 전환시킨 다음, 이어서 알콜을 상응하는 알데히드로 산화시킴으로써 (WO199850031) 제조할 수 있다. 이러한 알데히드에 접근하기 위한 에스테르 전구체는 본원에 기재된 방법 N, O, P에 따라 제조할 수 있다.
방법 F
화학식 (I-a-1)의 화합물 (즉 A가 O이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물) 또는 화학식 (I-a-2)의 화합물 (즉 A가 NH이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물)은 반응식 6에 나타낸 바와 같이 하기 단계를 포함하는 방법에 의해 제조할 수 있다:
- 화학식 (1)의 화합물을 방법 A에 기재된 바와 유사한 조건 하에 화학식 (19)의 아민 또는 그의 염 중 하나와 반응시켜 화학식 (21)의 화합물을 수득하는 단계,
- 화학식 (21)의 화합물을 탈수제에 이어서 히드록실아민 또는 히드라진으로 처리하여 하기 화학식 (20)의 화합물을 형성하는 단계,
- E1 및 E2가 히드록실인 경우에, 미츠노부 반응 조건을 사용하여 화학식 (20)의 화합물을 화학식 (I-a-1)의 화합물로 전환시키는 단계,
- E1이 할로겐이고 E2가 히드록실 또는 -NH2인 경우에, 화학식 (20)의 화합물을 염기의 존재 하에 화학식 (I-a-1) 또는 (I-a-2)의 화합물로 전환시키는 단계.
방법 F의 단계 2 및 단계 3은 방법 E에 기재된 바와 유사한 반응 조건을 사용하여 수행할 수 있다.
화학식 (19-a, E1 = 히드록실)의 아미노알콜은 상업적으로 입수가능하거나 또는 문헌 (Molecules, 9 (6), 405-426; 2004; WO2017203474)에 기재된 방법에 의해 제조가능할 수 있다. 화학식 (19-b, E1 = 할로겐)의 화합물 또는 그의 염 중 하나는 널리 공지된 방법에 의해 상응하는 아미노알콜로부터 수득할 수 있다.
방법 G
화학식 (I-a-1)의 화합물 (즉 A가 O이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물) 또는 화학식 (I-a-2)의 화합물 (즉, A가 NH이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물)은 반응식 7에 나타낸 바와 같이 하기 단계를 포함하는 방법에 의해 제조할 수 있다:
- 화학식 (5)의 화합물을 방법 A에 기재된 바와 유사한 조건 하에 화학식 (19)의 아민과 반응시켜 화학식 (22)의 화합물을 수득하는 단계,
- 화학식 (22)의 화합물을 탈수제에 이어서 히드록실아민 또는 히드라진으로 처리하여 화학식 (23)의 화합물을 형성하는 단계,
- E1 및 E2가 히드록실인 경우에, 화학식 (23)의 화합물을 미츠노부 반응 조건을 사용하여 화학식 (7)의 화합물로 전환시키는 단계,
- E1이 할로겐이고 E2가 히드록실 또는 -NH2인 경우에, 화학식 (23)의 화합물을 염기의 존재 하에 화학식 (7) 또는 (24)의 화합물로 전환시키는 단계,
- 화학식 (7) 또는 (24)의 화합물을 염기 (예를 들어 유기 또는 무기 염기)의 존재 하에 및 임의로 적합한 구리 염 또는 착물의 존재 하에 화학식 (8)의 화합물과 반응시켜 화학식 (I-a-1) 또는 (I-a-2)의 화합물을 수득하는 단계.
방법 H
화학식 (I-a-1)의 화합물 (즉 A가 O이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물), 화학식 (I-a-3)의 화합물 (즉, A가 CR1R2이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물), 화학식 (I-a-4)의 화합물 (즉, A가 C(=O)이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물) 또는 화학식 (I-a-5)의 화합물 (즉, A가 S(=O) 2 이고, T가 수소이고, m이 1 또는 2인 화학식 (I)의 화합물)은 반응식 8에 나타낸 바와 같이 하기 단계를 포함하는 방법에 의해 제조할 수 있다:
- 화학식 (9)의 화합물을 알콕시드로 처리하여 화학식 (25)의 화합물을 수득하는 단계,
- 화학식 (25)의 화합물을 각각 화학식 (26a-1), (26a-2), (26a-3) 또는 (26a-4)의 아민과 반응키는 단계.
대안적으로, 화학식 (I-a-5)의 화합물은 문헌 (J. Org. Chem. 1974, 39, 3080)에 기재된 방법과 유사하게 피리다진 4-카르복스아미딘 화합물을 트랜스-스티릴술포닐 클로라이드로 처리함으로써 제조할 수 있다.
화학식 (25)의 화합물은 문헌 (Heterocycles, 34, 1992, 929-935)에 기재된 방법에 따라 화학식 (9)의 화합물을 알콕시드 예컨대 나트륨 메탄올레이트 또는 나트륨 에탄올레이트로 처리하여 수득할 수 있다.
화학식 (25)의 화합물을 화학식 (26-a-1), (26-a-2), (26-a-3) 또는 (26-a-4)의 화합물로 처리하고, 산성 조건 하에 고리화시켜 각각 화학식 (I-a-1), (I-a-3), (I-a-4) 또는 (I-a-5)의 화합물을 형성한다. 이러한 방법론에 기초하여 이러한 변환을 수행하기 위한 반응 조건은 문헌 (Heterocycles 2016, 92, 2166-2200)에 기재되어 있다.
화학식 (26-a-1), (26-a-2), (26-a-3) 또는 (26-a-4)의 아민은 상업적으로 입수가능하거나, 또는 문헌 (Molecules, 9 (6), 405-426; 2004, WO2017203474; J. Med. Chem 1985, 28, 694-698; J. Med. Chem 2006, 49, 4333-4343)에 기재된 방법에 의해 및 본 발명의 방법 S에 의해 제조할 수 있다.
방법 I
화학식 (I-a-6)의 화합물 (즉 A가 O이고, T가 수소이고, m이 2인 화학식 (I)의 화합물)은 반응식 9에 나타낸 바와 같이 하기 단계를 포함하는 방법에 의해 제조할 수 있다:
- 화학식 (9)의 화합물을 본원에 기재된 바와 같은 적합한 염기의 존재 하에 히드록실아민 유도체 (27)로 처리하여 화학식 (28)의 화합물을 수득하는 단계,
- 화학식 (28)의 화합물을 금속 촉매 및 적합한 리간드의 존재 하에 화학식 (29)의 시약과 반응시켜 화학식 (30)의 화합물을 수득하는 단계,
- 화학식 (30)의 화합물을 아이오딘 및 페닐실란으로 처리하여 화학식 (I-a-6)의 화합물을 형성하는 단계.
화학식 (27)의 시약은 상업적으로 입수가능하거나 또는 문헌 (WO2010099279)에 기재된 방법에 의해 제조가능하다.
화학식 (29)의 시약은 상업적으로 입수가능하거나, 또는 공지된 방법에 의해 제조할 수 있다.
방법 J
화학식 (I-a-7)의 화합물 (즉 A가 CR1R2이고, T가 수소이고, m이 0인 화학식 (I)의 화합물)은 반응식 10에 나타낸 바와 같이 화학식 (1)의 화합물을 화학식 (31)의 디아민과 반응시키는 단계를 포함하는 방법에 의해 제조할 수 있다.
방법 J는 탈수제 예컨대 POCl3의 존재 하에 수행할 수 있다.
화학식 (31)의 디아민은 상업적으로 입수가능하거나, 또는 문헌에 기재된 방법에 의해 제조할 수 있다 (Eur. J. Med. Chem 1990, 25(1), 35-44; J. Org. Chem 2012, 77(9), 4375-4384; WO2009003867).
방법 K
화학식 (I-a)의 화합물은 문헌에 기재된 방법에 의해 반응식 11에 나타낸 바와 같은 1개 이상의 단계에서 상응하는 화합물 (I-b) 또는 (I-c)로 전환시킬 수 있다.
반응식 11에서, Re, Rf, Rg는 본원에 개시된 바와 같고, 지방족 및 시클릭 치환기 R7b, R7c, Re, Rf, Rg는 본원에 개시된 바와 같이 치환될 수 있다.
반응식 11에 따라 수행된 전환의 비제한적 예는 하기에 제공된다.
R7a가 염소 원자인 화학식 (I-a)의 화합물은 문헌 (예를 들어 WO2016185342, WO2007022937)에 기재된 방법에 의해, R7b가 브로민 또는 아이오딘 원자인 화학식 (I-b)의 화합물로 전환시킬 수 있다.
R7a가 할로겐 원자인 화학식 (I-a)의 화합물은 문헌 (Journal of Molecular Catalysis A: Chemical, 2014, 393, 191-209)에 보고된 바와 같이 팔라듐 촉매의 존재 하에 R7b가 수소 원자인 화학식 (I-b)의 화합물로 전환시킬 수 있다.
R7a가 수소 원자 또는 할로겐 원자인 화학식 (I-a)의 화합물은 본원에 기재된 바와 같은 전이 금속 촉매된 또는 금속-광산화환원 촉매된 방법에 의해 R7b가 시아노, C1-C6-알킬, C1-C6-할로알킬, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C3-C8-시클로알킬, C3-C6-시클로알케닐, 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, -N(Re)2 또는 -C(=O)(ORg)인 화학식 (I-b)의 화합물로 전환시킬 수 있다.
R7b가 C1-C3-알콕시에 의해 치환된 C2-C6-알케닐 기인 화학식 (I-b)의 화합물은 문헌 (예를 들어 문헌 [J. Org. Chem. 1993, 55, 3114])에 기재된 방법에 의해, R7c가 C1-C6-알킬카르보닐 기인 화학식 (I-c)의 화합물로 전환시킬 수 있다.
R7c가 C1-C6-알킬카르보닐 기인 화학식 (I-c)의 화합물은 문헌 (예를 들어 문헌 [Greene's Protective Groups in organic Synthesis; Peter G. M. Wuts; Wiley; Fifth Edition; 2014; 655, 661, 667])에 기재된 방법에 의해 R7c가 -C(=NRf)-C1-C6-알킬 기인 화학식 (I-c)의 화합물로 추가로 전환시킬 수 있다.
R7c가 C1-C6-알킬카르보닐 기인 화학식 (I-c)의 화합물은 MeOH 중 NaBH4의 존재 하에 전형적인 관능기 상호전환 예컨대 케톤의 알콜로의 환원에 의해 R7c가 C1-C6-히드록시알킬 기인 화학식 (I-c)의 화합물로 추가로 전환시킬 수 있다.
R7c가 C1-C6-히드록시알킬 기인 화학식 (I-c)의 화합물은 플루오린화제의 존재 하에 R7c가 C1-C6-플루오로알킬인 화학식 (I-c)의 화합물로 추가로 전환시킬 수 있다. 플루오린화제의 비제한적 예는 플루오린화황, 예컨대 사플루오린화황, 디에틸아미노황트리플루오라이드, 모르폴리노황 트리플루오라이드, 비스(2-메톡시에틸)아미노황 트리플루오라이드, 2,2-디플루오로-1,3-디메틸이미다졸리딘 또는 4-tert-부틸-2,6-디메틸페닐황 트리플루오라이드를 포함한다.
화학식 (I-a)의 화합물은 본원에 기재된 방법 중 하나 이상에 의해 제조할 수 있다.
방법 L
화학식 (I-a)의 화합물은 반응식 12에 나타낸 바와 같이 1개 이상의 단계에서 문헌에 기재된 방법에 의해 상응하는 화학식 (I-d)의 화합물 또는 화학식 (I-e)의 화합물로 전환시킬 수 있다.
반응식 12에 따라 수행된 전환의 비제한적 예는 하기에 제공된다.
화학식 (I-a)의 화합물은 문헌 (예를 들어, 문헌 [Org.Lett. 2009, 11, 1837])에 기재된 방법에 의해 염기 및 친전자체 예컨대 NCS, NBS, NIS, 헥사클로로에탄, 브로민 또는 아이오딘의 존재 하에 R8a가 할로겐 원자인 화학식 (I-d)의 화합물로 전환시킬 수 있다. 방법을 수행하기에 적합한 염기는 리튬-디이소프로필아미드, 리튬 2,2,6,6-테트라메틸피페리디드, n-부틸 리튬, 메틸 리튬, TMPZnCl.LiCl, TMP2Zn·2MgCl2·2LiCl로부터 선택될 수 있다 (예를 들어, 문헌 [Dissertation Albrecht Metzer 2010, University Munich] 참조).
화학식 (I-a)의 화합물은, 임의로 염기의 존재 하에, 및 적절한 경우에 본원에 기재된 바와 같은 전이 금속 촉매 예컨대 금속 염 또는 착물 및 리간드의 존재 하에, 또는 문헌 (Heterocycles 1976, 4(8), 1331)에 기재된 방법에 의해, R8a가 C1-C6-알킬, C1-C6-할로알킬, C1-C6-히드록시알킬, C3-C8-시클로알킬, C3-C8-할로시클로알킬, C3-C6-시클로알케닐, 방향족 C6-C14-카르보사이클, 5- 내지 14-원 방향족 헤테로사이클 또는 3- 내지 14-원 비-방향족 헤테로사이클인 화학식 (I-d)의 화합물로 전환시킬 수 있다.
R8a가 할로겐 원자인 화학식 (I-d)의 화합물은 염기의 존재 하에 및 임의로 전이 금속 촉매, 예컨대 금속 염 또는 착물의 존재 하에 및 적절한 경우에 리간드의 존재 하에 R8b가 시아노, 니트로, 아미노, 메르캅토, 히드록실, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C3-C8-시클로알킬, C3-C6-시클로알케닐, 방향족 5- 내지 14-원 헤테로사이클, C3-C8-시클로알킬옥시, 방향족 C6-C14-카르보시클릴옥시, 비-방향족 3- 내지 14-원 헤테로시클릴옥시, 방향족 5- 내지 14-원 헤테로시클릴옥시, -N(Rh)2 또는 -SRi를 나타내는 것인 화학식 (I-e)의 화합물로 전환시킬 수 있다.
R8b가 C2-C6-알케닐 기인 화학식 (I-e)의 화합물은, 화학식 (I-e)의 반응 화합물을 산소, 황 또는 아미노 기재 친핵체로 처리함으로써, R8b가 C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시-C1-C6-알콕시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클 및 -N(Ra')2이고, 여기서 Ra'는 수소, C1-C6-알킬, C1-C6-할로알킬 및 C3-C8-시클로알킬로 이루어진 군으로부터 독립적으로 선택됨)에 의해 치환된 C1-C6-알킬인 화학식 (I-e)의 화합물로 추가로 전환시킬 수 있다.
R8b가 SRi 기인 화학식 (I-e)의 화합물은 화학식 (I-a-8)의 출발 화합물을 산화제 예컨대 과산화수소와 반응시킴으로써 R8b이 -S(=O)Ri 또는 -S(=O)2Ri 기인 화학식 (I-a-8)의 화합물로 추가로 전환시킬 수 있다.
화학식 (I-a)의 화합물은 본원에 기재된 방법 중 하나 이상에 의해 제조할 수 있다.
방법 M
화학식 (I-f)의 화합물 (즉 T가 -C(=O)Ra1, -C(=O)(ORa1), -C(=O)N(Ra2) 2 , -S(=O)Ra1, -S(=O) 2 Ra1 및 -S(=O) 2 N(Ra2) 2 이고, 여기서 Ra1 및 Ra2는 본원에 기재된 바와 같은 것인 화학식 (I))은 반응식 13에 나타낸 바와 같이 화학식 (I-a)의 화합물을 화학식 (32)의 화합물과 반응시키는 단계를 포함하는 방법에 의해 제조할 수 있다.
방법 M은 문헌 (예를 들어 문헌 [Tetrahedron Lett. 1995, 36, 8949; Greene's Protective Groups in organic Synthesis; Peter G. M. Wuts; Wiley; Fifth Edition; 2014; 1174-1175])에 기재된 방법에 의해 수행할 수 있다.
화학식 (32)의 화합물은 상업적으로 입수가능하다.
화학식 (I-a)의 화합물은 본원에 기재된 방법 중 하나 이상에 의해 제조할 수 있다.
화학식 (1)의 화합물의 제조 방법
본원에 기재된 바와 같은 화학식 (1)의 화합물은 하기 기재된 방법 N을 수행함으로써 직접 수득할 수 있거나, 또는 본원에 기재된 방법에 따라 제조된 화학식 (1)의 또 다른 화합물의 전환 또는 유도체화에 의해 수득할 수 있다. 화학식 (1-a) - (1-e)의 화합물은 화학식 (1)의 다양한 하위세트이다.
방법 N
화학식 (1-a)의 화합물 (즉 R7 및 R8가 반응식 14에 정의된 바와 같은 것인 화학식 (1))은 염기의 존재 하에 반응식 14에 나타낸 바와 같이 화학식 (5)의 화합물을 화학식 (8)의 시약과 반응시키는 단계를 포함하는 방법에 의해 제조할 수 있다.
반응식 14에서, Re는 본원에 개시된 바와 같고, R7, R8 및 Re는 본원에 개시된 바와 같이 치환될 수 있다.
방법 N은 적합한 전이 금속 촉매 염 또는 착물의 존재 하에, 적절한 경우에 리간드의 존재 하에 수행할 수 있다.
이어서, 수득된 화학식 (1-a)의 화합물을 1개 이상의 단계에서 화학식 (1-b)의 화합물로 전환시킬 수 있다.
이러한 전환의 비제한적 예는 하기에 기재되어 있다:
U1이 C1-C6-알콕시인 화학식 (1-a)의 화합물은 널리 공지된 관능기 상호전환 방법에 의해, 예를 들어 THF/물 중 LiOH를 사용한 에스테르 기의 가수분해에 의해, U2가 히드록실 기인 화학식 (1-b)의 화합물시킬 전환시킬 수 있다.
U2가 히드록실인 화학식 (1-b)의 화합물은 널리 공지된 방법에 의해 할로겐화제의 존재 하에 U2가 할로겐인 화학식 (1-b)의 화합물로 전환시킬 수 있다. 적합한 할로겐화 시약은 삼브로민화인, 삼염화인, 오염화인, 삼염화인 옥시드, 옥살릴 클로라이드 또는 티오닐 클로라이드를 포함하나, 이에 제한되지는 않는다.
U2가 히드록실 또는 할로겐인 화학식 (1-b)의 화합물은 널리 공지된 방법에 의해 U2가 -N(CH3)OCH3인 화학식 (1-b)의 화합물로 전환시킬 수 있다.
화학식 (5)의 화합물은 상업적으로 입수가능하거나, 또는 본원에 기재된 방법 Q에 의해 제조할 수 있다.
화학식 (8)의 화합물은 상업적으로 입수가능하거나, 또는 널리 공지된 방법에 따라 화학식 (8)의 또 다른 화합물의 전환 또는 유도체화에 의해 수득될 수 있다.
방법 O
화학식 (1-c)의 화합물 (즉 R7이 반응식 15에 정의된 바와 같은 R7a인 화학식 (1))은 공지된 방법에 의해 상응하는 화학식 (1-d)의 화합물 (즉 R7이 반응식 15에 정의된 바와 같은 R7b인 화학식 (1)) 또는 화학식 (1-e)의 화합물 (즉 R7이 반응식 15에 정의된 바와 같은 R7c인 화학식 (1))로 반응식 15에 나타낸 바와 같이 1개 이상의 단계로 전환시킬 수 있다.
반응식 15에서, Re, Rf, Rg는 본원에 개시된 바와 같고, 지방족 및 시클릭 치환기 R7b, R7c, Re, Rf, Rg는 본원에 개시된 바와 같이 치환될 수 있다.
전환의 비제한적 예는 방법 K에서 제공된 설명에 따라 수행할 수 있다.
이어서, 수득된 화학식 (1-d) 및 (1-e)의 화합물은 U1 (C1-C6-알콕시)이 히드록실 또는 할로겐으로 대체된 화학식 (1-d) 및 (1-e)의 화합물로 전환시킬 수 있다.
이러한 전환의 예는 하기에 기재되어 있다.
U1이 C1-C6-알콕시인 화학식 (1-c), (1-d), (1-e)의 화합물은 널리 공지된 관능기 상호전환 방법에 의해, 예를 들어 THF/물 중 LiOH를 사용한 에스테르 기의 가수분해에 의해, U1이 히드록실 기로 대체된 화학식 (1-b), (1-c), (1-d)의 화합물로 전환시킬 수 있다.
이어서, U1이 히드록실로 대체된 화학식 (1-c), (1-d), (1-e)의 화합물은 널리 공지된 방법에 의해 할로겐화제의 존재 하에 히드록실이 할로겐으로 대체된 화학식 (1-b), (1-c), (1-d)의 화합물로 추가로 전환시킬 수 있다. 적합한 할로겐화 시약은 삼브로민화인, 삼염화인, 오염화인, 삼염화인 옥시드, 옥살릴 클로라이드 또는 티오닐 클로라이드를 포함하나, 이에 제한되지는 않는다.
U1이 히드록실 또는 할로겐인 화학식 (1-c), (1-d), (1-e)의 화합물은 널리 공지된 방법에 의해 U1이 -N(CH3)OCH3인 화학식 (1-c), (1-d), (1-e)의 화합물로 전환시킬 수 있다.
화학식 (1-c)의 화합물은 본원에 기재된 방법 중 1개 이상에 의해 제조할 수 있다.
방법 P
화학식 (1-f)의 화합물 (즉 R8이 H인 화학식 (1))은 문헌에 기재된 방법에 의해 반응식 16에 나타낸 바와 같이 1개 이상의 단계로 화학식 (1-g)의 상응하는 화합물 (즉 R8이 반응식 16에 정의된 바와 같은 R8a인 화학식 (1)) 또는 화학식 (1-h)의 화합물 (즉 R8이 반응식 16에 정의된 바와 같은 R8b인 화학식 (1))로 전환시킬 수 있다.
반응식 16에서, Rh 및 Ri는 본원에 개시된 바와 같고, 지방족 및 시클릭 치환기 R8a 및 R8b는 본원에 개시된 바와 같이 치환될 수 있다.
전환의 비제한적 예는 방법 L에서 제공된 설명에 따라 수행할 수 있다.
이어서, 화학식 (1-f) 및 (1-g)의 수득된 화합물은 U1 (C1-C6-알콕시)이 히드록실 또는 할로겐으로 대체된 화학식 (1-f) 및 (1-g)의 화합물로 전환시킬 수 있다.
U1이 C1-C6-알콕시인 화학식 (1-f), (1-g), (1-h)의 화합물은 널리 공지된 관능기 상호전환 방법에 의해, 예를 들어 THF/물 중 LiOH를 사용한 에스테르 기의 가수분해에 의해, U1이 히드록실 기로 대체된 화학식 (1-f), (1-g), (1-h)의 화합물로 전환시킬 수 있다.
이어서, U1이 히드록실로 대체된 화학식 (1-f), (1-g), (1-h)의 화합물은 널리 공지된 방법에 의해 할로겐화제의 존재 하에 히드록실이 할로겐으로 대체된 화학식 (1-f), (1-g), (1-h)의 화합물로 추가로 전환시킬 수 있다. 적합한 할로겐화 시약은 삼브로민화인, 삼염화인, 오염화인, 삼염화인 옥시드, 옥살릴 클로라이드 또는 티오닐 클로라이드를 포함하나, 이에 제한되지는 않는다.
U1이 히드록실 또는 할로겐인 화학식 (1-f), (1-g), (1-h)의 화합물은 널리 공지된 방법에 의해 U1이 -N(CH3)OCH3인 화학식 (1-f), (1-g), (1-h)의 화합물로 전환시킬 수 있다.
화합물 (1-f)는 본원에 기재된 방법 중 1개 이상에 의해 제조할 수 있다.
화학식 (5)의 화합물의 제조 방법
본원에 기재된 바와 같은 화학식 (5)의 화합물은 상업적으로 입수가능하거나 또는 하기 기재된 방법 Q를 수행함으로써 직접 수득할 수 있다. 화학식 (5-a) 및 (5-b)의 화합물은 화학식 (5)의 다양한 하위세트이다.
방법 Q
화학식 (5-a)의 화합물 (즉 R7이 할로겐인 화학식 5의 화합물)은 공지된 방법 (WO2000044755)에 의해 산소 (에탄올), 황 (티오에틸) 또는 아미노 (메틸아민) 기재 친핵체의 존재 하에, 임의로 반응식 17에 나타낸 바와 같은 염기의 존재 하에 화학식 (5-b)의 화합물 (즉 R7이 반응식 17에 나타낸 바와 같은 것인 화학식 5의 화합물)로 전환시킬 수 있다.
화학식 (5-a) 및 (5-b)의 화합물은 방법 N에 기재된 것과 동일한 조건을 사용하여 U1 (C1-C6-알콕시)이 히드록실 또는 할로겐으로 대체된 화학식 (5-a) 및 (5-b)의 화합물로 전환시킬 수 있다.
화학식 (5-a)의 출발 물질은 상업적으로 입수가능하다.
화학식 (9) 및 (13)의 화합물의 제조 방법
화학식 (9)의 화합물은 하기 기재된 방법 R을 수행함으로써 수득할 수 있거나, 또는 본원에 기재된 방법에 따라 제조된 화학식 (9-a)의 또 다른 화합물의 전환 또는 유도체화에 의해 수득할 수 있다. 화학식 (9-a) 및 (9-b)의 화합물은 화학식 (9)의 다양한 하위세트이다.
방법 R
화학식 (9-a)의 화합물은 문헌에 기재된 방법에 의해 반응식 18에 나타낸 바와 같은 1개 이상의 단계로 상응하는 화합물 (13)으로 전환시킬 수 있다.
화학식 (33)의 화합물은 상업적으로 입수가능하거나 또는 문헌 (Chemical & Pharmaceutical Bulletin 1977, 25(8), 1856-61)에 기재된 방법에 의해 제조가능하다.
화학식 (33)의 화합물은 방법 R의 단계 1에 따라 화학식 (8)의 시약 및 본원에 기재된 바와 같은 염기 (예를 들어, 유기 또는 무기 염기)의 존재 하에 화학식 (9-a)의 화합물로 전환시킬 수 있다.
(9-a)의 (9-b)로의 전환의 비제한적 예는 반응식 18에 따라 수행할 수 있다.
예를 들어, 화학식 (9-a)의 화합물은, 화학식 (9-a)의 화합물을 산소, 황 또는 아미노 기재 친핵체로 처리함으로써, R7이 히드록실, 메르캅토, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C3-C8-시클로알킬옥시, 방향족 C6-C14-카르보시클릴옥시, 방향족 5- 또는 6-원 모노시클릭 헤테로시클릴옥시, 비-방향족 3- 내지 7-원 모노시클릭 헤테로시클릴옥시, -N(Re)2인 화학식 (9-b)의 화합물로 추가로 전환시킬 수 있다.
화학식 (9-a)의 화합물은, 본원에 기재된 바와 같은 전이 금속 촉매된 또는 금속-광산화환원 촉매된 방법에 의해, R7이 시아노, C1-C6-알킬, C1-C6-할로알킬, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C3-C8-시클로알킬, C3-C6-시클로알케닐, 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클인 화학식 (9-b)의 화합물로 전환시킬 수 있다.
화학식 (13)의 중간체는 방법 R의 단계 3에 따라 화학식 (9)의 화합물을 임의로 염기의 존재 하에 널리 공지된 방법을 사용하여 화학식 (34)의 화합물로 처리함으로써 수득할 수 있다.
화학식 (8)의 화합물은 상업적으로 입수가능하거나, 또는 널리 공지된 방법에 따라 화학식 (8)의 또 다른 화합물의 전환 또는 유도체화에 의해 수득될 수 있다.
화학식 (2), (19), (26-a-1)의 화합물의 제조 방법
방법 S
화학식 (35)의 화합물을 반응식 19에 나타낸 바와 같이 1개 이상의 단계로 문헌에 기재된 방법에 의해 상응하는 화합물 (2), (19-a), (19-b) 및 (26-a-1)로 전환시킬 수 있다.
화학식 (35)의 아미노알콜은 상업적으로 입수가능하거나 또는 문헌 (Molecules, 9 (6), 405-426; 2004, WO2017203474)에 기재된 방법에 의해 제조가능할 수 있다.
화합물 35의 아미노 관능기를 공지된 방법에 따라 보호하여 화학식 (19-a)의 화합물을 수득한다.
후속적으로, 화학식 (19-a)의 화합물은 관련 기술분야의 통상의 기술자에게 공지된 전형적 미츠노부 반응 조건을 사용하여 방법 S의 단계 2에 의해 화학식 (2)의 화합물로 전환시킬 수 있다 (문헌 [Strategic Applications of Named Reactions in Organic Synthesis; Laszlo Kuerti, Barbara Czako; Elsevier; 2005; 294-295] 및 본원의 참고문헌).
화학식 (2)의 화합물은 널리 공지된 방법에 의해 화학식 (26-a-1)의 화합물로 전환시킬 수 있다.
화합물 (B)
본 발명에 따른 활성 화합물 조합물은 화합물 (B)로서 하기 군으로부터 선택된 적어도 1종의 추가의 활성 화합물을 포함한다:
(1) 에르고스테롤 합성의 억제제,
(2) 복합체 I 또는 II에서의 호흡 사슬의 억제제,
(3) 복합체 III에서의 호흡 사슬의 억제제,
(4) 유사분열 및 세포 분열의 억제제,
(5) 다중부위 작용을 가질 수 있는 화합물,
(6) 숙주 방어를 유도할 수 있는 화합물,
(7) 아미노산 및/또는 단백질 생합성의 억제제,
(8) ATP 생산 억제제,
(9) 세포벽 합성의 억제제,
(10) 지질 및 막 합성의 억제제,
(11) 멜라닌 생합성의 억제제,
(12) 핵산 합성의 억제제,
(13) 신호 전달의 억제제,
(14) 탈커플링제로서 작용할 수 있는 화합물,
(15) 하기로 이루어진 군으로부터 선택된 다른 살진균제: (15.001) 아브시스산, (15.002) 벤티아졸, (15.003) 베톡사진, (15.004) 캡시마이신, (15.005) 카르본, (15.006) 키노메티오나트, (15.007) 쿠프라넵, (15.008) 시플루페나미드, (15.009) 시목사닐, (15.010) 시프로술파미드, (15.011) 플루티아닐, (15.012) 포세틸-알루미늄, (15.013) 포세틸-칼슘, (15.014) 포세틸-소듐, (15.015) 메틸 이소티오시아네이트, (15.016) 메트라페논, (15.017) 밀디오마이신, (15.018) 나타마이신, (15.019) 니켈 디메틸디티오카르바메이트, (15.020) 니트로탈-이소프로필, (15.021) 옥사모카르브, (15.022) 옥사티아피프롤린, (15.023) 옥시펜티인, (15.024) 펜타클로로페놀 및 염, (15.025) 아인산 및 그의 염, (15.026) 프로파모카르브-포세틸레이트, (15.027) 피리오페논 (클라자페논), (15.028) 테부플로퀸, (15.029) 테클로프탈람, (15.030) 톨니파니드, (15.031) 1-(4-{4-[(5R)-5-(2,6-디플루오로페닐)-4,5-디히드로-1,2-옥사졸-3-일]-1,3-티아졸-2-일}피페리딘-1-일)-2-[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]에타논, (15.032) 1-(4-{4-[(5S)-5-(2,6-디플루오로페닐)-4,5-디히드로-1,2-옥사졸-3-일]-1,3-티아졸-2-일}피페리딘-1-일)-2-[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]에타논, (15.033) 2-(6-벤질피리딘-2-일)퀴나졸린, (15.034) 디피메티트론, (15.035) 2-[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]-1-[4-(4-{5-[2-(프로프-2-인-1-일옥시)페닐]-4,5-디히드로-1,2-옥사졸-3-일}-1,3-티아졸-2-일)피페리딘-1-일]에타논, (15.036) 2-[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]-1-[4-(4-{5-[2-클로로-6-(프로프-2-인-1-일옥시)페닐]-4,5-디히드로-1,2-옥사졸-3-일}-1,3-티아졸-2-일)피페리딘-1-일]에타논, (15.037) 2-[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]-1-[4-(4-{5-[2-플루오로-6-(프로프-2-인-1-일옥시)페닐]-4,5-디히드로-1,2-옥사졸-3-일}-1,3-티아졸-2-일)피페리딘-1-일]에타논, (15.038) 2-[6-(3-플루오로-4-메톡시페닐)-5-메틸피리딘-2-일]퀴나졸린, (15.039) 2-{(5R)-3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-4,5-디히드로-1,2-옥사졸-5-일}-3-클로로페닐 메탄술포네이트, (15.040) 2-{(5S)-3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-4,5-디히드로-1,2-옥사졸-5-일}-3-클로로페닐 메탄술포네이트, (15.041) 이플루페노퀸, (15.042) 2-{2-플루오로-6-[(8-플루오로-2-메틸퀴놀린-3-일)옥시]페닐}프로판-2-올, (15.043) 플루옥사피프롤린, (15.044) 2-{3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-4,5-디히드로-1,2-옥사졸-5-일}페닐 메탄술포네이트, (15.045) 2-페닐페놀 및 염, (15.046) 3-(4,4,5-트리플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀린, (15.047) 퀴노푸멜린, (15.048) 4-아미노-5-플루오로피리미딘-2-올 (호변이성질체 형태: 4-아미노-5-플루오로피리미딘-2(1H)-온), (15.049) 4-옥소-4-[(2-페닐에틸)아미노]부탄산, (15.050) 5-아미노-1,3,4-티아디아졸-2-티올, (15.051) 5-클로로-N'-페닐-N'-(프로프-2-인-1-일)티오펜-2-술포노히드라지드, (15.052) 5-플루오로-2-[(4-플루오로벤질)옥시]피리미딘-4-아민, (15.053) 5-플루오로-2-[(4-메틸벤질)옥시]피리미딘-4-아민, (15.054) 9-플루오로-2,2-디메틸-5-(퀴놀린-3-일)-2,3-디히드로-1,4-벤족사제핀, (15.055) 부트-3-인-1-일 {6-[({[(Z)-(1-메틸-1H-테트라졸-5-일)(페닐)메틸렌]아미노}옥시)메틸]피리딘-2-일}카르바메이트, (15.056) 에틸 (2Z)-3-아미노-2-시아노-3-페닐아크릴레이트, (15.057) 페나진-1-카르복실산, (15.058) 프로필 3,4,5-트리히드록시벤조에이트, (15.059) 퀴놀린-8-올, (15.060) 퀴놀린-8-올 술페이트 (2:1), (15.061) tert-부틸 {6-[({[(1-메틸-1H-테트라졸-5-일)(페닐)메틸렌]아미노}옥시)메틸]피리딘-2-일}카르바메이트, (15.062) 5-플루오로-4-이미노-3-메틸-1-[(4-메틸페닐)술포닐]-3,4-디히드로피리미딘-2(1H)-온, (15.063) 아미노피리펜, (15.064) (N'-[2-클로로-4-(2-플루오로페녹시)-5-메틸페닐]-N-에틸-N-메틸이미도포름아미드), (15.065) (N'-(2-클로로-5-메틸-4-페녹시페닐)-N-에틸-N-메틸이미도포름아미드), (15.066) (2-{2-[(7,8-디플루오로-2-메틸퀴놀린-3-일)옥시]-6-플루오로페닐}프로판-2-올), (15.067) (5-브로모-1-(5,6-디메틸피리딘-3-일)-3,3-디메틸-3,4-디히드로이소퀴놀린), (15.068) (3-(4,4-디플루오로-5,5-디메틸-4,5-디히드로티에노[2,3-c]피리딘-7-일)퀴놀린), (15.069) (1-(4,5-디메틸-1H-벤즈이미다졸-1-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린), (15.070) 8-플루오로-3-(5-플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀론, (15.071) 8-플루오로-3-(5-플루오로-3,3,4,4-테트라메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀론, (15.072) 3-(4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)-8-플루오로퀴놀린, (15.073) (N-메틸-N-페닐-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드), (15.074) 메틸 {4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐}카르바메이트, (15.075) (N-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}시클로프로판카르복스아미드), (15.076) N-메틸-4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.077) N-[(E)-메톡시이미노메틸]-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.078) N-[(Z)-메톡시이미노메틸]-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.079) N-[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]시클로프로판카르복스아미드, (15.080) N-(2-플루오로페닐)-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.081) 2,2-디플루오로-N-메틸-2-[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]아세트아미드, (15.082) N-알릴-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일)페닐]메틸]아세트아미드, (15.083) N-[(E)-N-메톡시-C-메틸-카본이미도일]-4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.084) N-[(Z)-N-메톡시-C-메틸-카본이미도일]-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.085) N-알릴-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]프로판아미드, (15.086) 4,4-디메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피롤리딘-2-온, (15.087) N-메틸-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤젠카르보티오아미드, (15.088) 5-메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피롤리딘-2-온, (15.089) N-((2,3-디플루오로-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]-3,3,3-트리플루오로-프로판아미드, (15.090) 1-메톡시-1-메틸-3-[[4-[5-(트리플루오로메틸}-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.091) 1,1-디에틸-3-[[4-[5-(트리플루오로메틸}-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.092) N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]프로판아미드, (15.093) N-메톡시-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]시클로프로판카르복스아미드, (15.094) 1-메톡시-3-메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.095) N-메톡시-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸)시클로프로판카르복스아미드, (15.096) N,2-디메톡시-N-[[4-[5-(트리플루오로메틸}-1,2,4-옥사디아졸-3-일]페닐]메틸]프로판아미드, (15.097) N-에틸-2-메틸-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일)페닐]메틸]프로판아미드, (15.098) 1-메톡시-3-메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.099) 1,3-디메톡시-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.100) 3-에틸-1-메톡시-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.101) 1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피페리딘-2-온, (15.102) 4,4-디메틸-2-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.103) 5,5-디메틸-2-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.104) 3,3-디메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피페리딘-2-온, (15.105) 1-[[3-플루오로-4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]아제판-2-온, (15.106) 4,4-디메틸-2-[[4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.107) 5,5-디메틸-2-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.108) 에틸 1-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}-1H-피라졸-4-카르복실레이트, (15.109) N,N-디메틸-1-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}-1H-1,2,4-트리아졸-3-아민, (15.110) N-{2,3-디플루오로-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}부탄아미드, (15.111) N-(1-메틸시클로프로필)-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.112) N-(2,4-디플루오로페닐)-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.113) 1-(5,6-디메틸피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.114) 1-(6-(디플루오로메틸)-5-메틸-피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.115) 1-(5-(플루오로메틸)-6-메틸-피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.116) 1-(6-(디플루오로메틸)-5-메톡시-피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.117) 4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐 디메틸카르바메이트, (15.118) N-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐}프로판아미드, (15.119) 3-[2-(1-{[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.120) 9-플루오로-3-[2-(1-{[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.121) 3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.122) 3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-9-플루오로-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.123) 1-(6,7-디메틸피라졸로[1,5-a]피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.124) 8-플루오로-N-(4,4,4-트리플루오로-2-메틸-1-페닐부탄-2-일)퀴놀린-3-카르복스아미드, (15.125) 8-플루오로-N-[(2S)-4,4,4-트리플루오로-2-메틸-1-페닐부탄-2-일]퀴놀린-3-카르복스아미드, (15.126) N-(2,4-디메틸-1-페닐펜탄-2-일)-8-플루오로퀴놀린-3-카르복스아미드, (15.127) N-[(2S)-2,4-디메틸-1-페닐펜탄-2-일]-8-플루오로퀴놀린-3-카르복스아미드, (15.128) D-타가토스.
(16) 하기 군으로부터 선택된 항박테리아제: 박테리아, 예컨대 (16.001) 바실루스 서브틸리스(Bacillus subtilis), 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피(Bayer CropScience LP)로부터 세레나데 옵티(SERENADE OPTI) 또는 세레나데 아소(SERENADE ASO) 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨); (16.002) 바실루스 아밀로리퀘파시엔스(Bacillus amyloliquefaciens), 특히 균주 D747 (미국 소재의 세르티스(Certis)로부터 더블 니켈(Double Nickel)™ 하에 입수가능함, 수탁 번호 FERM BP-8234를 갖고, 미국 특허 번호 7,094,592에 개시됨); (16.003) 바실루스 푸밀루스(Bacillus pumilus), 특히 균주 BU F-33 (NRRL 등록 번호 50185를 가짐); (16.004) 바실루스 서브틸리스 변종 아밀로리퀘파시엔스 균주 FZB24 (미국 노보자임스(Novozymes)로부터 타에그로(Taegro)® 하에 입수가능함); (16.005) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주; 및
진균, 예컨대 (16.006) 아우레오바시디움 풀루란스(Aureobasidium pullulans), 특히 균주 DSM14940의 출아포자; (16.007) 균주 DSM 14941의 아우레오바시디움 풀루란스 출아포자; (16.008) 아우레오바시디움 풀루란스, 특히 균주 DSM14940 및 DSM14941의 출아포자의 혼합물;
(17) 하기의 군으로부터 선택된 생물학적 살진균제: 박테리아, 예를 들어 (17.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨); (17.002) 바실루스 푸밀루스, 특히 균주 QST2808 (미국 소재 바이엘 크롭사이언스 엘피로부터 소나타(SONATA)® 하에 입수가능함, 수탁 번호 NRRL B-30087을 갖고, 미국 특허 번호 6,245,551에 기재됨); (17.003) 바실루스 푸밀루스, 특히 균주 GB34 (독일 소재 바이엘 아게(Bayer AG)로부터 일드 쉴드(Yield Shield)® 하에 입수가능함); (17.004) 바실루스 푸밀루스, 특히 균주 BU F-33 (NRRL 수탁 번호 50185를 가짐); (17.005) 바실루스 아밀로리퀘파시엔스(Bacillus amyloliquefaciens), 특히 균주 D747 (미국 세르티스로부터 더블 니켈™ 하에 입수가능함, 수탁 번호 FERM BP-8234를 갖고, 미국 특허 번호 7,094,592에 개시됨); (17.006) 바실루스 서브틸리스 Y1336 (대만 소재 비온-테크로부터 바이오박(BIOBAC)® WP 하에 입수가능함, 타이완에 등록 번호 4764, 5454, 5096 및 5277로 생물학적 살진균제로서 등록됨); (17.007) 바실루스 아밀로리퀘파시엔스 균주 MBI 600 (바스프 에스이(BASF SE)로부터 서브틸렉스(SUBTILEX) 하에 입수가능함); (17.008) 바실루스 서브틸리스 균주 GB03 (독일 소재 바이엘 아게로부터 코디악(Kodiak)® 하에 입수가능함); (17.009) 바실루스 서브틸리스 변종 아밀로리퀘파시엔스 균주 FZB24 (버지니아주 살렘 소재 노보자임스 바이올로지칼스 인크.(Novozymes Biologicals Inc.) 또는 노스 캐롤라이나주 그린스보 소재 신젠타 크롭 프로텍션, 엘엘씨(Syngenta Crop Protection, LLC)로부터 살진균제 타에그로® 또는 타에그로® ECO 하에 입수가능함 (EPA 등록 번호 70127-5); (17.010) 바실루스 미코이데스, 단리물 J (세르티스 유에스에이(Certis USA)로부터 BmJ TGAI 또는 WG 하에 입수가능함); (17.011) 바실루스 리케니포르미스(Bacillus licheniformis), 특히 균주 SB3086 (노보자임스로부터 에코가드(EcoGuard)™ 생물살진균제 및 그린 릴리프 하에 입수가능함); (17.012) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주,
(18) 지방산 또는 유도체, 예를 들어 (18.001) 불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%는 C14 내지 C20의 범위인 조성물 (예를 들어 알파바이오 페스티시드즈(AlphaBio Pesticides) 또는 바이엘 아게의 FLiPPER).
화합물 (B)는 바람직하게는 하기로부터 선택된다:
하기로 이루어진 군으로부터 선택된 에르고스테롤 생합성의 억제제: (1.001) 시프로코나졸, (1.002) 디페노코나졸, (1.003) 에폭시코나졸, (1.004) 펜헥사미드, (1.005) 펜프로피딘, (1.006) 펜프로피모르프, (1.007) 펜피라자민, (1.008) 플루퀸코나졸, (1.009) 플루트리아폴, (1.010) 이마잘릴, (1.011) 이마잘릴 술페이트, (1.012) 이프코나졸, (1.013) 메트코나졸, (1.014) 미클로부타닐, (1.015) 파클로부트라졸, (1.016) 프로클로라즈, (1.017) 프로피코나졸, (1.018) 프로티오코나졸, (1.019) 피르이속사졸, (1.020) 스피록사민, (1.021) 테부코나졸, (1.022) 테트라코나졸, (1.023) 트리아디메놀, (1.024) 트리데모르프, (1.025) 트리티코나졸, (1.026) (1R,2S,5S)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.027) (1S,2R,5R)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.028) (2R)-2-(1-클로로시클로프로필)-4-[(1R)-2,2-디클로로시클로프로필]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.029) (2R)-2-(1-클로로시클로프로필)-4-[(1S)-2,2-디클로로시클로프로필]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.030) (2R)-2-[4-(4-클로로페녹시)-2-(트리플루오로메틸)페닐]-1-(1H-1,2,4-트리아졸-1-일)프로판-2-올, (1.031) (2S)-2-(1-클로로시클로프로필)-4-[(1R)-2,2-디클로로시클로프로필]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.032) (2S)-2-(1-클로로시클로프로필)-4-[(1S)-2,2-디클로로시클로프로필]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.033) (2S)-2-[4-(4-클로로페녹시)-2-(트리플루오로메틸)페닐]-1-(1H-1,2,4-트리아졸-1-일)프로판-2-올, (1.034) (R)-[3-(4-클로로-2-플루오로페닐)-5-(2,4-디플루오로페닐)-1,2-옥사졸-4-일](피리딘-3-일)메탄올, (1.035) (S)-[3-(4-클로로-2-플루오로페닐)-5-(2,4-디플루오로페닐)-1,2-옥사졸-4-일](피리딘-3-일)메탄올, (1.036) [3-(4-클로로-2-플루오로페닐)-5-(2,4-디플루오로페닐)-1,2-옥사졸-4-일](피리딘-3-일)메탄올, (1.037) 1-({(2R,4S)-2-[2-클로로-4-(4-클로로페녹시)페닐]-4-메틸-1,3-디옥솔란-2-일}메틸)-1H-1,2,4-트리아졸, (1.038) 1-({(2S,4S)-2-[2-클로로-4-(4-클로로페녹시)페닐]-4-메틸-1,3-디옥솔란-2-일}메틸)-1H-1,2,4-트리아졸, (1.039) 1-{[3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸-5-일 티오시아네이트, (1.040) 1-{[rel(2R,3R)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸-5-일 티오시아네이트, (1.041) 1-{[rel(2R,3S)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸-5-일 티오시아네이트, (1.042) 2-[(2R,4R,5R)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.043) 2-[(2R,4R,5S)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.044) 2-[(2R,4S,5R)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.045) 2-[(2R,4S,5S)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.046) 2-[(2S,4R,5R)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.047) 2-[(2S,4R,5S)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.048) 2-[(2S,4S,5R)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.049) 2-[(2S,4S,5S)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.050) 2-[1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.051) 2-[2-클로로-4-(2,4-디클로로페녹시)페닐]-1-(1H-1,2,4-트리아졸-1-일)프로판-2-올, (1.052) 2-[2-클로로-4-(4-클로로페녹시)페닐]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.053) 2-[4-(4-클로로페녹시)-2-(트리플루오로메틸)페닐]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.054) 2-[4-(4-클로로페녹시)-2-(트리플루오로메틸)페닐]-1-(1H-1,2,4-트리아졸-1-일)펜탄-2-올, (1.055) 메펜트리플루코나졸, (1.056) 2-{[3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.057) 2-{[rel(2R,3R)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.058) 2-{[rel(2R,3S)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.059) 5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.060) 5-(알릴술파닐)-1-{[3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸, (1.061) 5-(알릴술파닐)-1-{[rel(2R,3R)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸, (1.062) 5-(알릴술파닐)-1-{[rel(2R,3S)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸, (1.063) N'-(2,5-디메틸-4-{[3-(1,1,2,2-테트라플루오로에톡시)페닐]술파닐}페닐)-N-에틸-N-메틸이미도포름아미드, (1.064) N'-(2,5-디메틸-4-{[3-(2,2,2-트리플루오로에톡시)페닐]술파닐}페닐)N-에틸-N-메틸이미도포름아미드, (1.065) N'-(2,5-디메틸-4-{[3-(2,2,3,3-테트라플루오로프로폭시)페닐]술파닐}페닐)-N-에틸-N-메틸이미도포름아미드, (1.066) N'-(2,5-디메틸-4-{[3-(펜타플루오로에톡시)페닐]술파닐}페닐)-N-에틸-N-메틸이미도포름아미드, (1.067) N'-(2,5-디메틸-4-{3-[(1,1,2,2-테트라플루오로에틸)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드, (1.068) N'-(2,5-디메틸-4-{3-[(2,2,2-트리플루오로에틸)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드, (1.069) N'-(2,5-디메틸-4-{3-[(2,2,3,3-테트라플루오로프로필)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드, (1.070) N'-(2,5-디메틸-4-{3-[(펜타플루오로에틸)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드, (1.071) N'-(2,5-디메틸-4-페녹시페닐)-N-에틸-N-메틸이미도포름아미드, (1.072) N'-(4-{[3-(디플루오로메톡시)페닐]술파닐}-2,5-디메틸페닐)-N-에틸-N-메틸이미도포름아미드, (1.073) N'-(4-{3-[(디플루오로메틸)술파닐]페녹시}-2,5-디메틸페닐)-N-에틸-N-메틸이미도포름아미드, (1.074) N'-[5-브로모-6-(2,3-디히드로-1H-인덴-2-일옥시)-2-메틸피리딘-3-일]-N-에틸-N-메틸이미도포름아미드, (1.075) N'-{4-[(4,5-디클로로-1,3-티아졸-2-일)옥시]-2,5-디메틸페닐}-N-에틸-N-메틸이미도포름아미드, (1.076) N'-{5-브로모-6-[(1R)-1-(3,5-디플루오로페닐)에톡시]-2-메틸피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.077) N'-{5-브로모-6-[(1S)-1-(3,5-디플루오로페닐)에톡시]-2-메틸피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.078) N'-{5-브로모-6-[(시스-4-이소프로필시클로헥실)옥시]-2-메틸피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.079) N'-{5-브로모-6-[(트랜스-4-이소프로필시클로헥실)옥시]-2-메틸피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.080) N'-{5-브로모-6-[1-(3,5-디플루오로페닐)에톡시]-2-메틸피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.081) 이프펜트리플루코나졸, (1.082) 2-[4-(4-클로로페녹시)-2-(트리플루오로메틸)페닐]-1-(1H-1,2,4-트리아졸-1-일)프로판-2-올, (1.083) 2-[6-(4-브로모페녹시)-2-(트리플루오로메틸)-3-피리딜]-1-(1,2,4-트리아졸-1-일)프로판-2-올, (1.084) 2-[6-(4-클로로페녹시)-2-(트리플루오로메틸)-3-피리딜]-1-(1,2,4-트리아졸-1-일)프로판-2-올, (1.085) 3-[2-(1-클로로시클로프로필)-3-(3-클로로-2-플루오로-페닐)-2-히드록시-프로필]이미다졸-4-카르보니트릴, (1.086) 4-[[6-[rac-(2R)-2-(2,4-디플루오로페닐)-1,1-디플루오로-2-히드록시-3-(5-티옥소-4H-1,2,4-트리아졸-1-일)프로필]-3-피리딜]옥시]벤조니트릴, (1.087) N-이소프로필-N'-[5-메톡시-2-메틸-4-(2,2,2-트리플루오로-1-히드록시-1-페닐에틸)페닐]-N-메틸이미도포름아미드, (1.088) N'-{5-브로모-2-메틸-6-[(1-프로폭시프로판-2-일)옥시]피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.089) 헥사코나졸, (1.090) 펜코나졸, (1.091) 펜부코나졸, (1.092) 메틸 2-[2-클로로-4-(4-클로로페녹시)페닐]-2-히드록시-3-(1,2,4-트리아졸-1-일)프로파노에이트,
하기로 이루어진 군으로부터 선택된 복합체 I 또는 II에서의 호흡 사슬의 억제제: (2.001) 벤조빈디플루피르, (2.002) 빅사펜, (2.003) 보스칼리드, (2.004) 카르복신, (2.005) 플루오피람, (2.006) 플루톨라닐, (2.007) 플룩사피록사드, (2.008) 푸라메트피르, (2.009) 이소페타미드, (2.010) 이소피라잠 (안티-에피머 거울상이성질체 1R,4S,9S), (2.011) 이소피라잠 (안티-에피머 거울상이성질체 1S,4R,9R), (2.012) 이소피라잠 (안티-에피머 라세미체 1RS,4SR,9SR), (2.013) 이소피라잠 (신-에피머 라세미체 1RS,4SR,9RS 및 안티-에피머 라세미체 1RS,4SR,9SR의 혼합물), (2.014) 이소피라잠 (신-에피머 거울상이성질체 1R,4S,9R), (2.015) 이소피라잠 (신-에피머 거울상이성질체 1S,4R,9S), (2.016) 이소피라잠 (신-에피머 라세미체 1RS,4SR,9RS), (2.017) 펜플루펜, (2.018) 펜티오피라드, (2.019) 피디플루메토펜, (2.020) 피라지플루미드, (2.021) 세닥산, (2.022) 1,3-디메틸-N-(1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일)-1H-피라졸-4-카르복스아미드, (2.023) 1,3-디메틸-N-[(3R)-1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일]-1H-피라졸-4-카르복스아미드, (2.024) 1,3-디메틸-N-[(3S)-1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일]-1H-피라졸-4-카르복스아미드, (2.025) 1-메틸-3-(트리플루오로메틸)-N-[2'-(트리플루오로메틸)비페닐-2-일]-1H-피라졸-4-카르복스아미드, (2.026) 2-플루오로-6-(트리플루오로메틸)-N-(1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일)벤즈아미드, (2.027) 3-(디플루오로메틸)-1-메틸-N-(1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일)-1H-피라졸-4-카르복스아미드, (2.028) 인피르플룩삼, (2.029) 3-(디플루오로메틸)-1-메틸-N-[(3S)-1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일]-1H-피라졸-4-카르복스아미드, (2.030) 플루인다피르, (2.031) 3-(디플루오로메틸)-N-[(3R)-7-플루오로-1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일]-1-메틸-1H-피라졸-4-카르복스아미드, (2.032) 3-(디플루오로메틸)-N-[(3S)-7-플루오로-1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일]-1-메틸-1H-피라졸-4-카르복스아미드, (2.033) 5,8-디플루오로-N-[2-(2-플루오로-4-{[4-(트리플루오로메틸)피리딘-2-일]옥시}페닐)에틸]퀴나졸린-4-아민, (2.034) N-(2-시클로펜틸-5-플루오로벤질)-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.035) N-(2-tert-부틸-5-메틸벤질)-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.036) N-(2-tert-부틸벤질)-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.037) N-(5-클로로-2-에틸벤질)-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.038) 이소플루시프람, (2.039) N-[(1R,4S)-9-(디클로로메틸렌)-1,2,3,4-테트라히드로-1,4-메타노나프탈렌-5-일]-3-(디플루오로메틸)-1-메틸-1H-피라졸-4-카르복스아미드, (2.040) N-[(1S,4R)-9-(디클로로메틸렌)-1,2,3,4-테트라히드로-1,4-메타노나프탈렌-5-일]-3-(디플루오로메틸)-1-메틸-1H-피라졸-4-카르복스아미드, (2.041) N-[1-(2,4-디클로로페닐)-1-메톡시프로판-2-일]-3-(디플루오로메틸)-1-메틸-1H-피라졸-4-카르복스아미드, (2.042) N-[2-클로로-6-(트리플루오로메틸)벤질]-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.043) N-[3-클로로-2-플루오로-6-(트리플루오로메틸)벤질]-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.044) N-[5-클로로-2-(트리플루오로메틸)벤질]-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.045) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-N-[5-메틸-2-(트리플루오로메틸)벤질]-1H-피라졸-4-카르복스아미드, (2.046) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-N-(2-플루오로-6-이소프로필벤질)-1-메틸-1H-피라졸-4-카르복스아미드, (2.047) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-N-(2-이소프로필-5-메틸벤질)-1-메틸-1H-피라졸-4-카르복스아미드, (2.048) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-N-(2-이소프로필벤질)-1-메틸-1H-피라졸-4-카르보티오아미드, (2.049) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-N-(2-이소프로필벤질)-1-메틸-1H-피라졸-4-카르복스아미드, (2.050) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-N-(5-플루오로-2-이소프로필벤질)-1-메틸-1H-피라졸-4-카르복스아미드, (2.051) N-시클로프로필-3-(디플루오로메틸)-N-(2-에틸-4,5-디메틸벤질)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.052) N-시클로프로필-3-(디플루오로메틸)-N-(2-에틸-5-플루오로벤질)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.053) N-시클로프로필-3-(디플루오로메틸)-N-(2-에틸-5-메틸벤질)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.054) N-시클로프로필-N-(2-시클로프로필-5-플루오로벤질)-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.055) N-시클로프로필-N-(2-시클로프로필-5-메틸벤질)-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.056) N-시클로프로필-N-(2-시클로프로필벤질)-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.057) 피라프로포인, (2.058) N-[rac-(1S,2S)-2-(2,4-디클로로페닐)시클로부틸]-2-(트리플루오로메틸)니코틴아미드, (2.059) N-[(1S,2S)-2-(2,4-디클로로페닐)시클로부틸]-2-(트리플루오로메틸)니코틴아미드, (2.060) 플루베네테람,
하기로 이루어진 군으로부터 선택된 복합체 III에서의 호흡 사슬의 억제제: (3.001) 아메톡트라딘, (3.002) 아미술브롬, (3.003) 아족시스트로빈, (3.004) 쿠메톡시스트로빈, (3.005) 쿠목시스트로빈, (3.006) 시아조파미드, (3.007) 디목시스트로빈, (3.008)에녹사스트로빈, (3.009) 파목사돈, (3.010) 페나미돈, (3.011) 플루페녹시스트로빈, (3.012) 플루옥사스트로빈, (3.013) 크레속심-메틸, (3.014) 메토미노스트로빈, (3.015) 오리사스트로빈, (3.016) 피콕시스트로빈, (3.017) 피라클로스트로빈, (3.018) 피라메토스트로빈, (3.019) 피라옥시스트로빈, (3.020) 트리플록시스트로빈, (3.021) (2E)-2-{2-[({[(1E)-1-(3-{[(E)-1-플루오로-2-페닐비닐]옥시}페닐)에틸리덴]아미노}옥시)메틸]페닐}-2-(메톡시이미노)-N-메틸아세트아미드, (3.022) (2E,3Z)-5-{[1-(4-클로로페닐)-1H-피라졸-3-일]옥시}-2-(메톡시이미노)-N,3-디메틸펜트-3-엔아미드, (3.023) (2R)-2-{2-[(2,5-디메틸페녹시)메틸]페닐}-2-메톡시-N-메틸아세트아미드, (3.024) (2S)-2-{2-[(2,5-디메틸페녹시)메틸]페닐}-2-메톡시-N-메틸아세트아미드, (3.025) 펜피콕사미드, (3.026) 만데스트로빈, (3.027) N-(3-에틸-3,5,5-트리메틸시클로헥실)-3-포름아미도-2-히드록시벤즈아미드, (3.028) (2E,3Z)-5-{[1-(4-클로로-2-플루오로페닐)-1H-피라졸-3-일]옥시}-2-(메톡시이미노)-N,3-디메틸펜트-3-엔아미드, (3.029) 메틸 {5-[3-(2,4-디메틸페닐)-1H-피라졸-1-일]-2-메틸벤질}카르바메이트, (3.030) 메틸테트라프롤, (3.031) 플로릴피콕사미드, (3.032) (2S,3S)-3-(o-톨릴)부탄-2-일 N-{[4-메톡시-3-(프로파노일옥시)-2-피리딜]카르보닐}-L-알라니네이트,
하기로 이루어진 군으로부터 선택된 유사분열 및 세포 분열의 억제제: (4.001) 카르벤다짐, (4.002) 디에토펜카르브, (4.003) 에타복삼, (4.004) 플루오피콜리드, (4.005) 펜시쿠론, (4.006) 티아벤다졸, (4.007) 티오파네이트-메틸, (4.008) 족사미드, (4.009) 피리다클로메틸, (4.010) 3-클로로-5-(4-클로로페닐)-4-(2,6-디플루오로페닐)-6-메틸피리다진, (4.011) 3-클로로-5-(6-클로로피리딘-3-일)-6-메틸-4-(2,4,6-트리플루오로페닐)피리다진, (4.012) 4-(2-브로모-4-플루오로페닐)-N-(2,6-디플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.013) 4-(2-브로모-4-플루오로페닐)-N-(2-브로모-6-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.014) 4-(2-브로모-4-플루오로페닐)-N-(2-브로모페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.015) 4-(2-브로모-4-플루오로페닐)-N-(2-클로로-6-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.016) 4-(2-브로모-4-플루오로페닐)-N-(2-클로로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.017) 4-(2-브로모-4-플루오로페닐)-N-(2-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.018) 4-(2-클로로-4-플루오로페닐)-N-(2,6-디플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.019) 4-(2-클로로-4-플루오로페닐)-N-(2-클로로-6-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.020) 4-(2-클로로-4-플루오로페닐)-N-(2-클로로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.021) 4-(2-클로로-4-플루오로페닐)-N-(2-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.022) 4-(4-클로로페닐)-5-(2,6-디플루오로페닐)-3,6-디메틸피리다진, (4.023) N-(2-브로모-6-플루오로페닐)-4-(2-클로로-4-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.024) N-(2-브로모페닐)-4-(2-클로로-4-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.025) N-(4-클로로-2,6-디플루오로페닐)-4-(2-클로로-4-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.026) 플루오피모미드,
하기로 이루어진 군으로부터 선택된 다중부위 작용을 가질 수 있는 화합물: (5.001) 보르도 혼합물, (5.002) 캅타폴, (5.003) 캅탄, (5.004) 클로로탈로닐, (5.005) 수산화구리, (5.006) 나프텐산구리, (5.007) 산화구리, (5.008) 옥시염화구리, (5.009) 황산구리(2+), (5.010) 디티아논, (5.011) 도딘, (5.012) 폴페트, (5.013) 만코제브, (5.014) 마네브, (5.015) 메티람, (5.016) 메티람 아연, (5.017) 옥신-구리, (5.018) 프로피네브, (5.019) 황 및 칼슘 폴리술피드를 포함하는 황 제제, (5.020) 티람, (5.021) 지네브, (5.022) 지람, (5.023) 6-에틸-5,7-디옥소-6,7-디히드로-5H-피롤로[3',4':5,6][1,4]디티이노[2,3-c][1,2]티아졸-3-카르보니트릴,
(6.001) 아시벤졸라르-S-메틸, (6.002) 이소티아닐, (6.003) 프로베나졸, (6.004) 티아디닐로 이루어진 군으로부터 선택된, 숙주 방어를 유도할 수 있는 화합물,
(7.001) 시프로디닐, (7.002) 카수가마이신, (7.003) 카수가마이신 히드로클로라이드 수화물, (7.004) 옥시테트라시클린, (7.005) 피리메타닐, (7.006) 3-(5-플루오로-3,3,4,4-테트라메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀린으로 이루어진 군으로부터 선택된 아미노산 및/또는 단백질 생합성의 억제제,
(8.001) 실티오팜으로 이루어진 군으로부터 선택된 ATP 생산 억제제,
하기로 이루어진 군으로부터 선택된 세포벽 합성의 억제제: (9.001) 벤티아발리카르브, (9.002) 디메토모르프, (9.003) 플루모르프, (9.004) 이프로발리카르브, (9.005) 만디프로파미드, (9.006) 피리모르프, (9.007) 발리페날레이트, (9.008) (2E)-3-(4-tert-부틸페닐)-3-(2-클로로피리딘-4-일)-1-(모르폴린-4-일)프로프-2-엔-1-온, (9.009) (2Z)-3-(4-tert-부틸페닐)-3-(2-클로로피리딘-4-일)-1-(모르폴린-4-일)프로프-2-엔-1-온,
(10.001) 프로파모카르브, (10.002) 프로파모카르브 히드로클로라이드, (10.003) 톨클로포스-메틸로 이루어진 군으로부터 선택된 지질 및 막 합성의 억제제,
(11.001) 트리시클라졸, (11.002) 톨프로카르브로 이루어진 군으로부터 선택된 멜라닌 생합성의 억제제,
(12.001) 베날락실, (12.002) 베날락실-M (키랄락실), (12.003) 메탈락실, (12.004) 메탈락실-M (메페녹삼)으로 이루어진 군으로부터 선택된 핵산 합성의 억제제,
(13.001) 플루디옥소닐, (13.002) 이프로디온, (13.003) 프로시미돈, (13.004) 프로퀴나지드, (13.005) 퀴녹시펜, (13.006) 빈클로졸린으로 이루어진 군으로부터 선택된 신호 전달의 억제제,
(14.001) 플루아지남, (14.002) 멥틸디노캅으로 이루어진 군으로부터 선택된 탈커플링제로서 작용할 수 있는 화합물,
하기로 이루어진 군으로부터 선택된 추가의 살진균제: (15.001) 아브시스산, (15.002) 벤티아졸, (15.003) 베톡사진, (15.004) 캡시마이신, (15.005) 카르본, (15.006) 키노메티오나트, (15.007) 쿠프라넵, (15.008) 시플루페나미드, (15.009) 시목사닐, (15.010) 시프로술파미드, (15.011) 플루티아닐, (15.012) 포세틸-알루미늄, (15.013) 포세틸-칼슘, (15.014) 포세틸-소듐, (15.015) 메틸 이소티오시아네이트, (15.016) 메트라페논, (15.017) 밀디오마이신, (15.018) 나타마이신, (15.019) 니켈 디메틸디티오카르바메이트, (15.020) 니트로탈-이소프로필, (15.021) 옥사모카르브, (15.022) 옥사티아피프롤린, (15.023) 옥시펜티인, (15.024) 펜타클로로페놀 및 염, (15.025) 아인산 및 그의 염, (15.026) 프로파모카르브-포세틸레이트, (15.027) 피리오페논 (클라자페논), (15.028) 테부플로퀸, (15.029) 테클로프탈람, (15.030) 톨니파니드, (15.031) 1-(4-{4-[(5R)-5-(2,6-디플루오로페닐)-4,5-디히드로-1,2-옥사졸-3-일]-1,3-티아졸-2-일}피페리딘-1-일)-2-[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]에타논, (15.032) 1-(4-{4-[(5S)-5-(2,6-디플루오로페닐)-4,5-디히드로-1,2-옥사졸-3-일]-1,3-티아졸-2-일}피페리딘-1-일)-2-[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]에타논, (15.033) 2-(6-벤질피리딘-2-일)퀴나졸린, (15.034) 디피메티트론, (15.035) 2-[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]-1-[4-(4-{5-[2-(프로프-2-인-1-일옥시)페닐]-4,5-디히드로-1,2-옥사졸-3-일}-1,3-티아졸-2-일)피페리딘-1-일]에타논, (15.036) 2-[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]-1-[4-(4-{5-[2-클로로-6-(프로프-2-인-1-일옥시)페닐]-4,5-디히드로-1,2-옥사졸-3-일}-1,3-티아졸-2-일)피페리딘-1-일]에타논, (15.037) 2-[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]-1-[4-(4-{5-[2-플루오로-6-(프로프-2-인-1-일옥시)페닐]-4,5-디히드로-1,2-옥사졸-3-일}-1,3-티아졸-2-일)피페리딘-1-일]에타논, (15.038) 2-[6-(3-플루오로-4-메톡시페닐)-5-메틸피리딘-2-일]퀴나졸린, (15.039) 2-{(5R)-3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-4,5-디히드로-1,2-옥사졸-5-일}-3-클로로페닐 메탄술포네이트, (15.040) 2-{(5S)-3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-4,5-디히드로-1,2-옥사졸-5-일}-3-클로로페닐 메탄술포네이트, (15.041) 이플루페노퀸, (15.042) 2-{2-플루오로-6-[(8-플루오로-2-메틸퀴놀린-3-일)옥시]페닐}프로판-2-올, (15.043) 플루옥사피프롤린, (15.044) 2-{3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-4,5-디히드로-1,2-옥사졸-5-일}페닐 메탄술포네이트, (15.045) 2-페닐페놀 및 염, (15.046) 3-(4,4,5-트리플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀린, (15.047) 퀴노푸멜린, (15.048) 4-아미노-5-플루오로피리미딘-2-올 (호변이성질체 형태: 4-아미노-5-플루오로피리미딘-2(1H)-온), (15.049) 4-옥소-4-[(2-페닐에틸)아미노]부탄산, (15.050) 5-아미노-1,3,4-티아디아졸-2-티올, (15.051) 5-클로로-N'-페닐-N'-(프로프-2-인-1-일)티오펜-2-술포노히드라지드, (15.052) 5-플루오로-2-[(4-플루오로벤질)옥시]피리미딘-4-아민, (15.053) 5-플루오로-2-[(4-메틸벤질)옥시]피리미딘-4-아민, (15.054) 9-플루오로-2,2-디메틸-5-(퀴놀린-3-일)-2,3-디히드로-1,4-벤족사제핀, (15.055) 부트-3-인-1-일 {6-[({[(Z)-(1-메틸-1H-테트라졸-5-일)(페닐)메틸렌]아미노}옥시)메틸]피리딘-2-일}카르바메이트, (15.056) 에틸 (2Z)-3-아미노-2-시아노-3-페닐아크릴레이트, (15.057) 페나진-1-카르복실산, (15.058) 프로필 3,4,5-트리히드록시벤조에이트, (15.059) 퀴놀린-8-올, (15.060) 퀴놀린-8-올 술페이트 (2:1), (15.061) tert-부틸 {6-[({[(1-메틸-1H-테트라졸-5-일)(페닐)메틸렌]아미노}옥시)메틸]피리딘-2-일}카르바메이트, (15.062) 5-플루오로-4-이미노-3-메틸-1-[(4-메틸페닐)술포닐]-3,4-디히드로피리미딘-2(1H)-온, (15.063) 아미노피리펜, (15.064) (N'-[2-클로로-4-(2-플루오로페녹시)-5-메틸페닐]-N-에틸-N-메틸이미도포름아미드), (15.065) (N'-(2-클로로-5-메틸-4-페녹시페닐)-N-에틸-N-메틸이미도포름아미드), (15.066) (2-{2-[(7,8-디플루오로-2-메틸퀴놀린-3-일)옥시]-6-플루오로페닐}프로판-2-올), (15.067) (5-브로모-1-(5,6-디메틸피리딘-3-일)-3,3-디메틸-3,4-디히드로이소퀴놀린), (15.068) (3-(4,4-디플루오로-5,5-디메틸-4,5-디히드로티에노[2,3-c]피리딘-7-일)퀴놀린), (15.069) (1-(4,5-디메틸-1H-벤즈이미다졸-1-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린), (15.070) 8-플루오로-3-(5-플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀론, (15.071) 8-플루오로-3-(5-플루오로-3,3,4,4-테트라메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀론, (15.072) 3-(4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)-8-플루오로퀴놀린, (15.073) (N-메틸-N-페닐-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드), (15.074) 메틸 {4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐}카르바메이트, (15.075) (N-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}시클로프로판카르복스아미드), (15.076) N-메틸-4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.077) N-[(E)-메톡시이미노메틸]-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.078) N-[(Z)-메톡시이미노메틸]-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.079) N-[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]시클로프로판카르복스아미드, (15.080) N-(2-플루오로페닐)-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.081) 2,2-디플루오로-N-메틸-2-[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]아세트아미드, (15.082) N-알릴-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일)페닐]메틸]아세트아미드, (15.083) N-[(E)-N-메톡시-C-메틸-카본이미도일]-4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.084) N-[(Z)-N-메톡시-C-메틸-카본이미도일]-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.085) N-알릴-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]프로판아미드, (15.086) 4,4-디메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피롤리딘-2-온, (15.087) N-메틸-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤젠카르보티오아미드, (15.088) 5-메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피롤리딘-2-온, (15.089) N-((2,3-디플루오로-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]-3,3,3-트리플루오로-프로판아미드, (15.090) 1-메톡시-1-메틸-3-[[4-[5-(트리플루오로메틸}-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.091) 1,1-디에틸-3-[[4-[5-(트리플루오로메틸}-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.092) N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]프로판아미드, (15.093) N-메톡시-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]시클로프로판카르복스아미드, (15.094) 1-메톡시-3-메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.095) N-메톡시-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸)시클로프로판카르복스아미드, (15.096) N,2-디메톡시-N-[[4-[5-(트리플루오로메틸}-1,2,4-옥사디아졸-3-일]페닐]메틸]프로판아미드, (15.097) N-에틸-2-메틸-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일)페닐]메틸]프로판아미드, (15.098) 1-메톡시-3-메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.099) 1,3-디메톡시-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.100) 3-에틸-1-메톡시-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.101) 1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피페리딘-2-온, (15.102) 4,4-디메틸-2-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.103) 5,5-디메틸-2-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.104) 3,3-디메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피페리딘-2-온, (15.105) 1-[[3-플루오로-4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]아제판-2-온, (15.106) 4,4-디메틸-2-[[4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.107) 5,5-디메틸-2-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.108) 에틸 1-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}-1H-피라졸-4-카르복실레이트, (15.109) N,N-디메틸-1-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}-1H-1,2,4-트리아졸-3-아민, (15.110) N-{2,3-디플루오로-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}부탄아미드, (15.111) N-(1-메틸시클로프로필)-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.112) N-(2,4-디플루오로페닐)-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.113) 1-(5,6-디메틸피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.114) 1-(6-(디플루오로메틸)-5-메틸-피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.115) 1-(5-(플루오로메틸)-6-메틸-피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.116) 1-(6-(디플루오로메틸)-5-메톡시-피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.117) 4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐 디메틸카르바메이트, (15.118) N-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐}프로판아미드, (15.119) 3-[2-(1-{[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.120) 9-플루오로-3-[2-(1-{[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.121) 3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.122) 3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-9-플루오로-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.123) 1-(6,7-디메틸피라졸로[1,5-a]피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.124) 8-플루오로-N-(4,4,4-트리플루오로-2-메틸-1-페닐부탄-2-일)퀴놀린-3-카르복스아미드, (15.125) 8-플루오로-N-[(2S)-4,4,4-트리플루오로-2-메틸-1-페닐부탄-2-일]퀴놀린-3-카르복스아미드, (15.126) N-(2,4-디메틸-1-페닐펜탄-2-일)-8-플루오로퀴놀린-3-카르복스아미드, (15.127) N-[(2S)-2,4-디메틸-1-페닐펜탄-2-일]-8-플루오로퀴놀린-3-카르복스아미드, (15.128) D-타가토스,
박테리아, 예컨대 (16.001) 바실루스 서브틸리스(Bacillus subtilis), 특히 균주 QST713/AQ713 (미국 소재의 바이엘 크롭사이언스 엘피(Bayer CropScience LP)로부터 세레나데 옵티(SERENADE OPTI) 또는 세레나데 아소(SERENADE ASO) 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨); (16.002) 바실루스 아밀로리퀘파시엔스(Bacillus amyloliquefaciens), 특히 균주 D747 (미국 소재의 세르티스(Certis)로부터 더블 니켈™ 하에 입수가능함, 수탁 번호 FERM BP-8234를 갖고, 미국 특허 번호 7,094,592에 개시됨); (16.003) 바실루스 푸밀루스(Bacillus pumilus), 특히 균주 BU F-33 (NRRL 수탁 번호 50185를 가짐); (16.004) 바실루스 서브틸리스 변종 아밀로리퀘파시엔스 균주 FZB24 (미국 소재 노보자임스로부터 타에그로® 하에 입수가능함); (16.005) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스(Paenibacillus) 종 균주; 및 진균, 예컨대 (16.006) 아우레오바시디움 풀루란스(Aureobasidium pullulans), 특히 균주 DSM14940의 출아포자; (16.007) 균주 DSM 14941의 아우레오바시디움 풀루란스 출아포자; (16.008) 아우레오바시디움 풀루란스, 특히 균주 DSM14940 및 DSM14941의 출아포자의 혼합물로 이루어진 군으로부터 선택된 항박테리아제,
박테리아로 이루어진 군으로부터 선택된 생물학적 살진균제, 예를 들어, (17.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨); (17.002) 바실루스 푸밀루스, 특히 균주 QST2808 (미국 소재 바이엘 크롭사이언스 엘피로부터 소나타(SONATA)® 하에 입수가능함, 수탁 번호 NRRL B-30087을 갖고, 미국 특허 번호 6,245,551에 기재됨); (17.003) 바실루스 푸밀루스, 특히 균주 GB34 (독일 소재 바이엘 아게로부터 일드 쉴드® 하에 입수가능함); (17.004) 바실루스 푸밀루스, 특히 균주 BU F-33 (NRRL 수탁 번호 50185를 가짐); (17.005) 바실루스 아밀로리퀘파시엔스(Bacillus amyloliquefaciens), 특히 균주 D747 (미국 세르티스로부터 더블 니켈™ 하에 입수가능함, 수탁 번호 FERM BP-8234를 갖고, 미국 특허 번호 7,094,592에 개시됨); (17.006) 바실루스 서브틸리스 Y1336 (대만 소재 비온-테크로부터 바이오박® WP 하에 입수가능함, 타이완에 등록 번호 4764, 5454, 5096 및 5277로 생물학적 살진균제로서 등록됨); (17.007) 바실루스 아밀로리퀘파시엔스 균주 MBI 600 (바스프 에스이(BASF SE)로부터 서브틸렉스(SUBTILEX) 하에 입수가능함); (17.008) 바실루스 서브틸리스 균주 GB03 (독일 소재 바이엘 아게로부터 코디악® 하에 입수가능함); (17.009) 바실루스 서브틸리스 변종 아밀로리퀘파시엔스 균주 FZB24 (버지니아주 살렘 소재 노보자임스 바이올로지칼스 인크. 또는 노스 캐롤라이나주 그린스보 소재 신젠타 크롭 프로텍션, 엘엘씨로부터 살진균제 타에그로® 또는 타에그로® ECO 하에 입수가능함 (EPA 등록 번호 70127-5); (17.010) 바실루스 미코이데스, 단리물 J (세르티스 유에스에이로부터 BmJ TGAI 또는 WG 하에 입수가능함); (17.011) 바실루스 리케니포르미스(Bacillus licheniformis), 특히 균주 SB3086 (노보자임스로부터 에코가드™ 생물살진균제 및 그린 릴리프 하에 입수가능함); (17.012) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주,
지방산 또는 유도체, 예를 들어 (18.001) 불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%는 C14 내지 C20의 범위인 조성물 (예를 들어 알파바이오 페스티시드즈 또는 바이엘 아게의 FLiPPER).
화합물 (B)는 보다 바람직하게는 하기로부터 선택된다:
(1.001) 시프로코나졸, (1.002) 디페노코나졸, (1.003) 에폭시코나졸, (1.004) 펜헥사미드, (1.010) 이마잘릴, (1.012) 이프코나졸, (1.013) 메트코나졸, (1.017) 프로피코나졸, (1.018) 프로티오코나졸, (1.020) 스피록사민, (1.021) 테부코나졸, (1.026) (1R,2S,5S)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.027) (1S,2R,5R)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.055) 메펜트리플루코나졸, (1.059) 5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.062) 플루옥시티오코나졸, (1.067) N'-(2,5-디메틸-4-{3-[(1,1,2,2-테트라플루오로에틸)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드, (1.081) 이프펜트리플루코나졸, (1.082) 2-[6-(4-브로모페녹시)-2-(트리플루오로메틸)-3-피리딜]-1-(1,2,4-트리아졸-1-일)프로판-2-올 및, (1.092) 메틸 2-[2-클로로-4-(4-클로로페녹시)페닐]-2-히드록시-3-(1,2,4-트리아졸-1-일)프로파노에이트
(2.001) 벤조빈디플루피르, (2.002) 빅사펜, (2.003) 보스칼리드, (2.005) 플루오피람, (2.007) 플룩사피록사드, (2.009) 이소페타미드, (2.010) 이소피라잠 (안티-에피머 거울상이성질체 1R,4S,9S), (2.011) 이소피라잠 (안티-에피머 거울상이성질체 1S,4R,9R), (2.012) 이소피라잠 (안티-에피머 라세미체 1RS,4SR,9SR), (2.013) 이소피라잠 (신-에피머 라세미체 1RS,4SR,9RS 및 안티-에피머 라세미체 1RS,4SR,9SR의 혼합물), (2.014) 이소피라잠 (신-에피머 거울상이성질체 1R,4S,9R), (2.015) 이소피라잠 (신-에피머 거울상이성질체 1S,4R,9S), (2.016) 이소피라잠 (신-에피머 라세미체 1RS,4SR,9RS), (2.017) 펜플루펜, (2.018) 펜티오피라드, (2.019) 피디플루메토펜, (2.021) 세닥산, (2.028) 인피르플룩삼, (2.030) 플루인다피르, (2.038) 이소플루시프람,
(3.003) 아족시스트로빈, (3.007) 디목시스트로빈, (3.012) 플루옥사스트로빈, (3.013) 크레속심-메틸, (3.016) 피콕시스트로빈, (3.017) 피라클로스트로빈, (3.020) 트리플록시스트로빈, (3.025) 펜피콕사미드, (3.026) 2-{2-[(2,5-디메틸페녹시)메틸]페닐}-2-메톡시-N-메틸아세트아미드, (3.030) 메틸테트라프롤, (3.031) 플로릴피콕사미드,
(4.005) 펜시쿠론, (4.007) 티오파네이트-메틸, (4.012) 4-(2-브로모-4-플루오로페닐)-N-(2,6-디플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.015) 4-(2-브로모-4-플루오로페닐)-N-(2-클로로-6-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.025) N-(4-클로로-2,6-디플루오로페닐)-4-(2-클로로-4-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민,
(5.003) 캅탄, (5.004) 클로로탈로닐, (5.010), 디티아논, (5.011) 도딘, (5.012) 폴페트, (5.013) 만코제브, (5.015) 메티람, (5.018) 프로피네브,
(6.002) 이소티아닐,
(7.001) 시프로디닐, (7.005) 피리메타닐,
(12.003) 메탈락실, (12.004) 메탈락실-M (메페녹삼),
(13.001) 플루디옥소닐, (13.002) 이프로디온, (13.004) 프로퀴나지드, (13.005) 퀴녹시펜,
(14.001) 플루아지남, (14.002) 멥틸디노캅,
(15.008) 시플루페나미드, (15.010) 시프로술파미드, (15.011) 플루티아닐, (15.012) 포세틸-알루미늄, (15.016) 메트라페논, (15.027) 피리오페논 (클라자페논), (15.043) 플루옥사피프롤린, (15.047) 3-(4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀론, (15.048) 4-아미노-5-플루오로피리미딘-2-올 (호변이성질체 형태: 4-아미노-5-플루오로피리미딘-2(1H)-온), (15.052) 5-플루오로-2-[(4-플루오로벤질)옥시]피리미딘-4-아민, (15.053) 5-플루오로-2-[(4-메틸벤질)옥시]피리미딘-4-아민, (15.062) 5-플루오로-4-이미노-3-메틸-1-[(4-메틸페닐)술포닐]-3,4-디히드로피리미딘-2(1H)-온, (15.063) 아미노피리펜, (15.064) (N'-[2-클로로-4-(2-플루오로페녹시)-5-메틸페닐]-N-에틸-N-메틸이미도포름아미드),
(16.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨),
(17.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨); (17.002) 바실루스 푸밀루스, 특히 균주 QST2808 (미국 소재 바이엘 크롭사이언스 엘피로부터 소나타(SONATA)® 하에 입수가능함, 수탁 번호 NRRL B-30087을 갖고, 미국 특허 번호 6,245,551에 기재됨); (17.003) 바실루스 푸밀루스, 특히 균주 GB34 (독일 소재 바이엘 아게로부터 일드 쉴드® 하에 입수가능함); (17.008) 바실루스 서브틸리스 균주 GB03 (독일 소재 바이엘 아게로부터 코디악® 하에 입수가능함); (17.009) 바실루스 서브틸리스 변종 아밀로리퀘파시엔스 균주 FZB24 (버지니아주 살렘 소재 노보자임스 바이올로지칼스 인크. 또는 노스 캐롤라이나주 그린스보 소재 신젠타 크롭 프로텍션, 엘엘씨로부터 살진균제 타에그로® 또는 타에그로® ECO 하에 입수가능함 (EPA 등록 번호 70127-5); (17.011) 바실루스 리케니포르미스(Bacillus licheniformis), 특히 균주 SB3086 (노보자임스로부터 에코가드™ 생물살진균제 및 그린 릴리프 하에 입수가능함); (17.012) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주,
(18.001) 불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%는 C14 내지 C20의 범위인 조성물 (예를 들어 알파바이오 페스티시드즈 또는 바이엘 아게의 FLiPPER).
화합물 (B)는 또한 보다 바람직하게는 하기로부터 선택된다:
(1.001) 시프로코나졸, (1.002) 디페노코나졸, (1.003) 에폭시코나졸, (1.004) 펜헥사미드, (1.010) 이마잘릴, (1.012) 이프코나졸, (1.013) 메트코나졸, (1.017) 프로피코나졸, (1.018) 프로티오코나졸, (1.020) 스피록사민, (1.021) 테부코나졸, (1.026) (1R,2S,5S)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.027) (1S,2R,5R)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.055) 메펜트리플루코나졸, (1.059) 5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.081) 이프펜트리플루코나졸, (1.082) 2-[6-(4-브로모페녹시)-2-(트리플루오로메틸)-3-피리딜]-1-(1,2,4-트리아졸-1-일)프로판-2-올 및, (1.092) 메틸 2-[2-클로로-4-(4-클로로페녹시)페닐]-2-히드록시-3-(1,2,4-트리아졸-1-일)프로파노에이트
(2.001) 벤조빈디플루피르, (2.002) 빅사펜, (2.003) 보스칼리드, (2.005) 플루오피람, (2.007) 플룩사피록사드, (2.009) 이소페타미드, (2.010) 이소피라잠 (안티-에피머 거울상이성질체 1R,4S,9S), (2.011) 이소피라잠 (안티-에피머 거울상이성질체 1S,4R,9R), (2.012) 이소피라잠 (안티-에피머 라세미체 1RS,4SR,9SR), (2.013) 이소피라잠 (신-에피머 라세미체 1RS,4SR,9RS 및 안티-에피머 라세미체 1RS,4SR,9SR의 혼합물), (2.014) 이소피라잠 (신-에피머 거울상이성질체 1R,4S,9R), (2.015) 이소피라잠 (신-에피머 거울상이성질체 1S,4R,9S), (2.016) 이소피라잠 (신-에피머 라세미체 1RS,4SR,9RS), (2.017) 펜플루펜, (2.018) 펜티오피라드, (2.019) 피디플루메토펜, (2.021) 세닥산, (2.028) 인피르플룩삼, (2.030) 플루인다피르, (2.038) 이소플루시프람,
(3.003) 아족시스트로빈, (3.007) 디목시스트로빈, (3.012) 플루옥사스트로빈, (3.013) 크레속심-메틸, (3.016) 피콕시스트로빈, (3.017) 피라클로스트로빈, (3.020) 트리플록시스트로빈, (3.025) 펜피콕사미드, (3.026) 2-{2-[(2,5-디메틸페녹시)메틸]페닐}-2-메톡시-N-메틸아세트아미드, (3.030) 메틸테트라프롤, (3.031) 플로릴피콕사미드,
(4.005) 펜시쿠론, (4.007) 티오파네이트-메틸, (4.012) 4-(2-브로모-4-플루오로페닐)-N-(2,6-디플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.015) 4-(2-브로모-4-플루오로페닐)-N-(2-클로로-6-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.025) N-(4-클로로-2,6-디플루오로페닐)-4-(2-클로로-4-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민,
(5.003) 캅탄, (5.004) 클로로탈로닐, (5.010), 디티아논, (5.011) 도딘, (5.012) 폴페트, (5.013) 만코제브, (5.015) 메티람, (5.018) 프로피네브,
(6.002) 이소티아닐,
(7.001) 시프로디닐, (7.005) 피리메타닐,
(12.003) 메탈락실, (12.004) 메탈락실-M (메페녹삼),
(13.001) 플루디옥소닐, (13.002) 이프로디온, (13.004) 프로퀴나지드, (13.005) 퀴녹시펜,
(14.001) 플루아지남, (14.002) 멥틸디노캅,
(15.008) 시플루페나미드, (15.010) 시프로술파미드, (15.011) 플루티아닐, (15.012) 포세틸-알루미늄, (15.016) 메트라페논, (15.027) 피리오페논 (클라자페논), (15.047) 3-(4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀론, (15.048) 4-아미노-5-플루오로피리미딘-2-올 (호변이성질체 형태: 4-아미노-5-플루오로피리미딘-2(1H)-온), (15.052) 5-플루오로-2-[(4-플루오로벤질)옥시]피리미딘-4-아민, (15.053) 5-플루오로-2-[(4-메틸벤질)옥시]피리미딘-4-아민, (15.062) 5-플루오로-4-이미노-3-메틸-1-[(4-메틸페닐)술포닐]-3,4-디히드로피리미딘-2(1H)-온, (15.063) 아미노피리펜, (15.064) (N'-[2-클로로-4-(2-플루오로페녹시)-5-메틸페닐]-N-에틸-N-메틸이미도포름아미드),
(16.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨),
(17.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨); (17.002) 바실루스 푸밀루스, 특히 균주 QST2808 (미국 소재 바이엘 크롭사이언스 엘피로부터 소나타(SONATA)® 하에 입수가능함, 수탁 번호 NRRL B-30087을 갖고, 미국 특허 번호 6,245,551에 기재됨); (17.003) 바실루스 푸밀루스, 특히 균주 GB34 (독일 소재 바이엘 아게로부터 일드 쉴드® 하에 입수가능함); (17.008) 바실루스 서브틸리스 균주 GB03 (독일 소재 바이엘 아게로부터 코디악® 하에 입수가능함); (17.009) 바실루스 서브틸리스 변종 아밀로리퀘파시엔스 균주 FZB24 (버지니아주 살렘 소재 노보자임스 바이올로지칼스 인크. 또는 노스 캐롤라이나주 그린스보 소재 신젠타 크롭 프로텍션, 엘엘씨로부터 살진균제 타에그로® 또는 타에그로® ECO 하에 입수가능함 (EPA 등록 번호 70127-5); (17.011) 바실루스 리케니포르미스(Bacillus licheniformis), 특히 균주 SB3086 (노보자임스로부터 에코가드™ 생물살진균제 및 그린 릴리프 하에 입수가능함); (17.012) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주,
(18.001) 불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%는 C14 내지 C20의 범위인 조성물 (예를 들어 알파바이오 페스티시드즈 또는 바이엘 아게의 FLiPPER).
화합물 (B)는 보다 더 바람직하게는 하기로부터 선택된다:
(1.002) 디페노코나졸, (1.004) 펜헥사미드, (1.010) 이마잘릴, (1.012) 이프코나졸, (1.018) 프로티오코나졸, (1.020) 스피록사민, (1.021) 테부코나졸, (1.026) (1R,2S,5S)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.027) (1S,2R,5R)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.055) 메펜트리플루코나졸, (1.059) 5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.062) 플루옥시티오코나졸, (1.067) N'-(2,5-디메틸-4-{3-[(1,1,2,2-테트라플루오로에틸)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드, (1.081) 이프펜트리플루코나졸, (1.082) 2-[6-(4-브로모페녹시)-2-(트리플루오로메틸)-3-피리딜]-1-(1,2,4-트리아졸-1-일)프로판-2-올 및, (1.092) 메틸 2-[2-클로로-4-(4-클로로페녹시)페닐]-2-히드록시-3-(1,2,4-트리아졸-1-일)프로파노에이트
(2.001) 벤조빈디플루피르, (2.002) 빅사펜, (2.003) 보스칼리드, (2.005) 플루오피람, (2.007) 플룩사피록사드, (2.017) 펜플루펜, (2.018) 펜티오피라드, (2.019) 피디플루메토펜, (2.021) 세닥산, (2.028) 인피르플룩삼, (2.030) 플루인다피르, (2.038) 이소플루시프람,
(3.003) 아족시스트로빈, (3.012) 플루옥사스트로빈, (3.016) 피콕시스트로빈, (3.017) 피라클로스트로빈, (3.020) 트리플록시스트로빈, (3.025) 펜피콕사미드, (3.026) 2-{2-[(2,5-디메틸페녹시)메틸]페닐}-2-메톡시-N-메틸아세트아미드, (3.030) 메틸테트라프롤, (3.031) 플로릴피콕사미드,
(4.005) 펜시쿠론, (4.007) 티오파네이트-메틸, (4.012) 4-(2-브로모-4-플루오로페닐)-N-(2,6-디플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.015) 4-(2-브로모-4-플루오로페닐)-N-(2-클로로-6-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.025) N-(4-클로로-2,6-디플루오로페닐)-4-(2-클로로-4-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민,
(5.003) 캅탄, (5.004) 클로로탈로닐, (5.010), 디티아논, (5.012) 폴페트, (5.013) 만코제브, (5.015) 메티람, (5.018) 프로피네브,
(6.002) 이소티아닐,
(7.005) 피리메타닐,
(12.003) 메탈락실, (12.004) 메탈락실-M (메페녹삼),
(13.001) 플루디옥소닐, (13.004) 프로퀴나지드, (13.005) 퀴녹시펜,
(14.001) 플루아지남, (14.002) 멥틸디노캅,
(15.008) 시플루페나미드, (15.012) 포세틸-알루미늄, (15.016) 메트라페논, (15.027) 피리오페논 (클라자페논), (15.043) 플루옥사피프롤린, (15.047) 3-(4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀론, (15.048) 4-아미노-5-플루오로피리미딘-2-올 (호변이성질체 형태: 4-아미노-5-플루오로피리미딘-2(1H)-온), (15.052) 5-플루오로-2-[(4-플루오로벤질)옥시]피리미딘-4-아민, (15.062) 5-플루오로-4-이미노-3-메틸-1-[(4-메틸페닐)술포닐]-3,4-디히드로피리미딘-2(1H)-온, (15.064) (N'-[2-클로로-4-(2-플루오로페녹시)-5-메틸페닐]-N-에틸-N-메틸이미도포름아미드),
(16.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨),
(17.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨); (17.012) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주,
(18.001) 불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%는 C14 내지 C20의 범위인 조성물 (예를 들어 알파바이오 페스티시드즈 또는 바이엘 아게의 FLiPPER).
