JPWO2021119514A5 - - Google Patents
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- JPWO2021119514A5 JPWO2021119514A5 JP2022535821A JP2022535821A JPWO2021119514A5 JP WO2021119514 A5 JPWO2021119514 A5 JP WO2021119514A5 JP 2022535821 A JP2022535821 A JP 2022535821A JP 2022535821 A JP2022535821 A JP 2022535821A JP WO2021119514 A5 JPWO2021119514 A5 JP WO2021119514A5
- Authority
- JP
- Japan
- Prior art keywords
- wax
- polymer
- resin
- composition according
- ceramic material
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
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- 239000001993 wax Substances 0.000 claims description 55
- 229920000642 polymer Polymers 0.000 claims description 54
- 229920005989 resin Polymers 0.000 claims description 48
- 239000011347 resin Substances 0.000 claims description 48
- 239000000203 mixture Substances 0.000 claims description 47
- 229910010293 ceramic material Inorganic materials 0.000 claims description 44
- 239000000758 substrate Substances 0.000 claims description 24
- 239000002131 composite material Substances 0.000 claims description 20
- -1 polyethylene Polymers 0.000 claims description 17
- 239000000463 material Substances 0.000 claims description 15
- 238000004132 cross linking Methods 0.000 claims description 12
- 230000004048 modification Effects 0.000 claims description 10
- 238000012986 modification Methods 0.000 claims description 10
- XLOMVQKBTHCTTD-UHFFFAOYSA-N Zinc monoxide Chemical compound [Zn]=O XLOMVQKBTHCTTD-UHFFFAOYSA-N 0.000 claims description 6
- 239000000919 ceramic Substances 0.000 claims description 6
- 229910052751 metal Inorganic materials 0.000 claims description 6
- 239000002184 metal Substances 0.000 claims description 6
- FYYHWMGAXLPEAU-UHFFFAOYSA-N Magnesium Chemical compound [Mg] FYYHWMGAXLPEAU-UHFFFAOYSA-N 0.000 claims description 5
- 230000015556 catabolic process Effects 0.000 claims description 5
- 238000006731 degradation reaction Methods 0.000 claims description 5
- XLYOFNOQVPJJNP-UHFFFAOYSA-M hydroxide Chemical compound [OH-] XLYOFNOQVPJJNP-UHFFFAOYSA-M 0.000 claims description 5
- 229910052749 magnesium Inorganic materials 0.000 claims description 5
- 239000011777 magnesium Substances 0.000 claims description 5
- WPBNNNQJVZRUHP-UHFFFAOYSA-L manganese(2+);methyl n-[[2-(methoxycarbonylcarbamothioylamino)phenyl]carbamothioyl]carbamate;n-[2-(sulfidocarbothioylamino)ethyl]carbamodithioate Chemical compound [Mn+2].[S-]C(=S)NCCNC([S-])=S.COC(=O)NC(=S)NC1=CC=CC=C1NC(=S)NC(=O)OC WPBNNNQJVZRUHP-UHFFFAOYSA-L 0.000 claims description 5
- XEEYBQQBJWHFJM-UHFFFAOYSA-N Iron Chemical compound [Fe] XEEYBQQBJWHFJM-UHFFFAOYSA-N 0.000 claims description 4
- PXHVJJICTQNCMI-UHFFFAOYSA-N Nickel Chemical compound [Ni] PXHVJJICTQNCMI-UHFFFAOYSA-N 0.000 claims description 4
- 239000000654 additive Substances 0.000 claims description 4
- 229910052782 aluminium Inorganic materials 0.000 claims description 4
- XAGFODPZIPBFFR-UHFFFAOYSA-N aluminium Chemical compound [Al] XAGFODPZIPBFFR-UHFFFAOYSA-N 0.000 claims description 4
- 239000004203 carnauba wax Substances 0.000 claims description 4
- 230000007797 corrosion Effects 0.000 claims description 4
- 238000005260 corrosion Methods 0.000 claims description 4
- 239000007788 liquid Substances 0.000 claims description 4
- 239000012188 paraffin wax Substances 0.000 claims description 4
- 239000011148 porous material Substances 0.000 claims description 4
- 239000002383 tung oil Substances 0.000 claims description 4
- TWNQGVIAIRXVLR-UHFFFAOYSA-N oxo(oxoalumanyloxy)alumane Chemical compound O=[Al]O[Al]=O TWNQGVIAIRXVLR-UHFFFAOYSA-N 0.000 claims description 3
- 239000011787 zinc oxide Substances 0.000 claims description 3
- DSEKYWAQQVUQTP-XEWMWGOFSA-N (2r,4r,4as,6as,6as,6br,8ar,12ar,14as,14bs)-2-hydroxy-4,4a,6a,6b,8a,11,11,14a-octamethyl-2,4,5,6,6a,7,8,9,10,12,12a,13,14,14b-tetradecahydro-1h-picen-3-one Chemical compound C([C@H]1[C@]2(C)CC[C@@]34C)C(C)(C)CC[C@]1(C)CC[C@]2(C)[C@H]4CC[C@@]1(C)[C@H]3C[C@@H](O)C(=O)[C@@H]1C DSEKYWAQQVUQTP-XEWMWGOFSA-N 0.000 claims description 2
- 229910000838 Al alloy Inorganic materials 0.000 claims description 2
- 229910000851 Alloy steel Inorganic materials 0.000 claims description 2
