JP2004155693A - Insecticidal, acaricidal, nematicidal, fungicidal or bactericidal composition, and method for controlling disease and insect pest - Google Patents

Insecticidal, acaricidal, nematicidal, fungicidal or bactericidal composition, and method for controlling disease and insect pest Download PDF

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JP2004155693A
JP2004155693A JP2002322041A JP2002322041A JP2004155693A JP 2004155693 A JP2004155693 A JP 2004155693A JP 2002322041 A JP2002322041 A JP 2002322041A JP 2002322041 A JP2002322041 A JP 2002322041A JP 2004155693 A JP2004155693 A JP 2004155693A
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Kohei Inoue
Toshiro Miyake
敏郎 三宅
公平 井上
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Nissan Chem Ind Ltd
日産化学工業株式会社
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    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02ATECHNOLOGIES FOR ADAPTATION TO CLIMATE CHANGE
    • Y02A50/00TECHNOLOGIES FOR ADAPTATION TO CLIMATE CHANGE in human health protection
    • Y02A50/30Against vector-borne diseases, e.g. mosquito-borne, fly-borne, tick-borne or waterborne diseases whose impact is exacerbated by climate change
    • Y02A50/31Vector control
    • Y02A50/32Vector control using natural substances as pesticides or insecticides, for fighting the disease vector
    • Y02A50/332Vector control using natural substances as pesticides or insecticides, for fighting the disease vector characterised by the natural substance
    • Y02A50/357Substances of mineral origin
    • Y02A50/358Sulfur

Abstract

<P>PROBLEM TO BE SOLVED: To obtain a new insecticidal, acaricidal, nematicidal, fungicidal or bactericidal composition and to provide a method for controlling diseases and insect pests. <P>SOLUTION: The insecticidal, acaricidal, nematicidal, fungicidal or bactericidal composition comprises one or more kinds of acrylonitrile compounds represented by formula (1) [A is a specific heterocyclic group which may be substituted with a specified group; B is H, a 2-4C haloalkyl, tetrahydropyranyl, or the like; G is H, a halogen, a 2-6C alkyl, or the like] and one or more kinds selected from a specific insecticidal, acaricidal, nematicidal, fungicidal and bactericidal compounds. The method for controlling diseases and insect pests comprises treatment with one or more kinds of the acrylonitrile compounds represented by formula (1) and one or more kinds selected from the specific insecticidal, acaricidal, nematicidal, fungicidal and bactericidal compounds simultaneously or adjacently. <P>COPYRIGHT: (C)2004,JPO

Description

【0001】 [0001]
【発明の属する技術分野】 BACKGROUND OF THE INVENTION
本発明は、アクリロニトリル化合物と、公知の殺虫剤、殺ダニ剤、殺線虫剤、殺菌剤又は殺バクテリア剤の有効成分化合物とを混合してなることを特徴とする病害虫防除剤に関するものである。 The present invention and acrylonitrile compounds, known insecticides, acaricides, nematicides, relates pest control agent characterized by comprising a mixture of the active ingredient compound of the fungicides or bactericides .
【0002】 [0002]
【従来の技術】 BACKGROUND OF THE INVENTION
アクリロニトリル誘導体が、農薬又は水中生物付着防止剤として使用されることが知られている(例えば、特許文献1参照。)。 Acrylonitrile derivatives have been known to be used as a pesticide or water anti-biofouling agents (e.g., see Patent Document 1.).
【0003】 [0003]
また、アクリロニトリル誘導体と公知の殺虫剤、殺ダニ剤、殺菌剤とを含有する組成物が知られている(例えば、特許文献2参照。)。 Also, an acrylonitrile derivative with known insecticides, acaricides composition containing a disinfectant is known (for example, see Patent Document 2.).
【0004】 [0004]
【特許文献1】 [Patent Document 1]
国際公開第97/040009号パンフレット【0005】 Pamphlet No. WO 97/040009 [0005]
【特許文献2】 [Patent Document 2]
特開平11−124306号公報【0006】 Japanese Unexamined Patent Publication No. 11-124306 [0006]
【発明が解決しようとする課題】 [Problems that the Invention is to Solve
今日、農園芸病害虫、森林病害虫、あるいは衛生病害虫等各種病害虫の防除を目的とする殺虫・殺ダニ・殺菌剤の開発が広く進められ、多種多様な薬剤が実用に供されている。 Today, agricultural and horticultural pests, forest pests or control the development of insecticidal and acaricidal, Fungicide for the purpose of hygienic pests such as various pest is advanced wide, a wide variety of drugs have been put to practical use. しかしながら、近年、こうした薬剤の長年にわたる使用により害虫が殺虫剤抵抗性を、また病原菌が殺菌剤耐性を獲得した結果、従来の薬剤による防除が困難となる場面が増えてきている。 However, in recent years, the longstanding pests insecticide resistance by the use of such agents, also results pathogens have acquired fungicide resistance, control by the conventional drugs has been increasing scene difficult. またこうした薬剤の一部は毒性が高く、あるものは環境中に長期に残留することにより生態系を撹乱しつつある。 Also some such agents are highly toxic, some are becoming disrupting the ecosystem by remaining long in the environment. よって、高度な病害虫防除効果を有するだけではなく、低毒性であり且つ低残留性の新規な薬剤の開発が常に期待されている。 Thus, not only it has a high degree of pest control effect, the development of low toxicity and is and low residual of novel agents have always been expected.
【0007】 [0007]
しかしその一方、生物群としての昆虫や病原菌の多様性、その加害様式、加害場面の多様性を考えれば、これら新規の薬剤、あるいは既存の公知薬剤を単独で使用するだけでは、全ての防除場面で全ての病害虫を有効に防除することははなはだ難しい。 However while the diversity of insects and pathogens as taxa, the perpetrator manner, given the diversity of offending scene, only use these new agents, or the existing known drugs alone, all control scenes it is woefully difficult to effectively control all the pests in. そこで、複数の殺虫、殺ダニ、殺線虫、殺菌または殺バクテリア剤を適切に組み合わせてより高い防除効力を誘導し、防除困難な有害生物を防除する新たな方法もまた、強く要望されるに至っている。 Therefore, a plurality of insecticidal, acaricidal, nematocidal, an appropriate combination of bactericidal or bactericides induced higher control effect, also new methods for controlling control difficult pests also to be strongly desired It has come.
【0008】 [0008]
【課題を解決するための手段】 In order to solve the problems]
本発明者らは、このような状況に鑑み、優れた防除活性を示し、かつ哺乳動物、魚類および天敵等の有用生物に対して悪影響の少ない病害虫防除剤を開発する為に鋭意研究を続けた結果、以下の式(1)で表されるアクリロニトリル化合物と、公知の殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア化合物を含有する殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア組成物が、単独の使用からは予測し得ない優れた相乗的殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア効果を奏することを見いだし、本発明を完成した。 The present inventors, in view of such circumstances, continued exhibits excellent control activity, and mammals, extensive studies in order to develop a small pest control agent having adverse effect on useful organisms such as fish and natural enemies result, acrylonitrile compound represented by the following formula (1), known insecticidal, acaricidal, nematocidal, insecticidal containing sterilization or bactericidal compounds, acaricidal, nematicidal, fungicidal or bactericidal composition but found excellent synergistic insecticidally not be predicted from the use of a single, acaricidal, nematicidal, that exhibits the sterilization, bactericidal effect, and have completed the present invention.
【0009】 [0009]
即ち、本発明は下記〔1〕又は〔2〕の組成物(以下、本発明組成物と称する。)、及び〔3〕〜〔6〕の防除方法(以下、本発明方法と称する。)に関するものである。 That is, the present invention is a composition of the following [1] or [2] (hereinafter, referred to as the present invention composition.), And [3] The method for controlling to [6] relates (hereinafter, the present invention method referred to.) it is intended.
【0010】 [0010]
〔1〕 以下の式(1)で表されるアクリロニトリル化合物の1種以上と、以下の化合物群Aより選ばれる化合物の1種以上を含有する殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア組成物。 [1] one or more of acrylonitrile compounds represented by the following formula (1) and, insecticide containing one or more compound selected from the following groups of compounds A, acaricidal, nematicidal, fungicidal or bactericidal Composition.
【0011】 [0011]
式(1): Equation (1):
【0012】 [0012]
【化7】 [Omitted]
【0013】 [0013]
[式中、 Aは、 [In the formula, A,
【0014】 [0014]
【化8】 [Of 8]
【0015】 [0015]
【化9】 [Omitted]
【0016】 [0016]
【化10】 [Of 10]
【0017】 [0017]
【化11】 [Of 11]
【0018】 [0018]
【化12】 [Of 12]
【0019】 [0019]
であり、 It is in,
Bは、H、CR 、CHR 、C 〜C ハロアルキル、テトラヒドロピラニル、Si(CH 、SO Re、SO NHRb、SO NRaRb、C(S)NHRb、C(S)NRaRb、C(O)Rf、P(O)RgRh、P(S)RgRh、アルカリ金属、アルカリ土類金属またはNHRiRjRkであり、Gは、H、ハロゲン、C 〜C アルキル、Rcで置換されたC 〜C アルキル、C 〜C ハロアルキル、C 〜C アルキルで置換されていてもよいC 〜C シクロアルキル、C 〜C アルコキシ、C 〜C アルケニルオキシ、C 〜C アルキニルオキシ、C 〜C ハロアルコキシ、C 〜C アルキルスルフェニル、C 〜C アルキルスルフィニ B is, H, CR 1 R 2 R 3, CHR 1 R 2, C 1 ~C 4 haloalkyl, tetrahydropyranyl, Si (CH 3) 3, SO 2 Re, SO 2 NHRb, SO 2 NRaRb, C (S ) NHRb, C (S) NRaRb , C (O) Rf, a P (O) RgRh, P ( S) RgRh, alkali metals, alkaline earth metals or NHRiRjRk, G is, H, halogen, C 1 -C 6 alkyl, C 1 -C 4 alkyl substituted by Rc, C 1 -C 4 haloalkyl, C 1 -C 3 alkyl optionally substituted C 3 -C 6 cycloalkyl, C 1 -C 6 alkoxy, C 2 -C 4 alkenyloxy, C 2 -C 4 alkynyloxy, C 1 -C 4 haloalkoxy, C 1 -C 4 alkylsulfenyl, C 1 -C 4 alkylsulfinyl 、C 〜C アルキルスルホニル、C 〜C アルケニルスルフェニル、C 〜C アルケニルスルフィニル、C 〜C アルケニルスルホニル、C 〜C アルキニルスルフェニル、C 〜C アルキニルスルフィニル、C 〜C アルキニルスルホニル、C 〜C ハロアルキルスルフェニル、C 〜C ハロアルキルスルフィニル、C 〜C ハロアルキルスルホニル、C 〜C ハロアルケニルスルフェニル、C 〜C ハロアルケニルスルフィニル、C 〜C ハロアルケニルスルホニル、NO 、CN、−NU 、ナフチル、Rcで置換されたメトキシ、C 〜C アルコキシカルボニル、C 〜C アルコキシアルキル、C 〜C アルキルカルボニル、C 〜C ハロアルキル , C 1 -C 4 alkylsulfonyl, C 2 -C 4 alkenyl Le phenyl, C 2 -C 4 alkenylsulfinyl, C 2 -C 4 alkenylsulfonyl, C 2 -C 4 alkyl Nils Le phenyl, C 2 -C 4 alkynylsulfinyl , C 2 -C 4 alkynylsulfonyl, C 1 -C 4 haloalkylsulfenyl, C 1 -C 4 haloalkylsulfinyl, C 1 -C 4 haloalkylsulfonyl, C 2 -C 4 halo alkenyl Le phenyl, C 2 -C 4 halo alkenylsulfinyl, C 2 -C 4 haloalkenyl sulfonyl, NO 2, CN, -NU 1 U 2, naphthyl, methoxy substituted by Rc, C 2 -C 5 alkoxycarbonyl, C 2 -C 4 alkoxyalkyl, C 2 -C 4 alkylcarbonyl, C 2 -C 4 haloalkyl カルボニル、C 〜C アルキルカルボニルオキシ、C 〜C ハロアルキルカルボニルオキシ、C 〜C ジアルキルアミノカルボニルオキシ、Zで置換されていてもよいフェニル、Zで置換されていてもよいフェノキシ、Zで置換されていてもよいベンゾイル、Zで置換されていてもよいピリジル、Zで置換されていてもよいピリジルオキシ、Zで置換されていてもよいチエニル、隣接した置換位置で結合したメチレンジオキシ、隣接した置換位置で結合したハロメチレンジオキシ及び−N=CT の中から選ばれる1ないし4個の置換基、または隣接した置換位置で結合したアルキレン基によって形成される5ないし8員環であり、 Carbonyl, C 2 -C 5 alkylcarbonyloxy, C 2 -C 5 halo alkylcarbonyloxy, C 3 -C 7 dialkylaminocarbonyloxy, phenyl optionally substituted by Z, which may be substituted with Z phenoxy, good benzoyl optionally substituted by Z, pyridyl optionally substituted by Z, which may be substituted with Z pyridyloxy, thienyl optionally substituted by Z, methylene di bound in adjacent substitution positions oxy, 1 to 4 substituents selected from among adjacent halo methylenedioxy and -N = CT 2 T 3 bound substituted position or 5 to be formed by an alkylene group attached at adjacent substitution positions, is an 8-membered ring,
Y、Y 及びY は、各々独立にH、ハロゲン、C 〜C アルキル、C 〜C ハロアルキル、C 〜C アルコキシ、C 〜C ハロアルコキシ、C 〜C アルキルスルフェニル、C 〜C アルキルスルフィニル、C 〜C アルキルスルホニル、C 〜C ハロアルキルスルフェニル、C 〜C ハロアルキルスルフィニル、C 〜C ハロアルキルスルホニル、NO またはCNであるか、または隣接した置換位置で結合したアルキレン基によって形成される5員環、6員環、7員環もしくは8員環であり、 Y, Y 1 and Y 2 are each independently H, halogen, C 1 -C 4 alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 alkoxy, C 1 -C 4 haloalkoxy, C 1 -C 4 alkylsulfenyl, C 1 -C 4 alkylsulfinyl, C 1 -C 4 alkylsulfonyl, C 1 -C 4 haloalkylsulfenyl, C 1 -C 4 haloalkylsulfinyl, C 1 -C 4 haloalkylsulfonyl, NO 2 or CN 5-membered ring formed by an alkylene group, or bound in adjacent substitution positions is a 6-membered ring, 7-membered ring or 8-membered ring,
は、C 〜C アルキルまたはC 〜C ハロアルキルであり、 Y 3 is a C 1 -C 4 alkyl or C 1 -C 4 haloalkyl,
Zは、各々独立して、ハロゲン、C 〜C アルキル、C 〜C ハロアルキル、C 〜C アルコキシ、C 〜C ハロアルコキシ、C 〜C アルキルスルフェニル、C 〜C アルキルスルフィニル、C 〜C アルキルスルホニル、C 〜C アルケニルスルフェニル、C 〜C アルケニルスルフィニル、C 〜C アルケニルスルホニル、C 〜C ハロアルキルスルフェニル、C 〜C ハロアルキルスルフィニル、C 〜C ハロアルキルスルホニル、NO 、CN、−NU 及びC 〜C アルコキシカルボニルの中から選ばれる1ないし5個の置換基であり、 Z are each independently halogen, C 1 -C 4 alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 alkoxy, C 1 -C 4 haloalkoxy, C 1 -C 4 alkylsulfenyl, C 1 -C 4 alkylsulfinyl, C 1 -C 4 alkylsulfonyl, C 2 -C 4 alkenyl Le phenyl, C 2 -C 4 alkenylsulfinyl, C 2 -C 4 alkenylsulfonyl, C 1 -C 4 haloalkylsulfenyl, C 1 -C 4 haloalkylsulfinyl, a C 1 -C 4 haloalkylsulfonyl, nO 2, CN, 1 to 5 substituents selected from among -NU 1 U 2 and C 2 -C 5 alkoxycarbonyl,
、R 、R 及びRaは、各々独立にC 〜C アルキルであり、 R 1, R 2, R 3 and Ra is C 1 -C 6 alkyl each independently,
Rbは、H、C 〜C アルキル、またはT で置換されていてもよいフェニルであり、 Rb is, H, a C 1 -C 6 alkyl or phenyl optionally substituted with T 1,,
Rcは、ハロゲン、C 〜C アルキル、C 〜C アルコキシ及びC 〜C ハロアルキルの中から任意に選ばれる1種以上で置換されていてもよいフェニルであり、 Rc is halogen, C 1 -C 4 alkyl, C 1 -C 4 alkoxy and C 1 -C 4 phenyl optionally substituted with one or more selected arbitrarily from among haloalkyl,
Rdは、ハロゲン、C 〜C アルキル及びC 〜C ハロアルキルの中から任意に選ばれる1種以上で置換されていてもよいベンゾイルであり、 Rd is halogen, C 1 -C 4 alkyl and C 1 -C 4 optionally benzoyl optionally substituted with one or more selected arbitrarily from among haloalkyl,
Reは、C 〜C アルキル、C 〜C ハロアルキル、またはT で置換されていてもよいフェニルであり、 Re is a C 1 -C 4 alkyl, C 1 -C 4 haloalkyl or phenyl optionally substituted with T 1,,
Rfは、C 〜C 20アルキル、C 〜C アルケニル、C 〜C ハロアルキル、C 〜C アルコキシアルキル、C 〜C ハロシクロアルキル、Rcで置換されたC 〜C アルキル、C 〜C アルキルで置換されていてもよいC 〜C シクロアルキル、Rcで置換されたシクロアルキル、Rc及びC 〜C アルキルで置換されたシクロプロピル、Rc及びハロゲンで置換されたC 〜C シクロアルキル基、T 及びC 〜C アルキルで置換されたシクロプロピル基、Rcで置換されたC 〜C アルケニル、C 〜C アルコキシ、C 〜C ハロアルコキシ、C 〜C アルケニルオキシ、C 〜C アルキルで置換されていてもよいC 〜C シクロアルコキシ、ベンジルオキシ Rf is, C 1 -C 20 alkyl, C 2 -C 6 alkenyl, C 1 -C 6 haloalkyl, C 2 -C 4 alkoxyalkyl, C 3 -C 6 halocycloalkyl, C 1 -C substituted with Rc 4 alkyl, C 1 -C 4 optionally substituted by alkyl C 3 -C 7 cycloalkyl, cycloalkyl substituted with Rc, Rc and C 1 -C 4 alkyl substituted cyclopropyl, Rc and halogen in substituted C 3 -C 4 cycloalkyl group, T 2, and C 1 -C 4 alkyl substituted cyclopropyl group, C 2 -C 4 alkenyl substituted with Rc, C 1 ~C 6 alkoxy, C 1 -C 4 haloalkoxy, C 2 -C 5 alkenyloxy, C 1 -C 3 may be alkyl substituted C 3 -C 6 cycloalkoxy, benzyloxy 、COORa、−NU 、T で置換されていてもよいフェニル、T で置換されていてもよいフェノキシ、ナフチル、T で置換されていてもよいピリジルまたはA−1〜A−140であり、 , COORa, -NU 1 U 2, T 3 optionally substituted by phenyl, optionally substituted with T 3 phenoxy, naphthyl, T 1 pyridyl or A-1~A- be substituted by is 140,
Rg及びRhは各々独立に、OH、フェニル、C 〜C アルキル、C 〜C アルコキシまたはC 〜C アルキルスルフェニルであり、 Rg and Rh are each independently, OH, phenyl, C 1 -C 6 alkyl, C 1 -C 6 alkoxy or C 1 -C 4 alkylsulfenyl,
Ri、Rj及びRkは各々独立に、H、C 〜C アルキル、C 〜C アルケニル、C 〜C アルキル基で置換されていてもよいC 〜C シクロアルキル基またはベンジルであるか、あるいはRi、Rj及びRkのうちの2個が、それぞれが結合している窒素原子と共に酸素原子、窒素原子または硫黄原子を含有していてもよい5ないし8員環基を形成してもよく、 Ri, Rj and Rk are each independently, H, C 1 -C 6 alkyl, C 1 -C 4 alkenyl, optionally substituted with C 1 -C 3 alkyl group C 3 -C 6 cycloalkyl group or a benzyl or is, or Ri, 2 pieces of Rj and Rk are an oxygen atom together with the nitrogen atom to which each is attached, to 5 which may contain a nitrogen atom or a sulfur atom to form a 8-membered ring group at best,
は、ハロゲン、C 〜C アルキル、C 〜C ハロアルキルまたはC 〜C アルコキシであり、 T 1 is halogen, C 1 -C 4 alkyl, C 1 -C 4 haloalkyl or C 1 -C 4 alkoxy,
は、ハロゲンで置換されていてもよいC 〜C アルケニルであり、 T 2 are a good C 2 -C 4 alkenyl optionally substituted by halogen,
は、ハロゲン、C 〜C アルキル、C 〜C ハロアルキル、C 〜C アルコキシ、C 〜C ハロアルコキシ、C 〜C アルキルスルフェニル、C 〜C アルキルスルフィニル、C 〜C アルキルスルホニル、C 〜C ハロアルキルスルフェニル、C 〜C ハロアルキルスルフィニル、C 〜C ハロアルキルスルホニル、NO 、CN、CHO、−NU 、フェニル及びフェノキシの中から任意に選ばれる1ないし5個の置換基であり、 T 3 is halogen, C 1 -C 4 alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 alkoxy, C 1 -C 4 haloalkoxy, C 1 -C 4 alkylsulfenyl, C 1 -C 4 alkyl sulfinyl, C 1 -C 4 alkylsulfonyl, C 1 -C 4 haloalkylsulfenyl, C 1 -C 4 haloalkylsulfinyl, C 1 -C 4 haloalkylsulfonyl, NO 2, CN, CHO, -NU 1 U 2, phenyl and it 1 is arbitrarily selected from among phenoxy are 5 substituents,
及びU は、各々独立に、H、C 〜C アルキル、COORa、フェニルまたはベンジルを表すか、あるいはU とU とが結合している窒素原子と共に酸素原子、窒素原子または硫黄原子を含有していてもよい5ないし8員環基を形成してもよく、 U 1 and U 2 are each independently, H, C 1 -C 6 alkyl, COORa, or represents phenyl or benzyl, or U 1 and U 2 and an oxygen atom together with the nitrogen atom to which they are attached a nitrogen atom or 5 to may contain a sulfur atom may form a 8-membered ring group,
mは、置換基の数を表し、0、1、2または3であり、 m represents the number of substituents is 0, 1, 2 or 3,
nは、置換基の数を表し、0、1、2、3または4であり、 n represents the number of substituents is 0, 1, 2, 3 or 4,
pは、置換基の数を表し、0、1または2であり、 p represents the number of substituents is 0, 1 or 2,
qは、置換基の数を表し、0または1である。 q represents the number of substituents is 0 or 1. (但し、m、n及びpが2以上の整数を表す場合は、その置換基は同一か相互に異なってもよい。)]。 (Where, m, when the n and p is an integer of 2 or more, the substituents may be different in the same or another.).