화합물 (B)는 또한 보다 더 바람직하게는 하기로부터 선택된다:
(1.002) 디페노코나졸, (1.004) 펜헥사미드, (1.010) 이마잘릴, (1.012) 이프코나졸, (1.018) 프로티오코나졸, (1.020) 스피록사민, (1.021) 테부코나졸, (1.026) (1R,2S,5S)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.027) (1S,2R,5R)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.055) 메펜트리플루코나졸, (1.059) 5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.081) 이프펜트리플루코나졸, (1.082) 2-[6-(4-브로모페녹시)-2-(트리플루오로메틸)-3-피리딜]-1-(1,2,4-트리아졸-1-일)프로판-2-올 및, (1.092) 메틸 2-[2-클로로-4-(4-클로로페녹시)페닐]-2-히드록시-3-(1,2,4-트리아졸-1-일)프로파노에이트
(2.001) 벤조빈디플루피르, (2.002) 빅사펜, (2.003) 보스칼리드, (2.005) 플루오피람, (2.007) 플룩사피록사드, (2.017) 펜플루펜, (2.018) 펜티오피라드, (2.019) 피디플루메토펜, (2.021) 세닥산, (2.028) 인피르플룩삼, (2.030) 플루인다피르, (2.038) 이소플루시프람,
(3.003) 아족시스트로빈, (3.012) 플루옥사스트로빈, (3.016) 피콕시스트로빈, (3.017) 피라클로스트로빈, (3.020) 트리플록시스트로빈, (3.025) 펜피콕사미드, (3.026) 2-{2-[(2,5-디메틸페녹시)메틸]페닐}-2-메톡시-N-메틸아세트아미드, (3.030) 메틸테트라프롤, (3.031) 플로릴피콕사미드,
(4.005) 펜시쿠론, (4.007) 티오파네이트-메틸, (4.012) 4-(2-브로모-4-플루오로페닐)-N-(2,6-디플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.015) 4-(2-브로모-4-플루오로페닐)-N-(2-클로로-6-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.025) N-(4-클로로-2,6-디플루오로페닐)-4-(2-클로로-4-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민,
(5.003) 캅탄, (5.004) 클로로탈로닐, (5.010), 디티아논, (5.012) 폴페트, (5.013) 만코제브, (5.015) 메티람, (5.018) 프로피네브,
(6.002) 이소티아닐,
(7.005) 피리메타닐,
(12.003) 메탈락실, (12.004) 메탈락실-M (메페녹삼),
(13.001) 플루디옥소닐, (13.004) 프로퀴나지드, (13.005) 퀴녹시펜,
(14.001) 플루아지남, (14.002) 멥틸디노캅,
(15.008) 시플루페나미드, (15.012) 포세틸-알루미늄, (15.016) 메트라페논, (15.027) 피리오페논 (클라자페논), (15.047) 3-(4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀론, (15.048) 4-아미노-5-플루오로피리미딘-2-올 (호변이성질체 형태: 4-아미노-5-플루오로피리미딘-2(1H)-온), (15.052) 5-플루오로-2-[(4-플루오로벤질)옥시]피리미딘-4-아민, (15.062) 5-플루오로-4-이미노-3-메틸-1-[(4-메틸페닐)술포닐]-3,4-디히드로피리미딘-2(1H)-온, (15.064) (N'-[2-클로로-4-(2-플루오로페녹시)-5-메틸페닐]-N-에틸-N-메틸이미도포름아미드),
(16.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨),
(17.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨); (17.012) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주,
(18.001) 불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%는 C14 내지 C20의 범위인 조성물 (예를 들어 알파바이오 페스티시드즈 또는 바이엘 아게의 FLiPPER).
화합물 (B)는 가장 바람직하게는 하기로부터 선택된다:
(1.002) 디페노코나졸, (1.018) 프로티오코나졸, (1.020) 스피록사민, (1.021) 테부코나졸, (1.055) 메펜트리플루코나졸, (1.062) 플루옥시티오코나졸, (1.067) N'-(2,5-디메틸-4-{3-[(1,1,2,2-테트라플루오로에틸)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드,
(2.002) 빅사펜, (2.005) 플루오피람, (2.028) 인피르플룩삼, (2.038) 이소플루시프람,
(3.020) 트리플록시스트로빈, (3.025) 펜피콕사미드,
(5.003) 캅탄, (5.010) 디티아논, (5.012) 폴페트, (5.013) 만코제브, (5.018) 프로피네브,
(6.002) 이소티아닐,
(7.005) 피리메타닐,
(13.001) 플루디옥소닐, (13.004) 프로퀴나지드, (13.005) 퀴녹시펜,
(15.012) 포세틸-알루미늄, (15.016) 메트라페논, (15.043) 플루옥사피프롤린 및, (15.064) (N'-[2-클로로-4-(2-플루오로페녹시)-5-메틸페닐]-N-에틸-N-메틸이미도포름아미드),
(17.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨),
(17.012) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주,
(18.001) 불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%는 C14 내지 C20의 범위인 조성물 (예를 들어 알파바이오 페스티시드즈 또는 바이엘 아게의 FLiPPER).
화합물 (B)는 마찬가지로 가장 바람직하게는 하기로부터 선택된다:
(1.002) 디페노코나졸, (1.018) 프로티오코나졸, (1.020) 스피록사민, (1.021) 테부코나졸, (1.055) 메펜트리플루코나졸,
(2.002) 빅사펜, (2.005) 플루오피람, (2.028) 인피르플룩삼, (2.038) 이소플루시프람,
(3.020) 트리플록시스트로빈, (3.025) 펜피콕사미드,
(5.003) 캅탄, (5.010) 디티아논, (5.012) 폴페트, (5.013) 만코제브, (5.018) 프로피네브,
(6.002) 이소티아닐,
(7.005) 피리메타닐,
(13.001) 플루디옥소닐, (13.004) 프로퀴나지드, (13.005) 퀴녹시펜,
(15.012) 포세틸-알루미늄, (15.016) 메트라페논 및, (15.064) (N'-[2-클로로-4-(2-플루오로페녹시)-5-메틸페닐]-N-에틸-N-메틸이미도포름아미드),
(17.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨),
(17.012) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주,
(18.001) 불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%는 C14 내지 C20의 범위인 조성물 (예를 들어 알파바이오 페스티시드즈 또는 바이엘 아게의 FLiPPER).
본 발명에 따른 화합물 조합물은 1, 2종 또는 보다 많은 화합물 (B)를 포함할 수 있다. 바람직하게는, 본 발명에 따른 화합물 조합물은 1 또는 2종의 화합물(들) (B)를 포함한다.
2종 이상의 화합물(들) (B)가 존재하는 경우에, 이들 화합물은 상이한 군 (1) 내지 (18)로부터 선택될 수 있다. 예를 들어, 1종의 화합물 (B)가 군 (1)로부터 선택되는 경우에, 추가의 화합물(들) (B)는 군 (2) 내지 (18)로부터 선택될 수 있다.
바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G1-1)로부터 선택된다:
(I-052) + (1.001), (I-052) + (1.002), (I-052) + (1.003), (I-052) + (1.004), (I-052) + (1.005), (I-052) + (1.006), (I-052) + (1.007), (I-052) + (1.008), (I-052) + (1.009), (I-052) + (1.010), (I-052) + (1.011), (I-052) + (1.012), (I-052) + (1.013), (I-052) + (1.014), (I-052) + (1.015), (I-052) + (1.016), (I-052) + (1.017), (I-052) + (1.018), (I-052) + (1.019), (I-052) + (1.020), (I-052) + (1.021), (I-052) + (1.022), (I-052) + (1.023), (I-052) + (1.024), (I-052) + (1.025), (I-052) + (1.026), (I-052) + (1.027), (I-052) + (1.028), (I-052) + (1.029), (I-052) + (1.030), (I-052) + (1.031), (I-052) + (1.032), (I-052) + (1.033), (I-052) + (1.034), (I-052) + (1.035), (I-052) + (1.036), (I-052) + (1.037), (I-052) + (1.038), (I-052) + (1.039), (I-052) + (1.040), (I-052) + (1.041), (I-052) + (1.042), (I-052) + (1.043), (I-052) + (1.044), (I-052) + (1.045), (I-052) + (1.046), (I-052) + (1.047), (I-052) + (1.048), (I-052) + (1.049), (I-052) + (1.050), (I-052) + (1.051), (I-052) + (1.052), (I-052) + (1.053), (I-052) + (1.054), (I-052) + (1.055), (I-052) + (1.056), (I-052) + (1.057), (I-052) + (1.058), (I-052) + (1.059), (I-052) + (1.060), (I-052) + (1.061), (I-052) + (1.062), (I-052) + (1.063), (I-052) + (1.064), (I-052) + (1.065), (I-052) + (1.066), (I-052) + (1.067), (I-052) + (1.068), (I-052) + (1.069), (I-052) + (1.070), (I-052) + (1.071), (I-052) + (1.072), (I-052) + (1.073), (I-052) + (1.074), (I-052) + (1.075), (I-052) + (1.076), (I-052) + (1.077), (I-052) + (1.078), (I-052) + (1.079), (I-052) + (1.080), (I-052) + (1.081), (I-052) + (1.082), (I-052) + (1.083), (I-052) + (1.084), (I-052) + (1.085), (I-052) + (1.086), (I-052) + (1.087), (I-052) + (1.088), (I-052) + (1.089), (I-052) + (1.090), (I-052) + (1.091), (I-052) + (1.092), (I-052) + (2.001), (I-052) + (2.002), (I-052) + (2.003), (I-052) + (2.004), (I-052) + (2.005), (I-052) + (2.006), (I-052) + (2.007), (I-052) + (2.008), (I-052) + (2.009), (I-052) + (2.010), (I-052) + (2.011), (I-052) + (2.012), (I-052) + (2.013), (I-052) + (2.014), (I-052) + (2.015), (I-052) + (2.016), (I-052) + (2.017), (I-052) + (2.018), (I-052) + (2.019), (I-052) + (2.020), (I-052) + (2.021), (I-052) + (2.022), (I-052) + (2.023), (I-052) + (2.024), (I-052) + (2.025), (I-052) + (2.026), (I-052) + (2.027), (I-052) + (2.028), (I-052) + (2.029), (I-052) + (2.030), (I-052) + (2.031), (I-052) + (2.032), (I-052) + (2.033), (I-052) + (2.034), (I-052) + (2.035), (I-052) + (2.036), (I-052) + (2.037), (I-052) + (2.038), (I-052) + (2.039), (I-052) + (2.040), (I-052) + (2.041), (I-052) + (2.042), (I-052) + (2.043), (I-052) + (2.044), (I-052) + (2.045), (I-052) + (2.046), (I-052) + (2.047), (I-052) + (2.048), (I-052) + (2.049), (I-052) + (2.050), (I-052) + (2.051), (I-052) + (2.052), (I-052) + (2.053), (I-052) + (2.054), (I-052) + (2.055), (I-052) + (2.056), (I-052) + (2.057), (I-052) + (2.058), (I-052) + (2.059), (I-052) + (2.060), (I-052) + (3.001), (I-052) + (3.002), (I-052) + (3.003), (I-052) + (3.004), (I-052) + (3.005), (I-052) + (3.006), (I-052) + (3.007), (I-052) + (3.008), (I-052) + (3.009), (I-052) + (3.010), (I-052) + (3.011), (I-052) + (3.012), (I-052) + (3.013), (I-052) + (3.014), (I-052) + (3.015), (I-052) + (3.016), (I-052) + (3.017), (I-052) + (3.018), (I-052) + (3.019), (I-052) + (3.020), (I-052) + (3.021), (I-052) + (3.022), (I-052) + (3.023), (I-052) + (3.024), (I-052) + (3.025), (I-052) + (3.026), (I-052) + (3.027), (I-052) + (3.028), (I-052) + (3.029), (I-052) + (3.030), (I-052) + (3.031), (I-052) + (3.032), (I-052) + (4.001), (I-052) + (4.002), (I-052) + (4.003), (I-052) + (4.004), (I-052) + (4.005), (I-052) + (4.006), (I-052) + (4.007), (I-052) + (4.008), (I-052) + (4.009), (I-052) + (4.010), (I-052) + (4.011), (I-052) + (4.012), (I-052) + (4.013), (I-052) + (4.014), (I-052) + (4.015), (I-052) + (4.016), (I-052) + (4.017), (I-052) + (4.018), (I-052) + (4.019), (I-052) + (4.020), (I-052) + (4.021), (I-052) + (4.022), (I-052) + (4.023), (I-052) + (4.024), (I-052) + (4.025), (I-052) + (4.026), (I-052) + (5.001), (I-052) + (5.002), (I-052) + (5.003), (I-052) + (5.004), (I-052) + (5.005), (I-052) + (5.006), (I-052) + (5.007), (I-052) + (5.008), (I-052) + (5.009), (I-052) + (5.010), (I-052) + (5.011), (I-052) + (5.012), (I-052) + (5.013), (I-052) + (5.014), (I-052) + (5.015), (I-052) + (5.016), (I-052) + (5.017), (I-052) + (5.018), (I-052) + (5.019), (I-052) + (5.020), (I-052) + (5.021), (I-052) + (5.022), (I-052) + (5.023), (I-052) + (6.001), (I-052) + (6.002), (I-052) + (6.003), (I-052) + (6.004), (I-052) + (7.001), (I-052) + (7.002), (I-052) + (7.003), (I-052) + (7.004), (I-052) + (7.005), (I-052) + (7.006), (I-052) + (8.001), (I-052) + (9.001), (I-052) + (9.002), (I-052) + (9.003), (I-052) + (9.004), (I-052) + (9.005), (I-052) + (9.006), (I-052) + (9.007), (I-052) + (9.008), (I-052) + (9.009), (I-052) + (10.001), (I-052) + (10.002), (I-052) + (10.003), (I-052) + (11.001), (I-052) + (11.002), (I-052) + (12.001), (I-052) + (12.002), (I-052) + (12.003), (I-052) + (12.004), (I-052) + (13.001), (I-052) + (13.002), (I-052) + (13.003), (I-052) + (13.004), (I-052) + (13.005), (I-052) + (13.006), (I-052) + (14.001), (I-052) + (14.002), (I-052) + (15.001), (I-052) + (15.002), (I-052) + (15.003), (I-052) + (15.004), (I-052) + (15.005), (I-052) + (15.006), (I-052) + (15.007), (I-052) + (15.008), (I-052) + (15.009), (I-052) + (15.010), (I-052) + (15.011), (I-052) + (15.012), (I-052) + (15.013), (I-052) + (15.014), (I-052) + (15.015), (I-052) + (15.016), (I-052) + (15.017), (I-052) + (15.018), (I-052) + (15.019), (I-052) + (15.020), (I-052) + (15.021), (I-052) + (15.022), (I-052) + (15.023), (I-052) + (15.024), (I-052) + (15.025), (I-052) + (15.026), (I-052) + (15.027), (I-052) + (15.028), (I-052) + (15.029), (I-052) + (15.030), (I-052) + (15.031), (I-052) + (15.032), (I-052) + (15.033), (I-052) + (15.034), (I-052) + (15.035), (I-052) + (15.036), (I-052) + (15.037), (I-052) + (15.038), (I-052) + (15.039), (I-052) + (15.040), (I-052) + (15.041), (I-052) + (15.042), (I-052) + (15.043), (I-052) + (15.044), (I-052) + (15.045), (I-052) + (15.046), (I-052) + (15.047), (I-052) + (15.048), (I-052) + (15.049), (I-052) + (15.050), (I-052) + (15.051), (I-052) + (15.052), (I-052) + (15.053), (I-052) + (15.054), (I-052) + (15.055), (I-052) + (15.056), (I-052) + (15.057), (I-052) + (15.058), (I-052) + (15.059), (I-052) + (15.060), (I-052) + (15.061), (I-052) + (15.062), (I-052) + (15.063) , (I-052) + (15.064), (I-052) + (15.065), (I-052) + (15.066), (I-052) + (15.067), (I-052) + (15.068), (I-052) + (15.069), (I-052) + (15.070), (I-052) + (15.071), (I-052) + (15.072), (I-052) + (15.073), (I-052) + (15.074), (I-052) + (15.075), (I-052) + (15.076), (I-052) + (15.077), (I-052) + (15.078), (I-052) + (15.079), (I-052) + (15.080), (I-052) + (15.081), (I-052) + (15.082), (I-052) + (15.083), (I-052) + (15.084), (I-052) + (15.085), (I-052) + (15.086), (I-052) + (15.087), (I-052) + (15.088), (I-052) + (15.089), (I-052) + (15.090), (I-052) + (15.091), (I-052) + (15.092), (I-052) + (15.093), (I-052) + (15.094), (I-052) + (15.095), (I-052) + (15.096), (I-052) + (15.097), (I-052) + (15.098), (I-052) + (15.099), (I-052) + (15.100), (I-052) + (15.101), (I-052) + (15.102), (I-052) + (15.103), (I-052) + (15.104), (I-052) + (15.105), (I-052) + (15.106), (I-052) + (15.107), (I-052) + (15.108), (I-052) + (15.109), (I-052) + (15.110), (I-052) + (15.111), (I-052) + (15.112), (I-052) + (15.113), (I-052) + (15.114), (I-052) + (15.115), (I-052) + (15.116), (I-052) + (15.117), (I-052) + (15.118), (I-052) + (15.119), (I-052) + (15.120), (I-052) + (15.121), (I-052) + (15.122), (I-052) + (15.123), (I-052) + (15.124), (I-052) + (15.125), (I-052) + (15.126), (I-052) + (15.127), (I-052) + (15.128), (I-052) + (16.001), (I-052) + (16.002), (I-052) + (16.003), (I-052) + (16.004), (I-052) + (16.005), (I-052) + (16.006), (I-052) + (16.007), (I-052) + (16.008), (I-052) + (17.001), (I-052) + (17.002), (I-052) + (17.003), (I-052) + (17.004), (I-052) + (17.005), (I-052) + (17.006), (I-052) + (17.007), (I-052) + (17.008), (I-052) + (17.009), (I-052) + (17.010), (I-052) + (17.011), (I-052) + (17.012) 및 (I-052) + (18.001).
바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G1)로부터 선택된다:
(I-052) + (1.001), (I-052) + (1.002), (I-052) + (1.003), (I-052) + (1.004), (I-052) + (1.005), (I-052) + (1.006), (I-052) + (1.007), (I-052) + (1.008), (I-052) + (1.009), (I-052) + (1.010), (I-052) + (1.011), (I-052) + (1.012), (I-052) + (1.013), (I-052) + (1.014), (I-052) + (1.015), (I-052) + (1.016), (I-052) + (1.017), (I-052) + (1.018), (I-052) + (1.019), (I-052) + (1.020), (I-052) + (1.021), (I-052) + (1.022), (I-052) + (1.023), (I-052) + (1.024), (I-052) + (1.025), (I-052) + (1.026), (I-052) + (1.027), (I-052) + (1.028), (I-052) + (1.029), (I-052) + (1.030), (I-052) + (1.031), (I-052) + (1.032), (I-052) + (1.033), (I-052) + (1.034), (I-052) + (1.035), (I-052) + (1.036), (I-052) + (1.037), (I-052) + (1.038), (I-052) + (1.039), (I-052) + (1.040), (I-052) + (1.041), (I-052) + (1.042), (I-052) + (1.043), (I-052) + (1.044), (I-052) + (1.045), (I-052) + (1.046), (I-052) + (1.047), (I-052) + (1.048), (I-052) + (1.049), (I-052) + (1.050), (I-052) + (1.051), (I-052) + (1.052), (I-052) + (1.053), (I-052) + (1.054), (I-052) + (1.055), (I-052) + (1.056), (I-052) + (1.057), (I-052) + (1.058), (I-052) + (1.059), (I-052) + (1.060), (I-052) + (1.061), (I-052) + (1.062), (I-052) + (1.063), (I-052) + (1.064), (I-052) + (1.065), (I-052) + (1.066), (I-052) + (1.067), (I-052) + (1.068), (I-052) + (1.069), (I-052) + (1.070), (I-052) + (1.071), (I-052) + (1.072), (I-052) + (1.073), (I-052) + (1.074), (I-052) + (1.075), (I-052) + (1.076), (I-052) + (1.077), (I-052) + (1.078), (I-052) + (1.079), (I-052) + (1.080), (I-052) + (1.081), (I-052) + (1.082), (I-052) + (1.083), (I-052) + (1.084), (I-052) + (1.085), (I-052) + (1.086), (I-052) + (1.087), (I-052) + (1.088), (I-052) + (1.089), (I-052) + (1.090), (I-052) + (1.091), (I-052) + (1.092), (I-052) + (2.001), (I-052) + (2.002), (I-052) + (2.003), (I-052) + (2.004), (I-052) + (2.005), (I-052) + (2.006), (I-052) + (2.007), (I-052) + (2.008), (I-052) + (2.009), (I-052) + (2.010), (I-052) + (2.011), (I-052) + (2.012), (I-052) + (2.013), (I-052) + (2.014), (I-052) + (2.015), (I-052) + (2.016), (I-052) + (2.017), (I-052) + (2.018), (I-052) + (2.019), (I-052) + (2.020), (I-052) + (2.021), (I-052) + (2.022), (I-052) + (2.023), (I-052) + (2.024), (I-052) + (2.025), (I-052) + (2.026), (I-052) + (2.027), (I-052) + (2.028), (I-052) + (2.029), (I-052) + (2.030), (I-052) + (2.031), (I-052) + (2.032), (I-052) + (2.033), (I-052) + (2.034), (I-052) + (2.035), (I-052) + (2.036), (I-052) + (2.037), (I-052) + (2.038), (I-052) + (2.039), (I-052) + (2.040), (I-052) + (2.041), (I-052) + (2.042), (I-052) + (2.043), (I-052) + (2.044), (I-052) + (2.045), (I-052) + (2.046), (I-052) + (2.047), (I-052) + (2.048), (I-052) + (2.049), (I-052) + (2.050), (I-052) + (2.051), (I-052) + (2.052), (I-052) + (2.053), (I-052) + (2.054), (I-052) + (2.055), (I-052) + (2.056), (I-052) + (2.057), (I-052) + (2.058), (I-052) + (2.059), (I-052) + (3.001), (I-052) + (3.002), (I-052) + (3.003), (I-052) + (3.004), (I-052) + (3.005), (I-052) + (3.006), (I-052) + (3.007), (I-052) + (3.008), (I-052) + (3.009), (I-052) + (3.010), (I-052) + (3.011), (I-052) + (3.012), (I-052) + (3.013), (I-052) + (3.014), (I-052) + (3.015), (I-052) + (3.016), (I-052) + (3.017), (I-052) + (3.018), (I-052) + (3.019), (I-052) + (3.020), (I-052) + (3.021), (I-052) + (3.022), (I-052) + (3.023), (I-052) + (3.024), (I-052) + (3.025), (I-052) + (3.026), (I-052) + (3.027), (I-052) + (3.028), (I-052) + (3.029), (I-052) + (3.030), (I-052) + (3.031), (I-052) + (4.001), (I-052) + (4.002), (I-052) + (4.003), (I-052) + (4.004), (I-052) + (4.005), (I-052) + (4.006), (I-052) + (4.007), (I-052) + (4.008), (I-052) + (4.009), (I-052) + (4.010), (I-052) + (4.011), (I-052) + (4.012), (I-052) + (4.013), (I-052) + (4.014), (I-052) + (4.015), (I-052) + (4.016), (I-052) + (4.017), (I-052) + (4.018), (I-052) + (4.019), (I-052) + (4.020), (I-052) + (4.021), (I-052) + (4.022), (I-052) + (4.023), (I-052) + (4.024), (I-052) + (4.025), (I-052) + (4.026), (I-052) + (5.001), (I-052) + (5.002), (I-052) + (5.003), (I-052) + (5.004), (I-052) + (5.005), (I-052) + (5.006), (I-052) + (5.007), (I-052) + (5.008), (I-052) + (5.009), (I-052) + (5.010), (I-052) + (5.011), (I-052) + (5.012), (I-052) + (5.013), (I-052) + (5.014), (I-052) + (5.015), (I-052) + (5.016), (I-052) + (5.017), (I-052) + (5.018), (I-052) + (5.019), (I-052) + (5.020), (I-052) + (5.021), (I-052) + (5.022), (I-052) + (5.023), (I-052) + (6.001), (I-052) + (6.002), (I-052) + (6.003), (I-052) + (6.004), (I-052) + (7.001), (I-052) + (7.002), (I-052) + (7.003), (I-052) + (7.004), (I-052) + (7.005), (I-052) + (7.006), (I-052) + (8.001), (I-052) + (9.001), (I-052) + (9.002), (I-052) + (9.003), (I-052) + (9.004), (I-052) + (9.005), (I-052) + (9.006), (I-052) + (9.007), (I-052) + (9.008), (I-052) + (9.009), (I-052) + (10.001), (I-052) + (10.002), (I-052) + (10.003), (I-052) + (11.001), (I-052) + (11.002), (I-052) + (12.001), (I-052) + (12.002), (I-052) + (12.003), (I-052) + (12.004), (I-052) + (13.001), (I-052) + (13.002), (I-052) + (13.003), (I-052) + (13.004), (I-052) + (13.005), (I-052) + (13.006), (I-052) + (14.001), (I-052) + (14.002), (I-052) + (15.001), (I-052) + (15.002), (I-052) + (15.003), (I-052) + (15.004), (I-052) + (15.005), (I-052) + (15.006), (I-052) + (15.007), (I-052) + (15.008), (I-052) + (15.009), (I-052) + (15.010), (I-052) + (15.011), (I-052) + (15.012), (I-052) + (15.013), (I-052) + (15.014), (I-052) + (15.015), (I-052) + (15.016), (I-052) + (15.017), (I-052) + (15.018), (I-052) + (15.019), (I-052) + (15.020), (I-052) + (15.021), (I-052) + (15.022), (I-052) + (15.023), (I-052) + (15.024), (I-052) + (15.025), (I-052) + (15.026), (I-052) + (15.027), (I-052) + (15.028), (I-052) + (15.029), (I-052) + (15.030), (I-052) + (15.031), (I-052) + (15.032), (I-052) + (15.033), (I-052) + (15.034), (I-052) + (15.035), (I-052) + (15.036), (I-052) + (15.037), (I-052) + (15.038), (I-052) + (15.039), (I-052) + (15.040), (I-052) + (15.041), (I-052) + (15.042), (I-052) + (15.043), (I-052) + (15.044), (I-052) + (15.045), (I-052) + (15.046), (I-052) + (15.047), (I-052) + (15.048), (I-052) + (15.049), (I-052) + (15.050), (I-052) + (15.051), (I-052) + (15.052), (I-052) + (15.053), (I-052) + (15.054), (I-052) + (15.055), (I-052) + (15.056), (I-052) + (15.057), (I-052) + (15.058), (I-052) + (15.059), (I-052) + (15.060), (I-052) + (15.061), (I-052) + (15.062), (I-052) + (15.063) , (I-052) + (15.064), (I-052) + (15.065), (I-052) + (15.066), (I-052) + (15.067), (I-052) + (15.068), (I-052) + (15.069), (I-052) + (15.070), (I-052) + (15.071), (I-052) + (15.072), (I-052) + (15.073), (I-052) + (15.074), (I-052) + (15.075), (I-052) + (15.076), (I-052) + (15.077), (I-052) + (15.078), (I-052) + (15.079), (I-052) + (15.080), (I-052) + (15.081), (I-052) + (15.082), (I-052) + (15.083), (I-052) + (15.084), (I-052) + (15.085), (I-052) + (15.086), (I-052) + (15.087), (I-052) + (15.088), (I-052) + (15.089), (I-052) + (15.090), (I-052) + (15.091), (I-052) + (15.092), (I-052) + (15.093), (I-052) + (15.094), (I-052) + (15.095), (I-052) + (15.096), (I-052) + (15.097), (I-052) + (15.098), (I-052) + (15.099), (I-052) + (15.100), (I-052) + (15.101), (I-052) + (15.102), (I-052) + (15.103), (I-052) + (15.104), (I-052) + (15.105), (I-052) + (15.106), (I-052) + (15.107), (I-052) + (15.108), (I-052) + (15.109), (I-052) + (15.110), (I-052) + (15.111), (I-052) + (15.112), (I-052) + (15.113), (I-052) + (15.114), (I-052) + (15.115), (I-052) + (15.116), (I-052) + (15.117), (I-052) + (15.118), (I-052) + (15.119), (I-052) + (15.120), (I-052) + (15.121), (I-052) + (15.122), (I-052) + (15.123), (I-052) + (15.124), (I-052) + (15.125), (I-052) + (15.126), (I-052) + (15.127), (I-052) + (16.001), (I-052) + (16.002), (I-052) + (16.003), (I-052) + (16.004), (I-052) + (16.005), (I-052) + (16.006), (I-052) + (16.007), (I-052) + (16.008), (I-052) + (17.001), (I-052) + (17.002), (I-052) + (17.003), (I-052) + (17.004), (I-052) + (17.005), (I-052) + (17.006), (I-052) + (17.007), (I-052) + (17.008), (I-052) + (17.009), (I-052) + (17.010), (I-052) + (17.011), (I-052) + (17.012) 및 (I-052) + (18.001).
또한 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G2-1)으로부터 선택된다:
(I-130) + (1.001), (I-130) + (1.002), (I-130) + (1.003), (I-130) + (1.004), (I-130) + (1.005), (I-130) + (1.006), (I-130) + (1.007), (I-130) + (1.008), (I-130) + (1.009), (I-130) + (1.010), (I-130) + (1.011), (I-130) + (1.012), (I-130) + (1.013), (I-130) + (1.014), (I-130) + (1.015), (I-130) + (1.016), (I-130) + (1.017), (I-130) + (1.018), (I-130) + (1.019), (I-130) + (1.020), (I-130) + (1.021), (I-130) + (1.022), (I-130) + (1.023), (I-130) + (1.024), (I-130) + (1.025), (I-130) + (1.026), (I-130) + (1.027), (I-130) + (1.028), (I-130) + (1.029), (I-130) + (1.030), (I-130) + (1.031), (I-130) + (1.032), (I-130) + (1.033), (I-130) + (1.034), (I-130) + (1.035), (I-130) + (1.036), (I-130) + (1.037), (I-130) + (1.038), (I-130) + (1.039), (I-130) + (1.040), (I-130) + (1.041), (I-130) + (1.042), (I-130) + (1.043), (I-130) + (1.044), (I-130) + (1.045), (I-130) + (1.046), (I-130) + (1.047), (I-130) + (1.048), (I-130) + (1.049), (I-130) + (1.050), (I-130) + (1.051), (I-130) + (1.052), (I-130) + (1.053), (I-130) + (1.054), (I-130) + (1.055), (I-130) + (1.056), (I-130) + (1.057), (I-130) + (1.058), (I-130) + (1.059), (I-130) + (1.060), (I-130) + (1.061), (I-130) + (1.062), (I-130) + (1.063), (I-130) + (1.064), (I-130) + (1.065), (I-130) + (1.066), (I-130) + (1.067), (I-130) + (1.068), (I-130) + (1.069), (I-130) + (1.070), (I-130) + (1.071), (I-130) + (1.072), (I-130) + (1.073), (I-130) + (1.074), (I-130) + (1.075), (I-130) + (1.076), (I-130) + (1.077), (I-130) + (1.078), (I-130) + (1.079), (I-130) + (1.080), (I-130) + (1.081), (I-130) + (1.082), (I-130) + (1.083), (I-130) + (1.084), (I-130) + (1.085), (I-130) + (1.086), (I-130) + (1.087), (I-130) + (1.088), (I-130) + (1.089), (I-130) + (1.090), (I-130) + (1.091), (I-130) + (1.092), (I-130) + (2.001), (I-130) + (2.002), (I-130) + (2.003), (I-130) + (2.004), (I-130) + (2.005), (I-130) + (2.006), (I-130) + (2.007), (I-130) + (2.008), (I-130) + (2.009), (I-130) + (2.010), (I-130) + (2.011), (I-130) + (2.012), (I-130) + (2.013), (I-130) + (2.014), (I-130) + (2.015), (I-130) + (2.016), (I-130) + (2.017), (I-130) + (2.018), (I-130) + (2.019), (I-130) + (2.020), (I-130) + (2.021), (I-130) + (2.022), (I-130) + (2.023), (I-130) + (2.024), (I-130) + (2.025), (I-130) + (2.026), (I-130) + (2.027), (I-130) + (2.028), (I-130) + (2.029), (I-130) + (2.030), (I-130) + (2.031), (I-130) + (2.032), (I-130) + (2.033), (I-130) + (2.034), (I-130) + (2.035), (I-130) + (2.036), (I-130) + (2.037), (I-130) + (2.038), (I-130) + (2.039), (I-130) + (2.040), (I-130) + (2.041), (I-130) + (2.042), (I-130) + (2.043), (I-130) + (2.044), (I-130) + (2.045), (I-130) + (2.046), (I-130) + (2.047), (I-130) + (2.048), (I-130) + (2.049), (I-130) + (2.050), (I-130) + (2.051), (I-130) + (2.052), (I-130) + (2.053), (I-130) + (2.054), (I-130) + (2.055), (I-130) + (2.056), (I-130) + (2.057), (I-130) + (2.058), (I-130) + (2.059), (I-130) + (2.060), (I-130) + (3.001), (I-130) + (3.002), (I-130) + (3.003), (I-130) + (3.004), (I-130) + (3.005), (I-130) + (3.006), (I-130) + (3.007), (I-130) + (3.008), (I-130) + (3.009), (I-130) + (3.010), (I-130) + (3.011), (I-130) + (3.012), (I-130) + (3.013), (I-130) + (3.014), (I-130) + (3.015), (I-130) + (3.016), (I-130) + (3.017), (I-130) + (3.018), (I-130) + (3.019), (I-130) + (3.020), (I-130) + (3.021), (I-130) + (3.022), (I-130) + (3.023), (I-130) + (3.024), (I-130) + (3.025), (I-130) + (3.026), (I-130) + (3.027), (I-130) + (3.028), (I-130) + (3.029), (I-130) + (3.030), (I-130) + (3.031), (I-130) + (3.032), (I-130) + (4.001), (I-130) + (4.002), (I-130) + (4.003), (I-130) + (4.004), (I-130) + (4.005), (I-130) + (4.006), (I-130) + (4.007), (I-130) + (4.008), (I-130) + (4.009), (I-130) + (4.010), (I-130) + (4.011), (I-130) + (4.012), (I-130) + (4.013), (I-130) + (4.014), (I-130) + (4.015), (I-130) + (4.016), (I-130) + (4.017), (I-130) + (4.018), (I-130) + (4.019), (I-130) + (4.020), (I-130) + (4.021), (I-130) + (4.022), (I-130) + (4.023), (I-130) + (4.024), (I-130) + (4.025), (I-130) + (4.026), (I-130) + (5.001), (I-130) + (5.002), (I-130) + (5.003), (I-130) + (5.004), (I-130) + (5.005), (I-130) + (5.006), (I-130) + (5.007), (I-130) + (5.008), (I-130) + (5.009), (I-130) + (5.010), (I-130) + (5.011), (I-130) + (5.012), (I-130) + (5.013), (I-130) + (5.014), (I-130) + (5.015), (I-130) + (5.016), (I-130) + (5.017), (I-130) + (5.018), (I-130) + (5.019), (I-130) + (5.020), (I-130) + (5.021), (I-130) + (5.022), (I-130) + (5.023), (I-130) + (6.001), (I-130) + (6.002), (I-130) + (6.003), (I-130) + (6.004), (I-130) + (7.001), (I-130) + (7.002), (I-130) + (7.003), (I-130) + (7.004), (I-130) + (7.005), (I-130) + (7.006), (I-130) + (8.001), (I-130) + (9.001), (I-130) + (9.002), (I-130) + (9.003), (I-130) + (9.004), (I-130) + (9.005), (I-130) + (9.006), (I-130) + (9.007), (I-130) + (9.008), (I-130) + (9.009), (I-130) + (10.001), (I-130) + (10.002), (I-130) + (10.003), (I-130) + (11.001), (I-130) + (11.002), (I-130) + (12.001), (I-130) + (12.002), (I-130) + (12.003), (I-130) + (12.004), (I-130) + (13.001), (I-130) + (13.002), (I-130) + (13.003), (I-130) + (13.004), (I-130) + (13.005), (I-130) + (13.006), (I-130) + (14.001), (I-130) + (14.002), (I-130) + (15.001), (I-130) + (15.002), (I-130) + (15.003), (I-130) + (15.004), (I-130) + (15.005), (I-130) + (15.006), (I-130) + (15.007), (I-130) + (15.008), (I-130) + (15.009), (I-130) + (15.010), (I-130) + (15.011), (I-130) + (15.012), (I-130) + (15.013), (I-130) + (15.014), (I-130) + (15.015), (I-130) + (15.016), (I-130) + (15.017), (I-130) + (15.018), (I-130) + (15.019), (I-130) + (15.020), (I-130) + (15.021), (I-130) + (15.022), (I-130) + (15.023), (I-130) + (15.024), (I-130) + (15.025), (I-130) + (15.026), (I-130) + (15.027), (I-130) + (15.028), (I-130) + (15.029), (I-130) + (15.030), (I-130) + (15.031), (I-130) + (15.032), (I-130) + (15.033), (I-130) + (15.034), (I-130) + (15.035), (I-130) + (15.036), (I-130) + (15.037), (I-130) + (15.038), (I-130) + (15.039), (I-130) + (15.040), (I-130) + (15.041), (I-130) + (15.042), (I-130) + (15.043), (I-130) + (15.044), (I-130) + (15.045), (I-130) + (15.046), (I-130) + (15.047), (I-130) + (15.048), (I-130) + (15.049), (I-130) + (15.050), (I-130) + (15.051), (I-130) + (15.052), (I-130) + (15.053), (I-130) + (15.054), (I-130) + (15.055), (I-130) + (15.056), (I-130) + (15.057), (I-130) + (15.058), (I-130) + (15.059), (I-130) + (15.060), (I-130) + (15.061), (I-130) + (15.062), (I-130) + (15.063) , (I-130) + (15.064), (I-130) + (15.065), (I-130) + (15.066), (I-130) + (15.067), (I-130) + (15.068), (I-130) + (15.069), (I-130) + (15.070), (I-130) + (15.071), (I-130) + (15.072), (I-130) + (15.073), (I-130) + (15.074), (I-130) + (15.075), (I-130) + (15.076), (I-130) + (15.077), (I-130) + (15.078), (I-130) + (15.079), (I-130) + (15.080), (I-130) + (15.081), (I-130) + (15.082), (I-130) + (15.083), (I-130) + (15.084), (I-130) + (15.085), (I-130) + (15.086), (I-130) + (15.087), (I-130) + (15.088), (I-130) + (15.089), (I-130) + (15.090), (I-130) + (15.091), (I-130) + (15.092), (I-130) + (15.093), (I-130) + (15.094), (I-130) + (15.095), (I-130) + (15.096), (I-130) + (15.097), (I-130) + (15.098), (I-130) + (15.099), (I-130) + (15.100), (I-130) + (15.101), (I-130) + (15.102), (I-130) + (15.103), (I-130) + (15.104), (I-130) + (15.105), (I-130) + (15.106), (I-130) + (15.107), (I-130) + (15.108), (I-130) + (15.109), (I-130) + (15.110), (I-130) + (15.111), (I-130) + (15.112), (I-130) + (15.113), (I-130) + (15.114), (I-130) + (15.115), (I-130) + (15.116), (I-130) + (15.117), (I-130) + (15.118), (I-130) + (15.119), (I-130) + (15.120), (I-130) + (15.121), (I-130) + (15.122), (I-130) + (15.123), (I-130) + (15.124), (I-130) + (15.125), (I-130) + (15.126), (I-130) + (15.127), (I-130) + (15.128), (I-130) + (16.001), (I-130) + (16.002), (I-130) + (16.003), (I-130) + (16.004), (I-130) + (16.005), (I-130) + (16.006), (I-130) + (16.007), (I-130) + (16.008), (I-130) + (17.001), (I-130) + (17.002), (I-130) + (17.003), (I-130) + (17.004), (I-130) + (17.005), (I-130) + (17.006), (I-130) + (17.007), (I-130) + (17.008), (I-130) + (17.009), (I-130) + (17.010), (I-130) + (17.011), (I-130) + (17.012) 및 (I-130) + (18.001).
또한 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G2)으로부터 선택된다:
(I-130) + (1.001), (I-130) + (1.002), (I-130) + (1.003), (I-130) + (1.004), (I-130) + (1.005), (I-130) + (1.006), (I-130) + (1.007), (I-130) + (1.008), (I-130) + (1.009), (I-130) + (1.010), (I-130) + (1.011), (I-130) + (1.012), (I-130) + (1.013), (I-130) + (1.014), (I-130) + (1.015), (I-130) + (1.016), (I-130) + (1.017), (I-130) + (1.018), (I-130) + (1.019), (I-130) + (1.020), (I-130) + (1.021), (I-130) + (1.022), (I-130) + (1.023), (I-130) + (1.024), (I-130) + (1.025), (I-130) + (1.026), (I-130) + (1.027), (I-130) + (1.028), (I-130) + (1.029), (I-130) + (1.030), (I-130) + (1.031), (I-130) + (1.032), (I-130) + (1.033), (I-130) + (1.034), (I-130) + (1.035), (I-130) + (1.036), (I-130) + (1.037), (I-130) + (1.038), (I-130) + (1.039), (I-130) + (1.040), (I-130) + (1.041), (I-130) + (1.042), (I-130) + (1.043), (I-130) + (1.044), (I-130) + (1.045), (I-130) + (1.046), (I-130) + (1.047), (I-130) + (1.048), (I-130) + (1.049), (I-130) + (1.050), (I-130) + (1.051), (I-130) + (1.052), (I-130) + (1.053), (I-130) + (1.054), (I-130) + (1.055), (I-130) + (1.056), (I-130) + (1.057), (I-130) + (1.058), (I-130) + (1.059), (I-130) + (1.060), (I-130) + (1.061), (I-130) + (1.062), (I-130) + (1.063), (I-130) + (1.064), (I-130) + (1.065), (I-130) + (1.066), (I-130) + (1.067), (I-130) + (1.068), (I-130) + (1.069), (I-130) + (1.070), (I-130) + (1.071), (I-130) + (1.072), (I-130) + (1.073), (I-130) + (1.074), (I-130) + (1.075), (I-130) + (1.076), (I-130) + (1.077), (I-130) + (1.078), (I-130) + (1.079), (I-130) + (1.080), (I-130) + (1.081), (I-130) + (1.082), (I-130) + (1.083), (I-130) + (1.084), (I-130) + (1.085), (I-130) + (1.086), (I-130) + (1.087), (I-130) + (1.088), (I-130) + (1.089), (I-130) + (1.090), (I-130) + (1.091), (I-130) + (1.092), (I-130) + (2.001), (I-130) + (2.002), (I-130) + (2.003), (I-130) + (2.004), (I-130) + (2.005), (I-130) + (2.006), (I-130) + (2.007), (I-130) + (2.008), (I-130) + (2.009), (I-130) + (2.010), (I-130) + (2.011), (I-130) + (2.012), (I-130) + (2.013), (I-130) + (2.014), (I-130) + (2.015), (I-130) + (2.016), (I-130) + (2.017), (I-130) + (2.018), (I-130) + (2.019), (I-130) + (2.020), (I-130) + (2.021), (I-130) + (2.022), (I-130) + (2.023), (I-130) + (2.024), (I-130) + (2.025), (I-130) + (2.026), (I-130) + (2.027), (I-130) + (2.028), (I-130) + (2.029), (I-130) + (2.030), (I-130) + (2.031), (I-130) + (2.032), (I-130) + (2.033), (I-130) + (2.034), (I-130) + (2.035), (I-130) + (2.036), (I-130) + (2.037), (I-130) + (2.038), (I-130) + (2.039), (I-130) + (2.040), (I-130) + (2.041), (I-130) + (2.042), (I-130) + (2.043), (I-130) + (2.044), (I-130) + (2.045), (I-130) + (2.046), (I-130) + (2.047), (I-130) + (2.048), (I-130) + (2.049), (I-130) + (2.050), (I-130) + (2.051), (I-130) + (2.052), (I-130) + (2.053), (I-130) + (2.054), (I-130) + (2.055), (I-130) + (2.056), (I-130) + (2.057), (I-130) + (2.058), (I-130) + (2.059), (I-130) + (3.001), (I-130) + (3.002), (I-130) + (3.003), (I-130) + (3.004), (I-130) + (3.005), (I-130) + (3.006), (I-130) + (3.007), (I-130) + (3.008), (I-130) + (3.009), (I-130) + (3.010), (I-130) + (3.011), (I-130) + (3.012), (I-130) + (3.013), (I-130) + (3.014), (I-130) + (3.015), (I-130) + (3.016), (I-130) + (3.017), (I-130) + (3.018), (I-130) + (3.019), (I-130) + (3.020), (I-130) + (3.021), (I-130) + (3.022), (I-130) + (3.023), (I-130) + (3.024), (I-130) + (3.025), (I-130) + (3.026), (I-130) + (3.027), (I-130) + (3.028), (I-130) + (3.029), (I-130) + (3.030), (I-130) + (3.031), (I-130) + (4.001), (I-130) + (4.002), (I-130) + (4.003), (I-130) + (4.004), (I-130) + (4.005), (I-130) + (4.006), (I-130) + (4.007), (I-130) + (4.008), (I-130) + (4.009), (I-130) + (4.010), (I-130) + (4.011), (I-130) + (4.012), (I-130) + (4.013), (I-130) + (4.014), (I-130) + (4.015), (I-130) + (4.016), (I-130) + (4.017), (I-130) + (4.018), (I-130) + (4.019), (I-130) + (4.020), (I-130) + (4.021), (I-130) + (4.022), (I-130) + (4.023), (I-130) + (4.024), (I-130) + (4.025), (I-130) + (4.026), (I-130) + (5.001), (I-130) + (5.002), (I-130) + (5.003), (I-130) + (5.004), (I-130) + (5.005), (I-130) + (5.006), (I-130) + (5.007), (I-130) + (5.008), (I-130) + (5.009), (I-130) + (5.010), (I-130) + (5.011), (I-130) + (5.012), (I-130) + (5.013), (I-130) + (5.014), (I-130) + (5.015), (I-130) + (5.016), (I-130) + (5.017), (I-130) + (5.018), (I-130) + (5.019), (I-130) + (5.020), (I-130) + (5.021), (I-130) + (5.022), (I-130) + (5.023), (I-130) + (6.001), (I-130) + (6.002), (I-130) + (6.003), (I-130) + (6.004), (I-130) + (7.001), (I-130) + (7.002), (I-130) + (7.003), (I-130) + (7.004), (I-130) + (7.005), (I-130) + (7.006), (I-130) + (8.001), (I-130) + (9.001), (I-130) + (9.002), (I-130) + (9.003), (I-130) + (9.004), (I-130) + (9.005), (I-130) + (9.006), (I-130) + (9.007), (I-130) + (9.008), (I-130) + (9.009), (I-130) + (10.001), (I-130) + (10.002), (I-130) + (10.003), (I-130) + (11.001), (I-130) + (11.002), (I-130) + (12.001), (I-130) + (12.002), (I-130) + (12.003), (I-130) + (12.004), (I-130) + (13.001), (I-130) + (13.002), (I-130) + (13.003), (I-130) + (13.004), (I-130) + (13.005), (I-130) + (13.006), (I-130) + (14.001), (I-130) + (14.002), (I-130) + (15.001), (I-130) + (15.002), (I-130) + (15.003), (I-130) + (15.004), (I-130) + (15.005), (I-130) + (15.006), (I-130) + (15.007), (I-130) + (15.008), (I-130) + (15.009), (I-130) + (15.010), (I-130) + (15.011), (I-130) + (15.012), (I-130) + (15.013), (I-130) + (15.014), (I-130) + (15.015), (I-130) + (15.016), (I-130) + (15.017), (I-130) + (15.018), (I-130) + (15.019), (I-130) + (15.020), (I-130) + (15.021), (I-130) + (15.022), (I-130) + (15.023), (I-130) + (15.024), (I-130) + (15.025), (I-130) + (15.026), (I-130) + (15.027), (I-130) + (15.028), (I-130) + (15.029), (I-130) + (15.030), (I-130) + (15.031), (I-130) + (15.032), (I-130) + (15.033), (I-130) + (15.034), (I-130) + (15.035), (I-130) + (15.036), (I-130) + (15.037), (I-130) + (15.038), (I-130) + (15.039), (I-130) + (15.040), (I-130) + (15.041), (I-130) + (15.042), (I-130) + (15.043), (I-130) + (15.044), (I-130) + (15.045), (I-130) + (15.046), (I-130) + (15.047), (I-130) + (15.048), (I-130) + (15.049), (I-130) + (15.050), (I-130) + (15.051), (I-130) + (15.052), (I-130) + (15.053), (I-130) + (15.054), (I-130) + (15.055), (I-130) + (15.056), (I-130) + (15.057), (I-130) + (15.058), (I-130) + (15.059), (I-130) + (15.060), (I-130) + (15.061), (I-130) + (15.062), (I-130) + (15.063) , (I-130) + (15.064), (I-130) + (15.065), (I-130) + (15.066), (I-130) + (15.067), (I-130) + (15.068), (I-130) + (15.069), (I-130) + (15.070), (I-130) + (15.071), (I-130) + (15.072), (I-130) + (15.073), (I-130) + (15.074), (I-130) + (15.075), (I-130) + (15.076), (I-130) + (15.077), (I-130) + (15.078), (I-130) + (15.079), (I-130) + (15.080), (I-130) + (15.081), (I-130) + (15.082), (I-130) + (15.083), (I-130) + (15.084), (I-130) + (15.085), (I-130) + (15.086), (I-130) + (15.087), (I-130) + (15.088), (I-130) + (15.089), (I-130) + (15.090), (I-130) + (15.091), (I-130) + (15.092), (I-130) + (15.093), (I-130) + (15.094), (I-130) + (15.095), (I-130) + (15.096), (I-130) + (15.097), (I-130) + (15.098), (I-130) + (15.099), (I-130) + (15.100), (I-130) + (15.101), (I-130) + (15.102), (I-130) + (15.103), (I-130) + (15.104), (I-130) + (15.105), (I-130) + (15.106), (I-130) + (15.107), (I-130) + (15.108), (I-130) + (15.109), (I-130) + (15.110), (I-130) + (15.111), (I-130) + (15.112), (I-130) + (15.113), (I-130) + (15.114), (I-130) + (15.115), (I-130) + (15.116), (I-130) + (15.117), (I-130) + (15.118), (I-130) + (15.119), (I-130) + (15.120), (I-130) + (15.121), (I-130) + (15.122), (I-130) + (15.123), (I-130) + (15.124), (I-130) + (15.125), (I-130) + (15.126), (I-130) + (15.127), (I-130) + (16.001), (I-130) + (16.002), (I-130) + (16.003), (I-130) + (16.004), (I-130) + (16.005), (I-130) + (16.006), (I-130) + (16.007), (I-130) + (16.008), (I-130) + (17.001), (I-130) + (17.002), (I-130) + (17.003), (I-130) + (17.004), (I-130) + (17.005), (I-130) + (17.006), (I-130) + (17.007), (I-130) + (17.008), (I-130) + (17.009), (I-130) + (17.010), (I-130) + (17.011), (I-130) + (17.012) 및 (I-130) + (18.001).
또한 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G3-1)으로부터 선택된다:
(I-300) + (1.001), (I-300) + (1.002), (I-300) + (1.003), (I-300) + (1.004), (I-300) + (1.005), (I-300) + (1.006), (I-300) + (1.007), (I-300) + (1.008), (I-300) + (1.009), (I-300) + (1.010), (I-300) + (1.011), (I-300) + (1.012), (I-300) + (1.013), (I-300) + (1.014), (I-300) + (1.015), (I-300) + (1.016), (I-300) + (1.017), (I-300) + (1.018), (I-300) + (1.019), (I-300) + (1.020), (I-300) + (1.021), (I-300) + (1.022), (I-300) + (1.023), (I-300) + (1.024), (I-300) + (1.025), (I-300) + (1.026), (I-300) + (1.027), (I-300) + (1.028), (I-300) + (1.029), (I-300) + (1.030), (I-300) + (1.031), (I-300) + (1.032), (I-300) + (1.033), (I-300) + (1.034), (I-300) + (1.035), (I-300) + (1.036), (I-300) + (1.037), (I-300) + (1.038), (I-300) + (1.039), (I-300) + (1.040), (I-300) + (1.041), (I-300) + (1.042), (I-300) + (1.043), (I-300) + (1.044), (I-300) + (1.045), (I-300) + (1.046), (I-300) + (1.047), (I-300) + (1.048), (I-300) + (1.049), (I-300) + (1.050), (I-300) + (1.051), (I-300) + (1.052), (I-300) + (1.053), (I-300) + (1.054), (I-300) + (1.055), (I-300) + (1.056), (I-300) + (1.057), (I-300) + (1.058), (I-300) + (1.059), (I-300) + (1.060), (I-300) + (1.061), (I-300) + (1.062), (I-300) + (1.063), (I-300) + (1.064), (I-300) + (1.065), (I-300) + (1.066), (I-300) + (1.067), (I-300) + (1.068), (I-300) + (1.069), (I-300) + (1.070), (I-300) + (1.071), (I-300) + (1.072), (I-300) + (1.073), (I-300) + (1.074), (I-300) + (1.075), (I-300) + (1.076), (I-300) + (1.077), (I-300) + (1.078), (I-300) + (1.079), (I-300) + (1.080), (I-300) + (1.081), (I-300) + (1.082), (I-300) + (1.083), (I-300) + (1.084), (I-300) + (1.085), (I-300) + (1.086), (I-300) + (1.087), (I-300) + (1.088), (I-300) + (1.089), (I-300) + (1.090), (I-300) + (1.091), (I-300) + (1.092), (I-300) + (2.001), (I-300) + (2.002), (I-300) + (2.003), (I-300) + (2.004), (I-300) + (2.005), (I-300) + (2.006), (I-300) + (2.007), (I-300) + (2.008), (I-300) + (2.009), (I-300) + (2.010), (I-300) + (2.011), (I-300) + (2.012), (I-300) + (2.013), (I-300) + (2.014), (I-300) + (2.015), (I-300) + (2.016), (I-300) + (2.017), (I-300) + (2.018), (I-300) + (2.019), (I-300) + (2.020), (I-300) + (2.021), (I-300) + (2.022), (I-300) + (2.023), (I-300) + (2.024), (I-300) + (2.025), (I-300) + (2.026), (I-300) + (2.027), (I-300) + (2.028), (I-300) + (2.029), (I-300) + (2.030), (I-300) + (2.031), (I-300) + (2.032), (I-300) + (2.033), (I-300) + (2.034), (I-300) + (2.035), (I-300) + (2.036), (I-300) + (2.037), (I-300) + (2.038), (I-300) + (2.039), (I-300) + (2.040), (I-300) + (2.041), (I-300) + (2.042), (I-300) + (2.043), (I-300) + (2.044), (I-300) + (2.045), (I-300) + (2.046), (I-300) + (2.047), (I-300) + (2.048), (I-300) + (2.049), (I-300) + (2.050), (I-300) + (2.051), (I-300) + (2.052), (I-300) + (2.053), (I-300) + (2.054), (I-300) + (2.055), (I-300) + (2.056), (I-300) + (2.057), (I-300) + (2.058), (I-300) + (2.059), (I-300) + (2.060), (I-300) + (3.001), (I-300) + (3.002), (I-300) + (3.003), (I-300) + (3.004), (I-300) + (3.005), (I-300) + (3.006), (I-300) + (3.007), (I-300) + (3.008), (I-300) + (3.009), (I-300) + (3.010), (I-300) + (3.011), (I-300) + (3.012), (I-300) + (3.013), (I-300) + (3.014), (I-300) + (3.015), (I-300) + (3.016), (I-300) + (3.017), (I-300) + (3.018), (I-300) + (3.019), (I-300) + (3.020), (I-300) + (3.021), (I-300) + (3.022), (I-300) + (3.023), (I-300) + (3.024), (I-300) + (3.025), (I-300) + (3.026), (I-300) + (3.027), (I-300) + (3.028), (I-300) + (3.029), (I-300) + (3.030), (I-300) + (3.031), (I-300) + (3.032), (I-300) + (4.001), (I-300) + (4.002), (I-300) + (4.003), (I-300) + (4.004), (I-300) + (4.005), (I-300) + (4.006), (I-300) + (4.007), (I-300) + (4.008), (I-300) + (4.009), (I-300) + (4.010), (I-300) + (4.011), (I-300) + (4.012), (I-300) + (4.013), (I-300) + (4.014), (I-300) + (4.015), (I-300) + (4.016), (I-300) + (4.017), (I-300) + (4.018), (I-300) + (4.019), (I-300) + (4.020), (I-300) + (4.021), (I-300) + (4.022), (I-300) + (4.023), (I-300) + (4.024), (I-300) + (4.025), (I-300) + (4.026), (I-300) + (5.001), (I-300) + (5.002), (I-300) + (5.003), (I-300) + (5.004), (I-300) + (5.005), (I-300) + (5.006), (I-300) + (5.007), (I-300) + (5.008), (I-300) + (5.009), (I-300) + (5.010), (I-300) + (5.011), (I-300) + (5.012), (I-300) + (5.013), (I-300) + (5.014), (I-300) + (5.015), (I-300) + (5.016), (I-300) + (5.017), (I-300) + (5.018), (I-300) + (5.019), (I-300) + (5.020), (I-300) + (5.021), (I-300) + (5.022), (I-300) + (5.023), (I-300) + (6.001), (I-300) + (6.002), (I-300) + (6.003), (I-300) + (6.004), (I-300) + (7.001), (I-300) + (7.002), (I-300) + (7.003), (I-300) + (7.004), (I-300) + (7.005), (I-300) + (7.006), (I-300) + (8.001), (I-300) + (9.001), (I-300) + (9.002), (I-300) + (9.003), (I-300) + (9.004), (I-300) + (9.005), (I-300) + (9.006), (I-300) + (9.007), (I-300) + (9.008), (I-300) + (9.009), (I-300) + (10.001), (I-300) + (10.002), (I-300) + (10.003), (I-300) + (11.001), (I-300) + (11.002), (I-300) + (12.001), (I-300) + (12.002), (I-300) + (12.003), (I-300) + (12.004), (I-300) + (13.001), (I-300) + (13.002), (I-300) + (13.003), (I-300) + (13.004), (I-300) + (13.005), (I-300) + (13.006), (I-300) + (14.001), (I-300) + (14.002), (I-300) + (15.001), (I-300) + (15.002), (I-300) + (15.003), (I-300) + (15.004), (I-300) + (15.005), (I-300) + (15.006), (I-300) + (15.007), (I-300) + (15.008), (I-300) + (15.009), (I-300) + (15.010), (I-300) + (15.011), (I-300) + (15.012), (I-300) + (15.013), (I-300) + (15.014), (I-300) + (15.015), (I-300) + (15.016), (I-300) + (15.017), (I-300) + (15.018), (I-300) + (15.019), (I-300) + (15.020), (I-300) + (15.021), (I-300) + (15.022), (I-300) + (15.023), (I-300) + (15.024), (I-300) + (15.025), (I-300) + (15.026), (I-300) + (15.027), (I-300) + (15.028), (I-300) + (15.029), (I-300) + (15.030), (I-300) + (15.031), (I-300) + (15.032), (I-300) + (15.033), (I-300) + (15.034), (I-300) + (15.035), (I-300) + (15.036), (I-300) + (15.037), (I-300) + (15.038), (I-300) + (15.039), (I-300) + (15.040), (I-300) + (15.041), (I-300) + (15.042), (I-300) + (15.043), (I-300) + (15.044), (I-300) + (15.045), (I-300) + (15.046), (I-300) + (15.047), (I-300) + (15.048), (I-300) + (15.049), (I-300) + (15.050), (I-300) + (15.051), (I-300) + (15.052), (I-300) + (15.053), (I-300) + (15.054), (I-300) + (15.055), (I-300) + (15.056), (I-300) + (15.057), (I-300) + (15.058), (I-300) + (15.059), (I-300) + (15.060), (I-300) + (15.061), (I-300) + (15.062), (I-300) + (15.063) , (I-300) + (15.064), (I-300) + (15.065), (I-300) + (15.066), (I-300) + (15.067), (I-300) + (15.068), (I-300) + (15.069), (I-300) + (15.070), (I-300) + (15.071), (I-300) + (15.072), (I-300) + (15.073), (I-300) + (15.074), (I-300) + (15.075), (I-300) + (15.076), (I-300) + (15.077), (I-300) + (15.078), (I-300) + (15.079), (I-300) + (15.080), (I-300) + (15.081), (I-300) + (15.082), (I-300) + (15.083), (I-300) + (15.084), (I-300) + (15.085), (I-300) + (15.086), (I-300) + (15.087), (I-300) + (15.088), (I-300) + (15.089), (I-300) + (15.090), (I-300) + (15.091), (I-300) + (15.092), (I-300) + (15.093), (I-300) + (15.094), (I-300) + (15.095), (I-300) + (15.096), (I-300) + (15.097), (I-300) + (15.098), (I-300) + (15.099), (I-300) + (15.100), (I-300) + (15.101), (I-300) + (15.102), (I-300) + (15.103), (I-300) + (15.104), (I-300) + (15.105), (I-300) + (15.106), (I-300) + (15.107), (I-300) + (15.108), (I-300) + (15.109), (I-300) + (15.110), (I-300) + (15.111), (I-300) + (15.112), (I-300) + (15.113), (I-300) + (15.114), (I-300) + (15.115), (I-300) + (15.116), (I-300) + (15.117), (I-300) + (15.118), (I-300) + (15.119), (I-300) + (15.120), (I-300) + (15.121), (I-300) + (15.122), (I-300) + (15.123), (I-300) + (15.124), (I-300) + (15.125), (I-300) + (15.126), (I-300) + (15.127), (I-300) + (15.128), (I-300) + (16.001), (I-300) + (16.002), (I-300) + (16.003), (I-300) + (16.004), (I-300) + (16.005), (I-300) + (16.006), (I-300) + (16.007), (I-300) + (16.008), (I-300) + (17.001), (I-300) + (17.002), (I-300) + (17.003), (I-300) + (17.004), (I-300) + (17.005), (I-300) + (17.006), (I-300) + (17.007), (I-300) + (17.008), (I-300) + (17.009), (I-300) + (17.010), (I-300) + (17.011), (I-300) + (17.012) 및 (I-300) + (18.001).
또한 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G3)으로부터 선택된다:
(I-300) + (1.001), (I-300) + (1.002), (I-300) + (1.003), (I-300) + (1.004), (I-300) + (1.005), (I-300) + (1.006), (I-300) + (1.007), (I-300) + (1.008), (I-300) + (1.009), (I-300) + (1.010), (I-300) + (1.011), (I-300) + (1.012), (I-300) + (1.013), (I-300) + (1.014), (I-300) + (1.015), (I-300) + (1.016), (I-300) + (1.017), (I-300) + (1.018), (I-300) + (1.019), (I-300) + (1.020), (I-300) + (1.021), (I-300) + (1.022), (I-300) + (1.023), (I-300) + (1.024), (I-300) + (1.025), (I-300) + (1.026), (I-300) + (1.027), (I-300) + (1.028), (I-300) + (1.029), (I-300) + (1.030), (I-300) + (1.031), (I-300) + (1.032), (I-300) + (1.033), (I-300) + (1.034), (I-300) + (1.035), (I-300) + (1.036), (I-300) + (1.037), (I-300) + (1.038), (I-300) + (1.039), (I-300) + (1.040), (I-300) + (1.041), (I-300) + (1.042), (I-300) + (1.043), (I-300) + (1.044), (I-300) + (1.045), (I-300) + (1.046), (I-300) + (1.047), (I-300) + (1.048), (I-300) + (1.049), (I-300) + (1.050), (I-300) + (1.051), (I-300) + (1.052), (I-300) + (1.053), (I-300) + (1.054), (I-300) + (1.055), (I-300) + (1.056), (I-300) + (1.057), (I-300) + (1.058), (I-300) + (1.059), (I-300) + (1.060), (I-300) + (1.061), (I-300) + (1.062), (I-300) + (1.063), (I-300) + (1.064), (I-300) + (1.065), (I-300) + (1.066), (I-300) + (1.067), (I-300) + (1.068), (I-300) + (1.069), (I-300) + (1.070), (I-300) + (1.071), (I-300) + (1.072), (I-300) + (1.073), (I-300) + (1.074), (I-300) + (1.075), (I-300) + (1.076), (I-300) + (1.077), (I-300) + (1.078), (I-300) + (1.079), (I-300) + (1.080), (I-300) + (1.081), (I-300) + (1.082), (I-300) + (1.083), (I-300) + (1.084), (I-300) + (1.085), (I-300) + (1.086), (I-300) + (1.087), (I-300) + (1.088), (I-300) + (1.089), (I-300) + (1.090), (I-300) + (1.091), (I-300) + (1.092), (I-300) + (2.001), (I-300) + (2.002), (I-300) + (2.003), (I-300) + (2.004), (I-300) + (2.005), (I-300) + (2.006), (I-300) + (2.007), (I-300) + (2.008), (I-300) + (2.009), (I-300) + (2.010), (I-300) + (2.011), (I-300) + (2.012), (I-300) + (2.013), (I-300) + (2.014), (I-300) + (2.015), (I-300) + (2.016), (I-300) + (2.017), (I-300) + (2.018), (I-300) + (2.019), (I-300) + (2.020), (I-300) + (2.021), (I-300) + (2.022), (I-300) + (2.023), (I-300) + (2.024), (I-300) + (2.025), (I-300) + (2.026), (I-300) + (2.027), (I-300) + (2.028), (I-300) + (2.029), (I-300) + (2.030), (I-300) + (2.031), (I-300) + (2.032), (I-300) + (2.033), (I-300) + (2.034), (I-300) + (2.035), (I-300) + (2.036), (I-300) + (2.037), (I-300) + (2.038), (I-300) + (2.039), (I-300) + (2.040), (I-300) + (2.041), (I-300) + (2.042), (I-300) + (2.043), (I-300) + (2.044), (I-300) + (2.045), (I-300) + (2.046), (I-300) + (2.047), (I-300) + (2.048), (I-300) + (2.049), (I-300) + (2.050), (I-300) + (2.051), (I-300) + (2.052), (I-300) + (2.053), (I-300) + (2.054), (I-300) + (2.055), (I-300) + (2.056), (I-300) + (2.057), (I-300) + (2.058), (I-300) + (2.059), (I-300) + (3.001), (I-300) + (3.002), (I-300) + (3.003), (I-300) + (3.004), (I-300) + (3.005), (I-300) + (3.006), (I-300) + (3.007), (I-300) + (3.008), (I-300) + (3.009), (I-300) + (3.010), (I-300) + (3.011), (I-300) + (3.012), (I-300) + (3.013), (I-300) + (3.014), (I-300) + (3.015), (I-300) + (3.016), (I-300) + (3.017), (I-300) + (3.018), (I-300) + (3.019), (I-300) + (3.020), (I-300) + (3.021), (I-300) + (3.022), (I-300) + (3.023), (I-300) + (3.024), (I-300) + (3.025), (I-300) + (3.026), (I-300) + (3.027), (I-300) + (3.028), (I-300) + (3.029), (I-300) + (3.030), (I-300) + (3.031), (I-300) + (4.001), (I-300) + (4.002), (I-300) + (4.003), (I-300) + (4.004), (I-300) + (4.005), (I-300) + (4.006), (I-300) + (4.007), (I-300) + (4.008), (I-300) + (4.009), (I-300) + (4.010), (I-300) + (4.011), (I-300) + (4.012), (I-300) + (4.013), (I-300) + (4.014), (I-300) + (4.015), (I-300) + (4.016), (I-300) + (4.017), (I-300) + (4.018), (I-300) + (4.019), (I-300) + (4.020), (I-300) + (4.021), (I-300) + (4.022), (I-300) + (4.023), (I-300) + (4.024), (I-300) + (4.025), (I-300) + (4.026), (I-300) + (5.001), (I-300) + (5.002), (I-300) + (5.003), (I-300) + (5.004), (I-300) + (5.005), (I-300) + (5.006), (I-300) + (5.007), (I-300) + (5.008), (I-300) + (5.009), (I-300) + (5.010), (I-300) + (5.011), (I-300) + (5.012), (I-300) + (5.013), (I-300) + (5.014), (I-300) + (5.015), (I-300) + (5.016), (I-300) + (5.017), (I-300) + (5.018), (I-300) + (5.019), (I-300) + (5.020), (I-300) + (5.021), (I-300) + (5.022), (I-300) + (5.023), (I-300) + (6.001), (I-300) + (6.002), (I-300) + (6.003), (I-300) + (6.004), (I-300) + (7.001), (I-300) + (7.002), (I-300) + (7.003), (I-300) + (7.004), (I-300) + (7.005), (I-300) + (7.006), (I-300) + (8.001), (I-300) + (9.001), (I-300) + (9.002), (I-300) + (9.003), (I-300) + (9.004), (I-300) + (9.005), (I-300) + (9.006), (I-300) + (9.007), (I-300) + (9.008), (I-300) + (9.009), (I-300) + (10.001), (I-300) + (10.002), (I-300) + (10.003), (I-300) + (11.001), (I-300) + (11.002), (I-300) + (12.001), (I-300) + (12.002), (I-300) + (12.003), (I-300) + (12.004), (I-300) + (13.001), (I-300) + (13.002), (I-300) + (13.003), (I-300) + (13.004), (I-300) + (13.005), (I-300) + (13.006), (I-300) + (14.001), (I-300) + (14.002), (I-300) + (15.001), (I-300) + (15.002), (I-300) + (15.003), (I-300) + (15.004), (I-300) + (15.005), (I-300) + (15.006), (I-300) + (15.007), (I-300) + (15.008), (I-300) + (15.009), (I-300) + (15.010), (I-300) + (15.011), (I-300) + (15.012), (I-300) + (15.013), (I-300) + (15.014), (I-300) + (15.015), (I-300) + (15.016), (I-300) + (15.017), (I-300) + (15.018), (I-300) + (15.019), (I-300) + (15.020), (I-300) + (15.021), (I-300) + (15.022), (I-300) + (15.023), (I-300) + (15.024), (I-300) + (15.025), (I-300) + (15.026), (I-300) + (15.027), (I-300) + (15.028), (I-300) + (15.029), (I-300) + (15.030), (I-300) + (15.031), (I-300) + (15.032), (I-300) + (15.033), (I-300) + (15.034), (I-300) + (15.035), (I-300) + (15.036), (I-300) + (15.037), (I-300) + (15.038), (I-300) + (15.039), (I-300) + (15.040), (I-300) + (15.041), (I-300) + (15.042), (I-300) + (15.043), (I-300) + (15.044), (I-300) + (15.045), (I-300) + (15.046), (I-300) + (15.047), (I-300) + (15.048), (I-300) + (15.049), (I-300) + (15.050), (I-300) + (15.051), (I-300) + (15.052), (I-300) + (15.053), (I-300) + (15.054), (I-300) + (15.055), (I-300) + (15.056), (I-300) + (15.057), (I-300) + (15.058), (I-300) + (15.059), (I-300) + (15.060), (I-300) + (15.061), (I-300) + (15.062), (I-300) + (15.063) , (I-300) + (15.064), (I-300) + (15.065), (I-300) + (15.066), (I-300) + (15.067), (I-300) + (15.068), (I-300) + (15.069), (I-300) + (15.070), (I-300) + (15.071), (I-300) + (15.072), (I-300) + (15.073), (I-300) + (15.074), (I-300) + (15.075), (I-300) + (15.076), (I-300) + (15.077), (I-300) + (15.078), (I-300) + (15.079), (I-300) + (15.080), (I-300) + (15.081), (I-300) + (15.082), (I-300) + (15.083), (I-300) + (15.084), (I-300) + (15.085), (I-300) + (15.086), (I-300) + (15.087), (I-300) + (15.088), (I-300) + (15.089), (I-300) + (15.090), (I-300) + (15.091), (I-300) + (15.092), (I-300) + (15.093), (I-300) + (15.094), (I-300) + (15.095), (I-300) + (15.096), (I-300) + (15.097), (I-300) + (15.098), (I-300) + (15.099), (I-300) + (15.100), (I-300) + (15.101), (I-300) + (15.102), (I-300) + (15.103), (I-300) + (15.104), (I-300) + (15.105), (I-300) + (15.106), (I-300) + (15.107), (I-300) + (15.108), (I-300) + (15.109), (I-300) + (15.110), (I-300) + (15.111), (I-300) + (15.112), (I-300) + (15.113), (I-300) + (15.114), (I-300) + (15.115), (I-300) + (15.116), (I-300) + (15.117), (I-300) + (15.118), (I-300) + (15.119), (I-300) + (15.120), (I-300) + (15.121), (I-300) + (15.122), (I-300) + (15.123), (I-300) + (15.124), (I-300) + (15.125), (I-300) + (15.126), (I-300) + (15.127), (I-300) + (16.001), (I-300) + (16.002), (I-300) + (16.003), (I-300) + (16.004), (I-300) + (16.005), (I-300) + (16.006), (I-300) + (16.007), (I-300) + (16.008), (I-300) + (17.001), (I-300) + (17.002), (I-300) + (17.003), (I-300) + (17.004), (I-300) + (17.005), (I-300) + (17.006), (I-300) + (17.007), (I-300) + (17.008), (I-300) + (17.009), (I-300) + (17.010), (I-300) + (17.011), (I-300) + (17.012) 및 (I-300) + (18.001).
또한 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G4-1)으로부터 선택된다:
(I-302) + (1.001), (I-302) + (1.002), (I-302) + (1.003), (I-302) + (1.004), (I-302) + (1.005), (I-302) + (1.006), (I-302) + (1.007), (I-302) + (1.008), (I-302) + (1.009), (I-302) + (1.010), (I-302) + (1.011), (I-302) + (1.012), (I-302) + (1.013), (I-302) + (1.014), (I-302) + (1.015), (I-302) + (1.016), (I-302) + (1.017), (I-302) + (1.018), (I-302) + (1.019), (I-302) + (1.020), (I-302) + (1.021), (I-302) + (1.022), (I-302) + (1.023), (I-302) + (1.024), (I-302) + (1.025), (I-302) + (1.026), (I-302) + (1.027), (I-302) + (1.028), (I-302) + (1.029), (I-302) + (1.030), (I-302) + (1.031), (I-302) + (1.032), (I-302) + (1.033), (I-302) + (1.034), (I-302) + (1.035), (I-302) + (1.036), (I-302) + (1.037), (I-302) + (1.038), (I-302) + (1.039), (I-302) + (1.040), (I-302) + (1.041), (I-302) + (1.042), (I-302) + (1.043), (I-302) + (1.044), (I-302) + (1.045), (I-302) + (1.046), (I-302) + (1.047), (I-302) + (1.048), (I-302) + (1.049), (I-302) + (1.050), (I-302) + (1.051), (I-302) + (1.052), (I-302) + (1.053), (I-302) + (1.054), (I-302) + (1.055), (I-302) + (1.056), (I-302) + (1.057), (I-302) + (1.058), (I-302) + (1.059), (I-302) + (1.060), (I-302) + (1.061), (I-302) + (1.062), (I-302) + (1.063), (I-302) + (1.064), (I-302) + (1.065), (I-302) + (1.066), (I-302) + (1.067), (I-302) + (1.068), (I-302) + (1.069), (I-302) + (1.070), (I-302) + (1.071), (I-302) + (1.072), (I-302) + (1.073), (I-302) + (1.074), (I-302) + (1.075), (I-302) + (1.076), (I-302) + (1.077), (I-302) + (1.078), (I-302) + (1.079), (I-302) + (1.080), (I-302) + (1.081), (I-302) + (1.082), (I-302) + (1.083), (I-302) + (1.084), (I-302) + (1.085), (I-302) + (1.086), (I-302) + (1.087), (I-302) + (1.088), (I-302) + (1.089), (I-302) + (1.090), (I-302) + (1.091), (I-302) + (1.092), (I-302) + (2.001), (I-302) + (2.002), (I-302) + (2.003), (I-302) + (2.004), (I-302) + (2.005), (I-302) + (2.006), (I-302) + (2.007), (I-302) + (2.008), (I-302) + (2.009), (I-302) + (2.010), (I-302) + (2.011), (I-302) + (2.012), (I-302) + (2.013), (I-302) + (2.014), (I-302) + (2.015), (I-302) + (2.016), (I-302) + (2.017), (I-302) + (2.018), (I-302) + (2.019), (I-302) + (2.020), (I-302) + (2.021), (I-302) + (2.022), (I-302) + (2.023), (I-302) + (2.024), (I-302) + (2.025), (I-302) + (2.026), (I-302) + (2.027), (I-302) + (2.028), (I-302) + (2.029), (I-302) + (2.030), (I-302) + (2.031), (I-302) + (2.032), (I-302) + (2.033), (I-302) + (2.034), (I-302) + (2.035), (I-302) + (2.036), (I-302) + (2.037), (I-302) + (2.038), (I-302) + (2.039), (I-302) + (2.040), (I-302) + (2.041), (I-302) + (2.042), (I-302) + (2.043), (I-302) + (2.044), (I-302) + (2.045), (I-302) + (2.046), (I-302) + (2.047), (I-302) + (2.048), (I-302) + (2.049), (I-302) + (2.050), (I-302) + (2.051), (I-302) + (2.052), (I-302) + (2.053), (I-302) + (2.054), (I-302) + (2.055), (I-302) + (2.056), (I-302) + (2.057), (I-302) + (2.058), (I-302) + (2.059), (I-302) + (2.060), (I-302) + (3.001), (I-302) + (3.002), (I-302) + (3.003), (I-302) + (3.004), (I-302) + (3.005), (I-302) + (3.006), (I-302) + (3.007), (I-302) + (3.008), (I-302) + (3.009), (I-302) + (3.010), (I-302) + (3.011), (I-302) + (3.012), (I-302) + (3.013), (I-302) + (3.014), (I-302) + (3.015), (I-302) + (3.016), (I-302) + (3.017), (I-302) + (3.018), (I-302) + (3.019), (I-302) + (3.020), (I-302) + (3.021), (I-302) + (3.022), (I-302) + (3.023), (I-302) + (3.024), (I-302) + (3.025), (I-302) + (3.026), (I-302) + (3.027), (I-302) + (3.028), (I-302) + (3.029), (I-302) + (3.030), (I-302) + (3.031), (I-302) + (3.032), (I-302) + (4.001), (I-302) + (4.002), (I-302) + (4.003), (I-302) + (4.004), (I-302) + (4.005), (I-302) + (4.006), (I-302) + (4.007), (I-302) + (4.008), (I-302) + (4.009), (I-302) + (4.010), (I-302) + (4.011), (I-302) + (4.012), (I-302) + (4.013), (I-302) + (4.014), (I-302) + (4.015), (I-302) + (4.016), (I-302) + (4.017), (I-302) + (4.018), (I-302) + (4.019), (I-302) + (4.020), (I-302) + (4.021), (I-302) + (4.022), (I-302) + (4.023), (I-302) + (4.024), (I-302) + (4.025), (I-302) + (4.026), (I-302) + (5.001), (I-302) + (5.002), (I-302) + (5.003), (I-302) + (5.004), (I-302) + (5.005), (I-302) + (5.006), (I-302) + (5.007), (I-302) + (5.008), (I-302) + (5.009), (I-302) + (5.010), (I-302) + (5.011), (I-302) + (5.012), (I-302) + (5.013), (I-302) + (5.014), (I-302) + (5.015), (I-302) + (5.016), (I-302) + (5.017), (I-302) + (5.018), (I-302) + (5.019), (I-302) + (5.020), (I-302) + (5.021), (I-302) + (5.022), (I-302) + (5.023), (I-302) + (6.001), (I-302) + (6.002), (I-302) + (6.003), (I-302) + (6.004), (I-302) + (7.001), (I-302) + (7.002), (I-302) + (7.003), (I-302) + (7.004), (I-302) + (7.005), (I-302) + (7.006), (I-302) + (8.001), (I-302) + (9.001), (I-302) + (9.002), (I-302) + (9.003), (I-302) + (9.004), (I-302) + (9.005), (I-302) + (9.006), (I-302) + (9.007), (I-302) + (9.008), (I-302) + (9.009), (I-302) + (10.001), (I-302) + (10.002), (I-302) + (10.003), (I-302) + (11.001), (I-302) + (11.002), (I-302) + (12.001), (I-302) + (12.002), (I-302) + (12.003), (I-302) + (12.004), (I-302) + (13.001), (I-302) + (13.002), (I-302) + (13.003), (I-302) + (13.004), (I-302) + (13.005), (I-302) + (13.006), (I-302) + (14.001), (I-302) + (14.002), (I-302) + (15.001), (I-302) + (15.002), (I-302) + (15.003), (I-302) + (15.004), (I-302) + (15.005), (I-302) + (15.006), (I-302) + (15.007), (I-302) + (15.008), (I-302) + (15.009), (I-302) + (15.010), (I-302) + (15.011), (I-302) + (15.012), (I-302) + (15.013), (I-302) + (15.014), (I-302) + (15.015), (I-302) + (15.016), (I-302) + (15.017), (I-302) + (15.018), (I-302) + (15.019), (I-302) + (15.020), (I-302) + (15.021), (I-302) + (15.022), (I-302) + (15.023), (I-302) + (15.024), (I-302) + (15.025), (I-302) + (15.026), (I-302) + (15.027), (I-302) + (15.028), (I-302) + (15.029), (I-302) + (15.030), (I-302) + (15.031), (I-302) + (15.032), (I-302) + (15.033), (I-302) + (15.034), (I-302) + (15.035), (I-302) + (15.036), (I-302) + (15.037), (I-302) + (15.038), (I-302) + (15.039), (I-302) + (15.040), (I-302) + (15.041), (I-302) + (15.042), (I-302) + (15.043), (I-302) + (15.044), (I-302) + (15.045), (I-302) + (15.046), (I-302) + (15.047), (I-302) + (15.048), (I-302) + (15.049), (I-302) + (15.050), (I-302) + (15.051), (I-302) + (15.052), (I-302) + (15.053), (I-302) + (15.054), (I-302) + (15.055), (I-302) + (15.056), (I-302) + (15.057), (I-302) + (15.058), (I-302) + (15.059), (I-302) + (15.060), (I-302) + (15.061), (I-302) + (15.062), (I-302) + (15.063) , (I-302) + (15.064), (I-302) + (15.065), (I-302) + (15.066), (I-302) + (15.067), (I-302) + (15.068), (I-302) + (15.069), (I-302) + (15.070), (I-302) + (15.071), (I-302) + (15.072), (I-302) + (15.073), (I-302) + (15.074), (I-302) + (15.075), (I-302) + (15.076), (I-302) + (15.077), (I-302) + (15.078), (I-302) + (15.079), (I-302) + (15.080), (I-302) + (15.081), (I-302) + (15.082), (I-302) + (15.083), (I-302) + (15.084), (I-302) + (15.085), (I-302) + (15.086), (I-302) + (15.087), (I-302) + (15.088), (I-302) + (15.089), (I-302) + (15.090), (I-302) + (15.091), (I-302) + (15.092), (I-302) + (15.093), (I-302) + (15.094), (I-302) + (15.095), (I-302) + (15.096), (I-302) + (15.097), (I-302) + (15.098), (I-302) + (15.099), (I-302) + (15.100), (I-302) + (15.101), (I-302) + (15.102), (I-302) + (15.103), (I-302) + (15.104), (I-302) + (15.105), (I-302) + (15.106), (I-302) + (15.107), (I-302) + (15.108), (I-302) + (15.109), (I-302) + (15.110), (I-302) + (15.111), (I-302) + (15.112), (I-302) + (15.113), (I-302) + (15.114), (I-302) + (15.115), (I-302) + (15.116), (I-302) + (15.117), (I-302) + (15.118), (I-302) + (15.119), (I-302) + (15.120), (I-302) + (15.121), (I-302) + (15.122), (I-302) + (15.123), (I-302) + (15.124), (I-302) + (15.125), (I-302) + (15.126), (I-302) + (15.127), (I-302) + (15.128), (I-302) + (16.001), (I-302) + (16.002), (I-302) + (16.003), (I-302) + (16.004), (I-302) + (16.005), (I-302) + (16.006), (I-302) + (16.007), (I-302) + (16.008), (I-302) + (17.001), (I-302) + (17.002), (I-302) + (17.003), (I-302) + (17.004), (I-302) + (17.005), (I-302) + (17.006), (I-302) + (17.007), (I-302) + (17.008), (I-302) + (17.009), (I-302) + (17.010), (I-302) + (17.011), (I-302) + (17.012) 및 (I-302) + (18.001).
또한 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G4)으로부터 선택된다:
(I-302) + (1.001), (I-302) + (1.002), (I-302) + (1.003), (I-302) + (1.004), (I-302) + (1.005), (I-302) + (1.006), (I-302) + (1.007), (I-302) + (1.008), (I-302) + (1.009), (I-302) + (1.010), (I-302) + (1.011), (I-302) + (1.012), (I-302) + (1.013), (I-302) + (1.014), (I-302) + (1.015), (I-302) + (1.016), (I-302) + (1.017), (I-302) + (1.018), (I-302) + (1.019), (I-302) + (1.020), (I-302) + (1.021), (I-302) + (1.022), (I-302) + (1.023), (I-302) + (1.024), (I-302) + (1.025), (I-302) + (1.026), (I-302) + (1.027), (I-302) + (1.028), (I-302) + (1.029), (I-302) + (1.030), (I-302) + (1.031), (I-302) + (1.032), (I-302) + (1.033), (I-302) + (1.034), (I-302) + (1.035), (I-302) + (1.036), (I-302) + (1.037), (I-302) + (1.038), (I-302) + (1.039), (I-302) + (1.040), (I-302) + (1.041), (I-302) + (1.042), (I-302) + (1.043), (I-302) + (1.044), (I-302) + (1.045), (I-302) + (1.046), (I-302) + (1.047), (I-302) + (1.048), (I-302) + (1.049), (I-302) + (1.050), (I-302) + (1.051), (I-302) + (1.052), (I-302) + (1.053), (I-302) + (1.054), (I-302) + (1.055), (I-302) + (1.056), (I-302) + (1.057), (I-302) + (1.058), (I-302) + (1.059), (I-302) + (1.060), (I-302) + (1.061), (I-302) + (1.062), (I-302) + (1.063), (I-302) + (1.064), (I-302) + (1.065), (I-302) + (1.066), (I-302) + (1.067), (I-302) + (1.068), (I-302) + (1.069), (I-302) + (1.070), (I-302) + (1.071), (I-302) + (1.072), (I-302) + (1.073), (I-302) + (1.074), (I-302) + (1.075), (I-302) + (1.076), (I-302) + (1.077), (I-302) + (1.078), (I-302) + (1.079), (I-302) + (1.080), (I-302) + (1.081), (I-302) + (1.082), (I-302) + (1.083), (I-302) + (1.084), (I-302) + (1.085), (I-302) + (1.086), (I-302) + (1.087), (I-302) + (1.088), (I-302) + (1.089), (I-302) + (1.090), (I-302) + (1.091), (I-302) + (1.092), (I-302) + (2.001), (I-302) + (2.002), (I-302) + (2.003), (I-302) + (2.004), (I-302) + (2.005), (I-302) + (2.006), (I-302) + (2.007), (I-302) + (2.008), (I-302) + (2.009), (I-302) + (2.010), (I-302) + (2.011), (I-302) + (2.012), (I-302) + (2.013), (I-302) + (2.014), (I-302) + (2.015), (I-302) + (2.016), (I-302) + (2.017), (I-302) + (2.018), (I-302) + (2.019), (I-302) + (2.020), (I-302) + (2.021), (I-302) + (2.022), (I-302) + (2.023), (I-302) + (2.024), (I-302) + (2.025), (I-302) + (2.026), (I-302) + (2.027), (I-302) + (2.028), (I-302) + (2.029), (I-302) + (2.030), (I-302) + (2.031), (I-302) + (2.032), (I-302) + (2.033), (I-302) + (2.034), (I-302) + (2.035), (I-302) + (2.036), (I-302) + (2.037), (I-302) + (2.038), (I-302) + (2.039), (I-302) + (2.040), (I-302) + (2.041), (I-302) + (2.042), (I-302) + (2.043), (I-302) + (2.044), (I-302) + (2.045), (I-302) + (2.046), (I-302) + (2.047), (I-302) + (2.048), (I-302) + (2.049), (I-302) + (2.050), (I-302) + (2.051), (I-302) + (2.052), (I-302) + (2.053), (I-302) + (2.054), (I-302) + (2.055), (I-302) + (2.056), (I-302) + (2.057), (I-302) + (2.058), (I-302) + (2.059), (I-302) + (3.001), (I-302) + (3.002), (I-302) + (3.003), (I-302) + (3.004), (I-302) + (3.005), (I-302) + (3.006), (I-302) + (3.007), (I-302) + (3.008), (I-302) + (3.009), (I-302) + (3.010), (I-302) + (3.011), (I-302) + (3.012), (I-302) + (3.013), (I-302) + (3.014), (I-302) + (3.015), (I-302) + (3.016), (I-302) + (3.017), (I-302) + (3.018), (I-302) + (3.019), (I-302) + (3.020), (I-302) + (3.021), (I-302) + (3.022), (I-302) + (3.023), (I-302) + (3.024), (I-302) + (3.025), (I-302) + (3.026), (I-302) + (3.027), (I-302) + (3.028), (I-302) + (3.029), (I-302) + (3.030), (I-302) + (3.031), (I-302) + (4.001), (I-302) + (4.002), (I-302) + (4.003), (I-302) + (4.004), (I-302) + (4.005), (I-302) + (4.006), (I-302) + (4.007), (I-302) + (4.008), (I-302) + (4.009), (I-302) + (4.010), (I-302) + (4.011), (I-302) + (4.012), (I-302) + (4.013), (I-302) + (4.014), (I-302) + (4.015), (I-302) + (4.016), (I-302) + (4.017), (I-302) + (4.018), (I-302) + (4.019), (I-302) + (4.020), (I-302) + (4.021), (I-302) + (4.022), (I-302) + (4.023), (I-302) + (4.024), (I-302) + (4.025), (I-302) + (4.026), (I-302) + (5.001), (I-302) + (5.002), (I-302) + (5.003), (I-302) + (5.004), (I-302) + (5.005), (I-302) + (5.006), (I-302) + (5.007), (I-302) + (5.008), (I-302) + (5.009), (I-302) + (5.010), (I-302) + (5.011), (I-302) + (5.012), (I-302) + (5.013), (I-302) + (5.014), (I-302) + (5.015), (I-302) + (5.016), (I-302) + (5.017), (I-302) + (5.018), (I-302) + (5.019), (I-302) + (5.020), (I-302) + (5.021), (I-302) + (5.022), (I-302) + (5.023), (I-302) + (6.001), (I-302) + (6.002), (I-302) + (6.003), (I-302) + (6.004), (I-302) + (7.001), (I-302) + (7.002), (I-302) + (7.003), (I-302) + (7.004), (I-302) + (7.005), (I-302) + (7.006), (I-302) + (8.001), (I-302) + (9.001), (I-302) + (9.002), (I-302) + (9.003), (I-302) + (9.004), (I-302) + (9.005), (I-302) + (9.006), (I-302) + (9.007), (I-302) + (9.008), (I-302) + (9.009), (I-302) + (10.001), (I-302) + (10.002), (I-302) + (10.003), (I-302) + (11.001), (I-302) + (11.002), (I-302) + (12.001), (I-302) + (12.002), (I-302) + (12.003), (I-302) + (12.004), (I-302) + (13.001), (I-302) + (13.002), (I-302) + (13.003), (I-302) + (13.004), (I-302) + (13.005), (I-302) + (13.006), (I-302) + (14.001), (I-302) + (14.002), (I-302) + (15.001), (I-302) + (15.002), (I-302) + (15.003), (I-302) + (15.004), (I-302) + (15.005), (I-302) + (15.006), (I-302) + (15.007), (I-302) + (15.008), (I-302) + (15.009), (I-302) + (15.010), (I-302) + (15.011), (I-302) + (15.012), (I-302) + (15.013), (I-302) + (15.014), (I-302) + (15.015), (I-302) + (15.016), (I-302) + (15.017), (I-302) + (15.018), (I-302) + (15.019), (I-302) + (15.020), (I-302) + (15.021), (I-302) + (15.022), (I-302) + (15.023), (I-302) + (15.024), (I-302) + (15.025), (I-302) + (15.026), (I-302) + (15.027), (I-302) + (15.028), (I-302) + (15.029), (I-302) + (15.030), (I-302) + (15.031), (I-302) + (15.032), (I-302) + (15.033), (I-302) + (15.034), (I-302) + (15.035), (I-302) + (15.036), (I-302) + (15.037), (I-302) + (15.038), (I-302) + (15.039), (I-302) + (15.040), (I-302) + (15.041), (I-302) + (15.042), (I-302) + (15.043), (I-302) + (15.044), (I-302) + (15.045), (I-302) + (15.046), (I-302) + (15.047), (I-302) + (15.048), (I-302) + (15.049), (I-302) + (15.050), (I-302) + (15.051), (I-302) + (15.052), (I-302) + (15.053), (I-302) + (15.054), (I-302) + (15.055), (I-302) + (15.056), (I-302) + (15.057), (I-302) + (15.058), (I-302) + (15.059), (I-302) + (15.060), (I-302) + (15.061), (I-302) + (15.062), (I-302) + (15.063) , (I-302) + (15.064), (I-302) + (15.065), (I-302) + (15.066), (I-302) + (15.067), (I-302) + (15.068), (I-302) + (15.069), (I-302) + (15.070), (I-302) + (15.071), (I-302) + (15.072), (I-302) + (15.073), (I-302) + (15.074), (I-302) + (15.075), (I-302) + (15.076), (I-302) + (15.077), (I-302) + (15.078), (I-302) + (15.079), (I-302) + (15.080), (I-302) + (15.081), (I-302) + (15.082), (I-302) + (15.083), (I-302) + (15.084), (I-302) + (15.085), (I-302) + (15.086), (I-302) + (15.087), (I-302) + (15.088), (I-302) + (15.089), (I-302) + (15.090), (I-302) + (15.091), (I-302) + (15.092), (I-302) + (15.093), (I-302) + (15.094), (I-302) + (15.095), (I-302) + (15.096), (I-302) + (15.097), (I-302) + (15.098), (I-302) + (15.099), (I-302) + (15.100), (I-302) + (15.101), (I-302) + (15.102), (I-302) + (15.103), (I-302) + (15.104), (I-302) + (15.105), (I-302) + (15.106), (I-302) + (15.107), (I-302) + (15.108), (I-302) + (15.109), (I-302) + (15.110), (I-302) + (15.111), (I-302) + (15.112), (I-302) + (15.113), (I-302) + (15.114), (I-302) + (15.115), (I-302) + (15.116), (I-302) + (15.117), (I-302) + (15.118), (I-302) + (15.119), (I-302) + (15.120), (I-302) + (15.121), (I-302) + (15.122), (I-302) + (15.123), (I-302) + (15.124), (I-302) + (15.125), (I-302) + (15.126), (I-302) + (15.127), (I-302) + (16.1001), (I-302) + (16.1002), (I-302) + (16.1003), (I-302) + (16.1004), (I-302) + (16.1005), (I-302) + (16.2001), (I-302) + (16.2002), (I-302) + (16.2003), (I-302) + (17.001), (I-302) + (17.002), (I-302) + (17.003), (I-302) + (17.004), (I-302) + (17.005), (I-302) + (17.006), (I-302) + (17.007), (I-302) + (17.008), (I-302) + (17.009), (I-302) + (17.010), (I-302) + (17.011), (I-302) + (17.012) 및 (I-302) + (18.001).
