KR102073472B1 - Distilled Liquor from A. distichum root and preparation method of the same - Google Patents

Distilled Liquor from A. distichum root and preparation method of the same Download PDF

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KR102073472B1
KR102073472B1 KR1020180025411A KR20180025411A KR102073472B1 KR 102073472 B1 KR102073472 B1 KR 102073472B1 KR 1020180025411 A KR1020180025411 A KR 1020180025411A KR 20180025411 A KR20180025411 A KR 20180025411A KR 102073472 B1 KR102073472 B1 KR 102073472B1
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distilled
distilled liquor
root
roots
liquor
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우종태
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    • CCHEMISTRY; METALLURGY
    • C12BIOCHEMISTRY; BEER; SPIRITS; WINE; VINEGAR; MICROBIOLOGY; ENZYMOLOGY; MUTATION OR GENETIC ENGINEERING
    • C12GWINE; PREPARATION THEREOF; ALCOHOLIC BEVERAGES; PREPARATION OF ALCOHOLIC BEVERAGES NOT PROVIDED FOR IN SUBCLASSES C12C OR C12H
    • C12G3/00Preparation of other alcoholic beverages
    • C12G3/04Preparation of other alcoholic beverages by mixing, e.g. for preparation of liqueurs
    • C12G3/05Preparation of other alcoholic beverages by mixing, e.g. for preparation of liqueurs with health-improving ingredients, e.g. flavonoids, flavones, polyphenols or polysaccharides
    • C12G3/055Preparation of other alcoholic beverages by mixing, e.g. for preparation of liqueurs with health-improving ingredients, e.g. flavonoids, flavones, polyphenols or polysaccharides extracted from plants
    • CCHEMISTRY; METALLURGY
    • C12BIOCHEMISTRY; BEER; SPIRITS; WINE; VINEGAR; MICROBIOLOGY; ENZYMOLOGY; MUTATION OR GENETIC ENGINEERING
    • C12GWINE; PREPARATION THEREOF; ALCOHOLIC BEVERAGES; PREPARATION OF ALCOHOLIC BEVERAGES NOT PROVIDED FOR IN SUBCLASSES C12C OR C12H
    • C12G3/00Preparation of other alcoholic beverages
    • C12G3/04Preparation of other alcoholic beverages by mixing, e.g. for preparation of liqueurs
    • CCHEMISTRY; METALLURGY
    • C12BIOCHEMISTRY; BEER; SPIRITS; WINE; VINEGAR; MICROBIOLOGY; ENZYMOLOGY; MUTATION OR GENETIC ENGINEERING
    • C12HPASTEURISATION, STERILISATION, PRESERVATION, PURIFICATION, CLARIFICATION OR AGEING OF ALCOHOLIC BEVERAGES; METHODS FOR ALTERING THE ALCOHOL CONTENT OF FERMENTED SOLUTIONS OR ALCOHOLIC BEVERAGES
    • C12H6/00Methods for increasing the alcohol content of fermented solutions or alcoholic beverages
    • C12H6/02Methods for increasing the alcohol content of fermented solutions or alcoholic beverages by distillation

Abstract

본 발명은 미선나무 뿌리로부터 알콜 침출액을 추출하여 그 침출액을 환류추출하여 획득하는 증류주에 관한 것으로 미선나무의 꽃, 잎에 비하여 수율, DDPH 소거능 및 폴리페놀 성분 함량이 높아 항염, 항암기능성이 증진되는 뛰어난 효과가 있으므로 주류산업상 매우 유용한 발명이다.The present invention relates to a distilled liquor obtained by extracting an alcoholic leaching solution from the roots of the aster tree and refluxing the leaching solution. It is a very useful invention in the liquor industry because of its excellent effect.

Description

미선나무 뿌리를 이용하여 제조되는 증류주 및 그 제조방법 {Distilled Liquor from A. distichum root and preparation method of the same}Distilled liquor prepared using bark roots and its preparation method {Distilled Liquor from A. distichum root and preparation method of the same}

본 발명은 미선나무 잎, 꽃, 뿌리를 이용하여 제조되는 증류주 및 그 제조방법에 관한 것이다.The present invention relates to a distilled liquor prepared using a stem leaf, flowers, roots and a method for producing the same.

미선나무(Abeliophy distichum, Nakai)는 물푸레나무과 식물로 열매모양이 둥근 부채를 닮아 미선나무라 호칭되는 낙엽관목으로 천연기념물 364호로 지정되어 있는 한국 충북 괴산 고유의 1속 1종 밖에 없는 자생식물이며 희귀종이다.Abeliophy distichum (Nakai) is a deciduous shrub that is named as amiaceae because it resembles a rounded fan-shaped plant. .