【0020】 [0020]
化合物群A:アシベンゾラルーS−メチル(acibenzolar−S−methyl)、アシルアミノベンザミド(acylaminobenzamide)、アンバム(amobam)、アムプロピルホス(ampropyfos)、アニラジン(anilazine)、アザコナゾール(azaconazole)、アゾキシストロビン(azoxystrobin)、ベナラキシル(benalaxyl)、ベノダニル(benodanil)、ベノミル(benomyl)、ベンチアゾール(benthiazole)、ベンザマクリル(benzamacril)、ビナパクリル(binapacryl)、ビフェニル(biphenyl)、ビテルタノール(bitertanol)、ベトキサジン(bethoxazin Compounds A: Ashibenzoraru S- methyl (acibenzolar-S-methyl), acylamino Benzalkonium bromide (acylaminobenzamide), Anbamu (amobam), Am propyl phosphite (ampropyfos), Anirajin (anilazine), azaconazole (azaconazole), azoxystrobin (azoxystrobin), benalaxyl (benalaxyl), Benodaniru (benodanil), benomyl (benomyl), bench azole (benthiazole), Benzamakuriru (benzamacril), binapacryl (binapacryl), biphenyl (biphenyl), bitertanol (bitertanol), Betokisajin (Bethoxazin )、ボルドー液(bordeaux mixture)、ブラストサイジン−S(blasticidin−S)、ブロモコナゾール(bromoconazole)、ブピリメート(bupirimate)、ブチオベート(buthiobate)、カルシウムポリスルフィド(calcium polysulfide)、キャプタフォール(captafol)、キャプタン(captan)、カッパーオキシクロリド(copper oxychloride)、カルプロパミド(carpropamid)、カルベンダジン(carbendazim)、カルボキシン(carboxin)、CGA−279202、キノメチオネート(chinomethionat)、クロベンチアゾン(chlobenthiazone)、 ), Bordeaux mixture (bordeaux Mixture), blasticidin -S (blasticidin-S), Bro Mokona tetrazole (Bromoconazole), bupirimate (Bupirimate), buthiobate (Buthiobate), calcium polysulfide (calcium polysulfide), cap data fall (Captafol), captan (captan), Copper oxychloride (copper oxychloride), carpropamid (carpropamid), carbendazim Jin (carbendazim), carboxin (carboxin), CGA-279202, Kinomechioneto (chinomethionat), black bench Azone (chlobenthiazone), ロルフェナゾール(chlorfenazol)、クロロネブ(chloroneb)、クロロタロニル(chlorothalonil)、クロゾリネート(chlozolinate)、クフラネブ(cufraneb)、シモキサニル(cymoxanil)、シプロコナゾール(cyproconazol)、シプロジニル(cyprodinil)、シプロフラム(cyprofuram)、ダゾメット(dazomet)、デバカルブ(debacarb)、ジクロロフェン(dichlorophen)、ジクロブトラゾール(diclobutrazol)、ジクロフラニド(diclhlofluanid)、ジクロメジン(diclomedine)、ジクロラン(dicloran)、ジエトフェンカルブ(diet Rorufenazoru (chlorfenazol), chloroneb (chloroneb), chlorothalonil (chlorothalonil), chlozolinate (chlozolinate), Kufuranebu (cufraneb), cymoxanil (cymoxanil), cyproconazole (cyproconazol), cyprodinil (cyprodinil), Shipurofuramu (cyprofuram), dazomet (dazomet), Debakarubu (debacarb), dichlorophen (dichlorophen), dicumyl Rob tiger tetrazole (diclobutrazol), Jikurofuranido (diclhlofluanid), Jikuromejin (diclomedine), dichloran (dicloran), diethofencarb (diet hofencarb)、ジクロシメット(diclocymet)、ジフェノコナゾール(difenoconazole)、ジフルメトリン(diflumetorim)、ジメチリモール(dimethirimol)、ジメトモルフ(dimethomorph)、ジニコナゾール(diniconazole)、ジニコナゾール−M(diniconazole−M)、ジノカップ(dinocap)、ジフェニルアミン(diphenylamine)、ジピリチオン(dipyrithione)、ジタリムホス(ditalimfos)、ジチアノン(dithianon)、ドデモルフ(dodemorph)、ドジン(dodine)、ドラゾクソロン(drazoxolon)、エデフェノホス(edifenphos hofencarb), diclocymet (diclocymet), difenoconazole (difenoconazole), Jifurumetorin (diflumetorim), dimethirimol (dimethirimol), dimethomorph (Dimethomorph), diniconazole (diniconazole), diniconazole -M (diniconazole-M), dinocap (dinocap), diphenylamine (diphenylamine ), Jipirichion (dipyrithione), Jitarimuhosu (ditalimfos), dithianon (dithianon), dodemorph (dodemorph), dodine (dodine), Dorazokusoron (drazoxolon), Edefenohosu (edifenphos 、エポキシコナゾール(epoxiconazole)、エタコナゾール(etaconazole)、エチリモル(ethirimol)、エトリジアノール(etridiazole)、ファモキサゾン(famoxadone)、フェナリモル(fenarimol)、フェブコナゾール(febuconazole)、フェナミドン(fenamidone)、フェンダゾスラム(fendazosulam)、フェンフラム(fenfuram)、フェンヘキサミド(fenhexamid)、フェンピクロニル(fenpiclonil)、フェンプロピジン(fenpropidin)、フェンプロピモルフ(fenpropimorph)、フェンチン(fentin)、フェルバン(ferbam)、フェリムゾン(f , Epoxiconazole (epoxiconazole), Etakonazoru (etaconazole), Echirimoru (ethirimol), Etorijianoru (etridiazole), Famokisazon (famoxadone), fenarimol (fenarimol), Febukonazoru (febuconazole), fenamidone (fenamidone), fender zone Slam (Fendazosulam ), Fenfuramu (fenfuram), fenhexamid (fenhexamid), fenpiclonil (fenpiclonil), fenpropidin (fenpropidin), fenpropimorph (fenpropimorph), fentin (fentin), Feruban (ferbam), ferimzone (f rimzone)、フルアジナム(fluazinam)、フルジオキソニル(fludioxonil)、フルオロイミド(fluoroimide)、フルキンコナゾール(fluquinconazole)、フルシラゾール(flusilazole)、フルスルファミド(flusulfamide)、フルトラニル(flutolanil)、フルトリアフォール(flutriafol)、フォルペット(folpet)、フォセチル−アルミニウム(fosetyl−aluminium)、フベリダゾール(fuberidazole)、フララキシル(furalaxyl)、フラメトピル(furametpyr)、グアザチン(guazatine)、ヘキサクロロベンゼン(hexachlorobenzene rimzone), fluazinam (fluazinam), fludioxonil (fludioxonil), fluoro imide (fluoroimide), fluquinconazole (fluquinconazole), flusilazole (flusilazole), flusulfamide (flusulfamide), flutolanil (flutolanil), full thoria Fall (flutriafol), folpet (folpet), fosetyl - aluminum (fosetyl-aluminium), fuberidazole (fuberidazole), furalaxyl (furalaxyl), furametpyr (furametpyr), guazatine (guazatine), hexachlorobenzene (hexachlorobenzene )、ヘキサコナゾール(hexaconazole)、ヒメキサゾール(hymexazol)、イマザリル(imazalil)、イミベンコナゾール(imibenconazole)、イミノクタジン(iminoctadine)、イプコナゾール(ipconazole)、イプロベンホス(iprobenfos)、イプロジオン(iprodione)、イソプロチオラン(isoprothiolane)、イプロバリカルブ(iprovalicarb)、カスガマイシン(kasugamycin)、クレソキシム−メチル(kresoxim−methyl)、マンカッパー(mancopper)、マンコゼブ(mancozeb)、マンネブ(maneb)、メパニピリム(mepanipyrim)、メプロニ ), Hexaconazole (Hexaconazole), hymexazol (Hymexazol), imazalil (Imazalil), imibenconazole (Imibenconazole), iminoctadine (Iminoctadine), ipconazole (Ipconazole), iprobenfos (Iprobenfos), iprodione (Iprodione), isoprothiolane (isoprothiolane) , iprovalicarb (iprovalicarb), kasugamycin (kasugamycin), kresoxim - methyl (kresoxim-methyl), Man Copper (mancopper), mancozeb (mancozeb), maneb (maneb), mepanipyrim (mepanipyrim), Mepuroni (mepronil)、メタラキシル(metalaxyl)、メトコナゾール(metconazole)、メタスルホカルブ(methasulfocarb)、メチラム(metiram)、メトミノストロビン(metominostrobin)、ミクロブタニル(myclobutanil)、MTF−753、ナバム(nabam)、ニッケルビス(ジメチルジチオカーバメート)(nickel bis(dimethyldithiocarbamate))、ニトロタール−イソプロピル(nitrothal−isopropyl)、ヌアリモル(nuarimol)、NNF−9425、オクチリノン(octhilinone)、オフレース(ofurace)、オキサジキシル(oxadixyl)、オキシカ (Mepronil), metalaxyl (metalaxyl), metconazole (metconazole), methasulfocarb (methasulfocarb), metiram (metiram), metominostrobin (metominostrobin), myclobutanil (myclobutanil), MTF-753, Nabamu (nabam), nickel bis ( dimethyl dithiocarbamate) (nickel bis (dimethyldithiocarbamate)), Nitorotaru - isopropyl (nitrothal-isopropyl), nuarimol (nuarimol), NNF-9425, octhilinone (octhilinone), ofurace (ofurace), oxadixyl (oxadixyl), Okishika ボキシン(oxycarboxin)、オキポコナゾールフマール酸塩(oxpoconazole fumarate)、ペフラゾエート(pefurzoate)、ペンコナゾール(penconazole)、ペンシクロン(pencycuron)、フタライド(phthalide)、ピペラリン(piperalin)、ポリオキシン(polyoxins)、炭酸水素カリウム(potassium hydrogen carbonate)、プロベナゾール(probenazole)、プロクロラズ(prochloraz)、プロシミドン(procymidone)、プロパモカルブ塩酸塩(propamocarb hydrochloride)、プロピコナゾール(propiconazole)、プロピネブ( Bokishin (oxycarboxin), Oki Poco Nazo Ruch Mar salt (oxpoconazole fumarate), pefurazoate (pefurzoate), penconazole (penconazole), pencycuron (pencycuron), phthalide (phthalide), Piperarin (piperalin), polyoxin (polyoxins), potassium bicarbonate ( potassium hydrogen carbonate), probenazole (probenazole), prochloraz (prochloraz), procymidone (procymidone), propamocarb hydrochloride (propamocarb hydrochloride), propiconazole (propiconazole), propineb ( ropineb)、ピラゾホス(pyrazophos)、ピリフェノックス(pyrifenox)、ピリメタニル(pyrimethanil)、ピロキュロン(pyroquilon)、キノメチオネート(quinomethionate)、キノキシフェン(quinoxyfen)、キントゼン(quintozene)、RH7281、炭酸水素ナトリウム(sodium hydrogen carbonate)、次亜塩素酸ナトリウム(sodium hypochlorite)、硫黄(sulfur)、スピロキサミン(spiroxamine)、テブコナゾール(tebuconazole)、テクナゼン(tecnazene)、テトラコナゾール(tetraconazole)、チアベンダゾール(thi ropineb), pyrazophos (pyrazophos), pyrifenox (pyrifenox), pyrimethanil (pyrimethanil), Pirokyuron (pyroquilon), Kinomechioneto (quinomethionate), quinoxyfen (quinoxyfen), quintozene (quintozene), RH7281, sodium bicarbonate (sodium hydrogen carbonate) , sodium hypochlorite (sodium hypochlorite), sulfur (sulfur), spiroxamine (spiroxamine), tebuconazole (tebuconazole), Tekunazen (tecnazene), Tetraconazole tetrazole (tetraconazole), thiabendazole (thi bendazole)、チアジアジン(thiadiazin/milneb)、チフルザミド(thifluzamide)、チオファネート−メチル(thiophanate−methyl)、チラム(thiram)、トルクロホス−メチル(tolclofos−methyl)、トリルフラニド(tolylfluanid)、トリアジメホン(triadimefon)、トリアジメノール(toriadimenol)、トリアゾキシド(triazoxide)、トリシクラゾール(tricyclazole)、トリデモルフ(tridemorph)、トリフルミゾール(triflumizole)、トリホリン(triforine)、トリチコナゾール(triticonazole)、バリダマイシン(va bendazole), thiadiazine (thiadiazin / milneb), thifluzamide (thifluzamide), thiophanate - methyl (thiophanate-methyl), thiram (thiram), tolclofos - methyl (tolclofos-methyl), Torirufuranido (tolylfluanid), triadimefon (triadimefon), Toriajime Nord (toriadimenol), triazoxide (triazoxide), tricyclazole (tricyclazole), tridemorph (tridemorph), triflumizole (triflumizole), triforine (triforine), triticonazole (triticonazole), validamycin (va lidamycin)、ビンクロゾリン(vinclozolin)、硫酸亜鉛(zinc sulfate)、ジネブ(zineb)、ジラム(ziram)、シイタケ菌糸体抽出物、ストレプトマイシン(streptomycin)、テクロフタラム(tecloftalam)、オキシテトラサイクリン(oxyterracycline)、オキソリニックアシド(oxolinic acid)、アルドキシカルブ(aldoxycarb)、カズサホス(cadusafos)、フォスチアゼート(fosthiazate)、フォスチエタン(fosthietan)、オキサミル(oxamyl)、フェナミホス(fenamiphos)、アセキノシル(acequinocyl)、ブロモプロピレート(bromopr Lidamycin), vinclozolin (Vinclozolin), zinc sulfate (zinc sulfate), zineb (zineb), ziram (Ziram), shiitake mycelium extract, streptomycin (streptomycin), tecloftalam (Tecloftalam), oxytetracycline (Oxyterracycline), oxolinic A Sid ( oxolinic acid), aldoxycarb (aldoxycarb), cadusafos (cadusafos), fosthiazate (fosthiazate), Fosuchietan (fosthietan), oxamyl (oxamyl), fenamiphos (fenamiphos), acequinocyl (acequinocyl), bromopropylate (Bromopr pylate)、チノメチオネート(chinomethionat)、クロロベンジラート(chlorobezilate)、サイヘキサチン(cyhexatine)、ジコフォール(dicofol)、ジエノクロール(dienochlor)、エトキサゾール(etoxazole)、フェナザキン(fenazaquin)、フェンブタチンオキシド(fenbutatin oxide)、フェンプロパトリン(fenpropathrin)、フェンプロキシメート(fenproximate)、ハルフェンプロックス(halfenprox)、ヘキシチアゾックス(hexythiazox)、ミルベメクチン(milbemectin)、プロパルギット(propargite)、ピリダベン(pyridab pylate), Chinomechioneto (chinomethionat), chlorobenzal benzilate (chlorobezilate), Saihekisachin (cyhexatine), dicofol (dicofol), Jienokuroru (dienochlor), etoxazole (etoxazole), fenazaquin (fenazaquin), fenbutatin oxide (fenbutatin oxide), phen Puropatorin (fenpropathrin), phen proxy formate (fenproximate), halfenprox (halfenprox), hexythiazox (hexythiazox), milbemectin (milbemectin), propargite (propargite), pyridaben (Pyridab n)、ピリミジフェン(pyrimidifen)、テブフェンピラド(tebufenpyrad)、アバメクチン(abamectin)、アセフェート(acephate)、アセタミピリド(acetamipirid)、アルディカルブ(aldicarb)、アレスリン(allethrin)、アジンホス−メチル(azinphos−methyl)、ベンジオカルブ(bendiocarb)、ベンフラカルブ(benfuracarb)、ベンスルタップ(bensultap)、ブプロフェジン(buprofezin)、ブトカルボキシン(butocarboxim)、カルバリル(carbaryl)、カルボフラン(carbofuran)、カルボスルファン(carbosulfan)、カルタップ(c n), pyrimidifen (pyrimidifen), tebufenpyrad (tebufenpyrad), abamectin (abamectin), acephate (acephate), Asetamipirido (acetamipirid), aldicarb (aldicarb), allethrin (allethrin), azinphos - methyl (azinphos-methyl), bendiocarb ( bendiocarb), benfuracarb (benfuracarb), bensultap (bensultap), buprofezin (buprofezin), Butokarubokishin (butocarboxim), carbaryl (carbaryl), carbofuran (carbofuran), carbosulfan (carbosulfan), cartap (c artap)、クロルフェナピル(chlorfenapyr)、クロルピリホス(chlorpyrifos)、クロルフェンビンホス(chlorfenvinphos)、クロルフルアズロン(chlorfluazuron)、クロチアニジン(clothianidin)、クロマフェノジド(chromafenozide)、クロピリホス−メチル(chlorpyrifos−methyl)、シクロプロトリン(cycloprothrin)、シフルトリン(cyfluthrin)、ベータ−シフルトリン(beta−cyfluthrin)、シペルメトリン(cypermethrin)、シロマジン(cyromazine)、シハロトリン(cyhalothrin)、ラムダ−シハロトリン(lambda artap), chlorfenapyr (chlorfenapyr), chlorpyrifos (chlorpyrifos), chlorfenvinphos (chlorfenvinphos), Chlorfluazuron (chlorfluazuron), clothianidin (clothianidin), chromafenozide (chromafenozide), Kuropirihosu - methyl (chlorpyrifos-methyl), Shikuropuro Trinh (cycloprothrin), cyfluthrin (cyfluthrin), beta - cyfluthrin (beta-cyfluthrin), cypermethrin (cypermethrin), cyromazine (cyromazine), cyhalothrin (cyhalothrin), lambda - cyhalothrin (lambda cyhalothrin)、デルタメトリン(deltamethrin)、ジアフェンチウロン(diafenthiuron)、ダイアジノン(diazinon)、ジアクロデン(diacloden)、ジフルベンズロン(diflubenzuron)、ジメチルビンホス(dimethylvinphos)、ジオフェノラン(diofenolan)、ジスルフォトン(disulfoton)、ジメトエート(dimethoate)、エマメクチンベンゾエート(emamectin−benzoate)、EPN、エスフェンバレレート(esfenvalerate)、エチオフェンカルブ(ethiofencarb)、エチプロール(ethiprole)、エトフェンプロックス(etofenprox)、 cyhalothrin), deltamethrin (deltamethrin), diafenthiuron (diafenthiuron), diazinon (diazinon), Jiakuroden (diacloden), diflubenzuron (diflubenzuron), dimethyl bottles phosphate (dimethylvinphos), diofenolan (diofenolan), Jisurufoton (disulfoton), dimethoate ( dimethoate), emamectin benzoate (emamectin-benzoate), EPN, esfenvalerate (esfenvalerate), ethiofencarb (ethiofencarb), ethiprole (ethiprole), etofenprox (etofenprox), トリムホス(etrimfos)、フェニトロチオン(fenitrothion)、フェノブカルブ(fenobucarb)、フェノキシカーブ(fenoxycarb)、フェンプロパトリン(fenpropathrin)、フェンバレレート(fenvalerate)、フィプロニル(fipronil)、フルアクリピリム(fluacrypyrim)、フルシトリネート(flucythrinate)、フルフェノクスウロン(flufenoxuron)、フルフェンプロックス(flufenprox)、タウ−フルバリネート(tau−fluvalinate)、ホノホス(fonophos)、フォルメタネート(formetanate)、フォルモチオン(formothion)、フラチオカルブ(f Torimuhosu (etrimfos), fenitrothion (fenitrothion), fenobucarb (fenobucarb), phenoxy curve (fenoxycarb), fenpropathrin (fenpropathrin), fenvalerate (fenvalerate), fipronil (Fipronil), fluacrypyrim (fluacrypyrim), flucythrinate (flucythrinate) , flufenoxuron uronic (flufenoxuron), full phen flufenprox (flufenprox), tau - fluvalinate (tau-fluvalinate), fonofos (fonophos), folder meth sulfonate (formetanate), formothion (formothion), furathiocarb (f urathiocarb)、ハロフェノジド(halofenozide)、ヘキサフルムロン(hexaflumuron)、ヒドラメチルノン(hydramethylnon)、イミダクロプリド(imidacloprid)、イソフェンホス(isofenphos)、インドキサカルブ(indoxacarb)、イソプロカルブ(isoprocarb)、イソキサチオン(isoxathion)、ルフェヌウロン(lufenuron)、マラチオン(malathion)、メタルデヒド(metaldehyde)、メタミドホス(methamidophos)、メチダチオン(methidathion)、メタクリホス(methacrifos)、メタルカルブ(metalcarb)、メソミル(meth urathiocarb), halofenozide (halofenozide), hexaflumuron (hexaflumuron), hydramethylnon (hydramethylnon), imidacloprid (imidacloprid), isofenphos (isofenphos), indoxacarb (indoxacarb), isoprocarb (isoprocarb), isoxathion (isoxathion), Rufenuuron (lufenuron), malathion (malathion), Metarudehido (metaldehyde), methamidophos (methamidophos), methidathion (methidathion), Metakurihosu (methacrifos), Metarukarubu (metalcarb), methomyl (meth myl)、メソプレン(methoprene)、メトキシクロール(methoxychlor)、メトキシフェノジド(methoxyfenozide)、モノクロトホス(monocrotophos)、ムスカルーレ(muscalure)、ニジノテフラン(nidinotefuran)、ニテンピラム(nitenpyram)、オメトエート(omethoate)、オキシデメトン−メチル(oxydemeton−methyl)、オキサミル(oxamyl)、パラチオン(parathion)、パラチオン−メチル(parathion−methyl)、ペルメトリン(permethrin)、フェントエート(phenthoate)、フォキシム(phoxim)、ホレート(phorate)、ホ myl), methoprene (methoprene), methoxychlor (methoxychlor), methoxyfenozide (methoxyfenozide), monocrotophos (monocrotophos), Musukarure (muscalure), two dinotefuran (nidinotefuran), nitenpyram (nitenpyram), omethoate (omethoate), oxydemeton - methyl ( oxydemeton-methyl), oxamyl (oxamyl), parathion (parathion), parathion - methyl (parathion-methyl), permethrin (permethrin), phenthoate (phenthoate), phoxim (phoxim), phorate (phorate), Ho ロン(phosalone)、ホスメット(phosmet)、ホスファミドン(phosphamidon)、ピリミカルブ(pirimicarb)、ピリミホス−メチル(pirimiphos−methyl)、プロフェノホス(profenofos)、プロトリフェンブト(protrifenbute)、ピメトロジン(pymetrozine)、ピラクロホス(pyraclofos)、ピリプロキシフェン(pyriproxyfen)、ロテノン(rotenone)、スルプロホス(sulprofos)、シラフルオフェン(silafluofen)、スピノサド(spinosad)、スルホテップ(sulfotep)、テブフェノジド(tebfenozide)、テフルベンズロン(tefluben Ron (phosalone), phosmet (phosmet), phosphamidon (phosphamidon), pirimicarb (pirimicarb), pirimiphos - methyl (pirimiphos-methyl), profenofos (profenofos), pro triphenedioxazine but-(protrifenbute), pymetrozine (pymetrozine), pyraclofos (Pyraclofos ), pyriproxyfen (pyriproxyfen), rotenone (rotenone), sulprophos (sulprofos), silafluofen (silafluofen), spinosad (spinosad), sulfotep (sulfotep), tebufenozide (Tebfenozide), teflubenzuron (Tefluben zuron)、テフルトリン(tefluthorin)、テルブホス(terbufos)、テトラクロロビンホス(tetrachlorvinphos)、チアクロプリド(thiacloprid)、チオシクラム(thiocyclam)、チオジカルブ(thiodicarb)、チアメトキサム(thiamethoxam)、チオファノックス(thiofanox)、チオメトン(thiometon)、トルフェンピラド(tolfenpyrad)、トラロメスリン(tralomethrin)、トリクロルホン(trichlorfon)、トリアズロン(triazuron)、トリフルムロン(triflumuron)、バミドチオン(vamidothion)及びエチオン(ethion)。 zuron), tefluthrin (tefluthorin), terbufos (terbufos), tetrachloride Robin phosphate (tetrachlorvinphos), thiacloprid (thiacloprid), thiocyclam (thiocyclam), thiodicarb (thiodicarb), thiamethoxam (thiamethoxam), thiofanox (thiofanox), thiometon ( thiometon), tolfenpyrad (tolfenpyrad), tralomethrin (tralomethrin), trichlorfon (trichlorfon), Toriazuron (triazuron), triflumuron (triflumuron), vamidothion (vamidothion) and ethion (ethion).
【0021】 [0021]
〔2〕 上記〔1〕記載の式(1)で表されるアクリロニトリル化合物の1種以上と、以下の化合物群Bより選ばれる化合物の1種以上を含有する殺ダニ組成物。 [2] [1] one or more and, acaricidal compositions containing one or more of the following compounds a compound selected from B acrylonitrile compounds represented by the formula (1) as claimed.
【0022】 [0022]
化合物群B:アセキノシル、ブロモプロピレート、チノメチオネート、ジコフォール、エトキサゾール、フェンブタチンオキシド、ミルベメクチン、プロパルギット、ピリダベン、アバメクチン、アルディカルブ、クロルピリフォス、ジフルベンズロン、クロルフェナピル、フェントエート、エマメクチンベンゾエート、メチダチオン、オキサミル、カルシウムポリスルフィド、マンコゼブ、マンネブ及びエチオン。 Compound group B: acequinocyl, bromopropylate, Chinomechioneto, dicofol, etoxazole, fenbutatin oxide, milbemectin, propargite, pyridaben, abamectin, aldicarb, chlorpyrifos, diflubenzuron, chlorfenapyr, phenthoate, emamectin benzoate, methidathion, oxamyl, calcium polysulfide, mancozeb, maneb and ethion.
【0023】 [0023]
〔3〕 ハダニ、フシダニ又はホコリダニの防除に用いる上記〔2〕記載の殺ダニ組成物。 [3] mites, Fushidani or the [2] acaricidal composition according used in the control of dust mite.
【0024】 [0024]
〔4〕 上記〔1〕記載の式(1)で表されるアクリロニトリル化合物の1種以上と、上記〔1〕記載の化合物群Aより選ばれる化合物の1種以上を同時に、又は近接して処理することを特徴とする、害虫又は病害の防除方法。 [4] [1] and one or more acrylonitrile compounds represented by the formula (1) according, to one or more of the above-mentioned [1] compounds compound selected from A according simultaneously, or in proximity to the process features to method for controlling pests or disease to.
【0025】 [0025]
〔5〕 上記〔1〕記載の式(1)で表されるアクリロニトリル化合物の1種以上と、上記〔2〕記載の化合物群Bより選ばれる化合物の1種以上を同時に、又は近接して処理することを特徴とする、ダニの防除方法。 [5] above and one or more [1] acrylonitrile compound represented by the formula (1) according, to one or more of the above-mentioned [2] compounds compound selected from B described simultaneously, or in proximity to the process it is characterized by, a method for controlling mites.
【0026】 [0026]
〔6〕 上記〔1〕記載の式(1)で表されるアクリロニトリル化合物の1種以上と、上記〔2〕記載の化合物群Bより選ばれる化合物の1種以上を同時に、又は近接して処理することを特徴とする、ハダニ、フシダニ又はホコリダニの防除方法。 [6] [1] or one acrylonitrile compound of the formula (1) as claimed and, one or more of the above-mentioned [2] compounds compound selected from B described simultaneously, or in proximity to the process characterized by, spider mites, Fushidani or dust mite control methods.
【0027】 [0027]
【発明の実施の形態】 DETAILED DESCRIPTION OF THE INVENTION
本発明組成物及び本発明方法における一方の有効成分化合物である式(1)で表されるアクリロニトリル化合物の−C(CN)=C(OB)−部は、E体およびZ体の2種の異性体が存在するが、両者とも本発明に含まれる。 -C acrylonitrile compounds represented by the formula (1), which is one of the active ingredient compound in the composition of the present invention and the present invention method (CN) = C (OB) - parts are, the two E-form and Z-form Although isomers, are included in both cases the present invention.
【0028】 [0028]
本発明組成物及び本発明方法における一方の有効成分化合物であるアクリロニトリル化合物は、式(1)中の置換基Bが水素原子の場合、下式で表される互変異性形で存在しうることは理解されるであろう。 Acrylonitrile compound which is one of the active ingredient compound in the composition of the present invention and the present invention method, when the substituent B in formula (1) is a hydrogen atom can exist in tautomeric forms represented by the following formula it will be appreciated.
【0029】 [0029]
【化13】 [Of 13]
【0030】 [0030]
該化合物は主としてエノール形(1′)で存在すると考えられるが、或条件下では互変異性形(2)およびエキソオレフィン形(2′)をとりうる。 The compounds predominantly enol form (1 ') is thought to exist in but tautomeric forms under certain conditions (2) and exo-olefin type (2' can take). 本発明は3つの互変異性形およびそれらの混合物を全て包含すると理解されるべきである。 The present invention should be understood as three tautomeric forms and includes all mixtures thereof.
【0031】 [0031]
本発明組成物に含有される又は本発明方法で使用される一方の有効成分である式(1)で表されるアクリロニトリル化合物は、作用性が従来の有機塩素系殺虫剤、有機リン系殺虫剤、カーバメート系殺虫剤およびピレスロイド系殺虫剤などの薬剤とは異なるものであり、またある種の害虫に対しては低薬量で死にいたらしめるとともに残効性も備え、結果的に顕著な防除効果を発揮するものである。 Acrylonitrile compounds represented by a one of the active ingredients used in the the invention or the method in the present compositions the formula (1) are acting conventional organochlorine insecticides, organophosphorus insecticides , carbamate is different from the drugs, such as insecticides and pyrethroids, also with respect to certain pests residual effect also provided with occupied when I die at a low dose, resulting in remarkable control effect it is intended to exhibit. 加えて、式(1)で表されるアクリロニトリル化合物は、ある種の病害に対し低薬量で予防活性、あるいは治病活性を示し、結果的に顕著な防除効果を発揮するものである。 In addition, acrylonitrile compounds represented by the formula (1) is prevented by a low dose to certain disease activity, or shows a Chibyo activity is intended to exert a resultant remarkable controlling effect. しかしながら、いうまでもなくこの式(1)で表されるアクリロニトリル化合物のみを使用することで全ての分野の全ての害虫、あるいは病害を防除することは不可能である。 However, it is needless to say that control all pests or diseases, all areas by using only the acrylonitrile compounds of the formula (1) is impossible.
【0032】 [0032]
本発明の式(1)で表されるアクリロニトリル化合物の中で、殺虫、殺ダニ又は殺線虫効果が高く、かつ哺乳動物、魚類および天敵等の有用生物に対して悪影響が少ない点で好ましい化合物は、以下の第1表に示す化合物である。 Among the acrylonitrile compounds represented by the formula (1) of the present invention, insecticidal, acaricidal or nematocidal effect is high and mammals, fish and preferred compounds in view is less adverse effect on useful organisms such as predators is a compound shown in table 1 below. 尚、第1表中の略号はそれぞれ以下の意味を示す。 Incidentally, abbreviations in Table 1 have the following meanings respectively.
【0033】 [0033]
Me:メチル基、Et:エチル基、Pr:プロピル基、Bu:ブチル基、Ph:フェニル基、i:イソ、t:ターシャリー。 Me: methyl group, Et: ethyl group, Pr: propyl group, Bu: butyl group, Ph: phenyl group, i: iso, t: tertiary.
【0034】 [0034]
また、第1表中の置換基Aの略号はそれぞれ以下の意味を示す。 Also, abbreviations of substituents A in Table 1 have the following meanings respectively.
【0035】 [0035]
【化14】 [Of 14]
【0036】 [0036]
〔第1表〕 [Table 1]
【0037】 [0037]
【化15】 [Of 15]
【0038】 [0038]
【表1】 [Table 1]
【0039】 [0039]
また、式(1)で表されるアクリロニトリル化合物と共に用いられる、もう一方の有効成分化合物は、殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア化合物として公知のものであり、以下の第2表に化合物No. Also, used with an acrylonitrile compound represented by the formula (1), the other active ingredient compound are those known insecticidal, as acaricidal, nematicidal, fungicidal or bactericidal compounds, Table 2 below compound No. と共に示す。 Together with. そして、これらの化合物には抵抗性害虫あるいは耐性菌の出現、更に殺虫殺菌スペクトラムや残効性の不足により、薬剤の散布薬量、散布回数が増加する傾向にあり、防除効果のみならず、人畜あるいは水生生物に対する危険性の増加など、環境安全性の面からも改善が求められているものもある。 The appearance of these resistant pests or resistant bacteria to the compound, the more the lack of insecticidal fungicidal spectrum and residual activity, application dose of the drug, there is a tendency that spraying number is increased, not only the control effect, humans and animals or an increase of the risk to aquatic organisms, some of which improved in terms of environmental safety has been desired.
【0040】 [0040]
【表2】 [Table 2]
【0041】 [0041]
本発明組成物及び本発明方法の特徴は、第1に、各薬剤の単独での施用の場合に比べ、その殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア効力が明らかに増強されるとともに、即効的な殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア効果が付与されることである。 Feature of the present invention compositions and method of the present invention, the first, compared to the case of application in the sole of each agent, the insecticidal, acaricidal, nematicidal, fungicidal or with bactericides efficacy is enhanced obviously is that the rapid-acting insecticidal, acaricidal, nematicidal, fungicidal or bactericidal effect is applied. 第2に、既存の殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア剤に観られない広い殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリアスペクトラムや、長い残効性が誘導されることである。 Second, existing insecticidal, acaricidal, nematocidal, broad insecticidal not be seen in the sterilization, bactericides, acaricides, nematicidal, fungicidal or killing and bacteria spectrum, long the residual activity is induced it is. 第3に、各薬剤を単独で使用した場合に比べ、投下薬量を低下させうることである。 Third, compared with the case of using each agent alone it is that may reduce the dropped application dose.