또한 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G5-1)으로부터 선택된다:
(I-337) + (1.001), (I-337) + (1.002), (I-337) + (1.003), (I-337) + (1.004), (I-337) + (1.005), (I-337) + (1.006), (I-337) + (1.007), (I-337) + (1.008), (I-337) + (1.009), (I-337) + (1.010), (I-337) + (1.011), (I-337) + (1.012), (I-337) + (1.013), (I-337) + (1.014), (I-337) + (1.015), (I-337) + (1.016), (I-337) + (1.017), (I-337) + (1.018), (I-337) + (1.019), (I-337) + (1.020), (I-337) + (1.021), (I-337) + (1.022), (I-337) + (1.023), (I-337) + (1.024), (I-337) + (1.025), (I-337) + (1.026), (I-337) + (1.027), (I-337) + (1.028), (I-337) + (1.029), (I-337) + (1.030), (I-337) + (1.031), (I-337) + (1.032), (I-337) + (1.033), (I-337) + (1.034), (I-337) + (1.035), (I-337) + (1.036), (I-337) + (1.037), (I-337) + (1.038), (I-337) + (1.039), (I-337) + (1.040), (I-337) + (1.041), (I-337) + (1.042), (I-337) + (1.043), (I-337) + (1.044), (I-337) + (1.045), (I-337) + (1.046), (I-337) + (1.047), (I-337) + (1.048), (I-337) + (1.049), (I-337) + (1.050), (I-337) + (1.051), (I-337) + (1.052), (I-337) + (1.053), (I-337) + (1.054), (I-337) + (1.055), (I-337) + (1.056), (I-337) + (1.057), (I-337) + (1.058), (I-337) + (1.059), (I-337) + (1.060), (I-337) + (1.061), (I-337) + (1.062), (I-337) + (1.063), (I-337) + (1.064), (I-337) + (1.065), (I-337) + (1.066), (I-337) + (1.067), (I-337) + (1.068), (I-337) + (1.069), (I-337) + (1.070), (I-337) + (1.071), (I-337) + (1.072), (I-337) + (1.073), (I-337) + (1.074), (I-337) + (1.075), (I-337) + (1.076), (I-337) + (1.077), (I-337) + (1.078), (I-337) + (1.079), (I-337) + (1.080), (I-337) + (1.081), (I-337) + (1.082), (I-337) + (1.083), (I-337) + (1.084), (I-337) + (1.085), (I-337) + (1.086), (I-337) + (1.087), (I-337) + (1.088), (I-337) + (1.089), (I-337) + (1.090), (I-337) + (1.091), (I-337) + (1.092), (I-337) + (2.001), (I-337) + (2.002), (I-337) + (2.003), (I-337) + (2.004), (I-337) + (2.005), (I-337) + (2.006), (I-337) + (2.007), (I-337) + (2.008), (I-337) + (2.009), (I-337) + (2.010), (I-337) + (2.011), (I-337) + (2.012), (I-337) + (2.013), (I-337) + (2.014), (I-337) + (2.015), (I-337) + (2.016), (I-337) + (2.017), (I-337) + (2.018), (I-337) + (2.019), (I-337) + (2.020), (I-337) + (2.021), (I-337) + (2.022), (I-337) + (2.023), (I-337) + (2.024), (I-337) + (2.025), (I-337) + (2.026), (I-337) + (2.027), (I-337) + (2.028), (I-337) + (2.029), (I-337) + (2.030), (I-337) + (2.031), (I-337) + (2.032), (I-337) + (2.033), (I-337) + (2.034), (I-337) + (2.035), (I-337) + (2.036), (I-337) + (2.037), (I-337) + (2.038), (I-337) + (2.039), (I-337) + (2.040), (I-337) + (2.041), (I-337) + (2.042), (I-337) + (2.043), (I-337) + (2.044), (I-337) + (2.045), (I-337) + (2.046), (I-337) + (2.047), (I-337) + (2.048), (I-337) + (2.049), (I-337) + (2.050), (I-337) + (2.051), (I-337) + (2.052), (I-337) + (2.053), (I-337) + (2.054), (I-337) + (2.055), (I-337) + (2.056), (I-337) + (2.057), (I-337) + (2.058), (I-337) + (2.059), (I-337) + (2.060), (I-337) + (3.001), (I-337) + (3.002), (I-337) + (3.003), (I-337) + (3.004), (I-337) + (3.005), (I-337) + (3.006), (I-337) + (3.007), (I-337) + (3.008), (I-337) + (3.009), (I-337) + (3.010), (I-337) + (3.011), (I-337) + (3.012), (I-337) + (3.013), (I-337) + (3.014), (I-337) + (3.015), (I-337) + (3.016), (I-337) + (3.017), (I-337) + (3.018), (I-337) + (3.019), (I-337) + (3.020), (I-337) + (3.021), (I-337) + (3.022), (I-337) + (3.023), (I-337) + (3.024), (I-337) + (3.025), (I-337) + (3.026), (I-337) + (3.027), (I-337) + (3.028), (I-337) + (3.029), (I-337) + (3.030), (I-337) + (3.031), (I-337) + (3.032), (I-337) + (4.001), (I-337) + (4.002), (I-337) + (4.003), (I-337) + (4.004), (I-337) + (4.005), (I-337) + (4.006), (I-337) + (4.007), (I-337) + (4.008), (I-337) + (4.009), (I-337) + (4.010), (I-337) + (4.011), (I-337) + (4.012), (I-337) + (4.013), (I-337) + (4.014), (I-337) + (4.015), (I-337) + (4.016), (I-337) + (4.017), (I-337) + (4.018), (I-337) + (4.019), (I-337) + (4.020), (I-337) + (4.021), (I-337) + (4.022), (I-337) + (4.023), (I-337) + (4.024), (I-337) + (4.025), (I-337) + (4.026), (I-337) + (5.001), (I-337) + (5.002), (I-337) + (5.003), (I-337) + (5.004), (I-337) + (5.005), (I-337) + (5.006), (I-337) + (5.007), (I-337) + (5.008), (I-337) + (5.009), (I-337) + (5.010), (I-337) + (5.011), (I-337) + (5.012), (I-337) + (5.013), (I-337) + (5.014), (I-337) + (5.015), (I-337) + (5.016), (I-337) + (5.017), (I-337) + (5.018), (I-337) + (5.019), (I-337) + (5.020), (I-337) + (5.021), (I-337) + (5.022), (I-337) + (5.023), (I-337) + (6.001), (I-337) + (6.002), (I-337) + (6.003), (I-337) + (6.004), (I-337) + (7.001), (I-337) + (7.002), (I-337) + (7.003), (I-337) + (7.004), (I-337) + (7.005), (I-337) + (7.006), (I-337) + (8.001), (I-337) + (9.001), (I-337) + (9.002), (I-337) + (9.003), (I-337) + (9.004), (I-337) + (9.005), (I-337) + (9.006), (I-337) + (9.007), (I-337) + (9.008), (I-337) + (9.009), (I-337) + (10.001), (I-337) + (10.002), (I-337) + (10.003), (I-337) + (11.001), (I-337) + (11.002), (I-337) + (12.001), (I-337) + (12.002), (I-337) + (12.003), (I-337) + (12.004), (I-337) + (13.001), (I-337) + (13.002), (I-337) + (13.003), (I-337) + (13.004), (I-337) + (13.005), (I-337) + (13.006), (I-337) + (14.001), (I-337) + (14.002), (I-337) + (15.001), (I-337) + (15.002), (I-337) + (15.003), (I-337) + (15.004), (I-337) + (15.005), (I-337) + (15.006), (I-337) + (15.007), (I-337) + (15.008), (I-337) + (15.009), (I-337) + (15.010), (I-337) + (15.011), (I-337) + (15.012), (I-337) + (15.013), (I-337) + (15.014), (I-337) + (15.015), (I-337) + (15.016), (I-337) + (15.017), (I-337) + (15.018), (I-337) + (15.019), (I-337) + (15.020), (I-337) + (15.021), (I-337) + (15.022), (I-337) + (15.023), (I-337) + (15.024), (I-337) + (15.025), (I-337) + (15.026), (I-337) + (15.027), (I-337) + (15.028), (I-337) + (15.029), (I-337) + (15.030), (I-337) + (15.031), (I-337) + (15.032), (I-337) + (15.033), (I-337) + (15.034), (I-337) + (15.035), (I-337) + (15.036), (I-337) + (15.037), (I-337) + (15.038), (I-337) + (15.039), (I-337) + (15.040), (I-337) + (15.041), (I-337) + (15.042), (I-337) + (15.043), (I-337) + (15.044), (I-337) + (15.045), (I-337) + (15.046), (I-337) + (15.047), (I-337) + (15.048), (I-337) + (15.049), (I-337) + (15.050), (I-337) + (15.051), (I-337) + (15.052), (I-337) + (15.053), (I-337) + (15.054), (I-337) + (15.055), (I-337) + (15.056), (I-337) + (15.057), (I-337) + (15.058), (I-337) + (15.059), (I-337) + (15.060), (I-337) + (15.061), (I-337) + (15.062), (I-337) + (15.063) , (I-337) + (15.064), (I-337) + (15.065), (I-337) + (15.066), (I-337) + (15.067), (I-337) + (15.068), (I-337) + (15.069), (I-337) + (15.070), (I-337) + (15.071), (I-337) + (15.072), (I-337) + (15.073), (I-337) + (15.074), (I-337) + (15.075), (I-337) + (15.076), (I-337) + (15.077), (I-337) + (15.078), (I-337) + (15.079), (I-337) + (15.080), (I-337) + (15.081), (I-337) + (15.082), (I-337) + (15.083), (I-337) + (15.084), (I-337) + (15.085), (I-337) + (15.086), (I-337) + (15.087), (I-337) + (15.088), (I-337) + (15.089), (I-337) + (15.090), (I-337) + (15.091), (I-337) + (15.092), (I-337) + (15.093), (I-337) + (15.094), (I-337) + (15.095), (I-337) + (15.096), (I-337) + (15.097), (I-337) + (15.098), (I-337) + (15.099), (I-337) + (15.100), (I-337) + (15.101), (I-337) + (15.102), (I-337) + (15.103), (I-337) + (15.104), (I-337) + (15.105), (I-337) + (15.106), (I-337) + (15.107), (I-337) + (15.108), (I-337) + (15.109), (I-337) + (15.110), (I-337) + (15.111), (I-337) + (15.112), (I-337) + (15.113), (I-337) + (15.114), (I-337) + (15.115), (I-337) + (15.116), (I-337) + (15.117), (I-337) + (15.118), (I-337) + (15.119), (I-337) + (15.120), (I-337) + (15.121), (I-337) + (15.122), (I-337) + (15.123), (I-337) + (15.124), (I-337) + (15.125), (I-337) + (15.126), (I-337) + (15.127), (I-337) + (15.128), (I-337) + (16.001), (I-337) + (16.002), (I-337) + (16.003), (I-337) + (16.004), (I-337) + (16.005), (I-337) + (16.006), (I-337) + (16.007), (I-337) + (16.008), (I-337) + (17.001), (I-337) + (17.002), (I-337) + (17.003), (I-337) + (17.004), (I-337) + (17.005), (I-337) + (17.006), (I-337) + (17.007), (I-337) + (17.008), (I-337) + (17.009), (I-337) + (17.010), (I-337) + (17.011), (I-337) + (17.012) 및 (I-337) + (18.001).
또한 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G5)으로부터 선택된다:
(I-337) + (1.001), (I-337) + (1.002), (I-337) + (1.003), (I-337) + (1.004), (I-337) + (1.005), (I-337) + (1.006), (I-337) + (1.007), (I-337) + (1.008), (I-337) + (1.009), (I-337) + (1.010), (I-337) + (1.011), (I-337) + (1.012), (I-337) + (1.013), (I-337) + (1.014), (I-337) + (1.015), (I-337) + (1.016), (I-337) + (1.017), (I-337) + (1.018), (I-337) + (1.019), (I-337) + (1.020), (I-337) + (1.021), (I-337) + (1.022), (I-337) + (1.023), (I-337) + (1.024), (I-337) + (1.025), (I-337) + (1.026), (I-337) + (1.027), (I-337) + (1.028), (I-337) + (1.029), (I-337) + (1.030), (I-337) + (1.031), (I-337) + (1.032), (I-337) + (1.033), (I-337) + (1.034), (I-337) + (1.035), (I-337) + (1.036), (I-337) + (1.037), (I-337) + (1.038), (I-337) + (1.039), (I-337) + (1.040), (I-337) + (1.041), (I-337) + (1.042), (I-337) + (1.043), (I-337) + (1.044), (I-337) + (1.045), (I-337) + (1.046), (I-337) + (1.047), (I-337) + (1.048), (I-337) + (1.049), (I-337) + (1.050), (I-337) + (1.051), (I-337) + (1.052), (I-337) + (1.053), (I-337) + (1.054), (I-337) + (1.055), (I-337) + (1.056), (I-337) + (1.057), (I-337) + (1.058), (I-337) + (1.059), (I-337) + (1.060), (I-337) + (1.061), (I-337) + (1.062), (I-337) + (1.063), (I-337) + (1.064), (I-337) + (1.065), (I-337) + (1.066), (I-337) + (1.067), (I-337) + (1.068), (I-337) + (1.069), (I-337) + (1.070), (I-337) + (1.071), (I-337) + (1.072), (I-337) + (1.073), (I-337) + (1.074), (I-337) + (1.075), (I-337) + (1.076), (I-337) + (1.077), (I-337) + (1.078), (I-337) + (1.079), (I-337) + (1.080), (I-337) + (1.081), (I-337) + (1.082), (I-337) + (1.083), (I-337) + (1.084), (I-337) + (1.085), (I-337) + (1.086), (I-337) + (1.087), (I-337) + (1.088), (I-337) + (1.089), (I-337) + (1.090), (I-337) + (1.091), (I-337) + (1.092), (I-337) + (2.001), (I-337) + (2.002), (I-337) + (2.003), (I-337) + (2.004), (I-337) + (2.005), (I-337) + (2.006), (I-337) + (2.007), (I-337) + (2.008), (I-337) + (2.009), (I-337) + (2.010), (I-337) + (2.011), (I-337) + (2.012), (I-337) + (2.013), (I-337) + (2.014), (I-337) + (2.015), (I-337) + (2.016), (I-337) + (2.017), (I-337) + (2.018), (I-337) + (2.019), (I-337) + (2.020), (I-337) + (2.021), (I-337) + (2.022), (I-337) + (2.023), (I-337) + (2.024), (I-337) + (2.025), (I-337) + (2.026), (I-337) + (2.027), (I-337) + (2.028), (I-337) + (2.029), (I-337) + (2.030), (I-337) + (2.031), (I-337) + (2.032), (I-337) + (2.033), (I-337) + (2.034), (I-337) + (2.035), (I-337) + (2.036), (I-337) + (2.037), (I-337) + (2.038), (I-337) + (2.039), (I-337) + (2.040), (I-337) + (2.041), (I-337) + (2.042), (I-337) + (2.043), (I-337) + (2.044), (I-337) + (2.045), (I-337) + (2.046), (I-337) + (2.047), (I-337) + (2.048), (I-337) + (2.049), (I-337) + (2.050), (I-337) + (2.051), (I-337) + (2.052), (I-337) + (2.053), (I-337) + (2.054), (I-337) + (2.055), (I-337) + (2.056), (I-337) + (2.057), (I-337) + (2.058), (I-337) + (2.059), (I-337) + (3.001), (I-337) + (3.002), (I-337) + (3.003), (I-337) + (3.004), (I-337) + (3.005), (I-337) + (3.006), (I-337) + (3.007), (I-337) + (3.008), (I-337) + (3.009), (I-337) + (3.010), (I-337) + (3.011), (I-337) + (3.012), (I-337) + (3.013), (I-337) + (3.014), (I-337) + (3.015), (I-337) + (3.016), (I-337) + (3.017), (I-337) + (3.018), (I-337) + (3.019), (I-337) + (3.020), (I-337) + (3.021), (I-337) + (3.022), (I-337) + (3.023), (I-337) + (3.024), (I-337) + (3.025), (I-337) + (3.026), (I-337) + (3.027), (I-337) + (3.028), (I-337) + (3.029), (I-337) + (3.030), (I-337) + (3.031), (I-337) + (4.001), (I-337) + (4.002), (I-337) + (4.003), (I-337) + (4.004), (I-337) + (4.005), (I-337) + (4.006), (I-337) + (4.007), (I-337) + (4.008), (I-337) + (4.009), (I-337) + (4.010), (I-337) + (4.011), (I-337) + (4.012), (I-337) + (4.013), (I-337) + (4.014), (I-337) + (4.015), (I-337) + (4.016), (I-337) + (4.017), (I-337) + (4.018), (I-337) + (4.019), (I-337) + (4.020), (I-337) + (4.021), (I-337) + (4.022), (I-337) + (4.023), (I-337) + (4.024), (I-337) + (4.025), (I-337) + (4.026), (I-337) + (5.001), (I-337) + (5.002), (I-337) + (5.003), (I-337) + (5.004), (I-337) + (5.005), (I-337) + (5.006), (I-337) + (5.007), (I-337) + (5.008), (I-337) + (5.009), (I-337) + (5.010), (I-337) + (5.011), (I-337) + (5.012), (I-337) + (5.013), (I-337) + (5.014), (I-337) + (5.015), (I-337) + (5.016), (I-337) + (5.017), (I-337) + (5.018), (I-337) + (5.019), (I-337) + (5.020), (I-337) + (5.021), (I-337) + (5.022), (I-337) + (5.023), (I-337) + (6.001), (I-337) + (6.002), (I-337) + (6.003), (I-337) + (6.004), (I-337) + (7.001), (I-337) + (7.002), (I-337) + (7.003), (I-337) + (7.004), (I-337) + (7.005), (I-337) + (7.006), (I-337) + (8.001), (I-337) + (9.001), (I-337) + (9.002), (I-337) + (9.003), (I-337) + (9.004), (I-337) + (9.005), (I-337) + (9.006), (I-337) + (9.007), (I-337) + (9.008), (I-337) + (9.009), (I-337) + (10.001), (I-337) + (10.002), (I-337) + (10.003), (I-337) + (11.001), (I-337) + (11.002), (I-337) + (12.001), (I-337) + (12.002), (I-337) + (12.003), (I-337) + (12.004), (I-337) + (13.001), (I-337) + (13.002), (I-337) + (13.003), (I-337) + (13.004), (I-337) + (13.005), (I-337) + (13.006), (I-337) + (14.001), (I-337) + (14.002), (I-337) + (15.001), (I-337) + (15.002), (I-337) + (15.003), (I-337) + (15.004), (I-337) + (15.005), (I-337) + (15.006), (I-337) + (15.007), (I-337) + (15.008), (I-337) + (15.009), (I-337) + (15.010), (I-337) + (15.011), (I-337) + (15.012), (I-337) + (15.013), (I-337) + (15.014), (I-337) + (15.015), (I-337) + (15.016), (I-337) + (15.017), (I-337) + (15.018), (I-337) + (15.019), (I-337) + (15.020), (I-337) + (15.021), (I-337) + (15.022), (I-337) + (15.023), (I-337) + (15.024), (I-337) + (15.025), (I-337) + (15.026), (I-337) + (15.027), (I-337) + (15.028), (I-337) + (15.029), (I-337) + (15.030), (I-337) + (15.031), (I-337) + (15.032), (I-337) + (15.033), (I-337) + (15.034), (I-337) + (15.035), (I-337) + (15.036), (I-337) + (15.037), (I-337) + (15.038), (I-337) + (15.039), (I-337) + (15.040), (I-337) + (15.041), (I-337) + (15.042), (I-337) + (15.043), (I-337) + (15.044), (I-337) + (15.045), (I-337) + (15.046), (I-337) + (15.047), (I-337) + (15.048), (I-337) + (15.049), (I-337) + (15.050), (I-337) + (15.051), (I-337) + (15.052), (I-337) + (15.053), (I-337) + (15.054), (I-337) + (15.055), (I-337) + (15.056), (I-337) + (15.057), (I-337) + (15.058), (I-337) + (15.059), (I-337) + (15.060), (I-337) + (15.061), (I-337) + (15.062), (I-337) + (15.063) , (I-337) + (15.064), (I-337) + (15.065), (I-337) + (15.066), (I-337) + (15.067), (I-337) + (15.068), (I-337) + (15.069), (I-337) + (15.070), (I-337) + (15.071), (I-337) + (15.072), (I-337) + (15.073), (I-337) + (15.074), (I-337) + (15.075), (I-337) + (15.076), (I-337) + (15.077), (I-337) + (15.078), (I-337) + (15.079), (I-337) + (15.080), (I-337) + (15.081), (I-337) + (15.082), (I-337) + (15.083), (I-337) + (15.084), (I-337) + (15.085), (I-337) + (15.086), (I-337) + (15.087), (I-337) + (15.088), (I-337) + (15.089), (I-337) + (15.090), (I-337) + (15.091), (I-337) + (15.092), (I-337) + (15.093), (I-337) + (15.094), (I-337) + (15.095), (I-337) + (15.096), (I-337) + (15.097), (I-337) + (15.098), (I-337) + (15.099), (I-337) + (15.100), (I-337) + (15.101), (I-337) + (15.102), (I-337) + (15.103), (I-337) + (15.104), (I-337) + (15.105), (I-337) + (15.106), (I-337) + (15.107), (I-337) + (15.108), (I-337) + (15.109), (I-337) + (15.110), (I-337) + (15.111), (I-337) + (15.112), (I-337) + (15.113), (I-337) + (15.114), (I-337) + (15.115), (I-337) + (15.116), (I-337) + (15.117), (I-337) + (15.118), (I-337) + (15.119), (I-337) + (15.120), (I-337) + (15.121), (I-337) + (15.122), (I-337) + (15.123), (I-337) + (15.124), (I-337) + (15.125), (I-337) + (15.126), (I-337) + (15.127), (I-337) + (16.001), (I-337) + (16.002), (I-337) + (16.003), (I-337) + (16.004), (I-337) + (16.005), (I-337) + (16.006), (I-337) + (16.007), (I-337) + (16.008), (I-337) + (17.001), (I-337) + (17.002), (I-337) + (17.003), (I-337) + (17.004), (I-337) + (17.005), (I-337) + (17.006), (I-337) + (17.007), (I-337) + (17.008), (I-337) + (17.009), (I-337) + (17.010), (I-337) + (17.011), (I-337) + (17.012) 및 (I-337) + (18.001).
또한 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G7-1)으로부터 선택된다:
(I-338) + (1.001), (I-338) + (1.002), (I-338) + (1.003), (I-338) + (1.004), (I-338) + (1.005), (I-338) + (1.006), (I-338) + (1.007), (I-338) + (1.008), (I-338) + (1.009), (I-338) + (1.010), (I-338) + (1.011), (I-338) + (1.012), (I-338) + (1.013), (I-338) + (1.014), (I-338) + (1.015), (I-338) + (1.016), (I-338) + (1.017), (I-338) + (1.018), (I-338) + (1.019), (I-338) + (1.020), (I-338) + (1.021), (I-338) + (1.022), (I-338) + (1.023), (I-338) + (1.024), (I-338) + (1.025), (I-338) + (1.026), (I-338) + (1.027), (I-338) + (1.028), (I-338) + (1.029), (I-338) + (1.030), (I-338) + (1.031), (I-338) + (1.032), (I-338) + (1.033), (I-338) + (1.034), (I-338) + (1.035), (I-338) + (1.036), (I-338) + (1.037), (I-338) + (1.038), (I-338) + (1.039), (I-338) + (1.040), (I-338) + (1.041), (I-338) + (1.042), (I-338) + (1.043), (I-338) + (1.044), (I-338) + (1.045), (I-338) + (1.046), (I-338) + (1.047), (I-338) + (1.048), (I-338) + (1.049), (I-338) + (1.050), (I-338) + (1.051), (I-338) + (1.052), (I-338) + (1.053), (I-338) + (1.054), (I-338) + (1.055), (I-338) + (1.056), (I-338) + (1.057), (I-338) + (1.058), (I-338) + (1.059), (I-338) + (1.060), (I-338) + (1.061), (I-338) + (1.062), (I-338) + (1.063), (I-338) + (1.064), (I-338) + (1.065), (I-338) + (1.066), (I-338) + (1.067), (I-338) + (1.068), (I-338) + (1.069), (I-338) + (1.070), (I-338) + (1.071), (I-338) + (1.072), (I-338) + (1.073), (I-338) + (1.074), (I-338) + (1.075), (I-338) + (1.076), (I-338) + (1.077), (I-338) + (1.078), (I-338) + (1.079), (I-338) + (1.080), (I-338) + (1.081), (I-338) + (1.082), (I-338) + (1.083), (I-338) + (1.084), (I-338) + (1.085), (I-338) + (1.086), (I-338) + (1.087), (I-338) + (1.088), (I-338) + (1.089), (I-338) + (1.090), (I-338) + (1.091), (I-338) + (1.092), (I-338) + (2.001), (I-338) + (2.002), (I-338) + (2.003), (I-338) + (2.004), (I-338) + (2.005), (I-338) + (2.006), (I-338) + (2.007), (I-338) + (2.008), (I-338) + (2.009), (I-338) + (2.010), (I-338) + (2.011), (I-338) + (2.012), (I-338) + (2.013), (I-338) + (2.014), (I-338) + (2.015), (I-338) + (2.016), (I-338) + (2.017), (I-338) + (2.018), (I-338) + (2.019), (I-338) + (2.020), (I-338) + (2.021), (I-338) + (2.022), (I-338) + (2.023), (I-338) + (2.024), (I-338) + (2.025), (I-338) + (2.026), (I-338) + (2.027), (I-338) + (2.028), (I-338) + (2.029), (I-338) + (2.030), (I-338) + (2.031), (I-338) + (2.032), (I-338) + (2.033), (I-338) + (2.034), (I-338) + (2.035), (I-338) + (2.036), (I-338) + (2.037), (I-338) + (2.038), (I-338) + (2.039), (I-338) + (2.040), (I-338) + (2.041), (I-338) + (2.042), (I-338) + (2.043), (I-338) + (2.044), (I-338) + (2.045), (I-338) + (2.046), (I-338) + (2.047), (I-338) + (2.048), (I-338) + (2.049), (I-338) + (2.050), (I-338) + (2.051), (I-338) + (2.052), (I-338) + (2.053), (I-338) + (2.054), (I-338) + (2.055), (I-338) + (2.056), (I-338) + (2.057), (I-338) + (2.058), (I-338) + (2.059), (I-338) + (2.060), (I-338) + (3.001), (I-338) + (3.002), (I-338) + (3.003), (I-338) + (3.004), (I-338) + (3.005), (I-338) + (3.006), (I-338) + (3.007), (I-338) + (3.008), (I-338) + (3.009), (I-338) + (3.010), (I-338) + (3.011), (I-338) + (3.012), (I-338) + (3.013), (I-338) + (3.014), (I-338) + (3.015), (I-338) + (3.016), (I-338) + (3.017), (I-338) + (3.018), (I-338) + (3.019), (I-338) + (3.020), (I-338) + (3.021), (I-338) + (3.022), (I-338) + (3.023), (I-338) + (3.024), (I-338) + (3.025), (I-338) + (3.026), (I-338) + (3.027), (I-338) + (3.028), (I-338) + (3.029), (I-338) + (3.030), (I-338) + (3.031), (I-338) + (3.032), (I-338) + (4.001), (I-338) + (4.002), (I-338) + (4.003), (I-338) + (4.004), (I-338) + (4.005), (I-338) + (4.006), (I-338) + (4.007), (I-338) + (4.008), (I-338) + (4.009), (I-338) + (4.010), (I-338) + (4.011), (I-338) + (4.012), (I-338) + (4.013), (I-338) + (4.014), (I-338) + (4.015), (I-338) + (4.016), (I-338) + (4.017), (I-338) + (4.018), (I-338) + (4.019), (I-338) + (4.020), (I-338) + (4.021), (I-338) + (4.022), (I-338) + (4.023), (I-338) + (4.024), (I-338) + (4.025), (I-338) + (4.026), (I-338) + (5.001), (I-338) + (5.002), (I-338) + (5.003), (I-338) + (5.004), (I-338) + (5.005), (I-338) + (5.006), (I-338) + (5.007), (I-338) + (5.008), (I-338) + (5.009), (I-338) + (5.010), (I-338) + (5.011), (I-338) + (5.012), (I-338) + (5.013), (I-338) + (5.014), (I-338) + (5.015), (I-338) + (5.016), (I-338) + (5.017), (I-338) + (5.018), (I-338) + (5.019), (I-338) + (5.020), (I-338) + (5.021), (I-338) + (5.022), (I-338) + (5.023), (I-338) + (6.001), (I-338) + (6.002), (I-338) + (6.003), (I-338) + (6.004), (I-338) + (7.001), (I-338) + (7.002), (I-338) + (7.003), (I-338) + (7.004), (I-338) + (7.005), (I-338) + (7.006), (I-338) + (8.001), (I-338) + (9.001), (I-338) + (9.002), (I-338) + (9.003), (I-338) + (9.004), (I-338) + (9.005), (I-338) + (9.006), (I-338) + (9.007), (I-338) + (9.008), (I-338) + (9.009), (I-338) + (10.001), (I-338) + (10.002), (I-338) + (10.003), (I-338) + (11.001), (I-338) + (11.002), (I-338) + (12.001), (I-338) + (12.002), (I-338) + (12.003), (I-338) + (12.004), (I-338) + (13.001), (I-338) + (13.002), (I-338) + (13.003), (I-338) + (13.004), (I-338) + (13.005), (I-338) + (13.006), (I-338) + (14.001), (I-338) + (14.002), (I-338) + (15.001), (I-338) + (15.002), (I-338) + (15.003), (I-338) + (15.004), (I-338) + (15.005), (I-338) + (15.006), (I-338) + (15.007), (I-338) + (15.008), (I-338) + (15.009), (I-338) + (15.010), (I-338) + (15.011), (I-338) + (15.012), (I-338) + (15.013), (I-338) + (15.014), (I-338) + (15.015), (I-338) + (15.016), (I-338) + (15.017), (I-338) + (15.018), (I-338) + (15.019), (I-338) + (15.020), (I-338) + (15.021), (I-338) + (15.022), (I-338) + (15.023), (I-338) + (15.024), (I-338) + (15.025), (I-338) + (15.026), (I-338) + (15.027), (I-338) + (15.028), (I-338) + (15.029), (I-338) + (15.030), (I-338) + (15.031), (I-338) + (15.032), (I-338) + (15.033), (I-338) + (15.034), (I-338) + (15.035), (I-338) + (15.036), (I-338) + (15.037), (I-338) + (15.038), (I-338) + (15.039), (I-338) + (15.040), (I-338) + (15.041), (I-338) + (15.042), (I-338) + (15.043), (I-338) + (15.044), (I-338) + (15.045), (I-338) + (15.046), (I-338) + (15.047), (I-338) + (15.048), (I-338) + (15.049), (I-338) + (15.050), (I-338) + (15.051), (I-338) + (15.052), (I-338) + (15.053), (I-338) + (15.054), (I-338) + (15.055), (I-338) + (15.056), (I-338) + (15.057), (I-338) + (15.058), (I-338) + (15.059), (I-338) + (15.060), (I-338) + (15.061), (I-338) + (15.062), (I-338) + (15.063) , (I-338) + (15.064), (I-338) + (15.065), (I-338) + (15.066), (I-338) + (15.067), (I-338) + (15.068), (I-338) + (15.069), (I-338) + (15.070), (I-338) + (15.071), (I-338) + (15.072), (I-338) + (15.073), (I-338) + (15.074), (I-338) + (15.075), (I-338) + (15.076), (I-338) + (15.077), (I-338) + (15.078), (I-338) + (15.079), (I-338) + (15.080), (I-338) + (15.081), (I-338) + (15.082), (I-338) + (15.083), (I-338) + (15.084), (I-338) + (15.085), (I-338) + (15.086), (I-338) + (15.087), (I-338) + (15.088), (I-338) + (15.089), (I-338) + (15.090), (I-338) + (15.091), (I-338) + (15.092), (I-338) + (15.093), (I-338) + (15.094), (I-338) + (15.095), (I-338) + (15.096), (I-338) + (15.097), (I-338) + (15.098), (I-338) + (15.099), (I-338) + (15.100), (I-338) + (15.101), (I-338) + (15.102), (I-338) + (15.103), (I-338) + (15.104), (I-338) + (15.105), (I-338) + (15.106), (I-338) + (15.107), (I-338) + (15.108), (I-338) + (15.109), (I-338) + (15.110), (I-338) + (15.111), (I-338) + (15.112), (I-338) + (15.113), (I-338) + (15.114), (I-338) + (15.115), (I-338) + (15.116), (I-338) + (15.117), (I-338) + (15.118), (I-338) + (15.119), (I-338) + (15.120), (I-338) + (15.121), (I-338) + (15.122), (I-338) + (15.123), (I-338) + (15.124), (I-338) + (15.125), (I-338) + (15.126), (I-338) + (15.127), (I-338) + (15.128), (I-338) + (16.001), (I-338) + (16.002), (I-338) + (16.003), (I-338) + (16.004), (I-338) + (16.005), (I-338) + (16.006), (I-338) + (16.007), (I-338) + (16.008), (I-338) + (17.001), (I-338) + (17.002), (I-338) + (17.003), (I-338) + (17.004), (I-338) + (17.005), (I-338) + (17.006), (I-338) + (17.007), (I-338) + (17.008), (I-338) + (17.009), (I-338) + (17.010), (I-338) + (17.011), (I-338) + (17.012) 및 (I-338) + (18.001).
또한 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G6-1)으로부터 선택된다:
(I-339) + (1.001), (I-339) + (1.002), (I-339) + (1.003), (I-339) + (1.004), (I-339) + (1.005), (I-339) + (1.006), (I-339) + (1.007), (I-339) + (1.008), (I-339) + (1.009), (I-339) + (1.010), (I-339) + (1.011), (I-339) + (1.012), (I-339) + (1.013), (I-339) + (1.014), (I-339) + (1.015), (I-339) + (1.016), (I-339) + (1.017), (I-339) + (1.018), (I-339) + (1.019), (I-339) + (1.020), (I-339) + (1.021), (I-339) + (1.022), (I-339) + (1.023), (I-339) + (1.024), (I-339) + (1.025), (I-339) + (1.026), (I-339) + (1.027), (I-339) + (1.028), (I-339) + (1.029), (I-339) + (1.030), (I-339) + (1.031), (I-339) + (1.032), (I-339) + (1.033), (I-339) + (1.034), (I-339) + (1.035), (I-339) + (1.036), (I-339) + (1.037), (I-339) + (1.038), (I-339) + (1.039), (I-339) + (1.040), (I-339) + (1.041), (I-339) + (1.042), (I-339) + (1.043), (I-339) + (1.044), (I-339) + (1.045), (I-339) + (1.046), (I-339) + (1.047), (I-339) + (1.048), (I-339) + (1.049), (I-339) + (1.050), (I-339) + (1.051), (I-339) + (1.052), (I-339) + (1.053), (I-339) + (1.054), (I-339) + (1.055), (I-339) + (1.056), (I-339) + (1.057), (I-339) + (1.058), (I-339) + (1.059), (I-339) + (1.060), (I-339) + (1.061), (I-339) + (1.062), (I-339) + (1.063), (I-339) + (1.064), (I-339) + (1.065), (I-339) + (1.066), (I-339) + (1.067), (I-339) + (1.068), (I-339) + (1.069), (I-339) + (1.070), (I-339) + (1.071), (I-339) + (1.072), (I-339) + (1.073), (I-339) + (1.074), (I-339) + (1.075), (I-339) + (1.076), (I-339) + (1.077), (I-339) + (1.078), (I-339) + (1.079), (I-339) + (1.080), (I-339) + (1.081), (I-339) + (1.082), (I-339) + (1.083), (I-339) + (1.084), (I-339) + (1.085), (I-339) + (1.086), (I-339) + (1.087), (I-339) + (1.088), (I-339) + (1.089), (I-339) + (1.090), (I-339) + (1.091), (I-339) + (1.092), (I-339) + (2.001), (I-339) + (2.002), (I-339) + (2.003), (I-339) + (2.004), (I-339) + (2.005), (I-339) + (2.006), (I-339) + (2.007), (I-339) + (2.008), (I-339) + (2.009), (I-339) + (2.010), (I-339) + (2.011), (I-339) + (2.012), (I-339) + (2.013), (I-339) + (2.014), (I-339) + (2.015), (I-339) + (2.016), (I-339) + (2.017), (I-339) + (2.018), (I-339) + (2.019), (I-339) + (2.020), (I-339) + (2.021), (I-339) + (2.022), (I-339) + (2.023), (I-339) + (2.024), (I-339) + (2.025), (I-339) + (2.026), (I-339) + (2.027), (I-339) + (2.028), (I-339) + (2.029), (I-339) + (2.030), (I-339) + (2.031), (I-339) + (2.032), (I-339) + (2.033), (I-339) + (2.034), (I-339) + (2.035), (I-339) + (2.036), (I-339) + (2.037), (I-339) + (2.038), (I-339) + (2.039), (I-339) + (2.040), (I-339) + (2.041), (I-339) + (2.042), (I-339) + (2.043), (I-339) + (2.044), (I-339) + (2.045), (I-339) + (2.046), (I-339) + (2.047), (I-339) + (2.048), (I-339) + (2.049), (I-339) + (2.050), (I-339) + (2.051), (I-339) + (2.052), (I-339) + (2.053), (I-339) + (2.054), (I-339) + (2.055), (I-339) + (2.056), (I-339) + (2.057), (I-339) + (2.058), (I-339) + (2.059), (I-339) + (2.060), (I-339) + (3.001), (I-339) + (3.002), (I-339) + (3.003), (I-339) + (3.004), (I-339) + (3.005), (I-339) + (3.006), (I-339) + (3.007), (I-339) + (3.008), (I-339) + (3.009), (I-339) + (3.010), (I-339) + (3.011), (I-339) + (3.012), (I-339) + (3.013), (I-339) + (3.014), (I-339) + (3.015), (I-339) + (3.016), (I-339) + (3.017), (I-339) + (3.018), (I-339) + (3.019), (I-339) + (3.020), (I-339) + (3.021), (I-339) + (3.022), (I-339) + (3.023), (I-339) + (3.024), (I-339) + (3.025), (I-339) + (3.026), (I-339) + (3.027), (I-339) + (3.028), (I-339) + (3.029), (I-339) + (3.030), (I-339) + (3.031), (I-339) + (3.032), (I-339) + (4.001), (I-339) + (4.002), (I-339) + (4.003), (I-339) + (4.004), (I-339) + (4.005), (I-339) + (4.006), (I-339) + (4.007), (I-339) + (4.008), (I-339) + (4.009), (I-339) + (4.010), (I-339) + (4.011), (I-339) + (4.012), (I-339) + (4.013), (I-339) + (4.014), (I-339) + (4.015), (I-339) + (4.016), (I-339) + (4.017), (I-339) + (4.018), (I-339) + (4.019), (I-339) + (4.020), (I-339) + (4.021), (I-339) + (4.022), (I-339) + (4.023), (I-339) + (4.024), (I-339) + (4.025), (I-339) + (4.026), (I-339) + (5.001), (I-339) + (5.002), (I-339) + (5.003), (I-339) + (5.004), (I-339) + (5.005), (I-339) + (5.006), (I-339) + (5.007), (I-339) + (5.008), (I-339) + (5.009), (I-339) + (5.010), (I-339) + (5.011), (I-339) + (5.012), (I-339) + (5.013), (I-339) + (5.014), (I-339) + (5.015), (I-339) + (5.016), (I-339) + (5.017), (I-339) + (5.018), (I-339) + (5.019), (I-339) + (5.020), (I-339) + (5.021), (I-339) + (5.022), (I-339) + (5.023), (I-339) + (6.001), (I-339) + (6.002), (I-339) + (6.003), (I-339) + (6.004), (I-339) + (7.001), (I-339) + (7.002), (I-339) + (7.003), (I-339) + (7.004), (I-339) + (7.005), (I-339) + (7.006), (I-339) + (8.001), (I-339) + (9.001), (I-339) + (9.002), (I-339) + (9.003), (I-339) + (9.004), (I-339) + (9.005), (I-339) + (9.006), (I-339) + (9.007), (I-339) + (9.008), (I-339) + (9.009), (I-339) + (10.001), (I-339) + (10.002), (I-339) + (10.003), (I-339) + (11.001), (I-339) + (11.002), (I-339) + (12.001), (I-339) + (12.002), (I-339) + (12.003), (I-339) + (12.004), (I-339) + (13.001), (I-339) + (13.002), (I-339) + (13.003), (I-339) + (13.004), (I-339) + (13.005), (I-339) + (13.006), (I-339) + (14.001), (I-339) + (14.002), (I-339) + (15.001), (I-339) + (15.002), (I-339) + (15.003), (I-339) + (15.004), (I-339) + (15.005), (I-339) + (15.006), (I-339) + (15.007), (I-339) + (15.008), (I-339) + (15.009), (I-339) + (15.010), (I-339) + (15.011), (I-339) + (15.012), (I-339) + (15.013), (I-339) + (15.014), (I-339) + (15.015), (I-339) + (15.016), (I-339) + (15.017), (I-339) + (15.018), (I-339) + (15.019), (I-339) + (15.020), (I-339) + (15.021), (I-339) + (15.022), (I-339) + (15.023), (I-339) + (15.024), (I-339) + (15.025), (I-339) + (15.026), (I-339) + (15.027), (I-339) + (15.028), (I-339) + (15.029), (I-339) + (15.030), (I-339) + (15.031), (I-339) + (15.032), (I-339) + (15.033), (I-339) + (15.034), (I-339) + (15.035), (I-339) + (15.036), (I-339) + (15.037), (I-339) + (15.038), (I-339) + (15.039), (I-339) + (15.040), (I-339) + (15.041), (I-339) + (15.042), (I-339) + (15.043), (I-339) + (15.044), (I-339) + (15.045), (I-339) + (15.046), (I-339) + (15.047), (I-339) + (15.048), (I-339) + (15.049), (I-339) + (15.050), (I-339) + (15.051), (I-339) + (15.052), (I-339) + (15.053), (I-339) + (15.054), (I-339) + (15.055), (I-339) + (15.056), (I-339) + (15.057), (I-339) + (15.058), (I-339) + (15.059), (I-339) + (15.060), (I-339) + (15.061), (I-339) + (15.062), (I-339) + (15.063) , (I-339) + (15.064), (I-339) + (15.065), (I-339) + (15.066), (I-339) + (15.067), (I-339) + (15.068), (I-339) + (15.069), (I-339) + (15.070), (I-339) + (15.071), (I-339) + (15.072), (I-339) + (15.073), (I-339) + (15.074), (I-339) + (15.075), (I-339) + (15.076), (I-339) + (15.077), (I-339) + (15.078), (I-339) + (15.079), (I-339) + (15.080), (I-339) + (15.081), (I-339) + (15.082), (I-339) + (15.083), (I-339) + (15.084), (I-339) + (15.085), (I-339) + (15.086), (I-339) + (15.087), (I-339) + (15.088), (I-339) + (15.089), (I-339) + (15.090), (I-339) + (15.091), (I-339) + (15.092), (I-339) + (15.093), (I-339) + (15.094), (I-339) + (15.095), (I-339) + (15.096), (I-339) + (15.097), (I-339) + (15.098), (I-339) + (15.099), (I-339) + (15.100), (I-339) + (15.101), (I-339) + (15.102), (I-339) + (15.103), (I-339) + (15.104), (I-339) + (15.105), (I-339) + (15.106), (I-339) + (15.107), (I-339) + (15.108), (I-339) + (15.109), (I-339) + (15.110), (I-339) + (15.111), (I-339) + (15.112), (I-339) + (15.113), (I-339) + (15.114), (I-339) + (15.115), (I-339) + (15.116), (I-339) + (15.117), (I-339) + (15.118), (I-339) + (15.119), (I-339) + (15.120), (I-339) + (15.121), (I-339) + (15.122), (I-339) + (15.123), (I-339) + (15.124), (I-339) + (15.125), (I-339) + (15.126), (I-339) + (15.127), (I-339) + (15.128), (I-339) + (16.001), (I-339) + (16.002), (I-339) + (16.003), (I-339) + (16.004), (I-339) + (16.005), (I-339) + (16.006), (I-339) + (16.007), (I-339) + (16.008), (I-339) + (17.001), (I-339) + (17.002), (I-339) + (17.003), (I-339) + (17.004), (I-339) + (17.005), (I-339) + (17.006), (I-339) + (17.007), (I-339) + (17.008), (I-339) + (17.009), (I-339) + (17.010), (I-339) + (17.011), (I-339) + (17.012) 및 (I-339) + (18.001).
또한 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G6)으로부터 선택된다:
(I-339) + (1.001), (I-339) + (1.002), (I-339) + (1.003), (I-339) + (1.004), (I-339) + (1.005), (I-339) + (1.006), (I-339) + (1.007), (I-339) + (1.008), (I-339) + (1.009), (I-339) + (1.010), (I-339) + (1.011), (I-339) + (1.012), (I-339) + (1.013), (I-339) + (1.014), (I-339) + (1.015), (I-339) + (1.016), (I-339) + (1.017), (I-339) + (1.018), (I-339) + (1.019), (I-339) + (1.020), (I-339) + (1.021), (I-339) + (1.022), (I-339) + (1.023), (I-339) + (1.024), (I-339) + (1.025), (I-339) + (1.026), (I-339) + (1.027), (I-339) + (1.028), (I-339) + (1.029), (I-339) + (1.030), (I-339) + (1.031), (I-339) + (1.032), (I-339) + (1.033), (I-339) + (1.034), (I-339) + (1.035), (I-339) + (1.036), (I-339) + (1.037), (I-339) + (1.038), (I-339) + (1.039), (I-339) + (1.040), (I-339) + (1.041), (I-339) + (1.042), (I-339) + (1.043), (I-339) + (1.044), (I-339) + (1.045), (I-339) + (1.046), (I-339) + (1.047), (I-339) + (1.048), (I-339) + (1.049), (I-339) + (1.050), (I-339) + (1.051), (I-339) + (1.052), (I-339) + (1.053), (I-339) + (1.054), (I-339) + (1.055), (I-339) + (1.056), (I-339) + (1.057), (I-339) + (1.058), (I-339) + (1.059), (I-339) + (1.060), (I-339) + (1.061), (I-339) + (1.062), (I-339) + (1.063), (I-339) + (1.064), (I-339) + (1.065), (I-339) + (1.066), (I-339) + (1.067), (I-339) + (1.068), (I-339) + (1.069), (I-339) + (1.070), (I-339) + (1.071), (I-339) + (1.072), (I-339) + (1.073), (I-339) + (1.074), (I-339) + (1.075), (I-339) + (1.076), (I-339) + (1.077), (I-339) + (1.078), (I-339) + (1.079), (I-339) + (1.080), (I-339) + (1.081), (I-339) + (1.082), (I-339) + (1.083), (I-339) + (1.084), (I-339) + (1.085), (I-339) + (1.086), (I-339) + (1.087), (I-339) + (1.088), (I-339) + (1.089), (I-339) + (1.090), (I-339) + (1.091), (I-339) + (1.092), (I-339) + (2.001), (I-339) + (2.002), (I-339) + (2.003), (I-339) + (2.004), (I-339) + (2.005), (I-339) + (2.006), (I-339) + (2.007), (I-339) + (2.008), (I-339) + (2.009), (I-339) + (2.010), (I-339) + (2.011), (I-339) + (2.012), (I-339) + (2.013), (I-339) + (2.014), (I-339) + (2.015), (I-339) + (2.016), (I-339) + (2.017), (I-339) + (2.018), (I-339) + (2.019), (I-339) + (2.020), (I-339) + (2.021), (I-339) + (2.022), (I-339) + (2.023), (I-339) + (2.024), (I-339) + (2.025), (I-339) + (2.026), (I-339) + (2.027), (I-339) + (2.028), (I-339) + (2.029), (I-339) + (2.030), (I-339) + (2.031), (I-339) + (2.032), (I-339) + (2.033), (I-339) + (2.034), (I-339) + (2.035), (I-339) + (2.036), (I-339) + (2.037), (I-339) + (2.038), (I-339) + (2.039), (I-339) + (2.040), (I-339) + (2.041), (I-339) + (2.042), (I-339) + (2.043), (I-339) + (2.044), (I-339) + (2.045), (I-339) + (2.046), (I-339) + (2.047), (I-339) + (2.048), (I-339) + (2.049), (I-339) + (2.050), (I-339) + (2.051), (I-339) + (2.052), (I-339) + (2.053), (I-339) + (2.054), (I-339) + (2.055), (I-339) + (2.056), (I-339) + (2.057), (I-339) + (2.058), (I-339) + (2.059), (I-339) + (3.001), (I-339) + (3.002), (I-339) + (3.003), (I-339) + (3.004), (I-339) + (3.005), (I-339) + (3.006), (I-339) + (3.007), (I-339) + (3.008), (I-339) + (3.009), (I-339) + (3.010), (I-339) + (3.011), (I-339) + (3.012), (I-339) + (3.013), (I-339) + (3.014), (I-339) + (3.015), (I-339) + (3.016), (I-339) + (3.017), (I-339) + (3.018), (I-339) + (3.019), (I-339) + (3.020), (I-339) + (3.021), (I-339) + (3.022), (I-339) + (3.023), (I-339) + (3.024), (I-339) + (3.025), (I-339) + (3.026), (I-339) + (3.027), (I-339) + (3.028), (I-339) + (3.029), (I-339) + (3.030), (I-339) + (3.031), (I-339) + (4.001), (I-339) + (4.002), (I-339) + (4.003), (I-339) + (4.004), (I-339) + (4.005), (I-339) + (4.006), (I-339) + (4.007), (I-339) + (4.008), (I-339) + (4.009), (I-339) + (4.010), (I-339) + (4.011), (I-339) + (4.012), (I-339) + (4.013), (I-339) + (4.014), (I-339) + (4.015), (I-339) + (4.016), (I-339) + (4.017), (I-339) + (4.018), (I-339) + (4.019), (I-339) + (4.020), (I-339) + (4.021), (I-339) + (4.022), (I-339) + (4.023), (I-339) + (4.024), (I-339) + (4.025), (I-339) + (4.026), (I-339) + (5.001), (I-339) + (5.002), (I-339) + (5.003), (I-339) + (5.004), (I-339) + (5.005), (I-339) + (5.006), (I-339) + (5.007), (I-339) + (5.008), (I-339) + (5.009), (I-339) + (5.010), (I-339) + (5.011), (I-339) + (5.012), (I-339) + (5.013), (I-339) + (5.014), (I-339) + (5.015), (I-339) + (5.016), (I-339) + (5.017), (I-339) + (5.018), (I-339) + (5.019), (I-339) + (5.020), (I-339) + (5.021), (I-339) + (5.022), (I-339) + (5.023), (I-339) + (6.001), (I-339) + (6.002), (I-339) + (6.003), (I-339) + (6.004), (I-339) + (7.001), (I-339) + (7.002), (I-339) + (7.003), (I-339) + (7.004), (I-339) + (7.005), (I-339) + (7.006), (I-339) + (8.001), (I-339) + (9.001), (I-339) + (9.002), (I-339) + (9.003), (I-339) + (9.004), (I-339) + (9.005), (I-339) + (9.006), (I-339) + (9.007), (I-339) + (9.008), (I-339) + (9.009), (I-339) + (10.001), (I-339) + (10.002), (I-339) + (10.003), (I-339) + (11.001), (I-339) + (11.002), (I-339) + (12.001), (I-339) + (12.002), (I-339) + (12.003), (I-339) + (12.004), (I-339) + (13.001), (I-339) + (13.002), (I-339) + (13.003), (I-339) + (13.004), (I-339) + (13.005), (I-339) + (13.006), (I-339) + (14.001), (I-339) + (14.002), (I-339) + (15.001), (I-339) + (15.002), (I-339) + (15.003), (I-339) + (15.004), (I-339) + (15.005), (I-339) + (15.006), (I-339) + (15.007), (I-339) + (15.008), (I-339) + (15.009), (I-339) + (15.010), (I-339) + (15.011), (I-339) + (15.012), (I-339) + (15.013), (I-339) + (15.014), (I-339) + (15.015), (I-339) + (15.016), (I-339) + (15.017), (I-339) + (15.018), (I-339) + (15.019), (I-339) + (15.020), (I-339) + (15.021), (I-339) + (15.022), (I-339) + (15.023), (I-339) + (15.024), (I-339) + (15.025), (I-339) + (15.026), (I-339) + (15.027), (I-339) + (15.028), (I-339) + (15.029), (I-339) + (15.030), (I-339) + (15.031), (I-339) + (15.032), (I-339) + (15.033), (I-339) + (15.034), (I-339) + (15.035), (I-339) + (15.036), (I-339) + (15.037), (I-339) + (15.038), (I-339) + (15.039), (I-339) + (15.040), (I-339) + (15.041), (I-339) + (15.042), (I-339) + (15.043), (I-339) + (15.044), (I-339) + (15.045), (I-339) + (15.046), (I-339) + (15.047), (I-339) + (15.048), (I-339) + (15.049), (I-339) + (15.050), (I-339) + (15.051), (I-339) + (15.052), (I-339) + (15.053), (I-339) + (15.054), (I-339) + (15.055), (I-339) + (15.056), (I-339) + (15.057), (I-339) + (15.058), (I-339) + (15.059), (I-339) + (15.060), (I-339) + (15.061), (I-339) + (15.062), (I-339) + (15.063) , (I-339) + (15.064), (I-339) + (15.065), (I-339) + (15.066), (I-339) + (15.067), (I-339) + (15.068), (I-339) + (15.069), (I-339) + (15.070), (I-339) + (15.071), (I-339) + (15.072), (I-339) + (15.073), (I-339) + (15.074), (I-339) + (15.075), (I-339) + (15.076), (I-339) + (15.077), (I-339) + (15.078), (I-339) + (15.079), (I-339) + (15.080), (I-339) + (15.081), (I-339) + (15.082), (I-339) + (15.083), (I-339) + (15.084), (I-339) + (15.085), (I-339) + (15.086), (I-339) + (15.087), (I-339) + (15.088), (I-339) + (15.089), (I-339) + (15.090), (I-339) + (15.091), (I-339) + (15.092), (I-339) + (15.093), (I-339) + (15.094), (I-339) + (15.095), (I-339) + (15.096), (I-339) + (15.097), (I-339) + (15.098), (I-339) + (15.099), (I-339) + (15.100), (I-339) + (15.101), (I-339) + (15.102), (I-339) + (15.103), (I-339) + (15.104), (I-339) + (15.105), (I-339) + (15.106), (I-339) + (15.107), (I-339) + (15.108), (I-339) + (15.109), (I-339) + (15.110), (I-339) + (15.111), (I-339) + (15.112), (I-339) + (15.113), (I-339) + (15.114), (I-339) + (15.115), (I-339) + (15.116), (I-339) + (15.117), (I-339) + (15.118), (I-339) + (15.119), (I-339) + (15.120), (I-339) + (15.121), (I-339) + (15.122), (I-339) + (15.123), (I-339) + (15.124), (I-339) + (15.125), (I-339) + (15.126), (I-339) + (15.127), (I-339) + (16.001), (I-339) + (16.002), (I-339) + (16.003), (I-339) + (16.004), (I-339) + (16.005), (I-339) + (16.006), (I-339) + (16.007), (I-339) + (16.008), (I-339) + (17.001), (I-339) + (17.002), (I-339) + (17.003), (I-339) + (17.004), (I-339) + (17.005), (I-339) + (17.006), (I-339) + (17.007), (I-339) + (17.008), (I-339) + (17.009), (I-339) + (17.010), (I-339) + (17.011), (I-339) + (17.012) 및 (I-339) + (18.001).
보다 바람직한 화합물 조합물은 군 (G1-1), (G2-1), (G3-1), (G4-1), (G6-1) 및 (G7-1)에 속하는 혼합물로부터 선택된다.
보다 바람직한 화합물 조합물은 군 (G1), (G3) 및 (G4)에 속하는 혼합물로부터 선택된다.
보다 더 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G1-1A)으로부터 선택된다:
(I-052) + (1.002), (I-052) + (1.004), (I-052) + (1.010), (I-052) + (1.012), (I-052) + (1.018), (I-052) + (1.020), (I-052) + (1.021), (I-052) + (1.026), (I-052) + (1.027), (I-052) + (1.055), (I-052) + (1.059), (I-052) + (1.062), (I-052) + (1.067), (I-052) + (1.081), (I-052) + (1.082), (I-052) + (1.092), (I-052) + (2.001), (I-052) + (2.002), (I-052) + (2.003), (I-052) + (2.005), (I-052) + (2.007), (I-052) + (2.017), (I-052) + (2.018), (I-052) + (2.019), (I-052) + (2.021), (I-052) + (2.028), (I-052) + (2.030), (I-052) + (2.038), (I-052) + (3.003), (I-052) + (3.012), (I-052) + (3.016), (I-052) + (3.017), (I-052) + (3.020), (I-052) + (3.025), (I-052) + (3.026), (I-052) + (3.030), (I-052) + (3.031), (I-052) + (4.005), (I-052) + (4.007), (I-052) + (4.012), (I-052) + (4.015), (I-052) + (4.025), (I-052) + (5.003), (I-052) + (5.004), (I-052) + (5.010), (I-052) + (5.012), (I-052) + (5.013), (I-052) + (5.015), (I-052) + (5.018), (I-052) + (6.002), (I-052) + (7.005), (I-052) + (9.004), (I-052) + (12.003), (I-052) + (12.004), (I-052) + (13.001), (I-052) + (13.004), (I-052) + (13.005), (I-052) + (14.001), (I-052) + (14.002), (I-052) + (15.008), (I-052) + (15.012), (I-052) + (15.016), (I-052) + (15.027), (I-052) + (15.043), (I-052) + (15.047), (I-052) + (15.048), (I-052) + (15.052), (I-052) + (15.062), (I-052) + (15.064), (I-052) + (16.001), (I-052) + (17.001), (I-052) + (17.012) 및 (I-052) + (18.001).
보다 더 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G1-A)으로부터 선택된다:
(I-052) + (1.002), (I-052) + (1.004), (I-052) + (1.010), (I-052) + (1.012), (I-052) + (1.018), (I-052) + (1.020), (I-052) + (1.021), (I-052) + (1.026), (I-052) + (1.027), (I-052) + (1.055), (I-052) + (1.059), (I-052) + (1.081), (I-052) + (1.082), (I-052) + (1.092), (I-052) + (2.001), (I-052) + (2.002), (I-052) + (2.003), (I-052) + (2.005), (I-052) + (2.007), (I-052) + (2.017), (I-052) + (2.018), (I-052) + (2.019), (I-052) + (2.021), (I-052) + (2.028), (I-052) + (2.030), (I-052) + (2.038), (I-052) + (3.003), (I-052) + (3.012), (I-052) + (3.016), (I-052) + (3.017), (I-052) + (3.020), (I-052) + (3.025), (I-052) + (3.026), (I-052) + (3.030), (I-052) + (3.031), (I-052) + (4.005), (I-052) + (4.007), (I-052) + (4.012), (I-052) + (4.015), (I-052) + (4.025), (I-052) + (5.003), (I-052) + (5.004), (I-052) + (5.010), (I-052) + (5.012), (I-052) + (5.013), (I-052) + (5.015), (I-052) + (5.018), (I-052) + (6.002), (I-052) + (7.005), (I-052) + (9.004), (I-052) + (12.003), (I-052) + (12.004), (I-052) + (13.001), (I-052) + (13.004), (I-052) + (13.005), (I-052) + (14.001), (I-052) + (14.002), (I-052) + (15.008), (I-052) + (15.012), (I-052) + (15.016), (I-052) + (15.027), (I-052) + (15.047), (I-052) + (15.048), (I-052) + (15.052), (I-052) + (15.062), (I-052) + (15.064), (I-052) + (16.001), (I-052) + (17.001), (I-052) + (17.012) 및 (I-052) + (18.001).
보다 더 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G2-1A)으로부터 선택된다:
(I-130) + (1.002), (I-130) + (1.004), (I-130) + (1.010), (I-130) + (1.012), (I-130) + (1.018), (I-130) + (1.020), (I-130) + (1.021), (I-130) + (1.026), (I-130) + (1.027), (I-130) + (1.055), (I-130) + (1.059), (I-130) + (1.062), (I-130) + (1.067), (I-130) + (1.081), (I-130) + (1.082), (I-130) + (1.092), (I-130) + (2.001), (I-130) + (2.002), (I-130) + (2.003), (I-130) + (2.005), (I-130) + (2.007), (I-130) + (2.017), (I-130) + (2.018), (I-130) + (2.019), (I-130) + (2.021), (I-130) + (2.028), (I-130) + (2.030), (I-130) + (2.038), (I-130) + (3.003), (I-130) + (3.012), (I-130) + (3.016), (I-130) + (3.017), (I-130) + (3.020), (I-130) + (3.025), (I-130) + (3.026), (I-130) + (3.030), (I-130) + (3.031), (I-130) + (4.005), (I-130) + (4.007), (I-130) + (4.012), (I-130) + (4.015), (I-130) + (4.025), (I-130) + (5.003), (I-130) + (5.004), (I-130) + (5.010), (I-130) + (5.012), (I-130) + (5.013), (I-130) + (5.015), (I-130) + (5.018), (I-130) + (6.002), (I-130) + (7.005), (I-130) + (9.004), (I-130) + (12.003), (I-130) + (12.004), (I-130) + (13.001), (I-130) + (13.004), (I-130) + (13.005), (I-130) + (14.001), (I-130) + (14.002), (I-130) + (15.008), (I-130) + (15.012), (I-130) + (15.016), (I-130) + (15.027), (I-130) + (15.043), (I-130) + (15.047), (I-130) + (15.048), (I-130) + (15.052), (I-130) + (15.062), (I-130) + (15.064), (I-130) + (16.001), (I-130) + (17.001), (I-130) + (17.012) 및 (I-130) + (18.001).
보다 더 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G3-1A)으로부터 선택된다:
(I-300) + (1.002), (I-300) + (1.004), (I-300) + (1.010), (I-300) + (1.012), (I-300) + (1.018), (I-300) + (1.020), (I-300) + (1.021), (I-300) + (1.026), (I-300) + (1.027), (I-300) + (1.055), (I-300) + (1.059), (I-300) + (1.062), (I-300) + (1.067), (I-300) + (1.081), (I-300) + (1.082), (I-300) + (1.092), (I-300) + (2.001), (I-300) + (2.002), (I-300) + (2.003), (I-300) + (2.005), (I-300) + (2.007), (I-300) + (2.017), (I-300) + (2.018), (I-300) + (2.019), (I-300) + (2.021), (I-300) + (2.028), (I-300) + (2.030), (I-300) + (2.038), (I-300) + (3.003), (I-300) + (3.012), (I-300) + (3.016), (I-300) + (3.017), (I-300) + (3.020), (I-300) + (3.025), (I-300) + (3.026), (I-300) + (3.030), (I-300) + (3.031), (I-300) + (4.005), (I-300) + (4.007), (I-300) + (4.012), (I-300) + (4.015), (I-300) + (4.025), (I-300) + (5.003), (I-300) + (5.004), (I-300) + (5.010), (I-300) + (5.012), (I-300) + (5.013), (I-300) + (5.015), (I-300) + (5.018), (I-300) + (6.002), (I-300) + (7.005), (I-300) + (9.004), (I-300) + (12.003), (I-300) + (12.004), (I-300) + (13.001), (I-300) + (13.004), (I-300) + (13.005), (I-300) + (14.001), (I-300) + (14.002), (I-300) + (15.008), (I-300) + (15.012), (I-300) + (15.016), (I-300) + (15.027), (I-300) + (15.043), (I-300) + (15.047), (I-300) + (15.048), (I-300) + (15.052), (I-300) + (15.062), (I-300) + (15.064), (I-300) + (16.001), (I-300) + (17.001), (I-300) + (17.012) 및 (I-300) + (18.001).
보다 더 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G3-A)으로부터 선택된다:
(I-300) + (1.002), (I-300) + (1.004), (I-300) + (1.010), (I-300) + (1.012), (I-300) + (1.018), (I-300) + (1.020), (I-300) + (1.021), (I-300) + (1.026), (I-300) + (1.027), (I-300) + (1.055), (I-300) + (1.059), (I-300) + (1.081), (I-300) + (1.082), (I-300) + (1.092), (I-300) + (2.001), (I-300) + (2.002), (I-300) + (2.003), (I-300) + (2.005), (I-300) + (2.007), (I-300) + (2.017), (I-300) + (2.018), (I-300) + (2.019), (I-300) + (2.021), (I-300) + (2.028), (I-300) + (2.030), (I-300) + (2.038), (I-300) + (3.003), (I-300) + (3.012), (I-300) + (3.016), (I-300) + (3.017), (I-300) + (3.020), (I-300) + (3.025), (I-300) + (3.026), (I-300) + (3.030), (I-300) + (3.031), (I-300) + (4.005), (I-300) + (4.007), (I-300) + (4.012), (I-300) + (4.015), (I-300) + (4.025), (I-300) + (5.003), (I-300) + (5.004), (I-300) + (5.010), (I-300) + (5.012), (I-300) + (5.013), (I-300) + (5.015), (I-300) + (5.018), (I-300) + (6.002), (I-300) + (7.005), (I-300) + (9.004), (I-300) + (12.003), (I-300) + (12.004), (I-300) + (13.001), (I-300) + (13.004), (I-300) + (13.005), (I-300) + (14.001), (I-300) + (14.002), (I-300) + (15.008), (I-300) + (15.012), (I-300) + (15.016), (I-300) + (15.027), (I-300) + (15.047), (I-300) + (15.048), (I-300) + (15.052), (I-300) + (15.062), (I-300) + (15.064), (I-300) + (16.001), (I-300) + (17.001), (I-300) + (17.012) 및 (I-300) + (18.001).
보다 더 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G4-1A)으로부터 선택된다:
(I-302) + (1.002), (I-302) + (1.004), (I-302) + (1.010), (I-302) + (1.012), (I-302) + (1.018), (I-302) + (1.020), (I-302) + (1.021), (I-302) + (1.026), (I-302) + (1.027), (I-302) + (1.055), (I-302) + (1.059), (I-302) + (1.062), (I-302) + (1.067), (I-302) + (1.081), (I-302) + (1.082), (I-302) + (1.092), (I-302) + (2.001), (I-302) + (2.002), (I-302) + (2.003), (I-302) + (2.005), (I-302) + (2.007), (I-302) + (2.017), (I-302) + (2.018), (I-302) + (2.019), (I-302) + (2.021), (I-302) + (2.028), (I-302) + (2.030), (I-302) + (2.038), (I-302) + (3.003), (I-302) + (3.012), (I-302) + (3.016), (I-302) + (3.017), (I-302) + (3.020), (I-302) + (3.025), (I-302) + (3.026), (I-302) + (3.030), (I-302) + (3.031), (I-302) + (4.005), (I-302) + (4.007), (I-302) + (4.012), (I-302) + (4.015), (I-302) + (4.025), (I-302) + (5.003), (I-302) + (5.004), (I-302) + (5.010), (I-302) + (5.012), (I-302) + (5.013), (I-302) + (5.015), (I-302) + (5.018), (I-302) + (6.002), (I-302) + (7.005), (I-302) + (9.004), (I-302) + (12.003), (I-302) + (12.004), (I-302) + (13.001), (I-302) + (13.004), (I-302) + (13.005), (I-302) + (14.001), (I-302) + (14.002), (I-302) + (15.008), (I-302) + (15.012), (I-302) + (15.016), (I-302) + (15.027), (I-302) + (15.043), (I-302) + (15.047), (I-302) + (15.048), (I-302) + (15.052), (I-302) + (15.062), (I-302) + (15.064), (I-302) + (16.001), (I-302) + (17.001), (I-302) + (17.012) 및 (I-302) + (18.001).
보다 더 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G4-A)으로부터 선택된다:
(I-302) + (1.002), (I-302) + (1.004), (I-302) + (1.010), (I-302) + (1.012), (I-302) + (1.018), (I-302) + (1.020), (I-302) + (1.021), (I-302) + (1.026), (I-302) + (1.027), (I-302) + (1.055), (I-302) + (1.059), (I-302) + (1.081), (I-302) + (1.082), (I-302) + (1.092), (I-302) + (2.001), (I-302) + (2.002), (I-302) + (2.003), (I-302) + (2.005), (I-302) + (2.007), (I-302) + (2.017), (I-302) + (2.018), (I-302) + (2.019), (I-302) + (2.021), (I-302) + (2.028), (I-302) + (2.030), (I-302) + (2.038), (I-302) + (3.003), (I-302) + (3.012), (I-302) + (3.016), (I-302) + (3.017), (I-302) + (3.020), (I-302) + (3.025), (I-302) + (3.026), (I-302) + (3.030), (I-302) + (3.031), (I-302) + (4.005), (I-302) + (4.007), (I-302) + (4.012), (I-302) + (4.015), (I-302) + (4.025), (I-302) + (5.003), (I-302) + (5.004), (I-302) + (5.010), (I-302) + (5.012), (I-302) + (5.013), (I-302) + (5.015), (I-302) + (5.018), (I-302) + (6.002), (I-302) + (7.005), (I-302) + (9.004), (I-302) + (12.003), (I-302) + (12.004), (I-302) + (13.001), (I-302) + (13.004), (I-302) + (13.005), (I-302) + (14.001), (I-302) + (14.002), (I-302) + (15.008), (I-302) + (15.012), (I-302) + (15.016), (I-302) + (15.027), (I-302) + (15.047), (I-302) + (15.048), (I-302) + (15.052), (I-302) + (15.062), (I-302) + (15.064), (I-302) + (16.001), (I-302) + (17.001), (I-302) + (17.012) 및 (I-302) + (18.001).
보다 더 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G6-1A)으로부터 선택된다:
(I-339) + (1.002), (I-339) + (1.004), (I-339) + (1.010), (I-339) + (1.012), (I-339) + (1.018), (I-339) + (1.020), (I-339) + (1.021), (I-339) + (1.026), (I-339) + (1.027), (I-339) + (1.055), (I-339) + (1.059), (I-339) + (1.062), (I-339) + (1.067), (I-339) + (1.081), (I-339) + (1.082), (I-339) + (1.092), (I-339) + (2.001), (I-339) + (2.002), (I-339) + (2.003), (I-339) + (2.005), (I-339) + (2.007), (I-339) + (2.017), (I-339) + (2.018), (I-339) + (2.019), (I-339) + (2.021), (I-339) + (2.028), (I-339) + (2.030), (I-339) + (2.038), (I-339) + (3.003), (I-339) + (3.012), (I-339) + (3.016), (I-339) + (3.017), (I-339) + (3.020), (I-339) + (3.025), (I-339) + (3.026), (I-339) + (3.030), (I-339) + (3.031), (I-339) + (4.005), (I-339) + (4.007), (I-339) + (4.012), (I-339) + (4.015), (I-339) + (4.025), (I-339) + (5.003), (I-339) + (5.004), (I-339) + (5.010), (I-339) + (5.012), (I-339) + (5.013), (I-339) + (5.015), (I-339) + (5.018), (I-339) + (6.002), (I-339) + (7.005), (I-339) + (9.004), (I-339) + (12.003), (I-339) + (12.004), (I-339) + (13.001), (I-339) + (13.004), (I-339) + (13.005), (I-339) + (14.001), (I-339) + (14.002), (I-339) + (15.008), (I-339) + (15.012), (I-339) + (15.016), (I-339) + (15.027), (I-339) + (15.043), (I-339) + (15.047), (I-339) + (15.048), (I-339) + (15.052), (I-339) + (15.062), (I-339) + (15.064), (I-339) + (16.001), (I-339) + (17.001), (I-339) + (17.012) 및 (I-339) + (18.001).
보다 더 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G7-1A)으로부터 선택된다:
(I-338) + (1.002), (I-338) + (1.004), (I-338) + (1.010), (I-338) + (1.012), (I-338) + (1.018), (I-338) + (1.020), (I-338) + (1.021), (I-338) + (1.026), (I-338) + (1.027), (I-338) + (1.055), (I-338) + (1.059), (I-338) + (1.062), (I-338) + (1.067), (I-338) + (1.081), (I-338) + (1.082), (I-338) + (1.092), (I-338) + (2.001), (I-338) + (2.002), (I-338) + (2.003), (I-338) + (2.005), (I-338) + (2.007), (I-338) + (2.017), (I-338) + (2.018), (I-338) + (2.019), (I-338) + (2.021), (I-338) + (2.028), (I-338) + (2.030), (I-338) + (2.038), (I-338) + (3.003), (I-338) + (3.012), (I-338) + (3.016), (I-338) + (3.017), (I-338) + (3.020), (I-338) + (3.025), (I-338) + (3.026), (I-338) + (3.030), (I-338) + (3.031), (I-338) + (4.005), (I-338) + (4.007), (I-338) + (4.012), (I-338) + (4.015), (I-338) + (4.025), (I-338) + (5.003), (I-338) + (5.004), (I-338) + (5.010), (I-338) + (5.012), (I-338) + (5.013), (I-338) + (5.015), (I-338) + (5.018), (I-338) + (6.002), (I-338) + (7.005), (I-338) + (9.004), (I-338) + (12.003), (I-338) + (12.004), (I-338) + (13.001), (I-338) + (13.004), (I-338) + (13.005), (I-338) + (14.001), (I-338) + (14.002), (I-338) + (15.008), (I-338) + (15.012), (I-338) + (15.016), (I-338) + (15.027), (I-338) + (15.043), (I-338) + (15.047), (I-338) + (15.048), (I-338) + (15.052), (I-338) + (15.062), (I-338) + (15.064), (I-338) + (16.001), (I-338) + (17.001), (I-338) + (17.012) 및 (I-338) + (18.001).
보다 더욱더 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G1-A)으로부터 선택된다:
(I-052) + (1.002), (I-052) + (1.018), (I-052) + (1.020), (I-052) + (1.021), (I-052) + (1.055), (I-052) + (2.002), (I-052) + (2.005), (I-052) + (2.028), (I-052) + (2.038), (I-052) + (3.020), (I-052) + (3.025), (I-052) + (5.003), (I-052) + (5.010), (I-052) + (5.012), (I-052) + (5.013), (I-052) + (5.018), (I-052) + (6.002), (I-052) + (7.005), (I-052) + (13.001), (I-052) + (13.004), (I-052) + (13.005), (I-052) + (15.012), (I-052) + (15.016), (I-052) + (15.064), (I-052) + (17.001), (I-052) + (17.012) 및 (I-052) + (18.001).
보다 더욱더 바람직한 화합물 조합물은 또한 하기 혼합물로 이루어진 군 (G3-A)으로부터 선택된다:
(I-300) + (1.002), (I-300) + (1.018), (I-300) + (1.020), (I-300) + (1.021), (I-300) + (1.055), (I-300) + (2.002), (I-300) + (2.005), (I-300) + (2.028), (I-300) + (2.038), (I-300) + (3.020), (I-300) + (3.025), (I-300) + (5.003), (I-300) + (5.010), (I-300) + (5.012), (I-300) + (5.013), (I-300) + (5.018), (I-300) + (6.002), (I-300) + (7.005), (I-300) + (13.001), (I-300) + (13.004), (I-300) + (13.005), (I-300) + (15.012), (I-300) + (15.016), (I-300) + (15.064), (I-300) + (17.001), (I-300) + (17.012) 및 (I-300) + (18.001).
보다 더욱더 바람직한 화합물 조합물은 또한 하기 혼합물로 이루어진 군 (G4-A)으로부터 선택된다:
(I-302) + (1.002), (I-302) + (1.018), (I-302) + (1.020), (I-302) + (1.021), (I-302) + (1.055), (I-302) + (2.002), (I-302) + (2.005), (I-302) + (2.028), (I-302) + (2.038), (I-302) + (3.020), (I-302) + (3.025), (I-302) + (5.003), (I-302) + (5.010), (I-302) + (5.012), (I-302) + (5.013), (I-302) + (5.018), (I-302) + (6.002), (I-302) + (7.005), (I-302) + (13.001), (I-302) + (13.004), (I-302) + (13.005), (I-302) + (15.012), (I-302) + (15.016), (I-302) + (15.064), (I-300) + (17.001), (I-302) + (17.012) 및 (I-302) + (18.001).
보다 더욱더 바람직한 화합물 조합물은 또한 하기 혼합물로 이루어진 군 (G2-1A)으로부터 선택된다:
(I-130) + (1.002), (I-130) + (1.018), (I-130) + (1.020), (I-130) + (1.021), (I-130) + (1.055), (I-130) + (1.067), (I-130) + (2.002), (I-130) + (2.005), (I-130) + (2.017), (I-130) + (2.028), (I-130) + (2.038), (I-130) + (3.012), (I-130) + (3.025), (I-130) + (3.030), (I-130) + (5.003), (I-130) + (5.010), (I-130) + (5.012), (I-130) + (5.013), (I-130) + (5.018), (I-130) + (6.002), (I-130) + (7.005), (I-130) + (12.004), (I-130) + (13.001), (I-130) + (13.004), (I-130) + (13.005), (I-130) + (15.012), (I-130) + (15.016), (I-130) + (15.043), (I-130) + (17.001) 및 (I-130) + (17.012)
보다 더욱더 바람직한 화합물 조합물은 또한 하기 혼합물로 이루어진 군 (G7-A1)으로부터 선택된다:
(I-338) + (1.002), (I-338) + (1.018), (I-338) + (1.020), (I-338) + (1.021), (I-338) + (1.055), (I-338) + (1.067), (I-338) + (2.002), (I-338) + (2.005), (I-338) + (2.017), (I-338) + (2.028), (I-338) + (2.038), (I-338) + (3.012), (I-338) + (3.020), (I-338) + (3.025), (I-338) + (3.030), (I-338) + (5.003), (I-338) + (5.010), (I-338) + (5.012), (I-338) + (5.013), (I-338) + (5.018), (I-338) + (6.002), (I-338) + (7.005), (I-338) + (12.004), (I-338) + (13.001), (I-338) + (13.004), (I-338) + (13.005), (I-338) + (15.012), (I-338) + (15.016), (I-338) + (15.043), (I-338) + (17.001) 및 (I-338) + (17.012)
보다 더욱더 바람직한 화합물 조합물은 또한 하기 혼합물로 이루어진 군 (G6-A1)으로부터 선택된다:
(I-339) + (1.002), (I-339) + (1.018), (I-339) + (1.020), (I-339) + (1.021), (I-339) + (1.055), (I-339) + (1.067), (I-339) + (2.002), (I-339) + (2.005), (I-339) + (2.017), (I-339) + (2.028), (I-339) + (2.038), (I-339) + (3.012), (I-339) + (3.020), (I-339) + (3.025), (I-339) + (3.030), (I-339) + (5.003), (I-339) + (5.010), (I-339) + (5.012), (I-339) + (5.013), (I-339) + (5.018), (I-339) + (6.002), (I-339) + (7.005), (I-339) + (12.004), (I-339) + (13.001), (I-339) + (13.004), (I-339) + (13.005), (I-339) + (15.012), (I-339) + (15.016), (I-339) + (15.043), (I-339) + (17.001) 및 (I-339) + (17.012)
2종의 화합물 (B)가 본 발명에 따른 조합물에 존재하는 경우, 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G1-C)으로부터 선택된다:
(I-052) + (1.001) + (1.002), (I-052) + (1.001) + (1.003), (I-052) + (1.001) + (1.004), (I-052) + (1.001) + (1.005), (I-052) + (1.001) + (1.006), (I-052) + (1.001) + (1.007), (I-052) + (1.001) + (1.008), (I-052) + (1.001) + (1.009), (I-052) + (1.001) + (1.010), (I-052) + (1.001) + (1.011), (I-052) + (1.001) + (1.012), (I-052) + (1.001) + (1.013), (I-052) + (1.001) + (1.014), (I-052) + (1.001) + (1.015), (I-052) + (1.001) + (1.016), (I-052) + (1.001) + (1.017), (I-052) + (1.001) + (1.018), (I-052) + (1.001) + (1.019), (I-052) + (1.001) + (1.020), (I-052) + (1.001) + (1.021), (I-052) + (1.001) + (1.022), (I-052) + (1.001) + (1.023), (I-052) + (1.001) + (1.024), (I-052) + (1.001) + (1.025), (I-052) + (1.001) + (1.026), (I-052) + (1.001) + (1.027), (I-052) + (1.001) + (1.028), (I-052) + (1.001) + (1.029), (I-052) + (1.001) + (1.030), (I-052) + (1.001) + (1.031), (I-052) + (1.001) + (1.032), (I-052) + (1.001) + (1.033), (I-052) + (1.001) + (1.034), (I-052) + (1.001) + (1.035), (I-052) + (1.001) + (1.036), (I-052) + (1.001) + (1.037), (I-052) + (1.001) + (1.038), (I-052) + (1.001) + (1.039), (I-052) + (1.001) + (1.040), (I-052) + (1.001) + (1.041), (I-052) + (1.001) + (1.042), (I-052) + (1.001) + (1.043), (I-052) + (1.001) + (1.044), (I-052) + (1.001) + (1.045), (I-052) + (1.001) + (1.046), (I-052) + (1.001) + (1.047), (I-052) + (1.001) + (1.048), (I-052) + (1.001) + (1.049), (I-052) + (1.001) + (1.050), (I-052) + (1.001) + (1.051), (I-052) + (1.001) + (1.052), (I-052) + (1.001) + (1.053), (I-052) + (1.001) + (1.054), (I-052) + (1.001) + (1.055), (I-052) + (1.001) + (1.056), (I-052) + (1.001) + (1.057), (I-052) + (1.001) + (1.058), (I-052) + (1.001) + (1.059), (I-052) + (1.001) + (1.060), (I-052) + (1.001) + (1.061), (I-052) + (1.001) + (1.062), (I-052) + (1.001) + (1.063), (I-052) + (1.001) + (1.064), (I-052) + (1.001) + (1.065), (I-052) + (1.001) + (1.066), (I-052) + (1.001) + (1.067), (I-052) + (1.001) + (1.068), (I-052) + (1.001) + (1.069), (I-052) + (1.001) + 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(I-052) + (5.011) + (9.001), (I-052) + (5.011) + (9.002), (I-052) + (5.011) + (9.003), (I-052) + (5.011) + (9.004), (I-052) + (5.011) + (9.005), (I-052) + (5.011) + (9.006), (I-052) + (5.011) + (9.007), (I-052) + (5.011) + (9.008), (I-052) + (5.011) + (9.009), (I-052) + (5.011) + (15.012), (I-052) + (5.011) + (15.016), (I-052) + (5.011) + (15.025), (I-052) + (5.011) + (15.027), (I-052) + (5.011) + (15.047), (I-052) + (5.011) + (15.063), (I-052) + (5.011) + (15.064),
(I-052) + (5.012) + (9.001), (I-052) + (5.012) + (9.002), (I-052) + (5.012) + (9.003), (I-052) + (5.012) + (9.004), (I-052) + (5.012) + (9.005), (I-052) + (5.012) + (9.006), (I-052) + (5.012) + (9.007), (I-052) + (5.012) + (9.008), (I-052) + (5.012) + (9.009), (I-052) + (5.012) + (15.012), (I-052) + (5.012) + (15.016), (I-052) + (5.012) + (15.025), (I-052) + (5.012) + (15.027), (I-052) + (5.012) + (15.047), (I-052) + (5.012) + (15.063), (I-052) + (5.012) + (15.064),
(I-052) + (5.013) + (9.001), (I-052) + (5.013) + (9.002), (I-052) + (5.013) + (9.003), (I-052) + (5.013) + (9.004), (I-052) + (5.013) + (9.005), (I-052) + (5.013) + (9.006), (I-052) + (5.013) + (9.007), (I-052) + (5.013) + (9.008), (I-052) + (5.013) + (9.009), (I-052) + (5.013) + (15.012), (I-052) + (5.013) + (15.016), (I-052) + (5.013) + (15.025), (I-052) + (5.013) + (15.027), (I-052) + (5.013) + (15.047), (I-052) + (5.013) + (15.063), (I-052) + (5.013) + (15.064),
(I-052) + (5.014) + (9.001), (I-052) + (5.014) + (9.002), (I-052) + (5.014) + (9.003), (I-052) + (5.014) + (9.004), (I-052) + (5.014) + (9.005), (I-052) + (5.014) + (9.006), (I-052) + (5.014) + (9.007), (I-052) + (5.014) + (9.008), (I-052) + (5.014) + (9.009), (I-052) + (5.014) + (15.012), (I-052) + (5.014) + (15.016), (I-052) + (5.014) + (15.025), (I-052) + (5.014) + (15.027), (I-052) + (5.014) + (15.047), (I-052) + (5.014) + (15.063), (I-052) + (5.014) + (15.064),
(I-052) + (5.015) + (9.001), (I-052) + (5.015) + (9.002), (I-052) + (5.015) + (9.003), (I-052) + (5.015) + (9.004), (I-052) + (5.015) + (9.005), (I-052) + (5.015) + (9.006), (I-052) + (5.015) + (9.007), (I-052) + (5.015) + (9.008), (I-052) + (5.015) + (9.009), (I-052) + (5.015) + (15.012), (I-052) + (5.015) + (15.016), (I-052) + (5.015) + (15.025), (I-052) + (5.015) + (15.027), (I-052) + (5.015) + (15.047), (I-052) + (5.015) + (15.063), (I-052) + (5.015) + (15.064),
(I-052) + (5.016) + (9.001), (I-052) + (5.016) + (9.002), (I-052) + (5.016) + (9.003), (I-052) + (5.016) + (9.004), (I-052) + (5.016) + (9.005), (I-052) + (5.016) + (9.006), (I-052) + (5.016) + (9.007), (I-052) + (5.016) + (9.008), (I-052) + (5.016) + (9.009), (I-052) + (5.016) + (15.012), (I-052) + (5.016) + (15.016), (I-052) + (5.016) + (15.025), (I-052) + (5.016) + (15.027), (I-052) + (5.016) + (15.047), (I-052) + (5.016) + (15.063), (I-052) + (5.016) + (15.064),
(I-052) + (5.017) + (9.001), (I-052) + (5.017) + (9.002), (I-052) + (5.017) + (9.003), (I-052) + (5.017) + (9.004), (I-052) + (5.017) + (9.005), (I-052) + (5.017) + (9.006), (I-052) + (5.017) + (9.007), (I-052) + (5.017) + (9.008), (I-052) + (5.017) + (9.009), (I-052) + (5.017) + (15.012), (I-052) + (5.017) + (15.016), (I-052) + (5.017) + (15.025), (I-052) + (5.017) + (15.027), (I-052) + (5.017) + (15.047), (I-052) + (5.017) + (15.063), (I-052) + (5.017) + (15.064),
(I-052) + (5.018) + (9.001), (I-052) + (5.018) + (9.002), (I-052) + (5.018) + (9.003), (I-052) + (5.018) + (9.004), (I-052) + (5.018) + (9.005), (I-052) + (5.018) + (9.006), (I-052) + (5.018) + (9.007), (I-052) + (5.018) + (9.008), (I-052) + (5.018) + (9.009), (I-052) + (5.018) + (15.012), (I-052) + (5.018) + (15.016), (I-052) + (5.018) + (15.025), (I-052) + (5.018) + (15.027), (I-052) + (5.018) + (15.047), (I-052) + (5.018) + (15.063), (I-052) + (5.018) + (15.064),
(I-052) + (5.019) + (9.001), (I-052) + (5.019) + (9.002), (I-052) + (5.019) + (9.003), (I-052) + (5.019) + (9.004), (I-052) + (5.019) + (9.005), (I-052) + (5.019) + (9.006), (I-052) + (5.019) + (9.007), (I-052) + (5.019) + (9.008), (I-052) + (5.019) + (9.009), (I-052) + (5.019) + (15.012), (I-052) + (5.019) + (15.016), (I-052) + (5.019) + (15.025), (I-052) + (5.019) + (15.027), (I-052) + (5.019) + (15.047), (I-052) + (5.019) + (15.063), (I-052) + (5.019) + (15.064),
(I-052) + (5.020) + (9.001), (I-052) + (5.020) + (9.002), (I-052) + (5.020) + (9.003), (I-052) + (5.020) + (9.004), (I-052) + (5.020) + (9.005), (I-052) + (5.020) + (9.006), (I-052) + (5.020) + (9.007), (I-052) + (5.020) + (9.008), (I-052) + (5.020) + (9.009), (I-052) + (5.020) + (15.012), (I-052) + (5.020) + (15.016), (I-052) + (5.020) + (15.025), (I-052) + (5.020) + (15.027), (I-052) + (5.020) + (15.047), (I-052) + (5.020) + (15.063), (I-052) + (5.020) + (15.064),
(I-052) + (5.021) + (9.001), (I-052) + (5.021) + (9.002), (I-052) + (5.021) + (9.003), (I-052) + (5.021) + (9.004), (I-052) + (5.021) + (9.005), (I-052) + (5.021) + (9.006), (I-052) + (5.021) + (9.007), (I-052) + (5.021) + (9.008), (I-052) + (5.021) + (9.009), (I-052) + (5.021) + (15.012), (I-052) + (5.021) + (15.016), (I-052) + (5.021) + (15.025), (I-052) + (5.021) + (15.027), (I-052) + (5.021) + (15.047), (I-052) + (5.021) + (15.063), (I-052) + (5.021) + (15.064),
(I-052) + (5.022) + (9.001), (I-052) + (5.022) + (9.002), (I-052) + (5.022) + (9.003), (I-052) + (5.022) + (9.004), (I-052) + (5.022) + (9.005), (I-052) + (5.022) + (9.006), (I-052) + (5.022) + (9.007), (I-052) + (5.022) + (9.008), (I-052) + (5.022) + (9.009), (I-052) + (5.022) + (15.012), (I-052) + (5.022) + (15.016), (I-052) + (5.022) + (15.025), (I-052) + (5.022) + (15.027), (I-052) + (5.022) + (15.047), (I-052) + (5.022) + (15.063), (I-052) + (5.022) + (15.064),
(I-052) + (5.023) + (9.001), (I-052) + (5.023) + (9.002), (I-052) + (5.023) + (9.003), (I-052) + (5.023) + (9.004), (I-052) + (5.023) + (9.005), (I-052) + (5.023) + (9.006), (I-052) + (5.023) + (9.007), (I-052) + (5.023) + (9.008), (I-052) + (5.023) + (9.009), (I-052) + (5.023) + (15.012), (I-052) + (5.023) + (15.016), (I-052) + (5.023) + (15.025), (I-052) + (5.023) + (15.027), (I-052) + (5.023) + (15.047), (I-052) + (5.023) + (15.063), (I-052) + (5.023) + (15.064).