- OYPRJOBELJOOCE-UHFFFAOYSA-N Calcium Chemical compound [Ca] OYPRJOBELJOOCE-UHFFFAOYSA-N 0.000 claims description 2
- 229910052684 Cerium Inorganic materials 0.000 claims description 2
- 229920002101 Chitin Polymers 0.000 claims description 2
- VYZAMTAEIAYCRO-UHFFFAOYSA-N Chromium Chemical compound [Cr] VYZAMTAEIAYCRO-UHFFFAOYSA-N 0.000 claims description 2
- RYGMFSIKBFXOCR-UHFFFAOYSA-N Copper Chemical compound [Cu] RYGMFSIKBFXOCR-UHFFFAOYSA-N 0.000 claims description 2
- 229920000742 Cotton Polymers 0.000 claims description 2
- 239000004971 Cross linker Substances 0.000 claims description 2
- 229910052693 Europium Inorganic materials 0.000 claims description 2
- 229940123457 Free radical scavenger Drugs 0.000 claims description 2
- 239000004166 Lanolin Substances 0.000 claims description 2
- 229910000990 Ni alloy Inorganic materials 0.000 claims description 2
- 239000004952 Polyamide Substances 0.000 claims description 2
- 239000004698 Polyethylene Substances 0.000 claims description 2
- 239000004642 Polyimide Substances 0.000 claims description 2
- 239000004721 Polyphenylene oxide Substances 0.000 claims description 2
- 239000004743 Polypropylene Substances 0.000 claims description 2
- 239000004793 Polystyrene Substances 0.000 claims description 2
- 239000004111 Potassium silicate Substances 0.000 claims description 2
- 229920001800 Shellac Polymers 0.000 claims description 2
- XUIMIQQOPSSXEZ-UHFFFAOYSA-N Silicon Chemical compound [Si] XUIMIQQOPSSXEZ-UHFFFAOYSA-N 0.000 claims description 2
- BQCADISMDOOEFD-UHFFFAOYSA-N Silver Chemical compound [Ag] BQCADISMDOOEFD-UHFFFAOYSA-N 0.000 claims description 2
- 239000004115 Sodium Silicate Substances 0.000 claims description 2
- 229910001069 Ti alloy Inorganic materials 0.000 claims description 2
- ATJFFYVFTNAWJD-UHFFFAOYSA-N Tin Chemical compound [Sn] ATJFFYVFTNAWJD-UHFFFAOYSA-N 0.000 claims description 2
- RTAQQCXQSZGOHL-UHFFFAOYSA-N Titanium Chemical compound [Ti] RTAQQCXQSZGOHL-UHFFFAOYSA-N 0.000 claims description 2
- 239000012963 UV stabilizer Substances 0.000 claims description 2
- 235000019498 Walnut oil Nutrition 0.000 claims description 2
- HCHKCACWOHOZIP-UHFFFAOYSA-N Zinc Chemical compound [Zn] HCHKCACWOHOZIP-UHFFFAOYSA-N 0.000 claims description 2
- QCWXUUIWCKQGHC-UHFFFAOYSA-N Zirconium Chemical compound [Zr] QCWXUUIWCKQGHC-UHFFFAOYSA-N 0.000 claims description 2
- 230000000996 additive effect Effects 0.000 claims description 2
- 229910052784 alkaline earth metal Inorganic materials 0.000 claims description 2
- 229910052788 barium Inorganic materials 0.000 claims description 2
- DSAJWYNOEDNPEQ-UHFFFAOYSA-N barium atom Chemical compound [Ba] DSAJWYNOEDNPEQ-UHFFFAOYSA-N 0.000 claims description 2
- 235000013871 bee wax Nutrition 0.000 claims description 2
- 239000012166 beeswax Substances 0.000 claims description 2
- 229940092738 beeswax Drugs 0.000 claims description 2
- 229910052791 calcium Inorganic materials 0.000 claims description 2
- 239000011575 calcium Substances 0.000 claims description 2
- 235000013869 carnauba wax Nutrition 0.000 claims description 2
- 229920002678 cellulose Polymers 0.000 claims description 2
- 239000001913 cellulose Substances 0.000 claims description 2
- GWXLDORMOJMVQZ-UHFFFAOYSA-N cerium Chemical compound [Ce] GWXLDORMOJMVQZ-UHFFFAOYSA-N 0.000 claims description 2
- 238000006243 chemical reaction Methods 0.000 claims description 2
- 229910052804 chromium Inorganic materials 0.000 claims description 2
- 239000011651 chromium Substances 0.000 claims description 2
- 229910017052 cobalt Inorganic materials 0.000 claims description 2
- 239000010941 cobalt Substances 0.000 claims description 2
- GUTLYIVDDKVIGB-UHFFFAOYSA-N cobalt atom Chemical compound [Co] GUTLYIVDDKVIGB-UHFFFAOYSA-N 0.000 claims description 2
- 229910052802 copper Inorganic materials 0.000 claims description 2
- 239000010949 copper Substances 0.000 claims description 2
- 230000007423 decrease Effects 0.000 claims description 2
- 230000007547 defect Effects 0.000 claims description 2
- 238000001035 drying Methods 0.000 claims description 2
- OGPBJKLSAFTDLK-UHFFFAOYSA-N europium atom Chemical compound [Eu] OGPBJKLSAFTDLK-UHFFFAOYSA-N 0.000 claims description 2
- 239000003063 flame retardant Substances 0.000 claims description 2
- 239000011521 glass Substances 0.000 claims description 2