【0042】 [0042]
即ち、本発明組成物及び本発明方法は、相乗的殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア効果を奏するものである。 That is, the present invention compositions and process of this invention are those which exhibit synergistic insecticidal, acaricidal, nematicidal, fungicidal or bactericidal effect. この相乗的殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア効果は、各単剤の有する殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア効果からは予測し得ぬものであり、本発明組成物及び本発明方法の有用性は各種病害虫に対して各化合物を単独で使用するよりも確実な防除効果を発揮し得る点にあるといえる。 The synergistic insecticidal, acaricidal, nematicidal, fungicidal or bactericidal effect, insecticidal included in each single agent, acaricidal, nematocidal, it is predicted N. things from sterilization or bactericidal effect, the present invention utility of the compositions and process of this invention can be said to be in a point capable of exhibiting reliable control effect than using each compound alone against various pests.
【0043】 [0043]
上記の第2表に示した化合物の中で、式(1)で表されるアクリロニトリル化合物と組み合わせることにより、特にダニに対する防除効果が、相乗的により向上する化合物を、以下の第3表に示す。 Among the compounds shown in Table 2 above, by combining acrylonitrile compound represented by the formula (1), the controlling effect particularly against mites, compounds that enhance the synergistic, shown below in Table 3 .
【0044】 [0044]
【表3】 [Table 3]
【0045】 [0045]
次に、相乗的病害虫防除効果を奏する化合物の組合せの具体例を以下に挙げる。 Next, Specific examples of the combination of compounds exhibits a synergistic pest control effect below. 以下の表記において、例えば「1+a」は、第1表のNo. In the following notation, for example "1 + a" is the Table 1 No. 1の化合物と、第2表のNo. And one of the compounds of Table 2 No. aのアシヘ゛ンソ゛ラル−S−メチルの組合せを表している。 It represents a combination of Ashihe Bu Nso Bu Lal -S- methyl a.
【0046】 [0046]
化合物の組合せの例:1+a,1+b,1+c,1+d,1+e,1+f,1+g,1+h,1+i,1+j,1+k,1+l,1+m,1+n,1+o,1+p,1+q,1+r,1+s,1+t,1+u,1+v,1+w,1+x,1+y,1+z,1+aa,1+ab,1+ac,1+ad,1+ae,1+af,1+ag,1+ah,1+ai,1+aj,1+ak,1+al,1+am,1+an,1+ao,1+ap,1+aq,1+ar,1+as,1+at,1+au,1+av,1+aw,1+ax,1+ay,1+az,1+ba,1+bb,1+bc,1+bd,1+be,1+bf,1+bg,1+bh,1+bi,1+bj,1+bk,1+bl,1+bm,1+bn,1+bo,1+bp,1+bq,1+br Combination examples of compounds: 1 + a, 1 + b, 1 + c, 1 + d, 1 + e, 1 + f, 1 + g, 1 + h, 1 + i, 1 + j, 1 + k, 1 + l, 1 + m, 1 + n, 1 + o, 1 + p, 1 + q, 1 + r, 1 + s, 1 + t, 1 + u, 1 + v, 1 + w, 1 + x, 1 + y, 1 + z, 1 + aa, 1 + ab, 1 + ac, 1 + ad, 1 + ae, 1 + af, 1 + ag, 1 + ah, 1 + ai, 1 + aj, 1 + ak, 1 + al, 1 + am, 1 + an, 1 + ao, 1 + ap, 1 + aq, 1 + ar, 1 + as, 1 + at, 1 + au, 1 + av, 1 + aw, 1 + ax, 1 + ay, 1 + az, 1 + ba, 1 + bb, 1 + bc, 1 + bd, 1 + be, 1 + bf, 1 + bg, 1 + bh, 1 + bi, 1 + bj, 1 + bk, 1 + bl, 1 + bm, 1 + bn, 1 + bo, 1 + bp, 1 + bq, 1 + br 1+bs,1+bt,1+bu,1+bv,1+bw,1+bx,1+by,1+bz,1+ca,1+cb,1+cc,1+cd,1+ce,1+cf,1+cg,1+ch,1+ci,1+cj,1+ck,1+cl,1+cm,1+cn,1+co,1+cp,1+cq,1+cr,1+cs,1+ct,1+cu,1+cv,1+cw,1+cx,1+cy,1+cz,1+da,1+db,1+dc,1+dd,1+de,1+df,1+dg,1+dh,1+di,1+dj,1+dk,1+dl,1+dm,1+dn,1+do,1+dp,1+dq,1+dr,1+ds,1+dt,1+du,1+dv,1+dw,1+dx,1+dy,1+dz,1+ea,1+eb,1+ec,1+ed,1+ee,1+ef,1+ 1 + bs, 1 + bt, 1 + bu, 1 + bv, 1 + bw, 1 + bx, 1 + by, 1 + bz, 1 + ca, 1 + cb, 1 + cc, 1 + cd, 1 + ce, 1 + cf, 1 + cg, 1 + ch, 1 + ci, 1 + cj, 1 + ck, 1 + cl, 1 + cm, 1 + cn, 1 + co, 1 + cp, 1 + cq, 1 + cr, 1 + cs, 1 + ct, 1 + cu, 1 + cv, 1 + cw, 1 + cx, 1 + cy, 1 + cz, 1 + da, 1 + db, 1 + dc, 1 + dd, 1 + de, 1 + df, 1 + dg, 1 + dh, 1 + di, 1 + dj, 1 + dk, 1 + dl, 1 + dm, 1 + dn, 1 + do, 1 + dp, 1 + dq, 1 + dr, 1 + ds, 1 + dt, 1 + du, 1 + dv, 1 + dw, 1 + dx, 1 + dy, 1 + dz, 1 + ea, 1 + eb, 1 + ec, 1 + ed, 1 + ee, 1 + ef, 1 + g,1+eh,1+ei,1+ej,1+ek,1+el,1+em,1+en,1+eo,1+ep,1+eq,1+er,1+es,1+et,1+eu,1+ev,1+ew,1+ex,1+ey,1+ez,1+fa,1+fb,1+fc,1+fd,1+fe,1+ff,1+fg,1+fh,1+fi,1+fj,1+fk,1+fl,1+fm,1+fn,1+fo,1+fp,1+fq,1+fr,1+fs,1+ft,1+fu,1+fv,1+fw,1+fx,1+fy,1+fz,1+ga,1+gb,1+gc,1+gd,1+ge,1+gf,1+gg,1+gh,1+gi,1+gj,1+gk,1+gl,1+gm,1+gn,1+go,1+gp,1+gq,1+gr,1+gs,1+gt,1+gu,1 g, 1 + eh, 1 + ei, 1 + ej, 1 + ek, 1 + el, 1 + em, 1 + en, 1 + eo, 1 + ep, 1 + eq, 1 + er, 1 + es, 1 + et, 1 + eu, 1 + ev, 1 + ew, 1 + ex, 1 + ey, 1 + ez, 1 + fa, 1 + fb, 1 + fc, 1 + fd, 1 + fe, 1 + ff, 1 + fg, 1 + fh, 1 + fi, 1 + fj, 1 + fk, 1 + fl, 1 + fm, 1 + fn, 1 + fo, 1 + fp, 1 + fq, 1 + fr, 1 + fs, 1 + ft, 1 + fu, 1 + fv, 1 + fw, 1 + fx, 1 + fy, 1 + fz, 1 + ga, 1 + gb, 1 + gc, 1 + gd, 1 + ge, 1 + gf, 1 + gg, 1 + gh, 1 + gi, 1 + gj, 1 + gk, 1 + gl, 1 + gm, 1 + gn, 1 + go, 1 + gp, 1 + gq, 1 + gr, 1 + gs, 1 + gt, 1 + gu, 1 +gv,1+gw,1+gx,1+gy,1+gz,1+ha,1+hb,1+hc,1+hd,1+he,1+hf,1+hg,1+hh,1+hi,1+hj,1+hk,1+hl,1+hm,1+hn,1+ho,1+hp,1+hq,1+hr,1+hs,1+ht,1+hu,1+hv,1+hw,1+hx,1+hy,1+hz,1+ia,1+ib,1+ic,1+id,1+ie,1+if,1+ig,1+ih,1+ii,1+ij,1+ik,1+il,1+im,1+in,1+io,1+ip,1+iq,1+ir,1+is,1+it,1+iu,1+iv,1+iw,1+ix,1+iy,1+iz,1+ja,1+jb,1+jc,1+jd,1+je,1+jf,1+jg,1+jh,1+ji,1+jj + Gv, 1 + gw, 1 + gx, 1 + gy, 1 + gz, 1 + ha, 1 + hb, 1 + hc, 1 + hd, 1 + he, 1 + hf, 1 + hg, 1 + hh, 1 + hi, 1 + hj, 1 + hk, 1 + hl, 1 + hm, 1 + hn, 1 + ho, 1 + hp, 1 + hq, 1 + hr, 1 + hs, 1 + ht, 1 + hu, 1 + hv, 1 + hw, 1 + hx, 1 + hy, 1 + hz, 1 + ia, 1 + ib, 1 + ic, 1 + id, 1 + ie, 1 + if, 1 + ig, 1 + ih, 1 + ii, 1 + ij, 1 + ik, 1 + il, 1 + im, 1 + in, 1 + io, 1 + ip, 1 + iq, 1 + ir, 1 + is, 1 + it, 1 + iu, 1 + iv, 1 + iw, 1 + ix, 1 + iy, 1 + iz, 1 + ja, 1 + jb, 1 + jc, 1 + jd, 1 + je, 1 + jf, 1 + jg, 1 + jh, 1 + ji, 1 + jj 1+jk,1+jl,1+jm,1+jn,1+jo,1+jp,1+jq,1+jr,1+js,1+jt,1+ju,1+jv,1+jw,1+jx,1+jy,1+jz,1+ka,1+kb,1+kc,1+kd,1+ke,1+kf,1+kg,1+kh,1+ki,1+kj,1+kk,1+kl,1+km,1+kn,1+ko,1+kp,1+kq,1+kr,1+ks,1+kt,1+ku,1+kv,1+kw,1+kx,1+ky,1+kz,1+la,1+lb,1+lc,1+ld,1+le,1+lf,1+lg,1+lh,1+li,1+lj,1+lk,1+ll,1+lm,1+ln,1+lo,1+lp,1+lq,1+lr,1+ls,1+lt,1+lu,1+lv,1+lw,1+lx,1+ 1 + jk, 1 + jl, 1 + jm, 1 + jn, 1 + jo, 1 + jp, 1 + jq, 1 + jr, 1 + js, 1 + jt, 1 + ju, 1 + jv, 1 + jw, 1 + jx, 1 + jy, 1 + jz, 1 + ka, 1 + kb, 1 + kc, 1 + kd, 1 + ke, 1 + kf, 1 + kg, 1 + kh, 1 + ki, 1 + kj, 1 + kk, 1 + kl, 1 + km, 1 + kn, 1 + ko, 1 + kp, 1 + kq, 1 + kr, 1 + ks, 1 + kt, 1 + ku, 1 + kv, 1 + kw, 1 + kx, 1 + ky, 1 + kz, 1 + la, 1 + lb, 1 + lc, 1 + ld, 1 + le, 1 + lf, 1 + lg, 1 + lh, 1 + li, 1 + lj, 1 + lk, 1 + ll, 1 + lm, 1 + ln, 1 + lo, 1 + lp, 1 + lq, 1 + lr, 1 + ls, 1 + lt, 1 + lu, 1 + lv, 1 + lw, 1 + lx, 1 + y,2+a,2+b,2+c,2+d,2+e,2+f,2+g,2+h,2+i,2+j,2+k,2+l,2+m,2+n,2+o,2+p,2+q,2+r,2+s,2+t,2+u,2+v,2+w,2+x,2+y,2+z,2+aa,2+ab,2+ac,2+ad,2+ae,2+af,2+ag,2+ah,2+ai,2+aj,2+ak,2+al,2+am,2+an,2+ao,2+ap,2+aq,2+ar,2+as,2+at,2+au,2+av,2+aw,2+ax,2+ay,2+az,2+ba,2+bb,2+bc,2+bd,2+be,2+bf,2+bg,2+bh,2+bi,2+bj,2+bk,2+bl,2+bm,2+bn,2+bo,2+bp,2+bq,2+br,2+bs,2+ y, 2 + a, 2 + b, 2 + c, 2 + d, 2 + e, 2 + f, 2 + g, 2 + h, 2 + i, 2 + j, 2 + k, 2 + l, 2 + m, 2 + n, 2 + o, 2 + p, 2 + q, 2 + r, 2 + s, 2 + t, 2 + u, 2 + v, 2 + w, 2 + x, 2 + y, 2 + z, 2 + aa, 2 + ab, 2 + ac, 2 + ad, 2 + ae, 2 + af, 2 + ag, 2 + ah, 2 + ai, 2 + aj, 2 + ak, 2 + al, 2 + am, 2 + an, 2 + ao, 2 + ap, 2 + aq, 2 + ar, 2 + as, 2 + at, 2 + au, 2 + av, 2 + aw, 2 + ax, 2 + ay, 2 + az, 2 + ba, 2 + bb, 2 + bc, 2 + bd, 2 + be, 2 + bf, 2 + bg, 2 + bh, 2 + bi, 2 + bj, 2 + bk, 2 + bl, 2 + bm, 2 + bn, 2 + bo, 2 + bp, 2 + bq, 2 + br, 2 + bs, 2 + bt,2+bu,2+bv,2+bw,2+bx,2+by,2+bz,2+ca,2+cb,2+cc,2+cd,2+ce,2+cf,2+cg,2+ch,2+ci,2+cj,2+ck,2+cl,2+cm,2+cn,2+co,2+cp,2+cq,2+cr,2+cs,2+ct,2+cu,2+cv,2+cw,2+cx,2+cy,2+cz,2+da,2+db,2+dc,2+dd,2+de,2+df,2+dg,2+dh,2+di,2+dj,2+dk,2+dl,2+dm,2+dn,2+do,2+dp,2+dq,2+dr,2+ds,2+dt,2+du,2+dv,2+dw,2+dx,2+dy,2+dz,2+ea,2+eb,2+ec,2+ed,2+ee,2+ef,2+eg,2+eh, bt, 2 + bu, 2 + bv, 2 + bw, 2 + bx, 2 + by, 2 + bz, 2 + ca, 2 + cb, 2 + cc, 2 + cd, 2 + ce, 2 + cf, 2 + cg, 2 + ch, 2 + ci, 2 + cj, 2 + ck, 2 + cl, 2 + cm, 2 + cn, 2 + co, 2 + cp, 2 + cq, 2 + cr, 2 + cs, 2 + ct, 2 + cu, 2 + cv, 2 + cw, 2 + cx, 2 + cy, 2 + cz, 2 + da, 2 + db, 2 + dc, 2 + dd, 2 + de, 2 + df, 2 + dg, 2 + dh, 2 + di, 2 + dj, 2 + dk, 2 + dl, 2 + dm, 2 + dn, 2 + do, 2 + dp, 2 + dq, 2 + dr, 2 + ds, 2 + dt, 2 + du, 2 + dv, 2 + dw, 2 + dx, 2 + dy, 2 + dz, 2 + ea, 2 + eb, 2 + ec, 2 + ed, 2 + ee, 2 + ef, 2 + eg, 2 + eh, +ei,2+ej,2+ek,2+el,2+em,2+en,2+eo,2+ep,2+eq,2+er,2+es,2+et,2+eu,2+ev,2+ew,2+ex,2+ey,2+ez,2+fa,2+fb,2+fc,2+fd,2+fe,2+ff,2+fg,2+fh,2+fi,2+fj,2+fk,2+fl,2+fm,2+fn,2+fo,2+fp,2+fq,2+fr,2+fs,2+ft,2+fu,2+fv,2+fw,2+fx,2+fy,2+fz,2+ga,2+gb,2+gc,2+gd,2+ge,2+gf,2+gg,2+gh,2+gi,2+gj,2+gk,2+gl,2+gm,2+gn,2+go,2+gp,2+gq,2+gr,2+gs,2+gt,2+gu,2+gv,2+g + Ei, 2 + ej, 2 + ek, 2 + el, 2 + em, 2 + en, 2 + eo, 2 + ep, 2 + eq, 2 + er, 2 + es, 2 + et, 2 + eu, 2 + ev, 2 + ew, 2 + ex, 2 + ey, 2 + ez, 2 + fa, 2 + fb, 2 + fc, 2 + fd, 2 + fe, 2 + ff, 2 + fg, 2 + fh, 2 + fi, 2 + fj, 2 + fk, 2 + fl, 2 + fm, 2 + fn, 2 + fo, 2 + fp, 2 + fq, 2 + fr, 2 + fs, 2 + ft, 2 + fu, 2 + fv, 2 + fw, 2 + fx, 2 + fy, 2 + fz, 2 + ga, 2 + gb, 2 + gc, 2 + gd, 2 + ge, 2 + gf, 2 + gg, 2 + gh, 2 + gi, 2 + gj, 2 + gk, 2 + gl, 2 + gm, 2 + gn, 2 + go, 2 + gp, 2 + gq, 2 + gr, 2 + gs, 2 + gt, 2 + gu, 2 + gv, 2 + g ,2+gx,2+gy,2+gz,2+ha,2+hb,2+hc,2+hd,2+he,2+hf,2+hg,2+hh,2+hi,2+hj,2+hk,2+hl,2+hm,2+hn,2+ho,2+hp,2+hq,2+hr,2+hs,2+ht,2+hu,2+hv,2+hw,2+hx,2+hy,2+hz,2+ia,2+ib,2+ic,2+id,2+ie,2+if,2+ig,2+ih,2+ii,2+ij,2+ik,2+il,2+im,2+in,2+io,2+ip,2+iq,2+ir,2+is,2+it,2+iu,2+iv,2+iw,2+ix,2+iy,2+iz,2+ja,2+jb,2+jc,2+jd,2+je,2+jf,2+jg,2+jh,2+ji,2+jj,2+jk,2+ , 2 + gx, 2 + gy, 2 + gz, 2 + ha, 2 + hb, 2 + hc, 2 + hd, 2 + he, 2 + hf, 2 + hg, 2 + hh, 2 + hi, 2 + hj, 2 + hk, 2 + hl, 2 + hm, 2 + hn, 2 + ho, 2 + hp, 2 + hq, 2 + hr, 2 + hs, 2 + ht, 2 + hu, 2 + hv , 2 + hw, 2 + hx, 2 + hy, 2 + hz, 2 + ia, 2 + ib, 2 + + ic, 2 + id, 2 + ie, 2 + if, 2 ig, 2 + ih, 2 + ii, 2 + ij, 2 + ik, 2 + il, 2 + im, 2 + in, 2 + io, 2 + ip, 2 + iq, 2 + ir, 2 + is, 2 + it, 2 + iu , 2 + iv, 2 + iw, 2 + ix, 2 + iy, 2 + iz, 2 + ja, 2 + jb, 2 + jc, 2 + jd, 2 + je, 2 + jf, 2 + jg, 2 + jh, 2 + ji, 2 + jj, 2 + jk, 2 + jl,2+jm,2+jn,2+jo,2+jp,2+jq,2+jr,2+js,2+jt,2+ju,2+jv,2+jw,2+jx,2+jy,2+jz,2+ka,2+kb,2+kc,2+kd,2+ke,2+kf,2+kg,2+kh,2+ki,2+kj,2+kk,2+kl,2+km,2+kn,2+ko,2+kp,2+kq,2+kr,2+ks,2+kt,2+ku,2+kv,2+kw,2+kx,2+ky,2+kz,2+la,2+lb,2+lc,2+ld,2+le,2+lf,2+lg,2+lh,2+li,2+lj,2+lk,2+ll,2+lm,2+ln,2+lo,2+lp,2+lq,2+lr,2+ls,2+lt,2+lu,2+lv,2+lw,2+lx,2+ly,3+a,3 jl, 2 + jm, 2 + jn, 2 + jo, 2 + jp, 2 + jq, 2 + jr, 2 + js, 2 + jt, 2 + ju, 2 + jv, 2 + jw, 2 + jx, 2 + jy, 2 + jz, 2 + ka, 2 + kb, 2 + kc, 2 + kd, 2 + ke, 2 + kf, 2 + kg, 2 + kh, 2 + ki, 2 + kj, 2 + kk, 2 + kl, 2 + km, 2 + kn, 2 + ko, 2 + kp, 2 + kq, 2 + kr, 2 + ks, 2 + kt, 2 + ku, 2 + kv, 2 + kw, 2 + kx, 2 + ky, 2 + kz, 2 + la, 2 + lb, 2 + lc, 2 + ld, 2 + le, 2 + lf, 2 + lg, 2 + lh, 2 + li, 2 + lj, 2 + lk, 2 + ll, 2 + lm, 2 + ln, 2 + lo, 2 + lp, 2 + lq, 2 + lr, 2 + ls, 2 + lt, 2 + lu, 2 + lv, 2 + lw, 2 + lx, 2 + ly, 3 + a, 3 b,3+c,3+d,3+e,3+f,3+g,3+h,3+i,3+j,3+k,3+l,3+m,3+n,3+o,3+p,3+q,3+r,3+s,3+t,3+u,3+v,3+w,3+x,3+y,3+z,3+aa,3+ab,3+ac,3+ad,3+ae,3+af,3+ag,3+ah,3+ai,3+aj,3+ak,3+al,3+am,3+an,3+ao,3+ap,3+aq,3+ar,3+as,3+at,3+au,3+av,3+aw,3+ax,3+ay,3+az,3+ba,3+bb,3+bc,3+bd,3+be,3+bf,3+bg,3+bh,3+bi,3+bj,3+bk,3+bl,3+bm,3+bn,3+bo,3+bp,3+bq,3+br,3+bs,3+bt,3+bu b, 3 + c, 3 + d, 3 + e, 3 + f, 3 + g, 3 + h, 3 + i, 3 ​​+ j, 3 + k, 3 + l, 3 + m, 3 + n, 3 + o, 3 + p, 3 + q, 3 + r, 3 + s, 3 + t, 3 + u, 3 + v, 3 + w, 3 + x, 3 + y, 3 + z, 3 + aa, 3 + ab, 3 + ac, 3 + ad, 3 + ae, 3 + af, 3 + ag, 3 + ah, 3 + ai, 3 + aj, 3 + ak, 3 + al, 3 + am, 3 + an, 3 + ao, 3 + ap, 3 + aq, 3 + ar, 3 + as, 3 + at, 3 + au, 3 + av, 3 + aw, 3 + ax, 3 + ay, 3 + az, 3 + ba, 3 + bb, 3 + bc, 3 + bd, 3 + be, 3 + bf, 3 + bg, 3 + bh, 3 + bi, 3 + bj, 3 + bk, 3 + bl, 3 + bm, 3 + bn, 3 + bo, 3 + bp, 3 + bq, 3 + br, 3 + bs, 3 + bt, 3 + bu 3+bv,3+bw,3+bx,3+by,3+bz,3+ca,3+cb,3+cc,3+cd,3+ce,3+cf,3+cg,3+ch,3+ci,3+cj,3+ck,3+cl,3+cm,3+cn,3+co,3+cp,3+cq,3+cr,3+cs,3+ct,3+cu,3+cv,3+cw,3+cx,3+cy,3+cz,3+da,3+db,3+dc,3+dd,3+de,3+df,3+dg,3+dh,3+di,3+dj,3+dk,3+dl,3+dm,3+dn,3+do,3+dp,3+dq,3+dr,3+ds,3+dt,3+du,3+dv,3+dw,3+dx,3+dy,3+dz,3+ea,3+eb,3+ec,3+ed,3+ee,3+ef,3+eg,3+eh,3+ei,3+e 3 + bv, 3 + bw, 3 + bx, 3 + by, 3 + bz, 3 + ca, 3 + cb, 3 + cc, 3 + cd, 3 + ce, 3 + cf, 3 + cg, 3 + ch, 3 + ci, 3 + cj, 3 + ck, 3 + cl, 3 + cm, 3 + cn, 3 + co, 3 + cp, 3 + cq, 3 + cr, 3 + cs, 3 + ct, 3 + cu, 3 + cv, 3 + cw, 3 + cx, 3 + cy, 3 + cz, 3 + da, 3 + db, 3 + dc, 3 + dd, 3 + de, 3 + df, 3 + dg, 3 + dh, 3 + di, 3 + dj, 3 + dk, 3 + dl, 3 + dm, 3 + dn, 3 + do, 3 + dp, 3 + dq, 3 + dr, 3 + ds, 3 + dt, 3 + du, 3 + dv, 3 + dw, 3 + dx, 3 + dy, 3 + dz, 3 + ea, 3 + eb, 3 + ec, 3 + ed, 3 + ee, 3 + ef, 3 + eg, 3 + eh, 3 + ei, 3 + e j,3+ek,3+el,3+em,3+en,3+eo,3+ep,3+eq,3+er,3+es,3+et,3+eu,3+ev,3+ew,3+ex,3+ey,3+ez,3+fa,3+fb,3+fc,3+fd,3+fe,3+ff,3+fg,3+fh,3+fi,3+fj,3+fk,3+fl,3+fm,3+fn,3+fo,3+fp,3+fq,3+fr,3+fs,3+ft,3+fu,3+fv,3+fw,3+fx,3+fy,3+fz,3+ga,3+gb,3+gc,3+gd,3+ge,3+gf,3+gg,3+gh,3+gi,3+gj,3+gk,3+gl,3+gm,3+gn,3+go,3+gp,3+gq,3+gr,3+gs,3+gt,3+gu,3+gv,3+gw,3+gx,3 j, 3 + ek, 3 + el, 3 + em, 3 + en, 3 + eo, 3 + ep, 3 + eq, 3 + er, 3 + es, 3 + et, 3 + eu, 3 + ev, 3 + ew, 3 + ex, 3 + ey, 3 + ez, 3 + fa, 3 + fb, 3 + fc, 3 + fd, 3 + fe, 3 + ff, 3 + fg, 3 + fh, 3 + fi, 3 + fj, 3 + fk, 3 + fl, 3 + fm, 3 + fn, 3 + fo, 3 + fp, 3 + fq, 3 + fr, 3 + fs, 3 + ft, 3 + fu, 3 + fv, 3 + fw, 3 + fx, 3 + fy, 3 + fz, 3 + ga, 3 + gb, 3 + gc, 3 + gd, 3 + ge, 3 + gf, 3 + gg, 3 + gh, 3 + gi, 3 + gj, 3 + gk, 3 + gl, 3 + gm, 3 + gn, 3 + go, 3 + gp, 3 + gq, 3 + gr, 3 + gs, 3 + gt, 3 + gu, 3 + gv, 3 + gw, 3 + gx, 3 gy,3+gz,3+ha,3+hb,3+hc,3+hd,3+he,3+hf,3+hg,3+hh,3+hi,3+hj,3+hk,3+hl,3+hm,3+hn,3+ho,3+hp,3+hq,3+hr,3+hs,3+ht,3+hu,3+hv,3+hw,3+hx,3+hy,3+hz,3+ia,3+ib,3+ic,3+id,3+ie,3+if,3+ig,3+ih,3+ii,3+ij,3+ik,3+il,3+im,3+in,3+io,3+ip,3+iq,3+ir,3+is,3+it,3+iu,3+iv,3+iw,3+ix,3+iy,3+iz,3+ja,3+jb,3+jc,3+jd,3+je,3+jf,3+jg,3+jh,3+ji,3+jj,3+jk,3+jl,3+jm gy, 3 + gz, 3 + ha, 3 + hb, 3 + hc, 3 + hd, 3 + he, 3 + hf, 3 + hg, 3 + hh, 3 + hi, 3 + hj, 3 + hk, 3 + hl, 3 + hm, 3 + hn, 3 + ho, 3 + hp, 3 + hq, 3 + hr, 3 + hs, 3 + ht, 3 + hu, 3 + hv, 3 + hw, 3 + hx, 3 + hy, 3 + hz, 3 + ia, 3 + ib, 3 + ic, 3 + id, 3 + ie, 3 + if, 3 + ig, 3 + ih, 3 + ii, 3 + ij, 3 + ik, 3 + il, 3 + im, 3 + in, 3 + io, 3 + ip, 3 + iq, 3 + ir, 3 + is, 3 + it, 3 + iu, 3 + iv, 3 + iw, 3 + ix, 3 + iy, 3 + iz, 3 + ja, 3 + jb, 3 + jc, 3 + jd, 3 + je, 3 + jf, 3 + jg, 3 + jh, 3 + ji, 3 + jj, 3 + jk, 3 + jl, 3 + jm 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+f,5+g,5+h,5+i,5+j,5+k,5+l,5+m,5+n,5+o,5+p,5+q,5+r,5+s,5+t,5+u,5+v,5+w,5+x,5+y,5+z,5+aa,5+ab,5+ac,5+ad,5+ae,5+af,5+ag,5+ah,5+ai,5+aj,5+ak,5+al,5+am,5+an,5+ao,5+ap,5+aq,5+ar,5+as,5+at,5+au,5+av,5+aw,5+ax,5+ay,5+az,5+ba,5+bb,5+bc,5+bd,5+be,5+bf,5+bg,5+bh,5+bi,5+bj,5+bk,5+bl,5+bm,5+bn,5+bo,5+bp,5+bq,5+br,5+bs,5+bt,5+bu,5+bv,5+bw,5+bx, + F, 5 + g, 5 + h, 5 + i, 5 + j, 5 + k, 5 + l, 5 + m, 5 + n, 5 + o, 5 + p, 5 + q, 5 + r, 5 + s, 5 + t, 5 + u, 5 + v, 5 + w, 5 + x, 5 + y, 5 + z, 5 + aa, 5 + ab, 5 + ac, 5 + ad, 5 + ae, 5 + af, 5 + ag, 5 + ah, 5 + ai, 5 + aj, 5 + ak, 5 + al, 5 + am, 5 + an, 5 + ao, 5 + ap, 5 + aq, 5 + ar, 5 + as, 5 + at, 5 + au, 5 + av, 5 + aw, 5 + ax, 5 + ay, 5 + az, 5 + ba, 5 + bb, 5 + bc, 5 + bd, 5 + be, 5 + bf, 5 + bg, 5 + bh, 5 + bi, 5 + bj, 5 + bk, 5 + bl, 5 + bm, 5 + bn, 5 + bo, 5 + bp, 5 + bq, 5 + br, 5 + bs, 5 + bt, 5 + bu, 5 + bv, 5 + bw, 5 + bx, 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hb,5+hc,5+hd,5+he,5+hf,5+hg,5+hh,5+hi,5+hj,5+hk,5+hl,5+hm,5+hn,5+ho,5+hp,5+hq,5+hr,5+hs,5+ht,5+hu,5+hv,5+hw,5+hx,5+hy,5+hz,5+ia,5+ib,5+ic,5+id,5+ie,5+if,5+ig,5+ih,5+ii,5+ij,5+ik,5+il,5+im,5+in,5+io,5+ip,5+iq,5+ir,5+is,5+it,5+iu,5+iv,5+iw,5+ix,5+iy,5+iz,5+ja,5+jb,5+jc,5+jd,5+je,5+jf,5+jg,5+jh,5+ji,5+jj,5+jk,5+jl,5+jm,5+jn,5+jo,5+jp, hb, 5 + hc, 5 + hd, 5 + he, 5 + hf, 5 + hg, 5 + hh, 5 + hi, 5 + hj, 5 + hk, 5 + hl, 5 + hm, 5 + hn, 5 + ho, 5 + hp, 5 + hq, 5 + hr, 5 + hs, 5 + ht, 5 + hu, 5 + hv, 5 + hw, 5 + hx, 5 + hy, 5 + hz, 5 + ia, 5 + ib, 5 + ic, 5 + id, 5 + ie, 5 + if, 5 + ig, 5 + ih, 5 + ii, 5 + ij, 5 + ik, 5 + il, 5 + im, 5 + in, 5 + io, 5 + ip, 5 + iq, 5 + ir, 5 + is, 5 + it, 5 + iu, 5 + iv, 5 + iw, 5 + ix, 5 + iy, 5 + iz, 5 + ja, 5 + jb, 5 + jc, 5 + jd, 5 + je, 5 + jf, 5 + jg, 5 + jh, 5 + ji, 5 + jj, 5 + jk, 5 + jl, 5 + jm, 5 + jn, 5 + jo, 5 + jp, 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6+fq,16+fr,16+fs,16+ft,16+fu,16+fv,16+fw,16+fx,16+fy,16+fz,16+ga,16+gb,16+gc,16+gd,16+ge,16+gf,16+gg,16+gh,16+gi,16+gj,16+gk,16+gl,16+gm,16+gn,16+go,16+gp,16+gq,16+gr,16+gs,16+gt,16+gu,16+gv,16+gw,16+gx,16+gy,16+gz,16+ha,16+hb,16+hc,16+hd,16+he,16+hf,16+hg,16+hh,16+hi,16+hj,16+hk,16+hl,16+hm,16+hn,16+ho,16+hp,16+hq,16+hr,16+hs,16+h 6 + fq, 16 + fr, 16 + fs, 16 + ft, 16 + fu, 16 + fv, 16 + fw, 16 + fx, 16 + fy, 16 + fz, 16 + ga, 16 + gb, 16 + gc, 16 + gd, 16 + ge, 16 + gf, 16 + gg, 16 + gh, 16 + gi, 16 + gj, 16 + gk, 16 + gl, 16 + gm, 16 + gn, 16 + go, 16 + gp, 16 + gq, 16 + gr, 16 + gs, 16 + gt, 16 + gu, 16 + gv, 16 + gw, 16 + gx, 16 + gy, 16 + gz, 16 + ha, 16 + hb, 16 + hc, 16 + hd, 16 + he, 16 + hf, 16 + hg, 16 + hh, 16 + hi, 16 + hj, 16 + hk, 16 + hl, 16 + hm, 16 + hn, 16 + ho, 16 + hp, 16 + hq, 16 + hr, 16 + hs, 16 + h 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7+c,17+d,17+e,17+f,17+g,17+h,17+i,17+j,17+k,17+l,17+m,17+n,17+o,17+p,17+q,17+r,17+s,17+t,17+u,17+v,17+w,17+x,17+y,17+z,17+aa,17+ab,17+ac,17+ad,17+ae,17+af,17+ag,17+ah,17+ai,17+aj,17+ak,17+al,17+am,17+an,17+ao,17+ap,17+aq,17+ar,17+as,17+at,17+au,17+av,17+aw,17+ax,17+ay,17+az,17+ba,17+bb,17+bc,17+bd,17+be,17+bf,17+bg,17+bh,17+bi,17+b 7 + c, 17 + d, 17 + e, 17 + f, 17 + g, 17 + h, 17 + i, 17 + j, 17 + k, 17 + l, 17 + m, 17 + n, 17 + o, 17 + p, 17 + q, 17 + r, 17 + s, 17 + t, 17 + u, 17 + v, 17 + w, 17 + x, 17 + y, 17 + z, 17 + aa, 17 + ab, 17 + ac, 17 + ad, 17 + ae, 17 + af, 17 + ag, 17 + ah, 17 + ai, 17 + aj, 17 + ak, 17 + al, 17 + am, 17 + an, 17 + ao, 17 + ap, 17 + aq, 17 + ar, 17 + as, 17 + at, 17 + au, 17 + av, 17 + aw, 17 + ax, 17 + ay, 17 + az, 17 + ba, 17 + bb, 17 + bc, 17 + bd, 17 + be, 17 + bf, 17 + bg, 17 + bh, 17 + bi, 17 + b ,17+bk,17+bl,17+bm,17+bn,17+bo,17+bp,17+bq,17+br,17+bs,17+bt,17+bu,17+bv,17+bw,17+bx,17+by,17+bz,17+ca,17+cb,17+cc,17+cd,17+ce,17+cf,17+cg,17+ch,17+ci,17+cj,17+ck,17+cl,17+cm,17+cn,17+co,17+cp,17+cq,17+cr,17+cs,17+ct,17+cu,17+cv,17+cw,17+cx,17+cy,17+cz,17+da,17+db,17+dc,17+dd,17+de,17+df,17+dg,17+dh,17+di,17+dj,17+dk,17+dl,17+dm,1 , 17 + bk, 17 + bl, 17 + bm, 17 + bn, 17 + bo, 17 + bp, 17 + bq, 17 + br, 17 + bs, 17 + bt, 17 + bu, 17 + bv, 17 + bw, 17 + bx, 17 + by, 17 + bz, 17 + ca, 17 + cb, 17 + cc, 17 + cd, 17 + ce, 17 + cf, 17 + cg, 17 + ch, 17 + ci , 17 + cj, 17 + ck, 17 + cl, 17 + cm, 17 + cn, 17 + co, 17 + cp, 17 + cq, 17 + cr, 17 + cs, 17 + ct, 17 + cu, 17 + cv, 17 + cw, 17 + cx, 17 + cy, 17 + cz, 17 + da, 17 + db, 17 + dc, 17 + dd, 17 + de, 17 + df, 17 + dg, 17 + dh , 17 + di, 17 + dj, 17 + dk, 17 + dl, 17 + dm, 1 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hu,17+hv,17+hw,17+hx,17+hy,17+hz,17+ia,17+ib,17+ic,17+id,17+ie,17+if,17+ig,17+ih,17+ii,17+ij,17+ik,17+il,17+im,17+in,17+io,17+ip,17+iq,17+ir,17+is,17+it,17+iu,17+iv,17+iw,17+ix,17+iy,17+iz,17+ja,17+jb,17+jc,17+jd,17+je,17+jf,17+jg,17+jh,17+ji,17+jj,17+jk,17+jl,17+jm,17+jn,17+jo,17+jp,17+jq,17+jr,17+js,17+jt,17+ju,17+jv,17+jw,17+jx hu, 17 + hv, 17 + hw, 17 + hx, 17 + hy, 17 + hz, 17 + ia, 17 + ib, 17 + ic, 17 + id, 17 + ie, 17 + if, 17 + ig, 17 + ih, 17 + ii, 17 + ij, 17 + ik, 17 + il, 17 + im, 17 + in, 17 + io, 17 + ip, 17 + iq, 17 + ir, 17 + is, 17 + it, 17 + iu, 17 + iv, 17 + iw, 17 + ix, 17 + iy, 17 + iz, 17 + ja, 17 + jb, 17 + jc, 17 + jd, 17 + je, 17 + jf, 17 + jg, 17 + jh, 17 + ji, 17 + jj, 17 + jk, 17 + jl, 17 + jm, 17 + jn, 17 + jo, 17 + jp, 17 + jq, 17 + jr, 17 + js, 17 + jt, 17 + ju, 17 + jv, 17 + jw, 17 + jx 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8+hv,18+hw,18+hx,18+hy,18+hz,18+ia,18+ib,18+ic,18+id,18+ie,18+if,18+ig,18+ih,18+ii,18+ij,18+ik,18+il,18+im,18+in,18+io,18+ip,18+iq,18+ir,18+is,18+it,18+iu,18+iv,18+iw,18+ix,18+iy,18+iz,18+ja,18+jb,18+jc,18+jd,18+je,18+jf,18+jg,18+jh,18+ji,18+jj,18+jk,18+jl,18+jm,18+jn,18+jo,18+jp,18+jq,18+jr,18+js,18+jt,18+ju,18+jv,18+jw,18+jx,18+ 8 + hv, 18 + hw, 18 + hx, 18 + hy, 18 + hz, 18 + ia, 18 + ib, 18 + ic, 18 + id, 18 + ie, 18 + if, 18 + ig, 18 + ih, 18 + ii, 18 + ij, 18 + ik, 18 + il, 18 + im, 18 + in, 18 + io, 18 + ip, 18 + iq, 18 + ir, 18 + is, 18 + it, 18 + iu, 18 + iv, 18 + iw, 18 + ix, 18 + iy, 18 + iz, 18 + ja, 18 + jb, 18 + jc, 18 + jd, 18 + je, 18 + jf, 18 + jg, 18 + jh, 18 + ji, 18 + jj, 18 + jk, 18 + jl, 18 + jm, 18 + jn, 18 + jo, 18 + jp, 18 + jq, 18 + jr, 18 + js, 18 + jt, 18 + ju, 18 + jv, 18 + jw, 18 + jx, 18 + y,18+jz,18+ka,18+kb,18+kc,18+kd,18+ke,18+kf,18+kg,18+kh,18+ki,18+kj,18+kk,18+kl,18+km,18+kn,18+ko,18+kp,18+kq,18+kr,18+ks,18+kt,18+ku,18+kv,18+kw,18+kx,18+ky,18+kz,18+la,18+lb,18+lc,18+ld,18+le,18+lf,18+lg,18+lh,18+li,18+lj,18+lk,18+ll,18+lm,18+ln,18+lo,18+lp,18+lq,18+lr,18+ls,18+lt,18+lu,18+lv,18+lw,18+lx,18+ly,19+a,19+b,19+c,19+d y, 18 + jz, 18 + ka, 18 + kb, 18 + kc, 18 + kd, 18 + ke, 18 + kf, 18 + kg, 18 + kh, 18 + ki, 18 + kj, 18 + kk, 18 + kl, 18 + km, 18 + kn, 18 + ko, 18 + kp, 18 + kq, 18 + kr, 18 + ks, 18 + kt, 18 + ku, 18 + kv, 18 + kw, 18 + kx, 18 + ky, 18 + kz, 18 + la, 18 + lb, 18 + lc, 18 + ld, 18 + le, 18 + lf, 18 + lg, 18 + lh, 18 + li, 18 + lj, 18 + lk, 18 + ll, 18 + lm, 18 + ln, 18 + lo, 18 + lp, 18 + lq, 18 + lr, 18 + ls, 18 + lt, 18 + lu, 18 + lv, 18 + lw, 18 + lx, 18 + ly, 19 + a, 19 + b, 19 + c, 19 + d 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9+bl,19+bm,19+bn,19+bo,19+bp,19+bq,19+br,19+bs,19+bt,19+bu,19+bv,19+bw,19+bx,19+by,19+bz,19+ca,19+cb,19+cc,19+cd,19+ce,19+cf,19+cg,19+ch,19+ci,19+cj,19+ck,19+cl,19+cm,19+cn,19+co,19+cp,19+cq,19+cr,19+cs,19+ct,19+cu,19+cv,19+cw,19+cx,19+cy,19+cz,19+da,19+db,19+dc,19+dd,19+de,19+df,19+dg,19+dh,19+di,19+dj,19+dk,19+dl,19+dm,19+dn,19+ 9 + bl, 19 + bm, 19 + bn, 19 + bo, 19 + bp, 19 + bq, 19 + br, 19 + bs, 19 + bt, 19 + bu, 19 + bv, 19 + bw, 19 + bx, 19 + by, 19 + bz, 19 + ca, 19 + cb, 19 + cc, 19 + cd, 19 + ce, 19 + cf, 19 + cg, 19 + ch, 19 + ci, 19 + cj, 19 + ck, 19 + cl, 19 + cm, 19 + cn, 19 + co, 19 + cp, 19 + cq, 19 + cr, 19 + cs, 19 + ct, 19 + cu, 19 + cv, 19 + cw, 19 + cx, 19 + cy, 19 + cz, 19 + da, 19 + db, 19 + dc, 19 + dd, 19 + de, 19 + df, 19 + dg, 19 + dh, 19 + di, 19 + dj, 19 + dk, 19 + dl, 19 + dm, 19 + dn, 19 + o,19+dp,19+dq,19+dr,19+ds,19+dt,19+du,19+dv,19+dw,19+dx,19+dy,19+dz,19+ea,19+eb,19+ec,19+ed,19+ee,19+ef,19+eg,19+eh,19+ei,19+ej,19+ek,19+el,19+em,19+en,19+eo,19+ep,19+eq,19+er,19+es,19+et,19+eu,19+ev,19+ew,19+ex,19+ey,19+ez,19+fa,19+fb,19+fc,19+fd,19+fe,19+ff,19+fg,19+fh,19+fi,19+fj,19+fk,19+fl,19+fm,19+fn,19+fo,19+fp,19+fq,19+fr,1 o, 19 + dp, 19 + dq, 19 + dr, 19 + ds, 19 + dt, 19 + du, 19 + dv, 19 + dw, 19 + dx, 19 + dy, 19 + dz, 19 + ea, 19 + eb, 19 + ec, 19 + ed, 19 + ee, 19 + ef, 19 + eg, 19 + eh, 19 + ei, 19 + ej, 19 + ek, 19 + el, 19 + em, 19 + en, 19 + eo, 19 + ep, 19 + eq, 19 + er, 19 + es, 19 + et, 19 + eu, 19 + ev, 19 + ew, 19 + ex, 19 + ey, 19 + ez, 19 + fa, 19 + fb, 19 + fc, 19 + fd, 19 + fe, 19 + ff, 19 + fg, 19 + fh, 19 + fi, 19 + fj, 19 + fk, 19 + fl, 19 + fm, 19 + fn, 19 + fo, 19 + fp, 19 + fq, 19 + fr, 1 9+fs,19+ft,19+fu,19+fv,19+fw,19+fx,19+fy,19+fz,19+ga,19+gb,19+gc,19+gd,19+ge,19+gf,19+gg,19+gh,19+gi,19+gj,19+gk,19+gl,19+gm,19+gn,19+go,19+gp,19+gq,19+gr,19+gs,19+gt,19+gu,19+gv,19+gw,19+gx,19+gy,19+gz,19+ha,19+hb,19+hc,19+hd,19+he,19+hf,19+hg,19+hh,19+hi,19+hj,19+hk,19+hl,19+hm,19+hn,19+ho,19+hp,19+hq,19+hr,19+hs,19+ht,19+hu,19+h 9 + fs, 19 + ft, 19 + fu, 19 + fv, 19 + fw, 19 + fx, 19 + fy, 19 + fz, 19 + ga, 19 + gb, 19 + gc, 19 + gd, 19 + ge, 19 + gf, 19 + gg, 19 + gh, 19 + gi, 19 + gj, 19 + gk, 19 + gl, 19 + gm, 19 + gn, 19 + go, 19 + gp, 19 + gq, 19 + gr, 19 + gs, 19 + gt, 19 + gu, 19 + gv, 19 + gw, 19 + gx, 19 + gy, 19 + gz, 19 + ha, 19 + hb, 19 + hc, 19 + hd, 19 + he, 19 + hf, 19 + hg, 19 + hh, 19 + hi, 19 + hj, 19 + hk, 19 + hl, 19 + hm, 19 + hn, 19 + ho, 19 + hp, 19 + hq, 19 + hr, 19 + hs, 19 + ht, 19 + hu, 19 + h 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e,20+f,20+g,20+h,20+i,20+j,20+k,20+l,20+m,20+n,20+o,20+p,20+q,20+r,20+s,20+t,20+u,20+v,20+w,20+x,20+y,20+z,20+aa,20+ab,20+ac,20+ad,20+ae,20+af,20+ag,20+ah,20+ai,20+aj,20+ak,20+al,20+am,20+an,20+ao,20+ap,20+aq,20+ar,20+as,20+at,20+au,20+av,20+aw,20+ax,20+ay,20+az,20+ba,20+bb,20+bc,20+bd,20+be,20+bf,20+bg,20+bh,20+bi,20+bj,20+bk,20+b e, 20 + f, 20 + g, 20 + h, 20 + i, 20 + j, 20 + k, 20 + l, 20 + m, 20 + n, 20 + o, 20 + p, 20 + q, 20 + r, 20 + s, 20 + t, 20 + u, 20 + v, 20 + w, 20 + x, 20 + y, 20 + z, 20 + aa, 20 + ab, 20 + ac, 20 + ad, 20 + ae, 20 + af, 20 + ag, 20 + ah, 20 + ai, 20 + aj, 20 + ak, 20 + al, 20 + am, 20 + an, 20 + ao, 20 + ap, 20 + aq, 20 + ar, 20 + as, 20 + at, 20 + au, 20 + av, 20 + aw, 20 + ax, 20 + ay, 20 + az, 20 + ba, 20 + bb, 20 + bc, 20 + bd, 20 + be, 20 + bf, 20 + bg, 20 + bh, 20 + bi, 20 + bj, 20 + bk, 20 + b 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+dp,20+dq,20+dr,20+ds,20+dt,20+du,20+dv,20+dw,20+dx,20+dy,20+dz,20+ea,20+eb,20+ec,20+ed,20+ee,20+ef,20+eg,20+eh,20+ei,20+ej,20+ek,20+el,20+em,20+en,20+eo,20+ep,20+eq,20+er,20+es,20+et,20+eu,20+ev,20+ew,20+ex,20+ey,20+ez,20+fa,20+fb,20+fc,20+fd,20+fe,20+ff,20+fg,20+fh,20+fi,20+fj,20+fk,20+fl,20+fm,20+fn,20+fo,20+fp,20+fq,20+fr,20+fs + Dp, 20 + dq, 20 + dr, 20 + ds, 20 + dt, 20 + du, 20 + dv, 20 + dw, 20 + dx, 20 + dy, 20 + dz, 20 + ea, 20 + eb, 20 + ec, 20 + ed, 20 + ee, 20 + ef, 20 + eg, 20 + eh, 20 + ei, 20 + ej, 20 + ek, 20 + el, 20 + em, 20 + en, 20 + eo, 20 + ep, 20 + eq, 20 + er, 20 + es, 20 + et, 20 + eu, 20 + ev, 20 + ew, 20 + ex, 20 + ey, 20 + ez, 20 + fa, 20 + fb, 20 + fc, 20 + fd, 20 + fe, 20 + ff, 20 + fg, 20 + fh, 20 + fi, 20 + fj, 20 + fk, 20 + fl, 20 + fm, 20 + fn, 20 + fo, 20 + fp, 20 + fq, 20 + fr, 20 + fs ,20+ft,20+fu,20+fv,20+fw,20+fx,20+fy,20+fz,20+ga,20+gb,20+gc,20+gd,20+ge,20+gf,20+gg,20+gh,20+gi,20+gj,20+gk,20+gl,20+gm,20+gn,20+go,20+gp,20+gq,20+gr,20+gs,20+gt,20+gu,20+gv,20+gw,20+gx,20+gy,20+gz,20+ha,20+hb,20+hc,20+hd,20+he,20+hf,20+hg,20+hh,20+hi,20+hj,20+hk,20+hl,20+hm,20+hn,20+ho,20+hp,20+hq,20+hr,20+hs,20+ht,20+hu,20+hv,20 , 20 + ft, 20 + fu, 20 + fv, 20 + fw, 20 + fx, 20 + fy, 20 + fz, 20 + ga, 20 + gb, 20 + gc, 20 + gd, 20 + ge, 20 + gf, 20 + gg, 20 + gh, 20 + gi, 20 + gj, 20 + gk, 20 + gl, 20 + gm, 20 + gn, 20 + go, 20 + gp, 20 + gq, 20 + gr , 20 + gs, 20 + gt, 20 + gu, 20 + gv, 20 + gw, 20 + gx, 20 + gy, 20 + gz, 20 + ha, 20 + hb, 20 + hc, 20 + hd, 20 + he, 20 + hf, 20 + hg, 20 + hh, 20 + hi, 20 + hj, 20 + hk, 20 + hl, 20 + hm, 20 + hn, 20 + ho, 20 + hp, 20 + hq , 20 + hr, 20 + hs, 20 + ht, 20 + hu, 20 + hv, 20 hw,20+hx,20+hy,20+hz,20+ia,20+ib,20+ic,20+id,20+ie,20+if,20+ig,20+ih,20+ii,20+ij,20+ik,20+il,20+im,20+in,20+io,20+ip,20+iq,20+ir,20+is,20+it,20+iu,20+iv,20+iw,20+ix,20+iy,20+iz,20+ja,20+jb,20+jc,20+jd,20+je,20+jf,20+jg,20+jh,20+ji,20+jj,20+jk,20+jl,20+jm,20+jn,20+jo,20+jp,20+jq,20+jr,20+js,20+jt,20+ju,20+jv,20+jw,20+jx,20+jy,20+jz hw, 20 + hx, 20 + hy, 20 + hz, 20 + ia, 20 + ib, 20 + ic, 20 + id, 20 + ie, 20 + if, 20 + ig, 20 + ih, 20 + ii, 20 + ij, 20 + ik, 20 + il, 20 + im, 20 + in, 20 + io, 20 + ip, 20 + iq, 20 + ir, 20 + is, 20 + it, 20 + iu, 20 + iv, 20 + iw, 20 + ix, 20 + iy, 20 + iz, 20 + ja, 20 + jb, 20 + jc, 20 + jd, 20 + je, 20 + jf, 20 + jg, 20 + jh, 20 + ji, 20 + jj, 20 + jk, 20 + jl, 20 + jm, 20 + jn, 20 + jo, 20 + jp, 20 + jq, 20 + jr, 20 + js, 20 + jt, 20 + ju, 20 + jv, 20 + jw, 20 + jx, 20 + jy, 20 + jz 20+ka,20+kb,20+kc,20+kd,20+ke,20+kf,20+kg,20+kh,20+ki,20+kj,20+kk,20+kl,20+km,20+kn,20+ko,20+kp,20+kq,20+kr,20+ks,20+kt,20+ku,20+kv,20+kw,20+kx,20+ky,20+kz,20+la,20+lb,20+lc,20+ld,20+le,20+lf,20+lg,20+lh,20+li,20+lj,20+lk,20+ll,20+lm,20+ln,20+lo,20+lp,20+lq,20+lr,20+ls,20+lt,20+lu,20+lv,20+lw,20+lx,20+ly,21+a,21+b,21+c,21+d,21+e,21 20 + ka, 20 + kb, 20 + kc, 20 + kd, 20 + ke, 20 + kf, 20 + kg, 20 + kh, 20 + ki, 20 + kj, 20 + kk, 20 + kl, 20 + km, 20 + kn, 20 + ko, 20 + kp, 20 + kq, 20 + kr, 20 + ks, 20 + kt, 20 + ku, 20 + kv, 20 + kw, 20 + kx, 20 + ky, 20 + kz, 20 + la, 20 + lb, 20 + lc, 20 + ld, 20 + le, 20 + lf, 20 + lg, 20 + lh, 20 + li, 20 + lj, 20 + lk, 20 + ll, 20 + lm, 20 + ln, 20 + lo, 20 + lp, 20 + lq, 20 + lr, 20 + ls, 20 + lt, 20 + lu, 20 + lv, 20 + lw, 20 + lx, 20 + ly, 21 + a, 21 + b, 21 + c, 21 + d, 21 + e, 21 +f,21+g,21+h,21+i,21+j,21+k,21+l,21+m,21+n,21+o,21+p,21+q,21+r,21+s,21+t,21+u,21+v,21+w,21+x,21+y,21+z,21+aa,21+ab,21+ac,21+ad,21+ae,21+af,21+ag,21+ah,21+ai,21+aj,21+ak,21+al,21+am,21+an,21+ao,21+ap,21+aq,21+ar,21+as,21+at,21+au,21+av,21+aw,21+ax,21+ay,21+az,21+ba,21+bb,21+bc,21+bd,21+be,21+bf,21+bg,21+bh,21+bi,21+bj,21+bk,21+bl,21 + F, 21 + g, 21 + h, 21 + i, 21 + j, 21 + k, 21 + l, 21 + m, 21 + n, 21 + o, 21 + p, 21 + q, 21 + r, 21 + s, 21 + t, 21 + u, 21 + v, 21 + w, 21 + x, 21 + y, 21 + z, 21 + aa, 21 + ab, 21 + ac, 21 + ad, 21 + ae, 21 + af, 21 + ag, 21 + ah, 21 + ai, 21 + aj, 21 + ak, 21 + al, 21 + am, 21 + an, 21 + ao, 21 + ap, 21 + aq, 21 + ar, 21 + as, 21 + at, 21 + au, 21 + av, 21 + aw, 21 + ax, 21 + ay, 21 + az, 21 + ba, 21 + bb, 21 + bc, 21 + bd, 21 + be, 21 + bf, 21 + bg, 21 + bh, 21 + bi, 21 + bj, 21 + bk, 21 + bl, 21 bm,21+bn,21+bo,21+bp,21+bq,21+br,21+bs,21+bt,21+bu,21+bv,21+bw,21+bx,21+by,21+bz,21+ca,21+cb,21+cc,21+cd,21+ce,21+cf,21+cg,21+ch,21+ci,21+cj,21+ck,21+cl,21+cm,21+cn,21+co,21+cp,21+cq,21+cr,21+cs,21+ct,21+cu,21+cv,21+cw,21+cx,21+cy,21+cz,21+da,21+db,21+dc,21+dd,21+de,21+df,21+dg,21+dh,21+di,21+dj,21+dk,21+dl,21+dm,21+dn,21+do,21+dp bm, 21 + bn, 21 + bo, 21 + bp, 21 + bq, 21 + br, 21 + bs, 21 + bt, 21 + bu, 21 + bv, 21 + bw, 21 + bx, 21 + by, 21 + bz, 21 + ca, 21 + cb, 21 + cc, 21 + cd, 21 + ce, 21 + cf, 21 + cg, 21 + ch, 21 + ci, 21 + cj, 21 + ck, 21 + cl, 21 + cm, 21 + cn, 21 + co, 21 + cp, 21 + cq, 21 + cr, 21 + cs, 21 + ct, 21 + cu, 21 + cv, 21 + cw, 21 + cx, 21 + cy, 21 + cz, 21 + da, 21 + db, 21 + dc, 21 + dd, 21 + de, 21 + df, 21 + dg, 21 + dh, 21 + di, 21 + dj, 21 + dk, 21 + dl, 21 + dm, 21 + dn, 21 + do, 21 + dp 