2종의 화합물 (B)가 본 발명에 따른 조합물에 존재하는 경우, 바람직한 화합물 조합물은 또한 하기 혼합물로 이루어진 군 (G2-C)으로부터 선택된다:
(I-130) + (1.001) + (1.002), (I-130) + (1.001) + (1.003), (I-130) + (1.001) + (1.004), (I-130) + (1.001) + (1.005), (I-130) + (1.001) + (1.006), (I-130) + (1.001) + (1.007), (I-130) + (1.001) + (1.008), (I-130) + (1.001) + (1.009), (I-130) + (1.001) + (1.010), (I-130) + (1.001) + (1.011), (I-130) + (1.001) + (1.012), (I-130) + (1.001) + (1.013), (I-130) + (1.001) + (1.014), (I-130) + (1.001) + (1.015), (I-130) + (1.001) + (1.016), (I-130) + (1.001) + (1.017), (I-130) + (1.001) + (1.018), (I-130) + (1.001) + (1.019), (I-130) + (1.001) + (1.020), (I-130) + (1.001) + (1.021), (I-130) + (1.001) + (1.022), (I-130) + (1.001) + (1.023), (I-130) + (1.001) + (1.024), (I-130) + (1.001) + (1.025), (I-130) + (1.001) + (1.026), (I-130) + (1.001) + (1.027), (I-130) + (1.001) + (1.028), (I-130) + (1.001) + (1.029), (I-130) + (1.001) + (1.030), (I-130) + (1.001) + (1.031), (I-130) + (1.001) + (1.032), (I-130) + (1.001) + (1.033), (I-130) + (1.001) + (1.034), (I-130) + (1.001) + (1.035), (I-130) + (1.001) + (1.036), (I-130) + (1.001) + (1.037), (I-130) + (1.001) + (1.038), (I-130) + (1.001) + (1.039), (I-130) + (1.001) + (1.040), (I-130) + (1.001) + (1.041), (I-130) + (1.001) + (1.042), (I-130) + (1.001) + (1.043), (I-130) + (1.001) + (1.044), (I-130) + (1.001) + (1.045), (I-130) + (1.001) + (1.046), (I-130) + (1.001) + (1.047), (I-130) + (1.001) + (1.048), (I-130) + (1.001) + (1.049), (I-130) + (1.001) + (1.050), (I-130) + (1.001) + (1.051), (I-130) + (1.001) + (1.052), (I-130) + (1.001) + (1.053), (I-130) + (1.001) + (1.054), (I-130) + (1.001) + (1.055), (I-130) + (1.001) + (1.056), (I-130) + (1.001) + (1.057), (I-130) + (1.001) + (1.058), (I-130) + (1.001) + (1.059), (I-130) + (1.001) + (1.060), (I-130) + (1.001) + (1.061), (I-130) + (1.001) + (1.062), (I-130) + (1.001) + (1.063), (I-130) + (1.001) + (1.064), (I-130) + (1.001) + (1.065), (I-130) + (1.001) + (1.066), (I-130) + (1.001) + (1.067), (I-130) + (1.001) + (1.068), (I-130) + (1.001) + (1.069), (I-130) + (1.001) + (1.070), (I-130) + (1.001) + (1.071), (I-130) + (1.001) + (1.072), (I-130) + (1.001) + (1.073), (I-130) + (1.001) + (1.074), (I-130) + (1.001) + (1.075), (I-130) + (1.001) + (1.076), (I-130) + (1.001) + (1.077), (I-130) + (1.001) + (1.078), (I-130) + (1.001) + (1.079), (I-130) + (1.001) + (1.080), (I-130) + (1.001) + (1.081), (I-130) + (1.001) + (1.082), (I-130) + (1.001) + (1.083), (I-130) + (1.001) + (1.084), (I-130) + (1.001) + (1.085), (I-130) + (1.001) + (1.086), (I-130) + (1.001) + (1.087), (I-130) + (1.001) + (1.088), (I-130) + (1.001) + (1.089), (I-130) + (1.001) + (1.090), (I-130) + (1.001) + (1.091), (I-130) + (1.001) + (1.092), (I-130) + (1.001) + (2.001), (I-130) + (1.001) + (2.002), (I-130) + (1.001) + (2.003), (I-130) + (1.001) + (2.004), (I-130) + (1.001) + (2.005), (I-130) + (1.001) + (2.006), (I-130) + (1.001) + (2.007), (I-130) + (1.001) + (2.008), (I-130) + (1.001) + (2.009), (I-130) + (1.001) + (2.010), (I-130) + (1.001) + (2.011), (I-130) + (1.001) + (2.012), (I-130) + (1.001) + (2.013), (I-130) + (1.001) + (2.014), (I-130) + (1.001) + (2.015), (I-130) + (1.001) + (2.016), (I-130) + (1.001) + (2.017), (I-130) + (1.001) + (2.018), (I-130) + (1.001) + (2.019), (I-130) + (1.001) + (2.020), (I-130) + (1.001) + (2.021), (I-130) + (1.001) + (2.022), (I-130) + (1.001) + (2.023), (I-130) + (1.001) + (2.024), (I-130) + (1.001) + (2.025), (I-130) + (1.001) + (2.026), (I-130) + (1.001) + (2.027), (I-130) + (1.001) + (2.028), (I-130) + (1.001) + (2.029), (I-130) + (1.001) + (2.030), (I-130) + (1.001) + (2.031), (I-130) + (1.001) + (2.032), (I-130) + (1.001) + (2.033), (I-130) + (1.001) + (2.034), (I-130) + (1.001) + (2.035), (I-130) + (1.001) + (2.036), (I-130) + (1.001) + (2.037), (I-130) + (1.001) + (2.038), (I-130) + (1.001) + (2.039), (I-130) + (1.001) + (2.040), (I-130) + (1.001) + (2.041), (I-130) + (1.001) + (2.042), (I-130) + (1.001) + (2.043), (I-130) + (1.001) + (2.044), (I-130) + (1.001) + (2.045), (I-130) + (1.001) + (2.046), (I-130) + 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(I-130) + (5.011) + (9.001), (I-130) + (5.011) + (9.002), (I-130) + (5.011) + (9.003), (I-130) + (5.011) + (9.004), (I-130) + (5.011) + (9.005), (I-130) + (5.011) + (9.006), (I-130) + (5.011) + (9.007), (I-130) + (5.011) + (9.008), (I-130) + (5.011) + (9.009), (I-130) + (5.011) + (15.012), (I-130) + (5.011) + (15.016), (I-130) + (5.011) + (15.025), (I-130) + (5.011) + (15.027), (I-130) + (5.011) + (15.047), (I-130) + (5.011) + (15.063), (I-130) + (5.011) + (15.064),
(I-130) + (5.012) + (9.001), (I-130) + (5.012) + (9.002), (I-130) + (5.012) + (9.003), (I-130) + (5.012) + (9.004), (I-130) + (5.012) + (9.005), (I-130) + (5.012) + (9.006), (I-130) + (5.012) + (9.007), (I-130) + (5.012) + (9.008), (I-130) + (5.012) + (9.009), (I-130) + (5.012) + (15.012), (I-130) + (5.012) + (15.016), (I-130) + (5.012) + (15.025), (I-130) + (5.012) + (15.027), (I-130) + (5.012) + (15.047), (I-130) + (5.012) + (15.063), (I-130) + (5.012) + (15.064),
(I-130) + (5.013) + (9.001), (I-130) + (5.013) + (9.002), (I-130) + (5.013) + (9.003), (I-130) + (5.013) + (9.004), (I-130) + (5.013) + (9.005), (I-130) + (5.013) + (9.006), (I-130) + (5.013) + (9.007), (I-130) + (5.013) + (9.008), (I-130) + (5.013) + (9.009), (I-130) + (5.013) + (15.012), (I-130) + (5.013) + (15.016), (I-130) + (5.013) + (15.025), (I-130) + (5.013) + (15.027), (I-130) + (5.013) + (15.047), (I-130) + (5.013) + (15.063), (I-130) + (5.013) + (15.064),
(I-130) + (5.014) + (9.001), (I-130) + (5.014) + (9.002), (I-130) + (5.014) + (9.003), (I-130) + (5.014) + (9.004), (I-130) + (5.014) + (9.005), (I-130) + (5.014) + (9.006), (I-130) + (5.014) + (9.007), (I-130) + (5.014) + (9.008), (I-130) + (5.014) + (9.009), (I-130) + (5.014) + (15.012), (I-130) + (5.014) + (15.016), (I-130) + (5.014) + (15.025), (I-130) + (5.014) + (15.027), (I-130) + (5.014) + (15.047), (I-130) + (5.014) + (15.063), (I-130) + (5.014) + (15.064),
(I-130) + (5.015) + (9.001), (I-130) + (5.015) + (9.002), (I-130) + (5.015) + (9.003), (I-130) + (5.015) + (9.004), (I-130) + (5.015) + (9.005), (I-130) + (5.015) + (9.006), (I-130) + (5.015) + (9.007), (I-130) + (5.015) + (9.008), (I-130) + (5.015) + (9.009), (I-130) + (5.015) + (15.012), (I-130) + (5.015) + (15.016), (I-130) + (5.015) + (15.025), (I-130) + (5.015) + (15.027), (I-130) + (5.015) + (15.047), (I-130) + (5.015) + (15.063), (I-130) + (5.015) + (15.064),
(I-130) + (5.016) + (9.001), (I-130) + (5.016) + (9.002), (I-130) + (5.016) + (9.003), (I-130) + (5.016) + (9.004), (I-130) + (5.016) + (9.005), (I-130) + (5.016) + (9.006), (I-130) + (5.016) + (9.007), (I-130) + (5.016) + (9.008), (I-130) + (5.016) + (9.009), (I-130) + (5.016) + (15.012), (I-130) + (5.016) + (15.016), (I-130) + (5.016) + (15.025), (I-130) + (5.016) + (15.027), (I-130) + (5.016) + (15.047), (I-130) + (5.016) + (15.063), (I-130) + (5.016) + (15.064),
(I-130) + (5.017) + (9.001), (I-130) + (5.017) + (9.002), (I-130) + (5.017) + (9.003), (I-130) + (5.017) + (9.004), (I-130) + (5.017) + (9.005), (I-130) + (5.017) + (9.006), (I-130) + (5.017) + (9.007), (I-130) + (5.017) + (9.008), (I-130) + (5.017) + (9.009), (I-130) + (5.017) + (15.012), (I-130) + (5.017) + (15.016), (I-130) + (5.017) + (15.025), (I-130) + (5.017) + (15.027), (I-130) + (5.017) + (15.047), (I-130) + (5.017) + (15.063), (I-130) + (5.017) + (15.064),
(I-130) + (5.018) + (9.001), (I-130) + (5.018) + (9.002), (I-130) + (5.018) + (9.003), (I-130) + (5.018) + (9.004), (I-130) + (5.018) + (9.005), (I-130) + (5.018) + (9.006), (I-130) + (5.018) + (9.007), (I-130) + (5.018) + (9.008), (I-130) + (5.018) + (9.009), (I-130) + (5.018) + (15.012), (I-130) + (5.018) + (15.016), (I-130) + (5.018) + (15.025), (I-130) + (5.018) + (15.027), (I-130) + (5.018) + (15.047), (I-130) + (5.018) + (15.063), (I-130) + (5.018) + (15.064),
(I-130) + (5.019) + (9.001), (I-130) + (5.019) + (9.002), (I-130) + (5.019) + (9.003), (I-130) + (5.019) + (9.004), (I-130) + (5.019) + (9.005), (I-130) + (5.019) + (9.006), (I-130) + (5.019) + (9.007), (I-130) + (5.019) + (9.008), (I-130) + (5.019) + (9.009), (I-130) + (5.019) + (15.012), (I-130) + (5.019) + (15.016), (I-130) + (5.019) + (15.025), (I-130) + (5.019) + (15.027), (I-130) + (5.019) + (15.047), (I-130) + (5.019) + (15.063), (I-130) + (5.019) + (15.064),
(I-130) + (5.020) + (9.001), (I-130) + (5.020) + (9.002), (I-130) + (5.020) + (9.003), (I-130) + (5.020) + (9.004), (I-130) + (5.020) + (9.005), (I-130) + (5.020) + (9.006), (I-130) + (5.020) + (9.007), (I-130) + (5.020) + (9.008), (I-130) + (5.020) + (9.009), (I-130) + (5.020) + (15.012), (I-130) + (5.020) + (15.016), (I-130) + (5.020) + (15.025), (I-130) + (5.020) + (15.027), (I-130) + (5.020) + (15.047), (I-130) + (5.020) + (15.063), (I-130) + (5.020) + (15.064),
(I-130) + (5.021) + (9.001), (I-130) + (5.021) + (9.002), (I-130) + (5.021) + (9.003), (I-130) + (5.021) + (9.004), (I-130) + (5.021) + (9.005), (I-130) + (5.021) + (9.006), (I-130) + (5.021) + (9.007), (I-130) + (5.021) + (9.008), (I-130) + (5.021) + (9.009), (I-130) + (5.021) + (15.012), (I-130) + (5.021) + (15.016), (I-130) + (5.021) + (15.025), (I-130) + (5.021) + (15.027), (I-130) + (5.021) + (15.047), (I-130) + (5.021) + (15.063), (I-130) + (5.021) + (15.064),
(I-130) + (5.022) + (9.001), (I-130) + (5.022) + (9.002), (I-130) + (5.022) + (9.003), (I-130) + (5.022) + (9.004), (I-130) + (5.022) + (9.005), (I-130) + (5.022) + (9.006), (I-130) + (5.022) + (9.007), (I-130) + (5.022) + (9.008), (I-130) + (5.022) + (9.009), (I-130) + (5.022) + (15.012), (I-130) + (5.022) + (15.016), (I-130) + (5.022) + (15.025), (I-130) + (5.022) + (15.027), (I-130) + (5.022) + (15.047), (I-130) + (5.022) + (15.063), (I-130) + (5.022) + (15.064),
(I-130) + (5.023) + (9.001), (I-130) + (5.023) + (9.002), (I-130) + (5.023) + (9.003), (I-130) + (5.023) + (9.004), (I-130) + (5.023) + (9.005), (I-130) + (5.023) + (9.006), (I-130) + (5.023) + (9.007), (I-130) + (5.023) + (9.008), (I-130) + (5.023) + (9.009), (I-130) + (5.023) + (15.012), (I-130) + (5.023) + (15.016), (I-130) + (5.023) + (15.025), (I-130) + (5.023) + (15.027), (I-130) + (5.023) + (15.047), (I-130) + (5.023) + (15.063), (I-130) + (5.023) + (15.064).
2종의 화합물 (B)가 본 발명에 따른 조합물에 존재하는 경우, 바람직한 화합물 조합물은 또한 하기 혼합물로 이루어진 군 (G3-C)으로부터 선택된다:
(I-300) + (1.001) + (1.002), (I-300) + (1.001) + (1.003), (I-300) + (1.001) + (1.004), (I-300) + (1.001) + (1.005), (I-300) + (1.001) + (1.006), (I-300) + (1.001) + (1.007), (I-300) + (1.001) + (1.008), (I-300) + (1.001) + (1.009), (I-300) + (1.001) + (1.010), (I-300) + (1.001) + (1.011), (I-300) + (1.001) + (1.012), (I-300) + (1.001) + (1.013), (I-300) + (1.001) + (1.014), (I-300) + (1.001) + (1.015), (I-300) + (1.001) + (1.016), (I-300) + (1.001) + (1.017), (I-300) + (1.001) + (1.018), (I-300) + (1.001) + (1.019), (I-300) + (1.001) + (1.020), (I-300) + (1.001) + (1.021), (I-300) + (1.001) + (1.022), (I-300) + (1.001) + (1.023), (I-300) + (1.001) + (1.024), (I-300) + (1.001) + (1.025), (I-300) + (1.001) + (1.026), (I-300) + (1.001) + (1.027), (I-300) + (1.001) + (1.028), (I-300) + (1.001) + (1.029), (I-300) + (1.001) + (1.030), (I-300) + (1.001) + (1.031), (I-300) + (1.001) + (1.032), (I-300) + (1.001) + (1.033), (I-300) + (1.001) + (1.034), (I-300) + (1.001) + (1.035), (I-300) + (1.001) + (1.036), (I-300) + (1.001) + (1.037), (I-300) + (1.001) + (1.038), (I-300) + (1.001) + (1.039), (I-300) + (1.001) + (1.040), (I-300) + (1.001) + (1.041), (I-300) + (1.001) + (1.042), (I-300) + (1.001) + (1.043), (I-300) + (1.001) + (1.044), (I-300) + (1.001) + (1.045), (I-300) + (1.001) + (1.046), (I-300) + (1.001) + (1.047), (I-300) + (1.001) + (1.048), (I-300) + (1.001) + (1.049), (I-300) + (1.001) + (1.050), (I-300) + (1.001) + (1.051), (I-300) + (1.001) + (1.052), (I-300) + (1.001) + (1.053), (I-300) + (1.001) + (1.054), (I-300) + (1.001) + (1.055), (I-300) + (1.001) + (1.056), (I-300) + (1.001) + (1.057), (I-300) + (1.001) + (1.058), (I-300) + (1.001) + (1.059), (I-300) + (1.001) + (1.060), (I-300) + (1.001) + (1.061), (I-300) + (1.001) + (1.062), (I-300) + (1.001) + (1.063), (I-300) + (1.001) + (1.064), (I-300) + (1.001) + (1.065), (I-300) + (1.001) + (1.066), (I-300) + (1.001) + (1.067), (I-300) + (1.001) + (1.068), (I-300) + (1.001) + (1.069), (I-300) + (1.001) + (1.070), (I-300) + (1.001) + (1.071), (I-300) + (1.001) + (1.072), (I-300) + (1.001) + (1.073), (I-300) + (1.001) + (1.074), (I-300) + (1.001) + (1.075), (I-300) + (1.001) + (1.076), (I-300) + (1.001) + (1.077), (I-300) + (1.001) + (1.078), (I-300) + (1.001) + (1.079), (I-300) + (1.001) + (1.080), (I-300) + (1.001) + (1.081), (I-300) + (1.001) + (1.082), (I-300) + (1.001) + (1.083), (I-300) + (1.001) + (1.084), (I-300) + (1.001) + (1.085), (I-300) + (1.001) + (1.086), (I-300) + (1.001) + (1.087), (I-300) + (1.001) + (1.088), (I-300) + (1.001) + (1.089), (I-300) + (1.001) + (1.090), (I-300) + (1.001) + (1.091), (I-300) + (1.001) + (1.092), (I-300) + (1.001) + (2.001), (I-300) + (1.001) + (2.002), (I-300) + (1.001) + (2.003), (I-300) + (1.001) + (2.004), (I-300) + (1.001) + (2.005), (I-300) + (1.001) + (2.006), (I-300) + (1.001) + (2.007), (I-300) + (1.001) + (2.008), (I-300) + (1.001) + (2.009), (I-300) + (1.001) + (2.010), (I-300) + (1.001) + (2.011), (I-300) + (1.001) + (2.012), (I-300) + (1.001) + (2.013), (I-300) + (1.001) + (2.014), (I-300) + (1.001) + (2.015), (I-300) + (1.001) + (2.016), (I-300) + (1.001) + (2.017), (I-300) + (1.001) + (2.018), (I-300) + (1.001) + (2.019), (I-300) + (1.001) + (2.020), (I-300) + (1.001) + (2.021), (I-300) + (1.001) + (2.022), (I-300) + (1.001) + (2.023), (I-300) + (1.001) + (2.024), (I-300) + (1.001) + (2.025), (I-300) + (1.001) + (2.026), (I-300) + (1.001) + (2.027), (I-300) + (1.001) + (2.028), (I-300) + (1.001) + (2.029), (I-300) + (1.001) + (2.030), (I-300) + (1.001) + (2.031), (I-300) + (1.001) + (2.032), (I-300) + (1.001) + (2.033), (I-300) + (1.001) + (2.034), (I-300) + (1.001) + (2.035), (I-300) + (1.001) + (2.036), (I-300) + (1.001) + (2.037), (I-300) + (1.001) + (2.038), (I-300) + (1.001) + (2.039), (I-300) + (1.001) + (2.040), (I-300) + (1.001) + (2.041), (I-300) + (1.001) + (2.042), (I-300) + (1.001) + (2.043), (I-300) + (1.001) + (2.044), (I-300) + (1.001) + (2.045), (I-300) + (1.001) + (2.046), (I-300) + 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(I-300) + (5.002) + (9.001), (I-300) + (5.002) + (9.002), (I-300) + (5.002) + (9.003), (I-300) + (5.002) + (9.004), (I-300) + (5.002) + (9.005), (I-300) + (5.002) + (9.006), (I-300) + (5.002) + (9.007), (I-300) + (5.002) + (9.008), (I-300) + (5.002) + (9.009), (I-300) + (5.002) + (15.012), (I-300) + (5.002) + (15.016), (I-300) + (5.002) + (15.025), (I-300) + (5.002) + (15.027), (I-300) + (5.002) + (15.047), (I-300) + (5.002) + (15.063), (I-300) + (5.002) + (15.064),
(I-300) + (5.003) + (9.001), (I-300) + (5.003) + (9.002), (I-300) + (5.003) + (9.003), (I-300) + (5.003) + (9.004), (I-300) + (5.003) + (9.005), (I-300) + (5.003) + (9.006), (I-300) + (5.003) + (9.007), (I-300) + (5.003) + (9.008), (I-300) + (5.003) + (9.009), (I-300) + (5.003) + (15.012), (I-300) + (5.003) + (15.016), (I-300) + (5.003) + (15.025), (I-300) + (5.003) + (15.027), (I-300) + (5.003) + (15.047), (I-300) + (5.003) + (15.063), (I-300) + (5.003) + (15.064),
(I-300) + (5.004) + (9.001), (I-300) + (5.004) + (9.002), (I-300) + (5.004) + (9.003), (I-300) + (5.004) + (9.004), (I-300) + (5.004) + (9.005), (I-300) + (5.004) + (9.006), (I-300) + (5.004) + (9.007), (I-300) + (5.004) + (9.008), (I-300) + (5.004) + (9.009), (I-300) + (5.004) + (15.012), (I-300) + (5.004) + (15.016), (I-300) + (5.004) + (15.025), (I-300) + (5.004) + (15.027), (I-300) + (5.004) + (15.047), (I-300) + (5.004) + (15.063), (I-300) + (5.004) + (15.064),
(I-300) + (5.005) + (9.001), (I-300) + (5.005) + (9.002), (I-300) + (5.005) + (9.003), (I-300) + (5.005) + (9.004), (I-300) + (5.005) + (9.005), (I-300) + (5.005) + (9.006), (I-300) + (5.005) + (9.007), (I-300) + (5.005) + (9.008), (I-300) + (5.005) + (9.009), (I-300) + (5.005) + (15.012), (I-300) + (5.005) + (15.016), (I-300) + (5.005) + (15.025), (I-300) + (5.005) + (15.027), (I-300) + (5.005) + (15.047), (I-300) + (5.005) + (15.063), (I-300) + (5.005) + (15.064),
(I-300) + (5.006) + (9.001), (I-300) + (5.006) + (9.002), (I-300) + (5.006) + (9.003), (I-300) + (5.006) + (9.004), (I-300) + (5.006) + (9.005), (I-300) + (5.006) + (9.006), (I-300) + (5.006) + (9.007), (I-300) + (5.006) + (9.008), (I-300) + (5.006) + (9.009), (I-300) + (5.006) + (15.012), (I-300) + (5.006) + (15.016), (I-300) + (5.006) + (15.025), (I-300) + (5.006) + (15.027), (I-300) + (5.006) + (15.047), (I-300) + (5.006) + (15.063), (I-300) + (5.006) + (15.064),
(I-300) + (5.007) + (9.001), (I-300) + (5.007) + (9.002), (I-300) + (5.007) + (9.003), (I-300) + (5.007) + (9.004), (I-300) + (5.007) + (9.005), (I-300) + (5.007) + (9.006), (I-300) + (5.007) + (9.007), (I-300) + (5.007) + (9.008), (I-300) + (5.007) + (9.009), (I-300) + (5.007) + (15.012), (I-300) + (5.007) + (15.016), (I-300) + (5.007) + (15.025), (I-300) + (5.007) + (15.027), (I-300) + (5.007) + (15.047), (I-300) + (5.007) + (15.063), (I-300) + (5.007) + (15.064),
(I-300) + (5.008) + (9.001), (I-300) + (5.008) + (9.002), (I-300) + (5.008) + (9.003), (I-300) + (5.008) + (9.004), (I-300) + (5.008) + (9.005), (I-300) + (5.008) + (9.006), (I-300) + (5.008) + (9.007), (I-300) + (5.008) + (9.008), (I-300) + (5.008) + (9.009), (I-300) + (5.008) + (15.012), (I-300) + (5.008) + (15.016), (I-300) + (5.008) + (15.025), (I-300) + (5.008) + (15.027), (I-300) + (5.008) + (15.047), (I-300) + (5.008) + (15.063), (I-300) + (5.008) + (15.064),
(I-300) + (5.009) + (9.001), (I-300) + (5.009) + (9.002), (I-300) + (5.009) + (9.003), (I-300) + (5.009) + (9.004), (I-300) + (5.009) + (9.005), (I-300) + (5.009) + (9.006), (I-300) + (5.009) + (9.007), (I-300) + (5.009) + (9.008), (I-300) + (5.009) + (9.009), (I-300) + (5.009) + (15.012), (I-300) + (5.009) + (15.016), (I-300) + (5.009) + (15.025), (I-300) + (5.009) + (15.027), (I-300) + (5.009) + (15.047), (I-300) + (5.009) + (15.063), (I-300) + (5.009) + (15.064),
(I-300) + (5.010) + (9.001), (I-300) + (5.010) + (9.002), (I-300) + (5.010) + (9.003), (I-300) + (5.010) + (9.004), (I-300) + (5.010) + (9.005), (I-300) + (5.010) + (9.006), (I-300) + (5.010) + (9.007), (I-300) + (5.010) + (9.008), (I-300) + (5.010) + (9.009), (I-300) + (5.010) + (15.012), (I-300) + (5.010) + (15.016), (I-300) + (5.010) + (15.025), (I-300) + (5.010) + (15.027), (I-300) + (5.010) + (15.047), (I-300) + (5.010) + (15.063), (I-300) + (5.010) + (15.064),
(I-300) + (5.011) + (9.001), (I-300) + (5.011) + (9.002), (I-300) + (5.011) + (9.003), (I-300) + (5.011) + (9.004), (I-300) + (5.011) + (9.005), (I-300) + (5.011) + (9.006), (I-300) + (5.011) + (9.007), (I-300) + (5.011) + (9.008), (I-300) + (5.011) + (9.009), (I-300) + (5.011) + (15.012), (I-300) + (5.011) + (15.016), (I-300) + (5.011) + (15.025), (I-300) + (5.011) + (15.027), (I-300) + (5.011) + (15.047), (I-300) + (5.011) + (15.063), (I-300) + (5.011) + (15.064),
(I-300) + (5.012) + (9.001), (I-300) + (5.012) + (9.002), (I-300) + (5.012) + (9.003), (I-300) + (5.012) + (9.004), (I-300) + (5.012) + (9.005), (I-300) + (5.012) + (9.006), (I-300) + (5.012) + (9.007), (I-300) + (5.012) + (9.008), (I-300) + (5.012) + (9.009), (I-300) + (5.012) + (15.012), (I-300) + (5.012) + (15.016), (I-300) + (5.012) + (15.025), (I-300) + (5.012) + (15.027), (I-300) + (5.012) + (15.047), (I-300) + (5.012) + (15.063), (I-300) + (5.012) + (15.064),
(I-300) + (5.013) + (9.001), (I-300) + (5.013) + (9.002), (I-300) + (5.013) + (9.003), (I-300) + (5.013) + (9.004), (I-300) + (5.013) + (9.005), (I-300) + (5.013) + (9.006), (I-300) + (5.013) + (9.007), (I-300) + (5.013) + (9.008), (I-300) + (5.013) + (9.009), (I-300) + (5.013) + (15.012), (I-300) + (5.013) + (15.016), (I-300) + (5.013) + (15.025), (I-300) + (5.013) + (15.027), (I-300) + (5.013) + (15.047), (I-300) + (5.013) + (15.063), (I-300) + (5.013) + (15.064),
(I-300) + (5.014) + (9.001), (I-300) + (5.014) + (9.002), (I-300) + (5.014) + (9.003), (I-300) + (5.014) + (9.004), (I-300) + (5.014) + (9.005), (I-300) + (5.014) + (9.006), (I-300) + (5.014) + (9.007), (I-300) + (5.014) + (9.008), (I-300) + (5.014) + (9.009), (I-300) + (5.014) + (15.012), (I-300) + (5.014) + (15.016), (I-300) + (5.014) + (15.025), (I-300) + (5.014) + (15.027), (I-300) + (5.014) + (15.047), (I-300) + (5.014) + (15.063), (I-300) + (5.014) + (15.064),
(I-300) + (5.015) + (9.001), (I-300) + (5.015) + (9.002), (I-300) + (5.015) + (9.003), (I-300) + (5.015) + (9.004), (I-300) + (5.015) + (9.005), (I-300) + (5.015) + (9.006), (I-300) + (5.015) + (9.007), (I-300) + (5.015) + (9.008), (I-300) + (5.015) + (9.009), (I-300) + (5.015) + (15.012), (I-300) + (5.015) + (15.016), (I-300) + (5.015) + (15.025), (I-300) + (5.015) + (15.027), (I-300) + (5.015) + (15.047), (I-300) + (5.015) + (15.063), (I-300) + (5.015) + (15.064),
(I-300) + (5.016) + (9.001), (I-300) + (5.016) + (9.002), (I-300) + (5.016) + (9.003), (I-300) + (5.016) + (9.004), (I-300) + (5.016) + (9.005), (I-300) + (5.016) + (9.006), (I-300) + (5.016) + (9.007), (I-300) + (5.016) + (9.008), (I-300) + (5.016) + (9.009), (I-300) + (5.016) + (15.012), (I-300) + (5.016) + (15.016), (I-300) + (5.016) + (15.025), (I-300) + (5.016) + (15.027), (I-300) + (5.016) + (15.047), (I-300) + (5.016) + (15.063), (I-300) + (5.016) + (15.064),
(I-300) + (5.017) + (9.001), (I-300) + (5.017) + (9.002), (I-300) + (5.017) + (9.003), (I-300) + (5.017) + (9.004), (I-300) + (5.017) + (9.005), (I-300) + (5.017) + (9.006), (I-300) + (5.017) + (9.007), (I-300) + (5.017) + (9.008), (I-300) + (5.017) + (9.009), (I-300) + (5.017) + (15.012), (I-300) + (5.017) + (15.016), (I-300) + (5.017) + (15.025), (I-300) + (5.017) + (15.027), (I-300) + (5.017) + (15.047), (I-300) + (5.017) + (15.063), (I-300) + (5.017) + (15.064),
(I-300) + (5.018) + (9.001), (I-300) + (5.018) + (9.002), (I-300) + (5.018) + (9.003), (I-300) + (5.018) + (9.004), (I-300) + (5.018) + (9.005), (I-300) + (5.018) + (9.006), (I-300) + (5.018) + (9.007), (I-300) + (5.018) + (9.008), (I-300) + (5.018) + (9.009), (I-300) + (5.018) + (15.012), (I-300) + (5.018) + (15.016), (I-300) + (5.018) + (15.025), (I-300) + (5.018) + (15.027), (I-300) + (5.018) + (15.047), (I-300) + (5.018) + (15.063), (I-300) + (5.018) + (15.064),
(I-300) + (5.019) + (9.001), (I-300) + (5.019) + (9.002), (I-300) + (5.019) + (9.003), (I-300) + (5.019) + (9.004), (I-300) + (5.019) + (9.005), (I-300) + (5.019) + (9.006), (I-300) + (5.019) + (9.007), (I-300) + (5.019) + (9.008), (I-300) + (5.019) + (9.009), (I-300) + (5.019) + (15.012), (I-300) + (5.019) + (15.016), (I-300) + (5.019) + (15.025), (I-300) + (5.019) + (15.027), (I-300) + (5.019) + (15.047), (I-300) + (5.019) + (15.063), (I-300) + (5.019) + (15.064),
(I-300) + (5.020) + (9.001), (I-300) + (5.020) + (9.002), (I-300) + (5.020) + (9.003), (I-300) + (5.020) + (9.004), (I-300) + (5.020) + (9.005), (I-300) + (5.020) + (9.006), (I-300) + (5.020) + (9.007), (I-300) + (5.020) + (9.008), (I-300) + (5.020) + (9.009), (I-300) + (5.020) + (15.012), (I-300) + (5.020) + (15.016), (I-300) + (5.020) + (15.025), (I-300) + (5.020) + (15.027), (I-300) + (5.020) + (15.047), (I-300) + (5.020) + (15.063), (I-300) + (5.020) + (15.064),
(I-300) + (5.021) + (9.001), (I-300) + (5.021) + (9.002), (I-300) + (5.021) + (9.003), (I-300) + (5.021) + (9.004), (I-300) + (5.021) + (9.005), (I-300) + (5.021) + (9.006), (I-300) + (5.021) + (9.007), (I-300) + (5.021) + (9.008), (I-300) + (5.021) + (9.009), (I-300) + (5.021) + (15.012), (I-300) + (5.021) + (15.016), (I-300) + (5.021) + (15.025), (I-300) + (5.021) + (15.027), (I-300) + (5.021) + (15.047), (I-300) + (5.021) + (15.063), (I-300) + (5.021) + (15.064),
(I-300) + (5.022) + (9.001), (I-300) + (5.022) + (9.002), (I-300) + (5.022) + (9.003), (I-300) + (5.022) + (9.004), (I-300) + (5.022) + (9.005), (I-300) + (5.022) + (9.006), (I-300) + (5.022) + (9.007), (I-300) + (5.022) + (9.008), (I-300) + (5.022) + (9.009), (I-300) + (5.022) + (15.012), (I-300) + (5.022) + (15.016), (I-300) + (5.022) + (15.025), (I-300) + (5.022) + (15.027), (I-300) + (5.022) + (15.047), (I-300) + (5.022) + (15.063), (I-300) + (5.022) + (15.064),
(I-300) + (5.023) + (9.001), (I-300) + (5.023) + (9.002), (I-300) + (5.023) + (9.003), (I-300) + (5.023) + (9.004), (I-300) + (5.023) + (9.005), (I-300) + (5.023) + (9.006), (I-300) + (5.023) + (9.007), (I-300) + (5.023) + (9.008), (I-300) + (5.023) + (9.009), (I-300) + (5.023) + (15.012), (I-300) + (5.023) + (15.016), (I-300) + (5.023) + (15.025), (I-300) + (5.023) + (15.027), (I-300) + (5.023) + (15.047), (I-300) + (5.023) + (15.063), (I-300) + (5.023) + (15.064).
2종의 화합물 (B)가 본 발명에 따른 조합물에 존재하는 경우, 바람직한 화합물 조합물은 또한 하기 혼합물로 이루어진 군 (G4-C)으로부터 선택된다:
(I-302) + (1.001) + (1.002), (I-302) + (1.001) + (1.003), (I-302) + (1.001) + (1.004), (I-302) + (1.001) + (1.005), (I-302) + (1.001) + (1.006), (I-302) + (1.001) + (1.007), (I-302) + (1.001) + (1.008), (I-302) + (1.001) + (1.009), (I-302) + (1.001) + (1.010), (I-302) + (1.001) + (1.011), (I-302) + (1.001) + (1.012), (I-302) + (1.001) + (1.013), (I-302) + (1.001) + (1.014), (I-302) + (1.001) + (1.015), (I-302) + (1.001) + (1.016), (I-302) + (1.001) + (1.017), (I-302) + (1.001) + (1.018), (I-302) + (1.001) + (1.019), (I-302) + (1.001) + (1.020), (I-302) + (1.001) + (1.021), (I-302) + (1.001) + (1.022), (I-302) + (1.001) + (1.023), (I-302) + (1.001) + (1.024), (I-302) + (1.001) + (1.025), (I-302) + (1.001) + (1.026), (I-302) + (1.001) + (1.027), (I-302) + (1.001) + (1.028), (I-302) + (1.001) + (1.029), (I-302) + (1.001) + (1.030), (I-302) + (1.001) + (1.031), (I-302) + (1.001) + (1.032), (I-302) + (1.001) + (1.033), (I-302) + (1.001) + (1.034), (I-302) + (1.001) + (1.035), (I-302) + (1.001) + (1.036), (I-302) + (1.001) + (1.037), (I-302) + (1.001) + (1.038), (I-302) + (1.001) + (1.039), (I-302) + (1.001) + (1.040), (I-302) + (1.001) + (1.041), (I-302) + (1.001) + (1.042), (I-302) + (1.001) + (1.043), (I-302) + (1.001) + (1.044), (I-302) + (1.001) + (1.045), (I-302) + (1.001) + (1.046), (I-302) + (1.001) + (1.047), (I-302) + (1.001) + (1.048), (I-302) + (1.001) + (1.049), (I-302) + (1.001) + (1.050), (I-302) + (1.001) + (1.051), (I-302) + (1.001) + (1.052), (I-302) + (1.001) + (1.053), (I-302) + (1.001) + (1.054), (I-302) + (1.001) + (1.055), (I-302) + (1.001) + (1.056), (I-302) + (1.001) + (1.057), (I-302) + (1.001) + (1.058), (I-302) + (1.001) + (1.059), (I-302) + (1.001) + (1.060), (I-302) + (1.001) + (1.061), (I-302) + (1.001) + (1.062), (I-302) + (1.001) + (1.063), (I-302) + (1.001) + (1.064), (I-302) + (1.001) + (1.065), (I-302) + (1.001) + (1.066), (I-302) + (1.001) + (1.067), (I-302) + (1.001) + (1.068), (I-302) + (1.001) + (1.069), (I-302) + (1.001) + (1.070), (I-302) + (1.001) + (1.071), (I-302) + (1.001) + (1.072), (I-302) + (1.001) + (1.073), (I-302) + (1.001) + (1.074), (I-302) + (1.001) + (1.075), (I-302) + (1.001) + (1.076), (I-302) + (1.001) + (1.077), (I-302) + (1.001) + (1.078), (I-302) + (1.001) + (1.079), (I-302) + (1.001) + (1.080), (I-302) + (1.001) + (1.081), (I-302) + (1.001) + (1.082), (I-302) + (1.001) + (1.083), (I-302) + (1.001) + (1.084), (I-302) + (1.001) + (1.085), (I-302) + (1.001) + (1.086), (I-302) + (1.001) + (1.087), (I-302) + (1.001) + (1.088), (I-302) + (1.001) + (1.089), (I-302) + (1.001) + (1.090), (I-302) + (1.001) + (1.091), (I-302) + (1.001) + (1.092), (I-302) + (1.001) + (2.001), (I-302) + (1.001) + (2.002), (I-302) + (1.001) + (2.003), (I-302) + (1.001) + (2.004), (I-302) + (1.001) + (2.005), (I-302) + (1.001) + (2.006), (I-302) + (1.001) + (2.007), (I-302) + (1.001) + (2.008), (I-302) + (1.001) + (2.009), (I-302) + (1.001) + (2.010), (I-302) + (1.001) + (2.011), (I-302) + (1.001) + (2.012), (I-302) + (1.001) + (2.013), (I-302) + (1.001) + (2.014), (I-302) + (1.001) + (2.015), (I-302) + (1.001) + (2.016), (I-302) + (1.001) + (2.017), (I-302) + (1.001) + (2.018), (I-302) + (1.001) + (2.019), (I-302) + (1.001) + (2.020), (I-302) + (1.001) + (2.021), (I-302) + (1.001) + (2.022), (I-302) + (1.001) + (2.023), (I-302) + (1.001) + (2.024), (I-302) + (1.001) + (2.025), (I-302) + (1.001) + (2.026), (I-302) + (1.001) + (2.027), (I-302) + (1.001) + (2.028), (I-302) + (1.001) + (2.029), (I-302) + (1.001) + (2.030), (I-302) + (1.001) + (2.031), (I-302) + (1.001) + (2.032), (I-302) + (1.001) + (2.033), (I-302) + (1.001) + (2.034), (I-302) + (1.001) + (2.035), (I-302) + (1.001) + (2.036), (I-302) + (1.001) + (2.037), (I-302) + (1.001) + (2.038), (I-302) + (1.001) + (2.039), (I-302) + (1.001) + (2.040), (I-302) + (1.001) + (2.041), (I-302) + (1.001) + (2.042), (I-302) + (1.001) + (2.043), (I-302) + (1.001) + (2.044), (I-302) + (1.001) + (2.045), (I-302) + (1.001) + (2.046), (I-302) + (1.001) + (2.047), (I-302) + (1.001) + (2.048), (I-302) + (1.001) + (2.049), (I-302) + (1.001) + (2.050), (I-302) + (1.001) + (2.051), (I-302) + (1.001) + (2.052), (I-302) + (1.001) + (2.053), (I-302) + (1.001) + (2.054), (I-302) + (1.001) + (2.055), (I-302) + (1.001) + (2.056), (I-302) + (1.001) + (2.057), (I-302) + (1.001) + (2.058), (I-302) + (1.001) + (2.059), (I-302) + (1.001) + (3.001), (I-302) + (1.001) + (3.002), (I-302) + (1.001) + (3.003), (I-302) + (1.001) + (3.004), (I-302) + (1.001) + (3.005), (I-302) + (1.001) + (3.006), (I-302) + (1.001) + (3.007), (I-302) + (1.001) + (3.008), (I-302) + (1.001) + (3.009), (I-302) + (1.001) + (3.010), (I-302) + (1.001) + (3.011), (I-302) + (1.001) + (3.012), (I-302) + (1.001) + (3.013), (I-302) + (1.001) + (3.014), (I-302) + (1.001) + (3.015), (I-302) + (1.001) + (3.016), (I-302) + (1.001) + (3.017), (I-302) + (1.001) + (3.018), (I-302) + (1.001) + (3.019), (I-302) + (1.001) + (3.020), (I-302) + (1.001) + (3.021), (I-302) + (1.001) + (3.022), (I-302) + (1.001) + (3.023), (I-302) + (1.001) + (3.024), (I-302) + (1.001) + (3.025), (I-302) + (1.001) + (3.026), (I-302) + (1.001) + (3.027), (I-302) + (1.001) + (3.028), (I-302) + (1.001) + (3.029), (I-302) + (1.001) + (3.030), (I-302) + (1.001) + (3.031), (I-302) + (1.001) + (5.001), (I-302) + (1.001) + (5.002), (I-302) + (1.001) + (5.003), (I-302) + (1.001) + (5.004), (I-302) + (1.001) + (5.005), (I-302) + (1.001) + (5.006), (I-302) + (1.001) + (5.007), (I-302) + (1.001) + (5.008), (I-302) + (1.001) + (5.009), (I-302) + (1.001) + (5.010), (I-302) + (1.001) + (5.011), (I-302) + (1.001) + (5.012), (I-302) + (1.001) + (5.013), (I-302) + (1.001) + (5.014), (I-302) + (1.001) + (5.015), (I-302) + (1.001) + (5.016), (I-302) + (1.001) + (5.017), (I-302) + (1.001) + (5.018), (I-302) + (1.001) + (5.019), (I-302) + (1.001) + (5.020), (I-302) + (1.001) + (5.021), (I-302) + (1.001) + (5.022), (I-302) + (1.001) + (5.023), (I-302) + (1.001) + (6.001), (I-302) + (1.001) + (6.002), (I-302) + (1.001) + (6.003), (I-302) + (1.001) + (6.004), (I-302) + (1.001) + (7.001), (I-302) + (1.001) + (7.002), (I-302) + (1.001) + (7.003), (I-302) + (1.001) + (7.004), (I-302) + (1.001) + (7.005), (I-302) + (1.001) + (7.006), (I-302) + (1.001) + (9.001), (I-302) + (1.001) + (9.002), (I-302) + (1.001) + (9.003), (I-302) + (1.001) + (9.004), (I-302) + (1.001) + (9.005), (I-302) + (1.001) + (9.006), (I-302) + (1.001) + (9.007), (I-302) + (1.001) + (9.008), (I-302) + (1.001) + (9.009), (I-302) + (1.001) + (14.001), (I-302) + (1.001) + (14.002), (I-302) + (1.001) + (15.008), (I-302) + (1.001) + (15.011), (I-302) + (1.001) + (15.012), (I-302) + (1.001) + (15.016), (I-302) + (1.001) + (15.025), (I-302) + (1.001) + (15.027), (I-302) + (1.001) + (15.047), (I-302) + (1.001) + (15.063), (I-302) + (1.001) + (15.064), (I-302) + (1.001) + (16.001), (I-302) + (1.001) + (16.002), (I-302) + (1.001) + (16.003), (I-302) + (1.001) + (16.004), (I-302) + (1.001) + (16.005), (I-302) + (1.001) + (16.006), (I-302) + (1.001) + (16.007), (I-302) + (1.001) + (16.008), (I-302) + (1.001) + (17.001), (I-302) + (1.001) + (17.002), (I-302) + (1.001) + (17.003), (I-302) + (1.001) + (17.004), (I-302) + (1.001) + (17.005), (I-302) + (1.001) + (17.006), (I-302) + (1.001) + (17.007), (I-302) + (1.001) + (17.008), (I-302) + (1.001) + (17.009), (I-302) + (1.001) + (17.010), (I-302) + (1.001) + (17.011), (I-302) + (1.001) + (17.012), (I-302) + (1.001) + (18.001),
(I-302) + (1.002) + (1.003), (I-302) + (1.002) + (1.004), (I-302) + (1.002) + (1.005), (I-302) + (1.002) + (1.006), (I-302) + (1.002) + (1.007), (I-302) + (1.002) + (1.008), (I-302) + (1.002) + (1.009), (I-302) + (1.002) + (1.010), (I-302) + (1.002) + (1.011), (I-302) + (1.002) + (1.012), (I-302) + (1.002) + (1.013), (I-302) + (1.002) + (1.014), (I-302) + (1.002) + (1.015), (I-302) + (1.002) + (1.016), (I-302) + (1.002) + (1.017), (I-302) + (1.002) + (1.018), (I-302) + (1.002) + (1.019), (I-302) + (1.002) + (1.020), (I-302) + (1.002) + (1.021), (I-302) + (1.002) + (1.022), (I-302) + (1.002) + (1.023), (I-302) + (1.002) + (1.024), (I-302) + (1.002) + (1.025), (I-302) + (1.002) + (1.026), (I-302) + (1.002) + (1.027), (I-302) + (1.002) + (1.028), (I-302) + (1.002) + (1.029), (I-302) + (1.002) + (1.030), (I-302) + (1.002) + (1.031), (I-302) + (1.002) + (1.032), (I-302) + (1.002) + (1.033), (I-302) + (1.002) + (1.034), (I-302) + (1.002) + (1.035), (I-302) + (1.002) + (1.036), (I-302) + (1.002) + (1.037), (I-302) + (1.002) + (1.038), (I-302) + (1.002) + (1.039), (I-302) + (1.002) + (1.040), (I-302) + (1.002) + (1.041), (I-302) + (1.002) + (1.042), (I-302) + (1.002) + (1.043), (I-302) + (1.002) + (1.044), (I-302) + (1.002) + (1.045), (I-302) + (1.002) + (1.046), (I-302) + (1.002) + (1.047), (I-302) + (1.002) + (1.048), (I-302) + (1.002) + (1.049), (I-302) + (1.002) + (1.050), (I-302) + (1.002) + (1.051), (I-302) + (1.002) + (1.052), (I-302) + (1.002) + (1.053), (I-302) + (1.002) + (1.054), (I-302) + (1.002) + (1.055), (I-302) + (1.002) + (1.056), (I-302) + (1.002) + (1.057), (I-302) + (1.002) + (1.058), (I-302) + (1.002) + (1.059), (I-302) + (1.002) + (1.060), (I-302) + (1.002) + (1.061), (I-302) + (1.002) + (1.062), (I-302) + (1.002) + (1.063), (I-302) + (1.002) + (1.064), (I-302) + (1.002) + (1.065), (I-302) + (1.002) + (1.066), (I-302) + (1.002) + (1.067), (I-302) + (1.002) + (1.068), (I-302) + (1.002) + (1.069), (I-302) + (1.002) + (1.070), (I-302) + (1.002) + (1.071), (I-302) + (1.002) + (1.072), (I-302) + (1.002) + (1.073), (I-302) + (1.002) + (1.074), (I-302) + (1.002) + (1.075), (I-302) + (1.002) + (1.076), (I-302) + (1.002) + (1.077), (I-302) + (1.002) + (1.078), (I-302) + (1.002) + (1.079), (I-302) + (1.002) + (1.080), (I-302) + (1.002) + (1.081), (I-302) + (1.002) + (1.082), (I-302) + (1.002) + (1.083), (I-302) + (1.002) + (1.084), (I-302) + (1.002) + (1.085), (I-302) + (1.002) + (1.086), (I-302) + (1.002) + (1.087), (I-302) + (1.002) + (1.088), (I-302) + (1.002) + (1.089), (I-302) + (1.002) + (1.090), (I-302) + (1.002) + (1.091), (I-302) + (1.002) + (1.092), (I-302) + (1.002) + (2.001), (I-302) + (1.002) + (2.002), (I-302) + (1.002) + (2.003), (I-302) + (1.002) + (2.004), (I-302) + (1.002) + (2.005), (I-302) + (1.002) + (2.006), (I-302) + (1.002) + (2.007), (I-302) + (1.002) + (2.008), (I-302) + (1.002) + (2.009), (I-302) + (1.002) + (2.010), (I-302) + (1.002) + (2.011), (I-302) + (1.002) + (2.012), (I-302) + (1.002) + (2.013), 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(I-302) + (5.002) + (9.001), (I-302) + (5.002) + (9.002), (I-302) + (5.002) + (9.003), (I-302) + (5.002) + (9.004), (I-302) + (5.002) + (9.005), (I-302) + (5.002) + (9.006), (I-302) + (5.002) + (9.007), (I-302) + (5.002) + (9.008), (I-302) + (5.002) + (9.009), (I-302) + (5.002) + (15.012), (I-302) + (5.002) + (15.016), (I-302) + (5.002) + (15.025), (I-302) + (5.002) + (15.027), (I-302) + (5.002) + (15.047), (I-302) + (5.002) + (15.063), (I-302) + (5.002) + (15.064),
(I-302) + (5.003) + (9.001), (I-302) + (5.003) + (9.002), (I-302) + (5.003) + (9.003), (I-302) + (5.003) + (9.004), (I-302) + (5.003) + (9.005), (I-302) + (5.003) + (9.006), (I-302) + (5.003) + (9.007), (I-302) + (5.003) + (9.008), (I-302) + (5.003) + (9.009), (I-302) + (5.003) + (15.012), (I-302) + (5.003) + (15.016), (I-302) + (5.003) + (15.025), (I-302) + (5.003) + (15.027), (I-302) + (5.003) + (15.047), (I-302) + (5.003) + (15.063), (I-302) + (5.003) + (15.064),
(I-302) + (5.004) + (9.001), (I-302) + (5.004) + (9.002), (I-302) + (5.004) + (9.003), (I-302) + (5.004) + (9.004), (I-302) + (5.004) + (9.005), (I-302) + (5.004) + (9.006), (I-302) + (5.004) + (9.007), (I-302) + (5.004) + (9.008), (I-302) + (5.004) + (9.009), (I-302) + (5.004) + (15.012), (I-302) + (5.004) + (15.016), (I-302) + (5.004) + (15.025), (I-302) + (5.004) + (15.027), (I-302) + (5.004) + (15.047), (I-302) + (5.004) + (15.063), (I-302) + (5.004) + (15.064),
(I-302) + (5.005) + (9.001), (I-302) + (5.005) + (9.002), (I-302) + (5.005) + (9.003), (I-302) + (5.005) + (9.004), (I-302) + (5.005) + (9.005), (I-302) + (5.005) + (9.006), (I-302) + (5.005) + (9.007), (I-302) + (5.005) + (9.008), (I-302) + (5.005) + (9.009), (I-302) + (5.005) + (15.012), (I-302) + (5.005) + (15.016), (I-302) + (5.005) + (15.025), (I-302) + (5.005) + (15.027), (I-302) + (5.005) + (15.047), (I-302) + (5.005) + (15.063), (I-302) + (5.005) + (15.064),
(I-302) + (5.006) + (9.001), (I-302) + (5.006) + (9.002), (I-302) + (5.006) + (9.003), (I-302) + (5.006) + (9.004), (I-302) + (5.006) + (9.005), (I-302) + (5.006) + (9.006), (I-302) + (5.006) + (9.007), (I-302) + (5.006) + (9.008), (I-302) + (5.006) + (9.009), (I-302) + (5.006) + (15.012), (I-302) + (5.006) + (15.016), (I-302) + (5.006) + (15.025), (I-302) + (5.006) + (15.027), (I-302) + (5.006) + (15.047), (I-302) + (5.006) + (15.063), (I-302) + (5.006) + (15.064),
(I-302) + (5.007) + (9.001), (I-302) + (5.007) + (9.002), (I-302) + (5.007) + (9.003), (I-302) + (5.007) + (9.004), (I-302) + (5.007) + (9.005), (I-302) + (5.007) + (9.006), (I-302) + (5.007) + (9.007), (I-302) + (5.007) + (9.008), (I-302) + (5.007) + (9.009), (I-302) + (5.007) + (15.012), (I-302) + (5.007) + (15.016), (I-302) + (5.007) + (15.025), (I-302) + (5.007) + (15.027), (I-302) + (5.007) + (15.047), (I-302) + (5.007) + (15.063), (I-302) + (5.007) + (15.064),
(I-302) + (5.008) + (9.001), (I-302) + (5.008) + (9.002), (I-302) + (5.008) + (9.003), (I-302) + (5.008) + (9.004), (I-302) + (5.008) + (9.005), (I-302) + (5.008) + (9.006), (I-302) + (5.008) + (9.007), (I-302) + (5.008) + (9.008), (I-302) + (5.008) + (9.009), (I-302) + (5.008) + (15.012), (I-302) + (5.008) + (15.016), (I-302) + (5.008) + (15.025), (I-302) + (5.008) + (15.027), (I-302) + (5.008) + (15.047), (I-302) + (5.008) + (15.063), (I-302) + (5.008) + (15.064),
(I-302) + (5.009) + (9.001), (I-302) + (5.009) + (9.002), (I-302) + (5.009) + (9.003), (I-302) + (5.009) + (9.004), (I-302) + (5.009) + (9.005), (I-302) + (5.009) + (9.006), (I-302) + (5.009) + (9.007), (I-302) + (5.009) + (9.008), (I-302) + (5.009) + (9.009), (I-302) + (5.009) + (15.012), (I-302) + (5.009) + (15.016), (I-302) + (5.009) + (15.025), (I-302) + (5.009) + (15.027), (I-302) + (5.009) + (15.047), (I-302) + (5.009) + (15.063), (I-302) + (5.009) + (15.064),
(I-302) + (5.010) + (9.001), (I-302) + (5.010) + (9.002), (I-302) + (5.010) + (9.003), (I-302) + (5.010) + (9.004), (I-302) + (5.010) + (9.005), (I-302) + (5.010) + (9.006), (I-302) + (5.010) + (9.007), (I-302) + (5.010) + (9.008), (I-302) + (5.010) + (9.009), (I-302) + (5.010) + (15.012), (I-302) + (5.010) + (15.016), (I-302) + (5.010) + (15.025), (I-302) + (5.010) + (15.027), (I-302) + (5.010) + (15.047), (I-302) + (5.010) + (15.063), (I-302) + (5.010) + (15.064),
(I-302) + (5.011) + (9.001), (I-302) + (5.011) + (9.002), (I-302) + (5.011) + (9.003), (I-302) + (5.011) + (9.004), (I-302) + (5.011) + (9.005), (I-302) + (5.011) + (9.006), (I-302) + (5.011) + (9.007), (I-302) + (5.011) + (9.008), (I-302) + (5.011) + (9.009), (I-302) + (5.011) + (15.012), (I-302) + (5.011) + (15.016), (I-302) + (5.011) + (15.025), (I-302) + (5.011) + (15.027), (I-302) + (5.011) + (15.047), (I-302) + (5.011) + (15.063), (I-302) + (5.011) + (15.064),
(I-302) + (5.012) + (9.001), (I-302) + (5.012) + (9.002), (I-302) + (5.012) + (9.003), (I-302) + (5.012) + (9.004), (I-302) + (5.012) + (9.005), (I-302) + (5.012) + (9.006), (I-302) + (5.012) + (9.007), (I-302) + (5.012) + (9.008), (I-302) + (5.012) + (9.009), (I-302) + (5.012) + (15.012), (I-302) + (5.012) + (15.016), (I-302) + (5.012) + (15.025), (I-302) + (5.012) + (15.027), (I-302) + (5.012) + (15.047), (I-302) + (5.012) + (15.063), (I-302) + (5.012) + (15.064),
(I-302) + (5.013) + (9.001), (I-302) + (5.013) + (9.002), (I-302) + (5.013) + (9.003), (I-302) + (5.013) + (9.004), (I-302) + (5.013) + (9.005), (I-302) + (5.013) + (9.006), (I-302) + (5.013) + (9.007), (I-302) + (5.013) + (9.008), (I-302) + (5.013) + (9.009), (I-302) + (5.013) + (15.012), (I-302) + (5.013) + (15.016), (I-302) + (5.013) + (15.025), (I-302) + (5.013) + (15.027), (I-302) + (5.013) + (15.047), (I-302) + (5.013) + (15.063), (I-302) + (5.013) + (15.064),
(I-302) + (5.014) + (9.001), (I-302) + (5.014) + (9.002), (I-302) + (5.014) + (9.003), (I-302) + (5.014) + (9.004), (I-302) + (5.014) + (9.005), (I-302) + (5.014) + (9.006), (I-302) + (5.014) + (9.007), (I-302) + (5.014) + (9.008), (I-302) + (5.014) + (9.009), (I-302) + (5.014) + (15.012), (I-302) + (5.014) + (15.016), (I-302) + (5.014) + (15.025), (I-302) + (5.014) + (15.027), (I-302) + (5.014) + (15.047), (I-302) + (5.014) + (15.063), (I-302) + (5.014) + (15.064),
(I-302) + (5.015) + (9.001), (I-302) + (5.015) + (9.002), (I-302) + (5.015) + (9.003), (I-302) + (5.015) + (9.004), (I-302) + (5.015) + (9.005), (I-302) + (5.015) + (9.006), (I-302) + (5.015) + (9.007), (I-302) + (5.015) + (9.008), (I-302) + (5.015) + (9.009), (I-302) + (5.015) + (15.012), (I-302) + (5.015) + (15.016), (I-302) + (5.015) + (15.025), (I-302) + (5.015) + (15.027), (I-302) + (5.015) + (15.047), (I-302) + (5.015) + (15.063), (I-302) + (5.015) + (15.064),
(I-302) + (5.016) + (9.001), (I-302) + (5.016) + (9.002), (I-302) + (5.016) + (9.003), (I-302) + (5.016) + (9.004), (I-302) + (5.016) + (9.005), (I-302) + (5.016) + (9.006), (I-302) + (5.016) + (9.007), (I-302) + (5.016) + (9.008), (I-302) + (5.016) + (9.009), (I-302) + (5.016) + (15.012), (I-302) + (5.016) + (15.016), (I-302) + (5.016) + (15.025), (I-302) + (5.016) + (15.027), (I-302) + (5.016) + (15.047), (I-302) + (5.016) + (15.063), (I-302) + (5.016) + (15.064),
(I-302) + (5.017) + (9.001), (I-302) + (5.017) + (9.002), (I-302) + (5.017) + (9.003), (I-302) + (5.017) + (9.004), (I-302) + (5.017) + (9.005), (I-302) + (5.017) + (9.006), (I-302) + (5.017) + (9.007), (I-302) + (5.017) + (9.008), (I-302) + (5.017) + (9.009), (I-302) + (5.017) + (15.012), (I-302) + (5.017) + (15.016), (I-302) + (5.017) + (15.025), (I-302) + (5.017) + (15.027), (I-302) + (5.017) + (15.047), (I-302) + (5.017) + (15.063), (I-302) + (5.017) + (15.064),
(I-302) + (5.018) + (9.001), (I-302) + (5.018) + (9.002), (I-302) + (5.018) + (9.003), (I-302) + (5.018) + (9.004), (I-302) + (5.018) + (9.005), (I-302) + (5.018) + (9.006), (I-302) + (5.018) + (9.007), (I-302) + (5.018) + (9.008), (I-302) + (5.018) + (9.009), (I-302) + (5.018) + (15.012), (I-302) + (5.018) + (15.016), (I-302) + (5.018) + (15.025), (I-302) + (5.018) + (15.027), (I-302) + (5.018) + (15.047), (I-302) + (5.018) + (15.063), (I-302) + (5.018) + (15.064),
(I-302) + (5.019) + (9.001), (I-302) + (5.019) + (9.002), (I-302) + (5.019) + (9.003), (I-302) + (5.019) + (9.004), (I-302) + (5.019) + (9.005), (I-302) + (5.019) + (9.006), (I-302) + (5.019) + (9.007), (I-302) + (5.019) + (9.008), (I-302) + (5.019) + (9.009), (I-302) + (5.019) + (15.012), (I-302) + (5.019) + (15.016), (I-302) + (5.019) + (15.025), (I-302) + (5.019) + (15.027), (I-302) + (5.019) + (15.047), (I-302) + (5.019) + (15.063), (I-302) + (5.019) + (15.064),
(I-302) + (5.020) + (9.001), (I-302) + (5.020) + (9.002), (I-302) + (5.020) + (9.003), (I-302) + (5.020) + (9.004), (I-302) + (5.020) + (9.005), (I-302) + (5.020) + (9.006), (I-302) + (5.020) + (9.007), (I-302) + (5.020) + (9.008), (I-302) + (5.020) + (9.009), (I-302) + (5.020) + (15.012), (I-302) + (5.020) + (15.016), (I-302) + (5.020) + (15.025), (I-302) + (5.020) + (15.027), (I-302) + (5.020) + (15.047), (I-302) + (5.020) + (15.063), (I-302) + (5.020) + (15.064),
(I-302) + (5.021) + (9.001), (I-302) + (5.021) + (9.002), (I-302) + (5.021) + (9.003), (I-302) + (5.021) + (9.004), (I-302) + (5.021) + (9.005), (I-302) + (5.021) + (9.006), (I-302) + (5.021) + (9.007), (I-302) + (5.021) + (9.008), (I-302) + (5.021) + (9.009), (I-302) + (5.021) + (15.012), (I-302) + (5.021) + (15.016), (I-302) + (5.021) + (15.025), (I-302) + (5.021) + (15.027), (I-302) + (5.021) + (15.047), (I-302) + (5.021) + (15.063), (I-302) + (5.021) + (15.064),
(I-302) + (5.022) + (9.001), (I-302) + (5.022) + (9.002), (I-302) + (5.022) + (9.003), (I-302) + (5.022) + (9.004), (I-302) + (5.022) + (9.005), (I-302) + (5.022) + (9.006), (I-302) + (5.022) + (9.007), (I-302) + (5.022) + (9.008), (I-302) + (5.022) + (9.009), (I-302) + (5.022) + (15.012), (I-302) + (5.022) + (15.016), (I-302) + (5.022) + (15.025), (I-302) + (5.022) + (15.027), (I-302) + (5.022) + (15.047), (I-302) + (5.022) + (15.063), (I-302) + (5.022) + (15.064),
(I-302) + (5.023) + (9.001), (I-302) + (5.023) + (9.002), (I-302) + (5.023) + (9.003), (I-302) + (5.023) + (9.004), (I-302) + (5.023) + (9.005), (I-302) + (5.023) + (9.006), (I-302) + (5.023) + (9.007), (I-302) + (5.023) + (9.008), (I-302) + (5.023) + (9.009), (I-302) + (5.023) + (15.012), (I-302) + (5.023) + (15.016), (I-302) + (5.023) + (15.025), (I-302) + (5.023) + (15.027), (I-302) + (5.023) + (15.047), (I-302) + (5.023) + (15.063), (I-302) + (5.023) + (15.064).
2종의 화합물 (B)가 본 발명에 따른 조합물에 존재하는 경우, 보다 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G1-C1)으로부터 선택된다:
(I-052) + (1.001) + (1.002), (I-052) + (1.001) + (1.003), (I-052) + (1.001) + (1.004), (I-052) + (1.001) + (1.005), (I-052) + (1.001) + (1.006), (I-052) + (1.001) + (1.007), (I-052) + (1.001) + (1.010), (I-052) + (1.001) + (1.011), (I-052) + (1.001) + (1.012), (I-052) + (1.001) + (1.013), (I-052) + (1.001) + (1.017), (I-052) + (1.001) + (1.018), (I-052) + (1.001) + (1.020), (I-052) + (1.001) + (1.021), (I-052) + (1.001) + (1.026), (I-052) + (1.001) + (1.027), (I-052) + (1.001) + (1.055), (I-052) + (1.001) + (1.059), (I-052) + (1.001) + (1.092), (I-052) + (1.001) + (2.001), (I-052) + (1.001) + (2.002), (I-052) + (1.001) + (2.003), (I-052) + (1.001) + (2.005), (I-052) + (1.001) + (2.007), (I-052) + (1.001) + (2.009), (I-052) + (1.001) + (2.010), (I-052) + (1.001) + (2.011), (I-052) + (1.001) + (2.012), (I-052) + (1.001) + (2.013), (I-052) + (1.001) + (2.014), (I-052) + (1.001) + (2.015), (I-052) + (1.001) + (2.016), (I-052) + (1.001) + (2.017), (I-052) + (1.001) + (2.018), (I-052) + (1.001) + (2.019), (I-052) + (1.001) + (2.021), (I-052) + (1.001) + (2.028), (I-052) + (1.001) + (2.030), (I-052) + (1.001) + (2.038), (I-052) + (1.001) + (3.003), (I-052) + (1.001) + (3.007), (I-052) + (1.001) + (3.012), (I-052) + (1.001) + (3.013), (I-052) + (1.001) + (3.016), (I-052) + (1.001) + (3.017), (I-052) + (1.001) + (3.020), (I-052) + (1.001) + (3.025), (I-052) + (1.001) + (3.026), (I-052) + (1.001) + (3.030), (I-052) + (1.001) + (3.031), (I-052) + (1.001) + (5.003), (I-052) + (1.001) + (5.004), (I-052) + (1.001) + (5.005), (I-052) + (1.001) + (5.008), (I-052) + (1.001) + (5.009), (I-052) + (1.001) + (5.011), (I-052) + (1.001) + (5.012), (I-052) + (1.001) + (5.013), (I-052) + (1.001) + (5.015), (I-052) + (1.001) + (5.018), (I-052) + (1.001) + (5.019), (I-052) + (1.001) + (6.002), (I-052) + (1.001) + (7.001), (I-052) + (1.001) + (7.005), (I-052) + (1.001) + (9.002), (I-052) + (1.001) + (9.004), (I-052) + (1.001) + (14.001), (I-052) + (1.001) + (14.002), (I-052) + (1.001) + (15.008), (I-052) + (1.001) + (15.011), (I-052) + (1.001) + (15.012), (I-052) + (1.001) + (15.016), (I-052) + (1.001) + (15.025), (I-052) + (1.001) + (15.027), (I-052) + (1.001) + (15.047), (I-052) + (1.001) + (15.063), (I-052) + (1.001) + (15.064), (I-052) + (1.001) + (16.001), (I-052) + (1.001) + (16.005), (I-052) + (1.001) + (17.001), (I-052) + (1.001) + (17.002), (I-052) + (1.001) + (17.003), (I-052) + (1.001) + (17.008), (I-052) + (1.001) + (18.001),
(I-052) + (1.002) + (1.001), (I-052) + (1.002) + (1.003), (I-052) + (1.002) + (1.004), (I-052) + (1.002) + (1.005), (I-052) + (1.002) + (1.006), (I-052) + (1.002) + (1.007), (I-052) + (1.002) + (1.010), (I-052) + (1.002) + (1.011), (I-052) + (1.002) + (1.012), (I-052) + (1.002) + (1.013), (I-052) + (1.002) + (1.017), (I-052) + (1.002) + (1.018), (I-052) + (1.002) + (1.020), (I-052) + (1.002) + (1.021), (I-052) + (1.002) + (1.026), (I-052) + (1.002) + (1.027), (I-052) + (1.002) + (1.055), (I-052) + (1.002) + (1.059), (I-052) + (1.002) + (1.092), (I-052) + (1.002) + (2.001), (I-052) + (1.002) + (2.002), (I-052) + (1.002) + (2.003), (I-052) + (1.002) + (2.005), (I-052) + (1.002) + (2.007), (I-052) + (1.002) + (2.009), (I-052) + (1.002) + (2.010), (I-052) + (1.002) + (2.011), (I-052) + (1.002) + (2.012), (I-052) + (1.002) + (2.013), (I-052) + (1.002) + (2.014), (I-052) + (1.002) + (2.015), (I-052) + (1.002) + (2.016), (I-052) + (1.002) + (2.017), (I-052) + (1.002) + (2.018), (I-052) + (1.002) + (2.019), (I-052) + (1.002) + (2.021), (I-052) + (1.002) + (2.028), (I-052) + (1.002) + (2.030), (I-052) + (1.002) + (2.038), (I-052) + (1.002) + (3.003), (I-052) + (1.002) + (3.007), (I-052) + (1.002) + (3.012), (I-052) + (1.002) + (3.013), (I-052) + (1.002) + (3.016), (I-052) + (1.002) + (3.017), (I-052) + (1.002) + (3.020), (I-052) + (1.002) + (3.025), (I-052) + (1.002) + (3.026), (I-052) + (1.002) + (3.030), (I-052) + (1.002) + (3.031), (I-052) + (1.002) + (5.003), (I-052) + (1.002) + (5.004), (I-052) + (1.002) + (5.005), (I-052) + (1.002) + (5.008), (I-052) + (1.002) + (5.009), (I-052) + (1.002) + (5.011), (I-052) + (1.002) + (5.012), (I-052) + (1.002) + (5.013), (I-052) + (1.002) + (5.015), (I-052) + (1.002) + (5.018), (I-052) + (1.002) + (5.019), (I-052) + (1.002) + (6.002), (I-052) + (1.002) + (7.001), (I-052) + (1.002) + (7.005), (I-052) + (1.002) + (9.002), (I-052) + (1.002) + (9.004), (I-052) + (1.002) + (14.001), (I-052) + (1.002) + (14.002), (I-052) + (1.002) + (15.008), (I-052) + (1.002) + (15.011), (I-052) + (1.002) + (15.012), (I-052) + (1.002) + (15.016), (I-052) + (1.002) + (15.025), (I-052) + (1.002) + (15.027), (I-052) + (1.002) + (15.047), (I-052) + (1.002) + (15.063), (I-052) + (1.002) + (15.064), (I-052) + (1.002) + (16.001), (I-052) + (1.002) + (16.005), (I-052) + (1.002) + (17.001), (I-052) + (1.002) + (17.002), (I-052) + (1.002) + (17.003), (I-052) + (1.002) + (17.008), (I-052) + (1.002) + (18.001),
(I-052) + (1.003) + (1.001), (I-052) + (1.003) + (1.002), (I-052) + (1.003) + (1.004), (I-052) + (1.003) + (1.005), (I-052) + (1.003) + (1.006), (I-052) + (1.003) + (1.007), (I-052) + (1.003) + (1.010), (I-052) + (1.003) + (1.011), (I-052) + (1.003) + (1.012), (I-052) + (1.003) + (1.013), (I-052) + (1.003) + (1.017), (I-052) + (1.003) + (1.018), (I-052) + (1.003) + (1.020), (I-052) + (1.003) + (1.021), (I-052) + (1.003) + (1.026), (I-052) + (1.003) + (1.027), (I-052) + (1.003) + (1.055), (I-052) + (1.003) + (1.059), (I-052) + (1.003) + (1.092), (I-052) + (1.003) + (2.001), (I-052) + (1.003) + (2.002), (I-052) + (1.003) + (2.003), (I-052) + (1.003) + (2.005), (I-052) + (1.003) + (2.007), (I-052) + (1.003) + (2.009), (I-052) + (1.003) + (2.010), (I-052) + (1.003) + (2.011), (I-052) + (1.003) + (2.012), (I-052) + (1.003) + (2.013), (I-052) + (1.003) + (2.014), (I-052) + (1.003) + (2.015), (I-052) + (1.003) + (2.016), (I-052) + (1.003) + (2.017), (I-052) + (1.003) + (2.018), (I-052) + (1.003) + (2.019), (I-052) + (1.003) + (2.021), (I-052) + (1.003) + (2.028), (I-052) + (1.003) + (2.030), (I-052) + (1.003) + (2.038), (I-052) + (1.003) + (3.003), (I-052) + (1.003) + (3.007), (I-052) + (1.003) + (3.012), (I-052) + (1.003) + (3.013), (I-052) + (1.003) + (3.016), (I-052) + (1.003) + (3.017), (I-052) + (1.003) + (3.020), (I-052) + (1.003) + (3.025), (I-052) + (1.003) + (3.026), (I-052) + (1.003) + (3.030), (I-052) + (1.003) + (3.031), (I-052) + (1.003) + (5.003), (I-052) + (1.003) + (5.004), (I-052) + (1.003) + (5.005), (I-052) + (1.003) + (5.008), (I-052) + (1.003) + (5.009), (I-052) + (1.003) + (5.011), (I-052) + (1.003) + (5.012), (I-052) + (1.003) + (5.013), (I-052) + (1.003) + (5.015), (I-052) + (1.003) + (5.018), (I-052) + (1.003) + (5.019), (I-052) + (1.003) + (6.002), (I-052) + (1.003) + (7.001), (I-052) + (1.003) + (7.005), (I-052) + (1.003) + (9.002), (I-052) + (1.003) + (9.004), (I-052) + (1.003) + (14.001), (I-052) + (1.003) + (14.002), (I-052) + (1.003) + (15.008), (I-052) + (1.003) + (15.011), (I-052) + (1.003) + (15.012), (I-052) + (1.003) + (15.016), (I-052) + (1.003) + (15.025), (I-052) + (1.003) + (15.027), (I-052) + (1.003) + (15.047), (I-052) + (1.003) + (15.063), (I-052) + (1.003) + (15.064), (I-052) + (1.003) + (16.001), (I-052) + (1.003) + (16.005), (I-052) + (1.003) + (17.001), (I-052) + (1.003) + (17.002), (I-052) + (1.003) + (17.003), (I-052) + (1.003) + (17.008), (I-052) + (1.003) + (18.001),
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(I-052) + (3.017) + (3.025), (I-052) + (3.017) + (3.030), (I-052) + (3.017) + (3.031), (I-052) + (3.017) + (5.003), (I-052) + (3.017) + (5.004), (I-052) + (3.017) + (5.005), (I-052) + (3.017) + (5.008), (I-052) + (3.017) + (5.009), (I-052) + (3.017) + (5.011), (I-052) + (3.017) + (5.012), (I-052) + (3.017) + (5.013), (I-052) + (3.017) + (5.015), (I-052) + (3.017) + (5.018), (I-052) + (3.017) + (5.019), (I-052) + (3.017) + (6.002), (I-052) + (3.017) + (7.001), (I-052) + (3.017) + (7.005), (I-052) + (3.017) + (9.002), (I-052) + (3.017) + (9.004), (I-052) + (3.017) + (14.001), (I-052) + (3.017) + (14.002), (I-052) + (3.017) + (15.008), (I-052) + (3.017) + (15.011), (I-052) + (3.017) + (15.012), (I-052) + (3.017) + (15.016), (I-052) + (3.017) + (15.025), (I-052) + (3.017) + (15.027), (I-052) + (3.017) + (15.047), (I-052) + (3.017) + (15.063), (I-052) + (3.017) + (15.064), (I-052) + (3.017) + (16.001), (I-052) + (3.017) + (16.005), (I-052) + (3.017) + (17.001), (I-052) + (3.017) + (17.002), (I-052) + (3.017) + (17.003), (I-052) + (3.017) + (17.008), (I-052) + (3.017) + (18.001),
(I-052) + (3.020) + (3.025), (I-052) + (3.020) + (3.030), (I-052) + (3.020) + (3.031), (I-052) + (3.020) + (5.003), (I-052) + (3.020) + (5.004), (I-052) + (3.020) + (5.005), (I-052) + (3.020) + (5.008), (I-052) + (3.020) + (5.009), (I-052) + (3.020) + (5.011), (I-052) + (3.020) + (5.012), (I-052) + (3.020) + (5.013), (I-052) + (3.020) + (5.015), (I-052) + (3.020) + (5.018), (I-052) + (3.020) + (5.019), (I-052) + (3.020) + (6.002), (I-052) + (3.020) + (7.001), (I-052) + (3.020) + (7.005), (I-052) + (3.020) + (9.002), (I-052) + (3.020) + (9.004), (I-052) + (3.020) + (14.001), (I-052) + (3.020) + (14.002), (I-052) + (3.020) + (15.008), (I-052) + (3.020) + (15.011), (I-052) + (3.020) + (15.012), (I-052) + (3.020) + (15.016), (I-052) + (3.020) + (15.025), (I-052) + (3.020) + (15.027), (I-052) + (3.020) + (15.047), (I-052) + (3.020) + (15.063), (I-052) + (3.020) + (15.064), (I-052) + (3.020) + (16.001), (I-052) + (3.020) + (16.005), (I-052) + (3.020) + (17.001), (I-052) + (3.020) + (17.002), (I-052) + (3.020) + (17.003), (I-052) + (3.020) + (17.008), (I-052) + (3.020) + (18.001),
(I-052) + (3.025) + (3.030), (I-052) + (3.025) + (3.031), (I-052) + (3.025) + (5.003), (I-052) + (3.025) + (5.004), (I-052) + (3.025) + (5.005), (I-052) + (3.025) + (5.008), (I-052) + (3.025) + (5.009), (I-052) + (3.025) + (5.011), (I-052) + (3.025) + (5.012), (I-052) + (3.025) + (5.013), (I-052) + (3.025) + (5.015), (I-052) + (3.025) + (5.018), (I-052) + (3.025) + (5.019), (I-052) + (3.025) + (6.002), (I-052) + (3.025) + (7.001), (I-052) + (3.025) + (7.005), (I-052) + (3.025) + (9.002), (I-052) + (3.025) + (9.004), (I-052) + (3.025) + (14.001), (I-052) + (3.025) + (14.002), (I-052) + (3.025) + (15.008), (I-052) + (3.025) + (15.011), (I-052) + (3.025) + (15.012), (I-052) + (3.025) + (15.016), (I-052) + (3.025) + (15.025), (I-052) + (3.025) + (15.027), (I-052) + (3.025) + (15.047), (I-052) + (3.025) + (15.063), (I-052) + (3.025) + (15.064), (I-052) + (3.025) + (16.001), (I-052) + (3.025) + (16.005), (I-052) + (3.025) + (17.001), (I-052) + (3.025) + (17.002), (I-052) + (3.025) + (17.003), (I-052) + (3.025) + (17.008), (I-052) + (3.025) + (18.001),
(I-052) + (3.026) + (3.025), (I-052) + (3.026) + (3.030), (I-052) + (3.026) + (3.031), (I-052) + (3.026) + (5.003), (I-052) + (3.026) + (5.004), (I-052) + (3.026) + (5.005), (I-052) + (3.026) + (5.008), (I-052) + (3.026) + (5.009), (I-052) + (3.026) + (5.011), (I-052) + (3.026) + (5.012), (I-052) + (3.026) + (5.013), (I-052) + (3.026) + (5.015), (I-052) + (3.026) + (5.018), (I-052) + (3.026) + (5.019), (I-052) + (3.026) + (6.002), (I-052) + (3.026) + (7.001), (I-052) + (3.026) + (7.005), (I-052) + (3.026) + (9.002), (I-052) + (3.026) + (9.004), (I-052) + (3.026) + (14.001), (I-052) + (3.026) + (14.002), (I-052) + (3.026) + (15.008), (I-052) + (3.026) + (15.011), (I-052) + (3.026) + (15.012), (I-052) + (3.026) + (15.016), (I-052) + (3.026) + (15.025), (I-052) + (3.026) + (15.027), (I-052) + (3.026) + (15.047), (I-052) + (3.026) + (15.063), (I-052) + (3.026) + (15.064), (I-052) + (3.026) + (16.001), (I-052) + (3.026) + (16.005), (I-052) + (3.026) + (17.001), (I-052) + (3.026) + (17.002), (I-052) + (3.026) + (17.003), (I-052) + (3.026) + (17.008), (I-052) + (3.026) + (18.001),
(I-052) + (3.030) + (3.025), (I-052) + (3.030) + (3.031), (I-052) + (3.030) + (5.003), (I-052) + (3.030) + (5.004), (I-052) + (3.030) + (5.005), (I-052) + (3.030) + (5.008), (I-052) + (3.030) + (5.009), (I-052) + (3.030) + (5.011), (I-052) + (3.030) + (5.012), (I-052) + (3.030) + (5.013), (I-052) + (3.030) + (5.015), (I-052) + (3.030) + (5.018), (I-052) + (3.030) + (5.019), (I-052) + (3.030) + (6.002), (I-052) + (3.030) + (7.001), (I-052) + (3.030) + (7.005), (I-052) + (3.030) + (9.002), (I-052) + (3.030) + (9.004), (I-052) + (3.030) + (14.001), (I-052) + (3.030) + (14.002), (I-052) + (3.030) + (15.008), (I-052) + (3.030) + (15.011), (I-052) + (3.030) + (15.012), (I-052) + (3.030) + (15.016), (I-052) + (3.030) + (15.025), (I-052) + (3.030) + (15.027), (I-052) + (3.030) + (15.047), (I-052) + (3.030) + (15.063), (I-052) + (3.030) + (15.064), (I-052) + (3.030) + (16.001), (I-052) + (3.030) + (16.005), (I-052) + (3.030) + (17.001), (I-052) + (3.030) + (17.002), (I-052) + (3.030) + (17.003), (I-052) + (3.030) + (17.008), (I-052) + (3.030) + (18.001),
(I-052) + (3.031) + (3.025), (I-052) + (3.031) + (3.030), (I-052) + (3.031) + (5.003), (I-052) + (3.031) + (5.004), (I-052) + (3.031) + (5.005), (I-052) + (3.031) + (5.008), (I-052) + (3.031) + (5.009), (I-052) + (3.031) + (5.011), (I-052) + (3.031) + (5.012), (I-052) + (3.031) + (5.013), (I-052) + (3.031) + (5.015), (I-052) + (3.031) + (5.018), (I-052) + (3.031) + (5.019), (I-052) + (3.031) + (6.002), (I-052) + (3.031) + (7.001), (I-052) + (3.031) + (7.005), (I-052) + (3.031) + (9.002), (I-052) + (3.031) + (9.004), (I-052) + (3.031) + (14.001), (I-052) + (3.031) + (14.002), (I-052) + (3.031) + (15.008), (I-052) + (3.031) + (15.011), (I-052) + (3.031) + (15.012), (I-052) + (3.031) + (15.016), (I-052) + (3.031) + (15.025), (I-052) + (3.031) + (15.027), (I-052) + (3.031) + (15.047), (I-052) + (3.031) + (15.063), (I-052) + (3.031) + (15.064), (I-052) + (3.031) + (16.001), (I-052) + (3.031) + (16.005), (I-052) + (3.031) + (17.001), (I-052) + (3.031) + (17.002), (I-052) + (3.031) + (17.003), (I-052) + (3.031) + (17.008), (I-052) + (3.031) + (18.001),
(I-052) + (5.003) + (9.002), (I-052) + (5.003) + (15.012), (I-052) + (5.003) + (15.016), (I-052) + (5.003) + (15.025), (I-052) + (5.003) + (15.027), (I-052) + (5.003) + (15.047), (I-052) + (5.003) + (15.063), (I-052) + (5.003) + (15.064),
(I-052) + (5.004) + (9.002), (I-052) + (5.004) + (15.012), (I-052) + (5.004) + (15.016), (I-052) + (5.004) + (15.025), (I-052) + (5.004) + (15.027), (I-052) + (5.004) + (15.047), (I-052) + (5.004) + (15.063), (I-052) + (5.004) + (15.064),
(I-052) + (5.005) + (9.002), (I-052) + (5.005) + (15.012), (I-052) + (5.005) + (15.016), (I-052) + (5.005) + (15.025), (I-052) + (5.005) + (15.027), (I-052) + (5.005) + (15.047), (I-052) + (5.005) + (15.063), (I-052) + (5.005) + (15.064),
(I-052) + (5.008) + (9.002), (I-052) + (5.008) + (15.012), (I-052) + (5.008) + (15.016), (I-052) + (5.008) + (15.025), (I-052) + (5.008) + (15.027), (I-052) + (5.008) + (15.047), (I-052) + (5.008) + (15.063), (I-052) + (5.008) + (15.064),
(I-052) + (5.009) + (9.002), (I-052) + (5.009) + (15.012), (I-052) + (5.009) + (15.016), (I-052) + (5.009) + (15.025), (I-052) + (5.009) + (15.027), (I-052) + (5.009) + (15.047), (I-052) + (5.009) + (15.063), (I-052) + (5.009) + (15.064),
(I-052) + (5.011) + (9.002), (I-052) + (5.011) + (15.012), (I-052) + (5.011) + (15.016), (I-052) + (5.011) + (15.025), (I-052) + (5.011) + (15.027), (I-052) + (5.011) + (15.047), (I-052) + (5.011) + (15.063), (I-052) + (5.011) + (15.064),
(I-052) + (5.012) + (9.002), (I-052) + (5.012) + (15.012), (I-052) + (5.012) + (15.016), (I-052) + (5.012) + (15.025), (I-052) + (5.012) + (15.027), (I-052) + (5.012) + (15.047), (I-052) + (5.012) + (15.063), (I-052) + (5.012) + (15.064),
(I-052) + (5.013) + (9.002), (I-052) + (5.013) + (15.012), (I-052) + (5.013) + (15.016), (I-052) + (5.013) + (15.025), (I-052) + (5.013) + (15.027), (I-052) + (5.013) + (15.047), (I-052) + (5.013) + (15.063), (I-052) + (5.013) + (15.064),
(I-052) + (5.015) + (9.002), (I-052) + (5.015) + (15.012), (I-052) + (5.015) + (15.016), (I-052) + (5.015) + (15.025), (I-052) + (5.015) + (15.027), (I-052) + (5.015) + (15.047), (I-052) + (5.015) + (15.063), (I-052) + (5.015) + (15.064),
(I-052) + (5.018) + (9.002), (I-052) + (5.018) + (15.012), (I-052) + (5.018) + (15.016), (I-052) + (5.018) + (15.025), (I-052) + (5.018) + (15.027), (I-052) + (5.018) + (15.047), (I-052) + (5.018) + (15.063), (I-052) + (5.018) + (15.064),
(I-052) + (5.019) + (9.002), (I-052) + (5.019) + (15.012), (I-052) + (5.019) + (15.016), (I-052) + (5.019) + (15.025), (I-052) + (5.019) + (15.027), (I-052) + (5.019) + (15.047), (I-052) + (5.019) + (15.063), (I-052) + (5.019) + (15.064).