- 150000004676 glycans Chemical class 0.000 claims description 2
- 229910052500 inorganic mineral Inorganic materials 0.000 claims description 2
- 229910052742 iron Inorganic materials 0.000 claims description 2
- 235000019388 lanolin Nutrition 0.000 claims description 2
- 229940039717 lanolin Drugs 0.000 claims description 2
- 239000000944 linseed oil Substances 0.000 claims description 2
- 235000021388 linseed oil Nutrition 0.000 claims description 2
- 239000000314 lubricant Substances 0.000 claims description 2
- QSHDDOUJBYECFT-UHFFFAOYSA-N mercury Chemical compound [Hg] QSHDDOUJBYECFT-UHFFFAOYSA-N 0.000 claims description 2
- 229910052753 mercury Inorganic materials 0.000 claims description 2
- 239000011707 mineral Substances 0.000 claims description 2
- 230000000116 mitigating effect Effects 0.000 claims description 2
- 239000003607 modifier Substances 0.000 claims description 2
- 229910052759 nickel Inorganic materials 0.000 claims description 2
- 239000003921 oil Substances 0.000 claims description 2
- 235000019198 oils Nutrition 0.000 claims description 2
- 230000003287 optical effect Effects 0.000 claims description 2
- 235000019809 paraffin wax Nutrition 0.000 claims description 2
- 235000019271 petrolatum Nutrition 0.000 claims description 2
- 239000012169 petroleum derived wax Substances 0.000 claims description 2
- 235000019381 petroleum wax Nutrition 0.000 claims description 2
- 239000000049 pigment Substances 0.000 claims description 2
- 239000004014 plasticizer Substances 0.000 claims description 2
- 229920001084 poly(chloroprene) Polymers 0.000 claims description 2
- 229920000435 poly(dimethylsiloxane) Polymers 0.000 claims description 2
- 229920003229 poly(methyl methacrylate) Polymers 0.000 claims description 2
- 229920000058 polyacrylate Polymers 0.000 claims description 2
- 229920002647 polyamide Polymers 0.000 claims description 2
- 229920000647 polyepoxide Polymers 0.000 claims description 2
- 229920000570 polyether Polymers 0.000 claims description 2
- 229920000573 polyethylene Polymers 0.000 claims description 2
- 229920000139 polyethylene terephthalate Polymers 0.000 claims description 2
- 239000005020 polyethylene terephthalate Substances 0.000 claims description 2
- 229920001721 polyimide Polymers 0.000 claims description 2
- 238000006116 polymerization reaction Methods 0.000 claims description 2
- 239000004926 polymethyl methacrylate Substances 0.000 claims description 2
- 229920001155 polypropylene Polymers 0.000 claims description 2
- 229920001282 polysaccharide Polymers 0.000 claims description 2
- 239000005017 polysaccharide Substances 0.000 claims description 2
- 229920001709 polysilazane Polymers 0.000 claims description 2
- 229920001296 polysiloxane Polymers 0.000 claims description 2
- 229920002223 polystyrene Polymers 0.000 claims description 2
- 239000004810 polytetrafluoroethylene Substances 0.000 claims description 2
- 229920001343 polytetrafluoroethylene Polymers 0.000 claims description 2
- 229920002635 polyurethane Polymers 0.000 claims description 2
- 239000004814 polyurethane Substances 0.000 claims description 2
- 229920002689 polyvinyl acetate Polymers 0.000 claims description 2
- 239000011118 polyvinyl acetate Substances 0.000 claims description 2
- 238000002459 porosimetry Methods 0.000 claims description 2
- 229910052913 potassium silicate Inorganic materials 0.000 claims description 2
- NNHHDJVEYQHLHG-UHFFFAOYSA-N potassium silicate Chemical compound [K+].[K+].[O-][Si]([O-])=O NNHHDJVEYQHLHG-UHFFFAOYSA-N 0.000 claims description 2
- 235000019353 potassium silicate Nutrition 0.000 claims description 2
- 230000001737 promoting effect Effects 0.000 claims description 2
- 239000002516 radical scavenger Substances 0.000 claims description 2
- 229910052761 rare earth metal Inorganic materials 0.000 claims description 2
- 230000009257 reactivity Effects 0.000 claims description 2
- 230000009467 reduction Effects 0.000 claims description 2
- 230000008439 repair process Effects 0.000 claims description 2
- 230000002940 repellent Effects 0.000 claims description 2
- 239000005871 repellent Substances 0.000 claims description 2
- 230000000979 retarding effect Effects 0.000 claims description 2