술은 발효주, 증류주 및 침출주로 분류되며 침출주는 양조주나 증류주에 원료물질을 첨가하여 침출하여서 제조된다. 인삼주, 매실주, 오가피주 등 다양한 침출주를 그 예로 들 수 있다.Alcohol is classified into fermented liquor, distilled liquor and leach liquor. Leach liquor is prepared by adding raw materials to brew or distilled liquor. For example, various leaching liquors such as ginseng wine, plum wine, and ogapi wine.

인삼 침출주는 국내특허 제10-0060213호, 녹차 침출주는 국내특허 제10--49498호, 지골피 침출주는 제10-33199호, 구기자 침출주는 제10-15306호, 신령버섯 침출주는 제10-135574호에 개시되어 있다. Ginseng leaching liquor No. 10-0060213, Green tea leaching liquor No. 10--49498, Gigolpi leaching liquor No. 10-33199, Gojigi leaching liquor No. 10-15306, Spirit mushroom leaching no. 10-135574 Is disclosed.

또, 미선나무 관련 선행기술을 살펴보면 미선나무추출물 및 이를 함유한 화장료 조성물이 제10-2009-19042호, 향료 조성물이 10-2008-119493호, 항염증제가 특허 제10-656287호, 항염제가 제10-706131호에 공지되어 있으나 지금까지 그 증류주는 공지된 바 없다.In addition, when looking at the prior art related to the bark tree, the bark extract and the cosmetic composition containing the same is No. 10-2009-19042, the fragrance composition is 10-2008-119493, the anti-inflammatory agent Patent No. 10-656287, the anti-inflammatory agent No. 10 It is known from -706131 but so far the distillate is not known.

따라서 본 발명은 지금까지 아무도 시도해본 바 없는 미선나무의 뿌리를 이용하여 제조되는 미선나무뿌리를 이용한 증류주와 그 제조방법을 제공하는 것을 그 목적으로 한다.Therefore, an object of the present invention is to provide a distilled liquor using a rootwood root prepared by using the root of the tailwood that no one has ever tried, and a method of manufacturing the same.

본 발명의 상기 목적은 미선나무의 꽃이 만개한 후 10월 초에서 11월 말에 채취한 뿌리의 절삭 건조물을 통풍이 잘되는 그늘에서 수분함량 25%가 되도록 자연건조하는 단계와; 상기 자연건조 단계에서 얻은 미선나무 건조된 뿌리 절삭물을 20도의 주정에 1:30~40(w/w) 비율로 배합하여 15℃에서 6개월간 활성성분을 침출시키는 단계와; 상기 침출 단계에서 얻은 미선나무 뿌리 침출액을 증류기에서 환류추출하여 증류주를 제조하는 단계로 이루어지고 최종 제조된 증류주의 활성성분 및 관능검사 결과 본 발명 제품을 평가하는 단계로 이루어진다.The above object of the present invention comprises the steps of naturally drying the cutting dry matter of the root taken in early October to the end of November after the flowers of the bark in full bloom to 25% moisture content in a well-ventilated shade; Blending the root wood dried root cuttings obtained in the natural drying step at a ratio of 1:30 to 40 (w / w) at 20 ° C to leach out the active ingredient at 15 ° C. for 6 months; Comprising the step of extracting the extract of the roots of the roots obtained in the leaching step to reflux in the distillation to prepare a distilled alcohol and the evaluation of the product of the present invention the active ingredient and sensory test result of the final distilled wine.

본 발명의 미선나무 뿌리를 이용한 증류주는 색도가 유백색으로 특이하고 풍미가 우수하여 관능검사 결과, 잎이나 꽃을 이용한 증류주에 비하여 생리활성성분 및 기호도가 현저히 뛰어난 효과가 있다.Distilled liquor using the root of the bark of the present invention, the color is milky white, and the taste is excellent, the sensory test results, compared to the distilled liquor using leaves or flowers, the biologically active ingredient and palatability is significantly superior.

이하, 본 발명의 구체적인 구성 및 효과를 실시예를 들어 더욱 상세히 설명한다.Hereinafter, specific configurations and effects of the present invention will be described in more detail with reference to Examples.

·제1공정: 미선나무 뿌리 채취 및 건조First step: extracting and drying the roots of the bark

10월 중순이 지나 낙엽이 떨어진 후 뿌리를 채취하여 수집한 다음 절삭하여 통풍이 잘되는 그늘에서 자연건조한다.After the leaves have fallen after mid-October, the roots are harvested, collected, cut and naturally dried in a well-ventilated shade.

·제2공정: 미선나무 뿌리 침출액의 제조2nd step: preparation of leachate root extract

제1공정에서 얻은 건조된 미선나무 뿌리를 절삭한 건조물(수분함량 25%)을 20도 소주에 중량비 1:30~40(w/w)으로 배합하여 15℃에서 6개월간 침지하여 침출액을 제조한다.A dried product (25% water content) cut from the dried bark roots obtained in the first step is blended in a weight ratio of 1:30 to 40 (w / w) in a 20-degree soju to be immersed at 15 ° C. for 6 months to prepare a leachate. .