2종의 화합물 (B)가 본 발명에 따른 조합물에 존재하는 경우, 보다 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G3-C1)으로부터 선택된다:
(I-300) + (1.001) + (1.002), (I-300) + (1.001) + (1.003), (I-300) + (1.001) + (1.004), (I-300) + (1.001) + (1.005), (I-300) + (1.001) + (1.006), (I-300) + (1.001) + (1.007), (I-300) + (1.001) + (1.010), (I-300) + (1.001) + (1.011), (I-300) + (1.001) + (1.012), (I-300) + (1.001) + (1.013), (I-300) + (1.001) + (1.017), (I-300) + (1.001) + (1.018), (I-300) + (1.001) + (1.020), (I-300) + (1.001) + (1.021), (I-300) + (1.001) + (1.026), (I-300) + (1.001) + (1.027), (I-300) + (1.001) + (1.055), (I-300) + (1.001) + (1.059), (I-300) + (1.001) + (1.092), (I-300) + (1.001) + (2.001), (I-300) + (1.001) + (2.002), (I-300) + (1.001) + (2.003), (I-300) + (1.001) + (2.005), (I-300) + (1.001) + (2.007), (I-300) + (1.001) + (2.009), (I-300) + (1.001) + (2.010), (I-300) + (1.001) + (2.011), (I-300) + (1.001) + (2.012), (I-300) + (1.001) + (2.013), (I-300) + (1.001) + (2.014), (I-300) + (1.001) + (2.015), (I-300) + (1.001) + (2.016), (I-300) + (1.001) + (2.017), (I-300) + (1.001) + (2.018), (I-300) + (1.001) + (2.019), (I-300) + (1.001) + (2.021), (I-300) + (1.001) + (2.028), (I-300) + (1.001) + (2.030), (I-300) + (1.001) + (2.038), (I-300) + (1.001) + (3.003), (I-300) + (1.001) + (3.007), (I-300) + (1.001) + (3.012), (I-300) + (1.001) + (3.013), (I-300) + (1.001) + (3.016), (I-300) + (1.001) + (3.017), (I-300) + (1.001) + (3.020), (I-300) + (1.001) + (3.025), (I-300) + (1.001) + (3.026), (I-300) + (1.001) + (3.030), (I-300) + (1.001) + (3.031), (I-300) + (1.001) + (5.003), (I-300) + (1.001) + (5.004), (I-300) + (1.001) + (5.005), (I-300) + (1.001) + (5.008), (I-300) + (1.001) + (5.009), (I-300) + (1.001) + (5.011), (I-300) + (1.001) + (5.012), (I-300) + (1.001) + (5.013), (I-300) + (1.001) + (5.015), (I-300) + (1.001) + (5.018), (I-300) + (1.001) + (5.019), (I-300) + (1.001) + (6.002), (I-300) + (1.001) + (7.001), (I-300) + (1.001) + (7.005), (I-300) + (1.001) + (9.002), (I-300) + (1.001) + (9.004), (I-300) + (1.001) + (14.001), (I-300) + (1.001) + (14.002), (I-300) + (1.001) + (15.008), (I-300) + (1.001) + (15.011), (I-300) + (1.001) + (15.012), (I-300) + (1.001) + (15.016), (I-300) + (1.001) + (15.025), (I-300) + (1.001) + (15.027), (I-300) + (1.001) + (15.047), (I-300) + (1.001) + (15.063), (I-300) + (1.001) + (15.064), (I-300) + (1.001) + (16.001), (I-300) + (1.001) + (16.005), (I-300) + (1.001) + (17.001), (I-300) + (1.001) + (17.002), (I-300) + (1.001) + (17.003), (I-300) + (1.001) + (17.008), (I-300) + (1.001) + (18.001),
(I-300) + (1.002) + (1.001), (I-300) + (1.002) + (1.003), (I-300) + (1.002) + (1.004), (I-300) + (1.002) + (1.005), (I-300) + (1.002) + (1.006), (I-300) + (1.002) + (1.007), (I-300) + (1.002) + (1.010), (I-300) + (1.002) + (1.011), (I-300) + (1.002) + (1.012), (I-300) + (1.002) + (1.013), (I-300) + (1.002) + (1.017), (I-300) + (1.002) + (1.018), (I-300) + (1.002) + (1.020), (I-300) + (1.002) + (1.021), (I-300) + (1.002) + (1.026), (I-300) + (1.002) + (1.027), (I-300) + (1.002) + (1.055), (I-300) + (1.002) + (1.059), (I-300) + (1.002) + (1.092), (I-300) + (1.002) + (2.001), (I-300) + (1.002) + (2.002), (I-300) + (1.002) + (2.003), (I-300) + (1.002) + (2.005), (I-300) + (1.002) + (2.007), (I-300) + (1.002) + (2.009), (I-300) + (1.002) + (2.010), (I-300) + (1.002) + (2.011), (I-300) + (1.002) + (2.012), (I-300) + (1.002) + (2.013), (I-300) + (1.002) + (2.014), (I-300) + (1.002) + (2.015), (I-300) + (1.002) + (2.016), (I-300) + (1.002) + (2.017), (I-300) + (1.002) + (2.018), (I-300) + (1.002) + (2.019), (I-300) + (1.002) + (2.021), (I-300) + (1.002) + (2.028), (I-300) + (1.002) + (2.030), (I-300) + (1.002) + (2.038), (I-300) + (1.002) + (3.003), (I-300) + (1.002) + (3.007), (I-300) + (1.002) + (3.012), (I-300) + (1.002) + (3.013), (I-300) + (1.002) + (3.016), (I-300) + (1.002) + (3.017), (I-300) + (1.002) + (3.020), (I-300) + (1.002) + (3.025), (I-300) + (1.002) + (3.026), (I-300) + (1.002) + (3.030), (I-300) + (1.002) + (3.031), (I-300) + (1.002) + (5.003), (I-300) + (1.002) + (5.004), (I-300) + (1.002) + (5.005), (I-300) + (1.002) + (5.008), (I-300) + (1.002) + (5.009), (I-300) + (1.002) + (5.011), (I-300) + (1.002) + (5.012), (I-300) + (1.002) + (5.013), (I-300) + (1.002) + (5.015), (I-300) + (1.002) + (5.018), (I-300) + (1.002) + (5.019), (I-300) + (1.002) + (6.002), (I-300) + (1.002) + (7.001), (I-300) + (1.002) + (7.005), (I-300) + (1.002) + (9.002), (I-300) + (1.002) + (9.004), (I-300) + (1.002) + (14.001), (I-300) + (1.002) + (14.002), (I-300) + (1.002) + (15.008), (I-300) + (1.002) + (15.011), (I-300) + (1.002) + (15.012), (I-300) + (1.002) + (15.016), (I-300) + (1.002) + (15.025), (I-300) + (1.002) + (15.027), (I-300) + (1.002) + (15.047), (I-300) + (1.002) + (15.063), (I-300) + (1.002) + (15.064), (I-300) + (1.002) + (16.001), (I-300) + (1.002) + (16.005), (I-300) + (1.002) + (17.001), (I-300) + (1.002) + (17.002), (I-300) + (1.002) + (17.003), (I-300) + (1.002) + (17.008), (I-300) + (1.002) + (18.001),
(I-300) + (1.003) + (1.001), (I-300) + (1.003) + (1.002), (I-300) + (1.003) + (1.004), (I-300) + (1.003) + (1.005), (I-300) + (1.003) + (1.006), (I-300) + (1.003) + (1.007), (I-300) + (1.003) + (1.010), (I-300) + (1.003) + (1.011), (I-300) + (1.003) + (1.012), (I-300) + (1.003) + (1.013), (I-300) + (1.003) + (1.017), (I-300) + (1.003) + (1.018), (I-300) + (1.003) + (1.020), (I-300) + (1.003) + (1.021), (I-300) + (1.003) + (1.026), (I-300) + (1.003) + (1.027), (I-300) + (1.003) + (1.055), (I-300) + (1.003) + (1.059), (I-300) + (1.003) + (1.092), (I-300) + (1.003) + (2.001), (I-300) + (1.003) + (2.002), (I-300) + (1.003) + (2.003), (I-300) + (1.003) + (2.005), (I-300) + (1.003) + (2.007), (I-300) + (1.003) + (2.009), (I-300) + (1.003) + (2.010), (I-300) + (1.003) + (2.011), (I-300) + (1.003) + (2.012), (I-300) + (1.003) + (2.013), (I-300) + (1.003) + (2.014), (I-300) + (1.003) + (2.015), (I-300) + (1.003) + (2.016), (I-300) + (1.003) + (2.017), (I-300) + (1.003) + (2.018), (I-300) + (1.003) + (2.019), (I-300) + (1.003) + (2.021), (I-300) + (1.003) + (2.028), (I-300) + (1.003) + (2.030), (I-300) + (1.003) + (2.038), (I-300) + (1.003) + (3.003), (I-300) + (1.003) + (3.007), (I-300) + (1.003) + (3.012), (I-300) + (1.003) + (3.013), (I-300) + (1.003) + (3.016), (I-300) + (1.003) + (3.017), (I-300) + (1.003) + (3.020), (I-300) + (1.003) + (3.025), (I-300) + (1.003) + (3.026), (I-300) + (1.003) + (3.030), (I-300) + (1.003) + (3.031), (I-300) + (1.003) + (5.003), (I-300) + (1.003) + (5.004), (I-300) + (1.003) + (5.005), (I-300) + (1.003) + (5.008), (I-300) + (1.003) + (5.009), (I-300) + (1.003) + (5.011), (I-300) + (1.003) + (5.012), (I-300) + (1.003) + (5.013), (I-300) + (1.003) + (5.015), (I-300) + (1.003) + (5.018), (I-300) + (1.003) + (5.019), (I-300) + (1.003) + (6.002), (I-300) + (1.003) + (7.001), (I-300) + (1.003) + (7.005), (I-300) + (1.003) + (9.002), (I-300) + (1.003) + (9.004), (I-300) + (1.003) + (14.001), (I-300) + (1.003) + (14.002), (I-300) + (1.003) + (15.008), (I-300) + (1.003) + (15.011), (I-300) + (1.003) + (15.012), (I-300) + (1.003) + (15.016), (I-300) + (1.003) + (15.025), (I-300) + (1.003) + (15.027), (I-300) + (1.003) + (15.047), (I-300) + (1.003) + (15.063), (I-300) + (1.003) + (15.064), (I-300) + (1.003) + (16.001), (I-300) + (1.003) + (16.005), (I-300) + (1.003) + (17.001), (I-300) + (1.003) + (17.002), (I-300) + (1.003) + (17.003), (I-300) + (1.003) + (17.008), (I-300) + (1.003) + (18.001),
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(I-300) + (3.017) + (3.025), (I-300) + (3.017) + (3.030), (I-300) + (3.017) + (3.031), (I-300) + (3.017) + (5.003), (I-300) + (3.017) + (5.004), (I-300) + (3.017) + (5.005), (I-300) + (3.017) + (5.008), (I-300) + (3.017) + (5.009), (I-300) + (3.017) + (5.011), (I-300) + (3.017) + (5.012), (I-300) + (3.017) + (5.013), (I-300) + (3.017) + (5.015), (I-300) + (3.017) + (5.018), (I-300) + (3.017) + (5.019), (I-300) + (3.017) + (6.002), (I-300) + (3.017) + (7.001), (I-300) + (3.017) + (7.005), (I-300) + (3.017) + (9.002), (I-300) + (3.017) + (9.004), (I-300) + (3.017) + (14.001), (I-300) + (3.017) + (14.002), (I-300) + (3.017) + (15.008), (I-300) + (3.017) + (15.011), (I-300) + (3.017) + (15.012), (I-300) + (3.017) + (15.016), (I-300) + (3.017) + (15.025), (I-300) + (3.017) + (15.027), (I-300) + (3.017) + (15.047), (I-300) + (3.017) + (15.063), (I-300) + (3.017) + (15.064), (I-300) + (3.017) + (16.001), (I-300) + (3.017) + (16.005), (I-300) + (3.017) + (17.001), (I-300) + (3.017) + (17.002), (I-300) + (3.017) + (17.003), (I-300) + (3.017) + (17.008), (I-300) + (3.017) + (18.001),
(I-300) + (3.020) + (3.025), (I-300) + (3.020) + (3.030), (I-300) + (3.020) + (3.031), (I-300) + (3.020) + (5.003), (I-300) + (3.020) + (5.004), (I-300) + (3.020) + (5.005), (I-300) + (3.020) + (5.008), (I-300) + (3.020) + (5.009), (I-300) + (3.020) + (5.011), (I-300) + (3.020) + (5.012), (I-300) + (3.020) + (5.013), (I-300) + (3.020) + (5.015), (I-300) + (3.020) + (5.018), (I-300) + (3.020) + (5.019), (I-300) + (3.020) + (6.002), (I-300) + (3.020) + (7.001), (I-300) + (3.020) + (7.005), (I-300) + (3.020) + (9.002), (I-300) + (3.020) + (9.004), (I-300) + (3.020) + (14.001), (I-300) + (3.020) + (14.002), (I-300) + (3.020) + (15.008), (I-300) + (3.020) + (15.011), (I-300) + (3.020) + (15.012), (I-300) + (3.020) + (15.016), (I-300) + (3.020) + (15.025), (I-300) + (3.020) + (15.027), (I-300) + (3.020) + (15.047), (I-300) + (3.020) + (15.063), (I-300) + (3.020) + (15.064), (I-300) + (3.020) + (16.001), (I-300) + (3.020) + (16.005), (I-300) + (3.020) + (17.001), (I-300) + (3.020) + (17.002), (I-300) + (3.020) + (17.003), (I-300) + (3.020) + (17.008), (I-300) + (3.020) + (18.001),
(I-300) + (3.025) + (3.030), (I-300) + (3.025) + (3.031), (I-300) + (3.025) + (5.003), (I-300) + (3.025) + (5.004), (I-300) + (3.025) + (5.005), (I-300) + (3.025) + (5.008), (I-300) + (3.025) + (5.009), (I-300) + (3.025) + (5.011), (I-300) + (3.025) + (5.012), (I-300) + (3.025) + (5.013), (I-300) + (3.025) + (5.015), (I-300) + (3.025) + (5.018), (I-300) + (3.025) + (5.019), (I-300) + (3.025) + (6.002), (I-300) + (3.025) + (7.001), (I-300) + (3.025) + (7.005), (I-300) + (3.025) + (9.002), (I-300) + (3.025) + (9.004), (I-300) + (3.025) + (14.001), (I-300) + (3.025) + (14.002), (I-300) + (3.025) + (15.008), (I-300) + (3.025) + (15.011), (I-300) + (3.025) + (15.012), (I-300) + (3.025) + (15.016), (I-300) + (3.025) + (15.025), (I-300) + (3.025) + (15.027), (I-300) + (3.025) + (15.047), (I-300) + (3.025) + (15.063), (I-300) + (3.025) + (15.064), (I-300) + (3.025) + (16.001), (I-300) + (3.025) + (16.005), (I-300) + (3.025) + (17.001), (I-300) + (3.025) + (17.002), (I-300) + (3.025) + (17.003), (I-300) + (3.025) + (17.008), (I-300) + (3.025) + (18.001),
(I-300) + (3.026) + (3.025), (I-300) + (3.026) + (3.030), (I-300) + (3.026) + (3.031), (I-300) + (3.026) + (5.003), (I-300) + (3.026) + (5.004), (I-300) + (3.026) + (5.005), (I-300) + (3.026) + (5.008), (I-300) + (3.026) + (5.009), (I-300) + (3.026) + (5.011), (I-300) + (3.026) + (5.012), (I-300) + (3.026) + (5.013), (I-300) + (3.026) + (5.015), (I-300) + (3.026) + (5.018), (I-300) + (3.026) + (5.019), (I-300) + (3.026) + (6.002), (I-300) + (3.026) + (7.001), (I-300) + (3.026) + (7.005), (I-300) + (3.026) + (9.002), (I-300) + (3.026) + (9.004), (I-300) + (3.026) + (14.001), (I-300) + (3.026) + (14.002), (I-300) + (3.026) + (15.008), (I-300) + (3.026) + (15.011), (I-300) + (3.026) + (15.012), (I-300) + (3.026) + (15.016), (I-300) + (3.026) + (15.025), (I-300) + (3.026) + (15.027), (I-300) + (3.026) + (15.047), (I-300) + (3.026) + (15.063), (I-300) + (3.026) + (15.064), (I-300) + (3.026) + (16.001), (I-300) + (3.026) + (16.005), (I-300) + (3.026) + (17.001), (I-300) + (3.026) + (17.002), (I-300) + (3.026) + (17.003), (I-300) + (3.026) + (17.008), (I-300) + (3.026) + (18.001),
(I-300) + (3.030) + (3.025), (I-300) + (3.030) + (3.031), (I-300) + (3.030) + (5.003), (I-300) + (3.030) + (5.004), (I-300) + (3.030) + (5.005), (I-300) + (3.030) + (5.008), (I-300) + (3.030) + (5.009), (I-300) + (3.030) + (5.011), (I-300) + (3.030) + (5.012), (I-300) + (3.030) + (5.013), (I-300) + (3.030) + (5.015), (I-300) + (3.030) + (5.018), (I-300) + (3.030) + (5.019), (I-300) + (3.030) + (6.002), (I-300) + (3.030) + (7.001), (I-300) + (3.030) + (7.005), (I-300) + (3.030) + (9.002), (I-300) + (3.030) + (9.004), (I-300) + (3.030) + (14.001), (I-300) + (3.030) + (14.002), (I-300) + (3.030) + (15.008), (I-300) + (3.030) + (15.011), (I-300) + (3.030) + (15.012), (I-300) + (3.030) + (15.016), (I-300) + (3.030) + (15.025), (I-300) + (3.030) + (15.027), (I-300) + (3.030) + (15.047), (I-300) + (3.030) + (15.063), (I-300) + (3.030) + (15.064), (I-300) + (3.030) + (16.001), (I-300) + (3.030) + (16.005), (I-300) + (3.030) + (17.001), (I-300) + (3.030) + (17.002), (I-300) + (3.030) + (17.003), (I-300) + (3.030) + (17.008), (I-300) + (3.030) + (18.001),
(I-300) + (3.031) + (3.025), (I-300) + (3.031) + (3.030), (I-300) + (3.031) + (5.003), (I-300) + (3.031) + (5.004), (I-300) + (3.031) + (5.005), (I-300) + (3.031) + (5.008), (I-300) + (3.031) + (5.009), (I-300) + (3.031) + (5.011), (I-300) + (3.031) + (5.012), (I-300) + (3.031) + (5.013), (I-300) + (3.031) + (5.015), (I-300) + (3.031) + (5.018), (I-300) + (3.031) + (5.019), (I-300) + (3.031) + (6.002), (I-300) + (3.031) + (7.001), (I-300) + (3.031) + (7.005), (I-300) + (3.031) + (9.002), (I-300) + (3.031) + (9.004), (I-300) + (3.031) + (14.001), (I-300) + (3.031) + (14.002), (I-300) + (3.031) + (15.008), (I-300) + (3.031) + (15.011), (I-300) + (3.031) + (15.012), (I-300) + (3.031) + (15.016), (I-300) + (3.031) + (15.025), (I-300) + (3.031) + (15.027), (I-300) + (3.031) + (15.047), (I-300) + (3.031) + (15.063), (I-300) + (3.031) + (15.064), (I-300) + (3.031) + (16.001), (I-300) + (3.031) + (16.005), (I-300) + (3.031) + (17.001), (I-300) + (3.031) + (17.002), (I-300) + (3.031) + (17.003), (I-300) + (3.031) + (17.008), (I-300) + (3.031) + (18.001),
(I-300) + (5.003) + (9.002), (I-300) + (5.003) + (15.012), (I-300) + (5.003) + (15.016), (I-300) + (5.003) + (15.025), (I-300) + (5.003) + (15.027), (I-300) + (5.003) + (15.047), (I-300) + (5.003) + (15.063), (I-300) + (5.003) + (15.064),
(I-300) + (5.004) + (9.002), (I-300) + (5.004) + (15.012), (I-300) + (5.004) + (15.016), (I-300) + (5.004) + (15.025), (I-300) + (5.004) + (15.027), (I-300) + (5.004) + (15.047), (I-300) + (5.004) + (15.063), (I-300) + (5.004) + (15.064),
(I-300) + (5.005) + (9.002), (I-300) + (5.005) + (15.012), (I-300) + (5.005) + (15.016), (I-300) + (5.005) + (15.025), (I-300) + (5.005) + (15.027), (I-300) + (5.005) + (15.047), (I-300) + (5.005) + (15.063), (I-300) + (5.005) + (15.064),
(I-300) + (5.008) + (9.002), (I-300) + (5.008) + (15.012), (I-300) + (5.008) + (15.016), (I-300) + (5.008) + (15.025), (I-300) + (5.008) + (15.027), (I-300) + (5.008) + (15.047), (I-300) + (5.008) + (15.063), (I-300) + (5.008) + (15.064),
(I-300) + (5.009) + (9.002), (I-300) + (5.009) + (15.012), (I-300) + (5.009) + (15.016), (I-300) + (5.009) + (15.025), (I-300) + (5.009) + (15.027), (I-300) + (5.009) + (15.047), (I-300) + (5.009) + (15.063), (I-300) + (5.009) + (15.064),
(I-300) + (5.011) + (9.002), (I-300) + (5.011) + (15.012), (I-300) + (5.011) + (15.016), (I-300) + (5.011) + (15.025), (I-300) + (5.011) + (15.027), (I-300) + (5.011) + (15.047), (I-300) + (5.011) + (15.063), (I-300) + (5.011) + (15.064),
(I-300) + (5.012) + (9.002), (I-300) + (5.012) + (15.012), (I-300) + (5.012) + (15.016), (I-300) + (5.012) + (15.025), (I-300) + (5.012) + (15.027), (I-300) + (5.012) + (15.047), (I-300) + (5.012) + (15.063), (I-300) + (5.012) + (15.064),
(I-300) + (5.013) + (9.002), (I-300) + (5.013) + (15.012), (I-300) + (5.013) + (15.016), (I-300) + (5.013) + (15.025), (I-300) + (5.013) + (15.027), (I-300) + (5.013) + (15.047), (I-300) + (5.013) + (15.063), (I-300) + (5.013) + (15.064),
(I-300) + (5.015) + (9.002), (I-300) + (5.015) + (15.012), (I-300) + (5.015) + (15.016), (I-300) + (5.015) + (15.025), (I-300) + (5.015) + (15.027), (I-300) + (5.015) + (15.047), (I-300) + (5.015) + (15.063), (I-300) + (5.015) + (15.064),
(I-300) + (5.018) + (9.002), (I-300) + (5.018) + (15.012), (I-300) + (5.018) + (15.016), (I-300) + (5.018) + (15.025), (I-300) + (5.018) + (15.027), (I-300) + (5.018) + (15.047), (I-300) + (5.018) + (15.063), (I-300) + (5.018) + (15.064),
(I-300) + (5.019) + (9.002), (I-300) + (5.019) + (15.012), (I-300) + (5.019) + (15.016), (I-300) + (5.019) + (15.025), (I-300) + (5.019) + (15.027), (I-300) + (5.019) + (15.047), (I-300) + (5.019) + (15.063), (I-300) + (5.019) + (15.064).
2종의 화합물 (B)가 본 발명에 따른 조합물에 존재하는 경우, 보다 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G4-C1)으로부터 선택된다:
(I-302) + (1.001) + (1.002), (I-302) + (1.001) + (1.003), (I-302) + (1.001) + (1.004), (I-302) + (1.001) + (1.005), (I-302) + (1.001) + (1.006), (I-302) + (1.001) + (1.007), (I-302) + (1.001) + (1.010), (I-302) + (1.001) + (1.011), (I-302) + (1.001) + (1.012), (I-302) + (1.001) + (1.013), (I-302) + (1.001) + (1.017), (I-302) + (1.001) + (1.018), (I-302) + (1.001) + (1.020), (I-302) + (1.001) + (1.021), (I-302) + (1.001) + (1.026), (I-302) + (1.001) + (1.027), (I-302) + (1.001) + (1.055), (I-302) + (1.001) + (1.059), (I-302) + (1.001) + (1.092), (I-302) + (1.001) + (2.001), (I-302) + (1.001) + (2.002), (I-302) + (1.001) + (2.003), (I-302) + (1.001) + (2.005), (I-302) + (1.001) + (2.007), (I-302) + (1.001) + (2.009), (I-302) + (1.001) + (2.010), (I-302) + (1.001) + (2.011), (I-302) + (1.001) + (2.012), (I-302) + (1.001) + (2.013), (I-302) + (1.001) + (2.014), (I-302) + (1.001) + (2.015), (I-302) + (1.001) + (2.016), (I-302) + (1.001) + (2.017), (I-302) + (1.001) + (2.018), (I-302) + (1.001) + (2.019), (I-302) + (1.001) + (2.021), (I-302) + (1.001) + (2.028), (I-302) + (1.001) + (2.030), (I-302) + (1.001) + (2.038), (I-302) + (1.001) + (3.003), (I-302) + (1.001) + (3.007), (I-302) + (1.001) + (3.012), (I-302) + (1.001) + (3.013), (I-302) + (1.001) + (3.016), (I-302) + (1.001) + (3.017), (I-302) + (1.001) + (3.020), (I-302) + (1.001) + (3.025), (I-302) + (1.001) + (3.026), (I-302) + (1.001) + (3.030), (I-302) + (1.001) + (3.031), (I-302) + (1.001) + (5.003), (I-302) + (1.001) + (5.004), (I-302) + (1.001) + (5.005), (I-302) + (1.001) + (5.008), (I-302) + (1.001) + (5.009), (I-302) + (1.001) + (5.011), (I-302) + (1.001) + (5.012), (I-302) + (1.001) + (5.013), (I-302) + (1.001) + (5.015), (I-302) + (1.001) + (5.018), (I-302) + (1.001) + (5.019), (I-302) + (1.001) + (6.002), (I-302) + (1.001) + (7.001), (I-302) + (1.001) + (7.005), (I-302) + (1.001) + (9.002), (I-302) + (1.001) + (9.004), (I-302) + (1.001) + (14.001), (I-302) + (1.001) + (14.002), (I-302) + (1.001) + (15.008), (I-302) + (1.001) + (15.011), (I-302) + (1.001) + (15.012), (I-302) + (1.001) + (15.016), (I-302) + (1.001) + (15.025), (I-302) + (1.001) + (15.027), (I-302) + (1.001) + (15.047), (I-302) + (1.001) + (15.063), (I-302) + (1.001) + (15.064), (I-302) + (1.001) + (16.001), (I-302) + (1.001) + (16.005), (I-302) + (1.001) + (17.001), (I-302) + (1.001) + (17.002), (I-302) + (1.001) + (17.003), (I-302) + (1.001) + (17.008), (I-302) + (1.001) + (18.001),
(I-302) + (1.002) + (1.001), (I-302) + (1.002) + (1.003), (I-302) + (1.002) + (1.004), (I-302) + (1.002) + (1.005), (I-302) + (1.002) + (1.006), (I-302) + (1.002) + (1.007), (I-302) + (1.002) + (1.010), (I-302) + (1.002) + (1.011), (I-302) + (1.002) + (1.012), (I-302) + (1.002) + (1.013), (I-302) + (1.002) + (1.017), (I-302) + (1.002) + (1.018), (I-302) + (1.002) + (1.020), (I-302) + (1.002) + (1.021), (I-302) + (1.002) + (1.026), (I-302) + (1.002) + (1.027), (I-302) + (1.002) + (1.055), (I-302) + (1.002) + (1.059), (I-302) + (1.002) + (1.092), (I-302) + (1.002) + (2.001), (I-302) + (1.002) + (2.002), (I-302) + (1.002) + (2.003), (I-302) + (1.002) + (2.005), (I-302) + (1.002) + (2.007), (I-302) + (1.002) + (2.009), (I-302) + (1.002) + (2.010), (I-302) + (1.002) + (2.011), (I-302) + (1.002) + (2.012), (I-302) + (1.002) + (2.013), (I-302) + (1.002) + (2.014), (I-302) + (1.002) + (2.015), (I-302) + (1.002) + (2.016), (I-302) + (1.002) + (2.017), (I-302) + (1.002) + (2.018), (I-302) + (1.002) + (2.019), (I-302) + (1.002) + (2.021), (I-302) + (1.002) + (2.028), (I-302) + (1.002) + (2.030), (I-302) + (1.002) + (2.038), (I-302) + (1.002) + (3.003), (I-302) + (1.002) + (3.007), (I-302) + (1.002) + (3.012), (I-302) + (1.002) + (3.013), (I-302) + (1.002) + (3.016), (I-302) + (1.002) + (3.017), (I-302) + (1.002) + (3.020), (I-302) + (1.002) + (3.025), (I-302) + (1.002) + (3.026), (I-302) + (1.002) + (3.030), (I-302) + (1.002) + (3.031), (I-302) + (1.002) + (5.003), (I-302) + (1.002) + (5.004), (I-302) + (1.002) + (5.005), (I-302) + (1.002) + (5.008), (I-302) + (1.002) + (5.009), (I-302) + (1.002) + (5.011), (I-302) + (1.002) + (5.012), (I-302) + (1.002) + (5.013), (I-302) + (1.002) + (5.015), (I-302) + (1.002) + (5.018), (I-302) + (1.002) + (5.019), (I-302) + (1.002) + (6.002), (I-302) + (1.002) + (7.001), (I-302) + (1.002) + (7.005), (I-302) + (1.002) + (9.002), (I-302) + (1.002) + (9.004), (I-302) + (1.002) + (14.001), (I-302) + (1.002) + (14.002), (I-302) + (1.002) + (15.008), (I-302) + (1.002) + (15.011), (I-302) + (1.002) + (15.012), (I-302) + (1.002) + (15.016), (I-302) + (1.002) + (15.025), (I-302) + (1.002) + (15.027), (I-302) + (1.002) + (15.047), (I-302) + (1.002) + (15.063), (I-302) + (1.002) + (15.064), (I-302) + (1.002) + (16.001), (I-302) + (1.002) + (16.005), (I-302) + (1.002) + (17.001), (I-302) + (1.002) + (17.002), (I-302) + (1.002) + (17.003), (I-302) + (1.002) + (17.008), (I-302) + (1.002) + (18.001),
(I-302) + (1.003) + (1.001), (I-302) + (1.003) + (1.002), (I-302) + (1.003) + (1.004), (I-302) + (1.003) + (1.005), (I-302) + (1.003) + (1.006), (I-302) + (1.003) + (1.007), (I-302) + (1.003) + (1.010), (I-302) + (1.003) + (1.011), (I-302) + (1.003) + (1.012), (I-302) + (1.003) + (1.013), (I-302) + (1.003) + (1.017), (I-302) + (1.003) + (1.018), (I-302) + (1.003) + (1.020), (I-302) + (1.003) + (1.021), (I-302) + (1.003) + (1.026), (I-302) + (1.003) + (1.027), (I-302) + (1.003) + (1.055), (I-302) + (1.003) + (1.059), (I-302) + (1.003) + (1.092), (I-302) + (1.003) + (2.001), (I-302) + (1.003) + (2.002), (I-302) + (1.003) + (2.003), (I-302) + (1.003) + (2.005), (I-302) + (1.003) + (2.007), (I-302) + (1.003) + (2.009), (I-302) + (1.003) + (2.010), (I-302) + (1.003) + (2.011), (I-302) + (1.003) + (2.012), (I-302) + (1.003) + (2.013), (I-302) + (1.003) + (2.014), (I-302) + (1.003) + (2.015), (I-302) + (1.003) + (2.016), (I-302) + (1.003) + (2.017), (I-302) + (1.003) + (2.018), (I-302) + (1.003) + (2.019), (I-302) + (1.003) + (2.021), (I-302) + (1.003) + (2.028), (I-302) + (1.003) + (2.030), (I-302) + (1.003) + (2.038), (I-302) + (1.003) + (3.003), (I-302) + (1.003) + (3.007), (I-302) + (1.003) + (3.012), (I-302) + (1.003) + (3.013), (I-302) + (1.003) + (3.016), (I-302) + (1.003) + (3.017), (I-302) + (1.003) + (3.020), (I-302) + (1.003) + (3.025), (I-302) + (1.003) + (3.026), (I-302) + (1.003) + (3.030), (I-302) + (1.003) + (3.031), (I-302) + (1.003) + (5.003), (I-302) + (1.003) + (5.004), (I-302) + (1.003) + (5.005), (I-302) + (1.003) + (5.008), (I-302) + (1.003) + (5.009), (I-302) + (1.003) + (5.011), (I-302) + (1.003) + (5.012), (I-302) + (1.003) + (5.013), (I-302) + (1.003) + (5.015), (I-302) + (1.003) + (5.018), (I-302) + (1.003) + (5.019), (I-302) + (1.003) + (6.002), (I-302) + (1.003) + (7.001), (I-302) + (1.003) + (7.005), (I-302) + (1.003) + (9.002), (I-302) + (1.003) + (9.004), (I-302) + (1.003) + (14.001), (I-302) + (1.003) + (14.002), (I-302) + (1.003) + (15.008), (I-302) + (1.003) + (15.011), (I-302) + (1.003) + (15.012), (I-302) + (1.003) + (15.016), (I-302) + (1.003) + (15.025), (I-302) + (1.003) + (15.027), (I-302) + (1.003) + (15.047), (I-302) + (1.003) + (15.063), (I-302) + (1.003) + (15.064), (I-302) + (1.003) + (16.001), (I-302) + (1.003) + (16.005), (I-302) + (1.003) + (17.001), (I-302) + (1.003) + (17.002), (I-302) + (1.003) + (17.003), (I-302) + (1.003) + (17.008), (I-302) + (1.003) + (18.001),
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(I-302) + (3.017) + (3.025), (I-302) + (3.017) + (3.030), (I-302) + (3.017) + (3.031), (I-302) + (3.017) + (5.003), (I-302) + (3.017) + (5.004), (I-302) + (3.017) + (5.005), (I-302) + (3.017) + (5.008), (I-302) + (3.017) + (5.009), (I-302) + (3.017) + (5.011), (I-302) + (3.017) + (5.012), (I-302) + (3.017) + (5.013), (I-302) + (3.017) + (5.015), (I-302) + (3.017) + (5.018), (I-302) + (3.017) + (5.019), (I-302) + (3.017) + (6.002), (I-302) + (3.017) + (7.001), (I-302) + (3.017) + (7.005), (I-302) + (3.017) + (9.002), (I-302) + (3.017) + (9.004), (I-302) + (3.017) + (14.001), (I-302) + (3.017) + (14.002), (I-302) + (3.017) + (15.008), (I-302) + (3.017) + (15.011), (I-302) + (3.017) + (15.012), (I-302) + (3.017) + (15.016), (I-302) + (3.017) + (15.025), (I-302) + (3.017) + (15.027), (I-302) + (3.017) + (15.047), (I-302) + (3.017) + (15.063), (I-302) + (3.017) + (15.064), (I-302) + (3.017) + (16.001), (I-302) + (3.017) + (16.005), (I-302) + (3.017) + (17.001), (I-302) + (3.017) + (17.002), (I-302) + (3.017) + (17.003), (I-302) + (3.017) + (17.008), (I-302) + (3.017) + (18.001),
(I-302) + (3.020) + (3.025), (I-302) + (3.020) + (3.030), (I-302) + (3.020) + (3.031), (I-302) + (3.020) + (5.003), (I-302) + (3.020) + (5.004), (I-302) + (3.020) + (5.005), (I-302) + (3.020) + (5.008), (I-302) + (3.020) + (5.009), (I-302) + (3.020) + (5.011), (I-302) + (3.020) + (5.012), (I-302) + (3.020) + (5.013), (I-302) + (3.020) + (5.015), (I-302) + (3.020) + (5.018), (I-302) + (3.020) + (5.019), (I-302) + (3.020) + (6.002), (I-302) + (3.020) + (7.001), (I-302) + (3.020) + (7.005), (I-302) + (3.020) + (9.002), (I-302) + (3.020) + (9.004), (I-302) + (3.020) + (14.001), (I-302) + (3.020) + (14.002), (I-302) + (3.020) + (15.008), (I-302) + (3.020) + (15.011), (I-302) + (3.020) + (15.012), (I-302) + (3.020) + (15.016), (I-302) + (3.020) + (15.025), (I-302) + (3.020) + (15.027), (I-302) + (3.020) + (15.047), (I-302) + (3.020) + (15.063), (I-302) + (3.020) + (15.064), (I-302) + (3.020) + (16.001), (I-302) + (3.020) + (16.005), (I-302) + (3.020) + (17.001), (I-302) + (3.020) + (17.002), (I-302) + (3.020) + (17.003), (I-302) + (3.020) + (17.008), (I-302) + (3.020) + (18.001),
(I-302) + (3.025) + (3.030), (I-302) + (3.025) + (3.031), (I-302) + (3.025) + (5.003), (I-302) + (3.025) + (5.004), (I-302) + (3.025) + (5.005), (I-302) + (3.025) + (5.008), (I-302) + (3.025) + (5.009), (I-302) + (3.025) + (5.011), (I-302) + (3.025) + (5.012), (I-302) + (3.025) + (5.013), (I-302) + (3.025) + (5.015), (I-302) + (3.025) + (5.018), (I-302) + (3.025) + (5.019), (I-302) + (3.025) + (6.002), (I-302) + (3.025) + (7.001), (I-302) + (3.025) + (7.005), (I-302) + (3.025) + (9.002), (I-302) + (3.025) + (9.004), (I-302) + (3.025) + (14.001), (I-302) + (3.025) + (14.002), (I-302) + (3.025) + (15.008), (I-302) + (3.025) + (15.011), (I-302) + (3.025) + (15.012), (I-302) + (3.025) + (15.016), (I-302) + (3.025) + (15.025), (I-302) + (3.025) + (15.027), (I-302) + (3.025) + (15.047), (I-302) + (3.025) + (15.063), (I-302) + (3.025) + (15.064), (I-302) + (3.025) + (16.001), (I-302) + (3.025) + (16.005), (I-302) + (3.025) + (17.001), (I-302) + (3.025) + (17.002), (I-302) + (3.025) + (17.003), (I-302) + (3.025) + (17.008), (I-302) + (3.025) + (18.001),
(I-302) + (3.026) + (3.025), (I-302) + (3.026) + (3.030), (I-302) + (3.026) + (3.031), (I-302) + (3.026) + (5.003), (I-302) + (3.026) + (5.004), (I-302) + (3.026) + (5.005), (I-302) + (3.026) + (5.008), (I-302) + (3.026) + (5.009), (I-302) + (3.026) + (5.011), (I-302) + (3.026) + (5.012), (I-302) + (3.026) + (5.013), (I-302) + (3.026) + (5.015), (I-302) + (3.026) + (5.018), (I-302) + (3.026) + (5.019), (I-302) + (3.026) + (6.002), (I-302) + (3.026) + (7.001), (I-302) + (3.026) + (7.005), (I-302) + (3.026) + (9.002), (I-302) + (3.026) + (9.004), (I-302) + (3.026) + (14.001), (I-302) + (3.026) + (14.002), (I-302) + (3.026) + (15.008), (I-302) + (3.026) + (15.011), (I-302) + (3.026) + (15.012), (I-302) + (3.026) + (15.016), (I-302) + (3.026) + (15.025), (I-302) + (3.026) + (15.027), (I-302) + (3.026) + (15.047), (I-302) + (3.026) + (15.063), (I-302) + (3.026) + (15.064), (I-302) + (3.026) + (16.001), (I-302) + (3.026) + (16.005), (I-302) + (3.026) + (17.001), (I-302) + (3.026) + (17.002), (I-302) + (3.026) + (17.003), (I-302) + (3.026) + (17.008), (I-302) + (3.026) + (18.001),
(I-302) + (3.030) + (3.025), (I-302) + (3.030) + (3.031), (I-302) + (3.030) + (5.003), (I-302) + (3.030) + (5.004), (I-302) + (3.030) + (5.005), (I-302) + (3.030) + (5.008), (I-302) + (3.030) + (5.009), (I-302) + (3.030) + (5.011), (I-302) + (3.030) + (5.012), (I-302) + (3.030) + (5.013), (I-302) + (3.030) + (5.015), (I-302) + (3.030) + (5.018), (I-302) + (3.030) + (5.019), (I-302) + (3.030) + (6.002), (I-302) + (3.030) + (7.001), (I-302) + (3.030) + (7.005), (I-302) + (3.030) + (9.002), (I-302) + (3.030) + (9.004), (I-302) + (3.030) + (14.001), (I-302) + (3.030) + (14.002), (I-302) + (3.030) + (15.008), (I-302) + (3.030) + (15.011), (I-302) + (3.030) + (15.012), (I-302) + (3.030) + (15.016), (I-302) + (3.030) + (15.025), (I-302) + (3.030) + (15.027), (I-302) + (3.030) + (15.047), (I-302) + (3.030) + (15.063), (I-302) + (3.030) + (15.064), (I-302) + (3.030) + (16.001), (I-302) + (3.030) + (16.005), (I-302) + (3.030) + (17.001), (I-302) + (3.030) + (17.002), (I-302) + (3.030) + (17.003), (I-302) + (3.030) + (17.008), (I-302) + (3.030) + (18.001),
(I-302) + (3.031) + (3.025), (I-302) + (3.031) + (3.030), (I-302) + (3.031) + (5.003), (I-302) + (3.031) + (5.004), (I-302) + (3.031) + (5.005), (I-302) + (3.031) + (5.008), (I-302) + (3.031) + (5.009), (I-302) + (3.031) + (5.011), (I-302) + (3.031) + (5.012), (I-302) + (3.031) + (5.013), (I-302) + (3.031) + (5.015), (I-302) + (3.031) + (5.018), (I-302) + (3.031) + (5.019), (I-302) + (3.031) + (6.002), (I-302) + (3.031) + (7.001), (I-302) + (3.031) + (7.005), (I-302) + (3.031) + (9.002), (I-302) + (3.031) + (9.004), (I-302) + (3.031) + (14.001), (I-302) + (3.031) + (14.002), (I-302) + (3.031) + (15.008), (I-302) + (3.031) + (15.011), (I-302) + (3.031) + (15.012), (I-302) + (3.031) + (15.016), (I-302) + (3.031) + (15.025), (I-302) + (3.031) + (15.027), (I-302) + (3.031) + (15.047), (I-302) + (3.031) + (15.063), (I-302) + (3.031) + (15.064), (I-302) + (3.031) + (16.001), (I-302) + (3.031) + (16.005), (I-302) + (3.031) + (17.001), (I-302) + (3.031) + (17.002), (I-302) + (3.031) + (17.003), (I-302) + (3.031) + (17.008), (I-302) + (3.031) + (18.001),
(I-302) + (5.003) + (9.002), (I-302) + (5.003) + (15.012), (I-302) + (5.003) + (15.016), (I-302) + (5.003) + (15.025), (I-302) + (5.003) + (15.027), (I-302) + (5.003) + (15.047), (I-302) + (5.003) + (15.063), (I-302) + (5.003) + (15.064),
(I-302) + (5.004) + (9.002), (I-302) + (5.004) + (15.012), (I-302) + (5.004) + (15.016), (I-302) + (5.004) + (15.025), (I-302) + (5.004) + (15.027), (I-302) + (5.004) + (15.047), (I-302) + (5.004) + (15.063), (I-302) + (5.004) + (15.064),
(I-302) + (5.005) + (9.002), (I-302) + (5.005) + (15.012), (I-302) + (5.005) + (15.016), (I-302) + (5.005) + (15.025), (I-302) + (5.005) + (15.027), (I-302) + (5.005) + (15.047), (I-302) + (5.005) + (15.063), (I-302) + (5.005) + (15.064),
(I-302) + (5.008) + (9.002), (I-302) + (5.008) + (15.012), (I-302) + (5.008) + (15.016), (I-302) + (5.008) + (15.025), (I-302) + (5.008) + (15.027), (I-302) + (5.008) + (15.047), (I-302) + (5.008) + (15.063), (I-302) + (5.008) + (15.064),
(I-302) + (5.009) + (9.002), (I-302) + (5.009) + (15.012), (I-302) + (5.009) + (15.016), (I-302) + (5.009) + (15.025), (I-302) + (5.009) + (15.027), (I-302) + (5.009) + (15.047), (I-302) + (5.009) + (15.063), (I-302) + (5.009) + (15.064),
(I-302) + (5.011) + (9.002), (I-302) + (5.011) + (15.012), (I-302) + (5.011) + (15.016), (I-302) + (5.011) + (15.025), (I-302) + (5.011) + (15.027), (I-302) + (5.011) + (15.047), (I-302) + (5.011) + (15.063), (I-302) + (5.011) + (15.064),
(I-302) + (5.012) + (9.002), (I-302) + (5.012) + (15.012), (I-302) + (5.012) + (15.016), (I-302) + (5.012) + (15.025), (I-302) + (5.012) + (15.027), (I-302) + (5.012) + (15.047), (I-302) + (5.012) + (15.063), (I-302) + (5.012) + (15.064),
(I-302) + (5.013) + (9.002), (I-302) + (5.013) + (15.012), (I-302) + (5.013) + (15.016), (I-302) + (5.013) + (15.025), (I-302) + (5.013) + (15.027), (I-302) + (5.013) + (15.047), (I-302) + (5.013) + (15.063), (I-302) + (5.013) + (15.064),
(I-302) + (5.015) + (9.002), (I-302) + (5.015) + (15.012), (I-302) + (5.015) + (15.016), (I-302) + (5.015) + (15.025), (I-302) + (5.015) + (15.027), (I-302) + (5.015) + (15.047), (I-302) + (5.015) + (15.063), (I-302) + (5.015) + (15.064),
(I-302) + (5.018) + (9.002), (I-302) + (5.018) + (15.012), (I-302) + (5.018) + (15.016), (I-302) + (5.018) + (15.025), (I-302) + (5.018) + (15.027), (I-302) + (5.018) + (15.047), (I-302) + (5.018) + (15.063), (I-302) + (5.018) + (15.064),
(I-302) + (5.019) + (9.002), (I-302) + (5.019) + (15.012), (I-302) + (5.019) + (15.016), (I-302) + (5.019) + (15.025), (I-302) + (5.019) + (15.027), (I-302) + (5.019) + (15.047), (I-302) + (5.019) + (15.063), (I-302) + (5.019) + (15.064).
2종의 화합물 (B)가 본 발명에 따른 조합물에 존재하는 경우, 바람직한 화합물 조합물은 또한 하기 혼합물로 이루어진 군 (G6-C)으로부터 선택된다:
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(I-339) + (5.011) + (9.001), (I-339) + (5.011) + (9.002), (I-339) + (5.011) + (9.003), (I-339) + (5.011) + (9.004), (I-339) + (5.011) + (9.005), (I-339) + (5.011) + (9.006), (I-339) + (5.011) + (9.007), (I-339) + (5.011) + (9.008), (I-339) + (5.011) + (9.009), (I-339) + (5.011) + (15.012), (I-339) + (5.011) + (15.016), (I-339) + (5.011) + (15.025), (I-339) + (5.011) + (15.027), (I-339) + (5.011) + (15.047), (I-339) + (5.011) + (15.063), (I-339) + (5.011) + (15.064),
(I-339) + (5.012) + (9.001), (I-339) + (5.012) + (9.002), (I-339) + (5.012) + (9.003), (I-339) + (5.012) + (9.004), (I-339) + (5.012) + (9.005), (I-339) + (5.012) + (9.006), (I-339) + (5.012) + (9.007), (I-339) + (5.012) + (9.008), (I-339) + (5.012) + (9.009), (I-339) + (5.012) + (15.012), (I-339) + (5.012) + (15.016), (I-339) + (5.012) + (15.025), (I-339) + (5.012) + (15.027), (I-339) + (5.012) + (15.047), (I-339) + (5.012) + (15.063), (I-339) + (5.012) + (15.064),
(I-339) + (5.013) + (9.001), (I-339) + (5.013) + (9.002), (I-339) + (5.013) + (9.003), (I-339) + (5.013) + (9.004), (I-339) + (5.013) + (9.005), (I-339) + (5.013) + (9.006), (I-339) + (5.013) + (9.007), (I-339) + (5.013) + (9.008), (I-339) + (5.013) + (9.009), (I-339) + (5.013) + (15.012), (I-339) + (5.013) + (15.016), (I-339) + (5.013) + (15.025), (I-339) + (5.013) + (15.027), (I-339) + (5.013) + (15.047), (I-339) + (5.013) + (15.063), (I-339) + (5.013) + (15.064),
(I-339) + (5.014) + (9.001), (I-339) + (5.014) + (9.002), (I-339) + (5.014) + (9.003), (I-339) + (5.014) + (9.004), (I-339) + (5.014) + (9.005), (I-339) + (5.014) + (9.006), (I-339) + (5.014) + (9.007), (I-339) + (5.014) + (9.008), (I-339) + (5.014) + (9.009), (I-339) + (5.014) + (15.012), (I-339) + (5.014) + (15.016), (I-339) + (5.014) + (15.025), (I-339) + (5.014) + (15.027), (I-339) + (5.014) + (15.047), (I-339) + (5.014) + (15.063), (I-339) + (5.014) + (15.064),
(I-339) + (5.015) + (9.001), (I-339) + (5.015) + (9.002), (I-339) + (5.015) + (9.003), (I-339) + (5.015) + (9.004), (I-339) + (5.015) + (9.005), (I-339) + (5.015) + (9.006), (I-339) + (5.015) + (9.007), (I-339) + (5.015) + (9.008), (I-339) + (5.015) + (9.009), (I-339) + (5.015) + (15.012), (I-339) + (5.015) + (15.016), (I-339) + (5.015) + (15.025), (I-339) + (5.015) + (15.027), (I-339) + (5.015) + (15.047), (I-339) + (5.015) + (15.063), (I-339) + (5.015) + (15.064),
(I-339) + (5.016) + (9.001), (I-339) + (5.016) + (9.002), (I-339) + (5.016) + (9.003), (I-339) + (5.016) + (9.004), (I-339) + (5.016) + (9.005), (I-339) + (5.016) + (9.006), (I-339) + (5.016) + (9.007), (I-339) + (5.016) + (9.008), (I-339) + (5.016) + (9.009), (I-339) + (5.016) + (15.012), (I-339) + (5.016) + (15.016), (I-339) + (5.016) + (15.025), (I-339) + (5.016) + (15.027), (I-339) + (5.016) + (15.047), (I-339) + (5.016) + (15.063), (I-339) + (5.016) + (15.064),
(I-339) + (5.017) + (9.001), (I-339) + (5.017) + (9.002), (I-339) + (5.017) + (9.003), (I-339) + (5.017) + (9.004), (I-339) + (5.017) + (9.005), (I-339) + (5.017) + (9.006), (I-339) + (5.017) + (9.007), (I-339) + (5.017) + (9.008), (I-339) + (5.017) + (9.009), (I-339) + (5.017) + (15.012), (I-339) + (5.017) + (15.016), (I-339) + (5.017) + (15.025), (I-339) + (5.017) + (15.027), (I-339) + (5.017) + (15.047), (I-339) + (5.017) + (15.063), (I-339) + (5.017) + (15.064),
(I-339) + (5.018) + (9.001), (I-339) + (5.018) + (9.002), (I-339) + (5.018) + (9.003), (I-339) + (5.018) + (9.004), (I-339) + (5.018) + (9.005), (I-339) + (5.018) + (9.006), (I-339) + (5.018) + (9.007), (I-339) + (5.018) + (9.008), (I-339) + (5.018) + (9.009), (I-339) + (5.018) + (15.012), (I-339) + (5.018) + (15.016), (I-339) + (5.018) + (15.025), (I-339) + (5.018) + (15.027), (I-339) + (5.018) + (15.047), (I-339) + (5.018) + (15.063), (I-339) + (5.018) + (15.064),
(I-339) + (5.019) + (9.001), (I-339) + (5.019) + (9.002), (I-339) + (5.019) + (9.003), (I-339) + (5.019) + (9.004), (I-339) + (5.019) + (9.005), (I-339) + (5.019) + (9.006), (I-339) + (5.019) + (9.007), (I-339) + (5.019) + (9.008), (I-339) + (5.019) + (9.009), (I-339) + (5.019) + (15.012), (I-339) + (5.019) + (15.016), (I-339) + (5.019) + (15.025), (I-339) + (5.019) + (15.027), (I-339) + (5.019) + (15.047), (I-339) + (5.019) + (15.063), (I-339) + (5.019) + (15.064),
(I-339) + (5.020) + (9.001), (I-339) + (5.020) + (9.002), (I-339) + (5.020) + (9.003), (I-339) + (5.020) + (9.004), (I-339) + (5.020) + (9.005), (I-339) + (5.020) + (9.006), (I-339) + (5.020) + (9.007), (I-339) + (5.020) + (9.008), (I-339) + (5.020) + (9.009), (I-339) + (5.020) + (15.012), (I-339) + (5.020) + (15.016), (I-339) + (5.020) + (15.025), (I-339) + (5.020) + (15.027), (I-339) + (5.020) + (15.047), (I-339) + (5.020) + (15.063), (I-339) + (5.020) + (15.064),
(I-339) + (5.021) + (9.001), (I-339) + (5.021) + (9.002), (I-339) + (5.021) + (9.003), (I-339) + (5.021) + (9.004), (I-339) + (5.021) + (9.005), (I-339) + (5.021) + (9.006), (I-339) + (5.021) + (9.007), (I-339) + (5.021) + (9.008), (I-339) + (5.021) + (9.009), (I-339) + (5.021) + (15.012), (I-339) + (5.021) + (15.016), (I-339) + (5.021) + (15.025), (I-339) + (5.021) + (15.027), (I-339) + (5.021) + (15.047), (I-339) + (5.021) + (15.063), (I-339) + (5.021) + (15.064),
(I-339) + (5.022) + (9.001), (I-339) + (5.022) + (9.002), (I-339) + (5.022) + (9.003), (I-339) + (5.022) + (9.004), (I-339) + (5.022) + (9.005), (I-339) + (5.022) + (9.006), (I-339) + (5.022) + (9.007), (I-339) + (5.022) + (9.008), (I-339) + (5.022) + (9.009), (I-339) + (5.022) + (15.012), (I-339) + (5.022) + (15.016), (I-339) + (5.022) + (15.025), (I-339) + (5.022) + (15.027), (I-339) + (5.022) + (15.047), (I-339) + (5.022) + (15.063), (I-339) + (5.022) + (15.064),
(I-339) + (5.023) + (9.001), (I-339) + (5.023) + (9.002), (I-339) + (5.023) + (9.003), (I-339) + (5.023) + (9.004), (I-339) + (5.023) + (9.005), (I-339) + (5.023) + (9.006), (I-339) + (5.023) + (9.007), (I-339) + (5.023) + (9.008), (I-339) + (5.023) + (9.009), (I-339) + (5.023) + (15.012), (I-339) + (5.023) + (15.016), (I-339) + (5.023) + (15.025), (I-339) + (5.023) + (15.027), (I-339) + (5.023) + (15.047), (I-339) + (5.023) + (15.063), (I-339) + (5.023) + (15.064).
2종의 화합물 (B)가 본 발명에 따른 조합물에 존재하는 경우, 바람직한 화합물 조합물은 하기 혼합물로 이루어진 군 (G7-C)으로부터 선택된다:
(I-338) + (1.001) + (1.002), (I-338) + (1.001) + (1.003), (I-338) + (1.001) + (1.004), (I-338) + (1.001) + (1.005), (I-338) + (1.001) + (1.006), (I-338) + (1.001) + (1.007), (I-338) + (1.001) + (1.008), (I-338) + (1.001) + (1.009), (I-338) + (1.001) + (1.010), (I-338) + (1.001) + (1.011), (I-338) + (1.001) + (1.012), (I-338) + (1.001) + (1.013), (I-338) + (1.001) + (1.014), (I-338) + (1.001) + (1.015), (I-338) + (1.001) + (1.016), (I-338) + (1.001) + (1.017), (I-338) + (1.001) + (1.018), (I-338) + (1.001) + (1.019), (I-338) + (1.001) + (1.020), (I-338) + (1.001) + (1.021), (I-338) + (1.001) + (1.022), (I-338) + (1.001) + (1.023), (I-338) + (1.001) + (1.024), (I-338) + (1.001) + (1.025), (I-338) + (1.001) + (1.026), (I-338) + (1.001) + (1.027), (I-338) + (1.001) + (1.028), (I-338) + (1.001) + (1.029), (I-338) + (1.001) + (1.030), (I-338) + (1.001) + (1.031), (I-338) + (1.001) + (1.032), (I-338) + (1.001) + (1.033), (I-338) + (1.001) + (1.034), (I-338) + (1.001) + (1.035), (I-338) + (1.001) + (1.036), (I-338) + (1.001) + (1.037), (I-338) + (1.001) + (1.038), (I-338) + (1.001) + (1.039), (I-338) + (1.001) + (1.040), (I-338) + (1.001) + (1.041), (I-338) + (1.001) + (1.042), (I-338) + (1.001) + (1.043), (I-338) + (1.001) + (1.044), (I-338) + (1.001) + (1.045), (I-338) + (1.001) + (1.046), (I-338) + (1.001) + (1.047), (I-338) + (1.001) + (1.048), (I-338) + (1.001) + (1.049), (I-338) + (1.001) + (1.050), (I-338) + (1.001) + (1.051), (I-338) + (1.001) + (1.052), (I-338) + (1.001) + (1.053), (I-338) + (1.001) + (1.054), (I-338) + (1.001) + (1.055), (I-338) + (1.001) + (1.056), (I-338) + (1.001) + (1.057), (I-338) + (1.001) + (1.058), (I-338) + (1.001) + (1.059), (I-338) + (1.001) + (1.060), (I-338) + (1.001) + (1.061), (I-338) + (1.001) + (1.062), (I-338) + (1.001) + (1.063), (I-338) + (1.001) + (1.064), (I-338) + (1.001) + (1.065), (I-338) + (1.001) + (1.066), (I-338) + (1.001) + (1.067), (I-338) + (1.001) + (1.068), (I-338) + (1.001) + (1.069), (I-338) + (1.001) + (1.070), (I-338) + (1.001) + (1.071), (I-338) + (1.001) + (1.072), (I-338) + (1.001) + (1.073), (I-338) + (1.001) + (1.074), (I-338) + (1.001) + (1.075), (I-338) + (1.001) + (1.076), (I-338) + (1.001) + (1.077), (I-338) + (1.001) + (1.078), (I-338) + (1.001) + (1.079), (I-338) + (1.001) + (1.080), (I-338) + (1.001) + (1.081), (I-338) + (1.001) + (1.082), (I-338) + (1.001) + (1.083), (I-338) + (1.001) + (1.084), (I-338) + (1.001) + (1.085), (I-338) + (1.001) + (1.086), (I-338) + (1.001) + (1.087), (I-338) + (1.001) + (1.088), (I-338) + (1.001) + (1.089), (I-338) + (1.001) + (1.090), (I-338) + (1.001) + (1.091), (I-338) + (1.001) + (1.092), (I-338) + (1.001) + (2.001), (I-338) + (1.001) + (2.002), (I-338) + (1.001) + (2.003), (I-338) + (1.001) + (2.004), (I-338) + (1.001) + (2.005), (I-338) + (1.001) + (2.006), (I-338) + (1.001) + (2.007), (I-338) + (1.001) + (2.008), (I-338) + (1.001) + (2.009), (I-338) + (1.001) + (2.010), (I-338) + (1.001) + (2.011), (I-338) + (1.001) + (2.012), (I-338) + (1.001) + (2.013), (I-338) + (1.001) + (2.014), (I-338) + (1.001) + (2.015), (I-338) + (1.001) + (2.016), (I-338) + (1.001) + (2.017), (I-338) + (1.001) + (2.018), (I-338) + (1.001) + (2.019), (I-338) + (1.001) + (2.020), (I-338) + (1.001) + (2.021), (I-338) + (1.001) + (2.022), (I-338) + (1.001) + (2.023), (I-338) + (1.001) + (2.024), (I-338) + (1.001) + (2.025), (I-338) + (1.001) + (2.026), (I-338) + (1.001) + (2.027), (I-338) + (1.001) + (2.028), (I-338) + (1.001) + (2.029), (I-338) + (1.001) + (2.030), (I-338) + (1.001) + (2.031), (I-338) + (1.001) + (2.032), (I-338) + (1.001) + (2.033), (I-338) + (1.001) + (2.034), (I-338) + (1.001) + (2.035), (I-338) + (1.001) + (2.036), (I-338) + (1.001) + (2.037), (I-338) + (1.001) + (2.038), (I-338) + (1.001) + (2.039), (I-338) + (1.001) + (2.040), (I-338) + (1.001) + (2.041), (I-338) + (1.001) + (2.042), (I-338) + (1.001) + (2.043), (I-338) + (1.001) + (2.044), (I-338) + (1.001) + (2.045), (I-338) + (1.001) + (2.046), (I-338) + 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(I-338) + (5.011) + (9.001), (I-338) + (5.011) + (9.002), (I-338) + (5.011) + (9.003), (I-338) + (5.011) + (9.004), (I-338) + (5.011) + (9.005), (I-338) + (5.011) + (9.006), (I-338) + (5.011) + (9.007), (I-338) + (5.011) + (9.008), (I-338) + (5.011) + (9.009), (I-338) + (5.011) + (15.012), (I-338) + (5.011) + (15.016), (I-338) + (5.011) + (15.025), (I-338) + (5.011) + (15.027), (I-338) + (5.011) + (15.047), (I-338) + (5.011) + (15.063), (I-338) + (5.011) + (15.064),
(I-338) + (5.012) + (9.001), (I-338) + (5.012) + (9.002), (I-338) + (5.012) + (9.003), (I-338) + (5.012) + (9.004), (I-338) + (5.012) + (9.005), (I-338) + (5.012) + (9.006), (I-338) + (5.012) + (9.007), (I-338) + (5.012) + (9.008), (I-338) + (5.012) + (9.009), (I-338) + (5.012) + (15.012), (I-338) + (5.012) + (15.016), (I-338) + (5.012) + (15.025), (I-338) + (5.012) + (15.027), (I-338) + (5.012) + (15.047), (I-338) + (5.012) + (15.063), (I-338) + (5.012) + (15.064),
(I-338) + (5.013) + (9.001), (I-338) + (5.013) + (9.002), (I-338) + (5.013) + (9.003), (I-338) + (5.013) + (9.004), (I-338) + (5.013) + (9.005), (I-338) + (5.013) + (9.006), (I-338) + (5.013) + (9.007), (I-338) + (5.013) + (9.008), (I-338) + (5.013) + (9.009), (I-338) + (5.013) + (15.012), (I-338) + (5.013) + (15.016), (I-338) + (5.013) + (15.025), (I-338) + (5.013) + (15.027), (I-338) + (5.013) + (15.047), (I-338) + (5.013) + (15.063), (I-338) + (5.013) + (15.064),
(I-338) + (5.014) + (9.001), (I-338) + (5.014) + (9.002), (I-338) + (5.014) + (9.003), (I-338) + (5.014) + (9.004), (I-338) + (5.014) + (9.005), (I-338) + (5.014) + (9.006), (I-338) + (5.014) + (9.007), (I-338) + (5.014) + (9.008), (I-338) + (5.014) + (9.009), (I-338) + (5.014) + (15.012), (I-338) + (5.014) + (15.016), (I-338) + (5.014) + (15.025), (I-338) + (5.014) + (15.027), (I-338) + (5.014) + (15.047), (I-338) + (5.014) + (15.063), (I-338) + (5.014) + (15.064),
(I-338) + (5.015) + (9.001), (I-338) + (5.015) + (9.002), (I-338) + (5.015) + (9.003), (I-338) + (5.015) + (9.004), (I-338) + (5.015) + (9.005), (I-338) + (5.015) + (9.006), (I-338) + (5.015) + (9.007), (I-338) + (5.015) + (9.008), (I-338) + (5.015) + (9.009), (I-338) + (5.015) + (15.012), (I-338) + (5.015) + (15.016), (I-338) + (5.015) + (15.025), (I-338) + (5.015) + (15.027), (I-338) + (5.015) + (15.047), (I-338) + (5.015) + (15.063), (I-338) + (5.015) + (15.064),
(I-338) + (5.016) + (9.001), (I-338) + (5.016) + (9.002), (I-338) + (5.016) + (9.003), (I-338) + (5.016) + (9.004), (I-338) + (5.016) + (9.005), (I-338) + (5.016) + (9.006), (I-338) + (5.016) + (9.007), (I-338) + (5.016) + (9.008), (I-338) + (5.016) + (9.009), (I-338) + (5.016) + (15.012), (I-338) + (5.016) + (15.016), (I-338) + (5.016) + (15.025), (I-338) + (5.016) + (15.027), (I-338) + (5.016) + (15.047), (I-338) + (5.016) + (15.063), (I-338) + (5.016) + (15.064),
(I-338) + (5.017) + (9.001), (I-338) + (5.017) + (9.002), (I-338) + (5.017) + (9.003), (I-338) + (5.017) + (9.004), (I-338) + (5.017) + (9.005), (I-338) + (5.017) + (9.006), (I-338) + (5.017) + (9.007), (I-338) + (5.017) + (9.008), (I-338) + (5.017) + (9.009), (I-338) + (5.017) + (15.012), (I-338) + (5.017) + (15.016), (I-338) + (5.017) + (15.025), (I-338) + (5.017) + (15.027), (I-338) + (5.017) + (15.047), (I-338) + (5.017) + (15.063), (I-338) + (5.017) + (15.064),
(I-338) + (5.018) + (9.001), (I-338) + (5.018) + (9.002), (I-338) + (5.018) + (9.003), (I-338) + (5.018) + (9.004), (I-338) + (5.018) + (9.005), (I-338) + (5.018) + (9.006), (I-338) + (5.018) + (9.007), (I-338) + (5.018) + (9.008), (I-338) + (5.018) + (9.009), (I-338) + (5.018) + (15.012), (I-338) + (5.018) + (15.016), (I-338) + (5.018) + (15.025), (I-338) + (5.018) + (15.027), (I-338) + (5.018) + (15.047), (I-338) + (5.018) + (15.063), (I-338) + (5.018) + (15.064),
(I-338) + (5.019) + (9.001), (I-338) + (5.019) + (9.002), (I-338) + (5.019) + (9.003), (I-338) + (5.019) + (9.004), (I-338) + (5.019) + (9.005), (I-338) + (5.019) + (9.006), (I-338) + (5.019) + (9.007), (I-338) + (5.019) + (9.008), (I-338) + (5.019) + (9.009), (I-338) + (5.019) + (15.012), (I-338) + (5.019) + (15.016), (I-338) + (5.019) + (15.025), (I-338) + (5.019) + (15.027), (I-338) + (5.019) + (15.047), (I-338) + (5.019) + (15.063), (I-338) + (5.019) + (15.064),
(I-338) + (5.020) + (9.001), (I-338) + (5.020) + (9.002), (I-338) + (5.020) + (9.003), (I-338) + (5.020) + (9.004), (I-338) + (5.020) + (9.005), (I-338) + (5.020) + (9.006), (I-338) + (5.020) + (9.007), (I-338) + (5.020) + (9.008), (I-338) + (5.020) + (9.009), (I-338) + (5.020) + (15.012), (I-338) + (5.020) + (15.016), (I-338) + (5.020) + (15.025), (I-338) + (5.020) + (15.027), (I-338) + (5.020) + (15.047), (I-338) + (5.020) + (15.063), (I-338) + (5.020) + (15.064),
(I-338) + (5.021) + (9.001), (I-338) + (5.021) + (9.002), (I-338) + (5.021) + (9.003), (I-338) + (5.021) + (9.004), (I-338) + (5.021) + (9.005), (I-338) + (5.021) + (9.006), (I-338) + (5.021) + (9.007), (I-338) + (5.021) + (9.008), (I-338) + (5.021) + (9.009), (I-338) + (5.021) + (15.012), (I-338) + (5.021) + (15.016), (I-338) + (5.021) + (15.025), (I-338) + (5.021) + (15.027), (I-338) + (5.021) + (15.047), (I-338) + (5.021) + (15.063), (I-338) + (5.021) + (15.064),
(I-338) + (5.022) + (9.001), (I-338) + (5.022) + (9.002), (I-338) + (5.022) + (9.003), (I-338) + (5.022) + (9.004), (I-338) + (5.022) + (9.005), (I-338) + (5.022) + (9.006), (I-338) + (5.022) + (9.007), (I-338) + (5.022) + (9.008), (I-338) + (5.022) + (9.009), (I-338) + (5.022) + (15.012), (I-338) + (5.022) + (15.016), (I-338) + (5.022) + (15.025), (I-338) + (5.022) + (15.027), (I-338) + (5.022) + (15.047), (I-338) + (5.022) + (15.063), (I-338) + (5.022) + (15.064),
(I-338) + (5.023) + (9.001), (I-338) + (5.023) + (9.002), (I-338) + (5.023) + (9.003), (I-338) + (5.023) + (9.004), (I-338) + (5.023) + (9.005), (I-338) + (5.023) + (9.006), (I-338) + (5.023) + (9.007), (I-338) + (5.023) + (9.008), (I-338) + (5.023) + (9.009), (I-338) + (5.023) + (15.012), (I-338) + (5.023) + (15.016), (I-338) + (5.023) + (15.025), (I-338) + (5.023) + (15.027), (I-338) + (5.023) + (15.047), (I-338) + (5.023) + (15.063), (I-338) + (5.023) + (15.064).
본 발명에 따르면, 표현 "조합물"은, 예를 들어 단일 "레디-믹스" 형태, 단일 활성 화합물의 개별 제제로부터 구성된 조합 분무 혼합물, 예컨대 "탱크-믹스", 및 순차적 방식으로, 즉 합리적으로 짧은 기간, 예컨대 수시간 또는 수일 내에 차례로 적용되는 경우의 단일 활성 성분의 조합 사용에서의 화합물 (A) 및 (B)의 다양한 조합물을 나타낸다. 바람직하게는 화합물 (A) 및 (B)를 적용하는 순서는 본 발명을 실시하는 데 필수적이지 않다.
본 발명에 따른 조합물에서, 화합물 (A) 및 (B)는 A:B의 넓은 범위의 유효 중량비, 예를 들어 250000:1 내지 1:250000의 범위, 바람직하게는 5000:1 내지 1:5000의 중량비, 보다 바람직하게는 1000:1 내지 1:1000의 중량비, 보다 더 바람직하게는 500:1 내지 1:500의 중량비, 가장 바람직하게는 100:1 내지 1:100의 중량비로 존재할 수 있다.
본 발명에 따라 사용될 수 있는 A:B의 추가의 비는 95:1 내지 1:95, 90:1 내지 1:90, 85:1 내지 1:85, 80:1 내지 1:80, 75:1 내지 1:75, 70:1 내지 1:70, 65:1 내지 1:65, 60:1 내지 1:60, 55:1 내지 1:55, 50:1 내지 1:50, 45:1 내지 1:45, 40:1 내지 1:40, 35:1 내지 1:35, 30:1 내지 1:30, 25:1 내지 1:25, 20:1 내지 1:20, 15:1 내지 1:15, 10:1 내지 1:10, 5:1 내지 1:5, 4:1 내지 1:4, 3:1 내지 1:3, 2:1 내지 1:2이다.
본 발명에 따라 사용될 수 있는 A:B의 추가의 비는 1000:1 내지 1:1, 500:1 내지 1:1, 250:1 내지 1:1, 100:1 내지 1:1, 95:1 내지 1:1, 90:1 내지 1:1, 85:1 내지 1:1, 80:1 내지 1:1, 75:1 내지 1:1, 70:1 내지 1:1, 65:1 내지 1:1, 60:1 내지 1:1, 55:1 내지 1:1, 50:1 내지 1:1, 45:1 내지 1:1, 40:1 내지 1:1, 35:1 내지 1:1, 30:1 내지 1:1, 25:1 내지 1:1, 20:1 내지 1:1, 15:1 내지 1:1, 10:1 내지 1:1, 5:1 내지 1:1, 4:1 내지 1:1, 3:1 내지 1:1, 2:1 내지 1:1이다.
본 발명에 따라 사용될 수 있는 A:B의 추가의 비는 1:1 내지 1:1000, 1:1 내지 1:500, 1:1 내지 1:250, 1:1 내지 1:100, 1:1 내지 1:95, 1:1 내지 1:90, 1:1 내지 1:85, 1:1 내지 1:80, 1:1 내지 1:75, 1:1 내지 1:70, 1:1 내지 1:65, 1:1 내지 1:60, 1:1 내지 1:55, 1:1 내지 1:50, 1:1 내지 1:45, 1:1 내지 1:40, 1:1 내지 1:35, 1:1 내지 1:30, 1:1 내지 1:25, 1:1 내지 1:20, 1:1 내지 1:15, 1:1 내지 1:10, 1:1 내지 1:5, 1:1 내지 1:4, 1:1 내지 1:3, 1:1 내지 1:2이다.
1종 초과, 예를 들어 2 또는 3종의 화합물 (B)가 존재하는 경우에, 중량비는 화합물 (B)의 총량, 즉 조합물에 존재하는 각각의 화합물 (B)의 양의 합계를 지칭한다. 이는 1종 초과, 예를 들어 2 또는 3종의 화합물 (A)가 존재하는 경우에 필요한 변경을 가하여 적용된다.
1종 초과, 예를 들어 2 또는 3종의 화합물 (B)가 본 발명에 따른 조합물에 존재하는 경우에, 개별 화합물 (B)는 넓은 범위의 유효 중량비로 존재할 수 있다. 하기에서 화합물 (B1) 및 (B2)로 지칭되는, 예를 들어 2종의 화합물 (B)가 존재하는 경우에, B1:B2의 유효 중량비는 예를 들어 100:1 내지 1:100의 범위, 바람직하게는 50:1 내지 1:50의 중량비, 가장 바람직하게는 20:1 내지 1:20의 중량비로 달라질 수 있다. 본 발명에 따라 사용될 수 있는 B1:B2의 추가의 비는 95:1 내지 1:95, 90:1 내지 1:90, 85:1 내지 1:85, 80:1 내지 1:80, 75:1 내지 1:75, 70:1 내지 1:70, 65:1 내지 1:65, 60:1 내지 1:60, 55:1 내지 1:55, 50:1 내지 1:50, 45:1 내지 1:45, 40:1 내지 1:40, 35:1 내지 1:35, 30:1 내지 1:30, 25:1 내지 1:25, 15:1 내지 1:15, 10:1 내지 1:10, 5:1 내지 1:5, 4:1 내지 1:4, 3:1 내지 1:3, 2:1 내지 1:2이다.
본 발명에 따라 사용될 수 있는 B1:B2의 추가의 비는 95:1 내지 1:1, 90:1 내지 1:1, 85:1 내지 1:1, 80:1 내지 1:1, 75:1 내지 1:1, 70:1 내지 1:1, 65:1 내지 1:1, 60:1 내지 1:1, 55:1 내지 1:1, 50:1 내지 1:1, 45:1 내지 1:1, 40:1 내지 1:1, 35:1 내지 1:1, 30:1 내지 1:1, 25:1 내지 1:1, 20:1 내지 1:1, 15:1 내지 1:1, 10:1 내지 1:1, 5:1 내지 1:1, 4:1 내지 1:1, 3:1 내지 1:1, 2:1 내지 1:1이다.
본 발명에 따라 사용될 수 있는 B1:B2의 추가의 비는 1:1 내지 1:95, 1:1 내지 1:90, 1:1 내지 1:85, 1:1 내지 1:80, 1:1 내지 1:75, 1:1 내지 1:70, 1:1 내지 1:65, 1:1 내지 1:60, 1:1 내지 1:55, 1:1 내지 1:50, 1:1 내지 1:45, 1:1 내지 1:40, 1:1 내지 1:35, 1:1 내지 1:30, 1:1 내지 1:25, 1:1 내지 1:20, 1:1 내지 1:15, 1:1 내지 1:10, 1:1 내지 1:5, 1:1 내지 1:4, 1:1 내지 1:3, 1:1 내지 1:2이다.
이성질체
화합물 (A)의 치환기의 성질 및 화합물 (B)의 성질에 따라, 이들 화합물은 상이한 입체이성질체의 형태로 본 발명의 화합물 조합물에 존재할 수 있다. 이들 입체이성질체는, 예를 들어 거울상이성질체, 부분입체이성질체, 회전장애이성질체 또는 기하 이성질체이다. 따라서, 본 발명은 순수한 입체이성질체 및 이들 이성질체의 임의의 혼합물 둘 다를 포괄한다. 화합물이 2종 이상의 호변이성질체 형태로 평형으로 존재할 수 있는 경우에, 하나의 호변이성질체 설명에 의한 화합물에 대한 언급은 모든 호변이성질체 형태를 포함하는 것으로 간주되어야 한다. 화합물이 이성질체 형태 및/또는 호변이성질체 형태로 존재할 수 있는 경우에, 이러한 화합물은 상기 및 하기에 또한, 적용가능한 경우에, 심지어 이들이 각각의 경우에 구체적으로 언급되지 않은 경우에도, 상응하는 이성질체 및/또는 호변이성질체 형태 또는 그의 혼합물을 포함하는 것으로 이해된다.
염 / N-옥시드
본 발명의 화합물 조합물에 존재하는 화합물은 서로 독립적으로 유리 화합물 및/또는 적용가능한 경우에, 그의 농약 활성 염 및/또는 N-옥시드의 형태로 존재할 수 있다.
농약 활성 염은 무기 및 유기 산의 산 부가염 뿐만 아니라 통상의 염기의 염을 포함한다. 무기 산의 예는 할로겐화수소산, 예컨대 플루오린화수소, 염화수소, 브로민화수소 및 아이오딘화수소, 황산, 인산 및 질산, 및 산성 염, 예컨대 중황산나트륨 및 중황산칼륨이다. 유용한 유기 산은, 예를 들어 포름산, 탄산 및 알칸산, 예컨대 아세트산, 트리플루오로아세트산, 트리클로로아세트산 및 프로피온산, 및 또한 글리콜산, 티오시안산, 락트산, 숙신산, 시트르산, 벤조산, 신남산, 옥살산, 6 내지 20개의 탄소 원자를 갖는 포화 또는 단일- 또는 이중불포화 지방산, 알킬황산 모노에스테르, 알킬술폰산 (1 내지 20개의 탄소 원자를 갖는 직쇄 또는 분지형 알킬 라디칼을 갖는 술폰산), 아릴술폰산 또는 아릴디술폰산 (1 또는 2개의 술폰산 기를 보유하는 방향족 라디칼, 예컨대 페닐 및 나프틸), 알킬포스폰산 (1 내지 20개의 탄소 원자를 갖는 직쇄 또는 분지형 알킬 라디칼을 갖는 포스폰산), 아릴포스폰산 또는 아릴디포스폰산 (1 또는 2개의 포스폰산 라디칼을 보유하는 방향족 라디칼, 예컨대 페닐 및 나프틸)을 포함하며, 여기서 알킬 및 아릴 라디칼은 추가의 치환기, 예를 들어 p-톨루엔술폰산, 살리실산, p-아미노살리실산, 2-페녹시벤조산, 2-아세톡시벤조산을 보유할 수 있다.
본 발명의 화합물 조합물 또는 그의 중간체에 존재하는 화합물의 N-옥시드는 통상적인 방법에 의해, 예를 들어 과산화수소 (H2O2), 과산, 예를 들어 퍼옥시 황산 또는 퍼옥시 카르복실산, 예컨대 메타-클로로퍼옥시벤조산 또는 퍼옥시모노황산 (카로산)을 사용한 N-산화에 의해 간단한 방식으로 수득할 수 있다.
예를 들어, 상응하는 N-옥시드는 각각의 화합물로부터 출발하여 통상의 산화 방법을 사용하여, 예를 들어 화합물을 유기 과산, 예컨대 메타클로로퍼벤조산 (예를 들어 WO-A 2003/64572 또는 문헌 [J. Med. Chem. 38 (11), 1892-1903, 1995]); 또는 무기 산화제, 예컨대 과산화수소 (예를 들어 문헌 [J. Heterocyc. Chem. 18 (7), 1305-1308, 1981]) 또는 옥손 (예를 들어 문헌 [J. Am. Chem. Soc. 123 (25), 5962-5973, 2001])으로 처리함으로써 제조할 수 있다. 산화는 순수한 모노-N-옥시드 또는 상이한 N-옥시드의 혼합물을 유도할 수 있으며, 이는 통상적인 방법, 예컨대 크로마토그래피에 의해 분리될 수 있다.
결정질 형태
본 발명의 화합물 조합물에 존재하는 화합물은 다중 결정질 및/또는 무정형 형태로 존재할 수 있다. 결정질 형태는 각 경우에 개별 화합물 또는 그의 부가물의 비용매화 결정질 형태, 용매화물 및 수화물을 포함한다.
본 발명의 화합물 조합물 또는 그의 염에 존재하는 화합물의 용매화물은 화합물과 용매의 화학량론적 조성이다.
제제
본 발명은 추가로 본 발명에 따른 화합물 조합물을 포함하는, 원치 않는 미생물을 방제하기 위한 조성물에 관한 것이다. 조성물은 미생물 및/또는 그의 서식지에 적용될 수 있다.
조성물은 본 발명의 화합물 조합물 및 적어도 1종의 농업상 적합한 보조제, 예를 들어 담체(들) 및/또는 계면활성제(들)를 포함한다.
담체는 일반적으로 불활성인 고체 또는 액체, 천연 또는 합성, 유기 또는 무기 물질이다. 담체는 일반적으로, 예를 들어 식물, 식물 부분 또는 종자에 대한 화합물의 적용을 개선시킨다. 적합한 고체 담체의 예는 암모늄 염, 특히 황산암모늄, 인산암모늄 및 질산암모늄, 천연 암분, 예컨대 카올린, 점토, 활석, 백악, 석영, 아타풀자이트, 몬모릴로나이트 및 규조토, 실리카 겔 및 합성 암분, 예컨대 미분 실리카, 알루미나 및 실리케이트를 포함하나, 이에 제한되지는 않는다. 과립을 제조하는 데 전형적으로 유용한 고체 담체의 예는 파쇄 및 분획화된 천연 암석, 예컨대 방해석, 대리석, 부석, 세피올라이트 및 돌로마이트, 무기 및 유기 가루의 합성 과립 및 유기 물질, 예컨대 종이, 톱밥, 코코넛 쉘, 옥수수 속대 및 담배 줄기의 과립을 포함하나, 이에 제한되지는 않는다. 적합한 액체 담체의 예는 물, 유기 용매 및 그의 조합을 포함하나, 이에 제한되지는 않는다. 적합한 용매의 예는 극성 및 비극성 유기 화학 액체, 예를 들어 방향족 및 비방향족 탄화수소 (예컨대 시클로헥산, 파라핀, 알킬벤젠, 크실렌, 톨루엔, 테트라히드로나프탈렌, 알킬나프탈렌, 염소화 방향족 또는 염소화 지방족 탄화수소, 예컨대 클로로벤젠, 클로로에틸렌 또는 메틸렌 클로라이드), 알콜 및 폴리올 (임의로 또한 치환, 에테르화 및/또는 에스테르화될 수 있음, 예컨대 에탄올, 프로판올, 부탄올, 벤질알콜, 시클로헥산올 또는 글리콜), 케톤 (예컨대 아세톤, 메틸 에틸 케톤, 메틸 이소부틸 케톤 또는 시클로헥사논), 에스테르 (지방 및 오일 포함) 및 (폴리)에테르, 비치환 및 치환된 아민, 아미드 (예컨대 디메틸포름아미드 또는 지방산 아미드) 및 그의 에스테르, 락탐 (예컨대 N-알킬피롤리돈, 특히 N-메틸피롤리돈) 및 락톤, 술폰 및 술폭시드 (예컨대 디메틸 술폭시드), 식물 또는 동물 기원의 오일의 부류로부터의 것을 포함한다. 담체는 또한 액화된 기체상 증량제, 즉 표준 온도에서 및 표준 압력 하에 기체상인 액체, 예를 들어 에어로졸 추진제, 예컨대 할로탄화수소, 부탄, 프로판, 질소 및 이산화탄소일 수 있다.
바람직한 고체 담체는 점토, 활석 및 실리카로부터 선택된다.
바람직한 액체 담체는 물, 지방산 아미드 및 그의 에스테르, 방향족 및 비방향족 탄화수소, 락탐 및 탄산 에스테르로부터 선택된다.
담체의 양은 전형적으로 조성물의 1 내지 99.99 중량%, 바람직하게는 5 내지 99.9 중량%, 보다 바람직하게는 10 내지 99.5 중량%, 가장 바람직하게는 20 내지 99 중량%의 범위이다.
액체 담체는 전형적으로 조성물의 20 내지 90 중량%, 예를 들어 30 내지 80 중량%의 범위로 존재한다.
고체 담체는 전형적으로 조성물의 0 내지 50 중량%, 바람직하게는 5 내지 45 중량%, 예를 들어 10 내지 30 중량%의 범위로 존재한다.
조성물이 2종 이상의 담체를 포함하는 경우에, 약술된 범위는 담체의 총량을 지칭한다.
계면활성제는 이온성 (양이온성 또는 음이온성), 양쪽성 또는 비-이온성 계면활성제, 예컨대 이온성 또는 비-이온성 유화제(들), 발포체 형성제(들), 분산제(들), 습윤제(들), 침투 증진제(들) 및 그의 임의의 혼합물일 수 있다. 적합한 계면활성제의 예는 폴리아크릴산의 염, 리그노술폰산의 염 (예컨대 소듐 리그노술포네이트), 페놀술폰산 또는 나프탈렌술폰산의 염, 에틸렌 옥시드 및/또는 프로필렌 옥시드와 지방 알콜, 지방산 또는 지방 아민의 중축합물 (예를 들어, 폴리옥시에틸렌 지방산 에스테르 예컨대 피마자 오일 에톡실레이트, 폴리옥시에틸렌 지방 알콜 에테르, 예를 들어 알킬아릴 폴리글리콜 에테르), 치환된 페놀 (바람직하게는 알킬페놀 또는 아릴페놀) 및 그의 에톡실레이트 (예컨대 트리스티릴페놀 에톡실레이트), 술포숙신산 에스테르의 염, 타우린 유도체 (바람직하게는 알킬 타우레이트), 폴리에톡실화 알콜 또는 페놀의 인산 에스테르, 폴리올의 지방 에스테르 (예컨대 글리세롤, 소르비톨 또는 수크로스의 지방산 에스테르), 술페이트 (예컨대 알킬 술페이트 및 알킬 에테르 술페이트), 술포네이트 (예를 들어, 알킬술포네이트, 아릴술포네이트 및 알킬벤젠 술포네이트), 포스페이트 에스테르, 단백질 가수분해물, 리그노술파이트 폐액 및 메틸셀룰로스를 포함하나, 이에 제한되지는 않는다. 이 단락에서 염에 대한 임의의 언급은 바람직하게는 각각의 알칼리, 알칼리 토류 및 암모늄 염을 지칭한다.
바람직한 계면활성제는 폴리옥시에틸렌 지방 알콜 에테르, 폴리옥시에틸렌 지방산 에스테르, 알킬벤젠 술포네이트, 예컨대 칼슘 도데실벤젠술포네이트, 피마자유 에톡실레이트, 나트륨 리그노술포네이트 및 아릴페놀 에톡실레이트, 예컨대 트리스티릴페놀 에톡실레이트로부터 선택된다.
계면활성제의 양은 전형적으로 조성물의 5 내지 40 중량%, 예를 들어 10 내지 20 중량%의 범위이다.
적합한 보조제의 추가의 예는 발수제, 건조제, 결합제 (접착제, 점착제, 고정제, 예컨대 카르복시메틸셀룰로스, 분말, 과립 또는 라텍스 형태의 천연 및 합성 중합체, 예컨대 아라비아 검, 폴리비닐 알콜 및 폴리비닐 아세테이트, 천연 인지질 예컨대 세팔린 및 레시틴 및 합성 인지질, 폴리비닐피롤리돈 및 틸로스), 증점제 및 2차 증점제 (예컨대 셀룰로스 에테르, 아크릴산 유도체, 크산탄 검, 개질된 점토, 예를 들어 명칭 벤톤(Bentone) 하에 입수가능한 제품, 및 미분된 실리카), 안정화제 (예를 들어 저온 안정화제, 보존제 (예를 들어 디클로로펜 및 벤질 알콜 헤미포르말), 항산화제, 광 안정화제, 특히 UV 안정화제, 또는 화학적 및/또는 물리적 안정성을 개선시키는 다른 작용제), 염료 또는 안료 (예컨대 무기 안료, 예를 들어 산화철, 산화티타늄 및 프러시안 블루; 유기 염료, 예를 들어 알리자린, 아조 및 금속 프탈로시아닌 염료), 소포제 (예를 들어 실리콘 소포제 및 스테아르산마그네슘), 동결방지제, 점착제, 지베렐린 및 가공 보조제, 미네랄 및 식물성 오일, 퍼퓸, 왁스, 영양소 (미량 영양소, 예컨대 철, 망가니즈, 붕소, 구리, 코발트, 몰리브데넘 및 아연의 염 포함), 보호 콜로이드, 요변성 물질, 침투제, 봉쇄제 및 착물 형성제를 포함한다.
보조제의 선택은 본 발명의 화합물 조합물의 의도된 적용 방식 및/또는 상기 화합물 조합물에 존재하는 활성 화합물(들)의 물리적 특성에 따라 달라진다. 또한, 보조제는 특정한 특성 (기술적, 물리적 및/또는 생물학적 특성)을 조성물 또는 그로부터 제조된 사용 형태에 부여하도록 선택될 수 있다. 보조제의 선택은 조성물을 특정 필요에 맞게 맞춤화할 수 있게 한다.
본 발명의 조성물은 즉시 사용가능한 제제로서 최종 사용자에게 제공될 수 있으며, 즉 조성물은 적합한 장치, 예컨대 분무 또는 살분 장치에 의해 식물 또는 종자에 직접 적용될 수 있다. 대안적으로, 조성물은 사용 전에 바람직하게는 물로 희석되어야 하는 농축물의 형태로 최종 사용자에게 제공될 수 있다.
본 발명의 조성물은 통상적인 방식으로, 예를 들어 본 발명의 화합물 조합물을 상기 본원에 개시된 바와 같은 1종 이상의 적합한 보조제와 혼합함으로써 제조될 수 있다.
조성물은 살진균 유효량의 본 발명의 화합물 조합물을 포함한다. 용어 "유효량"은 재배 식물 상에서 유해 진균을 방제하는 데 또는 물질의 보호에 충분하고 처리된 식물에 실질적인 손상을 초래하지 않는 양을 나타낸다. 이러한 양은 넓은 범위에서 달라질 수 있고, 다양한 인자, 예컨대 방제될 진균 종, 처리된 재배 식물 또는 물질, 기후 조건 및 사용된 본 발명의 구체적 화합물 조합에 따라 달라진다. 통상적으로, 본 발명에 따른 조성물은 0.01 내지 99 중량%, 바람직하게는 0.05 내지 98 중량%, 보다 바람직하게는 0.1 내지 95 중량%, 보다 더 바람직하게는 0.5 내지 90 중량%, 가장 바람직하게는 1 내지 80 중량%의 본 발명의 화합물 조합물을 함유한다.
본 발명의 조성물은 임의의 통상적인 조성물 유형, 예컨대 용액 (예를 들어 수용액), 에멀젼, 수성 및 유성 현탁액, 분말 (예를 들어 습윤성 분말, 가용성 분말), 더스트, 페이스트, 과립 (예를 들어 가용성 과립, 유포용 과립), 현탁에멀젼 농축물, 본 발명의 화합물 조합물로 함침된 천연 또는 합성 생성물, 비료 및 또한 중합체성 성분의 미세캡슐화일 수 있다. 본 발명의 화합물 조합물은 현탁, 유화 또는 용해된 형태로 존재할 수 있다. 특히 적합한 조성물 유형의 예는 용액, 수용성 농축물 (예를 들어, SL, LS), 분산성 농축물 (DC), 현탁액 및 현탁액 농축물 (예를 들어, SC, OD, OF, FS), 유화성 농축물 (예를 들어, EC), 에멀젼 (예를 들어, EW, EO, ES, ME, SE), 캡슐 (예를 들어, CS, ZC), 페이스트, 파스틸, 습윤성 분말 또는 분진 (예를 들어, WP, SP, WS, DP, DS), 프레싱 (예를 들어, BR, TB, DT), 과립 (예를 들어, WG, SG, GR, FG, GG, MG), 살곤충 물품 (예를 들어, LN), 뿐만 아니라 식물 번식 재료, 예컨대 종자의 처리를 위한 겔 제제 (예를 들어, GW, GF)이다. 이들 및 추가의 조성물 유형은 미국 식품 농업 기구 (FAO)에 의해 정의된다. 개관은 문헌 ["Catalogue of pesticide formulation types and international coding system", Technical Monograph No. 2, 6th Ed. May 2008, Croplife International]에 제공되어 있다.
바람직하게는, 본 발명의 조성물은 하기 유형 중 하나의 형태이다: EC, SC, FS, SE, OD 및 WG, 보다 바람직하게는 EC, SC,OD 및 WG.
조성물 유형의 예 및 그의 제조에 대한 추가의 세부사항은 하기에 제공된다. 본 발명의 화합물 조합물의 약술된 양은 본 발명의 화합물 조합물에 존재하는 화합물 (A) 및 (B)의 총량을 지칭한다. 조성물의 임의의 추가의 성분의 2종 이상의 대표물, 예를 들어 습윤제, 결합제가 존재하는 경우에, 각각의 성분의 약술된 양은 상기 성분의 모든 대표물, 예를 들어 모든 습윤제, 모든 결합제, 모든 용매 등의 총량을 지칭한다.
i) 수용성 농축물 (SL, LS)
10-60 중량%의 본 발명의 화합물 조합물 및 5-15 중량%의 계면활성제 (예를 들어, 폴리옥시에틸렌 지방 알콜 에테르)를, 총량이 100 중량%가 되도록 하는 양의 물 및/또는 수용성 용매 (예를 들어 프로필렌 글리콜과 같은 알콜 또는 프로필렌 카르보네이트와 같은 카르보네이트)에 용해시킨다. 적용 전에, 농축물을 물로 희석한다.
ii) 분산성 농축물 (DC)
5-25 중량%의 본 발명의 화합물 조합물 및 1-10 중량%의 계면활성제 및/또는 결합제 (예를 들어, 폴리비닐피롤리돈)를 총량이 100 중량%가 되도록 하는 양의 유기 용매 (예를 들어, 시클로헥사논)에 용해시킨다. 물로 희석하여 분산액을 수득한다.
iii) 유화성 농축물 (EC)
15-70 중량%의 본 발명의 화합물 조합물 및 5-10 중량%의 계면활성제 (예를 들어, 칼슘 도데실벤젠술포네이트 및 피마자유 에톡실레이트의 혼합물)를 총량이 100 중량%가 되도록 하는 양의 수불용성 유기 용매 (예를 들어, 방향족 탄화수소 또는 지방산 아미드) 및 필요한 경우 추가의 수용성 용매에 용해시킨다. 물로 희석하여 에멀젼을 수득한다.
iv) 에멀젼 (EW, EO, ES)
5-40 중량%의 본 발명의 화합물 조합물 및 1-10 중량% 계면활성제 (예를 들어, 칼슘 도데실벤젠술포네이트 및 피마자유 에톡실레이트의 혼합물)를 20-40 중량% 수불용성 유기 용매 (예를 들어, 방향족 탄화수소) 중에 용해시킨다. 이 혼합물을 유화기에 의해 총량이 100 중량%가 되도록 하는 양의 물에 첨가한다. 생성된 조성물은 균질 에멀젼이다. 적용 전에 에멀젼을 물로 추가로 희석할 수 있다.
v) 현탁액 및 현탁액 농축물
v-1) 수계 (SC, FS)
적합한 분쇄 장비, 예를 들어 교반 볼 밀에서, 20-60 중량%의 본 발명의 화합물 조합물을 2-10 중량%의 계면활성제 (예를 들어, 나트륨 리그노술포네이트 및 폴리옥시에틸렌 지방 알콜 에테르), 0.1-2 중량%의 증점제 (예를 들어, 크산탄 검) 및 물의 첨가와 함께 분쇄하여 미세 활성 물질 현탁액을 제공한다. 물을 총량이 100 중량%가 되도록 하는 양으로 첨가한다. 물로 희석하여 활성 물질의 안정한 현탁액을 수득한다. FS 유형 조성물의 경우, 40 중량% 이하의 결합제 (예를 들어, 폴리비닐알콜)를 첨가한다.
v-2) 오일-기재 (OD, OF)
적합한 분쇄 장치, 예를 들어 교반 볼 밀에서, 20-60 중량%의 본 발명의 화합물 조합물을 2-10 중량%의 계면활성제 (예를 들어, 나트륨 리그노술포네이트 및 폴리옥시에틸렌 지방 알콜 에테르), 0.1-2 중량%의 증점제 (예를 들어, 개질된 점토, 특히 벤톤, 또는 실리카) 및 유기 담체를 첨가하면서 분쇄하여 미세한 활성 물질 오일 현탁액을 제공한다. 유기 담체를 총량이 100 중량%가 되도록 하는 양으로 첨가한다. 물로 희석하여 활성 물질의 안정한 분산액을 제공한다.
vi) 수분산성 과립 및 수용성 과립 (WG, SG)
50-80 중량%의 본 발명의 화합물 조합물을 계면활성제 (예를 들어, 나트륨 리그노술포네이트 및 폴리옥시에틸렌 지방 알콜 에테르)의 첨가와 함께 미세하게 분쇄하고, 기술적 장치 (예를 들어, 압출, 분무탑, 유동층)에 의해 수분산성 또는 수용성 과립으로 전환시킨다. 계면활성제는 총량이 100 중량%가 되도록 하는 양으로 사용된다. 물로 희석하여 활성 물질의 안정한 분산액 또는 용액을 수득한다.
vii) 수분산성 분말 및 수용성 분말 (WP, SP, WS)
50-80 중량%의 본 발명의 화합물 조합물을 적합한 밀, 바람직하게는 회전자-고정자 밀에서 1-8 중량%의 계면활성제 (예를 들어, 나트륨 리그노술포네이트, 폴리옥시에틸렌 지방 알콜 에테르) 및 총량이 100 중량%가 되도록 하는 양의 고체 담체, 예를 들어 실리카 겔의 첨가와 함께 분쇄한다. 물로 희석하여 활성 물질의 안정한 분산액 또는 용액을 수득한다.
viii) 겔 (GW, GF)
적합한 밀, 예를 들어 교반 볼 밀에서, 5-25 중량%의 본 발명의 화합물 조합물을 3-10 중량%의 계면활성제 (예를 들어, 나트륨 리그노술포네이트), 1-5 중량%의 결합제 (예를 들어, 카르복시메틸셀룰로스) 및 100 중량%의 총량이 되도록 하는 양의 물의 첨가와 함께 분쇄한다. 이는 활성 물질의 미세 현탁액을 생성한다. 물로 희석하여 활성 물질의 안정한 현탁액을 수득한다.
ix) 마이크로에멀젼 (ME)
5-20 중량%의 본 발명의 화합물 조합물을 5-30 중량%의 유기 용매 블렌드 (예를 들어, 지방산 디메틸아미드 및 시클로헥사논), 10-25 중량%의 계면활성제 블렌드 (예를 들어, 폴리옥시에틸렌 지방 알콜 에테르 및 아릴페놀 에톡실레이트), 및 총량이 100 중량%가 되도록 하는 양의 물에 첨가한다. 이 혼합물을 1시간 동안 교반하여 자발적으로 열역학적으로 안정한 마이크로에멀젼을 수득한다.
x) 마이크로캡슐 (CS)
5-50 중량%의 본 발명의 화합물 조합물, 0-40 중량%의 수불용성 유기 용매 (예를 들어 방향족 탄화수소), 2-15 중량%의 아크릴 단량체 (예를 들어 메틸메타크릴레이트, 메타크릴산 및 디- 또는 트리아크릴레이트)를 포함하는 오일 상을 보호 콜로이드 (예를 들어 폴리비닐 알콜)의 수용액에 분산시킨다. 라디칼 개시제에 의해 개시되는 라디칼 중합은 폴리(메트)아크릴레이트 마이크로캡슐의 형성을 가져온다. 대안적으로, 5-50 중량%의 본 발명의 화합물 조합물, 0-40 중량%의 수불용성 유기 용매 (예를 들어, 방향족 탄화수소), 및 이소시아네이트 단량체 (예를 들어, 디페닐메텐-4,4'-디이소시아네이트)를 포함하는 오일 상을 보호 콜로이드 (예를 들어, 폴리비닐 알콜)의 수용액에 분산시킨다. 폴리아민 (예를 들어 헥사메틸렌디아민)의 첨가는 폴리우레아 마이크로캡슐의 형성을 가져온다. 단량체의 양은 총 CS 조성물의 1-10 중량%이다.
xi) 살분성 분말 (DP, DS)
1-10 중량%의 본 발명의 화합물 조합물을 미분하고, 100 중량%의 총량이 되도록 양의 고체 담체, 예를 들어 미분된 카올린과 친밀하게 혼합한다.
xii) 과립 (GR, FG)
0.5-30 중량%의 본 발명의 화합물 조합물을 미세하게 분쇄하고, 총량이 100 중량%가 되도록 하는 양의 고체 담체 (예를 들어, 실리케이트)와 회합한다. 과립화는 압출, 분무-건조 또는 유동층에 의해 달성된다.
xiii) 초저부피 액체 (UL)
1-50 중량%의 본 발명의 화합물 조합물을 총량이 100 중량%가 되도록 하는 양의 유기 용매, 예를 들어 방향족 탄화수소에 용해시킨다.