- 238000000926 separation method Methods 0.000 claims description 2
- 235000013874 shellac Nutrition 0.000 claims description 2
- 239000004208 shellac Substances 0.000 claims description 2
- ZLGIYFNHBLSMPS-ATJNOEHPSA-N shellac Chemical compound OCCCCCC(O)C(O)CCCCCCCC(O)=O.C1C23[C@H](C(O)=O)CCC2[C@](C)(CO)[C@@H]1C(C(O)=O)=C[C@@H]3O ZLGIYFNHBLSMPS-ATJNOEHPSA-N 0.000 claims description 2
- 229940113147 shellac Drugs 0.000 claims description 2
- 229910052710 silicon Inorganic materials 0.000 claims description 2
- 239000010703 silicon Substances 0.000 claims description 2
- 125000005625 siliconate group Chemical group 0.000 claims description 2
- 229910052709 silver Inorganic materials 0.000 claims description 2
- 239000004332 silver Substances 0.000 claims description 2
- 229910052911 sodium silicate Inorganic materials 0.000 claims description 2
- NTHWMYGWWRZVTN-UHFFFAOYSA-N sodium silicate Chemical compound [Na+].[Na+].[O-][Si]([O-])=O NTHWMYGWWRZVTN-UHFFFAOYSA-N 0.000 claims description 2
- 239000000126 substance Substances 0.000 claims description 2
- 229910052715 tantalum Inorganic materials 0.000 claims description 2
- GUVRBAGPIYLISA-UHFFFAOYSA-N tantalum atom Chemical compound [Ta] GUVRBAGPIYLISA-UHFFFAOYSA-N 0.000 claims description 2
- 229910052718 tin Inorganic materials 0.000 claims description 2
- 229910052719 titanium Inorganic materials 0.000 claims description 2
- 239000010936 titanium Substances 0.000 claims description 2
- 229910052723 transition metal Inorganic materials 0.000 claims description 2
- XTIIITNXEHRMQL-UHFFFAOYSA-N tripotassium methoxy(trioxido)silane Chemical compound [K+].[K+].[K+].CO[Si]([O-])([O-])[O-] XTIIITNXEHRMQL-UHFFFAOYSA-N 0.000 claims description 2
- XYRAEZLPSATLHH-UHFFFAOYSA-N trisodium methoxy(trioxido)silane Chemical compound [Na+].[Na+].[Na+].CO[Si]([O-])([O-])[O-] XYRAEZLPSATLHH-UHFFFAOYSA-N 0.000 claims description 2
- WFKWXMTUELFFGS-UHFFFAOYSA-N tungsten Chemical compound [W] WFKWXMTUELFFGS-UHFFFAOYSA-N 0.000 claims description 2
- 229910052721 tungsten Inorganic materials 0.000 claims description 2
- 239000010937 tungsten Substances 0.000 claims description 2
- 229910052720 vanadium Inorganic materials 0.000 claims description 2
- LEONUFNNVUYDNQ-UHFFFAOYSA-N vanadium atom Chemical compound [V] LEONUFNNVUYDNQ-UHFFFAOYSA-N 0.000 claims description 2
- 235000013311 vegetables Nutrition 0.000 claims description 2
- 239000008170 walnut oil Substances 0.000 claims description 2
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Chemical compound O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 claims description 2
- 239000002023 wood Substances 0.000 claims description 2
- 229910052725 zinc Inorganic materials 0.000 claims description 2
- 239000011701 zinc Substances 0.000 claims description 2
- 229910052726 zirconium Inorganic materials 0.000 claims description 2
- 150000004679 hydroxides Chemical class 0.000 claims 4
- 244000068988 Glycine max Species 0.000 claims 1
- 235000010469 Glycine max Nutrition 0.000 claims 1
- 244000043261 Hevea brasiliensis Species 0.000 claims 1
- BHEPBYXIRTUNPN-UHFFFAOYSA-N hydridophosphorus(.) (triplet) Chemical compound [PH] BHEPBYXIRTUNPN-UHFFFAOYSA-N 0.000 claims 1
- 229920003052 natural elastomer Polymers 0.000 claims 1
- 229920001194 natural rubber Polymers 0.000 claims 1
- 229920000915 polyvinyl chloride Polymers 0.000 claims 1
- 239000004800 polyvinyl chloride Substances 0.000 claims 1
- 150000004756 silanes Chemical class 0.000 claims 1
- 150000004760 silicates Chemical class 0.000 claims 1
- WNROFYMDJYEPJX-UHFFFAOYSA-K aluminium hydroxide Chemical compound [OH-].[OH-].[OH-].[Al+3] WNROFYMDJYEPJX-UHFFFAOYSA-K 0.000 description 2
- BPQQTUXANYXVAA-UHFFFAOYSA-N Orthosilicate Chemical compound [O-][Si]([O-])([O-])[O-] BPQQTUXANYXVAA-UHFFFAOYSA-N 0.000 description 1
- OAICVXFJPJFONN-UHFFFAOYSA-N Phosphorus Chemical compound [P] OAICVXFJPJFONN-UHFFFAOYSA-N 0.000 description 1
- BLRPTPMANUNPDV-UHFFFAOYSA-N Silane Chemical compound [SiH4] BLRPTPMANUNPDV-UHFFFAOYSA-N 0.000 description 1
- 150000001342 alkaline earth metals Chemical class 0.000 description 1
- 229920001206 natural gum Polymers 0.000 description 1
- 239000011574 phosphorus Substances 0.000 description 1
- 229910052698 phosphorus Inorganic materials 0.000 description 1