21+dq,21+dr,21+ds,21+dt,21+du,21+dv,21+dw,21+dx,21+dy,21+dz,21+ea,21+eb,21+ec,21+ed,21+ee,21+ef,21+eg,21+eh,21+ei,21+ej,21+ek,21+el,21+em,21+en,21+eo,21+ep,21+eq,21+er,21+es,21+et,21+eu,21+ev,21+ew,21+ex,21+ey,21+ez,21+fa,21+fb,21+fc,21+fd,21+fe,21+ff,21+fg,21+fh,21+fi,21+fj,21+fk,21+fl,21+fm,21+fn,21+fo,21+fp,21+fq,21+fr,21+fs,21+ 21 + dq, 21 + dr, 21 + ds, 21 + dt, 21 + du, 21 + dv, 21 + dw, 21 + dx, 21 + dy, 21 + dz, 21 + ea, 21 + eb, 21 + ec, 21 + ed, 21 + ee, 21 + ef, 21 + eg, 21 + eh, 21 + ei, 21 + ej, 21 + ek, 21 + el, 21 + em, 21 + en, 21 + eo, 21 + ep, 21 + eq, 21 + er, 21 + es, 21 + et, 21 + eu, 21 + ev, 21 + ew, 21 + ex, 21 + ey, 21 + ez, 21 + fa, 21 + fb, 21 + fc, 21 + fd, 21 + fe, 21 + ff, 21 + fg, 21 + fh, 21 + fi, 21 + fj, 21 + fk, 21 + fl, 21 + fm, 21 + fn, 21 + fo, 21 + fp, 21 + fq, 21 + fr, 21 + fs, 21 + ft,21+fu,21+fv,21+fw,21+fx,21+fy,21+fz,21+ga,21+gb,21+gc,21+gd,21+ge,21+gf,21+gg,21+gh,21+gi,21+gj,21+gk,21+gl,21+gm,21+gn,21+go,21+gp,21+gq,21+gr,21+gs,21+gt,21+gu,21+gv,21+gw,21+gx,21+gy,21+gz,21+ha,21+hb,21+hc,21+hd,21+he,21+hf,21+hg,21+hh,21+hi,21+hj,21+hk,21+hl,21+hm,21+hn,21+ho,21+hp,21+hq,21+hr,21+hs,21+ht,21+hu,21+hv,21+hw, ft, 21 + fu, 21 + fv, 21 + fw, 21 + fx, 21 + fy, 21 + fz, 21 + ga, 21 + gb, 21 + gc, 21 + gd, 21 + ge, 21 + gf, 21 + gg, 21 + gh, 21 + gi, 21 + gj, 21 + gk, 21 + gl, 21 + gm, 21 + gn, 21 + go, 21 + gp, 21 + gq, 21 + gr, 21+gs,21+gt,21+gu,21+gv,21+gw,21+gx,21+gy,21+gz,21+ha,21+hb,21+hc,21+hd,21+he,21+hf,21+hg,21+hh,21+hi,21+hj,21+hk,21+hl,21+hm,21+hn,21+ho,21+hp,21+hq, 21+hr,21+hs,21+ht,21+hu,21+hv,21+hw, 1+hx,21+hy,21+hz,21+ia,21+ib,21+ic,21+id,21+ie,21+if,21+ig,21+ih,21+ii,21+ij,21+ik,21+il,21+im,21+in,21+io,21+ip,21+iq,21+ir,21+is,21+it,21+iu,21+iv,21+iw,21+ix,21+iy,21+iz,21+ja,21+jb,21+jc,21+jd,21+je,21+jf,21+jg,21+jh,21+ji,21+jj,21+jk,21+jl,21+jm,21+jn,21+jo,21+jp,21+jq,21+jr,21+js,21+jt,21+ju,21+jv,21+jw,21+jx,21+jy,21+jz,21+ a,21+kb,21+kc,21+kd,21+ke,21+kf,21+kg,21+kh,21+ki,21+kj,21+kk,21+kl,21+km,21+kn,21+ko,21+kp,21+kq,21+kr,21+ks,21+kt,21+ku,21+kv,21+kw,21+kx,21+ky,21+kz,21+la,21+lb,21+lc,21+ld,21+le,21+lf,21+lg,21+lh,21+li,21+lj,21+lk,21+ll,21+lm,21+ln,21+lo,21+lp,21+lq,21+lr,21+ls,21+lt,21+lu,21+lv,21+lw,21+lx,21+ly,22+a,22+b,22+c,22+d,22+e,22+f,2 2+g,22+h,22+i,22+j,22+k,22+l,22+m,22+n,22+o,22+p,22+q,22+r,22+s,22+t,22+u,22+v,22+w,22+x,22+y,22+z,22+aa,22+ab,22+ac,22+ad,22+ae,22+af,22+ag,22+ah,22+ai,22+aj,22+ak,22+al,22+am,22+an,22+ao,22+ap,22+aq,22+ar,22+as,22+at,22+au,22+av,22+aw,22+ax,22+ay,22+az,22+ba,22+bb,22+bc,22+bd,22+be,22+bf,22+bg,22+bh,22+bi,22+bj,22+bk,22+bl,22+bm, 2+bn,22+bo,22+bp,22+bq,22+br,22+bs,22+bt,22+bu,22+bv,22+bw,22+bx,22+by,22+bz,22+ca,22+cb,22+cc,22+cd,22+ce,22+cf,22+cg,22+ch,22+ci,22+cj,22+ck,22+cl,22+cm,22+cn,22+co,22+cp,22+cq,22+cr,22+cs,22+ct,22+cu,22+cv,22+cw,22+cx,22+cy,22+cz,22+da,22+db,22+dc,22+dd,22+de,22+df,22+dg,22+dh,22+di,22+dj,22+dk,22+dl,22+dm,22+dn,22+do,22+dp,22+ q,22+dr,22+ds,22+dt,22+du,22+dv,22+dw,22+dx,22+dy,22+dz,22+ea,22+eb,22+ec,22+ed,22+ee,22+ef,22+eg,22+eh,22+ei,22+ej,22+ek,22+el,22+em,22+en,22+eo,22+ep,22+eq,22+er,22+es,22+et,22+eu,22+ev,22+ew,22+ex,22+ey,22+ez,22+fa,22+fb,22+fc,22+fd,22+fe,22+ff,22+fg,22+fh,22+fi,22+fj,22+fk,22+fl,22+fm,22+fn,22+fo,22+fp,22+fq,22+fr,22+fs,22+ft,2 2+fu,22+fv,22+fw,22+fx,22+fy,22+fz,22+ga,22+gb,22+gc,22+gd,22+ge,22+gf,22+gg,22+gh,22+gi,22+gj,22+gk,22+gl,22+gm,22+gn,22+go,22+gp,22+gq,22+gr,22+gs,22+gt,22+gu,22+gv,22+gw,22+gx,22+gy,22+gz,22+ha,22+hb,22+hc,22+hd,22+he,22+hf,22+hg,22+hh,22+hi,22+hj,22+hk,22+hl,22+hm,22+hn,22+ho,22+hp,22+hq,22+hr,22+hs,22+ht,22+hu,22+hv,22+hw,22+h 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8+br,28+bs,28+bt,28+bu,28+bv,28+bw,28+bx,28+by,28+bz,28+ca,28+cb,28+cc,28+cd,28+ce,28+cf,28+cg,28+ch,28+ci,28+cj,28+ck,28+cl,28+cm,28+cn,28+co,28+cp,28+cq,28+cr,28+cs,28+ct,28+cu,28+cv,28+cw,28+cx,28+cy,28+cz,28+da,28+db,28+dc,28+dd,28+de,28+df,28+dg,28+dh,28+di,28+dj,28+dk,28+dl,28+dm,28+dn,28+do,28+dp,28+dq,28+dr,28+ds,28+dt,28+ u,28+dv,28+dw,28+dx,28+dy,28+dz,28+ea,28+eb,28+ec,28+ed,28+ee,28+ef,28+eg,28+eh,28+ei,28+ej,28+ek,28+el,28+em,28+en,28+eo,28+ep,28+eq,28+er,28+es,28+et,28+eu,28+ev,28+ew,28+ex,28+ey,28+ez,28+fa,28+fb,28+fc,28+fd,28+fe,28+ff,28+fg,28+fh,28+fi,28+fj,28+fk,28+fl,28+fm,28+fn,28+fo,28+fp,28+fq,28+fr,28+fs,28+ft,28+fu,28+fv,28+fw,28+fx,2 8+fy,28+fz,28+ga,28+gb,28+gc,28+gd,28+ge,28+gf,28+gg,28+gh,28+gi,28+gj,28+gk,28+gl,28+gm,28+gn,28+go,28+gp,28+gq,28+gr,28+gs,28+gt,28+gu,28+gv,28+gw,28+gx,28+gy,28+gz,28+ha,28+hb,28+hc,28+hd,28+he,28+hf,28+hg,28+hh,28+hi,28+hj,28+hk,28+hl,28+hm,28+hn,28+ho,28+hp,28+hq,28+hr,28+hs,28+ht,28+hu,28+hv,28+hw,28+hx,28+hy,28+hz,28+ia,28+i ,28+ic,28+id,28+ie,28+if,28+ig,28+ih,28+ii,28+ij,28+ik,28+il,28+im,28+in,28+io,28+ip,28+iq,28+ir,28+is,28+it,28+iu,28+iv,28+iw,28+ix,28+iy,28+iz,28+ja,28+jb,28+jc,28+jd,28+je,28+jf,28+jg,28+jh,28+ji,28+jj,28+jk,28+jl,28+jm,28+jn,28+jo,28+jp,28+jq,28+jr,28+js,28+jt,28+ju,28+jv,28+jw,28+jx,28+jy,28+jz,28+ka,28+kb,28+kc,28+kd,28+ke,2 +kf,28+kg,28+kh,28+ki,28+kj,28+kk,28+kl,28+km,28+kn,28+ko,28+kp,28+kq,28+kr,28+ks,28+kt,28+ku,28+kv,28+kw,28+kx,28+ky,28+kz,28+la,28+lb,28+lc,28+ld,28+le,28+lf,28+lg,28+lh,28+li,28+lj,28+lk,28+ll,28+lm,28+ln,28+lo,28+lp,28+lq,28+lr,28+ls,28+lt,28+lu,28+lv,28+lw,28+lx,28+ly,29+a,29+b,29+c,29+d,29+e,29+f,29+g,29+h,29+i,29+j,29+k,29+l ,29+m,29+n,29+o,29+p,29+q,29+r,29+s,29+t,29+u,29+v,29+w,29+x,29+y,29+z,29+aa,29+ab,29+ac,29+ad,29+ae,29+af,29+ag,29+ah,29+ai,29+aj,29+ak,29+al,29+am,29+an,29+ao,29+ap,29+aq,29+ar,29+as,29+at,29+au,29+av,29+aw,29+ax,29+ay,29+az,29+ba,29+bb,29+bc,29+bd,29+be,29+bf,29+bg,29+bh,29+bi,29+bj,29+bk,29+bl,29+bm,29+bn,29+bo,29+bp,29+bq,29+b ,29+bs,29+bt,29+bu,29+bv,29+bw,29+bx,29+by,29+bz,29+ca,29+cb,29+cc,29+cd,29+ce,29+cf,29+cg,29+ch,29+ci,29+cj,29+ck,29+cl,29+cm,29+cn,29+co,29+cp,29+cq,29+cr,29+cs,29+ct,29+cu,29+cv,29+cw,29+cx,29+cy,29+cz,29+da,29+db,29+dc,29+dd,29+de,29+df,29+dg,29+dh,29+di,29+dj,29+dk,29+dl,29+dm,29+dn,29+do,29+dp,29+dq,29+dr,29+ds,29+dt,29+du,2 +dv,29+dw,29+dx,29+dy,29+dz,29+ea,29+eb,29+ec,29+ed,29+ee,29+ef,29+eg,29+eh,29+ei,29+ej,29+ek,29+el,29+em,29+en,29+eo,29+ep,29+eq,29+er,29+es,29+et,29+eu,29+ev,29+ew,29+ex,29+ey,29+ez,29+fa,29+fb,29+fc,29+fd,29+fe,29+ff,29+fg,29+fh,29+fi,29+fj,29+fk,29+fl,29+fm,29+fn,29+fo,29+fp,29+fq,29+fr,29+fs,29+ft,29+fu,29+fv,29+fw,29+fx,29+fy ,29+fz,29+ga,29+gb,29+gc,29+gd,29+ge,29+gf,29+gg,29+gh,29+gi,29+gj,29+gk,29+gl,29+gm,29+gn,29+go,29+gp,29+gq,29+gr,29+gs,29+gt,29+gu,29+gv,29+gw,29+gx,29+gy,29+gz,29+ha,29+hb,29+hc,29+hd,29+he,29+hf,29+hg,29+hh,29+hi,29+hj,29+hk,29+hl,29+hm,29+hn,29+ho,29+hp,29+hq,29+hr,29+hs,29+ht,29+hu,29+hv,29+hw,29+hx,29+hy,29+hz,29+ia,29+ib,29 ic,29+id,29+ie,29+if,29+ig,29+ih,29+ii,29+ij,29+ik,29+il,29+im,29+in,29+io,29+ip,29+iq,29+ir,29+is,29+it,29+iu,29+iv,29+iw,29+ix,29+iy,29+iz,29+ja,29+jb,29+jc,29+jd,29+je,29+jf,29+jg,29+jh,29+ji,29+jj,29+jk,29+jl,29+jm,29+jn,29+jo,29+jp,29+jq,29+jr,29+js,29+jt,29+ju,29+jv,29+jw,29+jx,29+jy,29+jz,29+ka,29+kb,29+kc,29+kd,29+ke,29+kf 29+kg,29+kh,29+ki,29+kj,29+kk,29+kl,29+km,29+kn,29+ko,29+kp,29+kq,29+kr,29+ks,29+kt,29+ku,29+kv,29+kw,29+kx,29+ky,29+kz,29+la,29+lb,29+lc,29+ld,29+le,29+lf,29+lg,29+lh,29+li,29+lj,29+lk,29+ll,29+lm,29+ln,29+lo,29+lp,29+lq,29+lr,29+ls,29+lt,29+lu,29+lv,29+lw,29+lx,29+ly,30+a,30+b,30+c,30+d,30+e,30+f,30+g,30+h,30+i,30+j,30+k,30+l,30+ m,30+n,30+o,30+p,30+q,30+r,30+s,30+t,30+u,30+v,30+w,30+x,30+y,30+z,30+aa,30+ab,30+ac,30+ad,30+ae,30+af,30+ag,30+ah,30+ai,30+aj,30+ak,30+al,30+am
,30+an,30+ao,30+ap,30+aq,30+ar,30+as,30+at,30+au,30+av,30+aw,30+ax,30+ay,30+az,30+ba,30+bb,30+bc,30+bd,30+be,30+bf,30+bg,30+bh,30+bi,30+bj,30+bk,30+bl,30+bm,30+bn,30+bo,30+bp,30+bq,30+br,30+bs,30+bt,30+bu,30+bv,30+bw,30+bx,30+by,30+bz,30+ca,30+cb,30+cc,30+cd,30+ce,30+cf,30+cg,30+ch,30+ci,30+cj,30+ck,30+cl,30+cm,30+cn,30+co,30+cp,30 , 30 + an, 30 + ao, 30 + ap, 30 + aq, 30 + ar, 30 + as, 30 + at, 30 + au, 30 + av, 30 + aw, 30 + ax, 30 + ay, 30 + az, 30 + ba, 30 + bb, 30 + bc, 30 + bd, 30 + be, 30 + bf, 30 + bg, 30 + bh, 30 + bi, 30 + bj, 30 + bk, 30 + bl , 30 + bm, 30 + bn, 30 + bo, 30 + bp, 30 + bq, 30 + br, 30 + bs, 30 + bt, 30 + bu, 30 + bv, 30 + bw, 30 + bx, 30 + by, 30 + bz, 30 + ca, 30 + cb, 30 + cc, 30 + cd, 30 + ce, 30 + cf, 30 + cg, 30 + ch, 30 + ci, 30 + cj, 30 + ck , 30 + cl, 30 + cm, 30 + cn, 30 + co, 30 + cp, 30 cq,30+cr,30+cs,30+ct,30+cu,30+cv,30+cw,30+cx,30+cy,30+cz,30+da,30+db,30+dc,30+dd,30+de,30+df,30+dg,30+dh,30+di,30+dj,30+dk,30+dl,30+dm,30+dn,30+do,30+dp,30+dq,30+dr,30+ds,30+dt,30+du,30+dv,30+dw,30+dx,30+dy,30+dz,30+ea,30+eb,30+ec,30+ed,30+ee,30+ef,30+eg,30+eh,30+ei,30+ej,30+ek,30+el,30+em,30+en,30+eo,30+ep,30+eq,30+er,30+es,30+et cq, 30 + cr, 30 + cs, 30 + ct, 30 + cu, 30 + cv, 30 + cw, 30 + cx, 30 + cy, 30 + cz, 30 + da, 30 + db, 30 + dc, 30 + dd, 30 + de, 30 + df, 30 + dg, 30 + dh, 30 + di, 30 + dj, 30 + dk, 30 + dl, 30 + dm, 30 + dn, 30 + do, 30 + dp, 30 + dq, 30 + dr, 30 + ds, 30 + dt, 30 + du, 30 + dv, 30 + dw, 30 + dx, 30 + dy, 30 + dz, 30 + ea, 30 + eb, 30 + ec, 30 + ed, 30 + ee, 30 + ef, 30 + eg, 30 + eh, 30 + ei, 30 + ej, 30 + ek, 30 + el, 30 + em, 30 + en, 30 + eo, 30 + ep, 30 + eq, 30 + er, 30 + es, 30 + et 30+eu,30+ev,30+ew,30+ex,30+ey,30+ez,30+fa,30+fb,30+fc,30+fd,30+fe,30+ff,30+fg,30+fh,30+fi,30+fj,30+fk,30+fl,30+fm,30+fn,30+fo,30+fp,30+fq,30+fr,30+fs,30+ft,30+fu,30+fv,30+fw,30+fx,30+fy,30+fz,30+ga,30+gb,30+gc,30+gd,30+ge,30+gf,30+gg,30+gh,30+gi,30+gj,30+gk,30+gl,30+gm,30+gn,30+go,30+gp,30+gq,30+gr,30+gs,30+gt,30+gu,30+gv,30+gw,30+ 30 + eu, 30 + ev, 30 + ew, 30 + ex, 30 + ey, 30 + ez, 30 + fa, 30 + fb, 30 + fc, 30 + fd, 30 + fe, 30 + ff, 30 + fg, 30 + fh, 30 + fi, 30 + fj, 30 + fk, 30 + fl, 30 + fm, 30 + fn, 30 + fo, 30 + fp, 30 + fq, 30 + fr, 30 + fs, 30 + ft, 30 + fu, 30 + fv, 30 + fw, 30 + fx, 30 + fy, 30 + fz, 30 + ga, 30 + gb, 30 + gc, 30 + gd, 30 + ge, 30 + gf, 30 + gg, 30 + gh, 30 + gi, 30 + gj, 30 + gk, 30 + gl, 30 + gm, 30 + gn, 30 + go, 30 + gp, 30 + gq, 30 + gr, 30 + gs, 30 + gt, 30 + gu, 30 + gv, 30 + gw, 30 + gx,30+gy,30+gz,30+ha,30+hb,30+hc,30+hd,30+he,30+hf,30+hg,30+hh,30+hi,30+hj,30+hk,30+hl,30+hm,30+hn,30+ho,30+hp,30+hq,30+hr,30+hs,30+ht,30+hu,30+hv,30+hw,30+hx,30+hy,30+hz,30+ia,30+ib,30+ic,30+id,30+ie,30+if,30+ig,30+ih,30+ii,30+ij,30+ik,30+il,30+im,30+in,30+io,30+ip,30+iq,30+ir,30+is,30+it,30+iu,30+iv,30+iw,30+ix,30+iy,30+iz,30+ja, gx, 30 + gy, 30 + gz, 30 + ha, 30 + hb, 30 + hc, 30 + hd, 30 + he, 30 + hf, 30 + hg, 30 + hh, 30 + hi, 30 + hj, 30 + hk, 30 + hl, 30 + hm, 30 + hn, 30 + ho, 30 + hp, 30 + hq, 30 + hr, 30 + hs, 30 + ht, 30 + hu, 30 + hv, 30 + hw, 30 + hx, 30 + hy, 30 + hz, 30 + ia, 30 + ib, 30 + ic, 30 + id, 30 + ie, 30 + if, 30 + ig, 30 + ih, 30 + ii, 30 + ij, 30 + ik, 30 + il, 30 + im, 30 + in, 30 + io, 30 + ip, 30 + iq, 30 + ir, 30 + is, 30 + it, 30 + iu, 30 + iv, 30 + iw, 30 + ix, 30 + iy, 30 + iz, 30 + ja, 0+jb,30+jc,30+jd,30+je,30+jf,30+jg,30+jh,30+ji,30+jj,30+jk,30+jl,30+jm,30+jn,30+jo,30+jp,30+jq,30+jr,30+js,30+jt,30+ju,30+jv,30+jw,30+jx,30+jy,30+jz,30+ka,30+kb,30+kc,30+kd,30+ke,30+kf,30+kg,30+kh,30+ki,30+kj,30+kk,30+kl,30+km,30+kn,30+ko,30+kp,30+kq,30+kr,30+ks,30+kt,30+ku,30+kv,30+kw,30+kx,30+ky,30+kz,30+la,30+lb,30+lc,30+ld,30+ 0 + jb, 30 + jc, 30 + jd, 30 + je, 30 + jf, 30 + jg, 30 + jh, 30 + ji, 30 + jj, 30 + jk, 30 + jl, 30 + jm, 30 + jn, 30 + jo, 30 + jp, 30 + jq, 30 + jr, 30 + js, 30 + jt, 30 + ju, 30 + jv, 30 + jw, 30 + jx, 30 + jy, 30 + jz, 30 + ka, 30 + kb, 30 + kc, 30 + kd, 30 + ke, 30 + kf, 30 + kg, 30 + kh, 30 + ki, 30 + kj, 30 + kk, 30 + kl, 30 + km, 30 + kn, 30 + ko, 30 + kp, 30 + kq, 30 + kr, 30 + ks, 30 + kt, 30 + ku, 30 + kv, 30 + kw, 30 + kx, 30 + ky, 30 + kz, 30 + la, 30 + lb, 30 + lc, 30 + ld, 30 + e,30+lf,30+lg,30+lh,30+li,30+lj,30+lk,30+ll,30+lm,30+ln,30+lo,30+lp,30+lq,30+lr,30+ls,30+lt,30+lu,30+lv,30+lw,30+lx,30+ly,31+a,31+b,31+c,31+d,31+e,31+f,31+g,31+h,31+i,31+j,31+k,31+l,31+m,31+n,31+o,31+p,31+q,31+r,31+s,31+t,31+u,31+v,31+w,31+x,31+y,31+z,31+aa,31+ab,31+ac,31+ad,31+ae,31+af,31+ag,31+ah,31+ai,31+aj,31+ak,31+al,31+am,31+ e, 30 + lf, 30 + lg, 30 + lh, 30 + li, 30 + lj, 30 + lk, 30 + ll, 30 + lm, 30 + ln, 30 + lo, 30 + lp, 30 + lq, 30 + lr, 30 + ls, 30 + lt, 30 + lu, 30 + lv, 30 + lw, 30 + lx, 30 + ly, 31 + a, 31 + b, 31 + c, 31 + d, 31 + e, 31 + f, 31 + g, 31 + h, 31 + i, 31 + j, 31 + k, 31 + l, 31 + m, 31 + n, 31 + o, 31 + p, 31 + q, 31 + r, 31 + s, 31 + t, 31 + u, 31 + v, 31 + w, 31 + x, 31 + y, 31 + z, 31 + aa, 31 + ab, 31 + ac, 31 + ad, 31 + ae, 31 + af, 31 + ag, 31 + ah, 31 + ai, 31 + aj, 31 + ak, 31 + al, 31 + am, 31 + an,31+ao,31+ap,31+aq,31+ar,31+as,31+at,31+au,31+av,31+aw,31+ax,31+ay,31+az,31+ba,31+bb,3 an, 31 + ao, 31 + ap, 31 + aq, 31 + ar, 31 + as, 31 + at, 31 + au, 31 + av, 31 + aw, 31 + ax, 31 + ay, 31 + az, 31 + ba, 31 + bb, 3