조성물 유형 i) 내지 xiii)은 임의로 추가의 보조제, 예컨대 0.1-1 중량%의 보존제, 0.1-1 중량%의 소포제, 0.1-1 중량%의 염료 및/또는 안료, 및 5-10 중량%의 동결방지제를 포함할 수 있다.
추가의 활성 성분
본 발명에 따른 화합물 조합물은 그 자체로 또는 그의 조성물 / 제제로 사용될 수 있고, 추가의 공지된 활성 성분, 예를 들어 생물학적 방제제, 살박테리아제, 살진드기제, 살선충제 또는 살곤충제와 혼합되어, 예를 들어 활성 스펙트럼을 넓히거나 또는 내성의 발생을 방지할 수 있다.
유용한 혼합 파트너는, 예를 들어 살곤충제, 살진드기제, 살선충제 및 살박테리아제를 포함한다 (또한 문헌 [Pesticide Manual, 14th ed.] 참조).
다른 공지된 활성 성분, 예컨대 제초제, 또는 비료 및 성장 조절제, 완화제 및/또는 신호화학물질과의 혼합물이 또한 가능하다.
"살곤충제" 뿐만 아니라 용어 "살곤충"은 곤충의 사멸률을 증가시키거나 성장 속도를 억제하는 물질의 능력을 지칭한다. 본원에 사용된 용어 "곤충"은 "곤충강"의 모든 유기체를 포함한다.
"살선충제" 및 "살선충"은 선충류의 사망률을 증가시키거나 성장 속도를 억제하는 물질의 능력을 지칭한다. 일반적으로, 용어 "선충류"는 상기 유기체의 알, 유충, 유충 및 성숙 형태를 포함한다.
"살진드기제" 및 "살진드기"는 거미강, 진드기 아강에 속하는 외부기생충의 사멸률을 증가시키거나 또는 성장 속도를 억제하는 물질의 능력을 지칭한다.
본원에 사용된 용어 "생물학적 방제"는 생물학적 방제제의 사용 또는 이용에 의한 유해 유기체, 예컨대 식물병원성 진균 및/또는 곤충 및/또는 진드기 및/또는 선충류의 방제로서 정의된다.
본원에 사용된 용어 "생물학적 방제제"는 생물학적 방제의 목적을 위한, 유해 유기체 이외의 유기체 및/또는 이러한 유기체에 의해 생산된 단백질 또는 2차 대사물로서 정의된다. 제2 유기체의 돌연변이체는 생물학적 방제제의 정의 내에 포함될 것이다. 용어 "돌연변이체"는 모 균주의 변이체 뿐만 아니라 살충 활성이 모 균주에 의해 발현되는 것보다 더 큰 돌연변이체 또는 변이체를 수득하는 방법을 지칭한다. "모 균주"는 돌연변이유발 전의 원래 균주로서 본원에 정의된다. 이러한 돌연변이체를 수득하기 위해, 모 균주를 화학물질, 예컨대 N-메틸-N'-니트로-N-니트로소구아니딘, 에틸메탄술폰으로, 또는 감마, X선 또는 UV-조사를 사용한 조사에 의해, 또는 통상의 기술자에게 널리 공지된 다른 수단에 의해 처리할 수 있다. 생물학적 방제제의 공지된 메카니즘은 뿌리의 표면 상의 공간에 대해 진균을 능가함으로써 뿌리썩음병을 방제하는 장 박테리아를 포함한다. 박테리아 독소, 예컨대 항생제는 병원체를 방제하는 데 사용되었다. 독소는 단리되어 식물에 직접 적용될 수 있거나, 또는 박테리아 종이 계내에서 독소를 생산하도록 투여될 수 있다.
"변이체"는 본문에 나타낸 바와 같은 NRRL 또는 ATCC 수탁 번호의 모든 식별 특성을 갖는 균주이고, 고엄격성 조건 하에 NRRL 또는 ATCC 수탁 번호의 게놈에 혼성화하는 게놈을 갖는 것으로 확인될 수 있다.
"혼성화"는 1개 이상의 폴리뉴클레오티드가 반응하여 뉴클레오티드 잔기의 염기 사이의 수소 결합을 통해 안정화되는 복합체를 형성하는 반응을 지칭한다. 수소 결합은 왓슨-크릭 염기쌍형성, 후그스타인(Hoogstein) 결합에 의해, 또는 임의의 다른 서열-특이적 방식으로 발생할 수 있다. 복합체는 듀플렉스 구조를 형성하는 2개의 가닥, 다중-가닥 복합체를 형성하는 3개 이상의 가닥, 단일 자기-혼성화 가닥, 또는 이들의 임의의 조합을 포함할 수 있다. 혼성화 반응은 상이한 "엄격도" 조건 하에 수행될 수 있다. 일반적으로, 낮은 엄격성 혼성화 반응은 10 X SSC 또는 등가 이온 강도/온도의 용액에서 약 40℃에서 수행된다. 중간의 엄격성 혼성화는 전형적으로 6 X SSC에서 약 50℃에서 수행되고, 높은 엄격성 혼성화 반응은 일반적으로 1 X SSC에서 약 60℃에서 수행된다.
표시된 NRRL 또는 ATCC 수탁 번호의 변이체는 또한 표시된 NRRL 또는 ATCC 수탁 번호의 게놈과 85% 초과, 보다 바람직하게는 90% 초과 또는 보다 바람직하게는 95% 초과의 서열 동일성을 갖는 게놈 서열을 갖는 균주로 정의될 수 있다. 폴리뉴클레오티드 또는 폴리뉴클레오티드 영역 (또는 폴리펩티드 또는 폴리펩티드 영역)이 또 다른 서열에 대해 특정 백분율 (예를 들어, 80%, 85%, 90% 또는 95%)의 "서열 동일성"을 갖는다는 것은, 정렬된 경우에 그 백분율의 염기 (또는 아미노산)가 2개의 서열의 비교시에 동일한 것을 의미한다. 이러한 정렬 및 퍼센트 상동성 또는 서열 동일성은 관련 기술분야에 공지된 소프트웨어 프로그램, 예를 들어 문헌 [Current Protocols in Molecular Biology (F. M. Ausubel et al., eds., 1987)]에 기재된 것을 사용하여 결정될 수 있다.
NRRL은 미국 61604 일리노이주 피오리아 노스 유니버시티 스트리트 1815 미국 농무부 농업 연구소 국립 농업 이용 연구 센터 소재의, 특허 절차의 목적상 미생물 기탁의 국제적 승인에 관한 부다페스트 조약 하에 미생물 균주를 기탁하는 목적을 위한 국제 기탁 기관인 아그리컬쳐럴 리서치 서비스 컬쳐 콜렉션(Agricultural Research Service Culture Collection)에 대한 약어이다.
ATCC는 미국 10110 버지니아주 마나사스 유니버시티 블러바드 10801 ATCC 페이턴트 디포지터리 소재의, 특허 절차의 목적상 미생물 기탁의 국제적 승인에 관한 부다페스트 조약 하에 미생물 균주를 기탁하는 목적을 위한 국제 기탁 기관인 아메리칸 타입 컬쳐 콜렉션(American Type Culture Collection)에 대한 약어이다.
본 발명의 화합물 조합물과 조합될 수 있는 생물학적 방제제의 예는 하기와 같다:
(A) 하기의 군으로부터 선택된 항박테리아제:
(A1) 박테리아, 예컨대 (A1.1) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (바이엘 크롭사이언스 엘피 (미국)로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고 미국 특허 번호 6,060,051에 기재됨); (A1.2) 바실루스 아밀로리퀘파시엔스(Bacillus amyloliquefaciens), 특히 균주 D747 (미국 세르티스로부터 더블 니켈™ 하에 입수가능함, 수탁 번호 FERM BP-8234이고 미국 특허 번호 7,094,592에 개시됨); (A1.3) 바실루스 푸밀루스, 특히 균주 BU F-33 (NRRL 수탁 번호 50185를 가짐); (A1.4) 바실루스 서브틸리스 변종 아밀로리퀘파시엔스 균주 FZB24 (미국 노보자임스로부터 타에그로® 하에 입수가능함); (A1.5) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주; 및
(A2) 진균, 예컨대 (A2.1) 아우레오바시디움 풀루란스, 특히 균주 DSM14940의 출아포자; (A2.2) 균주 DSM 14941의 아우레오바시디움 풀루란스 출아포자; (A2.3) 아우레오바시디움 풀루란스, 특히 균주 DSM14940 및 DSM14941의 출아포자의 혼합물;
(B) 하기의 군으로부터 선택된 생물학적 살진균제;
(B1) 박테리아, 예를 들어 (B1.1) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨); (B1.2) 바실루스 푸밀루스, 특히 균주 QST2808 (미국 소재 바이엘 크롭사이언스 엘피로부터 소나타® 하에 입수가능함, 수탁 번호 NRRL B-30087을 갖고 미국 특허 번호 6,245,551에 기재됨); (B1.3) 바실루스 푸밀루스, 특히 균주 GB34 (독일 소재 바이엘 아게로부터 일드 쉴드® 하에 입수가능함); (B1.4) 바실루스 푸밀루스, 특히 균주 BU F-33 (NRRL 수탁 번호 50185를 가짐); (B1.5) 바실루스 아밀로리퀘파시엔스(Bacillus amyloliquefaciens), 특히 균주 D747 (미국 소재 세르티스로부터 더블 니켈™ 하에 입수가능함, 수탁 번호 FERM BP-8234를 갖고, 미국 특허 번호 7,094,592에 개시됨); (B1.6) 바실루스 서브틸리스 Y1336 (대만 소재 비온-테크로부터 바이오박® WP 하에 입수가능함, 대만에 등록 번호 4764, 5454, 5096 및 5277로 생물학적 살진균제로서 등록됨); (B1.7) 바실루스 아밀로리퀘파시엔스 균주 MBI 600 (바스프 에스이로부터 서브틸렉스 하에 입수가능함); (B1.8) 바실루스 서브틸리스 균주 GB03 (독일 소재 바이엘 아게로부터 코디악® 하에 입수가능함); (B1.9) 바실루스 서브틸리스 변종 아밀로리퀘파시엔스 균주 FZB24 (버지니아주 살렘 소재 노보자임스 바이올로지칼스 인크. 또는 노스 캐롤라이나주 그린스보로 소재 신젠타 크롭 프로텍션, 엘엘씨로부터 살진균제 타에그로® 또는 타에그로® ECO 하에 입수가능함 (EPA 등록 번호 70127-5); (B1.10) 바실루스 미코이데스, 단리물 J (세르티스 유에스에이로부터 BmJ TGAI 또는 WG 하에 입수가능함); (B1.11) 바실루스 리케니포르미스, 특히 균주 SB3086 (노보자임스로부터 에코가드™ 생물살진균제 및 그린 릴리프 하에 입수가능함); (B1.12) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고, 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주,
(C1) 지방산 또는 유도체, 예를 들어 (C1.1) 불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%는 C14 내지 C20의 범위인 조성물 (예를 들어 알파바이오 페스티시드즈 또는 바이엘 아게의 FLiPPER).
일부 실시양태에서, 생물학적 방제제는 펜기신 또는 플리파스타틴-유형 화합물, 이투린-유형 화합물 및/또는 서팩틴-유형 화합물을 생산하는 바실루스 서브틸리스 또는 바실루스 아밀로리퀘파시엔스 균주이다. 배경기술에 대해서는, 하기 종설 논문을 참조한다: Ongena, M., et al., "Bacillus Lipopeptides: Versatile Weapons for Plant Disease Biocontrol," Trends in Microbiology, Vol 16, No. 3, March 2008, pp. 115-125. 리포펩티드를 생산할 수 있는 바실루스 균주는 바실루스 서브틸리스 QST713 (NRRL 수탁 번호 B21661을 갖고 미국 특허 번호 6,060,051에 기재된, 미국 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함), 바실루스 아밀로리퀘파시엔스 균주 D747 (미국 소재 세르티스로부터 더블 니켈™ 하에 입수가능함, 수탁 번호 FERM BP-8234를 갖고, 미국 특허 번호 7,094,592에 개시됨); 바실루스 서브틸리스 MBI600 (베커 언더우드(Becker Underwood)로부터 서브틸렉스® 하에 입수가능함, US EPA 등록 번호 71840-); 바실루스 서브틸리스 Y1336 (대만 소재 비온-테크로부터 바이오박® WP로 입수가능함, 등록 번호 4764, 5454, 5096 및 5277로 생물학적 살진균제로 등록됨); 바실루스 아밀로리퀘파시엔스, 특히 균주 FZB42 (독일 소재 ABiTEP로부터 리조비탈(RHIZOVITALR)® 하에 입수가능함); 및 바실루스 서브틸리스 변종 아밀로리퀘파시엔스 FZB24 (진균제 타에그로® 또는 타에그로® ECO (EPA 등록 번호 70127-5)로서 버지니아주 살렘 소재 노보자임스 바이올로지칼스 인크. 또는 노스 캐롤라이나주 그린스보로 소재 신젠타 크롭 프로텍션, 엘엘씨로부터 입수가능함); 및
(B2) 진균, 예를 들어: (B2.1) 코니오티리움 미니탄스(Coniothyrium minitans), 특히 균주 CON/M/91-8 (수탁 번호 DSM-9660; 예를 들어 바이엘로부터의 콘탄스(Contans)®); (B2.2) 메치니코위아 프룩티콜라(Metschnikowia fructicola), 특히 균주 NRRL Y-30752 (예를 들어 쉐머(Shemer)®); (B2.3) 미크로스파에롭시스 오크라세아(Microsphaeropsis ochracea) (예를 들어 프로피타(Prophyta)로부터의 미크록스(Microx)®); (B2.5) 트리코더마 아트로비리데(Trichoderma atroviride)를 포함한 트리코더마 종, 국제 출원 번호 PCT/IT2008/000196에 기재된 균주 SC1; (B2.6) 트리코더마 하르지아눔 리파이(Trichoderma harzianum rifai) 균주 KRL-AG2 (균주 T-22, /ATCC 208479로도 공지됨, 예를 들어 미국 소재 바이오웍스(BioWorks)로부터의 플랜트쉴드(PLANTSHIELD) T-22G, 루트쉴드(Rootshield)® 및 터프쉴드(TurfShield)); (B2.14) 더블유.에프. 스토네만 캄파니 엘엘씨(W.F. Stoneman Company LLC)로부터의 글리오클라디움 로세움(Gliocladium roseum), 균주 321U; (B2.35) 탈라로미세스 플라부스(Talaromyces flavus), 균주 V117b; (B2.36) 트리코더마 아스페렐룸(Trichoderma asperellum), 이사그로(Isagro)로부터의 균주 ICC 012, (B2.37) 트리코더마 아스페렐룸(Trichoderma asperellum), 균주 SKT-1 (예를 들어 쿠미아이 케미칼 인더스트리(Kumiai Chemical Industry)로부터의 에코-홉(ECO-HOPE)®; (B2.38) 트리코더마 아트로비리데(Trichoderma atroviride), 균주 CNCM I-1237 (예를 들어, 프랑스 아그라욱신 소재 에스퀴브(Esquive)® WP); (B2.39) 트리코더마 아트로비리데, 균주 번호 V08/002387; (B2.40) 트리코더마 아트로비리데, 균주 NMI 번호 V08/002388; (B2.41) 트리코더마 아트로비리데, 균주 NMI 번호 V08/002389; (B2.42) 트리코더마 아트로비리데, 균주 NMI 번호 V08/002390; (B2.43) 트리코더마 아트로비리데, 균주 LC52 (예를 들어 아그림 테크놀로지스 리미티드(Agrimm Technologies Limited)의 테네트(Tenet)); (B2.44) 트리코더마 아트로비리데, 균주 ATCC 20476 (IMI 206040); (B2.45) 트리코더마 아트로비리데, 균주 T11 (IMI352941/ CECT20498); (B2.46) 트리코더마 하르마툼(Trichoderma harmatum); (B2.47) 트리코더마 하르지아눔; (B2.48) 트리코더마 하르지아눔 리파이 T39 (예를 들어 미국 마크테심 소재 트리코덱스(Trichodex)®); (B2.49) 트리코더마 하르지아눔, 특히 균주 KD (예를 들어 바이올로지칼 컨트롤 프로덕츠(Biological Control Products), SA로부터의 트리코플러스(Trichoplus) (베커 언더우드에 의해 입수함)); (B2.50) 트리코더마 하르지아눔, 균주 ITEM 908 (예를 들어 코퍼트로부터의 트리아눔-P); (B2.51) 트리코더마 하르지아눔, 균주 TH35 (예를 들어, 미콘트롤(Mycontrol)의 루트-프로); (B2.52) 트리코더마 비렌스(Trichoderma virens) (글리오클라디움 비렌스(Gliocladium virens)로도 공지됨), 특히 균주 GL-21 (예를 들어 미국 세르티스의 소일가드(SoilGard) 12G); (B2.53) 트리코더마 비리데, 균주 TV1(예를 들어 코퍼트의 트리아눔-P); (B2.54) 암펠로미세스 퀴스쿠알리스(Ampelomyces quisqualis), 특히 균주 AQ 10 (예를 들어 인트라켐바이오 이탈리아(IntrachemBio Italia)의 AQ 10®); (B2.56) 아우레오바시디움 풀루란스, 특히 균주 DSM14940의 출아포자; (B2.57) 아우레오바시디움 풀루란스, 특히 균주 DSM 14941의 출아포자;(B2.58) 아우레오바시디움 풀루란스, 특히 균주 DSM14940 및 DSM 14941의 출아포자의 혼합물 (예를 들어 스위스 바이오-펌(bio-ferm)의 보텍터(Botector)®); (B2.64) 클라도스포리움 클라도스포리오이데스(Cladosporium cladosporioides), 균주 H39 (스티칭 디엔스트 란드부운디히 온데르조크(Stichting Dienst Landbouwkundig Onderzoek)에 의함); (B2.69) 글리오클라디움 카테눌라툼(Gliocladium catenulatum) (동의어: 클로노스타키스 로세아 에프. 카테눌라테(Clonostachys rosea f. catenulate)) 균주 J1446 (예를 들어 아그바이오 인크.(AgBio Inc.)의 프레스톱(Prestop)® 및 또한 예를 들어 케미라 아그로 오이(Kemira Agro Oy)의 프리마스톱(Primastop)®); (B2.70) 균주 KV01의 레카니실리움 레카니이(Lecanicillium lecanii) (이전에 베르티실리움 레카니이(Verticillium lecanii)로 공지됨) 분생자 (예를 들어 코퍼트(Koppert)/아리스타(Arysta)의 베르탈렉(Vertalec)®); (B2.71) 페니실리움 베르미쿨라툼(Penicillium vermiculatum); (B2.72) 피키아 아노말라(Pichia anomala), 균주 WRL-076 (NRRL Y-30842); (B2.75) 트리코더마 아트로비리데, 균주 SKT-1 (FERM P-16510); (B2.76) 트리코더마 아트로비리데, 균주 SKT-2 (FERM P-16511); (B2.77) 트리코더마 아트로비리데, 균주 SKT-3 (FERM P-17021); (B2.78) 트리코더마 감시이(Trichoderma gamsii) (이전에 티. 비리데(T. viride)), 균주 ICC080 (IMI CC 392151 CABI, 예를 들어 아그로비오솔 데 멕시코 에스.에이. 데 씨.브이.(AGROBIOSOL DE MEXICO, S.A. DE C.V.)의 바이오더마(BioDerma)); (B2.79) 트리코더마 하르지아눔, 균주 DB 103 (예를 들어, 다구타트 바이오랩(Dagutat Biolab)의 티-그로(T-Gro) 7456); (B2.80) 트리코더마 폴리스포룸(Trichoderma polysporum), 균주 IMI 206039 (예를 들어 스웨덴 소재 비나브 바이오-이노베이션 아베(BINAB Bio-Innovation AB)의 비나브 TF WP); (B2.81) 트리코더마 스트로마티쿰(Trichoderma stromaticum) (예를 들어 브라질 세플라크의 트리코밥(Tricovab)); (B2.83) 울로클라디움 오우데만시이(Ulocladium oudemansii), 특히 균주 HRU3 (예를 들어 뉴질랜드 소재 보트리-젠 리미티드(Botry-Zen Ltd)의한 보트리-젠(Botry-Zen)®); (B2.84) 베르티실리움 알보-아트룸(Verticillium albo-atrum) (이전에 브이. 달리아에(V. dahliae)), 균주 WCS850 (CBS 276.92; 예를 들어 트리 케어 이노베이션스(Tree Care Innovations)의 더치 트리그(Dutch Trig)); (B2.86) 베르티실리움 클라미도스포리움(Verticillium chlamydosporium); (B2.87) 트리코더마 아스페렐룸 균주 ICC 012 및 트리코더마 감시이 균주 ICC 080의 혼합물 (예를 들어 미국 바이엘 크롭사이언스 엘피로부터의 바이오-탐(BIO-TAM)™ 로 공지된 제품)을 포함한다.
본 발명의 화합물 조합물과 조합될 수 있는 생물학적 방제제의 추가의 예는 하기와 같다:
바실루스 세레우스, 특히 비. 세레우스 균주 CNCM I-1562 및 바실루스 피르무스, 균주 I-1582 (수탁 번호 CNCM I-1582), 바실루스 서브틸리스 균주 OST 30002 (수탁 번호 NRRL B-50421), 바실루스 투린기엔시스(Bacillus thuringiensis), 특히 비. 투린기엔시스 아종 이스라엘렌시스(israelensis) (혈청형 H-14), 균주 AM65-52 (수탁 번호 ATCC 1276), 비. 투린기엔시스 아종 아이자와이(aizawai), 특히 균주 ABTS-1857 (SD-1372), 비. 투린기엔시스 아종 쿠르스타키(kurstaki) 균주 HD-1, 비. 투린기엔시스 아종 테네브리오니스(tenebrionis) 균주 NB 176 (SD-5428), 파스테우리아 페네트란스(Pasteuria penetrans), 파스테우리아(Pasteuria) 종 (로틸렌쿨루스 레니포르미스(Rotylenchulus reniformis) 선충류)-PR3 (수탁 번호 ATCC SD-5834), 스트렙토미세스 미크로플라부스(Streptomyces microflavus) 균주 AQ6121 (= QRD 31.013, NRRL B-50550), 및 스트렙토미세스 갈부스(Streptomyces galbus) 균주 AQ 6047 (수탁 번호 NRRL 30232)로 이루어진 군으로부터 선택된 박테리아;
뷰베리아 바시아나(Beauveria bassiana), 특히 균주 ATCC 74040, 레카니실리움(Lecanicillium) 종, 특히 균주 HRO LEC 12, 메타리지움 아니소플리아에(Metarhizium anisopliae), 특히 균주 F52 (DSM3884 또는 ATCC 90448), 파에실로미세스 푸모소로세우스(Paecilomyces fumosoroseus) (현재: 이사리아 푸모소로세아(Isaria fumosorosea)), 특히 균주 IFPC 200613, 또는 균주 아폽카(Apopka) 97 (수탁 번호 ATCC 20874), 및 파에실로미세스 릴라시누스(Paecilomyces lilacinus), 특히 피. 릴라시누스(P. lilacinus) 균주 251 (AGAL 89/030550)로 이루어진 군으로부터 선택된 진균 및 효모;
아독소피에스 오라나(Adoxophyes orana) (여름 과일 토르트릭스)과립병 바이러스 (GV), 시디아 포모넬라(Cydia pomonella) (코들링 나방) 과립병 바이러스 (GV), 헬리코베르파 아르미게라(Helicoverpa armigera) (목화다래벌레) 핵 다각체병 바이러스 (NPV), 스포도프테라 엑시구아(Spodoptera exigua) (비트 거염벌레) mNPV, 스포도프테라 프루기페르다(Spodoptera frugiperda) (가을 거염벌레) mNPV, 및 스포도프테라 리토랄리스(Spodoptera littoralis) (아프리카 목화 잎벌레) NPV로 이루어진 군으로부터 선택된 바이러스.
식물 또는 식물 부분 또는 식물 기관에 '접종물'로서 첨가될 수 있고, 그의 특정한 특성에 의해 식물 성장 및 식물 건강을 촉진하는 박테리아 및 진균. 예는 아그로박테리움(Agrobacterium) 종, 아조리조비움 카울리노단스(Azorhizobium caulinodans), 아조스피릴룸(Azospirillum) 종, 아조토박터(Azotobacter) 종, 브라디리조비움(Bradyrhizobium) 종, 부르크홀데리아(Burkholderia) 종, 특히 부르크홀데리아 세파시아(Burkholderia cepacia) (이전에 슈도모나스 세파시아(Pseudomonas cepacia)로 공지됨), 기가스포라(Gigaspora) 종 또는 기가스포라 모노스포룸(Gigaspora monosporum), 글로무스(Glomus) 종, 락카리아(Laccaria) 종, 락토바실루스 부크네리(Lactobacillus buchneri), 파라글로무스(Paraglomus) 종, 피솔리투스 틴크토루스(Pisolithus tinctorus), 슈도모나스(Pseudomonas) 종, 리조비움(Rhizobium) 종, 특히 리조비움 트리폴리이(Rhizobium trifolii), 리조포곤(Rhizopogon) 종, 스클레로데르마(Scleroderma) 종, 수일루스(Suillus) 종 및 스트렙토미세스(Streptomyces) 종이다.
생물학적 방제제로서 사용될 수 있는 단백질 및 2차 대사물을 포함한 미생물에 의해 형성된 식물 추출물 및 생성물, 예컨대 알리움 사티붐(Allium sativum), 아르테미시아 아브신티움(Artemisia absinthium), 아자디라크틴(azadirachtin), 바이오키퍼 WP, 카시아 니그리칸스(Cassia nigricans), 셀라스트루스 안굴라투스(Celastrus angulatus), 케노포디움 안텔민티쿰(Chenopodium anthelminticum), 키틴(chitin), 아르무르-젠(Armour-Zen), 드리오프테리스 필릭스-마스(Dryopteris filix-mas), 에퀴세툼 아르벤세(Equisetum arvense), 포툰 아자(Fortune Aza), 푼가스톱(Fungastop), 헤드 업(Heads Up) (케노포디움 퀴노아 사포닌(Chenopodium quinoa saponin) 추출물), 피레트룸(Pyrethrum)/피레트린스(Pyrethrins), 쿠아시아 아마라(Quassia amara), 퀘르쿠스(Quercus), 퀼라야(Quillaja), 레갈리아(Regalia), "레퀴엠(Requiem)™ 살곤충제", 로테논, 리아니아(ryania)/리아노딘(ryanodine), 심피툼 오피시날레(Symphytum officinale), 타나세툼 불가레(Tanacetum vulgare), 티몰(thymol), 트리액트(Triact) 70, 트리콘(TriCon), 트로파에올룸 마주스(Tropaeulum majus), 우르티카 디오이카(Urtica dioica), 베라트린(Veratrin), 비스쿰 알붐(Viscum album), 브라시카세아에(Brassicaceae) 추출물, 특히 유지종자 평지 분말 또는 겨자 분말.
불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%는 C14 내지 C20의 범위인 조성물 (예를 들어, 알파바이오 페스티시드즈 또는 바이엘 아게의 FLiPPER).
본 발명의 화합물 조합물과 혼합될 수 있는 살곤충제, 살진드기제 및 살선충제 각각의 예는 하기와 같다:
(1) 아세틸콜린에스테라제 (AChE) 억제제, 예컨대, 예를 들어, 카르바메이트, 예를 들어 알라니카르브, 알디카르브, 벤디오카르브, 벤푸라카르브, 부토카르복심, 부톡시카르복심, 카르바릴, 카르보푸란, 카르보술판, 에티오펜카르브, 페노부카르브, 포르메타네이트, 푸라티오카르브, 이소프로카르브, 메티오카르브, 메토밀, 메톨카르브, 옥사밀, 피리미카르브, 프로폭수르, 티오디카르브, 티오파녹스, 트리아자메이트, 트리메타카르브, XMC 및 크실릴카르브; 또는 유기포스페이트, 예를 들어 아세페이트, 아자메티포스, 아진포스-에틸, 아진포스-메틸, 카두사포스, 클로르에톡시포스, 클로르펜빈포스, 클로르메포스, 클로르피리포스-메틸, 쿠마포스, 시아노포스, 데메톤-S-메틸, 디아지논, 디클로르보스/DDVP, 디크로토포스, 디메토에이트, 디메틸빈포스, 디술포톤, EPN, 에티온, 에토프로포스, 팜푸르, 페나미포스, 페니트로티온, 펜티온, 포스티아제이트, 헵테노포스, 이미시아포스, 이소펜포스, 이소프로필 O-(메톡시아미노티오포스포릴) 살리실레이트, 이속사티온, 말라티온, 메카르밤, 메타미도포스, 메티다티온, 메빈포스, 모노크로토포스, 날레드, 오메토에이트, 오시데메톤-메틸, 파라티온-메틸, 펜토에이트, 포레이트, 포살론, 포스메트, 포스파미돈, 폭심, 피리미포스-메틸, 프로페노포스, 프로페탐포스, 프로티오포스, 피라클로포스, 피리다펜티온, 퀴날포스, 술포텝, 테부피림포스, 테메포스, 테르부포스, 테트라클로르빈포스, 티오메톤, 트리아조포스, 트리클로르폰 및 바미도티온.
(2) GABA-게이팅 클로라이드 채널 차단제, 예컨대 예를 들어 시클로디엔-유기염소, 예를 들어 클로르단 및 엔도술판 또는 페닐피라졸 (피프롤), 예를 들어 에티프롤 및 피프로닐.
(3) 나트륨 채널 조정제, 예컨대, 예를 들어, 피레트로이드, 예를 들어 아크리나트린, 알레트린, d-시스-트랜스 알레트린, d-트랜스 알레트린, 비펜트린, 비오알레트린, 비오알레트린 s-시클로펜테닐 이성질체, 비오레스메트린, 시클로프로트린, 시플루트린, 베타-시플루트린, 시할로트린, 람다-시할로트린, 감마-시할로트린, 시페르메트린, 알파-시페르메트린, 베타-시페르메트린, 세타-시페르메트린, 제타-시페르메트린, 시페노트린 [(1R)-트랜스-이성질체], 델타메트린, 엠펜트린 [(EZ)-(1R)-이성질체], 에스펜발레레이트, 에토펜프록스, 펜프로파트린, 펜발레레이트, 플루시트리네이트, 플루메트린, 타우-플루발리네이트, 할펜프록스, 이미프로트린, 카데트린, 몸플루오로트린, 페르메트린, 페노트린 [(1R)-트랜스-이성질체], 프랄레트린, 피레트린 (피레트룸), 레스메트린, 실라플루오펜, 테플루트린, 테트라메트린, 테트라메트린 [(1R)- 이성질체)], 트랄로메트린 및 트랜스플루트린 또는 DDT 또는 메톡시클로르.
(4) 니코틴성 아세틸콜린 수용체 (nAChR) 경쟁적 조정제, 예컨대, 예를 들어, 네오니코티노이드, 예를 들어 아세타미프리드, 클로티아니딘, 디노테푸란, 이미다클로프리드, 니텐피람, 티아클로프리드 및 티아메톡삼 또는 니코틴 또는 술폭사플로르 또는 플루피라디푸론.
(5) 니코틴성 아세틸콜린 수용체 (nAChR) 알로스테릭 조정제, 예컨대, 예를 들어, 스피노신, 예를 들어 스피네토람 및 스피노사드.
(6) 글루타메이트-게이팅 클로라이드 채널 (GluCl) 알로스테릭 조정제, 예컨대, 예를 들어, 아베르멕틴/밀베마이신, 예를 들어 아바멕틴, 에마멕틴 벤조에이트, 레피멕틴 및 밀베멕틴.
(7) 유충 호르몬 모방체, 예컨대, 예를 들어, 유충 호르몬 유사체, 예를 들어 히드로프렌, 키노프렌 및 메토프렌 또는 페녹시카르브 또는 피리프록시펜.
(8) 기타 비-특이적 (다중-부위) 억제제, 예컨대, 예를 들어, 알킬 할라이드, 예를 들어 메틸 브로마이드 및 다른 알킬 할라이드; 또는 클로로피크린 또는 술푸릴 플루오라이드 또는 보락스 또는 토주석 또는 메틸 이소시아네이트 발생기, 예를 들어 디아조메트 및 메탐.
(9) 현음 기관의 조정제, 예컨대, 예를 들어 피메트로진 또는 플로니카미드.
(10) 응애 성장 억제제, 예컨대, 예를 들어 클로펜테진, 헥시티아족스 및 디플로비다진 또는 에톡사졸.
(11) 곤충 장 막의 미생물 파괴제, 예컨대, 예를 들어 바실루스 투린기엔시스 아종 이스라엘렌시스, 바실루스 스파에리쿠스, 바실루스 투린기엔시스 아종 아이자와이, 바실루스 투린기엔시스 아종 쿠르스타키, 바실루스 투린기엔시스 아종 테네브리오니스, 및 B.t. 식물 단백질: Cry1Ab, Cry1Ac, Cry1Fa, Cry1A.105, Cry2Ab, Vip3A, mCry3A, Cry3Ab, Cry3Bb, Cry34Ab1/35Ab1.
(12) 미토콘드리아 ATP 신타제의 억제제, 예컨대 ATP 교란제, 예컨대 디아펜티우론 또는 유기주석 화합물, 예를 들어 아조시클로틴, 시헥사틴 및 펜부타틴 옥시드 또는 프로파르기트 또는 테트라디폰.
(13) 양성자 구배의 파괴를 통한 산화성 인산화의 탈커플링제, 예컨대 예를 들어 클로르페나피르, DNOC 및 술플루라미드.
(14) 니코틴성 아세틸콜린 수용체 채널 차단제, 예컨대 예를 들어 벤술탑, 카르탑 히드로클로라이드, 티오실람 및 티오술탑-소듐.
(15) 제0형 키틴 생합성 억제제, 예컨대 예를 들어 비스트리플루론, 클로르플루아주론, 디플루벤주론, 플루시클록수론, 플루페녹수론, 헥사플루무론, 루페누론, 노발루론, 노비플루무론, 테플루벤주론 및 트리플루무론.
(16) 제1형 키틴 생합성 억제제, 예를 들어 부프로페진.
(17) 탈피 교란제 (특히 파리목, 즉 쌍시류), 예컨대, 예를 들어, 시로마진.
(18) 엑디손 수용체 효능제, 예컨대, 예를 들어, 크로마페노지드, 할로페노지드, 메톡시페노지드 및 테부페노지드.
(19) 옥토파민 수용체 효능제, 예컨대 예를 들어 아미트라즈.
(20) 미토콘드리아 복합체 III 전자 수송 억제제, 예컨대, 예를 들어, 히드라메틸논 또는 아세퀴노실 또는 플루아크리피림.
(21) 미토콘드리아 복합체 I 전자 수송 억제제, 예컨대 예를 들어 METI 살진드기제의 군으로부터의 것, 예를 들어 페나자퀸, 펜피록시메이트, 피리미디펜, 피리다벤, 테부펜피라드 및 톨펜피라드 또는 로테논 (데리스).
(22) 전압-의존성 나트륨 채널 차단제, 예컨대, 예를 들어 인독사카르브 또는 메타플루미존.
(23) 아세틸 CoA 카르복실라제의 억제제, 예컨대 테트론산 및 테트람산 유도체, 예를 들어 스피로디클로펜, 스피로메시펜 및 스피로테트라마트.
(24) 미토콘드리아 복합체 IV 전자 수송 억제제, 예컨대 예를 들어 포스핀, 예를 들어 알루미늄 포스피드, 칼슘 포스피드, 포스핀 및 아연 포스피드 또는 시아나이드, 예를 들어 칼슘 시아나이드, 칼륨 시아나이드 및 나트륨 시아나이드.
(25) 미토콘드리아 복합체 II 전자 수송 억제제, 예컨대 베타-케토니트릴 유도체, 예를 들어 시에노피라펜 및 시플루메토펜 및 카르복스아닐리드, 예컨대 예를 들어 피플루부미드.
(28) 리아노딘 수용체 조절제, 예컨대, 예를 들어, 디아미드, 예를 들어 클로란트라닐리프롤, 시안트라닐리프롤 및 플루벤디아미드,
추가의 활성 화합물, 예컨대 예를 들어 아피도피로펜, 아폭솔라너, 아자디라크틴, 벤클로티아즈, 벤족시메이트, 비페나제이트, 브로플라닐리드, 브로모프로필레이트, 키노메티오나트, 클로로프랄레트린, 크리올라이트, 시클라닐리프롤, 시클록사프리드, 시할로디아미드, 디클로로메조티아즈, 디코폴, 엡실론-메토플루트린, 엡실론-몸플루트린, 플로메토퀸, 플루아자인돌리진, 플루엔술폰, 플루페네림, 플루페녹시스트로빈, 플루피프롤, 플루헥사폰, 플루오피람, 플루랄라너, 플룩사메타미드, 푸페노지드, 구아디피르, 헵타플루트린, 이미다클로티즈, 이프로디온, 카파-비펜트린, 카파-테플루트린, 로틸라너, 메페르플루트린, 파이총딩, 피리달릴, 피리플루퀴나존, 피리미노스트로빈, 스피로부디클로펜, 테트라메틸플루트린, 테트라닐리프롤, 테트라클로란트라닐리프롤, 티골라너, 티옥사자펜, 티오플루옥시메이트, 트리플루메조피림 및 아이오도메탄; 또한 바실루스 피르무스(Bacillus firmus) (I-1582, 바이오님(BioNeem), 보티보(Votivo))를 기재로 하는 제제, 및 또한 하기 화합물: 1-{2-플루오로-4-메틸-5-[(2,2,2-트리플루오로에틸)술피닐]페닐}-3-(트리플루오로메틸)-1H-1,2,4-트리아졸-5-아민 (WO2006/043635로부터 공지됨) (CAS 885026-50-6), {1'-[(2E)-3-(4-클로로페닐)프로프-2-엔-1-일]-5-플루오로스피로[인돌-3,4'-피페리딘]-1(2H)-일}(2-클로로피리딘-4-일)메타논 (WO2003/106457로부터 공지됨) (CAS 637360-23-7), 2-클로로-N-[2-{1-[(2E)-3-(4-클로로페닐)프로프-2-엔-1-일]피페리딘-4-일}-4-(트리플루오로메틸)페닐]이소니코틴아미드 (WO2006/003494로부터 공지됨) (CAS 872999-66-1), 3-(4-클로로-2,6-디메틸페닐)-4-히드록시-8-메톡시-1,8-디아자스피로[4.5]데스-3-엔-2-온 (WO 2010052161로부터 공지됨) (CAS 1225292-17-0), 3-(4-클로로-2,6-디메틸페닐)-8-메톡시-2-옥소-1,8-디아자스피로[4.5]데스-3-엔-4-일 에틸 카르보네이트 (EP2647626으로부터 공지됨) (CAS 1440516-42-6), 4-(부트-2-인-1-일옥시)-6-(3,5-디메틸피페리딘-1-일)-5-플루오로피리미딘 (WO2004/099160으로부터 공지됨) (CAS 792914-58-0), PF1364 (JP2010/018586으로부터 공지됨) (CAS 1204776-60-2), N-[(2E)-1-[(6-클로로피리딘-3-일)메틸]피리딘-2(1H)-일리덴]-2,2,2-트리플루오로아세트아미드 (WO2012/029672로부터 공지됨) (CAS 1363400-41-2), (3E)-3-[1-[(6-클로로-3-피리딜)메틸]-2-피리딜리덴]-1,1,1-트리플루오로-프로판-2-온 (WO2013/144213으로부터 공지됨) (CAS 1461743-15-6), N-[3-(벤질카르바모일)-4-클로로페닐]-1-메틸-3-(펜타플루오로에틸)-4-(트리플루오로메틸)-1H-피라졸-5-카르복스아미드 (WO2010/051926으로부터 공지됨) (CAS 1226889-14-0), 5-브로모-4-클로로-N-[4-클로로-2-메틸-6-(메틸카르바모일)페닐]-2-(3-클로로-2-피리딜)피라졸-3-카르복스아미드 (CN103232431로부터 공지됨) (CAS 1449220-44-3), 4-[5-(3,5-디클로로페닐)-4,5-디히드로-5-(트리플루오로메틸)-3-이속사졸릴]-2-메틸-N-(시스-1-옥시도-3-티에타닐)-벤즈아미드, 4-[5-(3,5-디클로로페닐)-4,5-디히드로-5-(트리플루오로메틸)-3-이속사졸릴]-2-메틸-N-(트랜스-1-옥시도-3-티에타닐)-벤즈아미드 및 4-[(5S)-5-(3,5-디클로로페닐)-4,5-디히드로-5-(트리플루오로메틸)-3-이속사졸릴]-2-메틸-N-(시스-1-옥시도-3-티에타닐)벤즈아미드 (WO 2013/050317 A1로부터 공지됨) (CAS 1332628-83-7), N-[3-클로로-1-(3-피리디닐)-1H-피라졸-4-일]-N-에틸-3-[(3,3,3-트리플루오로프로필)술피닐]-프로판아미드, (+)-N-[3-클로로-1-(3-피리디닐)-1H-피라졸-4-일]-N-에틸-3-[(3,3,3-트리플루오로프로필)술피닐]-프로판아미드 및 (-)-N-[3-클로로-1-(3-피리디닐)-1H-피라졸-4-일]-N-에틸-3-[(3,3,3-트리플루오로프로필)술피닐]-프로판아미드 (WO 2013/162715 A2, WO 2013/162716 A2, US 2014/0213448 A1로부터 공지됨) (CAS 1477923-37-7), 5-[[(2E)-3-클로로-2-프로펜-1-일]아미노]-1-[2,6-디클로로-4-(트리플루오로메틸)페닐]-4-[(트리플루오로메틸)술피닐]-1H-피라졸-3-카르보니트릴 (CN 101337937 A로부터 공지됨) (CAS 1105672-77-2), 3-브로모-N-[4-클로로-2-메틸-6-[(메틸아미노)티옥소메틸]페닐]-1-(3-클로로-2-피리디닐)-1H-피라졸-5-카르복스아미드 (CN 103109816 A로부터 공지됨) (CAS 1232543-85-9); N-[4-클로로-2-[[(1,1-디메틸에틸)아미노]카르보닐]-6-메틸페닐]-1-(3-클로로-2-피리디닐)-3-(플루오로메톡시)-1H-피라졸-5-카르복스아미드 (WO 2012/034403 A1로부터 공지됨) (CAS 1268277-22-0), N-[2-(5-아미노-1,3,4-티아디아졸-2-일)-4-클로로-6-메틸페닐]-3-브로모-1-(3-클로로-2-피리디닐)-1H-피라졸-5-카르복스아미드 (WO 2011/085575 A1로부터 공지됨) (CAS 1233882-22-8), 4-[3-[2,6-디클로로-4-[(3,3-디클로로-2-프로펜-1-일)옥시]페녹시]프로폭시]-2-메톡시-6-(트리플루오로메틸)-피리미딘 (CN 101337940 A로부터 공지됨) (CAS 1108184-52-6); (2E)- 및 2(Z)-2-[2-(4-시아노페닐)-1-[3-(트리플루오로메틸)페닐]에틸리덴]-N-[4-(디플루오로메톡시)페닐]-히드라진카르복스아미드 (CN 101715774 A로부터 공지됨) (CAS 1232543-85-9); 3-(2,2-디클로로에테닐)-2,2-디메틸-4-(1H-벤즈이미다졸-2-일)페닐-시클로프로판카르복실산 에스테르 (CN 103524422 A로부터 공지됨) (CAS 1542271-46-4); (4aS)-7-클로로-2,5-디히드로-2-[[(메톡시카르보닐)[4-[(트리플루오로메틸)티오]페닐]아미노]카르보닐]-인데노[1,2-e][1,3,4]옥사디아진-4a(3H)-카르복실산 메틸 에스테르 (CN 102391261 A로부터 공지됨) (CAS 1370358-69-2); 6-데옥시-3-O-에틸-2,4-디-O-메틸-, 1-[N-[4-[1-[4-(1,1,2,2-펜타플루오로에톡시)페닐]-1H-1,2,4-트리아졸-3-일]페닐]카르바메이트]-α-L-만노피라노스 (US 2014/0275503 A1로부터 공지됨) (CAS 1181213-14-8); 8-(2-시클로프로필메톡시-4-트리플루오로메틸-페녹시)-3-(6-트리플루오로메틸-피리다진-3-일)-3-아자-비시클로[3.2.1]옥탄 (CAS 1253850-56-4), (8-안티)-8-(2-시클로프로필메톡시-4-트리플루오로메틸-페녹시)-3-(6-트리플루오로메틸-피리다진-3-일)-3-아자-비시클로[3.2.1]옥탄 (CAS 933798-27-7), (8-신)-8-(2-시클로프로필메톡시-4-트리플루오로메틸-페녹시)-3-(6-트리플루오로메틸-피리다진-3-일)-3-아자-비시클로[3.2.1]옥탄 (WO 2007040280 A1, WO 2007040282 A1로부터 공지됨) (CAS 934001-66-8), N-[3-클로로-1-(3-피리디닐)-1H-피라졸-4-일]-N-에틸-3-[(3,3,3-트리플루오로프로필)티오]-프로판아미드 (WO 2015/058021 A1, WO 2015/058028 A1로부터 공지됨) (CAS 1477919-27-9) 및 N-[4-(아미노티옥소메틸)-2-메틸-6-[(메틸아미노)카르보닐]페닐]-3-브로모-1-(3-클로로-2-피리디닐)-1H-피라졸-5-카르복스아미드 (CN 103265527 A로부터 공지됨) (CAS 1452877-50-7), 5-(1,3-디옥산-2-일)-4-[[4-(트리플루오로메틸)페닐]메톡시]-피리미딘 (WO 2013/115391 A1로부터 공지됨) (CAS 1449021-97-9), 3-(4-클로로-2,6-디메틸페닐)-4-히드록시-8-메톡시-1-메틸-1,8-디아자스피로[4.5]데스-3-엔-2-온 (WO 2010/066780 A1, WO 2011/151146 A1로부터 공지됨) (CAS 1229023-34-0), 3-(4-클로로-2,6-디메틸페닐)-8-메톡시-1-메틸-1,8-디아자스피로[4.5]데칸-2,4-디온 (WO 2014/187846 A1로부터 공지됨) (CAS 1638765-58-8), 3-(4-클로로-2,6-디메틸페닐)-8-메톡시-1-메틸-2-옥소-1,8-디아자스피로[4.5]데스-3-엔-4-일-탄산 에틸 에스테르 (WO 2010/066780 A1, WO 2011151146 A1로부터 공지됨) (CAS 1229023-00-0), N-[1-[(6-클로로-3-피리디닐)메틸]-2(1H)-피리디닐리덴]-2,2,2-트리플루오로-아세트아미드 (DE 3639877 A1, WO 2012029672 A1로부터 공지됨) (CAS 1363400-41-2), [N(E)]-N-[1-[(6-클로로-3-피리디닐)메틸]-2(1H)-피리디닐리덴]-2,2,2-트리플루오로-아세트아미드, (WO 2016005276 A1로부터 공지됨) (CAS 1689566-03-7), [N(Z)]-N-[1-[(6-클로로-3-피리디닐)메틸]-2(1H)-피리디닐리덴]-2,2,2-트리플루오로-아세트아미드, (CAS 1702305-40-5), 3-엔도-3-[2-프로폭시-4-(트리플루오로메틸)페녹시]-9-[[5-(트리플루오로메틸)-2-피리디닐]옥시]-9-아자비시클로[3.3.1]노난 (WO 2011/105506 A1, WO 2016/133011 A1로부터 공지됨) (CAS 1332838-17-1).
본 발명의 화합물 조합물과 혼합될 수 있는 완화제의 예는, 예를 들어 베녹사코르, 클로퀸토세트 (-멕실), 시오메트리닐, 시프로술파미드, 디클로르미드, 펜클로라졸 (-에틸), 펜클로림, 플루라졸, 플룩소페님, 푸릴라졸, 이속사디펜 (-에틸), 메펜피르 (-디에틸), 나프탈산 무수물, 옥사베트리닐, 2-메톡시-N-({4-[(메틸카르바모일)아미노]페닐}술포닐)벤즈아미드 (CAS 129531-12-0), 4-(디클로로아세틸)-1-옥사-4-아자스피로[4.5]데칸 (CAS 71526-07-3), 2,2,5-트리메틸-3-(디클로로아세틸)-1,3-옥사졸리딘 (CAS 52836-31-4)이다.
본 발명의 화합물 조합물과 혼합될 수 있는 제초제의 예는 하기와 같다:
아세토클로르, 아시플루오르펜, 아시플루오르펜-소듐, 아클로니펜, 알라클로르, 알리도클로르, 알록시딤, 알록시딤-소듐, 아메트린, 아미카르바존, 아미도클로르, 아미도술푸론, 4-아미노-3-클로로-5-플루오로-6-(7-플루오로-1H-인돌-6-일)피리딘-2-카르복실산, 아미노시클로피라클로르, 아미노시클로피라클로르-칼륨, 아미노시클로피라클로르-메틸, 아미노피랄리드, 아미트롤, 암모늄술파메이트, 아닐로포스, 아술람, 아트라진, 아자페니딘, 아짐술푸론, 베플루부타미드, 베나졸린, 베나졸린-에틸, 벤플루랄린, 벤푸레세이트, 벤술푸론, 벤술푸론-메틸, 벤술리드, 벤타존, 벤조비시클론, 벤조페납, 비시클로피론, 비페녹스, 빌라나포스, 빌라나포스-소듐, 비스피리박, 비스피리박-소듐, 빅슬로존, 브로마실, 브로모부티드, 브로모페녹심, 브로목시닐, 브로목시닐-부티레이트, -칼륨, -헵타노에이트, 및 -옥타노에이트, 부속시논, 부타클로르, 부타페나실, 부타미포스, 부테나클로르, 부트랄린, 부트록시딤, 부틸레이트, 카펜스트롤, 카르베타미드, 카르펜트라존, 카르펜트라존-에틸, 클로람벤, 클로르브로무론, 1-{2-클로로-3-[(3-시클로프로필-5-히드록시-1-메틸-1H-피라졸-4-일)카르보닐]-6-(트리플루오르메틸)페닐}피페리딘-2-온, 4-{2-클로로-3-[(3,5-디메틸-1H-피라졸-1-일)메틸]-4-(메틸술포닐)벤조일}-1,3-디메틸-1H-피라졸-5-일-1,3-디메틸-1H-피라졸-4-카르복실레이트, 클로르페낙, 클로르페낙-소듐, 클로르펜프로프, 클로르플루레놀, 클로르플루레놀-메틸, 클로리다존, 클로리무론, 클로리무론-에틸, 2-[2-클로로-4-(메틸술포닐)-3-(모르폴린-4일메틸)벤조일}-3-히드록시시클로헥스-2-엔-1-온, 4-{2-클로로-4-(메틸술포닐)-3-[(2,2,2-트리플루오로에톡시)메틸]벤조일}-1-에틸-1H-피라졸-5-일-1,3-디메틸-1H,피라졸-4-카르복실레이트, 클로로프탈림, 클로로톨루론, 클로르탈-디메틸, 3-[5-클로로-4-(트리플루오르메틸)피리딘-2-일]-4-히드록시-1-메틸이미다졸리딘-2-온, 클로르술푸론, 시니돈, 시니돈-에틸, 신메틸린, 시노술푸론, 클라시포스, 클레토딤, 클로디나포프, 클로디나포프-프로파르길, 클로마존, 클로메프로프, 클로피랄리드, 클로란술람, 클로란술람-메틸, 쿠밀루론, 시안아미드, 시아나진, 시클로에이트, 시클로피라닐, 시클로피리모레이트, 시클로술파무론, 시클록시딤, 시할로포프, 시할로포프-부틸, 시프라진, 2,4-D, 2,4-D-부토틸, -부틸, -디메틸암모늄, -디올라민, -에틸, -2-에틸헥실, -이소부틸, -이소옥틸, -이소프로필암모늄, -칼륨, -트리이소프로판올암모늄, 및 -트롤아민, 2,4-DB, 2,4-DB-부틸, -디메틸암모늄, -이소옥틸, -칼륨, 및 -소듐, 다이무론 (딤론), 달라폰, 다조메트, n-데칸올, 데스메디팜, 데토실-피라졸레이트 (DTP), 디캄바, 디클로베닐, 2-(2,4-디클로로벤질)-4,4-디메틸-1,2-옥사졸리딘-3-온, 2-(2,5-디클로로벤질)-4,4-디메틸-1,2-옥사졸리딘-3-온, 디클로르프로프, 디클로르프로프-P, 디클로포프, 디클로포프-메틸, 디클로포프-P-메틸, 디클로술람, 디펜조쿼트, 디플루페니칸, 디플루펜조피르, 디플루펜조피르-소듐, 디메푸론, 디메피페레이트, 디메타클로르, 디메타메트린, 디메테나미드, 디메테나미드-P, 3-(2,6-디메틸페닐)-6-[(2-히드록시-6-옥소시클로헥스-1-엔-1-일)카르보닐]-1-메틸키나졸린-2,4(1H,3H)-디온, 1,3-디메틸-4-[2-(메틸술포닐)-4-(트리플루오르메틸)벤조일]-1H-피라졸-5-일-1,3-디메틸-1H-피라졸-4-카르복실레이트, 디메트라술푸론, 디니트라민, 디노테르브, 디페나미드, 디쿼트, 디쿼트-디브로마이드, 디티오피르, 디우론, DMPA, DNOC, 엔도탈, EPTC, 에스프로카르브, 에탈플루랄린, 에타메트술푸론, 에타메트술푸론-메틸, 에티오진, 에토푸메세이트, 에톡시펜, 에톡시펜-에틸, 에톡시술푸론, 에토벤자니드, 에틸-[(3-{2-클로로-4-플루오로-5-[3-메틸-2,6-디옥소-4-(트리플루오르메틸)-3,6-디히드로피리미딘-1(2H)-일]페녹시}피리딘-2-일)옥시]아세테이트, F-9960, F-5231, 즉 N-{2-클로로-4-플루오로-5-[4-(3-플루오로프로필)-5-옥소-4,5-디히드로-1H-테트라졸-1-일]페닐}에탄술폰아미드, F-7967, 즉 3-[7-클로로-5-플루오로-2-(트리플루오로메틸)-1H-벤즈이미다졸-4-일]-1-메틸-6-(트리플루오로메틸)피리미딘-2,4(1H,3H)-디온, 페녹사프로프, 페녹사프로프-P, 페녹사프로프-에틸, 페녹사프로프-P-에틸, 페녹사술폰, 펜퀴노트리온, 펜트라자미드, 플람프로프, 플람프로프-M-이소프로필, 플람프로프-M-메틸, 플라자술푸론, 플로라술람, 플루아지포프, 플루아지포프-P, 플루아지포프-부틸, 플루아지포프-P-부틸, 플루카르바존, 플루카르바존-소듐, 플루세토술푸론, 플루클로랄린, 플루페나세트, 플루펜피르, 플루펜피르-에틸, 플루메트술람, 플루미클로락, 플루미클로락-펜틸, 플루미옥사진, 플루오메투론, 플루레놀, 플루레놀-부틸, -디메틸암모늄 및 -메틸, 플루오로글리코펜, 플루오로글리코펜-에틸, 플루프로파네이트, 플루피르술푸론, 플루피르술푸론-메틸-소듐, 플루리돈, 플루로클로리돈, 플루록시피르, 플루록시피르-멥틸, 플루르타몬, 플루티아세트, 플루티아세트-메틸, 포메사펜, 포메사펜-소듐, 포람술푸론, 포사민, 글루포시네이트, 글루포시네이트-암모늄, 글루포시네이트-P-소듐, 글루포시네이트-P-암모늄, 글루포시네이트-P-소듐, 글리포세이트, 글리포세이트-암모늄, -이소프로필암모늄, -디암모늄, -디메틸암모늄, -칼륨, -소듐, 및 -트리메슘, H-9201, 즉 O-(2,4-디메틸-6-니트로페닐) O-에틸 이소프로필포스포르아미도티오에이트, 할라욱시펜, 할라욱시펜-메틸 ,할로사펜, 할로술푸론, 할로술푸론-메틸, 할록시포프, 할록시포프-P, 할록시포프-에톡시에틸, 할록시포프-P-에톡시에틸, 할록시포프-메틸, 할록시포프-P-메틸, 헥사지논, HW-02, 즉 1-(디메톡시포스포릴) 에틸-(2,4-디클로로페녹시)아세테이트, 4-히드록시-1-메톡시-5-메틸-3-[4-트리플루오르메틸)피리딘-2-일]이미다졸리딘-2-온, 4-히드록시-1-메틸-3-[4-트리플루오르메틸)피리딘-2-일]이미다졸리딘-2-온, (5-히드록시-1-메틸-1H-피라졸-4-일)(3,3,4-트리메틸-1,1-디옥시도-2,3-디히드로-1-벤조티오펜-5-일)메타논, 6-[(2-히드록시-6-옥소시클로헥스-1-엔-1-일)카르보닐]-1,5-디메틸-3-(2-메틸페닐)키나졸린-2,4(1H,3H)-디온, 이마자메타벤즈, 이마자메타벤즈-메틸, 이마자목스, 이마자목스-암모늄, 이마자픽, 이마자픽-암모늄, 이마자피르, 이마자피르-이소프로필암모늄, 이마자퀸, 이마자퀸-암모늄, 이마제타피르, 이마제타피르-임모늄, 이마조술푸론, 인다노판, 인다지플람, 아이오도술푸론, 아이오도술푸론-메틸-소듐, 이옥시닐, 이옥시닐-옥타노에이트, -칼륨 및 -소듐, 이프펜카르바존, 이소프로투론, 이소우론, 이속사벤, 이속사플루톨, 카르부틸레이트, KUH-043, 즉 3-({[5-(디플루오로메틸)-1-메틸-3-(트리플루오로메틸)-1H-피라졸-4-일]메틸}술포닐)-5,5-디메틸-4,5-디히드로-1,2-옥사졸, 케토스피라독스, 락토펜, 레나실, 리누론, MCPA, MCPA-부토틸, -디메틸암모늄, -2-에틸헥실, -이소프로필암모늄, -칼륨, 및 -소듐, MCPB, MCPB-메틸, -에틸 및 -소듐, 메코프로프, 메코프로프-소듐, 및 -부토틸, 메코프로프-P, 메코프로프-P-부토틸, -디메틸암모늄, -2-에틸헥실, 및 -칼륨, 메페나세트, 메플루이디드, 메소술푸론, 메소술푸론-메틸, 메소트리온, 메타벤즈티아주론, 메탐, 메타미포프, 메타미트론, 메타자클로르, 메타조술푸론, 메타벤즈티아주론, 메티오피르술푸론, 메티오졸린, 2-({2-[(2-메톡시에톡시)메틸]-6-(트리플루오르메틸)피리딘-3-일}카르보닐)시클로헥산-1,3-디온, 메틸 이소티오시아네이트, 1-메틸-4-[(3,3,4-트리메틸-1,1-디옥시도-2,3-디히드로-1-벤조티오펜-5-일)카르보닐]-1H-피라졸-5-일프로판-1-술포나트, 메토브로무론, 메톨라클로르, S-메톨라클로르, 메토술람, 메톡수론, 메트리부진, 메트술푸론, 메트술푸론-메틸, 몰리나트, 모노리누론, 모노술푸론, 모노술푸론-에스테르, MT-5950, 즉 N-(3-클로로-4-이소프로필페닐)-2-메틸펜탄 아미드, NGGC-011, 나프로파미드, NC-310, 즉 [5-(벤질옥시)-1-메틸-1H-피라졸-4-일](2,4-디클로로페닐)메타논, 네부론, 니코술푸론, 노난산 (펠라르곤산), 노르플루라존, 올레산 (지방산), 오르벤카르브, 오르토술파무론, 오리잘린, 옥사디아르길, 옥사디아존, 옥사술푸론, 옥사지클로메폰, 옥시플루오르펜, 파라쿼트, 파라쿼트 디클로라이드, 페불레이트, 펜디메탈린, 페녹스술람, 펜타클로르페놀, 펜톡사존, 페톡사미드, 석유 오일, 펜메디팜, 피클로람, 피콜리나펜, 피녹사덴, 피페로포스, 프레틸라클로르, 프리미술푸론, 프리미술푸론-메틸, 프로디아민, 프로폭시딤, 프로메톤, 프로메트린, 프로파클로르, 프로파닐, 프로파퀴자포프, 프로파진, 프로팜, 프로피소클로르, 프로폭시카르바존, 프로폭시카르바존-소듐, 프로피리술푸론, 프로피자미드, 프로술포카르브, 프로술푸론, 피라클로닐, 피라플루펜, 피라플루펜-에틸, 피라술포톨, 피라졸리네이트 (피라졸레이트), 피라조술푸론, 피라조술푸론-에틸, 피라족시펜, 피리밤벤즈, 피리밤벤즈-이소프로필, 피리밤벤즈-프로필, 피리벤족심, 피리부티카르브, 피리다폴, 피리데이트, 피리프탈리드, 피리미노박, 피리미노박-메틸, 피리미술판, 피리티오박, 피리티오박-소듐, 피록사술폰, 피록스술람, 퀸클로락, 퀸메락, 퀴노클라민, 퀴잘로포프, 퀴잘로포프-에틸, 퀴잘로포프-P, 퀴잘로포프-P-에틸, 퀴잘로포프-P-테푸릴, QYM-201, QYR-301, 림술푸론, 사플루페나실, 세톡시딤, 시두론, 시마진, 시메트린, SL-261, 술코트리온, 술펜트라존, 술포메투론, 술포메투론-메틸, 술포술푸론, SYN-523, SYP-249, 즉 1-에톡시-3-메틸-1-옥소부트-3-엔-2-일 5-[2-클로로-4-(트리플루오로메틸)페녹시]-2-니트로벤조에이트, SYP-300, 즉 1-[7-플루오로-3-옥소-4-(프로프-2-인-1-일)-3,4-디히드로-2H-1,4-벤족사진-6-일]-3-프로필-2-티옥소이미다졸리딘-4,5-디온, 2,3,6-TBA, TCA (트리클로로아세트산), TCA-소듐, 테부티우론, 테푸릴트리온, 템보트리온, 테프랄록시딤, 테르바실, 테르부카르브, 테르부메톤, 테르부틸라진, 테르부트린, 테트라플루피롤리메트, 테닐클로르, 티아조피르, 티엔카르바존, 티엔카르바존-메틸, 티펜술푸론, 티펜술푸론-메틸, 티오벤카르브, 티아페나실, 톨피랄레이트, 토프라메존, 트랄콕시딤, 트리아파몬, 트리-알레이트, 트리아술푸론, 트리아지플람, 트리베누론, 트리베누론-메틸, 트리클로피르, 트리에타진, 트리플록시술푸론, 트리플록시술푸론-소듐, 트리플루디목사진, 트리플루랄린, 트리플루술푸론, 트리플루술푸론-메틸, 트리토술푸론, 우레아 술페이트, 베르놀레이트, XDE-848, ZJ-0862, 즉 3,4-디클로로-N-{2-[(4,6-디메톡시피리미딘-2-일)옥시]벤질}아닐린.
식물 성장 조절제의 예는 하기와 같다:
아시벤졸라, 아시벤졸라-S-메틸, 5-아미노레불린산, 안시미돌, 6-벤질아미노푸린, 브라시놀리드, 카테킨, 클로르메쿼트 클로라이드, 클로프로프, 시클라닐리드, 3-(시클로프로프-1-에닐) 프로피온산, 다미노지드, 다조메트, n-데칸올, 디케굴락, 디케굴락-나트륨, 엔도탈, 엔도탈-이칼륨, -이나트륨, 및 -모노(N,N-디메틸알킬암모늄), 에테폰, 플루메트랄린, 플루레놀, 플루레놀-부틸, 플루르프리미돌, 포르클로르페누론, 지베렐산, 이나벤피드, 인돌-3-아세트산 (IAA), 4-인돌-3-일부티르산, 이소프로티올란, 프로베나졸, 자스몬산, 말레산 히드라지드, 메피쿼트 클로라이드, 1-메틸시클로프로펜, 메틸 자스모네이트, 2-(1-나프틸)아세트아미드, 1-나프틸아세트산, 2-나프틸옥시아세트산, 니트로페놀레이트-혼합물, 파클로부트라졸, N-(2-페닐에틸)-베타-알라닌, N-페닐프탈람산, 프로헥사디온, 프로헥사디온-칼슘, 프로히드로자스몬, 살리실산, 스트리고락톤, 테크나젠, 티디아주론, 트리아콘탄올, 트리넥사팍, 트리넥사팍-에틸, 티토데프, 유니코나졸, 유니코나졸-P.
방법 및 용도
본 발명의 화합물 조합물 및 조성물은 강력한 살미생물 활성 및/또는 식물 방어 조절 잠재력을 갖는다. 이들은 식물 상의 원치 않는 미생물, 예컨대 원치 않는 진균 및 박테리아를 방제하는 데 사용될 수 있다. 이들은 작물 보호에 (이들은 식물 질병을 유발하는 미생물을 방제함) 또는 하기 본원에 보다 상세히 기재된 바와 같은 물질 (예를 들어 산업적 물질, 재목, 저장 제품)을 보호하는 데 특히 유용할 수 있다. 보다 구체적으로, 본 발명의 화합물 조합물 및 조성물은 종자, 발아 종자, 출아 묘목, 식물, 식물 부분, 과실, 수확 제품 및/또는 식물이 성장하는 토양을 원치 않는 미생물로부터 보호하는 데 사용될 수 있다.
본원에 사용된 바와 같은 방제 또는 방제는 원치 않는 미생물의 보호적, 치유적 및 박멸적 처리를 포괄한다. 원치 않는 미생물은 병원성 박테리아, 병원성 바이러스, 병원성 난균류 또는 병원성 진균, 보다 구체적으로 식물병원성 박테리아, 식물병원성 바이러스, 식물병원성 난균류 또는 식물병원성 진균일 수 있다. 하기 본원에 상술된 바와 같이, 이들 식물병원성 미생물은 광범위한 식물 질병의 병원체이다.
보다 구체적으로, 본 발명의 화합물 조합물 및 조성물은 살진균제로서 사용될 수 있다. 본 명세서의 목적상, 용어 "살진균제"는 원치 않는 진균, 예컨대 플라스모디오포로미세테스, 키트리디오미세테스, 지고미세테스, 아스코미세테스, 바시디오미세테스 및 듀테로미세테스의 방제 및/또는 오오미세테스의 방제를 위한 작물 보호에 사용될 수 있는 화합물 또는 조성물을 지칭한다.
본 발명의 화합물 조합물 및 조성물은 또한 항박테리아제로서 사용될 수 있다. 특히, 이들은 작물 보호에서, 예를 들어 원치 않는 박테리아, 예컨대 슈도모나다세아에(Pseudomonadaceae), 리조비아세아에(Rhizobiaceae), 크산토모나다세아에(Xanthomonadaceae), 엔테로박테리아세아에(Enterobacteriaceae), 코리네박테리아세아에(Corynebacteriaceae) 및 스트렙토미세타세아에(Streptomycetaceae)의 방제를 위해 사용될 수 있다.
본 발명은 또한 본 발명의 화합물 조합물 또는 조성물을 미생물 및/또는 그의 서식지에 (식물, 식물 부분, 종자, 과실에 또는 식물이 성장하는 토양에) 적용하는 단계를 포함하며, 여기서 화합물 (A) 및 (B)는 동시, 개별 또는 순차적 방식으로 적용될 수 있는 것인, 식물 상에서 원치 않는 미생물, 예컨대 원치 않는 진균, 난균류 및 박테리아를 방제하는 방법에 관한 것이다. 단일 화합물이 순차적 방식으로, 즉 상이한 시간에 적용되는 경우에, 이들은 상당히 짧은 기간, 예컨대 수시간 또는 수일 내에 차례로 적용된다.
전형적으로, 본 발명의 화합물 조합물 및 조성물이 식물병원성 진균 및/또는 식물병원성 난균류를 방제하기 위한 치유 또는 보호 방법에 사용되는 경우에, 그의 유효하고 식물-상용성인 양은 식물, 식물 부분, 과실, 종자 또는 식물이 성장하는 토양 또는 기질에 적용된다. 식물을 재배하는 데 사용될 수 있는 적합한 기재는 무기 기재 기재 기재, 예컨대 미네랄 울, 특히 스톤 울, 펄라이트, 샌드 또는 자갈; 유기 기재, 예컨대 토탄, 소나무 껍질 또는 톱밥; 및 석유계 기재, 예컨대 중합체 발포체 또는 플라스틱 비드를 포함한다. 유효하고 식물-상용성인 양은 농경지 상에 존재하거나 또는 나타나기 쉬운 진균을 방제 또는 파괴하기에 충분하고, 상기 작물에 대한 식물독성의 임의의 인지가능한 증상을 수반하지 않는 양을 의미한다. 이러한 양은 방제될 진균, 작물의 유형, 작물 성장 단계, 기후 조건 및 사용된 본 발명의 각각의 화합물 또는 조성물에 따라 폭넓은 범위 내에서 달라질 수 있다. 이 양은 관련 기술분야의 통상의 기술자의 능력 내에 있는 체계적 현장 시험에 의해 결정될 수 있다.
식물 및 식물 부분
본 발명의 화합물 조합물 및 조성물은 임의의 식물 또는 식물 부분에 적용될 수 있다.
식물은 모든 식물 및 식물 군집, 예컨대 목적하는 및 목적하지 않는 야생 식물 또는 작물 식물 (자연 발생 작물 식물 포함)을 의미한다. 작물 식물은 통상의 육종 및 최적화 방법에 의해 또는 생명공학 및 유전 공학 방법 또는 이들 방법의 조합에 의해 수득될 수 있는 식물일 수 있으며, 유전자 변형 식물 (GMO 또는 트랜스제닉 식물)을 포함하고, 식물 육종가의 권리에 의해 보호가능한 및 보호불가능한 식물 재배품종을 포함할 수 있다.
유전자 변형 식물 (GMO)
유전자 변형 식물 (GMO 또는 트랜스제닉 식물)은 이종 유전자가 게놈 내로 안정하게 통합된 식물이다. 표현 "이종 유전자"는 본질적으로 식물 외부에서 및 핵, 엽록체 또는 미토콘드리아 게놈에 도입될 때 제공되거나 조립되는 유전자를 의미한다. 이 유전자는 관심 단백질 또는 폴리펩티드를 발현시킴으로써 또는 식물에 존재하는 다른 유전자(들)를 하향조절 또는 침묵시킴으로써 (예를 들어, 안티센스 기술, 공동억제 기술, RNA 간섭 - RNAi - 기술 또는 마이크로RNA - miRNA - 기술을 사용함) 형질전환된 식물에 새로운 또는 개선된 농경학적 또는 다른 특성을 제공한다. 게놈에 위치하는 이종 유전자는 또한 트랜스진으로 불린다. 식물 게놈에서의 그의 특정한 위치에 의해 정의되는 트랜스진은 형질전환 또는 트랜스제닉 사건으로 불린다.
식물 재배품종은 새로운 특성 ("형질")을 갖고 통상적인 육종, 돌연변이유발 또는 재조합 DNA 기술에 의해 수득된 식물을 의미하는 것으로 이해된다. 이는 재배품종, 변종, 생물형 또는 유전자형일 수 있다.
식물 부분은 지면의 위 아래의 식물의 모든 부분 및 기관, 예컨대 싹, 잎, 가시, 자루, 줄기, 꽃, 과실체, 과실, 종자, 뿌리, 괴경 및 근경을 포함한다. 식물 부분은 또한 수확된 물질 및 영양 및 생식 번식 물질, 예를 들어 묘목, 괴경, 근경, 자른 가지 및 종자를 포함한다.
본 발명의 방법에 따라 처리될 수 있는 식물은 하기를 포함한다: 목화, 아마, 포도덩굴, 과일, 채소, 예컨대 로사세아에 종 (예를 들어 인과류 예컨대 사과 및 배, 또한 핵과류 예컨대 살구, 체리, 아몬드 및 복숭아, 및 장과류 예컨대 딸기), 리베시오이다에(Ribesioidae) 종, 주글란다세아에(Juglandaceae) 종, 베툴라세아에(Betulaceae) 종, 아나카르디아세아에(Anacardiaceae) 종, 파가세아에(Fagaceae) 종, 모라세아에(Moraceae) 종, 올레아세아에(Oleaceae) 종, 악티니다세아에(Actinidaceae) 종, 라우라세아에(Lauraceae) 종, 무사세아에(Musaceae) 종 (예를 들어 바나나 나무 및 농장), 루비아세아에(Rubiaceae) 종 (예를 들어 커피), 테아세아에(Theaceae) 종, 스테르쿨리세아에(Sterculiceae) 종, 루타세아에(Rutaceae) 종 (예를 들어 레몬, 오렌지 및 그레이프프루트); 솔라나세아에(Solanaceae) 종 (예를 들어 토마토), 릴리아세아에(Liliaceae) 종, 아스테라세아에(Asteraceae) 종 (예를 들어 상추), 움벨리페라에(Umbelliferae) 종, 크루시페라에(Cruciferae) 종, 케노포디아세아에(Chenopodiaceae) 종, 쿠쿠르비타세아에(Cucurbitaceae) 종 (예를 들어 오이), 알리아세아에(Alliaceae) 종 (예를 들어 리크, 양파), 파필리오나세아에(Papilionaceae) 종 (예를 들어 완두); 주요 작물 식물, 예컨대 그라미네아에(Gramineae) 종 (예를 들어 옥수수, 잔디, 곡류 예컨대 밀, 호밀, 벼, 보리, 귀리, 기장 및 트리티케일), 아스테라세아에(Asteraceae) 종 (예를 들어 해바라기), 브라시카세아에(Brassicaceae) 종 (예를 들어 백색 양배추, 적색 양배추, 브로콜리, 콜리플라워, 브뤼셀 스프라우트, 청경채, 콜라비, 무, 및 유지종자 평지, 겨자, 호스래디시 및 큰다닥냉이), 파바카에(Fabacae) 종 (예를 들어 콩, 땅콩), 파필리오나세아에(Papilionaceae) 종 (예를 들어 대두), 솔라나세아에(Solanaceae) 종 (예를 들어 감자), 케노포디아세아에(Chenopodiaceae) 종 (예를 들어 사탕무, 사료용 비트, 근대, 비트); 정원 및 수목지에 유용한 식물 및 관상 식물; 및 이들 식물 각각의 유전자 변형 품종.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종은 1종 이상의 생물적 스트레스에 대해 저항성인 식물 및 식물 재배품종을 포함하며, 즉 상기 식물은 동물 및 미생물 해충, 예컨대 선충류, 곤충, 응애, 식물병원성 진균, 박테리아, 바이러스 및/또는 바이로이드에 대해 보다 우수한 방어를 나타낸다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종은 1종 이상의 비생물적 스트레스에 저항성인 식물을 포함한다. 비생물적 스트레스 조건은, 예를 들어 가뭄, 저온 노출, 열 노출, 삼투 스트레스, 홍수, 토양 염도 증가, 미네랄 노출 증가, 오존 노출, 고도의 광 노출, 제한된 질소 영양소 이용성, 제한된 인 영양소 이용성, 음지 회피를 포함할 수 있다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종은 증진된 수확량 특징을 특징으로 하는 식물을 포함한다. 상기 식물에서의 수확량 증가는, 예를 들어 식물 생리학, 성장 및 발육, 예컨대 물 사용 효율, 수분 저류 효율의 개선, 질소 사용 개선, 탄소 동화 증진, 광합성 개선, 발아 효율 증가 및 성숙 가속화의 결과일 수 있다. 수확량은 (스트레스 및 비스트레스 조건 하에서), 조기 개화, 하이브리드 종자 생산을 위한 개화 조절, 묘목 활력, 식물 크기, 절간(internode) 수 및 거리, 뿌리 성장, 종자 크기, 과실 크기, 꼬투리 크기, 꼬투리 또는 이삭 수, 꼬투리 또는 이삭 당 종자 수, 종자 질량, 종자 충실률 증진, 종자 분산 감소, 꼬투리 열개 감소 및 도복 저항성을 포함하나 이에 제한되지는 않는 개선된 식물 아키텍쳐(architecture)에 또한 영향을 받을 수 있다. 추가의 수확량 형질은 종자 조성, 예컨대 탄수화물 함량 및 조성, 예를 들어 목화 또는 전분, 단백질 함량, 오일 함량 및 조성, 영양가, 반-영양 화합물의 감소, 개선된 가공성 및 보다 우수한 저장 안정성을 포함한다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종은 일반적으로 보다 높은 수확량, 활력, 건강 및 생물적 및 비생물적 스트레스에 대한 저항성을 유발하는 잡종강세 또는 하이브리드 활력의 특징을 이미 발현하는 하이브리드 식물인 식물 및 식물 재배품종을 포함한다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종 (식물 생명공학 방법, 예컨대 유전 공학에 의해 수득됨)은 제초제-내성 식물인 식물 및 식물 재배품종, 즉 1종 이상의 주어진 제초제에 대해 내성을 갖게 된 식물을 포함한다. 이러한 식물은 유전자 형질전환에 의해, 또는 이러한 제초제 내성을 부여하는 돌연변이를 함유하는 식물의 선택에 의해 수득될 수 있다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종 (식물 생명공학 방법 예컨대 유전 공학에 의해 수득됨)은 곤충-저항성 트랜스제닉 식물, 즉 특정 표적 곤충에 의한 공격에 대해 저항성이 된 식물인 식물 및 식물 재배품종을 포함한다. 이러한 식물은 유전자 형질전환에 의해, 또는 이러한 곤충 저항성을 부여하는 돌연변이를 함유하는 식물의 선택에 의해 수득될 수 있다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종 (식물 생명공학 방법 예컨대 유전 공학에 의해 수득됨)은 특정 표적 곤충에 의한 공격에 대해 저항성이 된 식물인 질병-저항성 트랜스제닉 식물인 식물 및 식물 재배품종을 포함한다. 이러한 식물은 유전자 형질전환에 의해, 또는 이러한 곤충 저항성을 부여하는 돌연변이를 함유하는 식물의 선택에 의해 수득될 수 있다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종 (식물 생명공학 방법 예컨대 유전 공학에 의해 수득됨)은 비생물적 스트레스에 내성인 식물 및 식물 재배품종을 포함한다. 이러한 식물은 유전자 형질전환에 의해, 또는 이러한 스트레스 저항성을 부여하는 돌연변이를 함유하는 식물의 선택에 의해 수득될 수 있다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종 (식물 생명공학 방법 예컨대 유전 공학에 의해 수득됨)은 수확된 산물의 변경된 양, 품질 및/또는 저장-안정성 및/또는 수확된 산물의 특정 성분의 변경된 특성을 나타내는 식물 및 식물 재배품종을 포함한다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종 (식물 생명공학 방법, 예컨대 유전 공학에 의해 수득됨)은 변경된 섬유 특징을 갖는 식물 및 식물 재배품종, 예컨대 목화 식물을 포함한다. 이러한 식물은 유전자 형질전환에 의해, 또는 이러한 변경된 섬유 특징을 부여하는 돌연변이를 함유하는 식물의 선택에 의해 수득될 수 있다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종 (식물 생명공학 방법, 예컨대 유전 공학에 의해 수득됨)은 변경된 오일 프로파일 특징을 갖는 식물 및 식물 재배품종, 예컨대 유지종자 평지 또는 관련 브라시카 식물을 포함한다. 이러한 식물은 유전자 형질전환에 의해, 또는 이러한 변경된 오일 프로파일 특징을 부여하는 돌연변이를 함유하는 식물의 선택에 의해 수득될 수 있다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종 (식물 생명공학 방법 예컨대 유전 공학에 의해 수득됨)은 변경된 종자 탈립 특징을 갖는 식물 및 식물 재배품종, 예컨대 유지종자 평지 또는 관련 브라시카 식물을 포함한다. 이러한 식물은 유전자 형질전환에 의해, 또는 이러한 변경된 종자 탈립 특징을 부여하는 돌연변이를 함유하는 식물의 선택에 의해 수득될 수 있고, 지연 또는 감소된 종자 탈립을 갖는 식물, 예컨대 유지종자 평지 식물을 포함한다.
상기 개시된 방법에 의해 처리될 수 있는 식물 및 식물 재배품종 (식물 생명공학 방법, 예컨대 유전 공학에 의해 수득됨)은 변경된 번역후 단백질 변형 패턴을 갖는 식물 및 식물 재배품종, 예컨대 담배 식물을 포함한다.
병원체
본 발명에 따라 처리될 수 있는 진균성 질병의 병원체의 비-제한적 예는 하기를 포함한다:
흰가루병 병원체, 예를 들어 블루메리아(Blumeria) 종, 예를 들어 블루메리아 그라미니스(Blumeria graminis); 포도스파에라(Podosphaera) 종, 예를 들어 포도스파에라 류코트리카(Podosphaera leucotricha); 스파에로테카(Sphaerotheca) 종, 예를 들어 스파에로테카 풀리기네아(Sphaerotheca fuliginea); 운시눌라(Uncinula) 종, 예를 들어 운시눌라 네카토르(Uncinula necator)로 인한 질병;
녹병 병원체, 예를 들어 김노스포란기움(Gymnosporangium) 종, 예를 들어 김노스포란기움 사비나에(Gymnosporangium sabinae); 헤밀레이아(Hemileia) 종, 예를 들어 헤밀레이아 바스타트릭스(Hemileia vastatrix); 파코프소라(Phakopsora) 종, 예를 들어 파코프소라 파키리지(Phakopsora pachyrhizi) 또는 파코프소라 메이보미아에(Phakopsora meibomiae); 푹시니아(Puccinia) 종, 예를 들어 푹시니아 레콘디타(Puccinia recondita), 푹시니아 그라미니스(Puccinia graminis) 또는 푹시니아 스트리이포르미스(Puccinia striiformis); 우로미세스(Uromyces) 종, 예를 들어 우로미세스 아펜디쿨라투스(Uromyces appendiculatus)로 인한 질병;
난균류, 예를 들어 알부고(Albugo) 종, 예를 들어 알부고 칸디다(Albugo candida); 브레미아(Bremia) 종, 예를 들어 브레미아 락투카에(Bremia lactucae); 페로노스포라(Peronospora) 종, 예를 들어 페로노스포라 피시(Peronospora pisi) 또는 피. 브라시카에(P. brassicae); 피토프토라(Phytophthora) 종, 예를 들어 피토프토라 인페스탄스(Phytophthora infestans); 플라스모파라(Plasmopara) 종, 예를 들어 플라스모파라 비티콜라(Plasmopara viticola); 슈도페로노스포라(Pseudoperonospora) 종, 예를 들어 슈도페로노스포라 휴물리(Pseudoperonospora humuli) 또는 슈도페로노스포라 쿠벤시스(Pseudoperonospora cubensis); 피티움(Pythium) 종, 예를 들어 피티움 울티뭄(Pythium ultimum)의 군으로부터의 병원체로 인한 질병;
예를 들어 알테르나리아(Alternaria) 종, 예를 들어 알테르나리아 솔라니(Alternaria solani) 및 알테르나리아 알테르나타(Alternaria alternate); 세르코스포라(Cercospora) 종, 예를 들어 세르코스포라 베티콜라(Cercospora beticola); 클라디오스포리움(Cladiosporium) 종, 예를 들어 클라디오스포리움 쿠쿠메리눔(Cladiosporium cucumerinum); 코클리오볼루스(Cochliobolus) 종, 예를 들어 코클리오볼루스 사티부스(Cochliobolus sativus) (분생자 형태: 드레크슬레라(Drechslera), 동의어: 헬민토스포리움(Helminthosporium)) 또는 코클리오볼루스 미야베아누스(Cochliobolus miyabeanus); 콜레토트리쿰(Colletotrichum) 종, 예를 들어 콜레토트리쿰 린데무타니움(Colletotrichum lindemuthanium); 코르다나(Cordana) 종, 예를 들어 코르다나 무사에(Cordana musae); 코리네스포라(Corynespora) 종, 예를 들어 코리네스포라 카시이콜라(Corynespora cassiicola); 시클로코니움(Cycloconium) 종, 예를 들어 시클로코니움 올레아기눔(Cycloconium oleaginum); 디아포르테(Diaporthe) 종, 예를 들어 디아포르테 시트리(Diaporthe citri); 엘시노에(Elsinoe) 종, 예를 들어 엘시노에 파우세티이(Elsinoe fawcettii); 글로에오스포리움(Gloeosporium) 종, 예를 들어 글로에오스포리움 라에티콜로르(Gloeosporium laeticolor); 글로메렐라(Glomerella) 종, 예를 들어 글로메렐라 신굴라타(Glomerella cingulata); 구이그나르디아(Guignardia) 종, 예를 들어 구이그나르디아 비드웰리(Guignardia bidwelli); 렙토스파에리아(Leptosphaeria) 종, 예를 들어 렙토스파에리아 마쿨란스(Leptosphaeria maculans); 마그나포르테(Magnaporthe) 종, 예를 들어 마그나포르테 그리세아(Magnaporthe grisea); 미크로도키움(Microdochium) 종, 예를 들어 미크로도키움 니발레(Microdochium nivale); 미코스파에렐라(Mycosphaerella) 종, 예를 들어 미코스파에렐라 그라미니콜라(Mycosphaerella graminicola), 미코스파에렐라 아라키디콜라(Mycosphaerella arachidicola) 또는 미코스파에렐라 피지엔시스(Mycosphaerella fijiensis); 파라스타고노스포라(Parastagonospora) 종, 예를 들어 파라스타고노스포라 노도룸(Parastagonospora nodorum); 파에오스파에리아(Phaeosphaeria) 종, 예를 들어 파에오스파에리아 노도룸(Phaeosphaeria nodorum); 피레노포라(Pyrenophora) 종, 예를 들어 피레노포라 테레스(Pyrenophora teres) 또는 피레노포라 트리티시 레펜티스(Pyrenophora tritici repentis); 라물라리아(Ramularia) 종, 예를 들어 라물라리아 콜로-시그니(Ramularia collo-cygni) 또는 라물라리아 아에로라(Ramularia areola); 린코스포리움(Rhynchosporium) 종, 예를 들어 린코스포리움 세칼리스(Rhynchosporium secalis); 세프토리아(Septoria) 종, 예를 들어 세프토리아 아피이(Septoria apii) 또는 세프토리아 리코페르시시(Septoria lycopersici); 스타고노스포라(Stagonospora) 종, 예를 들어 스타고노스포라 노도룸(Stagonospora nodorum); 티풀라(Typhula) 종, 예를 들어 티풀라 인카르나타(Typhula incarnata); 우스틸라고(Ustilago) 종, 예를 들어 우스틸라고 세게툼(Ustilago segetum); 벤투리아(Venturia) 종, 예를 들어 벤투리아 이나에쿠알리스(Venturia inaequalis)로 인한 잎무늬병 및 시들음병;
예를 들어 코르티시움(Corticium) 종, 예를 들어 코르티시움 그라미네아룸(Corticium graminearum); 푸사리움(Fusarium) 종, 예를 들어 푸사리움 옥시스포룸(Fusarium oxysporum); 가에우만노미세스(Gaeumannomyces) 종, 예를 들어 가에우만노미세스 그라미니스(Gaeumannomyces graminis); 플라스모디오포라(Plasmodiophora) 종, 예를 들어 플라스모디오포라 브라시카에(Plasmodiophora brassicae); 리족토니아(Rhizoctonia) 종, 예를 들어 리족토니아 솔라니(Rhizoctonia solani); 사로클라디움(Sarocladium) 종, 예를 들어 사로클라디움 오리자에(Sarocladium oryzae); 스클레로티움(Sclerotium) 종, 예를 들어 스클레로티움 오리자에(Sclerotium oryzae); 타페시아(Tapesia) 종, 예를 들어 타페시아 아쿠포르미스(Tapesia acuformis); 티엘라비옵시스(Thielaviopsis) 종, 예를 들어 티엘라비옵시스 바시콜라(Thielaviopsis basicola)로 인한 뿌리 및 줄기 질병;
예를 들어 알테르나리아(Alternaria) 종, 예를 들어 알테르나리아(Alternaria) 종; 아스페르길루스(Aspergillus) 종, 예를 들어 아스페르길루스 플라부스(Aspergillus flavus); 클라도스포리움(Cladosporium) 종, 예를 들어 클라도스포리움 클라도스포리오이데스(Cladosporium cladosporioides); 클라비셉스(Claviceps) 종, 예를 들어 클라비셉스 푸르푸레아(Claviceps purpurea); 푸사리움(Fusarium) 종, 예를 들어 푸사리움 쿨모룸(Fusarium culmorum); 지베렐라(Gibberella) 종, 예를 들어 지베렐라 제아에(Gibberella zeae); 모노그라펠라(Monographella) 종, 예를 들어 모노그라펠라 니발리스(Monographella nivalis); 스타그노스포라(Stagnospora) 종, 예를 들어 스타그노스포라 노도룸(Stagnospora nodorum)으로 인한 이삭 및 원추화서 질병 (옥수수 속대 포함);
깜부기병 진균, 예를 들어 스파셀로테카(Sphacelotheca) 종, 예를 들어 스파셀로테카 레일리아나(Sphacelotheca reiliana); 틸레티아(Tilletia) 종, 예를 들어 틸레티아 카리에스(Tilletia caries) 또는 틸레티아 콘트로베르사(Tilletia controversa); 우로시스티스(Urocystis) 종, 예를 들어 우로시스티스 오쿨타(Urocystis occulta); 우스틸이라고(Ustilago) 종, 예를 들어 우스틸이라고 누다(Ustilago nuda)로 인한 질병;
예를 들어 아스페르길루스(Aspergillus) 종, 예를 들어 아스페르길루스 플라부스(Aspergillus flavus); 보트리티스(Botrytis) 종, 예를 들어 보트리티스 시네레아(Botrytis cinerea); 모닐리니아(Monilinia) 종, 예를 들어 모닐리니아 락사(Monilinia laxa); 페니실리움(Penicillium) 종, 예를 들어 페니실리움 엑스판숨(Penicillium expansum) 또는 페니실리움 푸르푸로게눔(Penicillium purpurogenum); 리조푸스(Rhizopus) 종, 예를 들어 리조푸스 스톨로니페르(Rhizopus stolonifer); 스클레로티니아(Sclerotinia) 종, 예를 들어 스클레로티니아 스클레로티오룸(Sclerotinia sclerotiorum); 베르티실리움(Verticilium) 종, 예를 들어 베르티실리움 알보아트룸(Verticilium alboatrum)으로 인한 과실썩음병;
예를 들어 알테르나리아(Alternaria) 종, 예를 들어 알테르나리아 브라시시콜라(Alternaria brassicicola); 아파노미세스(Aphanomyces) 종, 예를 들어 아파노미세스 유테이케스(Aphanomyces euteiches); 아스코키타(Ascochyta) 종, 예를 들어 아스코키타 렌티스(Ascochyta lentis); 아스페르길루스(Aspergillus) 종, 예를 들어 아스페르길루스 플라부스(Aspergillus flavus); 클라도스포리움(Cladosporium) 종, 예를 들어 클라도스포리움 헤르바룸(Cladosporium herbarum); 코클리오볼루스(Cochliobolus) 종, 예를 들어 코클리오볼루스 사티부스(Cochliobolus sativus) (분생자 형태: 드레크슬레라(Drechslera), 비폴라리스 신(Bipolaris Syn): 헬민토스포리움(Helminthosporium)); 콜레토트리쿰(Colletotrichum) 종, 예를 들어 콜레토트리쿰 코코데스(Colletotrichum coccodes); 푸사리움(Fusarium) 종, 예를 들어 푸사리움 쿨모룸(Fusarium culmorum); 지베렐라(Gibberella) 종, 예를 들어 지베렐라 제아에(Gibberella zeae); 마크로포미나(Macrophomina) 종, 예를 들어 마크로포미나 파세올리나(Macrophomina phaseolina); 미크로도키움(Microdochium) 종, 예를 들어 미크로도키움 니발레(Microdochium nivale); 모노그라펠라(Monographella) 종, 예를 들어 모노그라펠라 니발리스(Monographella nivalis); 페니실리움 (Penicillium) 종, 예를 들어 페니실리움 엑스판숨(Penicillium expansum); 포마(Phoma) 종, 예를 들어 포마 린감(Phoma lingam); 포모프시스(Phomopsis) 종, 예를 들어 포모프시스 소자에(Phomopsis sojae); 피토프토라(Phytophthora) 종, 예를 들어 피토프토라 칵토룸(Phytophthora cactorum); 피레노포라(Pyrenophora) 종, 예를 들어 피레노포라 그라미네아(Pyrenophora graminea); 피리쿨라리아(Pyricularia) 종, 예를 들어 피리쿨라리아 오리자에(Pyricularia oryzae); 피티움(Pythium) 종, 예를 들어 피티움 울티뭄(Pythium ultimum); 리족토니아(Rhizoctonia) 종, 예를 들어 리족토니아 솔라니(Rhizoctonia solani); 리조푸스(Rhizopus) 종, 예를 들어 리조푸스 오리자에(Rhizopus oryzae); 스클레로티움(Sclerotium) 종, 예를 들어 스클레로티움 롤프시이(Sclerotium rolfsii); 세프토리아(Septoria) 종, 예를 들어 세프토리아 노도룸(Septoria nodorum); 티풀라(Typhula) 종, 예를 들어 티풀라 인카르나타(Typhula incarnata); 베르티실리움(Verticillium) 종, 예를 들어 베르티실리움 달리아에(Verticillium dahliae)로 인한 종자- 및 토양-매개 부패병 및 시들음병, 및 또한 묘목의 질병;
예를 들어 넥트리아(Nectria) 종, 예를 들어 넥트리아 갈리게나(Nectria galligena)에 의해 유발된 암, 혹 및 빗자루병;
예를 들어 베르티실리움(Verticillium) 종, 예를 들어 베르티실리움 롱기스포룸(Verticillium longisporum); 푸사리움(Fusarium) 종, 예를 들어 푸사리움 옥시스포룸(Fusarium oxysporum)으로 인한 시들음병;
예를 들어 엑소바시디움(Exobasidium) 종, 예를 들어 엑소바시디움 벡산스(Exobasidium vexans); 타프리나(Taphrina) 종, 예를 들어 타프리나 데포르만스(Taphrina deformans)로 인한 잎, 꽃 및 과실의 변형;
예를 들어 에스카(Esca) 종, 예를 들어 파에오모니엘라 클라미도스포라(Phaeomoniella chlamydospora), 파에오아크레모니움 알레오필룸(Phaeoacremonium aleophilum) 또는 포미티포리아 메디테라네아(Fomitiporia mediterranea); 가노더마(Ganoderma) 종, 예를 들어 가노더마 보니넨세(Ganoderma boninense)로 인한 목질 식물에서의 변성 질병;
예를 들어 리족토니아(Rhizoctonia) 종, 예를 들어 리족토니아 솔라니(Rhizoctonia solani); 헬민토스포리움(Helminthosporium) 종, 예를 들어 헬민토스포리움 솔라니(Helminthosporium solani)로 인한 식물 괴경의 질병;
박테리아 병원체, 예를 들어 크산토모나스(Xanthomonas) 종, 예를 들어 크산토모나스 캄페스트리스 병원체변종 오리자에(Xanthomonas campestris pv. oryzae); 슈도모나스(Pseudomonas) 종, 예를 들어 슈도모나스 시린가에 병원체변종 라크리만스(Pseudomonas syringae pv. lachrymans); 에르위니아(Erwinia) 종, 예를 들어 에르위니아 아밀로보라(Erwinia amylovora); 리베리박터(Liberibacter) 종, 예를 들어 리베리박터 아시아티쿠스(Liberibacter asiaticus); 크실라(Xyella) 종, 예를 들어 크실렐라 파스티디오사(Xylella fastidiosa); 랄스토니아(Ralstonia) 종, 예를 들어 랄스토니아 솔라나세아룸(Ralstonia solanacearum); 디케야(Dickeya) 종, 예를 들어 디케야 솔라니(Dickeya solani); 클라비박터(Clavibacter) 종, 예를 들어 클라비박터 미시가넨시스(Clavibacter michiganensis); 스트렙토미세스(Streptomyces) 종, 예를 들어 스트렙토미세스 스카비에스(Streptomyces scabies)로 인한 질병.