- 229910000077 silane Inorganic materials 0.000 description 1
- 239000012180 soy wax Substances 0.000 description 1
- 229920002554 vinyl polymer Polymers 0.000 description 1
Description
本明細書で引用するすべての刊行物、特許、及び特許出願は、すべての目的のために、それぞれの個別の刊行物、特許、または特許出願を、参照により、あたかも具体的かつ個別に示したものと同然に、参照により、それらの全内容を本明細書で援用する。
本発明の具体的態様は以下のとおりである。
[態様1]
(i)多孔質セラミック材料中に含浸されたポリマー、ワックス、及び/または樹脂を含む複合材料であって、前記多孔質セラミック材料が、セラミックの相互連結したネットワーク、及び少なくとも部分的に、前記ポリマー、ワックス、及び/または樹脂が充填されたアクセス可能な細孔容積を含む前記複合材料と、
(ii)基材と
を含み、
前記複合材料が前記基材と接触している組成物。
[態様2]
前記基材及び前記セラミック材料がそれぞれ一次金属を含み、前記セラミック材料中の前記一次金属が前記基材中の前記一次金属とは異なる、態様1に記載の組成物。
[態様3]
前記複合材料の厚さが約1マイクロメートル~約100マイクロメートルである、態様1に記載の組成物。
[態様4]
前記複合材料中の総セラミック含有量の少なくとも約20質量%が相互連結している、態様1に記載の組成物。
[態様5]
セラミック材料の相互連結したネットワークが約10平方マイクロメートルよりも大きい、態様1に記載の組成物。
[態様6]
前記複合材料が複数のセラミック材料の相互連結したネットワークを含む、態様1に記載の組成物。
[態様7]
前記複数のセラミック材料の相互連結したネットワーク内の1つのセラミック材料の相互連結したネットワークの面積の中央値が約10平方マイクロメートルよりも大きい、態様6に記載の組成物。
[態様8]
前記セラミック材料が、希土類元素、遷移金属元素、アルカリ土類金属元素、またはアルミニウムを含む、態様1~7のいずれか1項に記載の組成物。
[態様9]
前記セラミック材料が、酸化物、水酸化物、及び/または層状複水酸化物を含む、態様1~7のいずれか1項に記載の組成物。
[態様10]
前記酸化物、水酸化物、及び/または層状複水酸化物が、鉄、アルミニウム、マグネシウム、セリウム、亜鉛、マンガン、チタン、クロム、ニッケル、コバルト、銅、銀、タンタル、タングステン、ケイ素、リン、スズ、バナジウム、ジルコニウム、カルシウム、バリウム、またはユーロピウムを含む、態様9に記載の組成物。
[態様11]
前記基材が、アルミニウム合金、鋼合金、ニッケル合金、チタン合金、ポリマー、セルロース系材料、多糖、木材、綿、またはガラスを含む、態様1~7のいずれか1項に記載の組成物。
[態様12]
前記ポリマー、ワックス、及び/または樹脂が、同一の基材上に前記ポリマー、樹脂、及び/またはワックスを含まない同一のセラミック材料と比較して、向上した硬度、弾性、粘弾性、接着性、熱特性、審美的外観、撥液性、及び耐食性から選択される1種以上の機能的特性を付与する、態様1~7のいずれか1項に記載の組成物。
[態様13]
前記セラミック材料が結合剤不含セラミック材料である、態様1~7のいずれか1項に記載の組成物。
[態様14]
前記ポリマー、ワックス、及び/または樹脂が、桐油、亜麻仁油、胡桃油、天然ゴム、セルロース、またはキチン由来のポリマーを含む、態様1~7のいずれか1項に記載の組成物。
[態様15]
前記ポリマー、ワックス、及び/または樹脂が、ポリエチレン、ポリプロピレン、ポリスチレン、ポリテトラフルオロエチレン、ポリエチレンテレフタラート、ポリアクリラート、ポリ(メチルメタクリラート)、ポリ酢酸ビニル、ポリエーテル、ポリクロロプレン、ポリ(塩化ビニル)、ポリウレタン、ポリアミド、ポリイミド、シリコーン、ポリ(ジメチルシロキサン)、またはポリエポキシドポリマーを含む、態様1~7のいずれか1項に記載の組成物。
[態様16]
前記ポリマー、ワックス、及び/または樹脂が、シラン、ケイ酸塩、シリコナート、ポリシラザン、オルガノトリエトキシシラン、またはオルガノトリメトキシシランを含む、態様1~7のいずれか1項に記載の組成物。
[態様17]
前記ポリマー、ワックス、及び/または樹脂が、ケイ酸カリウムメチル、ケイ酸ナトリウム、ケイ酸カリウム、またはケイ酸ナトリウムメチルを含む、態様16に記載の組成物。
[態様18]
前記ポリマー、ワックス、及び/または樹脂が、石油ワックス、動物由来ワックス、植物由来ワックス、または鉱物由来ワックスを含む、態様1~7のいずれか1項に記載の組成物。
[態様19]
前記ポリマー、ワックス、及び/または樹脂が、パラフィンワックス、ミツロウ、ラノリン、シェラック、パームワックス、カルナウバワックス、大豆ワックス、セレシン、またはモンタンを含む、態様18に記載の組成物。
[態様20]
前記ポリマー、ワックス、及び/または樹脂が、潤滑剤、可塑剤、難燃剤、色素、UV安定剤、フリーラジカルスカベンジャー、及び架橋剤から選択される1種以上のさらなる添加剤を含む、態様1~7のいずれか1項に記載の組成物。
[態様21]
前記添加剤が、粘度、可撓性、可燃性、色彩、UV安定性、化学反応性、及び架橋度から選択される1種以上の特性を前記複合材料に付与する、態様20に記載の組成物。
[態様22]
水銀ポロシメトリー試験によって測定して、前記アクセス可能な細孔容積の約1%超に、前記ポリマー、ワックス、及び/または樹脂が充填されている、態様1~7のいずれか1項に記載の組成物。
[態様23]
前記ポリマー、樹脂、及び/またはワックスの厚さが、前記セラミック材料の厚さの約1.5倍未満である、態様1~7のいずれか1項に記載の組成物。
[態様24]
前記セラミック材料が前記ポリマー、ワックス、及び/または樹脂材料と相互作用し、それによって、前記ポリマー、ワックス、及び/もしくは樹脂の架橋速度ならびに/または架橋度が、前記ポリマー、ワックス、及び/もしくは樹脂が、前記セラミック材料を含まない同一の基材に直接塗布される場合の架橋速度ならびに/または架橋度と比較して増加する、態様1~7のいずれか1項に記載の組成物。
[態様25]
前記セラミック材料が前記ポリマー、ワックス、及び/または樹脂材料と相互作用し、それによって、前記ポリマー、ワックス、及び/または樹脂材料の結晶化度が、前記ポリマー、ワックス、及び/または樹脂材料が、前記セラミック材料を含まない同一の基材に直接塗布される場合の結晶化度と比較して増加する、態様1~7のいずれか1項に記載の組成物。
[態様26]
前記セラミック材料が前記ポリマー、ワックス、及び/または樹脂材料と相互作用し、それによって、前記ポリマー、ワックス、及び/または樹脂材料のUV分解の速度が、前記セラミック材料を含まない同一の基材に直接塗布された前記ポリマー、ワックス、及び/または樹脂材料のUV分解の速度と比較して低下する、態様1~7のいずれか1項に記載の組成物。
[態様27]
前記セラミック材料がマグネシウム、マンガン、酸化亜鉛、または酸化アルミニウムもしくは水酸化アルミニウムを含み、前記ポリマー、ワックス、及び/または樹脂が桐油またはパラフィンなどの乾性油を含む、態様1~7のいずれか1項に記載の組成物。
[態様28]
前記セラミック材料がマグネシウム、マンガン、酸化亜鉛、または酸化アルミニウムもしくは水酸化アルミニウムを含み、前記ポリマー、ワックス、及び/または樹脂が前記セラミック材料と化学的に反応して、前記ポリマー、ワックス、及び/または樹脂の特性を改変する、態様1~7のいずれか1項に記載の組成物。
[態様29]
前記ポリマー、ワックス、及び/または樹脂の前記特性を改変するための化学反応が、架橋、硬化、及び/または重合を含む、態様28に記載の組成物。
[態様30]
前記基材の腐食に対する保護;接着性及び/または表面汚れに対する耐久性改質剤;接着の促進または遅延の構成;表面の触覚改質;撥液用途;光学特性の改質;硬度、弾性、及び粘弾性などの機械的改質;表面ならびに引っかき傷の自己修復及び修復の目的;分離用途;電気的特性の改質または電気特性用途;氷、コンデンセート、及び霜の軽減ならびに/または改変;表面均一性;欠陥の低減;ならびに審美的特性から選択される1種以上の機能的特性を付与するために、前記基材に前記複合材料が塗布され、
同一の基材上の、前記ポリマー、樹脂、及び/もしくはワックスを含まない同一の多孔質セラミック材料と比較して、または前記ポリマー、樹脂、及び/もしくはワックスが直接塗布された同一の基材と比較して、前記機能的特性が改善されるか、あるいはその程度がより大きい、態様1~7のいずれか1項に記載の組成物。
[態様31]
前記複合材料が、前記複合材料の総容積の約40%を超えるセラミック容積濃度を含む、態様1~7のいずれか1項に記載の組成物。
All publications, patents, and patent applications cited herein are, for all purposes, referred to as if each individual publication, patent, or patent application were specifically and individually indicated by reference. The entire contents thereof are hereby incorporated by reference as if by reference.