1+bc,31+bd,31+be,31+bf,31+bg,31+bh,31+bi,31+bj,31+bk,31+bl,31+bm,31+bn,31+bo,31+bp,31+bq,31+br,31+bs,31+bt,31+bu,31+bv,31+bw,31+bx,31+by,31+bz,31+ca,31+cb,31+cc,31+cd,31+ce,31+cf,31+cg,31+ch,31+ci,31+cj,31+ck,31+cl,31+cm,31+cn,31+co,31+cp,31+cq,31+cr,31+cs,31+ct,31+cu,31+cv,31+cw,31+cx,31+cy,31+cz,31+da,31+db,31+dc,31+dd,31+de,31+d 1 + bc, 31 + bd, 31 + be, 31 + bf, 31 + bg, 31 + bh, 31 + bi, 31 + bj, 31 + bk, 31 + bl, 31 + bm, 31 + bn, 31 + bo, 31 + bp, 31 + bq, 31 + br, 31 + bs, 31 + bt, 31 + bu, 31 + bv, 31 + bw, 31 + bx, 31 + by, 31 + bz, 31 + ca, 31 + cb, 31 + cc, 31 + cd, 31 + ce, 31 + cf, 31 + cg, 31 + ch, 31 + ci, 31 + cj, 31 + ck, 31 + cl, 31 + cm, 31 + cn, 31 + co, 31 + cp, 31 + cq, 31 + cr, 31 + cs, 31 + ct, 31 + cu, 31 + cv, 31 + cw, 31 + cx, 31 + cy, 31 + cz, 31 + da, 31 + db, 31 + dc, 31 + dd, 31 + de, 31 + d ,31+dg,31+dh,31+di,31+dj,31+dk,31+dl,31+dm,31+dn,31+do,31+dp,31+dq,31+dr,31+ds,31+dt,31+du,31+dv,31+dw,31+dx,31+dy,31+dz,31+ea,31+eb,31+ec,31+ed,31+ee,31+ef,31+eg,31+eh,31+ei,31+ej,31+ek,31+el,31+em,31+en,31+eo,31+ep,31+eq,31+er,31+es,31+et,31+eu,31+ev,31+ew,31+ex,31+ey,31+ez,31+fa,31+fb,31+fc,31+fd,31+fe,31+ff,31+fg,31+fh,31+fi,3 , 31 + dg, 31 + dh, 31 + di, 31 + dj, 31 + dk, 31 + dl, 31 + dm, 31 + dn, 31 + do, 31 + dp, 31 + dq, 31 + dr, 31 + ds, 31 + dt, 31 + du, 31 + dv, 31 + dw, 31 + dx, 31 + dy, 31 + dz, 31 + ea, 31 + eb, 31 + ec, 31 + ed, 31 + ee , 31 + ef, 31 + eg, 31 + eh, 31 + ei, 31 + ej, 31 + ek, 31 + el, 31 + em, 31 + en, 31 + eo, 31 + ep, 31 + eq, 31 + er, 31 + es, 31 + et, 31 + eu, 31 + ev, 31 + ew, 31 + ex, 31 + ey, 31 + ez, 31 + fa, 31 + fb, 31 + fc, 31 + fd , 31 + fe, 31 + ff, 31 + fg, 31 + fh, 31 + fi, 3 +fj,31+fk,31+fl,31+fm,31+fn,31+fo,31+fp,31+fq,31+fr,31+fs,31+ft,31+fu,31+fv,31+fw,31+fx,31+fy,31+fz,31+ga,31+gb,31+gc,31+gd,31+ge,31+gf,31+gg,31+gh,31+gi,31+gj,31+gk,31+gl,31+gm,31+gn,31+go,31+gp,31+gq,31+gr,31+gs,31+gt,31+gu,31+gv,31+gw,31+gx,31+gy,31+gz,31+ha,31+hb,31+hc,31+hd,31+he,31+hf,31+hg,31+hh,31+hi,31+hj,31+hk,31+hl,31+hm + Fj, 31 + fk, 31 + fl, 31 + fm, 31 + fn, 31 + fo, 31 + fp, 31 + fq, 31 + fr, 31 + fs, 31 + ft, 31 + fu, 31 + fv, 31 + fw, 31 + fx, 31 + fy, 31 + fz, 31 + ga, 31 + gb, 31 + gc, 31 + gd, 31 + ge, 31 + gf, 31 + gg, 31 + gh, 31 + gi, 31 + gj, 31 + gk, 31 + gl, 31 + gm, 31 + gn, 31 + go, 31 + gp, 31 + gq, 31 + gr, 31 + gs, 31 + gt, 31 + gu, 31 + gv, 31 + gw, 31 + gx, 31 + gy, 31 + gz, 31 + ha, 31 + hb, 31 + hc, 31 + hd, 31 + he, 31 + hf, 31 + hg, 31 + hh, 31 + hi, 31 + hj, 31 + hk, 31 + hl, 31 + hm ,31+hn,31+ho,31+hp,31+hq,31+hr,31+hs,31+ht,31+hu,31+hv,31+hw,31+hx,31+hy,31+hz,31+ia,31+ib,31+ic,31+id,31+ie,31+if,31+ig,31+ih,31+ii,31+ij,31+ik,31+il,31+im,31+in,31+io,31+ip,31+iq,31+ir,31+is,31+it,31+iu,31+iv,31+iw,31+ix,31+iy,31+iz,31+ja,31+jb,31+jc,31+jd,31+je,31+jf,31+jg,31+jh,31+ji,31+jj,31+jk,31+jl,31+jm,31+jn,31+jo,31+jp,31 , 31 + hn, 31 + ho, 31 + hp, 31 + hq, 31 + hr, 31 + hs, 31 + ht, 31 + hu, 31 + hv, 31 + hw, 31 + hx, 31 + hy, 31 + hz, 31 + ia, 31 + ib, 31 + ic, 31 + id, 31 + ie, 31 + if, 31 + ig, 31 + ih, 31 + ii, 31 + ij, 31 + ik, 31 + il , 31 + im, 31 + in, 31 + io, 31 + ip, 31 + iq, 31 + ir, 31 + is, 31 + it, 31 + iu, 31 + iv, 31 + iw, 31 + ix, 31 + iy, 31 + iz, 31 + ja, 31 + jb, 31 + jc, 31 + jd, 31 + je, 31 + jf, 31 + jg, 31 + jh, 31 + ji, 31 + jj, 31 + jk , 31 + jl, 31 + jm, 31 + jn, 31 + jo, 31 + jp, 31 jq,31+jr,31+js,31+jt,31+ju,31+jv,31+jw,31+jx,31+jy,31+jz,31+ka,31+kb,31+kc,31+kd,31+ke,31+kf,31+kg,31+kh,31+ki,31+kj,31+kk,31+kl,31+km,31+kn,31+ko,31+kp,31+kq,31+kr,31+ks,31+kt,31+ku,31+kv,31+kw,31+kx,31+ky,31+kz,31+la,31+lb,31+lc,31+ld,31+le,31+lf,31+lg,31+lh,31+li,31+lj,31+lk,31+ll,31+lm,31+ln,31+lo,31+lp,31+lq,31+lr,31+ls,31+lt jq, 31 + jr, 31 + js, 31 + jt, 31 + ju, 31 + jv, 31 + jw, 31 + jx, 31 + jy, 31 + jz, 31 + ka, 31 + kb, 31 + kc, 31 + kd, 31 + ke, 31 + kf, 31 + kg, 31 + kh, 31 + ki, 31 + kj, 31 + kk, 31 + kl, 31 + km, 31 + kn, 31 + ko, 31 + kp, 31 + kq, 31 + kr, 31 + ks, 31 + kt, 31 + ku, 31 + kv, 31 + kw, 31 + kx, 31 + ky, 31 + kz, 31 + la, 31 + lb, 31 + lc, 31 + ld, 31 + le, 31 + lf, 31 + lg, 31 + lh, 31 + li, 31 + lj, 31 + lk, 31 + ll, 31 + lm, 31 + ln, 31 + lo, 31 + lp, 31 + lq, 31 + lr, 31 + ls, 31 + lt 31+lu,31+lv,31+lw,31+lx,31+ly,32+a,32+b,32+c,32+d,32+e,32+f,32+g,32+h,32+i,32+j,32+k,32+l,32+m,32+n,32+o,32+p,32+q,32+r,32+s,32+t,32+u,32+v,32+w,32+x,32+y,32+z,32+aa,32+ab,32+ac,32+ad,32+ae,32+af,32+ag,32+ah,32+ai,32+aj,32+ak,32+al,32+am,32+an,32+ao,32+ap,32+aq,32+ar,32+as,32+at,32+au,32+av,32+aw,32+ax,32+ay,32+az,32+ba,32+bb,32+bc 31 + lu, 31 + lv, 31 + lw, 31 + lx, 31 + ly, 32 + a, 32 + b, 32 + c, 32 + d, 32 + e, 32 + f, 32 + g, 32 + h, 32 + i, 32 + j, 32 + k, 32 + l, 32 + m, 32 + n, 32 + o, 32 + p, 32 + q, 32 + r, 32 + s, 32 + t, 32 + u, 32 + v, 32 + w, 32 + x, 32 + y, 32 + z, 32 + aa, 32 + ab, 32 + ac, 32 + ad, 32 + ae, 32 + af, 32 + ag, 32 + ah, 32 + ai, 32 + aj, 32 + ak, 32 + al, 32 + am, 32 + an, 32 + ao, 32 + ap, 32 + aq, 32 + ar, 32 + as, 32 + at, 32 + au, 32 + av, 32 + aw, 32 + ax, 32 + ay, 32 + az, 32 + ba, 32 + bb, 32 + bc ,32+bd,32+be,32+bf,32+bg,32+bh,32+bi,32+bj,32+bk,32+bl,32+bm,32+bn,32+bo,32+bp,32+bq,32+br,32+bs,32+bt,32+bu,32+bv,32+bw,32+bx,32+by,32+bz,32+ca,32+cb,32+cc,32+cd,32+ce,32+cf,32+cg,32+ch,32+ci,32+cj,32+ck,32+cl,32+cm,32+cn,32+co,32+cp,32+cq,32+cr,32+cs,32+ct,32+cu,32+cv,32+cw,32+cx,32+cy,32+cz,32+da,32+db,32+dc,32+dd,32+de,32+df,32 , 32 + bd, 32 + be, 32 + bf, 32 + bg, 32 + bh, 32 + bi, 32 + bj, 32 + bk, 32 + bl, 32 + bm, 32 + bn, 32 + bo, 32 + bp, 32 + bq, 32 + br, 32 + bs, 32 + bt, 32 + bu, 32 + bv, 32 + bw, 32 + bx, 32 + by, 32 + bz, 32 + ca, 32 + cb , 32 + cc, 32 + cd, 32 + ce, 32 + cf, 32 + cg, 32 + ch, 32 + ci, 32 + cj, 32 + ck, 32 + cl, 32 + cm, 32 + cn, 32 + co, 32 + cp, 32 + cq, 32 + cr, 32 + cs, 32 + ct, 32 + cu, 32 + cv, 32 + cw, 32 + cx, 32 + cy, 32 + cz, 32 + da , 32 + db, 32 + dc, 32 + dd, 32 + de, 32 + df, 32 dg,32+dh,32+di,32+dj,32+dk,32+dl,32+dm,32+dn,32+do,32+dp,32+dq,32+dr,32+ds,32+dt,32+du,32+dv,32+dw,32+dx,32+dy,32+dz,32+ea,32+eb,32+ec,32+ed,32+ee,32+ef,32+eg,32+eh,32+ei,32+ej,32+ek,32+el,32+em,32+en,32+eo,32+ep,32+eq,32+er,32+es,32+et,32+eu,32+ev,32+ew,32+ex,32+ey,32+ez,32+fa,32+fb,32+fc,32+fd,32+fe,32+ff,32+fg,32+fh,32+fi,32+fj dg, 32 + dh, 32 + di, 32 + dj, 32 + dk, 32 + dl, 32 + dm, 32 + dn, 32 + do, 32 + dp, 32 + dq, 32 + dr, 32 + ds, 32 + dt, 32 + du, 32 + dv, 32 + dw, 32 + dx, 32 + dy, 32 + dz, 32 + ea, 32 + eb, 32 + ec, 32 + ed, 32 + ee, 32 + ef, 32 + eg, 32 + eh, 32 + ei, 32 + ej, 32 + ek, 32 + el, 32 + em, 32 + en, 32 + eo, 32 + ep, 32 + eq, 32 + er, 32 + es, 32 + et, 32 + eu, 32 + ev, 32 + ew, 32 + ex, 32 + ey, 32 + ez, 32 + fa, 32 + fb, 32 + fc, 32 + fd, 32 + fe, 32 + ff, 32 + fg, 32 + fh, 32 + fi, 32 + fj 32+fk,32+fl,32+fm,32+fn,32+fo,32+fp,32+fq,32+fr,32+fs,32+ft,32+fu,32+fv,32+fw,32+fx,32+fy,32+fz,32+ga,32+gb,32+gc,32+gd,32+ge,32+gf,32+gg,32+gh,32+gi,32+gj,32+gk,32+gl,32+gm,32+gn,32+go,32+gp,32+gq,32+gr,32+gs,32+gt,32+gu,32+gv,32+gw,32+gx,32+gy,32+gz,32+ha,32+hb,32+hc,32+hd,32+he,32+hf,32+hg,32+hh,32+hi,32+hj,32+hk,32+hl,32+hm,32+ 32 + fk, 32 + fl, 32 + fm, 32 + fn, 32 + fo, 32 + fp, 32 + fq, 32 + fr, 32 + fs, 32 + ft, 32 + fu, 32 + fv, 32 + fw, 32 + fx, 32 + fy, 32 + fz, 32 + ga, 32 + gb, 32 + gc, 32 + gd, 32 + ge, 32 + gf, 32 + gg, 32 + gh, 32 + gi, 32 + gj, 32 + gk, 32 + gl, 32 + gm, 32 + gn, 32 + go, 32 + gp, 32 + gq, 32 + gr, 32 + gs, 32 + gt, 32 + gu, 32 + gv, 32 + gw, 32 + gx, 32 + gy, 32 + gz, 32 + ha, 32 + hb, 32 + hc, 32 + hd, 32 + he, 32 + hf, 32 + hg, 32 + hh, 32 + hi, 32 + hj, 32 + hk, 32 + hl, 32 + hm, 32 + hn,32+ho,32+hp,32+hq,32+hr,32+hs,32+ht,32+hu,32+hv,32+hw,32+hx,32+hy,32+hz,32+ia,32+ib,32+ic,32+id,32+ie,32+if,32+ig,32+ih,32+ii,32+ij,32+ik,32+il,32+im,32+in,32+io,32+ip,32+iq,32+ir,32+is,32+it,32+iu,32+iv,32+iw,32+ix,32+iy,32+iz,32+ja,32+jb,32+jc,32+jd,32+je,32+jf,32+jg,32+jh,32+ji,32+jj,32+jk,32+jl,32+jm,32+jn,32+jo,32+jp,32+jq, hn, 32 + ho, 32 + hp, 32 + hq, 32 + hr, 32 + hs, 32 + ht, 32 + hu, 32 + hv, 32 + hw, 32 + hx, 32 + hy, 32 + hz, 32 + ia, 32 + ib, 32 + ic, 32 + id, 32 + ie, 32 + if, 32 + ig, 32 + ih, 32 + ii, 32 + ij, 32 + ik, 32 + il, 32 + im, 32 + in, 32 + io, 32 + ip, 32 + iq, 32 + ir, 32 + is, 32 + it, 32 + iu, 32 + iv, 32 + iw, 32 + ix, 32 + iy, 32 + iz, 32 + ja, 32 + jb, 32 + jc, 32 + jd, 32 + je, 32 + jf, 32 + jg, 32 + jh, 32 + ji, 32 + jj, 32 + jk, 32 + jl, 32 + jm, 32 + jn, 32 + jo, 32 + jp, 32 + jq, 2+jr,32+js,32+jt,32+ju,32+jv,32+jw,32+jx,32+jy,32+jz,32+ka,32+kb,32+kc,32+kd,32+ke,32+kf,32+kg,32+kh,32+ki,32+kj,32+kk,32+kl,32+km,32+kn,32+ko,32+kp,32+kq,32+kr,32+ks,32+kt,32+ku,32+kv,32+kw,32+kx,32+ky,32+kz,32+la,32+lb,32+lc,32+ld,32+le,32+lf,32+lg,32+lh,32+li,32+lj,32+lk,32+ll,32+lm,32+ln,32+lo,32+lp,32+lq,32+lr,32+ls,32+lt,32+ 2 + jr, 32 + js, 32 + jt, 32 + ju, 32 + jv, 32 + jw, 32 + jx, 32 + jy, 32 + jz, 32 + ka, 32 + kb, 32 + kc, 32 + kd, 32 + ke, 32 + kf, 32 + kg, 32 + kh, 32 + ki, 32 + kj, 32 + kk, 32 + kl, 32 + km, 32 + kn, 32 + ko, 32 + kp, 32 + kq, 32 + kr, 32 + ks, 32 + kt, 32 + ku, 32 + kv, 32 + kw, 32 + kx, 32 + ky, 32 + kz, 32 + la, 32 + lb, 32 + lc, 32 + ld, 32 + le, 32 + lf, 32 + lg, 32 + lh, 32 + li, 32 + lj, 32 + lk, 32 + ll, 32 + lm, 32 + ln, 32 + lo, 32 + lp, 32 + lq, 32 + lr, 32 + ls, 32 + lt, 32 + u,32+lv,32+lw,32+lx,32+ly,33+a,33+b,33+c,33+d,33+e,33+f,33+g,33+h,33+i,33+j,33+k,33+l,33+m,33+n,33+o,33+p,33+q,33+r,33+s,33+t,33+u,33+v,33+w,33+x,33+y,33+z,33+aa,33+ab,33+ac,33+ad,33+ae,33+af,33+ag,33+ah,33+ai,33+aj,33+ak,33+al,33+am,33+an,33+ao,33+ap,33+aq,33+ar,33+as,33+at,33+au,33+av,33+aw,33+ax,33+ay,33+az,33+ba,33+bb,33+bc,33+ u, 32 + lv, 32 + lw, 32 + lx, 32 + ly, 33 + a, 33 + b, 33 + c, 33 + d, 33 + e, 33 + f, 33 + g, 33 + h, 33 + i, 33 + j, 33 + k, 33 + l, 33 + m, 33 + n, 33 + o, 33 + p, 33 + q, 33 + r, 33 + s, 33 + t, 33 + u, 33 + v, 33 + w, 33 + x, 33 + y, 33 + z, 33 + aa, 33 + ab, 33 + ac, 33 + ad, 33 + ae, 33 + af, 33 + ag, 33 + ah, 33 + ai, 33 + aj, 33 + ak, 33 + al, 33 + am, 33 + an, 33 + ao, 33 + ap, 33 + aq, 33 + ar, 33 + as, 33 + at, 33 + au, 33 + av, 33 + aw, 33 + ax, 33 + ay, 33 + az, 33 + ba, 33 + bb, 33 + bc, 33 + bd,33+be,33+bf,33+bg,33+bh,33+bi,33+bj,33+bk,33+bl,33+bm,33+bn,33+bo,33+bp,33+bq,33+br,33+bs,33+bt,33+bu,33+bv,33+bw,33+bx,33+by,33+bz,33+ca,33+cb,33+cc,33+cd,33+ce,33+cf,33+cg,33+ch,33+ci,33+cj,33+ck,33+cl,33+cm,33+cn,33+co,33+cp,33+cq,33+cr,33+cs,33+ct,33+cu,33+cv,33+cw,33+cx,33+cy,33+cz,33+da,33+db,33+dc,33+dd,33+de,33+df,33+dg, bd, 33 + be, 33 + bf, 33 + bg, 33 + bh, 33 + bi, 33 + bj, 33 + bk, 33 + bl, 33 + bm, 33 + bn, 33 + bo, 33 + bp, 33 + bq, 33 + br, 33 + bs, 33 + bt, 33 + bu, 33 + bv, 33 + bw, 33 + bx, 33 + by, 33 + bz, 33 + ca, 33 + cb, 33 + cc, 33 + cd, 33 + ce, 33 + cf, 33 + cg, 33 + ch, 33 + ci, 33 + cj, 33 + ck, 33 + cl, 33 + cm, 33 + cn, 33 + co, 33 + cp, 33 + cq, 33 + cr, 33 + cs, 33 + ct, 33 + cu, 33 + cv, 33 + cw, 33 + cx, 33 + cy, 33 + cz, 33 + da, 33 + db, 33 + dc, 33 + dd, 33 + de, 33 + df, 33 + dg, 3+dh,33+di,33+dj,33+dk,33+dl,33+dm,33+dn,33+do,33+dp,33+dq,33+dr,33+ds,33+dt,33+du,33+dv,33+dw,33+dx,33+dy,33+dz,33+ea,33+eb,33+ec,33+ed,33+ee,33+ef,33+eg,33+eh,33+ei,33+ej,33+ek,33+el,33+em,33+en,33+eo,33+ep,33+eq,33+er,33+es,33+et,33+eu,33+ev,33+ew,33+ex,33+ey,33+ez,33+fa,33+fb,33+fc,33+fd,33+fe,33+ff,33+fg,33+fh,33+fi,33+fj,33+ 3 + dh, 33 + di, 33 + dj, 33 + dk, 33 + dl, 33 + dm, 33 + dn, 33 + do, 33 + dp, 33 + dq, 33 + dr, 33 + ds, 33 + dt, 33 + du, 33 + dv, 33 + dw, 33 + dx, 33 + dy, 33 + dz, 33 + ea, 33 + eb, 33 + ec, 33 + ed, 33 + ee, 33 + ef, 33 + eg, 33 + eh, 33 + ei, 33 + ej, 33 + ek, 33 + el, 33 + em, 33 + en, 33 + eo, 33 + ep, 33 + eq, 33 + er, 33 + es, 33 + et, 33 + eu, 33 + ev, 33 + ew, 33 + ex, 33 + ey, 33 + ez, 33 + fa, 33 + fb, 33 + fc, 33 + fd, 33 + fe, 33 + ff, 33 + fg, 33 + fh, 33 + fi, 33 + fj, 33 + k,33+fl,33+fm,33+fn,33+fo,33+fp,33+fq,33+fr,33+fs,33+ft,33+fu,33+fv,33+fw,33+fx,33+fy,33+fz,33+ga,33+gb,33+gc,33+gd,33+ge,33+gf,33+gg,33+gh,33+gi,33+gj,33+gk,33+gl,33+gm,33+gn,33+go,33+gp,33+gq,33+gr,33+gs,33+gt,33+gu,33+gv,33+gw,33+gx,33+gy,33+gz,33+ha,33+hb,33+hc,33+hd,33+he,33+hf,33+hg,33+hh,33+hi,33+hj,33+hk,33+hl,33+hm,33+hn,3 k, 33 + fl, 33 + fm, 33 + fn, 33 + fo, 33 + fp, 33 + fq, 33 + fr, 33 + fs, 33 + ft, 33 + fu, 33 + fv, 33 + fw, 33 + fx, 33 + fy, 33 + fz, 33 + ga, 33 + gb, 33 + gc, 33 + gd, 33 + ge, 33 + gf, 33 + gg, 33 + gh, 33 + gi, 33 + gj, 33 + gk, 33 + gl, 33 + gm, 33 + gn, 33 + go, 33 + gp, 33 + gq, 33 + gr, 33 + gs, 33 + gt, 33 + gu, 33 + gv, 33 + gw, 33 + gx, 33 + gy, 33 + gz, 33 + ha, 33 + hb, 33 + hc, 33 + hd, 33 + he, 33 + hf, 33 + hg, 33 + hh, 33 + hi, 33 + hj, 33 + hk, 33 + hl, 33 + hm, 33 + hn, 3 3+ho,33+hp,33+hq,33+hr,33+hs,33+ht,33+hu,33+hv,33+hw,33+hx,33+hy,33+hz,33+ia,33+ib,33+ic,33+id,33+ie,33+if,33+ig,33+ih,33+ii,33+ij,33+ik,33+il,33+im,33+in,33+io,33+ip,33+iq,33+ir,33+is,33+it,33+iu,33+iv,33+iw,33+ix,33+iy,33+iz,33+ja,33+jb,33+jc,33+jd,33+je,33+jf,33+jg,33+jh,33+ji,33+jj,33+jk,33+jl,33+jm,33+jn,33+jo,33+jp,33+jq,33+j 3 + ho, 33 + hp, 33 + hq, 33 + hr, 33 + hs, 33 + ht, 33 + hu, 33 + hv, 33 + hw, 33 + hx, 33 + hy, 33 + hz, 33 + ia, 33 + ib, 33 + ic, 33 + id, 33 + ie, 33 + if, 33 + ig, 33 + ih, 33 + ii, 33 + ij, 33 + ik, 33 + il, 33 + im, 33 + in, 33 + io, 33 + ip, 33 + iq, 33 + ir, 33 + is, 33 + it, 33 + iu, 33 + iv, 33 + iw, 33 + ix, 33 + iy, 33 + iz, 33 + ja, 33 + jb, 33 + jc, 33 + jd, 33 + je, 33 + jf, 33 + jg, 33 + jh, 33 + ji, 33 + jj, 33 + jk, 33 + jl, 33 + jm, 33 + jn, 33 + jo, 33 + jp, 33 + jq, 33 + j ,33+js,33+jt,33+ju,33+jv,33+jw,33+jx,33+jy,33+jz,33+ka,33+kb,33+kc,33+kd,33+ke,33+kf,33+kg,33+kh,33+ki,33+kj,33+kk,33+kl,33+km,33+kn,33+ko,33+kp,33+kq,33+kr,33+ks,33+kt,33+ku,33+kv,33+kw,33+kx,33+ky,33+kz,33+la,33+lb,33+lc,33+ld,33+le,33+lf,33+lg,33+lh,33+li,33+lj,33+lk,33+ll,33+lm,33+ln,33+lo,33+lp,33+lq,33+lr,33+ls,33+lt,33+lu,3 , 33 + js, 33 + jt, 33 + ju, 33 + jv, 33 + jw, 33 + jx, 33 + jy, 33 + jz, 33 + + ka, 33 + kb, 33 + kc, 33 + kd, 33 ke, 33 + kf, 33 + kg, 33 + kh, 33 + ki, 33 + kj, 33 + kk, 33 + kl, 33 + km, 33 + kn, 33 + ko, 33 + kp, 33 + kq , 33 + kr, 33 + ks, 33 + kt, 33 + ku, 33 + kv, 33 + kw, 33 + kx, 33 + ky, 33 + kz, 33 + la, 33 + lb, 33 + lc, 33 + ld, 33 + le, 33 + lf, 33 + lg, 33 + lh, 33 + li, 33 + lj, 33 + lk, 33 + ll, 33 + lm, 33 + ln, 33 + lo, 33 + lp , 33 + lq, 33 + lr, 33 + ls, 33 + lt, 33 + lu, 3 +lv,33+lw,33+lx,33+ly,34+a,34+b,34+c,34+d,34+e,34+f,34+g,34+h,34+i,34+j,34+k,34+l,34+m,34+n,34+o,34+p,34+q,34+r,34+s,34+t,34+u,34+v,34+w,34+x,34+y,34+z,34+aa,34+ab,34+ac,34+ad,34+ae,34+af,34+ag,34+ah,34+ai,34+aj,34+ak,34+al,34+am,34+an,34+ao,34+ap,34+aq,34+ar,34+as,34+at,34+au,34+av,34+aw,34+ax,34+ay,34+az,34+ba,34+bb,34+bc,34+bd,3 + Lv, 33 + lw, 33 + lx, 33 + ly, 34 + a, 34 + b, 34 + c, 34 + d, 34 + e, 34 + f, 34 + g, 34 + h, 34 + i, 34 + j, 34 + k, 34 + l, 34 + m, 34 + n, 34 + o, 34 + p, 34 + q, 34 + r, 34 + s, 34 + t, 34 + u, 34 + v, 34 + w, 34 + x, 34 + y, 34 + z, 34 + aa, 34 + ab, 34 + ac, 34 + ad, 34 + ae, 34 + af, 34 + ag, 34 + ah, 34 + ai, 34 + aj, 34 + ak, 34 + al, 34 + am, 34 + an, 34 + ao, 34 + ap, 34 + aq, 34 + ar, 34 + as, 34 + at, 34 + au, 34 + av, 34 + aw, 34 + ax, 34 + ay, 34 + az, 34 + ba, 34 + bb, 34 + bc, 34 + bd, 3 4+be,34+bf,34+bg,34+bh,34+bi,34+bj,34+bk,34+bl,34+bm,34+bn,34+bo,34+bp,34+bq,34+br,34+bs,34+bt,34+bu,34+bv,34+bw,34+bx,34+by,34+bz,34+ca,34+cb,34+cc,34+cd,34+ce,34+cf,34+cg,34+ch,34+ci,34+cj,34+ck,34+cl,34+cm,34+cn,34+co,34+cp,34+cq,34+cr,34+cs,34+ct,34+cu,34+cv,34+cw,34+cx,34+cy,34+cz,34+da,34+db,34+dc,34+dd,34+de,34+df,34+dg,34+d 4 + be, 34 + bf, 34 + bg, 34 + bh, 34 + bi, 34 + bj, 34 + bk, 34 + bl, 34 + bm, 34 + bn, 34 + bo, 34 + bp, 34 + bq, 34 + br, 34 + bs, 34 + bt, 34 + bu, 34 + bv, 34 + bw, 34 + bx, 34 + by, 34 + bz, 34 + ca, 34 + cb, 34 + cc, 34 + cd, 34 + ce, 34 + cf, 34 + cg, 34 + ch, 34 + ci, 34 + cj, 34 + ck, 34 + cl, 34 + cm, 34 + cn, 34 + co, 34 + cp, 34 + cq, 34 + cr, 34 + cs, 34 + ct, 34 + cu, 34 + cv, 34 + cw, 34 + cx, 34 + cy, 34 + cz, 34 + da, 34 + db, 34 + dc, 34 + dd, 34 + de, 34 + df, 34 + dg, 34 + d ,34+di,34+dj,34+dk,34+dl,34+dm,34+dn,34+do,34+dp,34+dq,34+dr,34+ds,34+dt,34+du,34+dv,34+dw,34+dx,34+dy,34+dz,34+ea,34+eb,34+ec,34+ed,34+ee,34+ef,34+eg,34+eh,34+ei,34+ej,34+ek,34+el,34+em,34+en,34+eo,34+ep,34+eq,34+er,34+es,34+et,34+eu,34+ev,34+ew,34+ex,34+ey,34+ez,34+fa,34+fb,34+fc,34+fd,34+fe,34+ff,34+fg,34+fh,34+fi,34+fj,34+fk,3 , 34 + di, 34 + dj, 34 + dk, 34 + dl, 34 + dm, 34 + dn, 34 + do, 34 + dp, 34 + dq, 34 + dr, 34 + ds, 34 + dt, 34 + du, 34 + dv, 34 + dw, 34 + dx, 34 + dy, 34 + dz, 34 + ea, 34 + eb, 34 + ec, 34 + ed, 34 + ee, 34 + ef, 34 + eg , 34 + eh, 34 + ei, 34 + ej, 34 + ek, 34 + el, 34 + em, 34 + en, 34 + eo, 34 + ep, 34 + eq, 34 + er, 34 + es, 34 + et, 34 + eu, 34 + ev, 34 + ew, 34 + ex, 34 + ey, 34 + ez, 34 + fa, 34 + fb, 34 + fc, 34 + fd, 34 + fe, 34 + ff , 34 + fg, 34 + fh, 34 + fi, 34 + fj, 34 + fk, 3 +fl,34+fm,34+fn,34+fo,34+fp,34+fq,34+fr,34+fs,34+ft,34+fu,34+fv,34+fw,34+fx,34+fy,34+fz,34+ga,34+gb,34+gc,34+gd,34+ge,34+gf,34+gg,34+gh,34+gi,34+gj,34+gk,34+gl,34+gm,34+gn,34+go,34+gp,34+gq,34+gr,34+gs,34+gt,34+gu,34+gv,34+gw,34+gx,34+gy,34+gz,34+ha,34+hb,34+hc,34+hd,34+he,34+hf,34+hg,34+hh,34+hi,34+hj,34+hk,34+hl,34+hm,34+hn,34+ho + Fl, 34 + fm, 34 + fn, 34 + fo, 34 + fp, 34 + fq, 34 + fr, 34 + fs, 34 + ft, 34 + fu, 34 + fv, 34 + fw, 34 + fx, 34 + fy, 34 + fz, 34 + ga, 34 + gb, 34 + gc, 34 + gd, 34 + ge, 34 + gf, 34 + gg, 34 + gh, 34 + gi, 34 + gj, 34 + gk, 34 + gl, 34 + gm, 34 + gn, 34 + go, 34 + gp, 34 + gq, 34 + gr, 34 + gs, 34 + gt, 34 + gu, 34 + gv, 34 + gw, 34 + gx, 34 + gy, 34 + gz, 34 + ha, 34 + hb, 34 + hc, 34 + hd, 34 + he, 34 + hf, 34 + hg, 34 + hh, 34 + hi, 34 + hj, 34 + hk, 34 + hl, 34 + hm, 34 + hn, 34 + ho ,34+hp,34+hq,34+hr,34+hs,34+ht,34+hu,34+hv,34+hw,34+hx,34+hy,34+hz,34+ia,34+ib,34+ic,34+id,34+ie,34+if,34+ig,34+ih,34+ii,34+ij,34+ik,34+il,34+im,34+in,34+io,34+ip,34+iq,34+ir,34+is,34+it,34+iu,34+iv,34+iw,34+ix,34+iy,34+iz,34+ja,34+jb,34+jc,34+jd,34+je,34+jf,34+jg,34+jh,34+ji,34+jj,34+jk,34+jl,34+jm,34+jn,34+jo,34+jp,34+jq,34+jr,34 , 34 + hp, 34 + hq, 34 + hr, 34 + hs, 34 + ht, 34 + hu, 34 + hv, 34 + hw, 34 + hx, 34 + hy, 34 + hz, 34 + ia, 34 + ib, 34 + ic, 34 + id, 34 + ie, 34 + if, 34 + ig, 34 + ih, 34 + ii, 34 + ij, 34 + ik, 34 + il, 34 + im, 34 + in , 34 + io, 34 + ip, 34 + iq, 34 + ir, 34 + is, 34 + it, 34 + iu, 34 + iv, 34 + iw, 34 + ix, 34 + iy, 34 + iz, 34 + ja, 34 + jb, 34 + jc, 34 + jd, 34 + je, 34 + jf, 34 + jg, 34 + jh, 34 + ji, 34 + jj, 34 + jk, 34 + jl, 34 + jm , 34 + jn, 34 + jo, 34 + jp, 34 + jq, 34 + jr, 34 js,34+jt,34+ju,34+jv,34+jw,34+jx,34+jy,34+jz,34+ka,34+kb,34+kc,34+kd,34+ke,34+kf,34+kg,34+kh,34+ki,34+kj,34+kk,34+kl,34+km,34+kn,34+ko,34+kp,34+kq,34+kr,34+ks,34+kt,34+ku,34+kv,34+kw,34+kx,34+ky,34+kz,34+la,34+lb,34+lc,34+ld,34+le,34+lf,34+lg,34+lh,34+li,34+lj,34+lk,34+ll,34+lm,34+ln,34+lo,34+lp,34+lq,34+lr,34+ls,34+lt,34+lu,34+lv js, 34 + jt, 34 + ju, 34 + jv, 34 + jw, 34 + jx, 34 + jy, 34 + jz, 34 + ka, 34 + kb, 34 + kc, 34 + kd, 34 + ke, 34 + kf, 34 + kg, 34 + kh, 34 + ki, 34 + kj, 34 + kk, 34 + kl, 34 + km, 34 + kn, 34 + ko, 34 + kp, 34 + kq, 34 + kr, 34 + ks, 34 + kt, 34 + ku, 34 + kv, 34 + kw, 34 + kx, 34 + ky, 34 + kz, 34 + la, 34 + lb, 34 + lc, 34 + ld, 34 + le, 34 + lf, 34 + lg, 34 + lh, 34 + li, 34 + lj, 34 + lk, 34 + ll, 34 + lm, 34 + ln, 34 + lo, 34 + lp, 34 + lq, 34 + lr, 34 + ls, 34 + lt, 34 + lu, 34 + lv 34+lw,34+lx,34+ly,35+a,35+b,35+c,35+d,35+e,35+f,35+g,35+h,35+i,35+j,35+k,35+l,35+m,35+n,35+o,35+p,35+q,35+r,35+s,35+t,35+u,35+v,35+w,35+x,35+y,35+z,35+aa,35+ab,35+ac,35+ad,35+ae,35+af,35+ag,35+ah,35+ai,35+aj,35+ak,35+al,35+am,35+an,35+ao,35+ap,35+aq,35+ar,35+as,35+at,35+au,35+av,35+aw,35+ax,35+ay,35+az,35+ba,35+bb,35+bc,35+bd,35+be 34 + lw, 34 + lx, 34 + ly, 35 + a, 35 + b, 35 + c, 35 + d, 35 + e, 35 + f, 35 + g, 35 + h, 35 + i, 35 + j, 35 + k, 35 + l, 35 + m, 35 + n, 35 + o, 35 + p, 35 + q, 35 + r, 35 + s, 35 + t, 35 + u, 35 + v, 35 + w, 35 + x, 35 + y, 35 + z, 35 + aa, 35 + ab, 35 + ac, 35 + ad, 35 + ae, 35 + af, 35 + ag, 35 + ah, 35 + ai, 35 + aj, 35 + ak, 35 + al, 35 + am, 35 + an, 35 + ao, 35 + ap, 35 + aq, 35 + ar, 35 + as, 35 + at, 35 + au, 35 + av, 35 + aw, 35 + ax, 35 + ay, 35 + az, 35 + ba, 35 + bb, 35 + bc, 35 + bd, 35 + be ,35+bf,35+bg,35+bh,35+bi,35+bj,35+bk,35+bl,35+bm,35+bn,35+bo,35+bp,35+bq,35+br,35+bs,35+bt,35+bu,35+bv,35+bw,35+bx,35+by,35+bz,35+ca,35+cb,35+cc,35+cd,35+ce,35+cf,35+cg,35+ch,35+ci,35+cj,35+ck,35+cl,35+cm,35+cn,35+co,35+cp,35+cq,35+cr,35+cs,35+ct,35+cu,35+cv,35+cw,35+cx,35+cy,35+cz,35+da,35+db,35+dc,35+dd,35+de,35+df,35+dg,35+dh,35 , 35 + bf, 35 + bg, 35 + bh, 35 + bi, 35 + bj, 35 + bk, 35 + bl, 35 + bm, 35 + bn, 35 + bo, 35 + bp, 35 + bq, 35 + br, 35 + bs, 35 + bt, 35 + bu, 35 + bv, 35 + bw, 35 + bx, 35 + by, 35 + bz, 35 + ca, 35 + cb, 35 + cc, 35 + cd , 35 + ce, 35 + cf, 35 + cg, 35 + ch, 35 + ci, 35 + cj, 35 + ck, 35 + cl, 35 + cm, 35 + cn, 35 + co, 35 + cp, 35 + cq, 35 + cr, 35 + cs, 35 + ct, 35 + cu, 35 + cv, 35 + cw, 35 + cx, 35 + cy, 35 + cz, 35 + da, 35 + db, 35 + dc , 35 + dd, 35 + de, 35 + df, 35 + dg, 35 + dh, 35 di,35+dj,35+dk,35+dl,35+dm,35+dn,35+do,35+dp,35+dq,35+dr,35+ds,35+dt,35+du,35+dv,35+dw,35+dx,35+dy,35+dz,35+ea,35+eb,35+ec,35+ed,35+ee,35+ef,35+eg,35+eh,35+ei,35+ej,35+ek,35+el,35+em,35+en,35+eo,35+ep,35+eq,35+er,35+es,35+et,35+eu,35+ev,35+ew,35+ex,35+ey,35+ez,35+fa,35+fb,35+fc,35+fd,35+fe,35+ff,35+fg,35+fh,35+fi,35+fj,35+fk,35+fl di, 35 + dj, 35 + dk, 35 + dl, 35 + dm, 35 + dn, 35 + do, 35 + dp, 35 + dq, 35 + dr, 35 + ds, 35 + dt, 35 + du, 35 + dv, 35 + dw, 35 + dx, 35 + dy, 35 + dz, 35 + ea, 35 + eb, 35 + ec, 35 + ed, 35 + ee, 35 + ef, 35 + eg, 35 + eh, 35 + ei, 35 + ej, 35 + ek, 35 + el, 35 + em, 35 + en, 35 + eo, 35 + ep, 35 + eq, 35 + er, 35 + es, 35 + et, 35 + eu, 35 + ev, 35 + ew, 35 + ex, 35 + ey, 35 + ez, 35 + fa, 35 + fb, 35 + fc, 35 + fd, 35 + fe, 35 + ff, 35 + fg, 35 + fh, 35 + fi, 35 + fj, 35 + fk, 35 + fl 35+fm,35+fn,35+fo,35+fp,35+fq,35+fr,35+fs,35+ft,35+fu,35+fv,35+fw,35+fx,35+fy,35+fz,35+ga,35+gb,35+gc,35+gd,35+ge,35+gf,35+gg,35+gh,35+gi,35+gj,35+gk,35+gl,35+gm,35+gn,35+go,35+gp,35+gq,35+gr,35+gs,35+gt,35+gu,35+gv,35+gw,35+gx,35+gy,35+gz,35+ha,35+hb,35+hc,35+hd,35+he,35+hf,35+hg,35+hh,35+hi,35+hj,35+hk,35+hl,35+hm,35+hn,35+ho,35+ 35 + fm, 35 + fn, 35 + fo, 35 + fp, 35 + fq, 35 + fr, 35 + fs, 35 + ft, 35 + fu, 35 + fv, 35 + fw, 35 + fx, 35 + fy, 35 + fz, 35 + ga, 35 + gb, 35 + gc, 35 + gd, 35 + ge, 35 + gf, 35 + gg, 35 + gh, 35 + gi, 35 + gj, 35 + gk, 35 + gl, 35 + gm, 35 + gn, 35 + go, 35 + gp, 35 + gq, 35 + gr, 35 + gs, 35 + gt, 35 + gu, 35 + gv, 35 + gw, 35 + gx, 35 + gy, 35 + gz, 35 + ha, 35 + hb, 35 + hc, 35 + hd, 35 + he, 35 + hf, 35 + hg, 35 + hh, 35 + hi, 35 + hj, 35 + hk, 35 + hl, 35 + hm, 35 + hn, 35 + ho, 35 + hp,35+hq,35+hr,35+hs,35+ht,35+hu,35+hv,35+hw,35+hx,35+hy,35+hz,35+ia,35+ib,35+ic,35+id,35+ie,35+if,35+ig,35+ih,35+ii,35+ij,35+ik,35+il,35+im,35+in,35+io,35+ip,35+iq,35+ir,35+is,35+it,35+iu,35+iv,35+iw,35+ix,35+iy,35+iz,35+ja,35+jb,35+jc,35+jd,35+je,35+jf,35+jg,35+jh,35+ji,35+jj,35+jk,35+jl,35+jm,35+jn,35+jo,35+jp,35+jq,35+jr,35+js, hp, 35 + hq, 35 + hr, 35 + hs, 35 + ht, 35 + hu, 35 + hv, 35 + hw, 35 + hx, 35 + hy, 35 + hz, 35 + ia, 35 + ib, 35 + ic, 35 + id, 35 + ie, 35 + if, 35 + ig, 35 + ih, 35 + ii, 35 + ij, 35 + ik, 35 + il, 35 + im, 35 + in, 35 + io, 35 + ip, 35 + iq, 35 + ir, 35 + is, 35 + it, 35 + iu, 35 + iv, 35 + iw, 35 + ix, 35 + iy, 35 + iz, 35 + ja, 35 + jb, 35 + jc, 35 + jd, 35 + je, 35 + jf, 35 + jg, 35 + jh, 35 + ji, 35 + jj, 35 + jk, 35 + jl, 35 + jm, 35 + jn, 35 + jo, 35 + jp, 35 + jq, 35 + jr, 35 + js, 5+jt,35+ju,35+jv,35+jw,35+jx,35+jy,35+jz,35+ka,35+kb,35+kc,35+kd,35+ke,35+kf,35+kg,35+kh,35+ki,35+kj,35+kk,35+kl,35+km,35+kn,35+ko,35+kp,35+kq,35+kr,35+ks,35+kt,35+ku,35+kv,35+kw,35+kx,35+ky,35+kz,35+la,35+lb,35+lc,35+ld,35+le,35+lf,35+lg,35+lh,35+li,35+lj,35+lk,35+ll,35+lm,35+ln,35+lo,35+lp,35+lq,35+lr,35+ls,35+lt,35+lu,35+lv,35+ 5 + jt, 35 + ju, 35 + jv, 35 + jw, 35 + jx, 35 + jy, 35 + jz, 35 + ka, 35 + kb, 35 + kc, 35 + kd, 35 + ke, 35 + kf, 35 + kg, 35 + kh, 35 + ki, 35 + kj, 35 + kk, 35 + kl, 35 + km, 35 + kn, 35 + ko, 35 + kp, 35 + kq, 35 + kr, 35 + ks, 35 + kt, 35 + ku, 35 + kv, 35 + kw, 35 + kx, 35 + ky, 35 + kz, 35 + la, 35 + lb, 35 + lc, 35 + ld, 35 + le, 35 + lf, 35 + lg, 35 + lh, 35 + li, 35 + lj, 35 + lk, 35 + ll, 35 + lm, 35 + ln, 35 + lo, 35 + lp, 35 + lq, 35 + lr, 35 + ls, 35 + lt, 35 + lu, 35 + lv, 35 + w,35+lx,35+ly,36+a,36+b,36+c,36+d,36+e,36+f,36+g,36+h,36+i,36+j,36+k,36+l,36+m,36+n,36+o,36+p,36+q,36+r,36+s,36+t,36+u,36+v,36+w,36+x,36+y,36+z,36+aa,36+ab,36+ac,36+ad,36+ae,36+af,36+ag,36+ah,36+ai,36+aj,36+ak,36+al,36+am,36+an,36+ao,36+ap,36+aq,36+ar,36+as,36+at,36+au,36+av,36+aw,36+ax,36+ay,36+az,36+ba,36+bb,36+bc,36+bd,36+be,36+ w, 35 + lx, 35 + ly, 36 + a, 36 + b, 36 + c, 36 + d, 36 + e, 36 + f, 36 + g, 36 + h, 36 + i, 36 + j, 36 + k, 36 + l, 36 + m, 36 + n, 36 + o, 36 + p, 36 + q, 36 + r, 36 + s, 36 + t, 36 + u, 36 + v, 36 + w, 36 + x, 36 + y, 36 + z, 36 + aa, 36 + ab, 36 + ac, 36 + ad, 36 + ae, 36 + af, 36 + ag, 36 + ah, 36 + ai, 36 + aj, 36 + ak, 36 + al, 36 + am, 36 + an, 36 + ao, 36 + ap, 36 + aq, 36 + ar, 36 + as, 36 + at, 36 + au, 36 + av, 36 + aw, 36 + ax, 36 + ay, 36 + az, 36 + ba, 36 + bb, 36 + bc, 36 + bd, 36 + be, 36 + 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dm,41+dn,41+do,41+dp,41+dq,41+dr,41+ds,41+dt,41+du,41+dv,41+dw,41+dx,41+dy,41+dz,41+ea,41+eb,41+ec,41+ed,41+ee,41+ef,41+eg,41+eh,41+ei,41+ej,41+ek,41+el,41+em,41+en,41+eo,41+ep,41+eq,41+er,41+es,41+et,41+eu,41+ev,41+ew,41+ex,41+ey,41+ez,41+fa,41+fb,41+fc,41+fd,41+fe,41+ff,41+fg,41+fh,41+fi,41+fj,41+fk,41+fl,41+fm,41+fn,41+fo,41+fp 41+fq,41+fr,41+fs,41+ft,41+fu,41+fv,41+fw,41+fx,41+fy,41+fz,41+ga,41+gb,41+gc,41+gd,41+ge,41+gf,41+gg,41+gh,41+gi,41+gj,41+gk,41+gl,41+gm,41+gn,41+go,41+gp,41+gq,41+gr,41+gs,41+gt,41+gu,41+gv,41+gw,41+gx,41+gy,41+gz,41+ha,41+hb,41+hc,41+hd,41+he,41+hf,41+hg,41+hh,41+hi,41+hj,41+hk,41+hl,41+hm,41+hn,41+ho,41+hp,41+hq,41+hr,41+hs,41+ ht,41+hu,41+hv,41+hw,41+hx,41+hy,41+hz,41+ia,41+ib,41+ic,41+id,41+ie,41+if,41+ig,41+ih,41+ii,41+ij,41+ik,41+il,41+im,41+in,41+io,41+ip,41+iq,41+ir,41+is,41+it,41+iu,41+iv,41+iw,41+ix,41+iy,41+iz,41+ja,41+jb,41+jc,41+jd,41+je,41+jf,41+jg,41+jh,41+ji,41+jj,41+jk,41+jl,41+jm,41+jn,41+jo,41+jp,41+jq,41+jr,41+js,41+jt,41+ju,41+jv,41+jw, 1+jx,41+jy,41+jz,41+ka,41+kb,41+kc,41+kd,41+ke,41+kf,41+kg,41+kh,41+ki,41+kj,41+kk,41+kl,41+km,41+kn,41+ko,41+kp,41+kq,41+kr,41+ks,41+kt,41+ku,41+kv,41+kw,41+kx,41+ky,41+kz,41+la,41+lb,41+lc,41+ld,41+le,41+lf,41+lg,41+lh,41+li,41+lj,41+lk,41+ll,41+lm,41+ln,41+lo,41+lp,41+lq,41+lr,41+ls,41+lt,41+lu,41+lv,41+lw,41+lx,41+ly,42+a,42+b 42+c,42+d,42+e,42+f,42+g,42+h,42+i,42+j,42+k,42+l,42+m,42+n,42+o,42+p,42+q,42+r,42+s,42+t,42+u,42+v,42+w,42+x,42+y,42+z,42+aa,42+ab,42+ac,42+ad,42+ae,42+af,42+ag,42+ah,42+ai,42+aj,42+ak,42+al,42+am,42+an,42+ao,42+ap,42+aq,42+ar,42+as,42+at,42+au,42+av,42+aw,42+ax,42+ay,42+az,42+ba,42+bb,42+bc,42+bd,42+be,42+bf,42+bg,42+bh,42+bi,42+ bj,42+bk,42+bl,42+bm,42+bn,42+bo,42+bp,42+bq,42+br,42+bs,42+bt,42+bu,42+bv,42+bw,42+bx,42+by,42+bz,42+ca,42+cb,42+cc,42+cd,42+ce,42+cf,42+cg,42+ch,42+ci,42+cj,42+ck,42+cl,42+cm,42+cn,42+co,42+cp,42+cq,42+cr,42+cs,42+ct,42+cu,42+cv,42+cw,42+cx,42+cy,42+cz,42+da,42+db,42+dc,42+dd,42+de,42+df,42+dg,42+dh,42+di,42+dj,42+dk,42+dl,42+dm, 2+dn,42+do,42+dp,42+dq,42+dr,42+ds,42+dt,42+du,42+dv,42+dw,42+dx,42+dy,42+dz,42+ea,42+eb,42+ec,42+ed,42+ee,42+ef,42+eg,42+eh,42+ei,42+ej,42+ek,42+el,42+em,42+en,42+eo,42+ep,42+eq,42+er,42+es,42+et,42+eu,42+ev,42+ew,42+ex,42+ey,42+ez,42+fa,42+fb,42+fc,42+fd,42+fe,42+ff,42+fg,42+fh,42+fi,42+fj,42+fk,42+fl,42+fm,42+fn,42+fo,42+fp,42+ q,42+fr,42+fs,42+ft,42+fu,42+fv,42+fw,42+fx,42+fy,42+fz,42+ga,42+gb,42+gc,42+gd,42+ge,42+gf,42+gg,42+gh,42+gi,42+gj,42+gk,42+gl,42+gm,42+gn,42+go,42+gp,42+gq,42+gr,42+gs,42+gt,42+gu,42+gv,42+gw,42+gx,42+gy,42+gz,42+ha,42+hb,42+hc,42+hd,42+he,42+hf,42+hg,42+hh,42+hi,42+hj,42+hk,42+hl,42+hm,42+hn,42+ho,42+hp,42+hq,42+hr,42+hs,42+ht,4 2+hu,42+hv,42+hw,42+hx,42+hy,42+hz,42+ia,42+ib,42+ic,42+id,42+ie,42+if,42+ig,42+ih,42+ii,42+ij,42+ik,42+il,42+im,42+in,42+io,42+ip,42+iq,42+ir,42+is,42+it,42+iu,42+iv,42+iw,42+ix,42+iy,42+iz,42+ja,42+jb,42+jc,42+jd,42+je,42+jf,42+jg,42+jh,42+ji,42+jj,42+jk,42+jl,42+jm,42+jn,42+jo,42+jp,42+jq,42+jr,42+js,42+jt,42+ju,42+jv,42+jw,42+j ,42+jy,42+jz,42+ka,42+kb,42+kc,42+kd,42+ke,42+kf,42+kg,42+kh,42+ki,42+kj,42+kk,42+kl,42+km,42+kn,42+ko,42+kp,42+kq,42+kr,42+ks,42+kt,42+ku,42+kv,42+kw,42+kx,42+ky,42+kz,42+la,42+lb,42+lc,42+ld,42+le,42+lf,42+lg,42+lh,42+li,42+lj,42+lk,42+ll,42+lm,42+ln,42+lo,42+lp,42+lq,42+lr,42+ls,42+lt,42+lu,42+lv,42+lw,42+lx,42+ly,43+a,43+b,43+ ,43+d,43+e,43+f,43+g,43+h,43+i,43+j,43+k,43+l,43+m,43+n,43+o,43+p,43+q,43+r,43+s,43+t,43+u,43+v,43+w,43+x,43+y,43+z,43+aa,43+ab,43+ac,43+ad,43+ae,43+af,43+ag,43+ah,43+ai,43+aj,43+ak,43+al,43+am,43+an,43+ao,43+ap,43+aq,43+ar,43+as,43+at,43+au,43+av,43+aw,43+ax,43+ay,43+az,43+ba,43+bb,43+bc,43+bd,43+be,43+bf,43+bg,43+bh,43+bi,43+bj,4 3+bk,43+bl,43+bm,43+bn,43+bo,43+bp,43+bq,43+br,43+bs,43+bt,43+bu,43+bv,43+bw,43+bx,43+by,43+bz,43+ca,43+cb,43+cc,43+cd,43+ce,43+cf,43+cg,43+ch,43+ci,43+cj,43+ck,43+cl,43+cm,43+cn,43+co,43+cp,43+cq,43+cr,43+cs,43+ct,43+cu,43+cv,43+cw,43+cx,43+cy,43+cz,43+da,43+db,43+dc,43+dd,43+de,43+df,43+dg,43+dh,43+di,43+dj,43+dk,43+dl,43+dm,43+d ,43+do,43+dp,43+dq,43+dr,43+ds,43+dt,43+du,43+dv,43+dw,43+dx,43+dy,43+dz,43+ea,43+eb,43+ec,43+ed,43+ee,43+ef,43+eg,43+eh,43+ei,43+ej,43+ek,43+el,43+em,43+en,43+eo,43+ep,43+eq,43+er,43+es,43+et,43+eu,43+ev,43+ew,43+ex,43+ey,43+ez,43+fa,43+fb,43+fc,43+fd,43+fe,43+ff,43+fg,43+fh,43+fi,43+fj,43+fk,43+fl,43+fm,43+fn,43+fo,43+fp,43+fq,4 +fr,43+fs,43+ft,43+fu,43+fv,43+fw,43+fx,43+fy,43+fz,43+ga,43+gb,43+gc,43+gd,43+ge,43+gf,43+gg,43+gh,43+gi,43+gj,43+gk,43+gl,43+gm,43+gn,43+go,43+gp,43+gq,43+gr,43+gs,43+gt,43+gu,43+gv,43+gw,43+gx,43+gy,43+gz,43+ha,43+hb,43+hc,43+hd,43+he,43+hf,43+hg,43+hh,43+hi,43+hj,43+hk,43+hl,43+hm,43+hn,43+ho,43+hp,43+hq,43+hr,43+hs,43+ht,43+hu ,43+hv,43+hw,43+hx,43+hy,43+hz,43+ia,43+ib,43+ic,43+id,43+ie,43+if,43+ig,43+ih,43+ii,43+ij,43+ik,43+il,43+im,43+in,43+io,43+ip,43+iq,43+ir,43+is,43+it,43+iu,43+iv,43+iw,43+ix,43+iy,43+iz,43+ja,43+jb,43+jc,43+jd,43+je,43+jf,43+jg,43+jh,43+ji,43+jj,43+jk,43+jl,43+jm,43+jn,43+jo,43+jp,43+jq,43+jr,43+js,43+jt,43+ju,43+jv,43+jw,43+jx,43 jy,43+jz,43+ka,43+kb,43+kc,43+kd,43+ke,43+kf,43+kg,43+kh,43+ki,43+kj,43+kk,43+kl,43+km,43+kn,43+ko,43+kp,43+kq,43+kr,43+ks,43+kt,43+ku,43+kv,43+kw,43+kx,43+ky,43+kz,43+la,43+lb,43+lc,43+ld,43+le,43+lf,43+lg,43+lh,43+li,43+lj,43+lk,43+ll,43+lm,43+ln,43+lo,43+lp,43+lq,43+lr,43+ls,43+lt,43+lu,43+lv,43+lw,43+lx,43+ly.
【0047】 [0047]
本発明組成物及び本発明方法における式(1)で表される化合物と、化合物群Aから選ばれる化合物との好適な混合割合は、式(1)で表される化合物の1重量部に対して、化合物群Aから選ばれる化合物は通常0.001〜1000重量部、好ましくは0.01〜100重量部、より好ましくは0.1〜10重量部である。 A compound represented by the formula (1) in the present invention compositions and method of the present invention, a suitable mixing ratio of the compounds selected from the compound group A is, relative to 1 part by weight of the compound represented by formula (1) Te, compounds selected from the compound group a is usually 0.001 to 1000 parts by weight, preferably 0.01 to 100 parts by weight, more preferably 0.1 to 10 parts by weight.
【0048】 [0048]
本発明組成物及び本発明方法における有効成分化合物の好ましい処理量は、防除すべき対象病害虫の種類などにより左右されるが、通常式(1)で表される化合物が0.1〜1000gai/ha、化合物群Aから選ばれる化合物が0.1〜1000gai/haであり、好ましくは前者が1〜300gai/haであり、後者が1〜300gai/haである。 Preferred processes of the active ingredient compound in the composition of the present invention and the present invention method will depend the kind of the target pest to be controlled, the compound represented by the normal equation (1) is 0.1~1000gai / ha a compound 0.1~1000gai / ha selected from the compound group a, preferably the former is the 1~300gai / ha, the latter 1~300gai / ha.