대두의 질병:
예를 들어, 알테르나리아 점무늬병 (알테르나리아 종 아트란스 테누이시마(Alternaria spec. atrans tenuissima)), 탄저병 (콜레토트리쿰 글로에오스포로이데스 데마티움 변종 트룬카툼(Colletotrichum gloeosporoides dematium var. truncatum)), 갈색점무늬병 (셉토리아 글리시네스(Septoria glycines)), 세르코스포라 점무늬병 및 마름병 (세르코스포라 키쿠키이(Cercospora kikuchii)), 코아네포라 잎마름병 (코아네포라 인푼디불리페라 트리스포라(Choanephora infundibulifera trispora) (동의어)), 닥툴리오포라 점무늬병 (닥툴리오포라 글리시네스(Dactuliophora glycines)), 노균병 (페로노스포라 만슈리카(Peronospora manshurica)), 드레크슬레라 마름병 (드레크슬레라 글리시니(Drechslera glycini)), 콩점무늬병 (세르코스포라 소지나(Cercospora sojina)), 렙토스파에룰리나 점무늬병 (렙토스파에룰리나 트리폴리이(Leptosphaerulina trifolii)), 필로스티카 점무늬병 (필로스티카 소자에콜라(Phyllosticta sojaecola)), 꼬투리 및 줄기 마름병 (포몹시스 소자에(Phomopsis sojae)), 흰가루병 (미크로스파에라 디푸사(Microsphaera diffusa)), 피레노카에타 점무늬병 (피레노카에타 글리시네스(Pyrenochaeta glycines)), 리족토니아 기생, 잎, 및 거미마름병 (리족토니아 솔라니(Rhizoctonia solani)), 녹병 (파코프소라 파키리지(Phakopsora pachyrhizi), 파코프소라 메이보미아에(Phakopsora meibomiae)), 흑성병 (스파셀로마 글리시네스(Sphaceloma glycines)), 스템필리움 잎마름병 (스템필리움 보트리오숨(Stemphylium botryosum)), 돌연사 증후군 (푸사리움 비르굴리포르메(Fusarium virguliforme)), 표적 점무늬병 (코리네스포라 카시이콜라(Corynespora cassiicola))으로 인한 잎, 줄기, 꼬투리 및 종자 상의 진균성 질병.
예를 들어, 검은뿌리썩음병 (칼로넥트리아 크로탈라리아에(Calonectria crotalariae)), 목탄썩음병 (마크로포미나 파세올리나(Macrophomina phaseolina)), 푸사리움 마름병 또는 시들음병, 뿌리썩음병, 및 꼬투리 및 지제부 썩음병 (푸사리움 옥시스포룸(Fusarium oxysporum), 푸사리움 오르토세라스(Fusarium orthoceras), 푸사리움 세미텍툼(Fusarium semitectum), 푸사리움 에퀴세티(Fusarium equiseti)), 미콜렙토디스쿠스 뿌리썩음병(미콜렙토디스쿠스 테레스트리스(Mycoleptodiscus terrestris)), 네오코스모스포라 (네오코스모스포라 바신펙타(Neocosmospora vasinfecta)), 꼬투리 및 줄기 마름병 (디아포르테 파세올로룸(Diaporthe phaseolorum)), 줄기 동고병 (디아포르테 파세올로룸 변종 카울리보라(Diaporthe phaseolorum var. caulivora)), 피토프토라 썩음병 (피토프토라 메가스페르마(Phytophthora megasperma)), 갈색 줄기썩음병 (피알로포라 그레가타(Phialophora gregata)), 피티움 썩음병 (피티움 아파니더마툼(Pythium aphanidermatum), 피티움 이레굴라레(Pythium irregulare), 피티움 데바리아눔(Pythium debaryanum), 피티움 미리오틸룸(Pythium myriotylum), 피티움 울티뭄(Pythium ultimum)), 리족토니아 뿌리썩음병, 줄기 쇠퇴, 및 모잘록병 (리족토니아 솔라니(Rhizoctonia solani)), 스클레로티니아 줄기 쇠퇴 (스클레로티니아 스클레로티오룸(Sclerotinia sclerotiorum)), 스클레로티니아 서던 마름병 (스클레로티니아 롤프시이(Sclerotinia rolfsii)), 티엘라비옵시스 뿌리썩음병 (티엘라비옵시스 바시콜라(Thielaviopsis basicola))으로 인한 뿌리 및 줄기 기부 상의 진균성 질병.
미코톡신
또한, 본 발명의 화합물 조합물 및 조성물은 수확된 물질 및 그로부터 제조된 식품 및 사료 중의 미코톡신 함량을 감소시킬 수 있다. 미코톡신은 특히, 비제한적으로, 하기를 포함한다: 데옥시니발레놀 (DON), 니발레놀, 15-Ac-DON, 3-Ac-DON, T2- 및 HT2-독소, 푸모니신, 제아랄레논, 모닐리포르민, 푸사린, 디아세오톡시시르페놀 (DAS), 뷰베리신, 에니아틴, 푸사로프롤리페린, 푸사레놀, 오크라톡신, 파툴린, 맥각 알칼로이드 및 아플라톡신 (예를 들어, 하기 진균에 의해 생산될 수 있음): 푸사리움(Fusarium) 종, 예컨대 에프. 아쿠미나툼(F. acuminatum), 에프. 아시아티쿰(F. asiaticum), 에프. 아베나세움(F. avenaceum), 에프. 크룩웰렌세(F. crookwellense), 에프. 쿨모룸(F. culmorum), 에프. 그라미네아룸(F. graminearum) (지베렐라 제아에(Gibberella zeae)), 에프. 에퀴세티(F. equiseti), 에프. 푸지코로이(F. fujikoroi), 에프. 무사룸(F. musarum), 에프. 옥시스포룸(F. oxysporum), 에프. 프로리페라툼(F. proliferatum), 에프. 포아에(F. poae), 에프. 슈도그라미네아룸(F. pseudograminearum), 에프. 삼부시눔(F. sambucinum), 에프. 시르피(F. scirpi), 에프. 세미텍툼(F. semitectum), 에프. 솔라니(F. solani), 에프. 스포로트리코이데스(F. sporotrichoides), 에프. 랑세티아에(F. langsethiae), 에프. 서브글루티난스(F. subglutinans), 에프. 트리신크툼(F. tricinctum), 에프. 베르티실리오이데스(F. verticillioides), 및 또한 아스페르길루스(Aspergillus) 종, 예컨대 에이. 플라부스(A. flavus), 에이. 파라시티쿠스(A. parasiticus), 에이. 노미우스(A. nomius), 에이. 오크라세우스(A. ochraceus), 에이. 클라바투스(A. clavatus), 에이. 테레우스(A. terreus), 에이. 베르시콜로르(A. versicolor), 페니실리움(Penicillium) 종, 예컨대 피. 베루코숨(P. verrucosum), 피. 비리디카툼(P. viridicatum), 피. 시트리눔(P. citrinum), 피. 엑스판숨(P. expansum), 피. 클라비포르메(P. claviforme), 피. 로퀘포르티(P. roqueforti), 클라비셉스(Claviceps) 종, 예컨대 씨. 푸르푸레아(C. purpurea), 씨. 푸시포르미스(C. fusiformis), 씨. 파스팔리(C. paspali), 씨. 아프리카나(C. africana), 스타키보트리스(Stachybotrys) 종 등.
물질 보호
본 발명의 화합물 조합물 및 조성물은 또한 물질의 보호, 특히 식물병원성 진균에 의한 공격 및 파괴에 대한 산업 물질의 보호에 사용될 수 있다.
또한, 본 발명의 화합물 조합물 및 조성물은 단독으로 또는 다른 활성 성분과의 조합으로써 항부착물 조성물로서 사용될 수 있다.
본 발명의 문맥에서 산업적 물질은 산업에서 사용하기 위해 제조된 무생물 물질을 의미하는 것으로 이해된다. 예를 들어, 미생물 변경 또는 파괴로부터 보호되어야 하는 산업적 물질은 접착제, 글루, 종이, 벽지 및 보드/카드보드, 텍스타일, 카펫, 가죽, 목재, 섬유 및 티슈, 페인트 및 플라스틱 물품, 냉각 윤활제, 및 미생물에 의해 감염 또는 파괴될 수 있는 다른 물질일 수 있다. 미생물의 증식에 의해 손상될 수 있는 생산 플랜트 및 건물의 부분, 예를 들어 냉각수 회로, 냉각 및 가열 시스템 및 환기 및 공기-조화 유닛이 또한 보호될 물질의 범주 내에서 언급될 수 있다. 본 발명의 범위 내의 산업적 물질은 바람직하게는 접착제, 사이즈, 종이 및 카드, 가죽, 목재, 페인트, 냉각 윤활제 및 열 전달 유체, 보다 바람직하게는 목재를 포함한다.
본 발명의 화합물 조합물 및 조성물은 부작용, 예컨대 부패, 변색, 탈색 또는 곰팡이 형성을 방지할 수 있다.
목재 처리의 경우에, 본 발명의 화합물 조합물 및 조성물은 또한 재목 상에서 또는 재목 내부에서 성장하기 쉬운 진균성 질병에 대해 사용될 수 있다.
재목은 모든 유형의 목재 종, 및 건설을 위한 이러한 목재의 모든 유형의 작업물, 예를 들어 중실 목재, 고밀도 목재, 적층 목재 및 합판을 의미한다. 또한, 본 발명의 화합물 및 조성물은 염수 또는 기수와 접촉하는 물체, 특히 선체, 스크린, 그물, 건물, 계선구 및 신호 시스템을 오손으로부터 보호하는 데 사용될 수 있다.
본 발명의 화합물 조합물 및 조성물은 또한 저장 제품을 보호하기 위해 사용될 수 있다. 저장 제품은 식물 또는 동물 기원의 천연 물질 또는 천연 기원의 그의 가공 제품을 의미하는 것으로 이해되며, 이를 위해 장기 보호가 요구된다. 식물성 기원의 저장 제품, 예를 들어 식물 또는 식물 부분, 예컨대 줄기, 잎, 괴경, 종자, 과실, 곡물은 신선하게 수확되거나 또는 (예비)건조, 습윤화, 파분쇄, 분쇄, 압착 또는 로스팅에 의한 가공 후에 보호될 수 있다. 저장 제품은 또한 가공되지 않은 재목, 예컨대 건설용 재목, 전기 폴 및 배리어, 또는 완성된 제품, 예컨대 가구 형태를 둘 다를 포함한다. 동물 기원의 저장 제품은, 예를 들어 히드, 가죽, 모피 및 모발이다. 본 발명의 화합물 조합물 및 조성물은 부작용, 예컨대 부패, 변색, 탈색 또는 곰팡이 형성을 방지할 수 있다.
산업 재료를 분해 또는 변경시킬 수 있는 미생물은, 예를 들어 박테리아, 진균, 효모, 조류 및 점액 유기체를 포함한다. 본 발명의 화합물 조합물 및 조성물은 바람직하게는 진균, 특히 곰팡이, 목재-변색 및 목재-파괴 진균 (아스코미세테스(Ascomycetes), 바시디오미세테스(Basidiomycetes), 듀테로미세테스(Deuteromycetes) 및 지고미세테스(Zygomycetes)), 및 점액 유기체 및 조류에 대해 작용한다. 예는 하기 속의 미생물을 포함한다: 알테르나리아(Alternaria), 예컨대 알테르나리아 테누이스(Alternaria tenuis); 아스페르길루스(Aspergillus), 예컨대 아스페르길루스 니거(Aspergillus niger); 카에토미움(Chaetomium), 예컨대 카에토미움 글로보숨(Chaetomium globosum); 코니오포라(Coniophora), 예컨대 코니오포라 푸에타나(Coniophora puetana); 렌티누스(Lentinus), 예컨대 렌티누스 티그리누스(Lentinus tigrinus); 페니실리움(Penicillium), 예컨대 페니실리움 글라우쿰(Penicillium glaucum); 폴리포루스(Polyporus), 예컨대 폴리포루스 베르시콜로르(Polyporus versicolor); 아우레오바시디움(Aureobasidium), 예컨대 아우레오바시디움 풀루란스(Aureobasidium pullulans); 스클레로포마(Sclerophoma), 예컨대 스클레로포마 피티오필라(Sclerophoma pityophila); 트리코더마(Trichoderma), 예컨대 트리코더마 비리데(Trichoderma viride); 오피오스토마(Ophiostoma) 종, 세라토시스티스(Ceratocystis) 종, 휴미콜라(Humicola) 종, 페트리엘라(Petriella) 종, 트리쿠루스(Trichurus) 종, 코리올루스(Coriolus) 종, 글로에오필룸(Gloeophyllum) 종, 플레우로투스(Pleurotus) 종, 포리아(Poria) 종, 세르풀라(Serpula) 종 및 티로미세스(Tyromyces) 종, 클라도스포리움(Cladosporium) 종, 파에실로미세스(Paecilomyces) 종, 무코르(Mucor) 종, 에스케리키아(Escherichia), 예컨대 에스케리키아 콜라이(Escherichia coli); 슈도모나스(Pseudomonas), 예컨대 슈도모나스 아에루기노사(Pseudomonas aeruginosa); 스타필로코쿠스(Staphylococcus), 예컨대 스타필로코쿠스 아우레우스(Staphylococcus aureus), 칸디다(Candida) 종 및 사카로미세스(Saccharomyces) 종, 예컨대 사카로미세스 세레비사에(Saccharomyces cerevisae).
종자 처리
본 발명의 화합물 조합물 및 조성물은 또한 원치 않는 미생물, 예컨대 식물병원성 미생물, 예를 들어 식물병원성 진균 또는 식물병원성 난균류로부터 종자를 보호하는 데 사용될 수 있다. 본원에 사용된 용어 종자(들)는 휴면 종자, 프라이밍된 종자, 발아전 종자 및 발아된 뿌리 및 잎을 갖는 종자를 포함한다.
따라서, 본 발명은 또한 종자를 본 발명의 화합물 조합물 또는 조성물로 처리하는 단계를 포함하고, 여기서 종자는 동시에, 개별적으로 또는 순차적으로 화합물 (A) 및 (B)로 처리될 수 있는, 원치 않는 미생물로부터 종자를 보호하는 방법에 관한 것이다.
본 발명의 화합물 조합물 또는 조성물로의 종자의 처리는 식물병원성 미생물로부터 종자를 보호할 뿐만 아니라, 처리된 종자로부터의 출아 후 발아 종자, 출아 묘목 및 식물을 보호한다. 따라서, 본 발명은 또한 종자, 발아 종자 및 신생 묘목을 보호하는 방법에 관한 것이다.
종자 처리는 파종 전에, 파종 시에 또는 그 직후에 수행될 수 있다.
종자 처리가 파종 전에 수행되는 경우 (예를 들어 소위 종자-적용), 종자 처리는 하기와 같이 수행될 수 있다: 종자는 목적하는 양의 본 발명의 화합물 조합물 또는 조성물과 함께 혼합기에 넣을 수 있고, 종자 및 본 발명의 화합물 조합물 또는 조성물은 종자 상의 균질 분포가 달성될 때까지 혼합된다. 적절한 경우에, 종자는 이어서 건조될 수 있다.
본 발명은 또한 본 발명의 화합물 조합물 또는 조성물로 코팅된 종자에 관한 것이다.
바람직하게는, 종자는 처리 과정에서 손상이 발생하지 않도록 충분히 안정한 상태로 처리된다. 일반적으로, 종자는 수확 사이 및 파종 직후의 임의의 시점에 처리될 수 있다. 식물로부터 분리되고 속대, 껍질, 줄기, 외피, 털 또는 과육이 제거된 종자를 사용하는 것이 통상적이다. 예를 들어, 수확되고, 세정되고, 15 중량% 미만의 수분 함량으로 건조된 종자를 사용하는 것이 가능하다. 대안적으로, 건조 후에, 예를 들어 물로 처리한 다음 다시 건조시킨 종자, 또는 프라이밍 직후의 종자, 또는 프라이밍된 조건 하에 저장된 종자 또는 예비-발아된 종자, 또는 육묘 트레이, 테이프 또는 종이 상에 파종된 종자를 사용하는 것이 또한 가능하다.
종자에 적용되는 본 발명의 화합물 조합물 또는 조성물의 양은 전형적으로 종자의 발아가 손상되지 않거나 또는 생성된 식물이 손상되지 않도록 하는 양이다. 이는 특히 본 발명의 화합물 조합물에 함유된 화합물이 특정 적용률에서 식물독성 효과를 나타내는 경우에 보장되어야 한다. 트랜스제닉 식물의 고유 표현형은 또한 최소량의 화합물을 사용하면서 최적의 종자 및 발아 식물 보호를 달성하기 위해 종자에 적용되는 본 발명의 화합물 조합물의 양을 결정할 때 고려되어야 한다.
본 발명의 화합물 조합물에 함유된 화합물은 그대로, 즉 임의의 다른 성분의 사용 없이 및 희석 없이 종자에 직접 적용될 수 있다. 이들은 동시, 개별 또는 순차 방식으로 적용될 수 있다. 또한, 본 발명의 화합물 조합물에 함유된 화합물을 함유하는 조성물, 예컨대 본 발명의 조성물은 종자에 적용될 수 있다.
본 발명의 화합물 조합물 및 조성물은 임의의 식물 품종의 종자를 보호하는 데 적합하다. 바람직한 종자는 곡류 (예컨대 밀, 보리, 호밀, 기장, 라이밀 및 귀리), 유지종자 평지, 옥수수, 목화, 대두, 벼, 감자, 해바라기, 콩, 커피, 완두콩, 비트 (예를 들어 사탕무 및 사료용 비트), 땅콩, 채소 (예컨대 토마토, 오가, 양파 및 상추), 잔디 및 관상 식물의 종자이다. 밀, 대두, 유지종자 평지, 옥수수 및 벼의 종자가 보다 바람직하다.
본 발명의 화합물 조합물 및 조성물은 트랜스제닉 종자, 특히 해충, 제초 손상 또는 비생물적 스트레스에 대해 작용하는 폴리펩티드 또는 단백질을 발현할 수 있는 식물의 종자를 처리하여 보호 효과를 증가시키는 데 사용될 수 있다. 해충, 제초 손상 또는 비생물적 스트레스에 대해 작용하는 폴리펩티드 또는 단백질을 발현할 수 있는 식물의 종자는 상기 폴리펩티드 또는 단백질의 발현을 허용하는 적어도 1종의 이종 유전자를 함유할 수 있다. 트랜스제닉 종자에서의 이들 이종 유전자는, 예를 들어 바실루스, 리조비움, 슈도모나스, 세라티아, 트리코더마, 클라비박터, 글로무스 또는 글리오클라디움 종의 미생물로부터 유래될 수 있다. 이들 이종 유전자는 바람직하게는 바실루스 종으로부터 유래되고, 이 경우에 유전자 산물은 유럽 옥수수 천공충 및/또는 서부 옥수수 뿌리벌레에 대해 효과적이다. 특히 바람직하게는, 이종 유전자는 바실루스 투린기엔시스로부터 유래된다.
적용
본 발명의 화합물 조합물은 그 자체로, 또는 예를 들어 즉시 사용가능한 용액, 에멀젼, 물- 또는 오일-기재 현탁액, 분말, 습윤성 분말, 페이스트, 가용성 분말, 분진, 가용성 과립, 살포용 과립, 유현탁액 농축물, 화합물 조합물로 함침된 천연 생성물, 화합물 조합물로 함침된 합성 물질, 비료 또는 중합체 물질 중의 마이크로캡슐화물의 형태로 적용될 수 있다.
적용은 통상의 방식으로, 예를 들어 살수, 분무, 살포, 살분, 발포 또는 스프레딩-온에 의해 달성된다. 또한, 점적 관개 시스템 또는 드렌치 적용을 통해 초저부피 방법에 의해 본 발명의 화합물 조합물을 배치하여, 이를 고랑 내에 적용하거나 또는 이를 토양 줄기 또는 몸통 내로 주입하는 것이 가능하다. 본 발명의 화합물 조합물을 상처 실, 페인트 또는 다른 상처 드레싱에 의해 적용하는 것이 추가로 가능하다. 식물, 식물 부분, 과실, 종자 또는 토양에 적용되는 본 발명의 화합물 조합물의 유효하고 식물-상용성인 양은 다양한 인자, 예컨대 사용되는 화합물/조성물, 처리의 대상 (식물, 식물 부분, 과실, 종자 또는 토양), 처리의 유형 (살분, 분무, 종자 드레싱), 처리의 목적 (치유 및 보호), 미생물의 유형, 미생물의 발생 단계, 미생물의 감수성, 작물 성장 단계 및 환경 조건에 따라 달라질 것이다.
본 발명의 화합물 조합물이 살진균제로서 사용되는 경우에, 적용률은 적용의 종류에 따라 비교적 넓은 범위 내에서 달라질 수 있다. 식물 부분, 예컨대 잎의 처리의 경우, 적용률은 0.1 내지 10,000 g/ha, 바람직하게는 10 내지 1000 g/ha, 보다 바람직하게는 50 내지 300 g/ha의 범위일 수 있다 (살수 또는 점적에 의한 적용의 경우에, 특히 불활성 기재, 예컨대 암면 또는 펄라이트가 사용되는 경우에, 적용률을 감소시키는 것이 심지어 가능함). 종자의 처리의 경우, 적용률은 종자 100 kg당 0.1 내지 200 g, 바람직하게는 종자 100 kg당 1 내지 150 g, 보다 바람직하게는 종자 100 kg당 2.5 내지 25 g, 보다 더 바람직하게는 종자 100 kg당 2.5 내지 12.5 g의 범위일 수 있다. 토양의 처리의 경우, 적용률은 0.1 내지 10,000 g/ha, 바람직하게는 1 내지 5000 g/ha의 범위일 수 있다. 약술된 적용률은 본 발명의 화합물 조합물에 존재하는 화합물 (A) 및 (B) 총 적용률을 지칭한다.
이들 적용률은 단지 예일 뿐이며, 본 발명의 범주를 제한하는 것으로 의도되지 않는다.
본 발명의 화합물 조합물 및 조성물은, 예를 들어 현장 특이적 작물 관리, 위성 농업, 정밀 농업 또는 정밀 농업을 위한 컴퓨터 프로그램에 내장된 모델과 조합되어 사용될 수 있다. 이러한 모델은 환경의 수익성, 지속성 및 보호를 최적화하기 위한 목적으로 토양, 기후, 작물 (예를 들어 유형, 성장 단계, 식물 건강), 잡초 (예를 들어 유형, 성장 단계), 질병, 해충, 영양소, 물, 수분, 바이오매스, 위성 데이터, 수율 등과 같은 다양한 공급원으로부터의 데이터로 농업 사이트의 사이트 특이적 관리를 지지한다. 특히, 이러한 모델은 농경학적 결정을 최적화하고, 살충제 적용의 정밀도를 제어하고, 수행된 작업을 기록하는 것을 보조할 수 있다.
예로서, 본 발명의 화합물은, 모델이 진균성 질병의 발병을 모델링하고, 본 발명의 화합물을 작물 식물에 적용하는 것이 권장될 수 있는 역치에 도달하였음을 계산하는 경우, 적절한 투여 요법에 따라 작물 식물에 적용될 수 있다.
농경 모델을 포함하는 상업적으로 입수가능한 시스템은, 예를 들어 더 클리메이트 코포레이션(The Climate Corporation)으로부터의 필드스크립츠(FieldScripts)™, 바스프(BASF)로부터의 자르비오(Xarvio)™, 존 디어(John Deere)로부터의 아글로직(AGLogic)™ 등이다.
본 발명의 화합물은 또한 스마트 분무 장비, 예컨대 예를 들어 농장 차량, 예컨대 트랙터, 로봇, 헬리콥터, 비행기, 무인 항공 차량 (UAV), 예컨대 드론 등에 부착되거나 또는 그 내에 수용된 스팟 분무 또는 정밀 분무 장비와 조합되어 사용될 수 있다. 이러한 장비는 통상적으로 입력 센서 (예컨대 예를 들어 카메라), 및 입력 데이터를 분석하도록 구성되고 입력 데이터의 분석에 기초한 결정을 제공하여 본 발명의 화합물을 작물 식물 (각각 잡초)에 특정하고 정확한 방식으로 적용하도록 구성된 처리 유닛을 포함한다. 이러한 스마트 스프레이 장비의 사용은 통상적으로 또한, 기록된 데이터를 위치파악하고 농장 차량을 안내 또는 제어하기 위한 위치 시스템 (예를 들어 GPS 수신기); 지능형 지도 상의 정보를 나타내기 위한 지리적 정보 시스템 (GIS), 및 분무와 같은 요구되는 농장 조치를 수행하기 위한 적절한 농장 차량을 필요로 한다.
한 예에서, 진균성 질병은 카메라에 의해 획득된 영상으로부터 검출될 수 있다. 한 예에서, 진균성 질병은 그 영상에 기초하여 확인 및/또는 분류될 수 있다. 이러한 식별 및/또는 분류는 영상 처리 알고리즘을 이용할 수 있다. 이러한 영상 처리 알고리즘은 기계 학습 알고리즘, 예컨대 훈련된 중성 네트워크, 의사결정 트리를 이용할 수 있고, 인공 지능 알고리즘을 이용할 수 있다. 이러한 방식으로, 본원에 기재된 화합물은 필요한 경우에만 적용될 수 있다.
실시예
일반
LogP 값의 측정
본원에 제공된 바와 같은 LogP 값의 측정은 하기 방법으로 역상 칼럼 상에서 HPLC (고성능 액체 크로마토그래피)에 의해 EEC 지침 79/831 부록 V.A8에 따라 수행하였다:
[a] LogP 값은 LC-UV의 측정에 의해, 산성 범위 내에서, 용리액으로서 0.1% 포름산/물 및 아세토니트릴 (10% 아세토니트릴에서 95% 아세토니트릴의 선형 구배)을 사용하여 결정한다.
[b] LogP 값은 LC-UV의 측정에 의해, 중성 범위 내에서, 용리액으로서 0.001 몰 아세트산암모늄 용액/물 및 아세토니트릴 (10% 아세토니트릴에서 95% 아세토니트릴의 선형 구배)을 사용하여 결정한다.
[c] LogP 값은 LC-UV의 측정에 의해, 산성 범위 내에서, 용리액으로서 0.1% 인산 및 아세토니트릴 (10% 아세토니트릴에서 95% 아세토니트릴의 선형 구배)을 사용하여 결정한다.
1개 초과의 LogP 값이 동일한 방법 내에서 이용가능한 경우, 모든 값이 주어지고 "+"로 분리된다.
보정은 기지의 LogP 값을 갖는 직쇄 알칸2-온 (3 내지 16개의 탄소 원자를 가짐)을 사용하여 수행하였다 (연속적 알카논 사이에 선형 내삽으로 체류 시간을 사용한 LogP 값의 측정). 람다-최대-값은 200 nm 내지 400 nm의 UV-스펙트럼 및 크로마토그래피 신호의 피크 값을 사용하여 결정하였다.
1H-NMR 데이터
본원에 제공된 바와 같은 선택된 실시예의 1H-NMR 데이터는 1H-NMR-피크 목록의 형태로 표기된다. 각각의 신호 피크에 대해 δ-값 (ppm) 및 둥근 괄호 안의 신호 강도가 열거된다. δ-값 - 신호 강도 쌍 사이에 구분 기호로서 세미콜론이 존재한다.
따라서, 실시예의 피크 목록은 하기 형태를 갖는다:
δ1 (강도1); δ2 (강도2);........; δi (강도i);......; δn (강도n)
예리한 신호의 강도는 NMR 스펙트럼의 출력된 예에서의 신호의 높이 (cm)와 상관관계가 있고, 신호 강도의 실제 관계를 나타낸다. 넓은 신호로부터 여러 피크 또는 신호의 중간 및 스펙트럼에서의 가장 강한 신호와 비교한 그의 상대 강도가 제시될 수 있다.
1H 스펙트럼에 대한 화학적 이동을 보정하기 위해, 본 발명자들은 테트라메틸실란 및/또는 특히 DMSO 중에서 측정된 스펙트럼의 경우에 사용된 용매의 화학적 이동을 사용한다. 따라서 NMR 피크 목록에서, 테트라메틸실란 피크가 발생할 수 있으나 반드시 그러한 것은 아니다.
1H-NMR 피크 목록은 전형적인 1H-NMR 출력물과 유사하며, 따라서 통상적으로 전형적인 NMR-해석에서 열거되는 모든 피크를 함유한다.
추가적으로 이들은, 용매, 또한 본 발명의 목적인 목적 화합물의 입체이성질체, 및/또는 불순물의 피크의 신호를 전형적인 1H-NMR 출력물과 같이 나타낼 수 있다.
용매 및/또는 물의 델타-범위 내의 화합물 신호를 나타내기 위해, 용매의 통상적인 피크, 예를 들어 DMSO-D6 중 DMSO의 피크 및 물의 피크가 본 발명자들의 1H-NMR 피크 목록에 제시되며, 통상적으로 평균적으로 높은 강도를 갖는다.
목적 화합물의 입체이성질체의 피크 및/또는 불순물의 피크는 통상적으로 목적 화합물 (예를 들어 >90%의 순도를 가짐)의 피크보다 평균적으로 더 낮은 강도를 갖는다.
이러한 입체이성질체 및/또는 불순물은 특정 제조 방법에 전형적일 수 있다. 따라서 이들의 피크는 "부산물-지문"을 통해 본 발명자들의 제조 방법의 재현을 인식하는 데 도움이 될 수 있다.
공지된 방법 (MestreC, ACD-시뮬레이션, 또한 실험적으로 평가된 예상치 포함)으로 목적 화합물의 피크를 계산하는 전문가는 필요에 따라 임의로 추가의 강도 필터를 사용하여 목적 화합물의 피크를 단리할 수 있다. 상기 단리는 전형적인 1H-NMR 해석에서의 관련 피크 선별과 유사할 것이다.
피크 목록의 NMR-데이터 설명의 추가의 세부사항은 간행물 ["Citation of NMR Peaklist Data within Patent Applications" of the Research Disclosure Database Number 564025]에서 찾아볼 수 있다.
거울상이성질체의 분리
라세미체의 거울상이성질체 분리는 이동상으로서의 초임계 이산화탄소 및 개질제로서의 저급 알콜, 보다 바람직하게는 15 내지 30 부피%에 포함되는 비의 메탄올, 에탄올 또는 이소프로판올을 사용하는 정제용 초임계 유체 크로마토그래피에 의해 수행된다. 총 유량은 70-100 ml/분의 범위이고, 크로마토그래피 분리는 30℃ 내지 50℃ 범위의 온도 및 70 bar 내지 130 bar 범위의 배압에서, 상업적으로 입수가능하고 하기와 같이 공지된 온도조절된 키랄 고정상 중 하나에서 수행된다:
- 다이셀 케미칼 인더스트리즈, 리미티드(Daicel Chemical Industries, Ltd.)로부터 키랄팩(ChiralPak)® IA, 250x20mm.
- 룩스(Lux)® 아밀로스-1, 250x21.2mm 5 μm, 페노메넥스 인크.(Axia packed from Phenomenex Inc.)로부터 패킹된 악시아.
- 룩스® 셀룰로스-1, 250x21.2mm 5 μm, 페노메넥스 인크.로부터 패킹된 악시아.
- 룩스® i-셀룰로스-5, 250x21.2mm 5 μm, 페노메넥스 인크.로부터 패킹된 악시아.
정제용 규모의 분리는 210nm 내지 280nm, 바람직하게는 220 내지 254nm 범위의 UV-검출을 갖는 피크 솔루션(Pic Solution)으로부터의 장치 SFC-피클랩 하이브리드(PICLAB Hybrid) 10-150에서 수행하였다.
하기 실시예는 본 발명에 따른 화학식 (I)의 화합물의 제조예 및 생물학적 활성을 비제한적인 방식으로 설명한다.
화학식 (I)의 화합물 및 중간체의 합성
화학식 (I)의 화합물의 합성
실시예 1의 제조: rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.059)의 제조
단계 1: 에틸 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복실레이트의 제조
아르곤 하에, 수소화나트륨 (2.8 g, 70 mmol)을 DMF (30 mL) 중 3-(트리플루오로메틸)페놀 (9.7 g, 60 mmol)의 용액에 첨가하였다. 반응 혼합물을 실온에서 1시간 동안 교반한 다음, 에틸 3,6-디클로로피리다진-4-카르복실레이트 (13.8 g, 50 mmol)를 용액에 조금씩 첨가하였다. 반응 혼합물을 실온에서 18시간 동안 교반한 다음, 물로 희석하고, 에테르 (3 x 200 mL)로 추출하였다. 유기 추출물을 물 및 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하여, 용매를 증발시킨 후, 에틸 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복실레이트 20 g (90% 순도, 100% 수율)을 오일로서 수득하였다.
단계 2: 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복실산의 제조
디옥산/물 2:1 (75 mL) 중 에틸 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복실레이트 (15 g, 35 mmol)의 용액에 수산화리튬 (2.5 g, 105 mmol)을 첨가하였다. 반응물을 실온에서 4시간 동안 교반한 다음, 물로 희석하였다. 수성 상을 1M 수성 HCl 용액을 사용하여 산성화시키고, 에틸 아세테이트 (3 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복실산 9.7 g (98% 순도, 85% 수율)을 고체로서 수득하였다.
단계 3: 6-클로로-N-[rac-1-[(2,4-디메틸페닐)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (화합물 3-16)의 제조
아르곤 하에, DMF (100 mL) 중 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복실산 (5.0 g, 15.7 mmol) 및 HATU (6.56 g, 17.26 mmol)의 용액에 0℃에서 2-[rac-2-아미노-3-(2,4-디메틸페닐)프로폭시]이소인돌린-1,3-디온;2,2,2-트리플루오로아세트산 (7.57 g, 17.26 mmol) 및 N,N-디이소프로필에틸아민 (8.2 mL, 47.07 mmol)을 연속적으로 첨가하였다. 0℃에서 15분 후, 반응 혼합물을 실온에서 3시간 동안 교반하였다. 이어서, 이를 물로 희석하고, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, 6-클로로-N-[rac-1-[(2,4-디메틸페닐)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 7.95 g (100% 순도, 81% 수율)을 백색 고체로서 수득하였다.
단계 4: 6-클로로-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페닐)에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (화합물 4-17)의 제조
아르곤 하에, 히드라진 1수화물 (2.31 mL, 37.92 mmol)을 DCM/MeOH (110 mL, 1:1) 중 6-클로로-N-[rac-1-[(2,4-디메틸페닐)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (7.9 g, 12.64 mmol)의 용액에 첨가하였다. 반응 혼합물을 실온에서 4시간 동안 교반하고, 농축시켰다. 이어서, 이를 물로 희석하고, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 6-클로로-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페닐)에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 6.35 g (97% 순도, 98% 수율)을 황색 오일로서 수득하였다.
단계 5: rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진의 제조
아르곤 하에, POCl3 (3.56 mL, 38.19 mmol)를 80℃에서 AcCN (114 mL) 중 6-클로로-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페닐)에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (6.3 g, 12.73 mmol)의 용액에 첨가하였다. 반응 혼합물을 80℃에서 18시간 동안 교반하였다. 실온으로 냉각시킨 후, 혼합물을 포화 중탄산나트륨 용액에 부는 다음, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하여, 용매를 증발시킨 후, rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 2.52 g (98% 순도, 41% 수율)을 황색 고체로서 수득하였다.
실시예 2의 제조: rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.059)의 제조
단계 1: 6-클로로-N-[1-(클로로메틸)-2-(2,4-디메틸페닐)에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (화합물 21-01)의 제조
디클로로메탄 (2 mL) 중 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복실산 (100 mg, 0.31 mmol)의 용액에 실온에서 옥살릴 클로라이드 (119 mg, 0.94 mmol) 및 한 방울의 디메틸포름아미드를 첨가하였다. 30분 후, 반응물을 감압 하에 농축시켰다. 잔류물을 디클로로메탄 (2 mL) 중에 용해시키고, 0℃에서 디클로로메탄 (1 mL) 중 1-클로로-3-(2,4-디메틸페닐)프로판-2-아민;히드로클로라이드 (73 mg, 0.31 mmol)의 현탁액에 첨가한 다음, 이어서 N,N-디이소프로필에틸아민 (0.16 mL, 0.94 mmol)을 첨가하였다. 반응 혼합물을 실온에서 1시간 동안 교반한 다음, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, 6-클로로-N-[1-(클로로메틸)-2-(2,4-디메틸페닐)에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 142 mg (87% 순도, 79% 수율)을 무색 오일로서 수득하였다.
단계 2: 6-클로로-N-[1-(클로로메틸)-2-(2,4-디메틸페닐)에틸]-N'-히드록시-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (화합물 20-01)의 제조
AcCN (2 mL) 중 6-클로로-N-[1-(클로로메틸)-2-(2,4-디메틸페닐)에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (130 mg, 0.23 mmol)의 용액에 오염화인 (205 mg, 0.99 mmol)을 첨가하였다. 반응 혼합물을 실온에서 18시간 동안 교반한 다음, 감압 하에 농축시켰다. 잔류물을 AcCN (5 mL) 중에 용해시키고, 물 중 히드록실아민의 용액 (300 mg, 4.53 mmol, 물 중 50%)을 반응 혼합물에 첨가하였다. 실온에서 1시간 동안 교반한 후, 반응 혼합물을 물 및 톨루엔으로 희석하고, 에틸 아세테이트 (3 x 50 mL)로 추출하였다. 유기 추출물을 물 및 염수로 세척하고, 황산나트륨 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 6-클로로-N-[1-(클로로메틸)-2-(2,4-디메틸페닐)에틸]-N'-히드록시-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 150 mg (65% 순도, 83% 수율)을 황색 오일로서 수득하였다.
단계 3: rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진의 제조
AcCN (2 mL) 중 6-클로로-N-[1-(클로로메틸)-2-(2,4-디메틸페닐)에틸]-N'-히드록시-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (150 mg, 0.23 mmol)의 용액에 포타슘 tert-부톡시드 (47.3 mg, 0.42 mmol)를 첨가하였다. 반응 혼합물을 실온에서 1시간 30분 동안 교반한 다음, 포화 염화암모늄 용액으로 희석하고, 디클로로메탄 (2 x 50 mL)으로 추출하였다. 유기 추출물을 황산나트륨 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 56 mg (87% 순도, 43% 수율)을 황색 고체로서 수득하였다.
실시예 3의 제조: rac-5-(4-클로로페닐)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.040)의 제조
단계 1: 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르보니트릴 (화합물 9-03)의 제조
아르곤 하에, 수소화나트륨 (1.30 g, 32 mmol)을 0℃에서 THF (100 mL) 중 3-(트리플루오로메틸)페놀 (4.6 g, 28 mmol)의 용액에 첨가하였다. 30분 후, 3,6-디클로로피리다진-4-카르보니트릴 (5.0 g, 28.7 mmol)을 용액에 조금씩 첨가하였다. 반응 혼합물을 실온에서 3시간 동안 교반한 다음, 포화 염화암모늄 용액으로 희석하고, EtOAc (3 x 200 mL)로 추출하였다. 유기 추출물을 물 및 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하여, 용매를 증발시킨 후, 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르보니트릴 6.1 g (95% 순도, 67% 수율)을 오일로서 수득하였다.
단계 2: 6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르보니트릴 (화합물 9-02)의 제조
아르곤 하에, 2,4,6-트리메틸-1,3,5,2,4,6-트리옥사트리보리난 (12.57 g, 50.0 mmol)을 디옥산 (30 mL) 중 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르보니트릴 (3.0 g, 10.0 mmol), 디클로로메탄과의 [1,1'-비스(디페닐포스피노)페로센]디클로로팔라듐(II) 착물 (64 mg, 0.10 mmol) 및 탄산세슘 (4.89 g, 15.0 mmol)의 교반 용액에 첨가하였다. 반응 혼합물을 100℃에서 4시간 동안 교반한 다음, 물로 희석하고, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하여, 용매를 증발시킨 후, 6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르보니트릴 1.82 g (100% 순도, 65% 수율)을 고체로서 수득하였다.
단계 3: N'-히드록시-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (화합물 10-02)의 제조
EtOH (32 mL) 중 6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르보니트릴 (1.82 g, 6.52 mmol)의 용액에 히드록실아민 히드로클로라이드 (1.13 g, 16.29 mmol) 및 탄산칼륨 (2.25 g, 16.29 mmol)을 첨가하였다. 반응 혼합물을 60℃에서 2시간 동안 교반하였다. 침전물을 여과하였다. 여과물을 농축시키고, 물로 희석하고, EtOAc (2 x 100 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, N'-히드록시-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 1.38 g (91% 순도, 62% 수율)을 황색 고체로서 수득하였다.
단계 4: N'-[2-(4-클로로페닐)-2-옥소-에톡시]-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (화합물 12-03)의 제조
아르곤 하에, 2-tert-부틸이미노-N,N-디에틸-1,3-디메틸-1,3,2람다5-디아자포스피난-2-아민 (BEMP) (210.9 mg, 0.77 mmol)을 AcCN (2.7 mL) 중 N'-히드록시-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (200 mg, 0.64 mmol)의 용액에 실온에서 첨가하였다. 15분 후, 2-브로모-1-(4-클로로페닐)에타논 (224 mg, 0.96 mmol)을 첨가하고, 반응물을 추가로 3시간 동안 교반한 다음, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, N'-[2-(4-클로로페닐)-2-옥소-에톡시]-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 65.6 mg (91% 순도, 20% 수율)을 오일로서 수득하였다.
단계 5: rac-5-(4-클로로페닐)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진의 제조
아르곤 하에, N'-[2-(4-클로로페닐)-2-옥소-에톡시]-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (69.2 mg, 0.13 mmol)을 MeOH (0.94 mL) 및 아세트산 (0.21 mL) 중에 용해시키고, 60℃로 가열하였다. 1시간 후, 소듐 시아노보로히드라이드 (9.3 mg, 0.15 mmol)를 첨가하고, 반응물을 추가로 2시간 동안 교반하였다. 실온으로 냉각시킨 후, 혼합물을 1M NaOH 용액에 붓고, 에틸 아세테이트 (2 x 20 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 정제용 HPLC에 의해 정제하고, 용매를 증발시킨 후, rac-5-(4-클로로페닐)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 29 mg (100% 순도, 47% 수율)을 고체로서 수득하였다.
실시예 4의 제조: rac-5-(1-메틸인돌-3-일)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.011)의 제조
단계 1: N'-알릴옥시-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (화합물 13-01)의 제조
아르곤 하에, O-알릴히드록실아민 히드로클로라이드 (658 mg, 5.4 mmol)를 실온에서 MeOH 중 6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르보니트릴 (500 mg, 1.79 mol) 및 NaHCO3 (752.1 mg, 8.95 mmol)의 교반 용액에 첨가하였다. 생성된 혼합물을 60℃에서 36시간 동안 교반하고, 실온으로 냉각시키고, 진공 하에 농축시켰다. 생성된 혼합물을 디클로로메탄 (3 x 200 mL)으로 추출하였다. 유기 추출물을 염수로 세척하고, 황산나트륨 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 PE/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, N'-알릴옥시-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 400 mg (98% 순도, 63% 수율)을 갈색 오일로서 수득하였다.
단계 2: rac-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진-5-올 (화합물 14-01)의 제조
50 mL 둥근 바닥 플라스크에서 OsO4 (902 mg, 0.14 mmol, 물 중 4% wt) 및 NaIO4 (759 mg, 3.55 mmol)를 THF (20 mL) 및 물 (5 mL) 중 N'-알릴옥시-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (500 mg, 1.42 mmol)의 용액에 실온에서 첨가하였다. 반응 혼합물을 실온에서 2시간 동안 교반한 다음, 포화 염화암모늄 용액으로 희석하고, 에틸 아세테이트 (2 x 100 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, rac-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진-5-올 260 mg (100% 순도, 51% 수율)을 백색 고체로서 수득하였다.
단계 3: rac-5-(1-메틸인돌-3-일)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진의 제조
50 mL 둥근 바닥 플라스크에서, 1-메틸인돌 (37 mg, 0.28 mmol)을 포름산 (2 mL) 중 rac-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진-5-올 (50 mg, 0.14 mmol)의 용액에 첨가하였다. 반응 혼합물을 50℃에서 45분 동안 교반한 다음, 실온으로 냉각시키고, 추가로 3시간 동안 교반하였다. 용매를 감압 하에 제거하였다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, rac-5-(1-메틸인돌-3-일)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 59 mg (100% 순도, 89% 수율)을 분홍색 고체로서 수득하였다.
실시예 5의 제조: rac-5-[(4-브로모-2-클로로-페닐)메틸]-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.016)의 제조
단계 1: 메틸 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스이미데이트 (화합물 25-02)의 제조
아르곤 하에, 소듐 메탄올레이트 (32 mg, 0.59 mmol)를 0℃에서 MeOH (1.5 mL) 중 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르보니트릴 (160 mg, 0.33 mmol)의 용액에 첨가하였다. 반응 혼합물을 0℃에서 30분 동안 교반하였다. 용액은 53%의 메틸 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스이미데이트를 함유하였고, 후속 단계에 추가 정제 없이 사용하였다.
단계 2: rac-5-[(4-브로모-2-클로로-페닐)메틸]-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진의 제조
상기 용액에 MeOH/아세트산 (1 mL, 1:1) 중에 용해시킨 O-[rac-2-아미노-3-(4-브로모-2-클로로-페닐)프로필]히드록실아민 (157 mg, 0.51 mmol)을 첨가하였다. 반응 혼합물을 실온에서 3시간 동안 교반한 다음, 100℃에서 7시간 동안 가열하였다. 실온으로 냉각시킨 후, 혼합물을 포화 중탄산나트륨 용액에 붓고, 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 염수로 세척하고, 황산나트륨 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 정제용 HPLC에 의해 정제하고, 용매를 증발시킨 후, rac-5-[(4-브로모-2-클로로-페닐)메틸]-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 5 mg (93% 순도, 2% 수율)을 오일로서 수득하였다.
실시예 6의 제조: rac-3-[6-클로로-3-(2-플루오로-3-메톡시-페녹시)피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.005)의 제조
단계 1: 3,6-디클로로-N-[rac-1-[(2,4-디메틸페닐)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]피리다진-4-카르복스아미드 (화합물 6-01)의 제조
아르곤 하에, DMF (25 mL) 중 3,6-디클로로피리다진-4-카르복실산 (700 mg, 3.62 mmol) 및 HATU (1.52 g, 3.99 mmol)의 용액에 0℃에서 2-[rac-2-아미노-3-(2,4-디메틸페닐)프로폭시]이소인돌린-1,3-디온;2,2,2-트리플루오로아세트산 (1.75 g, 4.0 mmol) 및 N,N-디이소프로필에틸아민 (1.89 mL, 10.88 mmol)을 연속적으로 첨가하였다. 0℃에서 15분 후, 반응 혼합물을 실온에서 18시간 동안 교반하였다. 이어서, 이를 물로 희석하고, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, 3,6-디클로로-N-[rac-1-[(2,4-디메틸페닐)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]피리다진-4-카르복스아미드 1.15 g (87% 순도, 55% 수율)을 백색 고체로서 수득하였다.
단계 2: 3,6-디클로로-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페닐)에틸]피리다진-4-카르복스아미드 (화합물 6-02)의 제조
아르곤 하에, 히드라진 1수화물 (0.42 mL, 6.91 mmol)을 DCM/MeOH (15 mL, 1:1) 중 3,6-디클로로-N-[rac-1-[(2,4-디메틸페닐)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]피리다진-4-카르복스아미드 (1.15 g, 2.3 mmol)의 용액에 첨가하였다. 반응 혼합물을 실온에서 3시간 동안 교반하고, 농축시켰다. 이어서, 이를 물로 희석하고, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 3,6-디클로로-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페닐)에틸]피리다진-4-카르복스아미드 900 mg (74% 순도, 78% 수율)을 황색 고체로서 수득하였다.
단계 3: rac-3-(3,6-디클로로피리다진-4-일)-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 7-01)의 제조
아르곤 하에, POCl3 (0.56 mL, 6.0 mmol)를 80℃에서 AcCN (15 mL) 중 3,6-디클로로-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페닐)에틸]피리다진-4-카르복스아미드 (738 mg, 2.0 mmol)의 용액에 첨가하였다. 반응 혼합물을 80℃에서 18시간 동안 교반하였다. 실온으로 냉각시킨 후, 혼합물을 포화 중탄산나트륨 용액에 부는 다음, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 정제용 HPLC에 의해 정제하고, 용매를 증발시킨 후, rac-3-(3,6-디클로로피리다진-4-일)-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 90 mg (92% 순도, 17% 수율)을 황색 고체로서 수득하였다.
단계 4: rac-3-[6-클로로-3-(2-플루오로-3-메톡시-페녹시)피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진의 제조
AcCN (1 mL) 중 rac-3-(3,6-디클로로피리다진-4-일)-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (60 mg, 0.17 mmol)의 용액에 2-플루오로-3-메톡시-페놀 (27 mg, 0.19 mmol) 및 탄산칼륨 (47 mg, 0.34 mmol)을 첨가하였다. 반응 혼합물을 50℃에서 5시간 동안 교반한 다음, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, rac-3-[6-클로로-3-(2-플루오로-3-메톡시-페녹시)피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 74 mg (97% 순도, 90% 수율)을 황색 오일로서 수득하였다.
실시예 7의 제조: 1-[5-[rac-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진-3-일]-6-[3-(트리플루오로메틸)페녹시]피리다진-3-일]에타논 (화합물 I.042)의 제조
단계 1: rac-5-[(2,4-디메틸페닐)메틸]-3-[6-(1-에톡시비닐)-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.009)의 제조
마이크로웨이브 바이알에서, rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (500 mg, 1.05 mmol), 트리부틸(1-에톡시비닐)스탄난 (473 mg, 1.31 mmol) 및 비스(트리페닐포스핀)팔라듐 디클로라이드 (73 mg, 0.103 mmol)를 아르곤 하에 DMF (0.5 mL) 중에 용해시켰다. 튜브를 밀봉하고, 반응 혼합물을 마이크로웨이브에서 120℃에서 20분 동안 가열하였다. 반응 혼합물을 물로 희석하고, 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 물 및 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, rac-5-[(2,4-디메틸페닐)메틸]-3-[6-(1-에톡시비닐)-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 435 mg (100% 순도, 80% 수율)을 오일로서 수득하였다.
단계 2: 1-[5-[rac-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진-3-일]-6-[3-(트리플루오로메틸)페녹시]피리다진-3-일]에타논의 제조
THF (1 mL) 중 rac-5-[(2,4-디메틸페닐)메틸]-3-[6-(1-에톡시비닐)-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 (100 mg, 0.19 mmol)의 용액에 실온에서 2M 수성 HCl 용액 (0.15 mL, 0.30 mmol)을 첨가하였다. 반응물을 30분 동안 교반한 다음, 물로 희석하고, 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 물 및 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하여 용매를 증발시킨 후, 1-[5-[rac-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진-3-일]-6-[3-(트리플루오로메틸)페녹시]피리다진-3-일]에타논 35 mg (100% 순도, 37% 수율)을 오일로서 수득하였다.
실시예 8의 제조: 3-클로로-N-시클로프로필-5-[rac-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진-3-일]-6-[3-(트리플루오로메틸)페녹시]피리다진-4-아민 (화합물 I.041)의 제조
단계 1: rac-3-[6-클로로-5-아이오도-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.065)의 제조
아르곤 하에, TMPZnCl.LiCl의 용액 (2.77 mmol, 5.1 mL, THF 중 17%, CAS 번호 109-99-9)을 THF (60 mL) 중 rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (600 mg, 1.26 mmol)에 첨가하였다. 실온에서 1시간 동안 교반한 후, NIS (566 mg, 2.52 mmol)를 조금씩 첨가하였다. 반응 혼합물을 실온에서 2시간 동안 교반한 다음, 이를 포화 티오황산나트륨 용액 및 포화 중탄산나트륨 용액으로 희석하고, 에틸 아세테이트 (2 x 250 mL)로 추출하였다. 유기 추출물을 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 정제용 HPLC에 의해 정제하고, 용매를 증발시킨 후, rac-3-[6-클로로-5-아이오도-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 178 mg (70% 순도, 16% 수율)을 황색 고체로서 수득하였다.
단계 2: 3-클로로-N-시클로프로필-5-[rac-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진-3-일]-6-[3-(트리플루오로메틸)페녹시]피리다진-4-아민의 제조
아르곤 하에, 시클로프로필아민 (6 mg, 0.10 mmol) 및 N,N-디이소프로필에틸아민 (0.017 mL, 0.10 mmol)을 AcCN (0.7 mL) 중 rac-3-[6-클로로-5-아이오도-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (50 mg, 0.08 mmol)의 용액에 실온에서 첨가하였다. 반응 혼합물을 50℃에서 18시간 동안 교반한 다음, 이것을 물로 희석하고, 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 3-클로로-N-시클로프로필-5-[rac-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진-3-일]-6-[3-(트리플루오로메틸)페녹시]피리다진-4-아민 42 mg (98% 순도, 93% 수율)을 오일로서 수득하였다.
실시예 9의 제조: 6-클로로-4-[rac-5-[(2,4-디클로로페닐)메틸]-4,5-디히드로-1H-이미다졸-2-일]-3-[3-(트리플루오로메틸)페녹시]피리다진 (화합물 I.007)의 제조
POCl3 (1.05 mL, 11.3 mmol)의 용액을 실온에서 1,4-디옥산 (10 mL) 중 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복실산 (400 mg, 1.25 mmol) 및 3-(2,4-디클로로페닐)프로판-1,2-디아민 (550 mg, 2.51 mmol)의 혼합물에 첨가하였다. 반응물을 환류 하에 가열하고, 36시간 동안 교반하였다. 냉각시킨 후, 반응 혼합물을 0℃에서 포화 중탄산나트륨 용액에 부는 다음, 에틸 아세테이트 (2 x 100 mL)로 추출하였다. 유기 추출물을 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 정제용 HPLC에 의해 정제하고, 용매를 증발시킨 후, 6-클로로-4-[rac-5-[(2,4-디클로로페닐)메틸]-4,5-디히드로-1H-이미다졸-2-일]-3-[3-(트리플루오로메틸)페녹시]피리다진 90 mg (98% 순도, 14% 수율)을 황색 오일로서 수득하였다.
실시예 10의 제조: (5S)-5-벤질-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I-070)의 제조
단계 1: 6-클로로-N-메톡시-N-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (화합물 1.03)의 제조
디클로로메탄 (75 mL) 중 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복실산 (5.0 g, 16.7 mmol)의 현탁액에 옥살릴 클로라이드 (3.19 g, 25.14 mmol)를 첨가한 다음, 이어서 2 방울의 DMF를 첨가하였다. 반응 혼합물을 실온에서 1시간 동안 교반하였다. 미리 형성된 아실 클로라이드에 N-메톡시메탄아민;히드로클로라이드 (2.12 g, 21.79 mmol) 및 트리에틸아민 (8.17 mL, 58.68 mmol)을 첨가하였다. 반응 혼합물을 실온에서 2시간 동안 교반한 다음, 이것을 물로 희석하고, 디클로로메탄 (2 x 200 mL)으로 추출하였다. 유기 추출물을 물 및 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 디클로로메탄으로 희석하고, 실리카 겔 상에서 여과하였다. 용매를 증발시켜 6-클로로-N-메톡시-N-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 3.38 g (95% 순도, 56% 수율)을 오일로서 수득하였다.
단계 2: 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르브알데히드 (화합물 16-01)의 제조
아르곤 하에, DIBAL-H의 용액 (0.88 mL, 0.88 mmol, 헥산 중 1M)을 THF (1.8 mL) 중 6-클로로-N-메톡시-N-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (100 mg, 0.29 mmol)의 용액에 -50℃에서 첨가하였다. -30℃에서 4시간 후, 반응을 포화 염화암모늄 용액의 첨가에 의해 정지시킨 다음, 혼합물을 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르브알데히드 43.6 mg (90% 순도, 47% 수율)을 오일로서 수득하였다.
단계 3: 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르브알데히드 옥심 (화합물 17-01)의 제조
아르곤 하에, 히드록실아민;히드로클로라이드 (156 mg, 2.24 mmol) 및 아세트산칼륨 (415 mg, 4.23 mmol)을 EtOH (40 mL) 중 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르브알데히드 (400 mg, 1.32 mmol)에 첨가하였다. 반응 혼합물을 환류 하에 2시간 동안 교반하고, 물 중에 희석하고, 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르브알데히드 옥심 215 mg (90% 순도, 47% 수율)을 고체로서 수득하였다.
단계 4: (5S)-5-벤질-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진의 제조
AcCN (0.2 mL) 중 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르브알데히드 옥심 (10 mg, 0.031 mmol)의 용액에 실온에서 NCS (5.4 mg, 0.04 mmol)를 첨가하였다. 반응 혼합물을 1시간 동안 교반한 다음, AcCN/물 (0.3 mL, 2:1) 중 (2S)-1-브로모-3-페닐-프로판-2-아민;2,2,2-트리플루오로아세트산 (15.4 mg, 0.047 mmol)의 용액을 첨가하였다. 반응물을 실온에서 5시간 동안 교반한 다음, 1,2-비스(디메틸아미노)에탄 (18.3 mg, 0.16 mmol)을 반응 혼합물에 첨가하였다. 30분 후, 탄산나트륨의 용액 (34 mg, 0.31 mmol, 물 중 1M)을 첨가하고, 반응물을 실온에서 1시간 동안 추가로 교반하였다. 반응 혼합물을 물 및 디클로로메탄으로 희석하고, 수성 상을 디클로로메탄 (2 x 50 mL)으로 추출하였다. 유기 층을 황산나트륨 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 정제용 HPLC에 의해 정제하여, 용매를 증발시킨 후, (5S)-5-벤질-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 10.9 mg (85% 순도, 65% 수율)을 황색 고체로서 수득하였다.
실시예 11의 제조: rac-3-[6-클로로-5-(2-메톡시에톡시)-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.072)의 제조
아르곤 하에, 2-메톡시에탄올 (0.15 mL, 0.30 mmol) 및 수소화나트륨 (11 mg, 0.27 mmol)을 AcCN (2 mL) 중 rac-3-[6-클로로-5-아이오도-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (150 mg, 0.25 mmol)의 용액에 실온에서 첨가하였다. 반응 혼합물을 실온에서 1시간 동안 교반한 다음, 이것을 물로 희석하고, 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, rac-3-[6-클로로-5-(2-메톡시에톡시)-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 30 mg (90% 순도, 19% 수율)을 무색 오일로서 수득하였다.
실시예 12의 제조: rac-3-[6-클로로-5-(4-피리딜)-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.088)의 제조
아르곤 하에, TMPZnCl·LiCl의 용액 (0.22 mmol, 0.40 mL, THF 중 17%, CAS 번호 109-99-9)을 THF (3 mL) 중 rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (50 mg, 0.10 mmol)에 첨가하고, 이어서 4-브로모피리딘 (20 mg, 0.12 mmol), Pd(dba)2 (18 mg, 0.031 mmol) 및 트리푸릴포스핀 (15 μ, 0.063 mmol)을 첨가하였다. 반응 혼합물을 60℃에서 4시간 동안 교반한 다음, 포화 염화암모늄 용액 및 포화 중탄산나트륨 용액으로 희석하고, 에틸 아세테이트 (2 x 100 mL)로 추출하였다. 유기 추출물을 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 정제용 HPLC에 의해 정제하고, 용매를 증발시킨 후, rac-3-[6-클로로-5-(4-피리딜)-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 32 mg (86% 순도, 47% 수율)을 오일로서 수득하였다.
실시예 13의 제조: rac-5-[(2,4-디메틸페닐)메틸]-3-[6-(2-메톡시에틸술파닐)-5-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.187)의 제조
아르곤 하에, 2-메톡시에탄티올 (20mg, 0.22 mmol) 및 수소화나트륨 (8 mg, 0.22 mmol)을 0℃에서 THF (2 mL) 중 rac-3-[6-클로로-5-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (100 mg, 0.20 mmol)의 용액에 첨가하였다. 반응 혼합물을 0℃에서 2시간 동안 교반한 다음, 이것을 물로 희석하고, 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, rac-5-[(2,4-디메틸페닐)메틸]-3-[6-(2-메톡시에틸술파닐)-5-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 21 mg (96% 순도, 18% 수율)을 무색 오일로서 수득하였다.
실시예 14의 제조: rac-2-[6-클로로-3-(3-시클로프로필페녹시)피리다진-4-일]-6-[(2,4-디메틸페닐)메틸]-5,6-디히드로-1H-피리미딘-4-온 (화합물 I.078)의 제조
단계 1: 메틸 6-클로로-3-(3-시클로프로필페녹시)피리다진-4-카르복스이미데이트 (화합물 25-01)의 제조
아르곤 하에, 소듐 메탄올레이트 (43 mg, 0.81 mmol)를 0℃에서 MeOH (2 mL) 중 6-클로로-3-(3-시클로프로필페녹시)피리다진-4-카르보니트릴 (200 mg, 0.74 mmol)의 용액에 첨가하였다. 반응 혼합물을 0℃에서 30분 동안 교반하였다. 조 용액은 48%의 메틸 6-클로로-3-(3-시클로프로필페녹시)피리다진-4-카르복스이미데이트를 함유하였고, 이를 후속 단계에 추가 정제 없이 사용하였다.
단계 2: rac-2-[6-클로로-3-(3-시클로프로필페녹시)피리다진-4-일]-6-[(2,4-디메틸페닐)메틸]-5,6-디히드로-1H-피리미딘-4-온의 제조
이전 용액에 MeOH (0.5 mL) 및 아세트산 (17 μL) 중에 용해시킨 rac-3-아미노-4-(2,4-디메틸페닐)부탄아미드 (93 mg, 0.45 mmol)를 첨가하였다. 반응 혼합물을 실온에서 15분 동안 교반한 다음, 60℃에서 18시간 동안 가열하였다. 실온으로 냉각시킨 후, 혼합물을 포화 중탄산나트륨 용액에 붓고, 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 염수로 세척하고, 황산나트륨 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 정제용 HPLC에 의해 정제하고, 용매를 증발시킨 후, rac-2-[6-클로로-3-(3-시클로프로필페녹시)피리다진-4-일]-6-[(2,4-디메틸페닐)메틸]-5,6-디히드로-1H-피리미딘-4-온 40.7 mg (100% 순도, 29% 수율)을 오일로서 수득하였다.
실시예 15의 제조: rac-5-[(2,4-디메틸페녹시)메틸]-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.144)의 제조
단계 1: tert-부틸 rac-4-[(2,4-디메틸페녹시)메틸]-2,2-디메틸-옥사졸리딘-3-카르복실레이트의 제조
아르곤 하에, 디이소프로필 아조디카르복실레이트 (1.92 g, 9.51 mmol)를 2-메틸테트라히드로푸란 (30 mL) 중 tert-부틸 rac-4-(히드록시메틸)-2,2-디메틸-옥사졸리딘-3-카르복실레이트 (2.0 g, 8.64 mmol), 2,4-디메틸페놀 (1.16 g, 9.51 mmol) 및 트리페닐포스핀 (2.49 g, 9.51 mmol)의 용액에 첨가하였다. 반응 혼합물을 80℃에서 3시간 동안 가열하고, 실온으로 냉각시키고, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 층을 1M 수성 NaOH 용액 및 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, tert-부틸 rac-4-[(2,4-디메틸페녹시)메틸]-2,2-디메틸-옥사졸리딘-3-카르복실레이트 1.82 g (95% 순도, 59% 수율)을 무색 오일로서 수득하였다.
단계 2: rac-2-아미노-3-(2,4-디메틸페녹시)프로판-1-올의 제조
tert-부틸 rac-4-[(2,4-디메틸페녹시)메틸]-2,2-디메틸-옥사졸리딘-3-카르복실레이트 (1.8 g, 5.37 mmol)의 용액을 MeOH (25 mL) 및 수성 1M HCl 용액 (15 mL) 중에 용해시켰다. 반응 혼합물을 50℃에서 2시간 동안 교반하였다. 실온으로 냉각시킨 후, 용매를 증발시키고, 잔류물을 포화 중탄산나트륨 용액에 붓고, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 rac-2-아미노-3-(2,4-디메틸페녹시)프로판-1-올 833 mg (87% 순도, 69% 수율)을 황색 오일로서 수득하였다.
단계 3: tert-부틸 N-[rac-1-[(2,4-디메틸페녹시)메틸]-2-히드록시-에틸]카르바메이트의 제조
디-tert-부틸 디카르보네이트 (1.02 mL, 4.46 mmol) 및 N,N-디이소프로필에틸아민 (1.55 mL, 8.93 mmol)을 2-메틸테트라히드로푸란 (5.5 mL) 중 rac-2-아미노-3-(2,4-디메틸페녹시)프로판-1-올 (830 mg, 4.25 mmol)의 용액에 연속적으로 첨가하였다. 반응 혼합물을 실온에서 1시간 30분 동안 교반한 다음, 이것을 염수로 희석하고, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, tert-부틸 N-[rac-1-[(2,4-디메틸페녹시)메틸]-2-히드록시-에틸]카르바메이트 909 mg (97% 순도, 70% 수율)을 무색 오일로서 수득하였다.
단계 4: tert-부틸 N-[rac-1-[(2,4-디메틸페녹시)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]카르바메이트 (화합물 2-13)의 제조
아르곤 하에, 디이소프로필 아조디카르복실레이트 (684 mg, 3.38 mmol)를 2-메틸테트라히드로푸란 (10 mL) 중 tert-부틸 N-[rac-1-[(2,4-디메틸페녹시)메틸]-2-히드록시-에틸]카르바메이트 (909 mg, 3.0 mmol), N-히드록시프탈이미드 (552.2 mg, 3.38 mmol) 및 트리페닐포스핀 (888 mg, 3.38 mmol)의 용액에 첨가하였다. 반응 혼합물을 실온에서 2시간 동안 교반한 다음, 에틸아세테이트 (2 x 200 mL)로 추출하였다. 유기 층을 1M 수성 NaOH 용액 및 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, tert-부틸 N-[rac-1-[(2,4-디메틸페녹시)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]카르바메이트 1.16 g (92% 순도, 79% 수율)을 무색 오일로서 수득하였다.
단계 5: 2-[rac-2-아미노-3-(2,4-디메틸페녹시)프로폭시]이소인돌린-1,3-디온 2,2,2-트리플루오로아세테이트 (화합물 2-12)의 제조
1,2-디클로로에탄 (15 mL) 중 tert-부틸 N-[rac-1-[(2,4-디메틸페녹시)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]카르바메이트 (1.16 g, 2.63 mmol)의 용액에 트리플루오로아세트산 (1.014 mL, 13.17 mmol)을 첨가하였다. 반응 혼합물을 실온에서 4시간 동안 교반하였다. 용매를 증발시켜 2-[rac-2-아미노-3-(2,4-디메틸페녹시)프로폭시]이소인돌린-1,3-디온;2,2,2-트리플루오로아세트산 1.4g (79% 순도, 93% 수율)을 황색 오일로서 수득하였다.
단계 6: 6-메틸-N-[rac-1-[(2,4-디메틸페녹시)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (화합물 3-33)의 제조
아르곤 하에, DMF (10 mL) 중 6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복실산 (405 mg, 1.36 mmol) 및 HATU (542 mg, 1.42 mmol)의 용액에 2-[rac-2-아미노-3-(2,4-디메틸페녹시)프로폭시]이소인돌린-1,3-디온;2,2,2-트리플루오로아세트산 (647 mg, 1.42 mmol) 및 N,N-디이소프로필에틸아민 (0.71 mL, 4.07 mmol)을 연속적으로 첨가하였다. 반응 혼합물을 실온에서 1시간 동안 교반하였다. 이어서, 이를 물로 희석하고, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, 6-메틸-N-[rac-1-[(2,4-디메틸페녹시)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 550 mg (93% 순도, 60% 수율)을 무색 오일로서 수득하였다.
단계 7: 6-메틸-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페녹시)에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (화합물 4-33)의 제조
아르곤 하에, 히드라진 1수화물 (0.16 mL, 2.66 mmol)을 DCM/MeOH (16 mL, 1:1) 중 6-메틸-N-[rac-1-[(2,4-디메틸페녹시)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (550 mg, 0.89 mmol)의 용액에 첨가하였다. 반응 혼합물을 실온에서 2시간 동안 교반한 다음, 농축시켰다. 잔류물을 물로 희석하고, 디클로로메탄 (2 x 200 mL)으로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 6-메틸-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페녹시)에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 490 mg (75% 순도, 84% 수율)을 백색 오일로서 수득하였다.
단계 8: rac-5-[(2,4-디메틸페녹시)메틸]-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진의 제조
아르곤 하에, POCl3 (0.22 mL, 2.39 mmol)를 80℃에서 AcCN (10 mL) 중 6-메틸-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페녹시)에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (490 mg, 0.80 mmol)의 용액에 첨가하였다. 반응 혼합물을 80℃에서 4시간 동안 교반하였다. 실온으로 냉각시킨 후, 혼합물을 포화 중탄산나트륨 용액에 부는 다음, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, rac-5-[(2,4-디메틸페녹시)메틸]-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진 89 mg (95% 순도, 22% 수율)을 갈색 오일로서 수득하였다.
실시예 16의 제조: rac-5-(1-메틸인돌-5-일)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-4,5,6,7-테트라히드로-1,2,4-옥사디아제핀 (화합물 I.062)의 제조
단계 1: 실시예 4의 단계 1과 유사하게 N'-알릴옥시-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘의 제조.
단계 2: 6-메틸-N'-[3-(1-메틸인돌-5-일)알릴옥시]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (화합물 30-01)의 제조
아르곤 하에, AcCN (5 mL) 중 N'-알릴옥시-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (500 mg, 1.42 mmol), 5-브로모-1-메틸-인돌 (596 mg, 2.83 mmol), 트리에틸아민 (0.40 mL, 2.84 mmol), 아세트산팔라듐(II) (32 mg, 0.14 mmol) 및 트리-2톨릴포스핀 (86 mg, 0.28 mmol)의 혼합물을 환류 하에 18시간 동안 교반하였다. 실온으로 냉각시킨 후, 반응 혼합물을 포화 염화암모늄 용액으로 희석하고, 에틸 아세테이트 (3 x 30 mL)로 추출하였다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, 6-메틸-N'-[3-(1-메틸인돌-5-일)알릴옥시]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 203 mg (93% 순도, 27% 수율)을 오일로서 수득하였다.
단계 3: rac-5-(1-메틸인돌-5-일)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-4,5,6,7-테트라히드로-1,2,4-옥사디아제핀의 제조
디클로로메탄 (5 mL) 중 아이오딘 (13.2 mg, 0.052 mmol) 및 페닐실란 (11.2 mg, 0.104 mmol)의 용액을 실온에서 30분 동안 교반한 다음, 6-메틸-N'-[3-(1-메틸인돌-5-일)알릴옥시]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (25.0 mg, 0.052 mmol)을 첨가하였다. 반응 혼합물을 1시간 동안 교반한 다음, 포화 티오황산나트륨 용액으로 희석하고, 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 정제용 HPLC에 의해 정제하고, 용매를 증발시킨 후, rac-5-(1-메틸인돌-5-일)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-4,5,6,7-테트라히드로-1,2,4-옥사디아제핀 8 mg (88% 순도, 28% 수율)을 오일로서 수득하였다.
실시예 17의 제조: rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-1,4,5,6-테트라히드로-1,2,4-트리아진 (화합물 I.173)의 제조
단계 1: 6-클로로-N-[1-(클로로메틸)-2-(2,4-디메틸페닐)에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드의 제조
실시예 2의 단계 1을 참조한다.
단계 2: rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-1,4,5,6-테트라히드로-1,2,4-트리아진의 제조
톨루엔 (6 mL) 중 6-클로로-N-[1-(클로로메틸)-2-(2,4-디메틸페닐)에틸]-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미드 (339 mg, 0.68 mmol)의 용액에 오염화인 (425 mg, 2.04 mmol)을 첨가하였다. 반응 혼합물을 75℃에서 1시간 30분 동안 교반한 다음, 감압 하에 농축시켰다. 잔류물을 AcCN (4 mL) 중에 용해시키고, 히드라진 수화물 (170.27 mg, 3.40 mmol)의 용액을 실온에서 반응 혼합물에 첨가하였다. 실온에서 1시간 동안 교반한 후, 반응 혼합물을 물로 희석하고, 에틸 아세테이트 (2 x 100 mL)로 추출하였다. 유기 추출물을 물 및 염수로 세척하고, 황산나트륨 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, rac-3-[6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-1,4,5,6-테트라히드로-1,2,4-트리아진 197 mg (100% 순도, 60% 수율)을 수득하였다.
실시예 18의 제조: 6-클로로-4-[rac-6-[(2,4-디메틸페닐)메틸]-1,4,5,6-테트라히드로피리미딘-2-일]-3-[3-(트리플루오로메틸)페녹시]피리다진 (화합물 I.117)의 제조
단계 1: tert-부틸 N-[rac-1-[(2,4-디메틸페닐)메틸]-3-히드록시-프로필]카르바메이트의 제조
디-tert-부틸 디카르보네이트 (2.13 g, 9.79 mmol) 및 트리메틸아민 (2.73 mL, 19.6 mmol)을 테트라히드로푸란 (10 mL) 중 rac-3-아미노-4-(2,4-디메틸페닐)부탄-1-올 히드로클로라이드 (1.5 g, 6.52 mmol)의 현탁액에 0℃에서 연속적으로 첨가하였다. 반응 혼합물을 실온에서 18시간 동안 교반한 다음, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, tert-부틸 N-[rac-1-[(2,4-디메틸페닐)메틸]-3-히드록시-프로필]카르바메이트 1.8 g (97% 순도, 91% 수율)을 백색 고체로서 수득하였다.
단계 2: tert-부틸 N-[rac-1-[(2,4-디메틸페닐)메틸]-3-(1,3-디옥소이소인돌린-2-일)프로필]카르바메이트의 제조
아르곤 하에, 디에틸 아조디카르복실레이트 (6.87 g, 15.3 mmol)를 0℃에서 테트라히드로푸란 (200 mL) 중 tert-부틸 N-[rac-1-[(2,4-디메틸페닐)메틸]-3-히드록시-프로필]카르바메이트 (1.8 g, 6.13 mmol), 프탈이미드 (5.41 g, 36.8 mmol) 및 트리페닐포스핀 (9.65 g, 36.8 mmol)의 용액에 첨가하였다. 반응 혼합물을 실온에서 24시간 동안 교반하고, 물로 희석하고, 에틸아세테이트 (3 x 200 mL)로 추출하였다. 유기 층을 염수로 세척하고, 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, tert-부틸 N-[rac-1-[(2,4-디메틸페닐)메틸]-3-(1,3-디옥소이소인돌린-2-일)프로필]카르바메이트 2.0 g (84% 순도, 60% 수율)을 무색 오일로서 수득하였다.
단계 3: 2-[rac-3-아미노-4-(2,4-디메틸페닐)부틸]이소인돌린-1,3-디온;2,2,2-트리플루오로아세테이트의 제조
디클로로메탄 (20 mL) 중 tert-부틸 N-[rac-1-[(2,4-디메틸페닐)메틸]-3-(1,3-디옥소이소인돌린-2-일)프로필]카르바메이트 (1.2 g, 2.84 mmol)의 용액에 트리플루오로아세트산 (0.65 mL, 8.52 mmol)을 첨가하였다. 반응 혼합물을 실온에서 3일 동안 교반하였다. 용매를 증발시켜 2-[rac-3-아미노-4-(2,4-디메틸페닐)부틸]이소인돌린-1,3-디온;2,2,2-트리플루오로아세트산 1.2g (54% 순도, 52% 수율)을 고체로서 수득하였다.
단계 4: rac-4-(2,4-디메틸페닐)부탄-1,3-디아민의 제조
아르곤 하에, 히드라진 1수화물 (3.73 mL, 41.24 mmol)을 EtOH (5 mL) 중 2-[rac-3-아미노-4-(2,4-디메틸페닐)부틸]이소인돌린-1,3-디온;2,2,2-트리플루오로아세트산 (1.2 g, 2.75 mmol)의 용액에 첨가하였다. 반응 혼합물을 실온에서 3일 동안 교반한 다음, 농축시켰다. 이어서, 이를 물로 희석하고, 디클로로메탄 (2 x 200 mL)으로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 MTBE 중에서 교반하고, 형성된 백색 고체를 여과하였다. 여과물을 농축시켜 rac-4-(2,4-디메틸페닐)부탄-1,3-디아민 520 mg (95% 순도, 93% 수율)을 백색 고체로서 수득하였다.
단계 5: 메틸 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스이미데이트의 제조
6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르보니트릴 (100 mg, 0.33 mmol)로부터 출발하여 실시예 5의 단계 1을 참조한다.
단계 6: 6-클로로-4-[rac-6-[(2,4-디메틸페닐)메틸]-1,4,5,6-테트라히드로피리미딘-2-일]-3-[3-(트리플루오로메틸)페녹시]피리다진의 제조
메틸 6-클로로-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스이미데이트의 이전 용액에 MeOH (0.5 mL) 및 아세트산 (9 μL) 중에 용해시킨 rac-4-(2,4-디메틸페닐)부탄-1,3-디아민 (124 mg, 0.45 mmol)을 0℃에서 첨가하였다. 반응 혼합물을 실온에서 5시간 동안 교반한 다음, 혼합물을 포화 중탄산나트륨 용액에 붓고, 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 염수로 세척하고, 황산나트륨 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, 6-클로로-4-[rac-6-[(2,4-디메틸페닐)메틸]-1,4,5,6-테트라히드로피리미딘-2-일]-3-[3-(트리플루오로메틸)페녹시]피리다진 26 mg (90% 순도, 16% 수율)을 황색 오일로서 수득하였다.
실시예 19의 제조: rac-6,6-디플루오로-5-(4-메톡시페닐)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-4,5-디히드로-1,2,4-옥사디아진 (화합물 I.154)의 제조
단계 1: N'-히드록시-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (화합물 10-02)의 제조
실시예 3의 단계 3을 참조한다.
단계 2: N'-[1,1-디플루오로-2-(4-메톡시페닐)-2-옥소-에톡시]-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (화합물 12-14)의 제조
아르곤 하에, 2-tert-부틸이미노-N,N-디에틸-1,3-디메틸-1,3,2람다5-디아자포스피난-2-아민 (BEMP) (105 mg, 0.38 mmol)을 AcCN (1.5 mL) 중 N'-히드록시-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (100 mg, 0.32 mmol)의 용액에 실온에서 첨가하였다. 15분 후, 2-브로모-2,2-디플루오로-1-(4-메톡시페닐)에타논 (127 mg, 0.48 mmol)을 첨가하고, 반응물을 추가로 15분 동안 교반하였다. 반응 혼합물을 포화 염화암모늄 용액으로 희석하고, 에틸 아세테이트 (2 x 50 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 N'-[1,1-디플루오로-2-(4-메톡시페닐)-2-옥소-에톡시]-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 222 mg (27% 순도, 80% 수율)을 오일로서 수득하였다.
단계 3: rac-6,6-디플루오로-5-(4-메톡시페닐)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-4,5-디히드로-1,2,4-옥사디아진의 제조
아르곤 하에, N'-[1,1-디플루오로-2-(4-메톡시페닐)-2-옥소-에톡시]-6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-카르복스아미딘 (222 mg, 0.25 mmol)을 tert-부탄올 (6.4 mL) 및 아세트산 (1.6 mL) 중에 용해시키고, 80℃로 가열하였다. 30분 후, 소듐 시아노보로히드라이드 (21 mg, 0.34 mmol)를 첨가하고, 반응물을 추가로 2시간 동안 교반하였다. 실온으로 냉각시킨 후, 혼합물을 1M 수성 NaOH 용액에 붓고, 에틸 아세테이트 (2 x 20 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 정제용 HPLC에 의해 정제하고, 용매를 증발시킨 후, rac-6,6-디플루오로-5-(4-메톡시페닐)-3-[6-메틸-3-[3-(트리플루오로메틸)페녹시]피리다진-4-일]-4,5-디히드로-1,2,4-옥사디아진 4 mg (96% 순도, 3% 수율)을 황색 고체로서 수득하였다.
실시예 20의 제조: rac-3-[6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 (화합물 I.058)의 제조
단계 1: 이소프로필 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-피리다진-4-카르복실레이트 (화합물 1-24)의 제조
디메틸 술폭시드 (2.5 mL) 중 이소프로필 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)피리다진-4-카르복실레이트 (800 mg, 2.28 mmol)의 용액에 니트로메탄 (0.62 mL, 11.40 mmol)을 첨가하였다. 반응물을 실온에서 30분 동안 교반한 다음, 트리에틸아민 (0.48 mL, 3.42 mmol)을 첨가하였다. 반응물을 실온에서 24시간 동안 교반한 다음, 이를 물로 희석하고, 에틸 아세테이트 (2 x 100 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 이소프로필 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-피리다진-4-카르복실레이트 917 mg (76% 순도, 84% 수율)을 오렌지색 오일로서 수득하였다.
단계 2: 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-피리다진-4-카르복실산 (화합물 1-02)의 제조
테트라히드로푸란 (4 mL) 중 이소프로필 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-피리다진-4-카르복실레이트 (927 mg, 2.5 mmol)의 용액에 수산화리튬의 2M 수용액 (182 mg, 7.62 mmol)을 첨가하였다. 반응물을 실온에서 4일 동안 교반한 다음, 이것을 물로 희석하였다. 수성 상을 1M 수성 HCl 용액을 사용하여 산성화시키고, 에틸 아세테이트 (3 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-피리다진-4-카르복실산 617 mg (81% 순도, 60% 수율)을 고체로서 수득하였다.
단계 3: 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-N-[rac-1-[(2,4-디메틸페닐)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]피리다진-4-카르복스아미드의 제조
아르곤 하에, DMF (10 mL) 중 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-피리다진-4-카르복실산 (500 mg, 1.55 mmol) 및 HATU (648 mg, 1.70 mmol)의 용액에 0℃에서 2-[rac-2-아미노-3-(2,4-디메틸페닐)프로폭시]이소인돌린-1,3-디온 2,2,2-트리플루오로아세테이트 (747 mg, 1.70 mmol) 및 N,N-디이소프로필에틸아민 (0.80 mL, 4.64 mmol)을 연속적으로 첨가하였다. 0℃에서 15분 후, 반응 혼합물을 실온에서 18시간 동안 교반하였다. 이어서, 이를 물로 희석하고, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하여, 용매를 증발시킨 후, 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-N-[rac-1-[(2,4-디메틸페닐)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]피리다진-4-카르복스아미드 639.5 g (100% 순도, 65% 수율)을 고체로서 수득하였다.
단계 4: 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페닐)에틸]피리다진-4-카르복스아미드의 제조
아르곤 하에, 히드라진 1수화물 (0.18 mL, 3.0 mmol)을 DCM/MeOH (12 mL, 1:1) 중 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-N-[rac-1-[(2,4-디메틸페닐)메틸]-2-(1,3-디옥소이소인돌린-2-일)옥시-에틸]피리다진-4-카르복스아미드 (639 mg, 1.0 mmol)의 용액에 첨가하였다. 반응 혼합물을 실온에서 18시간 동안 교반하고, 농축시켰다. 이어서, 이를 물로 희석하고, 디클로로메탄 (2 x 200 mL)으로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 용매를 증발시켜 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페닐)에틸]피리다진-4-카르복스아미드 453 mg (100% 순도, 89% 수율)을 백색 오일로서 수득하였다.
단계 5: rac-3-[6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진의 제조
아르곤 하에, POCl3 (0.25 mL, 2.72 mmol)를 80℃에서 AcCN (5 mL) 중 6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-N-[rac-1-(아미노옥시메틸)-2-(2,4-디메틸페닐)에틸]피리다진-4-카르복스아미드 (453 mg, 0.90 mmol)의 용액에 첨가하였다. 반응 혼합물을 80℃에서 18시간 동안 교반하였다. 실온으로 냉각시킨 후, 혼합물을 포화 중탄산나트륨 용액에 부는 다음, 에틸 아세테이트 (2 x 200 mL)로 추출하였다. 유기 추출물을 황산마그네슘 상에서 건조시키고, 여과하고, 감압 하에 농축시켰다. 잔류물을 실리카 겔 상에서 칼럼 크로마토그래피 (구배 헵탄/EtOAc)에 의해 정제하고, 용매를 증발시킨 후, rac-3-[6-클로로-3-(3-시클로프로필-2-플루오로-페녹시)-5-메틸-피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진 196 mg (100% 순도, 44% 수율)을 황색 고체로서 수득하였다.
하기 표 1에 제시된 바와 같은 화합물을 상기 제공된 실시예와 유사하게 또는 본원에 기재된 방법에 따라 제조하였다. 이들 화합물의 1H-NMR 데이터는 표 2에 제시된다.
표 1. 화학식 (I)에 따른 화합물
표 1에서, "#"는 L-R6 기에 대한 부착 지점을 나타내고, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
(*) 실시예 I-051 및 I-053은 실시예 I-059의 2종의 거울상이성질체임
실시예 I-051: 광회전: +92.7˚ (c=0.95, DCM, 25℃); 농도 c는 g/100 mL로 표현된다.
실시예 I-053: 광회전: -86.6˚ (c=1,04, DCM, 25℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex I-119 및 I-130은 Ex I-052의 2종의 거울상이성질체임
실시예 I-119: 광회전: +95.3˚ (c=1.05, CDCl3, 20℃); 농도 c는 g/100 mL로 표현된다.
실시예 I-130: 광회전: -93.3˚ (c=1.20, CDCl3, 20℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex I-145 및 I-146은 Ex I-055의 2종의 거울상이성질체임
실시예 I-145: 광회전: +86.3˚ (c=1.62, CDCl3, 20℃); 농도 c는 g/100 mL로 표현된다.