Specific embodiments of the present invention are as follows.
[Aspect 1]
(i) a composite material comprising a polymer, wax, and/or resin impregnated in a porous ceramic material, wherein said porous ceramic material comprises an interconnected network of ceramics and, at least in part, said polymer said composite material comprising accessible pore volumes filled with , wax, and/or resin;
(ii) base material and
including;
A composition in which the composite material is in contact with the substrate.
[Aspect 2]
2. The composition of claim 1, wherein the substrate and the ceramic material each include a primary metal, and the primary metal in the ceramic material is different from the primary metal in the substrate.
[Aspect 3]
The composition of embodiment 1, wherein the composite material has a thickness of about 1 micrometer to about 100 micrometers.
[Aspect 4]
The composition of embodiment 1, wherein at least about 20% by weight of the total ceramic content in the composite material is interconnected.
[Aspect 5]
The composition of embodiment 1, wherein the interconnected network of ceramic materials is larger than about 10 square micrometers.
[Aspect 6]
A composition according to aspect 1, wherein the composite material comprises an interconnected network of a plurality of ceramic materials.
[Aspect 7]
7. The composition of embodiment 6, wherein the median area of an interconnected network of ceramic materials in the plurality of interconnected networks of ceramic materials is greater than about 10 square micrometers.
[Aspect 8]
A composition according to any one of aspects 1 to 7, wherein the ceramic material comprises a rare earth element, a transition metal element, an alkaline earth metal element, or aluminum.
[Aspect 9]
Composition according to any one of aspects 1 to 7, wherein the ceramic material comprises an oxide, a hydroxide and/or a layered double hydroxide.
[Aspect 10]
The oxide, hydroxide, and/or layered double hydroxide may be iron, aluminum, magnesium, cerium, zinc, manganese, titanium, chromium, nickel, cobalt, copper, silver, tantalum, tungsten, silicon, phosphorus, A composition according to aspect 9, comprising tin, vanadium, zirconium, calcium, barium, or europium.
[Aspect 11]
A composition according to any one of aspects 1 to 7, wherein the substrate comprises an aluminum alloy, a steel alloy, a nickel alloy, a titanium alloy, a polymer, a cellulosic material, a polysaccharide, wood, cotton, or glass.
[Aspect 12]
said polymer, wax and/or resin has improved hardness, elasticity, viscoelasticity, adhesion on the same substrate compared to the same ceramic material without said polymer, resin and/or wax; A composition according to any one of aspects 1 to 7, which imparts one or more functional properties selected from thermal properties, aesthetic appearance, liquid repellency, and corrosion resistance.
[Aspect 13]
A composition according to any one of aspects 1 to 7, wherein the ceramic material is a binder-free ceramic material.
[Aspect 14]
Composition according to any one of aspects 1 to 7, wherein the polymer, wax and/or resin comprises a polymer derived from tung oil, linseed oil, walnut oil, natural gum, cellulose or chitin.
[Aspect 15]
The polymer, wax, and/or resin may be polyethylene, polypropylene, polystyrene, polytetrafluoroethylene, polyethylene terephthalate, polyacrylate, poly(methyl methacrylate), polyvinyl acetate, polyether, polychloroprene, poly(chlorinated) 8. The composition according to any one of aspects 1 to 7, comprising a poly(vinyl), polyurethane, polyamide, polyimide, silicone, poly(dimethylsiloxane), or polyepoxide polymer.
[Aspect 16]
A composition according to any one of aspects 1 to 7, wherein the polymer, wax, and/or resin comprises a silane, a silicate, a siliconate, a polysilazane, an organotriethoxysilane, or an organotrimethoxysilane.
[Aspect 17]
17. The composition of embodiment 16, wherein the polymer, wax, and/or resin comprises potassium methyl silicate, sodium silicate, potassium silicate, or sodium methyl silicate.
[Aspect 18]
A composition according to any one of aspects 1 to 7, wherein the polymer, wax, and/or resin comprises a petroleum wax, an animal-derived wax, a vegetable-derived wax, or a mineral-derived wax.
[Aspect 19]
19. The composition of embodiment 18, wherein the polymer, wax, and/or resin comprises paraffin wax, beeswax, lanolin, shellac, palm wax, carnauba wax, soy wax, ceresin, or montan.
[Aspect 20]
Embodiments 1 to 2, wherein the polymer, wax, and/or resin comprises one or more further additives selected from lubricants, plasticizers, flame retardants, pigments, UV stabilizers, free radical scavengers, and crosslinkers. 7. The composition according to any one of 7.
[Aspect 21]
A composition according to aspect 20, wherein the additive imparts to the composite material one or more properties selected from viscosity, flexibility, flammability, color, UV stability, chemical reactivity, and degree of crosslinking. thing.
[Aspect 22]
8. According to any one of embodiments 1 to 7, more than about 1% of the accessible pore volume is filled with the polymer, wax, and/or resin, as measured by mercury porosimetry testing. Composition.
[Aspect 23]
8. The composition of any one of aspects 1-7, wherein the thickness of the polymer, resin, and/or wax is less than about 1.5 times the thickness of the ceramic material.
[Aspect 24]
The ceramic material interacts with the polymer, wax, and/or resin material such that the crosslinking rate and/or degree of crosslinking of the polymer, wax, and/or resin is influenced by the polymer, wax, and/or resin. The composition according to any one of the preceding aspects, wherein the composition has an increased crosslinking rate and/or degree of crosslinking when applied directly to the same substrate without said ceramic material.