·제3공정: 미선나무 증류주의 제조Third process: manufacture of stir wood distilled spirit

상기 제2공정에서 얻은 침출액을 환류 추출기에 넣어 통상의 방법으로 증류시킴으로서 알코올 농도 50도의 유백색 증류주를 수득한다.The leachate obtained in the second step was put in a reflux extractor and distilled by a conventional method to obtain a milky white distilled liquor having an alcohol concentration of 50 degrees.

미선나무의 흰꽃은 잎보다 먼저 개화하는 총상화서로서 향기가 좋으나 개화기가 3~4월에 제한되고 키가 커서 그 채취가 용이하지 않을뿐 아니라, 잎을 이용하여 제조되는 증류주는 독특한 쓴 맛으로 인하여 침출주로 사용하기에는 녹색이며 그로 인하여 풀냄새, 쓴맛으로 인해 기호도가 매우 떨어져 적합성과 실용성이 매우 적다. 한편, 10~11월에는 장광 단일하에서 잎을 통하여 합성된 다양한 광합성물질이 뿌리에 저장되어 특히 항염, 항암기능성 생리활성물질이 증진되고 당도와 폴리페놀 성분이 증대되어 침출주로 적합성과 실용성을 확인하기 위해 예의 연구하여 본 발명을 완성하였다.The white flowers of the thorn tree are fragrant flowers that bloom before the leaves, but they have good fragrance. However, since the flowering period is limited to March and April, they are not easy to collect because of the tall flowers. It is green to be used as a leaching liquor, and because of it, it has very low palatability due to the smell of grass and bitter taste. On the other hand, in October-November, various photosynthetic materials synthesized through leaves under Jangwang single are stored in the roots, especially anti-inflammatory and anti-cancer bioactive substances are enhanced, and sugar and polyphenol components are increased to confirm their suitability and practicality. The present invention was completed by earnest research.

이하,실시예를 따라 실험결과를 제시하나 본 발명 권리범위가 여기에 제시한 점들에 제한되지 않는 것은 명백하다.Hereinafter, the experimental results are presented according to the examples, but it is obvious that the scope of the present invention is not limited to the points set forth herein.

실시예1.Example 1

2016.10.1일에서 11.30까지 채취한 미선나무 뿌리를 채취하여 절삭하고 그늘에서 건조하여(가장 바람직하게는 수분함량 25%) 그 100g의 건조 절삭물을 알코올 농도 20도의 소주 3.5L에 침지하여 6개월간 그활성성분을 침출하여 그 침출액 3.505L를 수득하였다.The roots of the bark collected from January 30, 2016 to 11.30 are collected, cut, dried in the shade (preferably 25% moisture content), and 100 g of the dried cuttings are immersed in 3.5 liters of soju at 20 ° C for 6 months. The active ingredient was leached to obtain 3.505 L of the leaching solution.

상기에서 수득한 침출액을 환류 추출기에 전량을 넣어 증류시킨후 알콜농도 50도의 유백색 증류주 1.8L를 획득하였다.After distilling the leachate obtained above in a reflux extractor, 1.8L of a milky white distilled spirit having an alcohol concentration of 50 degrees was obtained.

비교예 1.Comparative Example 1.

미선나무 꽃을 사용한 것 외에는 모두 동일한 조건으로 실시하였다.All of them were carried out under the same conditions except that the flowers of the stems were used.

비교예2.Comparative Example 2.

미선나무 잎을 사용한 것 외에는 모두 동일한 조건으로 실시하였다.All of them were carried out under the same conditions except that the leaves of the stems were used.

실험예 1. 항산화 활성 및 수율Experimental Example 1. Antioxidant Activity and Yield

본 발명에 따라 상기 실시예1 및 비교예 1 내지 2에서 획득한 증류주의 항산화 활성을 특정지표 1, 1-diphenyl-2-picrylhydrazyl(DPPH) 방법으로 환원능을 측정하였다. DPPH 12.5mg을 에탄올 100mL에 용해한 용액 800μL를 본 발명에 따른 증류주 시료 200μL에 첨가하여 10분간 반응시킨후 525nm에서 흡광도(optical density)를 측정하여 비교한 결과는 다음 표 1과 같이 본 발명 뿌리 침출액으로부터 얻은 것이 소거활성과 수율이 가장 효과적이었다.According to the present invention, the antioxidant activity of the distilled wine obtained in Example 1 and Comparative Examples 1 and 2 was measured by the specific index 1, 1-diphenyl-2-picrylhydrazyl (DPPH) method. 800 μL of a solution of 12.5 mg of DPPH dissolved in 100 mL of ethanol was added to 200 μL of a distilled liquor sample according to the present invention and reacted for 10 minutes, and then the optical density was measured at 525 nm. The obtained one was most effective in scavenging activity and yield.