실시예 I-146: 광회전: -90˚ (c=1.60, CDCl3, 20℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex I-151 및 I-152는 Ex I-025의 2종의 거울상이성질체임
실시예 I-151: 광회전: +54.8˚ (c=1,1, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
실시예 I-152: 광회전: -51.4˚ (c=1,09, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex I-160 및 I-161은 Ex I-013의 2종의 거울상이성질체임
실시예 I-160: 광회전: +85.6˚ (c=2.15, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
실시예 I-161: 광회전: -78.1˚ (c=2.15, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex I-162 및 I-163은 Ex I-016의 2종의 거울상이성질체임
실시예 I-162: 광회전: +52.2˚ (c=1.15, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
실시예 I-163: 광회전: -72˚ (c=1.0, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
(*) 실시예 I-164 및 I-165는 실시예 I-017의 2종의 거울상이성질체임
실시예 I-164: 광회전: +78.3˚ (c=1.15, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
실시예 I-165: 광회전: -85.5˚ (c=1.1, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
(*) 실시예 I-166 및 I-167은 실시예 I-011의 2종의 거울상이성질체임
실시예 I-166: 광회전: 0˚ (c=0.95, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
실시예 I-167: 광회전: -7.3˚ (c=1.1, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex I-245 및 I-250은 Ex I-030의 2종의 거울상이성질체임
실시예 I-245: 광회전: +57.1˚ (c=0.67, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
Ex I-250: 광회전: -63.8˚ (c=0.69, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex I-246 및 I-247은 Ex I-027의 2종의 거울상이성질체임
Ex I-246: 광회전: +60˚ (c=0.6, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
Ex I-247: 광회전: -55˚ (c=0.8, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex I-312 및 I-313은 Ex I-239의 2종의 거울상이성질체임
실시예 I-312: 광회전: -88.6˚ (c=3.50, DCM, 20℃); 농도 c는 g/100 mL로 표현된다.
실시예 I-313: 광회전: +73.2˚ (c=2.95, DCM, 20℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex I-322 및 I-323은 Ex I-056의 2종의 거울상이성질체임
(*) Ex I-336 및 I-337은 Ex I-300의 2종의 거울상이성질체임
실시예 I-336: 광회전: +71.6˚ (c=1.01, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
실시예 I-337: 광회전: -72.5˚ (c=1.02, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex I-338 및 I-339는 Ex I-302의 2종의 거울상이성질체임
실시예 I-338: 광회전: +71.5˚ (c=1.04, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
실시예 I-339: 광회전: -75.2˚ (c=1.01, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex I-070은 단일 입체이성질체임
실시예 I-070: 광회전: -78.1˚ (c=2.51, CDCl3, 25℃); 농도 c는 g/100 mL로 표현된다.
표 2:
하기 표 3, 5, 7, 9, 11, 13, 15, 17, 19, 21, 23, 25, 27, 29, 31, 33, 35, 37, 39, 41 및 43에 제시된 바와 같은 화합물을 상기 제공된 실시예와 유사하게 또는 본원에 기재된 방법에 따라 제조하였다. 이들 화합물의 1H-NMR 데이터를 각각 표 4, 6, 8, 10, 12, 14, 16, 18, 20, 22, 24, 26, 28, 30, 32, 34, 36, 38 40, 42 및 44에 나타냈다.
표 3: 화학식 (1)에 따른 화합물
표 4:
표 5: 화학식 (2)에 따른 화합물
표 5에서, "#"는 L-R6 기에 대한 부착 지점을 나타낸다.
표 6:
표 7: 화학식 (3)에 따른 화합물
표 7에서, "#"는 L-R6 기에 대한 부착 지점을 나타내고, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
표 8:
표 9: 화학식 (4)에 따른 화합물
표 9에서, "#"는 L-R6 기에 대한 부착 지점을 나타내고, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
표 10:
표 11: 화학식 (6)에 따른 화합물
표 11에서, "#"는 L-R6 기에 대한 부착 지점을 나타내고, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
표 12:
표 13: 화학식 (7)에 따른 화합물
표 13에서, "#"는 L-R6 기에 대한 부착 지점을 나타내고, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
(*) Ex 7-07 및 7-08은 Ex 7-05의 2종의 거울상이성질체임
실시예 7-07: 광회전: +61.9˚ (c=2.23, CDCl3, 20℃); 농도 c는 g/100 mL로 표현된다.
실시예 7-08: 광회전: -59.6˚ (c=2.45, CDCl3, 20℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex 7-09 및 7-10은 Ex 7-06의 2종의 거울상이성질체임
실시예 7-09: 광회전: + 62.4˚ (c=2.28, CDCl3, 20℃); 농도 c는 g/100 mL로 표현된다.
실시예 7-10: 광회전: - 59.6˚ (c=2.35, CDCl3, 20℃); 농도 c는 g/100 mL로 표현된다.
(*) 실시예 7-11 및 7-12는 실시예 7-01의 2종의 거울상이성질체임
실시예 7-11: 광회전: - 90.1˚ (c=2.18, CDCl3, 20℃); 농도 c는 g/100 mL로 표현된다.
실시예 7-12: 광회전: + 93.2˚ (c=1.83, CDCl3, 20℃); 농도 c는 g/100 mL로 표현된다.
(*) Ex 7-03은 단일 입체이성질체이고; Ex 7-04는 라세미체이다.
표 14:
표 43: 화학식 (8)에 따른 화합물
표 44:
표 15: 화학식 (9)에 따른 화합물
표 16:
표 17: 화학식 (10)에 따른 화합물
표 18:
표 19: 화학식 (12)에 따른 화합물
표 19에서, "#"는 L-R6 기에 대한 부착 지점을 나타내고, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
표 20:
표 21: 화학식 (13)에 따른 화합물
표 21에서, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
표 22:
표 23: 화학식 (14)에 따른 화합물
표 23에서, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
표 24:
표 25: 화학식 (16)에 따른 화합물
표 26:
표 27: 화학식 (17)에 따른 화합물
표 28:
표 31: 화학식 (19)에 따른 화합물
표 31에서, "#"는 L-R6 기에 대한 부착 지점을 나타낸다.
표 32:
표 29: 화학식 (20)에 따른 화합물
표 29에서, "#"는 L-R6 기에 대한 부착 지점을 나타내고, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
표 30:
표 33: 화학식 (21)에 따른 화합물
표 33에서, "#"는 L-R6 기에 대한 부착 지점을 나타내고, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
표 34:
표 35: 화학식 (22)에 따른 화합물
표 35에서, "#"는 L-R6 기에 대한 부착 지점을 나타내고, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
표 35:
표 37: 화학식 (23)에 따른 화합물
표 37에서, "#"는 L-R6 기에 대한 부착 지점을 나타내고, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
표 38:
표 39: 화학식 (25)에 따른 화합물
표 40:
표 41: 화학식 (30)에 따른 화합물
표 41에서, "#"는 R6 기에 대한 부착 지점을 나타내고, "*"는 피리다진-4-일 기에 대한 부착 지점을 나타낸다.
표 42:
생물학적 데이터
본 발명에 따른 활성 화합물 조합물의 고도의 살진균 활성은 하기 실시예로부터 명백하다. 개별 활성 화합물은 살진균 활성과 관련하여 약점을 나타내지만, 조합물은 활성의 단순 상가성을 초과하는 활성을 갖는다.
활성 화합물 조합물의 살진균 활성이 개별적으로 적용되는 경우의 활성 화합물의 총 활성을 초과하는 경우에, 살진균제의 상승작용적 효과가 항상 존재한다. 2종의 활성 화합물의 주어진 조합에 대해 예상되는 활성은 하기와 같이 계산될 수 있다 (문헌 [Colby, S.R., "Calculating Synergistic and Antagonistic Responses of Herbicide Combinations", Weeds 1967, 15, 20-22] 참조):
X가 활성 화합물 A를 m ppm (또는 g/ha)의 적용률로 적용하는 경우의 효능이고,
Y가 활성 화합물 B를 n ppm (또는 g/ha)의 적용률로 적용하는 경우의 효능이고,
E가 활성 화합물 A 및 B를 각각 m 및 n ppm (또는 g/ha)의 적용률로 적용하는 경우의 효능인 경우에,
%로 표현된 효능의 정도는 하기를 나타낸다: 0%는 대조군의 효능에 상응하는 효능을 의미하는 반면, 100%의 효능은 질병이 관찰되지 않음을 의미한다.
실제 살진균 활성이 계산치를 초과하는 경우, 조합물의 활성은 초-상가적이며, 즉 상승작용적 효과가 존재한다. 이 경우에, 실제로 관찰된 효능은 상기 언급된 식으로부터 계산된 기대 효능 (E)에 대한 값보다 더 커야 한다.
상승작용적 효과를 입증하는 추가의 방식은 타메스(Tammes)의 방법이다 (문헌 ["Isoboles, a graphic representation of synergism in pesticides" in Neth. J. Plant Path., 1964, 70, 73-80] 참조).
본 발명은 하기 실시예에 의해 예시된다. 그러나, 본 발명은 실시예에 제한되지 않는다.
실시예: 진균 미생물을 사용한 시험관내-시험
방법 A
96-웰 마이크로타이터 플레이트의 웰에 메탄올 + 유화제 알킬아릴-폴리글리콜-에테르 중 시험 화합물 또는 화합물 조합물의 제제 10μl을 채운다. 그 후, 용매를 후드에서 증발시킨다. 다음 단계에서, 100μl의 액체 감자 덱스트로스 배지를 시험 진균의 적절한 농도의 포자 또는 균사체 현탁액으로 조정된 각각의 웰 내로 제공한다.
광도계의 도움으로, 모든 웰에서의 흡광도를 620nm의 파장에서 결정한다.
마이크로타이터 플레이트를 20℃ 및 85% 상대 습도에서 인큐베이션한다. 적용 3-5일 후에 성장 억제를 다시 광도계로 측정한다. 효능은 비처리 대조군과 비교하여 계산하고, 0% 효능은 비처리 대조군만큼 높은 진균 성장을 의미하는 반면, 100% 효능은 진균 성장이 측정되지 않았음을 의미한다.
방법 B
96-웰 마이크로타이터 플레이트의 웰에 메탄올 + 유화제 알킬아릴-폴리글리콜-에테르 중 시험 화합물 또는 화합물 조합물의 제제 30μl를 채운다. 그 후, 용매를 후드에서 증발시킨다. 다음 단계에서, 시험 진균의 적절한 농도의 포자 또는 균사체 현탁액으로 조정된 200μl의 액체 성장 배지를 제공한다.
광도계의 도움으로, 모든 웰에서의 흡광도를 600nm의 파장에서 측정한다.
마이크로타이터 플레이트를 20℃ 및 85% 상대 습도에서 3 내지 7일 동안 인큐베이션한다. 인큐베이션 후에 성장의 억제를 광도계로 결정한다. 효능은 비처리 대조군과 비교하여 계산하고, 0% 효능은 비처리 대조군만큼 높은 진균 성장을 의미하는 반면, 100% 효능은 진균 성장이 측정되지 않았음을 의미한다.
표 A1 내지 A12, B1 내지 B14, C1 내지 C10, D1 내지 D8, E1 내지 E8, F1 내지 F11, G1 내지 G4, H1 내지 H4 및 I1 내지 I5의 데이터를 방법 A에 따라 수집하였다. 표 A13 내지 A22, B15 내지 B18, C11 내지 C20, E9 내지 E16, F12 내지 F15, G5 내지 G15, H5 내지 H8, I6 내지 I11 및 J1 내지 J11의 데이터를 방법 B에 따라 수집하였다.
표 A1: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A2: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A3: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A4: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A5: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A6: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A7: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A8: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A9: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A10: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A11: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A12: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A13: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A14: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A15: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A16: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A17: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A18: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A19: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A20: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A21: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 A22: 시험관내 - 알테르나리아 알테르나타를 사용한 시험
표 B1: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B2: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B3: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B4: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B5: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B6: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B7: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B8: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B9: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B10: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B11: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B12: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B13: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B14: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B15: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B16: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B17: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 B18: 시험관내 - 보트리티스 시네레아를 사용한 시험
표 C1: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C2: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C3: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C4: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C5: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C6: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C7: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C8: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C9: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C10: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C11: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C12: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C13: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C14: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C15: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C16: 시험관내 - 세르코스포라 베티콜라에 의한 시험
표 C17: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C18: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C19: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 C20: 시험관내 - 세르코스포라 베티콜라를 사용한 시험
표 D1: 시험관내 - 콜레토트리쿰 린데무티아눔을 사용한 시험
표 D2: 시험관내 - 콜레토트리쿰 린데무티아눔을 사용한 시험
표 D3: 시험관내 - 콜레토트리쿰 린데무티아눔을 사용한 시험
표 D4: 시험관내 - 콜레토트리쿰 린데무티아눔을 사용한 시험
표 D5: 시험관내 - 콜레토트리쿰 린데무티아눔을 사용한 시험
표 D6: 시험관내 - 콜레토트리쿰 린데무티아눔을 사용한 시험
표 D7: 시험관내 - 콜레토트리쿰 린데무티아눔을 사용한 시험
표 D8: 시험관내 - 콜레토트리쿰 린데무티아눔을 사용한 시험
표 E1: 시험관내 - 코르다나 무사에를 사용한 시험
표 E2: 시험관내 - 코르다나 무사에를 사용한 시험
표 E3: 시험관내 - 코르다나 무사에를 사용한 시험
표 E4: 시험관내 - 코르다나 무사에를 사용한 시험
표 E5: 시험관내 - 코르다나 무사에를 사용한 시험
표 E6: 시험관내 - 코르다나 무사에를 사용한 시험
표 E7: 시험관내 - 코르다나 무사에를 사용한 시험
표 E8: 시험관내 - 코르다나 무사에를 사용한 시험
표 E9: 시험관내 - 코르다나 무사에를 사용한 시험
표 E10: 시험관내 - 코르다나 무사에를 사용한 시험
표 E11: 시험관내 - 코르다나 무사에를 사용한 시험
표 E12: 시험관내 - 코르다나 무사에를 사용한 시험
표 E13: 시험관내 - 코르다나 무사에를 사용한 시험
표 E14: 시험관내 - 코르다나 무사에를 사용한 시험
표 E15: 시험관내 - 코르다나 무사에를 사용한 시험
표 E16: 시험관내 - 코르다나 무사에를 사용한 시험
표 F2: 시험관내 - 디아포르트 시트리를 사용한 시험
표 F3: 시험관내 - 디아포르트 시트리를 사용한 시험
표 F4: 시험관내 - 디아포르트 시트리를 사용한 시험
표 F5: 시험관내 - 디아포르트 시트리를 사용한 시험
표 F5: 시험관내 - 디아포르트 시트리를 사용한 시험
표 F6: 시험관내 - 디아포르트 시트리를 사용한 시험
표 F7: 시험관내 - 디아포르트 시트리를 사용한 시험
표 F8: 시험관내 - 디아포르트 시트리를 사용한 시험
표 F9: 시험관내 - 디아포르트 시트리를 사용한 시험
표 F10: 시험관내 - 디아포르테 시트리를 사용한 시험
표 F11: 시험관내 - 디아포르테 시트리를 사용한 시험
표 F12: 시험관내 - 디아포르테시트리를 사용한 시험
표 F13: 시험관내 - 디아포르테 시트리를 사용한 시험
표 F14: 시험관내 - 디아포르테 시트리를 사용한 시험
표 F15: 시험관내 - 디아포르테 시트리를 사용한 시험
표 G1: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G2: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G3: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G4: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G5: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G6: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G7: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G8: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G9: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G10: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G11: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G12: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G13: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G14: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 G15: 시험관내 - 푸사리움 쿨모룸을 사용한 시험
표 H1: 시험관내 - 파라스타고노스포라 노도룸을 사용한 시험
표 H2: 시험관내 - 파라스타고노스포라 노도룸을 사용한 시험
표 H3: 시험관내 - 파라스타고노스포라 노도룸을 사용한 시험
표 H4: 시험관내 - 파라스타고노스포라 노도룸을 사용한 시험
표 H5: 시험관내 - 파라스타고노스포라 노도룸을 사용한 시험
표 H6: 시험관내 - 파라스타고노스포라 노도룸을 사용한 시험
표 H7: 시험관내 - 파라스타고노스포라 노도룸을 사용한 시험
표 H8: 시험관내 - 파라스타고노스포라 노도룸을 사용한 시험
표 I1: 시험관내 - 우스틸라고 세게툼 변종 아베나에를 사용한 시험
표 I2: 시험관내 - 우스틸라고 세게툼 변종 아베나에를 사용한 시험
표 I3: 시험관내 - 우스틸라고 세게툼 변종 아베나에를 사용한 시험
표 I4: 시험관내 - 우스틸라고 세게툼 변종 아베나에를 사용한 시험
표 I5: 시험관내 - 우스틸라고 세게툼 변종 아베나에를 사용한 시험
표 I6: 시험관내 - 우스틸라고 세게툼 변종 아베나에를 사용한 시험
표 I7: 시험관내 - 우스틸라고 세게툼 변종 아베나에를 사용한 시험
표 I8: 시험관내 - 우스틸라고 세게툼 변종 아베나에를 사용한 시험
표 I9: 시험관내 - 우스틸라고 세게툼 변종 아베나에를 사용한 시험
표 I10: 시험관내 - 우스틸라고 세게툼 변종 아베나에를 사용한 시험
표 I11: 시험관내 - 우스틸라고 세게툼 변종 아베나에를 사용한 시험
표 J1: 시험관내 - 콜레토트리쿰 코코데스를 사용한 시험
표 J2: 시험관내 - 콜레토트리쿰 코코데스를 사용한 시험
표 J3: 시험관내 - 콜레토트리쿰 코코데스를 사용한 시험
표 J4: 시험관내 - 콜레토트리쿰 코코데스를 사용한 시험
표 J5: 시험관내 - 콜레토트리쿰 코코데스를 사용한 시험
표 J6: 시험관내 - 콜레토트리쿰 코코데스를 사용한 시험
표 J7: 시험관내 - 콜레토트리쿰 코코데스를 사용한 시험
표 J8: 시험관내 - 콜레토트리쿰 코코데스를 사용한 시험
표 J9: 시험관내 - 콜레토트리쿰 코코데스를 사용한 시험
표 J10: 시험관내 - 콜레토트리쿰 코코데스를 사용한 시험
표 J11: 시험관내 - 콜레토트리쿰 코코데스를 사용한 시험
Claims (14)
- 하기를 포함하는 활성 화합물 조합물:
(A) 화학식 (I)의 적어도 1종의 화합물
여기서
A는 O, S, C(=O), S(=O), S(=O)2, NR1 및 CR1R2로 이루어진 군으로부터 선택되고, 여기서 R1 및 R2는 독립적으로 수소, C1-C6-알킬 및 C3-C8-시클로알킬로 이루어진 군으로부터 선택되거나, 또는 R1 및 R2는 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬 또는 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 형성하고;
m은 0, 1 또는 2이고;
T는 수소, 히드록실, C1-C6-알킬, -C(=O)Ra1, -C(=O)(ORa1), -C(=O)N(Ra2)2, -S(=O)Ra1, -S(=O)2Ra1 및 S(=O)2N(Ra2)2로 이루어진 군으로부터 선택되고,
여기서 Ra1은 C1-C6-알킬, C1-C6-할로알킬, C3-C8-시클로알킬 및 C2-C6-알케닐로 이루어진 군으로부터 선택되고,
여기서 Ra2는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬, C3-C8-시클로알킬 및 C2-C6-알케닐로 이루어진 군으로부터 선택되고;
R3 및 R4는 독립적으로 수소, 할로겐, 시아노, 히드록실, 포르밀, 카르복실, C1-C6-알킬, C1-C6-알콕시, C1-C6-알킬카르보닐, C1-C6-알콕시카르보닐, C2-C6-알케닐, C2-C6-알키닐, C3-C8-시클로알킬, 방향족 C6-C14-카르보사이클, 방향족 5- 내지 14-원 헤테로사이클, 비-방향족 3- 내지 14-원 헤테로사이클 및 -O-Si(C1-C6-알킬)3으로 이루어진 군으로부터 선택되거나, 또는 R3 및 R4는 이들이 부착되어 있는 탄소 원자와 함께, 카르보닐, 메틸리덴, C3-C8-시클로알킬 또는 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 형성하고;
R5는 수소, 히드록실, C1-C6-알킬, C1-C6-알콕시, C1-C6-알킬카르보닐옥시, C1-C6-알킬술파닐, C1-C6-알킬술피닐, C1-C6-알킬술포닐, C3-C8-시클로알킬 및 -O-Si(C1-C6-알킬)3으로 이루어진 군으로부터 선택되고;
여기서 지방족 R1, R2, R3, R4 및 R5 치환기는 할로겐, 시아노, 아미노, 니트로, 히드록실, 포르밀, 카르복실, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -O-Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 치환기로 치환될 수 있고;
여기서 시클릭 R1, R2, R3, R4 및 R5 치환기는 할로겐, 시아노, 니트로, 히드록실, 포르밀, 옥소, 메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -O-Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 치환기로 치환될 수 있고;
R3 또는 R4, 및 R5는 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬을 형성할 수 있고;
L은 직접 결합을 나타내거나, 또는 L은 카르보닐, C1-C6-알킬렌, 동일한 탄소 원자 상에서 치환기가 부착되어 있는 탄소 원자와 함께 C3-C8-시클로알킬을 형성하는 2개의 치환기에 의해 치환된 C1-C6-알킬렌, 동일한 탄소 원자 상에서 치환기가 부착되어 있는 탄소 원자와 함께 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 형성하는 2개의 치환기에 의해 치환된 C1-C6-알킬렌, C2-C6-알케닐렌, C2-C6-알키닐렌, C3-C8-시클로알킬렌, C1-C6-알킬렌-C3-C8-시클로알킬렌, C3-C8-시클로알킬렌-C1-C6-알킬렌, C1-C6-알킬렌-C3-C8-시클로알킬렌-C1-C6-알킬렌, C1-C6-알킬렌-(C=O), C(=O)-C1-C6-알킬렌, C3-C8-시클로알케닐렌, C1-C6-알킬렌-C3-C8-시클로알케닐렌, C3-C8-시클로알케닐렌-C1-C6-알킬렌, C1-C6-알킬렌-C3-C8-시클로알케닐렌-C1-C6-알킬렌, 비-방향족 3- 내지 7-원 모노시클릭 헤테로시클릴렌, -NRaL1-, -NRaL1(C=O)-, -C(=O)NRaL1-, -NRaL1S(=O)2-, -S(=O)2NRaL1-, -C(=NORaL2)-, -C(=N-N(RaL2)2) 및 -C(=NRaL2)-로 이루어진 군으로부터 선택되고;
여기서 RaL1은 수소 및 C1-C6-알킬로 이루어진 군으로부터 선택되고,
여기서 RaL2는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬, C3-C8-시클로알킬 및 C2-C6-알킬레닐로 이루어진 군으로부터 선택되고,
여기서 지방족 L 치환기는 동일하거나 상이할 수 있는 1개 이상의 LSa 치환기로 치환될 수 있고,
여기서 L 치환기의 시클릭 또는 시클릭 모이어티는 동일하거나 상이할 수 있는 1개 이상의 LSc 치환기로 치환될 수 있고,
Lsa는 할로겐, 시아노, 히드록실, 카르복실, 메틸리덴, 할로메틸리덴, C1-C6-알콕시, C1-C6-할로알콕시, C3-C8-시클로알킬, C3-C8-할로시클로알킬, C1-C6-알콕시카르보닐, -O-Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
LSc는 할로겐, 시아노, 니트로, 히드록실, 포르밀, 카르복실, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -O-Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고/거나, 2개의 LSc 치환기가 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬을 형성하고;
R6은 비-방향족 C3-C12-카르보사이클, 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클, 방향족 5- 내지 14-원 헤테로사이클, 비-방향족 C3-C12-카르보시클릴옥시, 방향족 C6-C14-카르보시클릴옥시, 방향족 5- 내지 14-원 헤테로시클릴옥시, 비-방향족 5- 내지 14-원 헤테로시클릴옥시, 비-방향족 C3-C12-카르보시클릴술파닐, 방향족 C6-C14-카르보시클릴술파닐, 방향족 5- 내지 14-원 헤테로시클릴술파닐, 비-방향족 5- 내지 14-원 헤테로시클릴술파닐, 비-방향족 C3-C12-카르보시클릴술피닐, 방향족 C6-C14-카르보시클릴술피닐, 방향족 5- 내지 14-원 헤테로시클릴술피닐, 비-방향족 5- 내지 14-원 헤테로시클릴술피닐, 비-방향족 C3-C12-카르보시클릴술포닐, 방향족 C6-C14-카르보시클릴술포닐, 방향족 5- 내지 14-원 헤테로시클릴술포닐, 비-방향족 5- 내지 14-원 헤테로시클릴술포닐, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-알콕시, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-알콕시, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-알콕시, 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-알콕시, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-할로알콕시, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-할로알콕시, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-할로알콕시, 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-할로알콕시, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-술파닐, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-술파닐, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술파닐 및 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술파닐, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-술피닐, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-술피닐, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술피닐 및 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술피닐, 비-방향족 C3-C12-카르보사이클에 의해 치환된 C1-C3-술포닐, 방향족 C6-C14-카르보사이클에 의해 치환된 C1-C3-술포닐, 비-방향족 3- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술포닐 및 방향족 5- 내지 14-원 헤테로사이클에 의해 치환된 C1-C3-술포닐로 이루어진 군으로부터 선택되고;
여기서 R6 치환기의 시클릭 또는 시클릭 모이어티는 동일하거나 상이할 수 있는 1개 이상의 R6S 치환기로 치환될 수 있고,
R6S는 할로겐, 시아노, 이소시아노, 니트로, 히드록실, 메르캅토, 펜타플루오로술파닐, 옥소, 메틸리덴, 할로메틸리덴, 포르밀, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C2-C6-알킬닐옥시, C2-C6-할로알킬닐옥시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C3-C8-시클로알킬술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C3-C8-시클로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, C3-C8-시클로알킬술포닐, C3-C8-시클로알킬, C3-C8-시클로알킬옥시, C3-C8-시클로알케닐, 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, -N(Rc)2, -O-(C=O)Rd, -C(=O)Rd, -C(=O)(ORd), -C(=O)N(Rd)2, -S(=O)2N(Rd)2, -O-Si(C1-C6-알킬)3 및 -Si(C1-C6-알킬)3으로 이루어진 군으로부터 선택되거나, 또는 2개의 R6S 치환기는 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬을 형성할 수 있고,
여기서 Rc는 독립적으로 수소, C1-C6-알킬 및 C3-C8-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 Rd는 독립적으로 수소, C1-C6-알킬 및 C1-C6-할로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 R6S, Rc 및 Rd 치환기는 시아노, 할로겐, 히드록실, C1-C6-알콕시, C1-C6-할로알콕시, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, C3-C8-시클로알킬, C3-C8-할로시클로알킬 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 치환기로 치환될 수 있고,
여기서 R6S의 시클릭 또는 시클릭 모이어티 및 시클릭 Rc 치환기는 할로겐, 시아노, 니트로, 히드록실, 포르밀, 카르복실, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C2-C6-알케닐, C3-C8-시클로알킬 및 C3-C8-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 치환기로 치환될 수 있고/거나, R6S 치환기의 시클릭 또는 시클릭 모이어티는 치환기가 부착되어 있는 탄소 원자와 함께 C3-C8-시클로알킬을 형성하는 2개의 치환기로 치환될 수 있고;
R7은 수소, 할로겐, 시아노, 이소시아노, 히드록실, 메르캅토, 니트로, 아미노, 포르밀, C1-C6-알킬, C1-C6-할로알킬, C1-C6-히드록시알킬, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알킬카르보닐, C1-C6-할로알킬카르보닐, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C2-C6-알키닐옥시, C2-C6-할로알키닐옥시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C3-C8-시클로알킬술파닐, C2-C6-알케닐술파닐, C2-C6-알키닐술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C3-C8-시클로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, C3-C8-시클로알킬술포닐, C3-C8-시클로알킬, C3-C6-시클로알케닐, 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, C3-C8-시클로알킬옥시, 방향족 C6-C14-카르보시클릴옥시, 방향족 5- 또는 6-원 모노시클릭 헤테로시클릴옥시, 비-방향족 3- 내지 7-원 모노시클릭 헤테로시클릴옥시, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, -N(Re)2, -C(=NRf)Rf, NRgC(=O)Rg, -C(=O)(ORg), -C(=O)N(Rg)2, -S(=O)2N(Rg)2 및 -S(=O)(=NRg)Rg으로 이루어진 군으로부터 선택되고,
여기서 Re는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, 방향족 C6-C14-카르보사이클, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 Rf는 독립적으로 히드록실, 아미노, 시아노, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-알킬아미노 및 디(C1-C6-알킬)아미노로 이루어진 군으로부터 선택되고,
여기서 Rg는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬 및 C3-C8-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 R7, Re, Rf 및 Rg 치환기는 동일하거나 상이할 수 있는 1개 이상의 R7Sa 치환기로 치환될 수 있고,
여기서 R7의 시클릭 또는 시클릭 모이어티, 시클릭 Re 및 시클릭 Rg 치환기는 동일하거나 상이할 수 있는 1개 이상의 R7Sc 치환기로 치환될 수 있고,
R7Sa는 시아노, 히드록실, 카르복실, C1-C6-알콕시, C1-C6-할로알콕시, C3-C8-시클로알킬, C3-C8-할로시클로알킬, C1-C6-알콕시카르보닐, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, 방향족 C6-C14-카르보사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
R7Sc는 할로겐, 시아노, 니트로, 히드록실, 포르밀, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬 C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -O-Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되거나, 또는 2개의 R7Sc 치환기는 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬을 형성하고;
R8은 수소, 할로겐, 시아노, 이소시아노, 아미노, 니트로, 히드록실, 메르캅토, 카르복실, C1-C6-알콕시카르보닐, C1-C6-알킬, C1-C6-할로알킬, C1-C6-히드록시알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C2-C6-알키닐옥시, C2-C6-할로알키닐옥시, C3-C8-시클로알킬, C3-C6-시클로알케닐, 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클, 방향족 5- 내지 14-원 헤테로사이클, C3-C8-시클로알킬옥시, 방향족 C6-C14-카르보시클릴옥시, 비-방향족 3- 내지 14-원 헤테로시클릴옥시, 방향족 5- 내지 14-원 헤테로시클릴옥시, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, -N(Rh)2, -SRi, -S(=O)Ri 및 -S(=O)2Ri로 이루어진 군으로부터 선택되고,
여기서 Rh는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, 방향족 C6-C14-카르보사이클, 방향족 5- 내지 14-원 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 Ri는 C1-C6-알킬, C1-C6-할로알킬, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, 방향족 C6-C14-카르보사이클, 방향족 5- 내지 14-원 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 지방족 R8, Rh 및 Ri 치환기는 동일하거나 상이할 수 있는 1개 이상의 R8Sa 치환기로 치환될 수 있고,
여기서 R8의 시클릭 또는 시클릭 모이어티, 시클릭 Rh 및 시클릭 Ri 치환기는 동일하거나 상이할 수 있는 1개 이상의 R8Sc 치환기로 치환될 수 있고,
R8Sa는 시아노, 아미노, 니트로, 히드록실, 포르밀, 카르복실, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시-C1-C6-알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C1-C6-알킬카르보닐, C1-C6-할로알킬카르보닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클 및 -N(Ra')2로 이루어진 군으로부터 선택되고, 여기서 Ra'는 독립적으로 수소, 포르밀, C1-C6-알킬, C1-C6-할로알킬, C3-C8-시클로알킬 및 C1-C6-알킬카르보닐로 이루어진 군으로부터 선택되고, 여기서 상기 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클 R8Sa는 동일하거나 상이할 수 있는 1개 이상의 C1-C6-알킬 치환기로 치환될 수 있고,
R8Sc는 할로겐, 시아노, 아미노, 니트로, 히드록실, 포르밀, 카르복실, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C2-C6-알케닐, C1-C6-알킬술파닐, C1-C6-알킬술피닐, C1-C6-알킬술포닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -O-Si(C1-C6-알킬)3 및 동일하거나 상이할 수 있는 1개 이상의 C1-C6-알킬 치환기로 치환될 수 있는 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되거나, 또는 2개의 R8Sc 치환기는 이들이 부착되어 있는 탄소 원자와 함께, C3-C8-시클로알킬 또는 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 형성하고, 여기서 상기 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클은 동일하거나 상이할 수 있는 1개 이상의 C1-C6-알킬 치환기로 치환될 수 있고;
Q는 방향족 C6-C14-카르보사이클, 비-방향족 C3-C12-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클 및 방향족 5- 내지 14-원 헤테로사이클로 이루어진 군으로부터 선택되고, 여기서 상기 카르보사이클 또는 헤테로사이클 기 중 임의의 것은 동일하거나 상이할 수 있는 1개 이상의 QS 치환기로 치환될 수 있고,
QS는 할로겐, 시아노, 이소시아노, 니트로, 히드록실, 메르캅토, 포르밀, 카르복실, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알킬카르보닐, C1-C6-할로알킬카르보닐, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C2-C6-알케닐옥시, C2-C6-할로알케닐옥시, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C1-C6-알킬술피닐, C1-C6-할로알킬술피닐, C1-C6-알킬술포닐, C1-C6-할로알킬술포닐, C3-C8-시클로알킬, C3-C8-시클로알킬옥시, C3-C6-시클로알케닐, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, 방향족 C6-C14-카르보사이클, 방향족 5- 내지 14-원 헤테로사이클, -O-Si(C1-C6-알킬)3, -Si(C1-C6-알킬)3, -O-C(=O)Rj, -NRjC(=O)Rj, -C(=O)N(Rj)2, -C(=S)Rj, -C(=S)N(Rj)2, -C(=NRj)Rj 및 -C(=NORj)Rj 및 -N(Rk)2로 이루어진 군으로부터 선택되고,
여기서 Rj는 독립적으로 수소, C1-C6-알킬, C1-C6-할로알킬 및 C1-C6-알콕시로 이루어진 군으로부터 선택되고,
여기서 Rk는 독립적으로 수소, 히드록실, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C2-C6-알케닐, C2-C6-할로알케닐 및 C3-C8-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 QS, Rj 및 Rk 치환기는 시아노, 아미노, 니트로, 히드록실, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, -Si(C1-C6-알킬)3 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 치환기로 치환될 수 있고,
여기서 QS의 시클릭 또는 시클릭 모이어티 및 시클릭 Rk 치환기는 할로겐, 시아노, 아미노, 니트로, 히드록실, 포르밀, 카르복실, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C1-C6-알콕시카르보닐, C1-C6-할로알콕시카르보닐, C3-C8-시클로알킬, C3-C8-할로시클로알킬, C2-C6-알케닐 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 독립적으로 선택된 1개 이상의 RQs 치환기로 치환될 수 있고, 여기서 시클릭 RQs 치환기는 치환기가 부착되어 있는 탄소 원자와 함께 C3-C8-시클로알킬을 형성하는 2개의 치환기로 치환될 수 있음,
및
(B) 하기로부터 선택된 적어도 1종의 추가의 활성 화합물
(1) 에르고스테롤 합성의 억제제,
(2) 복합체 I 또는 II에서의 호흡 사슬의 억제제,
(3) 복합체 III에서의 호흡 사슬의 억제제,
(4) 유사분열 및 세포 분열의 억제제,
(5) 다중부위 작용을 가질 수 있는 화합물,
(6) 숙주 방어를 유도할 수 있는 화합물,
(7) 아미노산 및/또는 단백질 생합성의 억제제,
(8) ATP 생산 억제제,
(9) 세포벽 합성의 억제제,
(10) 지질 및 막 합성의 억제제,
(11) 멜라닌 생합성의 억제제,
(12) 핵산 합성의 억제제,
(13) 신호 전달의 억제제,
(14) 탈커플링제로서 작용할 수 있는 화합물,
(15) 다른 살진균제,
(16) 항박테리아제,
(17) 생물학적 살진균제 및
(18) 지방산 또는 그의 유도체. - 제1항에 있어서,
화학식 (I)의 화합물은
A가 O, S, C(=O), S(=O), S(=O)2, NR1 및 CR1R2로 이루어진 군으로부터 선택되고, 여기서 R1 및 R2는 독립적으로 수소, C1-C4-알킬 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
m이 0, 1 또는 2이고;
T가 수소 및 C1-C4-알킬로 이루어진 군으로부터 선택되고,
R3 및 R4가 독립적으로 수소, 플루오린, 염소, C1-C4-알킬, C2-C4-알케닐, C2-C4-알키닐, C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
R5가 수소, 히드록실, C1-C4-알킬, C1-C4-알콕시, C1-C4-알킬술파닐로 이루어진 군으로부터 선택되고,
여기서 지방족 R1, R2, R3, R4 및 R5 치환기는 플루오린, 염소, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬, C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 치환기로 치환될 수 있고,
여기서 시클릭 R1, R2, R3, R4 및 R5 치환기는 플루오린, 염소, 옥소, 메틸리덴, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C3-C6-시클로알킬, C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 치환기로 치환될 수 있고,
R3 또는 R4, 및 R5가 이들이 부착되어 있는 탄소 원자와 함께, C3-C6-시클로알킬을 형성할 수 있고;
L이 직접 결합을 나타내거나, 또는 L은 C1-C6-알킬렌, 동일한 탄소 원자 상에서 치환기가 부착되어 있는 탄소 원자와 함께 C3-C6-시클로알킬을 형성하는 2개의 치환기에 의해 치환된 C1-C6-알킬렌, 동일한 탄소 원자 상에서
치환기가 부착되어 있는 탄소 원자와 함께 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클을 형성하는 2개의 치환기에 의해 치환된 C1-C6-알킬렌으로 이루어진 군으로부터 선택되고,
여기서 지방족 L 치환기는 플루오린, 염소, 히드록실, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬 및 C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 LSa 치환기로 치환될 수 있고,
여기서 L 치환기의 시클릭 또는 시클릭 모이어티는 플루오린, 염소, 히드록실, 옥소, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C3-C6-시클로알킬 및 C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 LSc 치환기로 치환될 수 있고,
R6이 비-방향족 C3-C12-카르보사이클, 방향족 C6-C14-카르보사이클, 비-방향족 3- 내지 14-원 헤테로사이클, 방향족 5- 내지 14-원 헤테로사이클, 비-방향족 C3-C12-카르보시클릴옥시, 방향족 C6-C14-카르보시클릴옥시, 방향족 5- 내지 14-원 헤테로시클릴옥시, 비-방향족 5- 내지 14-원 헤테로시클릴옥시, 비-방향족 C3-C12-카르보시클릴술파닐, 방향족 C6-C14-카르보시클릴술파닐, 방향족 5- 내지 14-원 헤테로시클릴술파닐 및 비-방향족 5- 내지 14-원 헤테로시클릴술파닐로 이루어진 군으로부터 선택되고,
여기서 R6 치환기의 시클릭 또는 시클릭 모이어티는 동일하거나 상이할 수 있는 1 내지 3개의 R6S 치환기로 치환될 수 있고,
R6S가 할로겐, 시아노, 니트로, 히드록실, 메르캅토, 펜타플루오로술파닐, 옥소, 메틸리덴, 할로메틸리덴, C1-C6-알킬, C1-C6-할로알킬, C1-C6-알콕시, C1-C6-할로알콕시, C2-C6-알케닐, C2-C6-할로알케닐, C2-C6-알키닐, C2-C6-할로알키닐, C1-C6-알킬술파닐, C1-C6-할로알킬술파닐, C3-C6-시클로알킬술파닐, C3-C6-시클로알킬, C3-C6-시클로알킬옥시, 페닐, 나프틸 방향족 5- 또는 6-원 모노시클릭 헤테로사이클, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, -C(=O)(ORd) 및 -C(=O)N(Rd)2로 이루어진 군으로부터 선택되고,
여기서 Rd는 독립적으로 수소, C1-C4-알킬 및 C1-C4-할로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 R6S, Rc 및 Rd 치환기는 플루오린, 염소, 히드록실, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬 및 C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 치환기로 치환될 수 있고, 여기서 R6S의 시클릭 또는 시클릭 모이어티 및 시클릭 Rc 치환기는 플루오린, 염소, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시 및 C1-C4-할로알콕시로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 치환기로 치환될 수 있고,
R7이 수소, 할로겐, 시아노, 히드록실, 메르캅토, C1-C4-알킬, C1-C4-할로알킬, C1-C4-히드록시알킬, C1-C4-알콕시, C1-C4-할로알콕시, C1-C4-알킬카르보닐, C1-C4-할로알킬카르보닐, C2-C4-알케닐, C2-C4-할로알케닐, C2-C4-알키닐, C2-C4-할로알키닐, C1-C4-알킬술파닐, C1-C4-할로알킬술파닐, C3-C6-시클로알킬술파닐, C1-C4-알킬술피닐, C1-C4-할로알킬술피닐, C3-C6-시클로알킬술피닐, C1-C4-알킬술포닐, C1-C4-할로알킬술포닐, C3-C6-시클로알킬술포닐, C3-C6-시클로알킬, C3-C6-시클로알케닐, 페닐, 나프틸, 방향족 5- 또는 6-원 모노시클릭 헤테로사이클, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, C3-C8-시클로알킬옥시, 방향족 C6-C14-카르보시클릴옥시, 방향족 5- 또는 6-원 모노시클릭 헤테로시클릴옥시, 비-방향족 3- 내지 7-원 모노시클릭 헤테로시클릴옥시, -N(Re)2, -C(=NRf)Rf, NRgC(=O)Rg, -C(=O)(ORg), -C(=O)N(Rg)2, -S(=O)2N(Rg)2 및 -S(=O)(=NRg)Rg으로 이루어진 군으로부터 선택되고,
여기서 Re는 독립적으로 수소, C1-C4-알킬, C1-C4-할로알킬, C2-C4-알케닐, C2-C4-할로알케닐, C2-C4-알키닐, C2-C4-할로알키닐, C3-C6-시클로알킬, C3-C6-할로시클로알킬로 이루어진 군으로부터 선택되고,
여기서 Rf는 독립적으로 히드록실, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시로 이루어진 군으로부터 선택되고,
여기서 Rg는 독립적으로 수소, C1-C4-알킬, C1-C4-할로알킬 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 R7, Re, Rf 및 Rg 치환기는 동일하거나 상이할 수 있는 1 내지 3개의 R7Sa 치환기로 치환될 수 있고,
여기서 R7의 시클릭 또는 시클릭 모이어티, 시클릭 Re 및 시클릭 Rg 치환기는 동일하거나 상이할 수 있는 1 내지 3개의 R7Sc 치환기로 치환될 수 있고,
R7Sa가 히드록실, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬로 이루어진 군으로부터 선택되고, R7Sc는 플루오린, 염소, 히드록실, 옥소, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
R8이 수소, 할로겐, 아미노, 히드록실, 메르캅토, C1-C4-알킬, C1-C4-할로알킬, C1-C4-히드록시알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C2-C4-할로알케닐, C2-C4-알키닐, C2-C4-할로알키닐, C2-C4-알케닐옥시, C2-C4-할로알케닐옥시, C2-C4-알키닐옥시, C2-C4-할로알키닐옥시, C3-C6-시클로알킬, C3-C6-시클로알케닐, 페닐, 나프틸, 비-방향족 3- 내지 7-원 헤테로사이클, 방향족 5- 또는 6-원 헤테로사이클, C3-C6-시클로알킬옥시, 페닐옥시, 나프틸옥시, 비-방향족 3- 내지 7-원 헤테로시클릴옥시, 방향족 5- 또는 6-원 헤테로시클릴옥시, -N(Rh)2, -SRi , -S(=O)Ri 및 -S(=O)2Ri로 이루어진 군으로부터 선택되고,
여기서 Rh는 독립적으로 수소, C1-C4-알킬, C1-C4-할로알킬, C2-C4-알케닐, C2-C4-할로알케닐, C3-C6-시클로알킬, C3-C6-할로시클로알킬, 페닐, 나프틸 방향족 5- 또는 6-원 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 Ri는 C1-C4-알킬, C1-C4-할로알킬, C2-C4-알케닐, C2-C4-할로알케닐, C2-C4-알키닐, C2-C4-할로알키닐, C3-C6-시클로알킬, C3-C6-할로시클로알킬, 페닐, 나프틸, 방향족 5- 또는 6-원 헤테로사이클 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 지방족 R8, Rh 및 Ri 치환기는 동일하거나 상이할 수 있는 1 내지 3개의 R8Sa 치환기로 치환될 수 있고,
여기서 R8의 시클릭 또는 시클릭 모이어티, 시클릭 Rh 및 시클릭 Ri 치환기는 동일하거나 상이할 수 있는 1 내지 3개의 R8Sc 치환기로 치환될 수 있고,
R8Sa가 히드록실, 카르복실, C1-C4-알콕시, C1-C4-할로알콕시, C1-C4-알콕시카르보닐, C1-C4-할로알콕시카르보닐, C3-C6-시클로알킬, C3-C6-할로시클로알킬, C1-C4-알킬술파닐, C1-C4-할로알킬술파닐, C1-C4-알킬술피닐, C1-C4-할로알킬술피닐, C1-C4-알킬술포닐, C1-C4-할로알킬술포닐, 및 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클로 이루어진 군으로부터 선택되고, 여기서 상기 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클 R8Sa는 동일하거나 상이할 수 있는 1 또는 2개의 C1-C4-알킬 치환기로 치환될 수 있고,
R8Sc가 할로겐, 옥소, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
Q가 페닐, 나프틸, 비-방향족 C5-C10-카르보사이클, 비-방향족 5- 내지 10-원 헤테로사이클 및 방향족 5- 내지 10-원 헤테로사이클로 이루어진 군으로부터 선택되고, 여기서 상기 카르보사이클 또는 헤테로사이클 기 중 임의의 것은 동일하거나 상이할 수 있는 1 내지 3개의 QS 치환기로 치환될 수 있고,
QS가 할로겐, 시아노, 니트로, 포르밀, 카르복실, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알킬카르보닐, C1-C4-할로알킬카르보닐, C1-C4-알콕시, C1-C4-할로알콕시, C1-C4-알콕시카르보닐, C1-C4-할로알콕시카르보닐, C2-C4-알케닐, C2-C4-할로알케닐, C2-C4-알키닐, C2-C4-할로알키닐, C1-C4-알킬술파닐, C1-C4-할로알킬술파닐, C1-C4-알킬술피닐, C1-C4-할로알킬술피닐, C1-C4-알킬술포닐, C1-C4-할로알킬술포닐, C3-C6-시클로알킬, 비-방향족 3- 내지 7-원 모노시클릭 헤테로사이클, 페닐, 나프틸 및 방향족 5- 내지 10-원 헤테로사이클로 이루어진 군으로부터 선택되고,
여기서 지방족 QS, Rj 및 Rk 치환기는 히드록실, C1-C4-알콕시, C1-C4-할로알콕시, C3-C6-시클로알킬 및 C3-C6-할로시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 치환기로 치환될 수 있고, 여기서 QS의 시클릭 또는 시클릭 모이어티 및 시클릭 Rk 치환기는 플루오린, 염소, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시 및 C3-C6-시클로알킬로 이루어진 군으로부터 독립적으로 선택된 1 내지 3개의 RQs 치환기로 치환될 수 있는 것인 화학식 (I)의 화합물인
활성 화합물 조합물. - 제1항 또는 제2항에 있어서,
화학식 (I)의 화합물은
A가 O, NR1 및 CR1R2로 이루어진 군으로부터 선택되고, 여기서 R1 및 R2는 독립적으로 수소, 메틸 또는 에틸로 이루어진 군으로부터 선택되고,
m이 1이고;
T가 수소이고,
R3 및 R4가 독립적으로 수소 또는 플루오린으로 이루어진 군으로부터 선택되고,
R5가 수소이고,
L이 직접 결합을 나타내거나 또는 L이 메틸렌이고,
R6이 인다닐, 1,2,3,4-테트라히드로나프탈레닐, 페닐, 나프틸, 2,3-디히드로벤조푸라닐, 2,3-디히드로-1,4-벤조디옥시닐, 티에닐, 피리디닐, 인돌릴, 벤조푸라닐, 벤조티오페닐 또는 페녹시이고,
여기서 R6 치환기의 시클릭 또는 시클릭 모이어티는 동일하거나 상이할 수 있는 1 또는 2개의 R6S 치환기로 치환될 수 있고,
R6S는 할로겐, 시아노, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C2-C4-알키닐, C1-C4-할로알킬술파닐, C3-C5-시클로알킬, 피리디닐, 옥세타닐 및 테트라히드로푸라닐로 이루어진 군으로부터 선택되고,
R7은 할로겐, 시아노, C1-C4-알킬, C1-C4-할로알킬, C1-C4-히드록시알킬, C1-C4-알콕시, C1-C4-알킬카르보닐, C3-C6-시클로알킬, 이미다졸릴, 피라졸릴, 티아졸릴 및 피리디닐로 이루어진 군으로부터 선택되고,
여기서 지방족 R7 치환기는 히드록실, 메톡시, 에톡시 및 시클로프로필로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 R7Sa 치환기로 치환될 수 있고,
여기서 R7 치환기의 시클릭 또는 시클릭 모이어티는 플루오린, 메틸, 에틸 및 시클로프로필로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 R7Sc 치환기로 치환될 수 있고,
R8은 수소, 할로겐, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C3-C6-시클로알킬옥시 및 -N(Rh)2로 이루어진 군으로부터 선택되고,
여기서 Rh는 독립적으로 수소, C1-C4-알킬, C1-C4-할로알킬, C2-C4-알케닐, 및 C3-C6-시클로알킬로 이루어진 군으로부터 선택되고,
여기서 지방족 R8 및 Rh 치환기는 히드록실, 메톡시 및 에톡시로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 R8Sa 치환기로 치환될 수 있고,
여기서 R8의 시클릭 또는 시클릭 모이어티 및 시클릭 Rh 치환기는 플루오린, 메틸, 에틸 및 시클로프로필로 이루어진 군으로부터 독립적으로 선택된 1 또는 2개의 R8Sc 치환기로 치환될 수 있고,
Q는 페닐, 3-비시클로[4.2.0]옥타-1,3,5-트리에닐, 피라졸릴, 티아졸릴, 티에닐 및 피리디닐로 이루어진 군으로부터 선택되고,
여기서 임의의 상기 카르보사이클 또는 헤테로사이클 기는 동일하거나 상이할 수 있는 1 내지 3개의 QS 치환기로 치환될 수 있고,
QS는 할로겐, 시아노, 니트로, 포르밀, C1-C4-알킬, C1-C4-할로알킬, C1-C4-알콕시, C1-C4-할로알콕시, C2-C4-알케닐, C2-C4-알키닐, C1-C4-알킬술파닐, C3-C5-시클로알킬, 옥시라닐 및 옥세타닐로 이루어진 군으로부터 선택되는 것인 화학식 (I)의 화합물인
활성 화합물 조합물. - 제1항 내지 제3항 중 어느 한 항에 있어서,
화학식 (I)의 화합물은
A가 O이고,
m이 1이고;
T가 수소이고,
R3 및 R4가 수소이고,
R5가 수소이고,
L이 메틸렌이고,
R6이 2,4-디메틸페닐, 2-메틸-4-브로모페닐 또는 2-클로로-4-메틸페닐이고,
R7이 메틸이고,
R8이 수소이고,
Q가 2-플루오로-3-클로로페닐, 2-플루오로-3-브로모페닐 또는 2-플루오로-3-시클로프로필페닐인 화학식 (I)의 화합물인
활성 화합물 조합물. - 제1항 내지 제4항 중 어느 한 항에 있어서, 화학식 (I)의 화합물은 (I-052) rac-3-[3-(3-시클로프로필-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-[(2,4-디메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-130) (5S)-3-[3-(3-시클로프로필-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2,4-디메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진, (I-300) rac-5-[(4-브로모-2-메틸페닐)메틸]-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-302) rac-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-[(2-클로로-4-메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-337) (5S)-5-[(4-브로모-2-메틸페닐)메틸]-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-338) (5R)-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2-클로로-4-메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진 및 (I-339) (5S)-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2-클로로-4-메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진으로 이루어진 군으로부터 선택된 화학식 (I)의 화합물인 활성 화합물 조합물.
- 제1항 내지 제5항 중 어느 한 항에 있어서, 화학식 (I)의 화합물은 (I-302) rac-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-[(2-클로로-4-메틸페닐)메틸]-5,6-디히드로-4H-1,2,4-옥사디아진, (I-338) (5R)-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2-클로로-4-메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진 및 (I-339) (5S)-3-[3-(3-클로로-2-플루오로페녹시)-6-메틸피리다진-4-일]-5-(2-클로로-4-메틸벤질)-5,6-디히드로-4H-1,2,4-옥사디아진으로 이루어진 군으로부터 선택된 화학식 (I)의 화합물인 활성 화합물 조합물.
- 제1항 내지 제6항 중 어느 한 항에 있어서, 추가의 활성 화합물은 하기로 이루어진 군으로부터 선택된 것인 활성 화합물 조합물:
하기로 이루어진 군으로부터 선택된 에르고스테롤 생합성의 억제제: (1.001) 시프로코나졸, (1.002) 디페노코나졸, (1.003) 에폭시코나졸, (1.004) 펜헥사미드, (1.005) 펜프로피딘, (1.006) 펜프로피모르프, (1.007) 펜피라자민, (1.008) 플루퀸코나졸, (1.009) 플루트리아폴, (1.010) 이마잘릴, (1.011) 이마잘릴 술페이트, (1.012) 이프코나졸, (1.013) 메트코나졸, (1.014) 미클로부타닐, (1.015) 파클로부트라졸, (1.016) 프로클로라즈, (1.017) 프로피코나졸, (1.018) 프로티오코나졸, (1.019) 피르이속사졸, (1.020) 스피록사민, (1.021) 테부코나졸, (1.022) 테트라코나졸, (1.023) 트리아디메놀, (1.024) 트리데모르프, (1.025) 트리티코나졸, (1.026) (1R,2S,5S)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.027) (1S,2R,5R)-5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.028) (2R)-2-(1-클로로시클로프로필)-4-[(1R)-2,2-디클로로시클로프로필]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.029) (2R)-2-(1-클로로시클로프로필)-4-[(1S)-2,2-디클로로시클로프로필]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.030) (2R)-2-[4-(4-클로로페녹시)-2-(트리플루오로메틸)페닐]-1-(1H-1,2,4-트리아졸-1-일)프로판-2-올, (1.031) (2S)-2-(1-클로로시클로프로필)-4-[(1R)-2,2-디클로로시클로프로필]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.032) (2S)-2-(1-클로로시클로프로필)-4-[(1S)-2,2-디클로로시클로프로필]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.033) (2S)-2-[4-(4-클로로페녹시)-2-(트리플루오로메틸)페닐]-1-(1H-1,2,4-트리아졸-1-일)프로판-2-올, (1.034) (R)-[3-(4-클로로-2-플루오로페닐)-5-(2,4-디플루오로페닐)-1,2-옥사졸-4-일](피리딘-3-일)메탄올, (1.035) (S)-[3-(4-클로로-2-플루오로페닐)-5-(2,4-디플루오로페닐)-1,2-옥사졸-4-일](피리딘-3-일)메탄올, (1.036) [3-(4-클로로-2-플루오로페닐)-5-(2,4-디플루오로페닐)-1,2-옥사졸-4-일](피리딘-3-일)메탄올, (1.037) 1-({(2R,4S)-2-[2-클로로-4-(4-클로로페녹시)페닐]-4-메틸-1,3-디옥솔란-2-일}메틸)-1H-1,2,4-트리아졸, (1.038) 1-({(2S,4S)-2-[2-클로로-4-(4-클로로페녹시)페닐]-4-메틸-1,3-디옥솔란-2-일}메틸)-1H-1,2,4-트리아졸, (1.039) 1-{[3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸-5-일 티오시아네이트, (1.040) 1-{[rel(2R,3R)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸-5-일 티오시아네이트, (1.041) 1-{[rel(2R,3S)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸-5-일 티오시아네이트, (1.042) 2-[(2R,4R,5R)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.043) 2-[(2R,4R,5S)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.044) 2-[(2R,4S,5R)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.045) 2-[(2R,4S,5S)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.046) 2-[(2S,4R,5R)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.047) 2-[(2S,4R,5S)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.048) 2-[(2S,4S,5R)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.049) 2-[(2S,4S,5S)-1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.050) 2-[1-(2,4-디클로로페닐)-5-히드록시-2,6,6-트리메틸헵탄-4-일]-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.051) 2-[2-클로로-4-(2,4-디클로로페녹시)페닐]-1-(1H-1,2,4-트리아졸-1-일)프로판-2-올, (1.052) 2-[2-클로로-4-(4-클로로페녹시)페닐]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.053) 2-[4-(4-클로로페녹시)-2-(트리플루오로메틸)페닐]-1-(1H-1,2,4-트리아졸-1-일)부탄-2-올, (1.054) 2-[4-(4-클로로페녹시)-2-(트리플루오로메틸)페닐]-1-(1H-1,2,4-트리아졸-1-일)펜탄-2-올, (1.055) 메펜트리플루코나졸, (1.056) 2-{[3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.057) 2-{[rel(2R,3R)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.058) 2-{[rel(2R,3S)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-2,4-디히드로-3H-1,2,4-트리아졸-3-티온, (1.059) 5-(4-클로로벤질)-2-(클로로메틸)-2-메틸-1-(1H-1,2,4-트리아졸-1-일메틸)시클로펜탄올, (1.060) 5-(알릴술파닐)-1-{[3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸, (1.061) 5-(알릴술파닐)-1-{[rel(2R,3R)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸, (1.062) 5-(알릴술파닐)-1-{[rel(2R,3S)-3-(2-클로로페닐)-2-(2,4-디플루오로페닐)옥시란-2-일]메틸}-1H-1,2,4-트리아졸, (1.063) N'-(2,5-디메틸-4-{[3-(1,1,2,2-테트라플루오로에톡시)페닐]술파닐}페닐)-N-에틸-N-메틸이미도포름아미드, (1.064) N'-(2,5-디메틸-4-{[3-(2,2,2-트리플루오로에톡시)페닐]술파닐}페닐)N-에틸-N-메틸이미도포름아미드, (1.065) N'-(2,5-디메틸-4-{[3-(2,2,3,3-테트라플루오로프로폭시)페닐]술파닐}페닐)-N-에틸-N-메틸이미도포름아미드, (1.066) N'-(2,5-디메틸-4-{[3-(펜타플루오로에톡시)페닐]술파닐}페닐)-N-에틸-N-메틸이미도포름아미드, (1.067) N'-(2,5-디메틸-4-{3-[(1,1,2,2-테트라플루오로에틸)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드, (1.068) N'-(2,5-디메틸-4-{3-[(2,2,2-트리플루오로에틸)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드, (1.069) N'-(2,5-디메틸-4-{3-[(2,2,3,3-테트라플루오로프로필)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드, (1.070) N'-(2,5-디메틸-4-{3-[(펜타플루오로에틸)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드, (1.071) N'-(2,5-디메틸-4-페녹시페닐)-N-에틸-N-메틸이미도포름아미드, (1.072) N'-(4-{[3-(디플루오로메톡시)페닐]술파닐}-2,5-디메틸페닐)-N-에틸-N-메틸이미도포름아미드, (1.073) N'-(4-{3-[(디플루오로메틸)술파닐]페녹시}-2,5-디메틸페닐)-N-에틸-N-메틸이미도포름아미드, (1.074) N'-[5-브로모-6-(2,3-디히드로-1H-인덴-2-일옥시)-2-메틸피리딘-3-일]-N-에틸-N-메틸이미도포름아미드, (1.075) N'-{4-[(4,5-디클로로-1,3-티아졸-2-일)옥시]-2,5-디메틸페닐}-N-에틸-N-메틸이미도포름아미드, (1.076) N'-{5-브로모-6-[(1R)-1-(3,5-디플루오로페닐)에톡시]-2-메틸피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.077) N'-{5-브로모-6-[(1S)-1-(3,5-디플루오로페닐)에톡시]-2-메틸피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.078) N'-{5-브로모-6-[(시스-4-이소프로필시클로헥실)옥시]-2-메틸피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.079) N'-{5-브로모-6-[(트랜스-4-이소프로필시클로헥실)옥시]-2-메틸피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.080) N'-{5-브로모-6-[1-(3,5-디플루오로페닐)에톡시]-2-메틸피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.081) 이프펜트리플루코나졸, (1.082) 2-[4-(4-클로로페녹시)-2-(트리플루오로메틸)페닐]-1-(1H-1,2,4-트리아졸-1-일)프로판-2-올, (1.083) 2-[6-(4-브로모페녹시)-2-(트리플루오로메틸)-3-피리딜]-1-(1,2,4-트리아졸-1-일)프로판-2-올, (1.084) 2-[6-(4-클로로페녹시)-2-(트리플루오로메틸)-3-피리딜]-1-(1,2,4-트리아졸-1-일)프로판-2-올, (1.085) 3-[2-(1-클로로시클로프로필)-3-(3-클로로-2-플루오로-페닐)-2-히드록시-프로필]이미다졸-4-카르보니트릴, (1.086) 4-[[6-[rac-(2R)-2-(2,4-디플루오로페닐)-1,1-디플루오로-2-히드록시-3-(5-티옥소-4H-1,2,4-트리아졸-1-일)프로필]-3-피리딜]옥시]벤조니트릴, (1.087) N-이소프로필-N'-[5-메톡시-2-메틸-4-(2,2,2-트리플루오로-1-히드록시-1-페닐에틸)페닐]-N-메틸이미도포름아미드, (1.088) N'-{5-브로모-2-메틸-6-[(1-프로폭시프로판-2-일)옥시]피리딘-3-일}-N-에틸-N-메틸이미도포름아미드, (1.089) 헥사코나졸, (1.090) 펜코나졸, (1.091) 펜부코나졸, (1.092) 메틸 2-[2-클로로-4-(4-클로로페녹시)페닐]-2-히드록시-3-(1,2,4-트리아졸-1-일)프로파노에이트,
하기로 이루어진 군으로부터 선택된 복합체 I 또는 II에서의 호흡 사슬의 억제제: (2.001) 벤조빈디플루피르, (2.002) 빅사펜, (2.003) 보스칼리드, (2.004) 카르복신, (2.005) 플루오피람, (2.006) 플루톨라닐, (2.007) 플룩사피록사드, (2.008) 푸라메트피르, (2.009) 이소페타미드, (2.010) 이소피라잠 (안티-에피머 거울상이성질체 1R,4S,9S), (2.011) 이소피라잠 (안티-에피머 거울상이성질체 1S,4R,9R), (2.012) 이소피라잠 (안티-에피머 라세미체 1RS,4SR,9SR), (2.013) 이소피라잠 (신-에피머 라세미체 1RS,4SR,9RS 및 안티-에피머 라세미체 1RS,4SR,9SR의 혼합물), (2.014) 이소피라잠 (신-에피머 거울상이성질체 1R,4S,9R), (2.015) 이소피라잠 (신-에피머 거울상이성질체 1S,4R,9S), (2.016) 이소피라잠 (신-에피머 라세미체 1RS,4SR,9RS), (2.017) 펜플루펜, (2.018) 펜티오피라드, (2.019) 피디플루메토펜, (2.020) 피라지플루미드, (2.021) 세닥산, (2.022) 1,3-디메틸-N-(1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일)-1H-피라졸-4-카르복스아미드, (2.023) 1,3-디메틸-N-[(3R)-1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일]-1H-피라졸-4-카르복스아미드, (2.024) 1,3-디메틸-N-[(3S)-1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일]-1H-피라졸-4-카르복스아미드, (2.025) 1-메틸-3-(트리플루오로메틸)-N-[2'-(트리플루오로메틸)비페닐-2-일]-1H-피라졸-4-카르복스아미드, (2.026) 2-플루오로-6-(트리플루오로메틸)-N-(1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일)벤즈아미드, (2.027) 3-(디플루오로메틸)-1-메틸-N-(1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일)-1H-피라졸-4-카르복스아미드, (2.028) 인피르플룩삼, (2.029) 3-(디플루오로메틸)-1-메틸-N-[(3S)-1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일]-1H-피라졸-4-카르복스아미드, (2.030) 플루인다피르, (2.031) 3-(디플루오로메틸)-N-[(3R)-7-플루오로-1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일]-1-메틸-1H-피라졸-4-카르복스아미드, (2.032) 3-(디플루오로메틸)-N-[(3S)-7-플루오로-1,1,3-트리메틸-2,3-디히드로-1H-인덴-4-일]-1-메틸-1H-피라졸-4-카르복스아미드, (2.033) 5,8-디플루오로-N-[2-(2-플루오로-4-{[4-(트리플루오로메틸)피리딘-2-일]옥시}페닐)에틸]퀴나졸린-4-아민, (2.034) N-(2-시클로펜틸-5-플루오로벤질)-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.035) N-(2-tert-부틸-5-메틸벤질)-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.036) N-(2-tert-부틸벤질)-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.037) N-(5-클로로-2-에틸벤질)-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.038) 이소플루시프람, (2.039) N-[(1R,4S)-9-(디클로로메틸렌)-1,2,3,4-테트라히드로-1,4-메타노나프탈렌-5-일]-3-(디플루오로메틸)-1-메틸-1H-피라졸-4-카르복스아미드, (2.040) N-[(1S,4R)-9-(디클로로메틸렌)-1,2,3,4-테트라히드로-1,4-메타노나프탈렌-5-일]-3-(디플루오로메틸)-1-메틸-1H-피라졸-4-카르복스아미드, (2.041) N-[1-(2,4-디클로로페닐)-1-메톡시프로판-2-일]-3-(디플루오로메틸)-1-메틸-1H-피라졸-4-카르복스아미드, (2.042) N-[2-클로로-6-(트리플루오로메틸)벤질]-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.043) N-[3-클로로-2-플루오로-6-(트리플루오로메틸)벤질]-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.044) N-[5-클로로-2-(트리플루오로메틸)벤질]-N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.045) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-1-메틸-N-[5-메틸-2-(트리플루오로메틸)벤질]-1H-피라졸-4-카르복스아미드, (2.046) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-N-(2-플루오로-6-이소프로필벤질)-1-메틸-1H-피라졸-4-카르복스아미드, (2.047) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-N-(2-이소프로필-5-메틸벤질)-1-메틸-1H-피라졸-4-카르복스아미드, (2.048) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-N-(2-이소프로필벤질)-1-메틸-1H-피라졸-4-카르보티오아미드, (2.049) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-N-(2-이소프로필벤질)-1-메틸-1H-피라졸-4-카르복스아미드, (2.050) N-시클로프로필-3-(디플루오로메틸)-5-플루오로-N-(5-플루오로-2-이소프로필벤질)-1-메틸-1H-피라졸-4-카르복스아미드, (2.051) N-시클로프로필-3-(디플루오로메틸)-N-(2-에틸-4,5-디메틸벤질)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.052) N-시클로프로필-3-(디플루오로메틸)-N-(2-에틸-5-플루오로벤질)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.053) N-시클로프로필-3-(디플루오로메틸)-N-(2-에틸-5-메틸벤질)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.054) N-시클로프로필-N-(2-시클로프로필-5-플루오로벤질)-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.055) N-시클로프로필-N-(2-시클로프로필-5-메틸벤질)-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.056) N-시클로프로필-N-(2-시클로프로필벤질)-3-(디플루오로메틸)-5-플루오로-1-메틸-1H-피라졸-4-카르복스아미드, (2.057) 피라프로포인, (2.058) N-[rac-(1S,2S)-2-(2,4-디클로로페닐)시클로부틸]-2-(트리플루오로메틸)니코틴아미드, (2.059) N-[(1S,2S)-2-(2,4-디클로로페닐)시클로부틸]-2-(트리플루오로메틸)니코틴아미드, (2.060) 플루베네테람,
하기로 이루어진 군으로부터 선택된 복합체 III에서의 호흡 사슬의 억제제: (3.001) 아메톡트라딘, (3.002) 아미술브롬, (3.003) 아족시스트로빈, (3.004) 쿠메톡시스트로빈, (3.005) 쿠목시스트로빈, (3.006) 시아조파미드, (3.007) 디목시스트로빈, (3.008) 에녹사스트로빈, (3.009) 파목사돈, (3.010) 페나미돈, (3.011) 플루페녹시스트로빈, (3.012) 플루옥사스트로빈, (3.013) 크레속심-메틸, (3.014) 메토미노스트로빈, (3.015) 오리사스트로빈, (3.016) 피콕시스트로빈, (3.017) 피라클로스트로빈, (3.018) 피라메토스트로빈, (3.019) 피라옥시스트로빈, (3.020) 트리플록시스트로빈, (3.021) (2E)-2-{2-[({[(1E)-1-(3-{[(E)-1-플루오로-2-페닐비닐]옥시}페닐)에틸리덴]아미노}옥시)메틸]페닐}-2-(메톡시이미노)-N-메틸아세트아미드, (3.022) (2E,3Z)-5-{[1-(4-클로로페닐)-1H-피라졸-3-일]옥시}-2-(메톡시이미노)-N,3-디메틸펜트-3-엔아미드, (3.023) (2R)-2-{2-[(2,5-디메틸페녹시)메틸]페닐}-2-메톡시-N-메틸아세트아미드, (3.024) (2S)-2-{2-[(2,5-디메틸페녹시)메틸]페닐}-2-메톡시-N-메틸아세트아미드, (3.025) 펜피콕사미드, (3.026) 만데스트로빈, (3.027) N-(3-에틸-3,5,5-트리메틸시클로헥실)-3-포름아미도-2-히드록시벤즈아미드, (3.028) (2E,3Z)-5-{[1-(4-클로로-2-플루오로페닐)-1H-피라졸-3-일]옥시}-2-(메톡시이미노)-N,3-디메틸펜트-3-엔아미드, (3.029) 메틸 {5-[3-(2,4-디메틸페닐)-1H-피라졸-1-일]-2-메틸벤질}카르바메이트, (3.030) 메틸테트라프롤, (3.031) 플로릴피콕사미드, (3.032) (2S,3S)-3-(o-톨릴)부탄-2-일 N-{[4-메톡시-3-(프로파노일옥시)-2-피리딜]카르보닐}-L-알라니네이트,
하기로 이루어진 군으로부터 선택된 유사분열 및 세포 분열의 억제제: (4.001) 카르벤다짐, (4.002) 디에토펜카르브, (4.003)에타복삼, (4.004) 플루오피콜리드, (4.005) 펜시쿠론, (4.006) 티아벤다졸, (4.007) 티오파네이트-메틸, (4.008) 족사미드, (4.009) 피리다클로메틸, (4.010) 3-클로로-5-(4-클로로페닐)-4-(2,6-디플루오로페닐)-6-메틸피리다진, (4.011) 3-클로로-5-(6-클로로피리딘-3-일)-6-메틸-4-(2,4,6-트리플루오로페닐)피리다진, (4.012) 4-(2-브로모-4-플루오로페닐)-N-(2,6-디플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.013) 4-(2-브로모-4-플루오로페닐)-N-(2-브로모-6-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.014) 4-(2-브로모-4-플루오로페닐)-N-(2-브로모페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.015) 4-(2-브로모-4-플루오로페닐)-N-(2-클로로-6-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.016) 4-(2-브로모-4-플루오로페닐)-N-(2-클로로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.017) 4-(2-브로모-4-플루오로페닐)-N-(2-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.018) 4-(2-클로로-4-플루오로페닐)-N-(2,6-디플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.019) 4-(2-클로로-4-플루오로페닐)-N-(2-클로로-6-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.020) 4-(2-클로로-4-플루오로페닐)-N-(2-클로로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.021) 4-(2-클로로-4-플루오로페닐)-N-(2-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.022) 4-(4-클로로페닐)-5-(2,6-디플루오로페닐)-3,6-디메틸피리다진, (4.023) N-(2-브로모-6-플루오로페닐)-4-(2-클로로-4-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.024) N-(2-브로모페닐)-4-(2-클로로-4-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.025) N-(4-클로로-2,6-디플루오로페닐)-4-(2-클로로-4-플루오로페닐)-1,3-디메틸-1H-피라졸-5-아민, (4.026) 플루오피모미드,
하기로 이루어진 군으로부터 선택된 다중부위 작용을 가질 수 있는 화합물: (5.001) 보르도 혼합물, (5.002) 캅타폴, (5.003) 캅탄, (5.004) 클로로탈로닐, (5.005) 수산화구리, (5.006) 나프텐산구리, (5.007) 산화구리, (5.008) 옥시염화구리, (5.009) 황산구리(2+), (5.010) 디티아논, (5.011) 도딘, (5.012) 폴페트, (5.013) 만코제브, (5.014) 마네브, (5.015) 메티람, (5.016) 메티람 아연, (5.017) 옥신-구리, (5.018) 프로피네브, (5.019) 황 및 칼슘 폴리술피드를 포함하는 황 제제, (5.020) 티람, (5.021) 지네브, (5.022) 지람, (5.023) 6-에틸-5,7-디옥소-6,7-디히드로-5H-피롤로[3',4':5,6][1,4]디티이노[2,3-c][1,2]티아졸-3-카르보니트릴,
(6.001) 아시벤졸라르-S-메틸, (6.002) 이소티아닐, (6.003) 프로베나졸, (6.004) 티아디닐로 이루어진 군으로부터 선택된, 숙주 방어를 유도할 수 있는 화합물,
(7.001) 시프로디닐, (7.002) 카수가마이신, (7.003) 카수가마이신 히드로클로라이드 수화물, (7.004) 옥시테트라시클린, (7.005) 피리메타닐, (7.006) 3-(5-플루오로-3,3,4,4-테트라메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀린으로 이루어진 군으로부터 선택된 아미노산 및/또는 단백질 생합성의 억제제,
(8.001) 실티오팜으로 이루어진 군으로부터 선택된 ATP 생산 억제제,
하기로 이루어진 군으로부터 선택된 세포벽 합성의 억제제: (9.001) 벤티아발리카르브, (9.002) 디메토모르프, (9.003) 플루모르프, (9.004)이프로발리카르브, (9.005) 만디프로파미드, (9.006) 피리모르프, (9.007) 발리페날레이트, (9.008) (2E)-3-(4-tert-부틸페닐)-3-(2-클로로피리딘-4-일)-1-(모르폴린-4-일)프로프-2-엔-1-온, (9.009) (2Z)-3-(4-tert-부틸페닐)-3-(2-클로로피리딘-4-일)-1-(모르폴린-4-일)프로프-2-엔-1-온,
(10.001) 프로파모카르브, (10.002) 프로파모카르브 히드로클로라이드, (10.003) 톨클로포스-메틸로 이루어진 군으로부터 선택된 지질 및 막 합성의 억제제,
(11.001) 트리시클라졸, (11.002) 톨프로카르브로 이루어진 군으로부터 선택된 멜라닌 생합성의 억제제,
(12.001) 베날락실, (12.002) 베날락실-M (키랄락실), (12.003) 메탈락실, (12.004) 메탈락실-M (메페녹삼)으로 이루어진 군으로부터 선택된 핵산 합성의 억제제,
(13.001) 플루디옥소닐, (13.002) 이프로디온, (13.003) 프로시미돈, (13.004) 프로퀴나지드, (13.005) 퀴녹시펜, (13.006) 빈클로졸린으로 이루어진 군으로부터 선택된 신호 전달의 억제제,
(14.001) 플루아지남, (14.002) 멥틸디노캅으로 이루어진 군으로부터 선택된 탈커플링제로서 작용할 수 있는 화합물,
하기로 이루어진 군으로부터 선택된 추가의 살진균제: (15.001) 아브시스산, (15.002) 벤티아졸, (15.003) 베톡사진, (15.004) 캡시마이신, (15.005) 카르본, (15.006) 키노메티오나트, (15.007) 쿠프라넵, (15.008) 시플루페나미드, (15.009) 시목사닐, (15.010) 시프로술파미드, (15.011) 플루티아닐, (15.012) 포세틸-알루미늄, (15.013) 포세틸-칼슘, (15.014) 포세틸-소듐, (15.015) 메틸 이소티오시아네이트, (15.016) 메트라페논, (15.017) 밀디오마이신, (15.018) 나타마이신, (15.019) 니켈 디메틸디티오카르바메이트, (15.020) 니트로탈-이소프로필, (15.021) 옥사모카르브, (15.022) 옥사티아피프롤린, (15.023) 옥시펜티인, (15.024) 펜타클로로페놀 및 염, (15.025) 아인산 및 그의 염, (15.026) 프로파모카르브-포세틸레이트, (15.027) 피리오페논 (클라자페논), (15.028) 테부플로퀸, (15.029) 테클로프탈람, (15.030) 톨니파니드, (15.031) 1-(4-{4-[(5R)-5-(2,6-디플루오로페닐)-4,5-디히드로-1,2-옥사졸-3-일]-1,3-티아졸-2-일}피페리딘-1-일)-2-[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]에타논, (15.032) 1-(4-{4-[(5S)-5-(2,6-디플루오로페닐)-4,5-디히드로-1,2-옥사졸-3-일]-1,3-티아졸-2-일}피페리딘-1-일)-2-[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]에타논, (15.033) 2-(6-벤질피리딘-2-일)퀴나졸린, (15.034) 디피메티트론, (15.035) 2-[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]-1-[4-(4-{5-[2-(프로프-2-인-1-일옥시)페닐]-4,5-디히드로-1,2-옥사졸-3-일}-1,3-티아졸-2-일)피페리딘-1-일]에타논, (15.036) 2-[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]-1-[4-(4-{5-[2-클로로-6-(프로프-2-인-1-일옥시)페닐]-4,5-디히드로-1,2-옥사졸-3-일}-1,3-티아졸-2-일)피페리딘-1-일]에타논, (15.037) 2-[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]-1-[4-(4-{5-[2-플루오로-6-(프로프-2-인-1-일옥시)페닐]-4,5-디히드로-1,2-옥사졸-3-일}-1,3-티아졸-2-일)피페리딘-1-일]에타논, (15.038) 2-[6-(3-플루오로-4-메톡시페닐)-5-메틸피리딘-2-일]퀴나졸린, (15.039) 2-{(5R)-3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-4,5-디히드로-1,2-옥사졸-5-일}-3-클로로페닐 메탄술포네이트, (15.040) 2-{(5S)-3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-4,5-디히드로-1,2-옥사졸-5-일}-3-클로로페닐 메탄술포네이트, (15.041) 이플루페노퀸, (15.042) 2-{2-플루오로-6-[(8-플루오로-2-메틸퀴놀린-3-일)옥시]페닐}프로판-2-올, (15.043) 플루옥사피프롤린, (15.044) 2-{3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-4,5-디히드로-1,2-옥사졸-5-일}페닐 메탄술포네이트, (15.045) 2-페닐페놀 및 염, (15.046) 3-(4,4,5-트리플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀린, (15.047) 퀴노푸멜린, (15.048) 4-아미노-5-플루오로피리미딘-2-올 (호변이성질체 형태: 4-아미노-5-플루오로피리미딘-2(1H)-온), (15.049) 4-옥소-4-[(2-페닐에틸)아미노]부탄산, (15.050) 5-아미노-1,3,4-티아디아졸-2-티올, (15.051) 5-클로로-N'-페닐-N'-(프로프-2-인-1-일)티오펜-2-술포노히드라지드, (15.052) 5-플루오로-2-[(4-플루오로벤질)옥시]피리미딘-4-아민, (15.053) 5-플루오로-2-[(4-메틸벤질)옥시]피리미딘-4-아민, (15.054) 9-플루오로-2,2-디메틸-5-(퀴놀린-3-일)-2,3-디히드로-1,4-벤족사제핀, (15.055) 부트-3-인-1-일 {6-[({[(Z)-(1-메틸-1H-테트라졸-5-일)(페닐)메틸렌]아미노}옥시)메틸]피리딘-2-일}카르바메이트, (15.056) 에틸 (2Z)-3-아미노-2-시아노-3-페닐아크릴레이트, (15.057) 페나진-1-카르복실산, (15.058) 프로필 3,4,5-트리히드록시벤조에이트, (15.059) 퀴놀린-8-올, (15.060) 퀴놀린-8-올 술페이트 (2:1), (15.061) tert-부틸 {6-[({[(1-메틸-1H-테트라졸-5-일)(페닐)메틸렌]아미노}옥시)메틸]피리딘-2-일}카르바메이트, (15.062) 5-플루오로-4-이미노-3-메틸-1-[(4-메틸페닐)술포닐]-3,4-디히드로피리미딘-2(1H)-온, (15.063) 아미노피리펜, (15.064) (N'-[2-클로로-4-(2-플루오로페녹시)-5-메틸페닐]-N-에틸-N-메틸이미도포름아미드), (15.065) (N'-(2-클로로-5-메틸-4-페녹시페닐)-N-에틸-N-메틸이미도포름아미드), (15.066) (2-{2-[(7,8-디플루오로-2-메틸퀴놀린-3-일)옥시]-6-플루오로페닐}프로판-2-올), (15.067) (5-브로모-1-(5,6-디메틸피리딘-3-일)-3,3-디메틸-3,4-디히드로이소퀴놀린), (15.068) (3-(4,4-디플루오로-5,5-디메틸-4,5-디히드로티에노[2,3-c]피리딘-7-일)퀴놀린), (15.069) (1-(4,5-디메틸-1H-벤즈이미다졸-1-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린), (15.070) 8-플루오로-3-(5-플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀론, (15.071) 8-플루오로-3-(5-플루오로-3,3,4,4-테트라메틸-3,4-디히드로이소퀴놀린-1-일)퀴놀론, (15.072) 3-(4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린-1-일)-8-플루오로퀴놀린, (15.073) (N-메틸-N-페닐-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드), (15.074) 메틸 {4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐}카르바메이트, (15.075) (N-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}시클로프로판카르복스아미드), (15.076) N-메틸-4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.077) N-[(E)-메톡시이미노메틸]-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.078) N-[(Z)-메톡시이미노메틸]-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.079) N-[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]시클로프로판카르복스아미드, (15.080) N-(2-플루오로페닐)-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.081) 2,2-디플루오로-N-메틸-2-[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]아세트아미드, (15.082) N-알릴-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일)페닐]메틸]아세트아미드, (15.083) N-[(E)-N-메톡시-C-메틸-카본이미도일]-4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.084) N-[(Z)-N-메톡시-C-메틸-카본이미도일]-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.085) N-알릴-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]프로판아미드, (15.086) 4,4-디메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피롤리딘-2-온, (15.087) N-메틸-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤젠카르보티오아미드, (15.088) 5-메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피롤리딘-2-온, (15.089) N-((2,3-디플루오로-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]-3,3,3-트리플루오로-프로판아미드, (15.090) 1-메톡시-1-메틸-3-[[4-[5-(트리플루오로메틸}-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.091) 1,1-디에틸-3-[[4-[5-(트리플루오로메틸}-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.092) N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]프로판아미드, (15.093) N-메톡시-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]시클로프로판카르복스아미드, (15.094) 1-메톡시-3-메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.095) N-메톡시-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸)시클로프로판카르복스아미드, (15.096) N,2-디메톡시-N-[[4-[5-(트리플루오로메틸}-1,2,4-옥사디아졸-3-일]페닐]메틸]프로판아미드, (15.097) N-에틸-2-메틸-N-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일)페닐]메틸]프로판아미드, (15.098) 1-메톡시-3-메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.099) 1,3-디메톡시-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.100) 3-에틸-1-메톡시-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]우레아, (15.101) 1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피페리딘-2-온, (15.102) 4,4-디메틸-2-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.103) 5,5-디메틸-2-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.104) 3,3-디메틸-1-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]피페리딘-2-온, (15.105) 1-[[3-플루오로-4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]아제판-2-온, (15.106) 4,4-디메틸-2-[[4-(5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.107) 5,5-디메틸-2-[[4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐]메틸]이속사졸리딘-3-온, (15.108) 에틸 1-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}-1H-피라졸-4-카르복실레이트, (15.109) N,N-디메틸-1-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}-1H-1,2,4-트리아졸-3-아민, (15.110) N-{2,3-디플루오로-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤질}부탄아미드, (15.111) N-(1-메틸시클로프로필)-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.112) N-(2,4-디플루오로페닐)-4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]벤즈아미드, (15.113) 1-(5,6-디메틸피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.114) 1-(6-(디플루오로메틸)-5-메틸-피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.115) 1-(5-(플루오로메틸)-6-메틸-피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.116) 1-(6-(디플루오로메틸)-5-메톡시-피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.117) 4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐 디메틸카르바메이트, (15.118) N-{4-[5-(트리플루오로메틸)-1,2,4-옥사디아졸-3-일]페닐}프로판아미드, (15.119) 3-[2-(1-{[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.120) 9-플루오로-3-[2-(1-{[5-메틸-3-(트리플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.121) 3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.122) 3-[2-(1-{[3,5-비스(디플루오로메틸)-1H-피라졸-1-일]아세틸}피페리딘-4-일)-1,3-티아졸-4-일]-9-플루오로-1,5-디히드로-2,4-벤조디옥세핀-6-일 메탄술포네이트, (15.123) 1-(6,7-디메틸피라졸로[1,5-a]피리딘-3-일)-4,4-디플루오로-3,3-디메틸-3,4-디히드로이소퀴놀린, (15.124) 8-플루오로-N-(4,4,4-트리플루오로-2-메틸-1-페닐부탄-2-일)퀴놀린-3-카르복스아미드, (15.125) 8-플루오로-N-[(2S)-4,4,4-트리플루오로-2-메틸-1-페닐부탄-2-일]퀴놀린-3-카르복스아미드, (15.126) N-(2,4-디메틸-1-페닐펜탄-2-일)-8-플루오로퀴놀린-3-카르복스아미드, (15.127) N-[(2S)-2,4-디메틸-1-페닐펜탄-2-일]-8-플루오로퀴놀린-3-카르복스아미드, (15.128) D-타가토스,
박테리아, 예컨대 (16.001) 바실루스 서브틸리스(Bacillus subtilis), 특히 균주 QST713/AQ713 (미국 소재의 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨); (16.002) 바실루스 아밀로리퀘파시엔스(Bacillus amyloliquefaciens), 특히 균주 D747 (미국 소재의 세르티스로부터 더블 니켈™ 하에 입수가능함, 수탁 번호 FERM BP-8234를 갖고, 미국 특허 번호 7,094,592에 개시됨); (16.003) 바실루스 푸밀루스(Bacillus pumilus), 특히 균주 BU F-33 (NRRL 수탁 번호 50185를 가짐); (16.004) 바실루스 서브틸리스 변종 아밀로리퀘파시엔스 균주 FZB24 (미국 소재 노보자임스로부터 타에그로® 하에 입수가능함); (16.005) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스(Paenibacillus) 종 균주; 및 진균, 예컨대 (16.006) 아우레오바시디움 풀루란스(Aureobasidium pullulans), 특히 균주 DSM14940의 출아포자; (16.007) 균주 DSM 14941의 아우레오바시디움 풀루란스 출아포자; (16.008) 아우레오바시디움 풀루란스, 특히 균주 DSM14940 및 DSM14941의 출아포자의 혼합물로 이루어진 군으로부터 선택된 항박테리아제,
박테리아로 이루어진 군으로부터 선택된 생물학적 살진균제, 예를 들어, (17.001) 바실루스 서브틸리스, 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨); (17.002) 바실루스 푸밀루스, 특히 균주 QST2808 (미국 소재 바이엘 크롭사이언스 엘피로부터 소나타® 하에 입수가능함, 수탁 번호 NRRL B-30087을 갖고, 미국 특허 번호 6,245,551에 기재됨); (17.003) 바실루스 푸밀루스, 특히 균주 GB34 (독일 소재 바이엘 아게로부터 일드 쉴드® 하에 입수가능함); (17.004) 바실루스 푸밀루스, 특히 균주 BU F-33 (NRRL 수탁 번호 50185를 가짐); (17.005) 바실루스 아밀로리퀘파시엔스(Bacillus amyloliquefaciens), 특히 균주 D747 (미국 세르티스로부터 더블 니켈™ 하에 입수가능함, 수탁 번호 FERM BP-8234를 갖고, 미국 특허 번호 7,094,592에 개시됨); (17.006) 바실루스 서브틸리스 Y1336 (대만 소재 비온-테크로부터 바이오박® WP 하에 입수가능함, 타이완에 등록 번호 4764, 5454, 5096 및 5277로 생물학적 살진균제로서 등록됨); (17.007) 바실루스 아밀로리퀘파시엔스 균주 MBI 600 (바스프 에스이로부터 서브틸렉스 하에 입수가능함); (17.008) 바실루스 서브틸리스 균주 GB03 (독일 소재 바이엘 아게로부터 코디악® 하에 입수가능함); (17.009) 바실루스 서브틸리스 변종 아밀로리퀘파시엔스 균주 FZB24 (버지니아주 살렘 소재 노보자임스 바이올로지칼스 인크. 또는 노스 캐롤라이나주 그린스보 소재 신젠타 크롭 프로텍션, 엘엘씨로부터 살진균제 타에그로® 또는 타에그로® ECO 하에 입수가능함 (EPA 등록 번호 70127-5); (17.010) 바실루스 미코이데스, 단리물 J (세르티스 유에스에이로부터 BmJ TGAI 또는 WG 하에 입수가능함); (17.011) 바실루스 리케니포르미스(Bacillus licheniformis), 특히 균주 SB3086 (노보자임스로부터 에코가드™ 생물살진균제 및 그린 릴리프 하에 입수가능함); (17.012) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스 종 균주,
지방산 또는 유도체, 예를 들어 (18.001) 불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%는 C14 내지 C20의 범위인 조성물 (예를 들어 알파바이오 페스티시드즈 또는 바이엘 아게의 FLiPPER). - 제1항 내지 제7항 중 어느 한 항에 있어서,
추가의 활성 화합물 (B)는
(1.002) 디페노코나졸, (1.018) 프로티오코나졸, (1.020) 스피록사민, (1.021) 테부코나졸, (1.055) 메펜트리플루코나졸, (1.062) 플루옥시티오코나졸, (1.067) N'-(2,5-디메틸-4-{3-[(1,1,2,2-테트라플루오로에틸)술파닐]페녹시}페닐)-N-에틸-N-메틸이미도포름아미드, (2.002) 빅사펜, (2.005) 플루오피람, (2.028) 인피르플룩삼, (2.038) 이소플루시프람, (3.020) 트리플록시스트로빈, (3.025) 펜피콕사미드, (5.003) 캅탄, (5.010) 디티아논, (5.012) 폴페트, (5.013) 만코제브, (5.018) 프로피네브, (6.002) 이소티아닐, (7.005) 피리메타닐, (13.001) 플루디옥소닐, (13.004) 프로퀴나지드, (13.005) 퀴녹시펜, (15.012) 포세틸-알루미늄, (15.016) 메트라페논, (15.043) 플루옥사피프롤린 및 (15.064) (N'-[2-클로로-4-(2-플루오로페녹시)-5-메틸페닐]-N-에틸-N-메틸이미도포름아미드), (17.001) 바실루스 서브틸리스(Bacillus subtilis), 특히 균주 QST713/AQ713 (미국 소재 바이엘 크롭사이언스 엘피로부터 세레나데 옵티 또는 세레나데 아소 하에 입수가능함, NRRL 수탁 번호 B21661을 갖고, 미국 특허 번호 6,060,051에 기재됨), (17.012) 수탁 번호 NRRL B-50972 또는 수탁 번호 NRRL B-67129를 갖고 국제 특허 공개 번호 WO 2016/154297에 기재된 파에니바실루스(Paenibacillus) 종 균주 및 (18.001) 불포화 및 포화 C12-C24 지방산, 그의 염, 그의 에스테르 또는 상기 중 임의의 것의 혼합물로부터 선택된 1종 이상의 지방산 또는 그의 유도체를 포함하며, 여기서 상기 지방산 또는 그의 유도체의 적어도 95%가 C14 내지 C20의 범위인 조성물 (예를 들어, 알파바이오 페스티시드즈 또는 바이엘 아게의 FLiPPER)
로 이루어진 군으로부터 선택된 것인 활성 화합물 조합물. - 적어도 1종의 증량제 및/또는 계면활성제와, 제1항 내지 제8항 중 어느 한 항에 따른 활성 화합물 조합물을 함유하는 것을 특징으로 하는, 작물 보호 및 물질 보호에서 유해 미생물, 바람직하게는 식물병원성 유해 진균을 방제하기 위한 조성물.
- 제1항 내지 제8항 중 어느 한 항에 따른 활성 화합물 조합물 또는 제9항에 따른 조성물을 유해 미생물 및/또는 그의 서식지에 적용하는 것을 특징으로 하는, 작물 보호 및 물질 보호에서 유해 미생물, 바람직하게는 식물병원성 유해 진균을 방제하는 방법.
- 작물 보호 및 물질 보호에서 유해 미생물, 바람직하게는 식물병원성 유해 진균의 방제를 위한 제1항 내지 제8항 중 어느 한 항에 따른 활성 화합물 조합물 또는 제9항에 따른 조성물의 용도.
- 트랜스제닉 식물의 처리를 위한 제1항 내지 제8항 중 어느 한 항에 따른 활성 화합물 조합물 또는 제9항에 따른 조성물의 용도.
- 종자, 바람직하게는 트랜스제닉 식물의 종자의 처리를 위한 제1항 내지 제8항 중 어느 한 항에 따른 활성 화합물 조합물 또는 제9항에 따른 조성물의 용도.
- 제1항 내지 제8항 중 어느 한 항에 따른 활성 화합물 조합물 또는 제9항에 따른 조성물로 코팅된 종자.
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