[Aspect 25]
The ceramic material interacts with the polymer, wax and/or resin material such that the crystallinity of the polymer, wax and/or resin material is A composition according to any one of aspects 1 to 7, which has an increased degree of crystallinity when applied directly to the same substrate without said ceramic material.
[Aspect 26]
The ceramic material interacts with the polymer, wax, and/or resin material such that the rate of UV degradation of the polymer, wax, and/or resin material decreases on the same substrate without the ceramic material. Composition according to any one of aspects 1 to 7, wherein the rate of UV degradation is reduced compared to the rate of UV degradation of the directly applied polymer, wax and/or resin material.
[Aspect 27]
Any one of embodiments 1 to 7, wherein the ceramic material comprises magnesium, manganese, zinc oxide, or aluminum oxide or aluminum hydroxide, and the polymer, wax, and/or resin comprises a drying oil, such as tung oil or paraffin. The composition described in .
[Aspect 28]
The ceramic material comprises magnesium, manganese, zinc oxide, or aluminum oxide or aluminum hydroxide, and the polymer, wax, and/or resin is chemically reacted with the ceramic material to form the polymer, wax, and/or A composition according to any one of aspects 1 to 7, which modifies the properties of the resin.
[Aspect 29]
29. The composition of embodiment 28, wherein the chemical reaction to modify the properties of the polymer, wax, and/or resin comprises crosslinking, curing, and/or polymerization.
[Aspect 30]
protection against corrosion of the substrate; durability modifiers against adhesion and/or surface fouling; configurations for promoting or retarding adhesion; tactile modification of surfaces; liquid repellent applications; modification of optical properties; hardness, elasticity, mechanical modification such as and viscoelasticity; self-healing and repair purposes of surfaces and scratches; separation applications; modification of electrical properties or electrical property applications; ice, condensate, and frost mitigation and/or modification; surfaces the composite material is applied to the substrate to impart one or more functional properties selected from uniformity; reduction of defects; and aesthetic properties;
Compared to the same porous ceramic material without said polymer, resin and/or wax on the same substrate or with the same substrate directly applied with said polymer, resin and/or wax. Composition according to any one of aspects 1 to 7, wherein, in comparison, said functional properties are improved or to a greater extent.
[Aspect 31]
The composition of any one of aspects 1-7, wherein the composite material comprises a ceramic volume concentration greater than about 40% of the total volume of the composite material.
Claims (15)
(ii)基材と
を含み、
前記複合材料が前記基材と接触している組成物。 (i) a composite material comprising a polymer, wax, and/or resin impregnated in a porous ceramic material, wherein said porous ceramic material comprises an interconnected network of ceramics and, at least in part, said polymer said composite material comprising accessible pore volumes filled with , wax, and/or resin;
(ii) a base material;
A composition in which the composite material is in contact with the substrate.
(ii)前記複合材料の厚さが約1マイクロメートル~約100マイクロメートルである、又は
(iii)前記複合材料中の総セラミック含有量の少なくとも約20質量%が相互連結している、又は
(iv)セラミック材料の相互連結したネットワークが約10平方マイクロメートルよりも大きい、
請求項1に記載の組成物。 (i) the substrate and the ceramic material each include a primary metal, and the primary metal in the ceramic material is different from the primary metal in the substrate; or
(ii) the composite material has a thickness of about 1 micrometer to about 100 micrometers, or
(iii) at least about 20% by weight of the total ceramic content in the composite material is interconnected; or
(iv) the interconnected network of ceramic materials is larger than about 10 square micrometers;
A composition according to claim 1.
任意選択で、前記複数のセラミック材料の相互連結したネットワーク内の1つのセラミック材料の相互連結したネットワークの面積の中央値が約10平方マイクロメートルよりも大きい、請求項1に記載の組成物。 the composite material includes an interconnected network of a plurality of ceramic materials;
Optionally, the composition of claim 1, wherein the median area of one interconnected network of ceramic materials within the plurality of interconnected networks of ceramic materials is greater than about 10 square micrometers.
(i)希土類元素、遷移金属元素、アルカリ土類金属元素、またはアルミニウムを含む、又は
(ii)酸化物、水酸化物、及び/または層状複水酸化物を含み、任意選択で、前記酸化物、水酸化物、及び/または層状複水酸化物が、鉄、アルミニウム、マグネシウム、セリウム、亜鉛、マンガン、チタン、クロム、ニッケル、コバルト、銅、銀、タンタル、タングステン、ケイ素、リン、スズ、バナジウム、ジルコニウム、カルシウム、バリウム、またはユーロピウムを含む、
請求項1~3のいずれか1項に記載の組成物。 The ceramic material is
(i) Contains rare earth elements, transition metal elements, alkaline earth metal elements, or aluminum; or
(ii) oxides, hydroxides, and/or layered double hydroxides, optionally said oxides, hydroxides, and/or layered double hydroxides containing iron, aluminum, magnesium, cerium; , zinc, manganese, titanium, chromium, nickel, cobalt, copper, silver, tantalum, tungsten, silicon, phosphorous, tin, vanadium, zirconium, calcium, barium, or europium,
The composition according to any one of claims 1 to 3 .
(i)同一の基材上に前記ポリマー、樹脂、及び/またはワックスを含まない同一のセラミック材料と比較して、向上した硬度、弾性、粘弾性、接着性、熱特性、審美的外観、撥液性、及び耐食性から選択される1種以上の機能的特性を付与する、又は
(ii)桐油、亜麻仁油、胡桃油、天然ゴム、セルロース、またはキチン由来のポリマーを含む、又は
(iii)ポリエチレン、ポリプロピレン、ポリスチレン、ポリテトラフルオロエチレン、ポリエチレンテレフタラート、ポリアクリラート、ポリ(メチルメタクリラート)、ポリ酢酸ビニル、ポリエーテル、ポリクロロプレン、ポリ(塩化ビニル)、ポリウレタン、ポリアミド、ポリイミド、シリコーン、ポリ(ジメチルシロキサン)、またはポリエポキシドポリマーを含む、
請求項1~3のいずれか1項に記載の組成物。 The polymer, wax, and/or resin is
(i) improved hardness, elasticity, viscoelasticity, adhesion, thermal properties, aesthetic appearance, and repellency compared to the same ceramic material without said polymers, resins, and/or waxes on the same substrate; imparting one or more functional properties selected from liquid properties and corrosion resistance, or
(ii) contains polymers derived from tung oil, linseed oil, walnut oil, natural rubber, cellulose, or chitin; or
(iii) polyethylene, polypropylene, polystyrene, polytetrafluoroethylene, polyethylene terephthalate, polyacrylate, poly(methyl methacrylate), polyvinyl acetate, polyether, polychloroprene, poly(vinyl chloride), polyurethane, polyamide, polyimide , silicone, poly(dimethylsiloxane), or polyepoxide polymers,
The composition according to any one of claims 1 to 3 .