(IC50㎍/mL)(IC 50 μg / mL) 구분division 실시예 1Example 1 비교예 1Comparative Example 1 비교예 2Comparative Example 2 비고Remarks 소거활성Scavenging activity 20.3020.30 83.6883.68 125.32125.32 150.93150.93 수율(%)yield(%) 50.250.2 19.319.3 20.120.1 --

[주]비고는 원물의 수추출물.[Note] Remarks are water extracts of the original.

실험예 2. 생리활성성분(ppm)Experimental Example 2. Bioactive Components (ppm)

상기 본 발명 실시예1 및 비교예 1 내지 2에 따라 미선나무로부터 획득한 증류주는 알콜에 침지하여 저장중 숙성기간동안 프루프랄(furfural), 폴리페놀, 당 등의 생리활성 성분이 증가하였으나 뿌리가 가장 우수하였다(표 2).Distilled liquor obtained from S. aureus according to Example 1 and Comparative Examples 1 and 2 of the present invention was immersed in alcohol, and bioactive components such as furfural, polyphenol, and sugar were increased during aging period during storage. Best of all (Table 2).

구분division 실시예 1Example 1 비교예 1Comparative Example 1 비교예 2Comparative Example 2 비고Remarks 폴리페놀Polyphenols 102.4102.4 31.231.2 18.118.1 NDND 프루프랄Pruprral 29.029.0 5.45.4 3.23.2 NDND 당(%)Party(%) 0.210.21 0.780.78 NDND NDND

[주]1. ND = Not detected[Note] 1. ND = Not detected

2. 비고는 원물의 수추출물.    2. Remarks The water extract of the original.

실험예 3. 관능검사Experimental Example 3. Sensory Test

상기 본 발명 실시예1 및 비교예 1 내지 2에 따라 미선나무로부터 획득한 색도가 유백색인 증류주 10mL를 20~50대 청장년층 남녀 10명씩 Random sampling하여 풍미, 목넘김(부드러움), 이미취, 전반적인 기호도를 5점 평점법(5점: 좋다, 3점: 보통, 1점: 나쁘다)로 조사하여 그 평균값을 구한 결과는 하기 표 3과 같았다.According to Examples 1 and 2 of the present invention, 10 mL of distilled liquor having a milky white color obtained from the aster tree was randomly sampled by 10 men and women in their 20s to 50s, and was used for flavor, throbbing (softness), anesthesia, and overall preference. The average value of the results obtained by the five-point scoring method (five points: good, three points: normal, one point: bad) was obtained as shown in Table 3 below.

구분division 실시예 1Example 1 비교예 1Comparative Example 1 비교예 2Comparative Example 2 풍미zest 4.54.5 4.24.2 2.92.9 목넘김(부드러움)Thirsty (soft) 4.64.6 3.83.8 2.52.5 이미취Already 4.74.7 3.73.7 2.82.8 기호도Symbol 4.54.5 3.53.5 3.33.3

Claims (2)

미선나무의 꽃이 만개한 후 10월 초에서 11월 말에 채취한 뿌리의 절삭 건조물을 통풍이 잘되는 그늘에서 수분함량 25%가 되도록 자연건조하는 단계와; 상기 건조 단계에서 얻은 미선나무의 건조된 뿌리 절삭물을 20도의 주정에 1:30~40(w/w) 비율로 배합하여 15℃에서 6개월간 침출시키는 단계와; 상기 침출 단계에서 얻은 미선나무 뿌리의 침출액을 증류기에서 증류하여 증류주를 제조하는 단계로 이루어진 것을 특징으로 하는 미선나무 뿌리를 이용한 미선나무 증류주의 제조방법.Naturally drying the cutting dried material of the roots taken from the beginning of October to the end of November after the flowers of the bark tree are in full bloom so that the moisture content is 25% in a well-ventilated shade; Blending the dried root cuttings of the crypts obtained in the drying step at a ratio of 1:30 to 40 (w / w) at 20 degrees, and leaching at 15 ° C. for 6 months; Distilled liquor obtained from the leaching step of distilled from the roots of a distilled liquor to prepare a distilled liquor, characterized in that the method of producing a distilled liquor from the bark wood roots. 제1항의 방법으로 제조된 알콜농도 50도이며 유백색의 미선나무 뿌리 증류주.An alcohol concentration of 50 degrees prepared by the method of claim 1, milky white, distilled root.
KR1020180025411A 2018-03-02 2018-03-02 Distilled Liquor from A. distichum root and preparation method of the same KR102073472B1 (en)

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