前記添加剤が、任意選択で、粘度、可撓性、可燃性、色彩、UV安定性、化学反応性、及び架橋度から選択される1種以上の特性を前記複合材料に付与する、
請求項1~3のいずれか1項に記載の組成物。 the polymers, waxes and/or resins comprising one or more further additives selected from lubricants, plasticizers, flame retardants, pigments, UV stabilizers, free radical scavengers, and crosslinkers;
the additive optionally imparts to the composite material one or more properties selected from viscosity, flexibility, flammability, color, UV stability, chemical reactivity, and degree of crosslinking;
The composition according to any one of claims 1 to 3 .
(ii)前記ポリマー、樹脂、及び/またはワックスの厚さが、前記セラミック材料の厚さの約1.5倍未満である、
請求項1~3のいずれか1項に記載の組成物。 (i) more than about 1% of the accessible pore volume is filled with the polymer, wax, and/or resin, as determined by mercury porosimetry testing; or
(ii) the thickness of the polymer, resin, and/or wax is less than about 1.5 times the thickness of the ceramic material;
The composition according to any one of claims 1 to 3 .
(i)前記ポリマー、ワックス、及び/もしくは樹脂の架橋速度ならびに/または架橋度が、前記ポリマー、ワックス、及び/もしくは樹脂が、前記セラミック材料を含まない同一の基材に直接塗布される場合の架橋速度ならびに/または架橋度と比較して増加する、又は
(ii)前記ポリマー、ワックス、及び/または樹脂材料の結晶化度が、前記ポリマー、ワックス、及び/または樹脂材料が、前記セラミック材料を含まない同一の基材に直接塗布される場合の結晶化度と比較して増加する、又は
(iii)前記ポリマー、ワックス、及び/または樹脂材料のUV分解の速度が、前記セラミック材料を含まない同一の基材に直接塗布された前記ポリマー、ワックス、及び/または樹脂材料のUV分解の速度と比較して低下する、
請求項1~3のいずれか1項に記載の組成物。 The ceramic material interacts with the polymer, wax and/or resin material, thereby
(i) the crosslinking rate and/or degree of crosslinking of said polymer, wax and/or resin when said polymer, wax and/or resin is applied directly to the same substrate without said ceramic material; increases compared to crosslinking rate and/or degree of crosslinking, or
(ii) the degree of crystallinity of said polymer, wax and/or resin material is crystallized when said polymer, wax and/or resin material is applied directly to the same substrate free of said ceramic material; increase compared to the degree, or
(iii) the rate of UV degradation of said polymer, wax and/or resin material is the rate of UV degradation of said polymer, wax and/or resin material applied directly to the same substrate without said ceramic material; decreases compared to
The composition according to any one of claims 1 to 3 .
(i)桐油またはパラフィンなどの乾性油を含む、又は
(ii)前記セラミック材料と化学的に反応して、前記ポリマー、ワックス、及び/または樹脂の特性を改変し、任意選択で、前記ポリマー、ワックス、及び/または樹脂の前記特性を改変するための化学反応が、架橋、硬化、及び/または重合を含む、
請求項1~3のいずれか1項に記載の組成物。 The ceramic material contains magnesium, manganese, zinc oxide, or aluminum oxide or hydroxide, and the polymer, wax, and/or resin
(i) contains a drying oil such as tung oil or paraffin; or
(ii) chemically reacting with said ceramic material to modify the properties of said polymer, wax and/or resin, optionally for modifying said properties of said polymer, wax and/or resin; the chemical reaction includes crosslinking, curing, and/or polymerization;
The composition according to any one of claims 1 to 3 .
同一の基材上の、前記ポリマー、樹脂、及び/もしくはワックスを含まない同一の多孔質セラミック材料と比較して、または前記ポリマー、樹脂、及び/もしくはワックスが直接塗布された同一の基材と比較して、前記機能的特性が改善されるか、あるいはその程度がより大きい、請求項1~3のいずれか1項に記載の組成物。 protection against corrosion of the substrate; durability modifiers against adhesion and/or surface fouling; configurations for promoting or retarding adhesion; tactile modification of surfaces; liquid repellent applications; modification of optical properties; hardness, elasticity, mechanical modification such as and viscoelasticity; self-healing and repair purposes of surfaces and scratches; separation applications; modification of electrical properties or electrical property applications; ice, condensate, and frost mitigation and/or modification; surfaces the composite material is applied to the substrate to impart one or more functional properties selected from uniformity; reduction of defects; and aesthetic properties;
Compared to the same porous ceramic material without said polymer, resin and/or wax on the same substrate or with the same substrate directly applied with said polymer, resin and/or wax. Composition according to any one of claims 1 to 3 , wherein, in comparison, the functional properties are improved or to a greater extent.
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US202062989150P | 2020-03-13 | 2020-03-13 | |
US202062989092P | 2020-03-13 | 2020-03-13 | |
US62/989,092 | 2020-03-13 | ||
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US63/039,965 | 2020-06-16 | ||
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CN (5) | CN115087708A (en) |
MX (1) | MX2022007226A (en) |
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2020
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- 2020-12-11 WO PCT/US2020/064395 patent/WO2021119372A1/en unknown
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- 2020-12-11 EP EP20898487.2A patent/EP4073019A4/en active Pending
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