【0049】 [0049]
本発明組成物は、農園芸作物および樹木などを加害するいわゆる農業害虫、農業病害、家畜家禽類に寄生するいわゆる家畜害虫、家屋等の人間の生活環境で悪影響を与えるいわゆる衛生害虫、および同様の場面で発生加害するダニ類や線虫類に対して適用できる。 The composition of the present invention, so-called agricultural pests infesting and horticultural crops and trees, agricultural diseases, so-called livestock insect pests which are parasitic on livestock poultry, so-called sanitary insect pests adversely affect the human living environment of a house or the like, and the like It can be applied to mites and nematodes that occur perpetrators at the scene. 本発明組成物を用いて防除しうる害虫、ダニ類、線虫類、病害には具体的には次に示すものがあるが、それらのみに限定されるものではない。 Pests which can control using the present compositions, mites, nematodes, although the disease are those shown below in particular, are not limited only to them.
【0050】 [0050]
害虫としては、ハスモンヨトウ(Spodoptera litura)、コブノメイガ(Cnaphalocrocis medinalis)、コナガ(Plutella xylostella)、ヨトウガ(Mamestra brassicae)、モンシロチョウ(Pieris rapae crucivora)、カブラヤガ(Agrotis segetum)、チャノコカクモンハマキ(Adoxophyes sp.)、チャハマキ(Homona magnanima)、タバコバットワーム(Heliothis virescens)、ヨーロピアンコーンボーラー(Ostrinia nubilalis)、フォールアーミーワーム(Spodoptera frugiperda)、コーンイヤーワーム(Helicov The pest, common cutworm (Spodoptera litura), leaf roller (Cnaphalocrocis medinalis), diamondback moth (Plutella xylostella), cabbage armyworm (Mamestra brassicae), cabbage butterfly (Pieris rapae crucivora), Kaburayaga (Agrotis segetum), smaller tea tortrix (Adoxophyes sp.) , Chahamaki (Homona magnanima), tobacco bat worm (Heliothis virescens), European corn borer (Ostrinia nubilalis), fall armyworm (Spodoptera frugiperda), corn earworm (Helicov rpa zea)などの鱗翅目害虫、ツマグロヨコバイ(Nephotettix cincticeps)、トビイロウンカ(Nilaparvata lugens)、モモアカアブラムシ(Myzus persicae)、クサギカメムシ(Halyomorpha mista)、トコジラミ(Cimex lectularius)などの半翅目害虫、ニジュウヤホシテントウ(Epilachna vigintioctpunctata)、ドウガネブイブイ(Anomala cuprea)、イネミズゾウムシ(Lissorhopterus oryzophilus)、サザンコーンルートワーム(、ノーザンコーンルートワーム(Diabrotica barberi)、ウェスタンコーンルートワーム(Diabroti rpa zea) lepidopteran pests such as, green rice leafhopper (Nephotettix cincticeps), brown planthopper (Nilaparvata lugens), green peach aphid (Myzus persicae), brown marmorated stink bug (Halyomorpha mista), Hemiptera pests such as bed bugs (Cimex lectularius), Nijuuya Hoshitentou (Epilachna vigintioctpunctata), cupreous chafer (Anomala cuprea), rice water weevil (Lissorhopterus oryzophilus), Southern corn rootworm (northern corn rootworm (Diabrotica barberi), western corn rootworm (Diabroti a virgifera virgifera)、ココクゾウ(Sitophilus oryzae)などの鞘翅目害虫、イエバエ(Musca domestica)、アカイエカ(Culex pipiens pallens)、マメハモグリバエ(Liriomyza trifolii)、ウリミバエ(Dacus cucurbitae)などの双翅目害虫、ミナミキイロアザミウマ(Thrips palmi)、ネギアザミウマ(Thrips tabaci)、ミカンキイロアザミウマ(Frankliniella occidentalis)などの総翅目害虫、ネコノミ(Ctenocephalidae felis)、ケオプスネズミノミ(Xenopsylla cheopis)、などの等翅目害虫、ニワトリオオハジラ a virgifera virgifera), Kokokuzou (Sitophilus oryzae) Coleoptera pests such as, housefly (Musca domestica), Culex (Culex pipiens pallens), legume leafminer (Liriomyza trifolii), Diptera pests such as melon fly (Dacus cucurbitae), Minamikiiro thrips (thrips palmi), green onion thrips (thrips tabaci), western flower thrips (Frankliniella occidentalis) Thysanoptera pests such as, cat flea (Ctenocephalidae felis), Quai rat flea (Xenopsylla cheopis), Isoptera pests such as, chicken Oohajira (Menacanthus stramineus)、ウシハジラミ(Bovicola bovis)などのハジラミ目害虫、ウシジラミ(Haematopinus eurysternus)、ウシホソジラミ(Linognathus vituli)などのシラミ目害虫、ミカンハダニ(Panonychus citri)、ナミハダニ(Tetranychus urticae)、カンザワハダニ(Tetranychus kanzawai)などのハダニ類、ミカンサビダニ(Aculops pelekassi)、チャノナガサビダニ(Acaphylla theavagrans)などのフシダニ類、チャノホコリダニ(Polyphagotarsonemus latus)、シクラメンホコリダニ(Steneota (Menacanthus stramineus), Ushihajirami (Bovicola bovis) Mallophaga pests such as, Ushijirami (Haematopinus eurysternus), Ushihosojirami (Linognathus vituli) Anoplura pests such as, citrus red mite (Panonychus citri), two-spotted spider mite (Tetranychus urticae), kanzawai (Tetranychus kanzawai) spider mites such as, tangerine rust mite (Aculops pelekassi), Fushidani such as tea Roh Naga rust mite (Acaphylla theavagrans), Chanohokoridani (Polyphagotarsonemus latus), cyclamen dust mites (Steneota sonemus pallidus)などのホコリダニ類、ケナガコナダニ(Tyrophagus putrescentiae)、ロビンネダニ(Rhizoglyphus robini)などのコナダニ類、オウシマダニ(Boophilusmicroplus)、フタトゲチマダニなどのマダニ類、ウサギキュウセンダニ(Psoroptes cuniculi)、ヒツジキュウセンダニ(Psoroptes ovis)などのキュウセンダニ類、ヒゼンダニ(Sarcoptes scabiei)などのヒゼンダニ類、サツマイモネコブセンチュウ(Meloidogyne javanica)、キタネグサレセンチュウ(Pratylenchus penetrans)およびジャガイモシストセンチュウ(Globode sonemus pallidus) dust mite such as, Tyrophagus (Tyrophagus putrescentiae), the bulb mite, Rhizoglyphus (Rhizoglyphus robini) grain mites such as Boophilus microplus (Boophilusmicroplus), ticks such as Haemaphysalis longicornis, rabbit 9,000 mites (Psoroptes cuniculi), sheep 9,000 mites (Psoroptes ovis) Kyuusendani such as, mites such as mites (Sarcoptes scabiei), Meloidogyne incognita (Meloidogyne javanica), northern Negu Saleh nematode (Pratylenchus penetrans) and potato cyst nematode (Globode ra rostochiensis)などの線虫類などが挙げられる。 ra rostochiensis) and the like nematodes, such as.
【0051】 [0051]
一方、病害としては、イネのいもち病(Pyricularia oryzae)、ごま葉枯病(Cochliobolus miyabeanus)、紋枯病(Rhizoctonia solani)、ムギ類のうどんこ病(Erysiphe graminis f.sp.hordei, f.sp.tritici)、斑葉病(Pyrenophoragraminea)、網斑病(Pyrenophora teres)、赤かび病(Gibberella zeae)、さび病(Puccinia striiformis, P.graminis, P.recondita, P.hordei)、雪腐病(Tipula sp., Micronectriella nivais)、裸黒穂病(Ustilago tritici, U. On the other hand, as the diseases, rice blast (Pyricularia oryzae), Gomaha spot (Cochliobolus miyabeanus), sheath blight (Rhizoctonia solani), wheat powdery mildew (Erysiphe graminis f.sp.hordei, f.sp .tritici), Madarahabyo (Pyrenophoragraminea), net blotch (Pyrenophora teres), Fusarium head blight (Gibberella zeae), rust (Puccinia striiformis, P.graminis, P.recondita, P.hordei), snow mold disease ( Tipula sp., Micronectriella nivais), loose smut (Ustilago tritici, U. uda)、アイスポット(Pseudocercosporella herpotrichoides)、雲形病(Rhynchosporium secalis)、葉枯病(Septoria tritici)、ふ枯病(Leptosphaeria nodorum)、カンキツの黒点病(Diaporthe citri)、そうか病(Elsinoe fawcetti)、果実腐敗病(Penicillium digitalum, P.italicum)、リンゴのモニリア病(Selerotinia mali)、腐らん病(Valsa mali)、うどんこ病(Podosphaera lcucotricha)、斑点落葉病(Alternaria mali)、黒星病(Venturia inaequalis)、ナ uda), eye spot (Pseudocercosporella herpotrichoides), scald (Rhynchosporium secalis), leaf blight (Septoria tritici), glume blotch (Leptosphaeria nodorum), citrus black spot disease (Diaporthe citri), scab (Elsinoe fawcetti), fruit rot (Penicillium digitalum, P.italicum), apple blossom disease (Selerotinia mali), canker (Valsa mali), powdery mildew (Podosphaera lcucotricha), leaf spot disease (Alternaria mali), scab (Venturia inaequalis) , Na の黒星病(Venturia nashicola)、黒斑病(Alternaria kikuchiana)、赤星病(Gymnosporangium haracanum)、モモの灰星病(Sclerolinia cinerea)、黒星病(Cleadosporium carpophilum)、フォモプシス腐敗病(Phomopsis sp.)、ブドウのべと病(Plasmopara viticola)、黒とう病(Elsinoe ampelina)、晩腐病(Glomerella cingulata)、うどんこ病(Uncinula necator)、さび病(Phakopsora ampelopsidis)、カキの炭そ病(Gloeosporium kakj)、落葉病(Cercospora ka Of scab (Venturia nashicola), black spot disease (Alternaria kikuchiana), gymnosporangium (Gymnosporangium haracanum), peach Haiboshi disease (Sclerolinia cinerea), scab (Cleadosporium carpophilum), Phomopsis rot (Phomopsis sp.), Grapes total mildew (Plasmopara viticola), sphaceloma disease (Elsinoe ampelina), ripe rot (Glomerella cingulata), powdery mildew (Uncinula necator), rust (Phakopsora ampelopsidis), oysters of anthracnose (Gloeosporium kakj), deciduous disease (Cercospora ka j,Mycosphaerella nawae)、ウリ類のべと病(Pseudoperenospora cubensis)、炭そ病(Colletotrichum lagenarium)、うどんこ病(Sphaerotheca fuliginea)、つる枯病(Mycosphaerella melonis)、トマトの疫病(Phytophthora infestans)、輪紋病(Alternaria solani)、葉かび病(Cladosporium fulvum)、ナスの褐紋病(Phomopsis vexans)、うどんこ病(Erysiphe cichoracoarum)、アブラナ科野菜の黒斑病(Alternaria japonica)、白斑病(Cercosporella brass j, Mycosphaerella nawae), Cucurbitaceae of downy mildew (Pseudoperenospora cubensis), anthracnose (Colletotrichum lagenarium), powdery mildew (Sphaerotheca fuliginea), vine blight (Mycosphaerella melonis), tomato late blight (Phytophthora infestans), wheel crest disease (Alternaria solani), leaf mold disease (Cladosporium fulvum), eggplant 褐紋 disease (Phomopsis vexans), powdery mildew (Erysiphe cichoracoarum), black spot disease of cruciferous vegetables (Alternaria japonica), white spot disease (Cercosporella brass icae)、ネギのさび病(Puccinia allii)、ダイズの紫斑病(Cercospora kikuchii)、黒とう病(Elsinoe glycines)、黒点病(Diaporthe phaseololum)、インゲンの炭そ病(Colletotrichum lindemuthianum)、ラッカセイの黒渋病(Mycosphaerella personatum)、褐斑病(Cercospora arachidicola)、エンドウのうどんこ病(Erysiphe pisi)、ジャガイモの夏疫病(Alternaria solani)、イチゴのうどんこ病(Sphaerotheca humuli)、チャの網もち病(Exobasidium reticulatum)、白星病(Els icae), leek rust (Puccinia allii), soybean purpura (Cercospora kikuchii), sphaceloma disease (Elsinoe glycines), black spot disease (Diaporthe phaseololum), green beans of anthracnose (Colletotrichum lindemuthianum), black astringency of peanut disease (Mycosphaerella personatum), brown spot disease (Cercospora arachidicola), pea powdery mildew (Erysiphe pisi), early blight of potatoes (Alternaria solani), strawberry powdery mildew (Sphaerotheca humuli), tea of ​​the net have disease (Exobasidium reticulatum), white star disease (Els noe leucospila)、タバコの赤星病(Alternaria lingipes)、うどんこ病(Erysiphe cichoracearum)、炭そ病(Colletotrichum tabacum)、テンサイの褐斑病(Cercospora beticola)、バラの黒星病(Diplocarpon rosae)、うどんこ病(Sphaerotheca pannosa)、キクの褐斑病(Septoria chrysanthemiindici)、白さび病(Puccinia horiana)、種々の作物の灰色かび病(Botrytis cinerea)および種々の作物の菌核病(Sclerotinia sclerotiorum)等が挙げられる。 noe leucospila), tobacco gymnosporangium (Alternaria lingipes), powdery mildew (Erysiphe cichoracearum), anthracnose (Colletotrichum tabacum), sugar beet of brown spot disease (Cercospora beticola), rose of scab (Diplocarpon rosae), powdery mildew disease (Sphaerotheca pannosa), chrysanthemum brown spot disease (Septoria chrysanthemiindici), like white rust (Puccinia horiana), gray mold of various crops (Botrytis cinerea) and various crops Rot (Sclerotinia sclerotiorum) and the like It is.
【0052】 [0052]
式(1)で表されるアクリロニトリル化合物と前記の第2表に示した化合物を組み合わせた場合に、本発明組成物及び本発明方法は、特にダニに対して優れた相乗効果を奏するが、ダニの中でもミカンハダニ、ナミハダニ、カンザワハダニなどのハダニ類、チャノナガサビダニ、カーネーションサビダニ、チューリップサビダニ、ミカンサビダニ、モモサビダニ、リンゴサビダニ、チャノサビダニ、ブドウサビダニ、ナシサビダニ、ニセナシサビダニなどのフシダニ類、チャノホコリダニ、シクラメンホコリダニなどのホコリダニ類に対して、より優れた相乗効果を奏する。 When combined compounds shown in Table 2 acrylonitrile compound of the formula (1), the present invention compositions and method of the present invention, particularly exhibits an excellent synergistic effect against mites, mite spider mites of the citrus red mite, two-spotted spider mite, such as kanzawai among, tea Roh Naga rust mite, carnation rust mite, tulip rust mite, tangerine rust mite, peach silver mite, Aculus. induced, apple rust mite, Chanosabidani, grape rust mite, Nashisabidani, Fushidani such as false pear rust mite, Chanohokoridani, cyclamen dust mites, etc. against dust mite such exhibits better synergy.
【0053】 [0053]
本発明の式(1)で表されるアクリロニトリル化合物は、下記スキーム1に記載した方法によって合成できる。 Acrylonitrile compounds represented by the formula (1) of the present invention can be synthesized by the method described in Scheme 1. 即ち、一般式(2)で表されるシアノメチルベンゼン誘導体と一般式(3)で表されるカルボン酸誘導体とを塩基存在下で反応させることにより(1 )を合成することができ、更にこれを一般式(4)で表される化合物と反応させることにより式(1)で表される化合物が得られる。 That is, by reacting the general formula (2) with a cyano methylbenzene derivative with the general formula represented with a carboxylic acid derivative represented by (3) in the presence of a base (1) can be synthesized, further This compound represented by the general formula wherein by reacting the compound represented by (4) (1) is obtained.
〔スキーム1〕 [Scheme 1]
【0054】 [0054]
【化16】 [Of 16]
【0055】 [0055]
[スキーム1中のG、A及びBは前記と同じ意味を表し、L 及びL は良好な脱離基、例えば塩素原子、臭素原子、ヨウ素原子、C 〜C アルキルスルホニルオキシ、ベンゼンスルホニルオキシ、トルエンスルホニルオキシ、1−イミダゾリル及び1−ピラゾリル等である。 [G in Scheme 1, A and B are as defined above, L 1 and L 2 are good leaving group such as chlorine atom, bromine atom, iodine atom, C 1 -C 4 alkylsulfonyloxy, benzene sulfonyloxy, toluenesulfonyloxy, 1-imidazolyl and 1-pyrazolyl, and the like. ]。 ].
【0056】 [0056]
上記の方法は塩基を用いたほうが好ましい場合もある。 The above method may be preferred better with a base. 用いられる塩基としてはナトリウムエトキシド、ナトリウムメトキシド及びtーブトキシカリウム等のアルカリ金属アルコキシド類、水酸化ナトリウム及び水酸化カリウム等のアルカリ金属水酸化物、炭酸ナトリウム及び炭酸カリウム等のアルカリ金属炭酸塩、トリエチルアミン、ピリジン及びDBU等の有機塩基、ブチルリチウム等の有機リチウム化合物、リチウムジイソプロプロピルアミド及びリチウムビストリメチルシリルアミド等のリチウムアミド類並びに水素化ナトリウム等が挙げられる。 Alkali metal alkoxides such as sodium ethoxide, sodium methoxide and t-butoxy potassium and as the base used include alkali metal hydroxides, alkali metal carbonates such as sodium carbonate and potassium carbonate, such as sodium hydroxide and potassium hydroxide , triethylamine, pyridine and DBU and organic bases, organic lithium compounds such as butyl lithium, and lithium amide and sodium hydride such as lithium di-iso-propyl amide and lithium bis (trimethylsilyl) amide and the like.
【0057】 [0057]
上記の反応は、反応に不活性な溶媒中で行う事ができ、溶媒としてはメタノール及びエタノール等の低級アルコール類、ベンゼン及びトルエン等の芳香族炭化水素類、ジエチルエーテル、テトラヒドロフラン、1,4−ジオキサン、1,2−ジメトキシエタン及び1,2−ジエトキシエタン等のエーテル類、アセトン、メチルエチルケトン及びメチルイソブチルケトン等のケトン類、塩化メチレン、クロロホルム及び1,2−ジクロロエタン等のハロゲン化炭化水素類、ジメチルホルムアミド、ジメチルアセトアミド及び1,3−ジメチルイミダゾリジノン等のアミド類、アセトニトリル等のニトリル類、ジメチルスルホキシド並びにこれらの混合溶媒等が挙げられる。 The above reaction can be carried out in a solvent inert to the reaction, lower alcohols such as solvents such as methanol and ethanol, aromatic hydrocarbons such as benzene and toluene, diethyl ether, tetrahydrofuran, 1,4 dioxane, 1,2-dimethoxyethane and 1,2 ethers of diethoxy ethane acids, ketones such as acetone and methyl ethyl ketone and methyl isobutyl ketone, methylene chloride, chloroform and 1,2 halogenated hydrocarbons dichloroethane , dimethylformamide, amides such as dimethylacetamide and 1,3-dimethyl imidazolidinone, nitriles such as acetonitrile, dimethyl sulfoxide and mixed solvents thereof. 場合によっては、これらの溶媒と水との混合溶媒も用いる事ができ、テトラ−n−ブチルアンモニウムブロマイド等の4級アンモニウム塩を触媒として添加する事により好結果が得られる場合もある。 In some cases, a mixed solvent of these solvents with water can also be used, in some cases good results are obtained by adding a quaternary ammonium salt such as tetra -n- butylammonium bromide as catalyst. 反応温度は−70℃から200℃の任意の温度に設定する事が可能であり、0℃から150℃または溶媒を用いる場合には−70℃から溶媒の沸点の範囲が好ましい。 The reaction temperature is can be set to any temperature of 200 ° C. from -70 ° C., preferably the boiling point of the solvent -70 ° C. in the case of using a 0.99 ° C. or solvent from 0 ° C.. 塩基は反応基質の0.05から10当量を、好ましくは0.05から3当量の範囲である。 Base 0.05 to 10 equivalents of the reaction substrate, preferably in the range of 3 equivalents of 0.05.
【0058】 [0058]
式(1)で表される化合物は、常法により反応液から得ることができるが、式(1)で表される化合物を精製する必要が生じた場合には再結晶、カラムクロマトグラフィー等の任意の精製法によって分離、精製することができる。 Compounds of formula (1) can be usual manner obtained from the reaction solution, recrystallization if necessary to purify the compound represented by the formula (1) has occurred, such as column chromatography separated by any purification method, it can be purified.
【0059】 [0059]
なお、式(1)で表される化合物が不斉炭素を有する場合には、式(1)で表される化合物は、光学活性な化合物(+)体、(−)体、又は両者を任意の比率で含むラセミ体の何れであってもよい。 In the case where the compound represented by the formula (1) have asymmetric carbons, the compound represented by formula (1) is an optically active compound (+) form, (-) Optional body, or both it may be any one of a racemate comprising a ratio of.
【0060】 [0060]
本発明組成物は、式(1)で表されるアクリトニトリル化合物の少なくとも1種と、化合物群Aの中から選ばれる少なくとも1種とを混合物としてそのまま使用することもできるが、通常適当な固体担体又は液体担体と混合し、更に所望により界面活性剤、浸透剤、展着剤、増粘剤、凍結防止剤、結合剤、固結防止剤、崩壊剤、消泡剤、防腐剤および分解防止剤等を添加して、液剤(soluble concentrate)、乳剤(emulsifiable concentrate)、水和剤(wettable powder)、水溶剤(water soluble powder)、顆粒水和剤(water dispersible granule)、顆粒水溶剤(water soluble granule)、懸濁剤(susp The compositions of the invention, at least one acrylate preparative nitrile compound represented by the formula (1), but it can also be used as a mixture with at least one selected from the group of compounds A, usually appropriate mixed with a solid carrier or liquid carrier, further optionally a surfactant, a penetrant, spreader, thickener, anti-freezing agents, binders, anti-caking agents, disintegrants, defoaming agents, preservatives and degradation by adding inhibitors such as, liquid (soluble concentrate), emulsions (emulsifiable concentrate), wettable powders (wettable powder), soluble powders (water soluble powder), water dispersible granules (water dispersible granule), water soluble granules ( water soluble granule), suspending agent (susp nsion concentrate)、乳濁剤(concentrated emulsion)、サスポエマルジョン(suspoemulsion)、マイクロエマルジョン(microemulsion)、粉剤(dustable powder)、粒剤(granule)およびゲル剤(gel)等任意の剤型の製剤にて実用に供することができる。 nsion concentrate), emulsions (concentrated emulsion), suspoemulsions (suspoemulsion), microemulsion (microemulsion), dusts (dustable powder), granules (granule) and gels (gel) in such an arbitrary dosage form of the formulation it can be subjected to practical use Te. また、省力化および安全性向上の観点から、上記任意の剤型の製剤を、水溶性カプセルおよび水溶性フィルムの袋等の水溶性包装体に封入して供することもできる。 From the viewpoint of laborsaving and safety improvement, the arbitrary dosage form of the preparation, may be subjected to encapsulation in a water-soluble package of bags such as water-soluble capsules and water-soluble film.
【0061】 [0061]
固体担体としては、例えば石英、カオリナイト、パイロフィライト、セリサイト、タルク、ベントナイト、酸性白土、アタパルジャイト、ゼオライトおよび珪藻土等の天然鉱物質類、炭酸カルシウム、硫酸アンモニウム、硫酸ナトリウムおよび塩化カリウム等の無機塩類、合成シリカならびに合成シリケートが挙げられる。 Examples of the solid carrier, such as quartz, kaolinite, pyrophyllite, sericite, talc, bentonite, acid clay, attapulgite, natural mineral such as zeolite and diatomaceous earth, calcium carbonate, ammonium sulfate, such as sodium sulfate and potassium chloride inorganic salts, synthetic silica and synthetic silicates may be mentioned.
【0062】 [0062]
液体担体としては、例えばエチレングリコール、プロピレングリコールおよびイソプロパノール等のアルコール類、キシレン、アルキルベンゼンおよびアルキルナフタレン等の芳香族炭化水素類、ブチルセロソルブ等のエーテル類、シクロヘキサノン等のケトン類、γ−ブチロラクトン等のエステル類、N−メチルピロリドンおよびN−オクチルピロリドン等の酸アミド類、大豆油、ナタネ油、綿実油およびヒマシ油等の植物油ならびに水が挙げられる。 Examples of the liquid carrier, such as ethylene glycol, alcohols such as propylene glycol and isopropanol, xylene, aromatic hydrocarbons such as alkylbenzenes and alkylnaphthalenes, ethers such as butyl cellosolve, ketones such as cyclohexanone, esters such as γ- butyrolactone s, N- methylpyrrolidone and N- octylpyrrolidone acid amides such as, soybean oil, rapeseed oil, vegetable oils and water, such as cottonseed oil and castor oil.
【0063】 [0063]
これら固体および液体担体は、単独で用いても2種以上を併用してもよい。 These solid and liquid carriers may be used in combination of two or more kinds thereof may be used alone.
【0064】 [0064]
界面活性剤としては、例えばポリオキシエチレンアルキルエーテル、ポリオキシエチレンアルキルアリールエーテル、ポリオキシエチレンスチリルフェニルエーテル、ポリオキシエチレンポリオキシプロピレンブロックコポリマー、ポリオキシエチレン脂肪酸エステル、ソルビタン脂肪酸エステルおよびポリオキシエチレンソルビタン脂肪酸エステル等のノニオン性界面活性剤、アルキル硫酸塩、アルキルベンゼンスルホン酸塩、リグニンスルホン酸塩、アルキルスルホコハク酸塩、ナフタレンスルホン酸塩、アルキルナフタレンスルホン酸塩、ナフタレンスルホン酸のホルマリン縮合物の塩、アルキルナフタレンスルホン酸のホルマリン縮合物の塩、ポリオキシエチレンアルキルアリールエーテル硫酸および燐酸塩、ポリオキシエチレンス Examples of the surfactant include polyoxyethylene alkyl ethers, polyoxyethylene alkyl aryl ether, polyoxyethylene styryl phenyl ether, polyoxyethylene polyoxypropylene block copolymers, polyoxyethylene fatty acid esters, sorbitan fatty acid esters and polyoxyethylene sorbitan nonionic surfactants such as fatty acid esters, alkyl sulfates, alkylbenzene sulfonates, lignin sulfonates, alkyl sulfosuccinates, naphthalene sulfonates, alkylnaphthalene sulfonates, salts of formalin condensate of naphthalenesulfonic acid, salts of formalin condensate of alkylnaphthalene sulfonic acid, polyoxyethylene alkyl aryl ether sulfates and phosphates, polyoxyethylene scan リルフェニルエーテル硫酸および燐酸塩、ポリカルボン酸塩およびポリスチレンスルホン酸塩等のアニオン性界面活性剤、アルキルアミン塩およびアルキル4級アンモニウム塩等のカチオン性界面活性剤ならびにアミノ酸型およびベタイン型等の両性界面活性剤が挙げられる。 Phenyl ether sulfates and phosphates, anionic surfactants such as polycarboxylate and polystyrene sulfonate, amphoteric cationic surfactants and amino acid type and betaine type, such as alkylamine salts and alkyl quaternary ammonium salts surfactants.
【0065】 [0065]
これら界面活性剤の含有量は、特に限定されるものではないが、本発明の製剤100重量部に対し、通常0.05〜20重量部の範囲が望ましい。 The content of these surfactants is not particularly limited with respect to the formulation 100 parts by weight of the present invention, the range of usually 0.05 to 20 parts by weight is desirable. また、これら界面活性剤は、単独で用いても2種以上を併用してもよい。 These surfactants may be used in combination of two or more kinds thereof may be used alone.
【0066】 [0066]
次に本発明組成物を用いる場合の製剤の配合例を示す。 Following the formulation examples of formulations in the case of using the present composition. 但し本発明の配合例は、これらのみに限定されるものではない。 However formulation of the present invention is not limited thereto. なお、以下の配合例において「部」は重量部を意味する。 Incidentally, "parts" in the following formulation examples are parts by weight.
【0067】 [0067]
〔水和剤(wettable powder)〕 [Wettable powders (wettable powder)]
有効成分化合物 0.1〜80部固体担体 5〜98.9部界面活性剤 1〜10部その他 0〜 5部その他として、例えば固結防止剤、分解防止剤等があげれらる。 Active ingredient compound 0.1-80 parts Solid carrier 5 to 98.9 parts Surfactant 1 to 10 parts Others 0-5 parts As other, for example, anti-caking agents, stabilizing agents and the like Agereraru.
【0068】 [0068]
〔乳 剤(emulsifiable concentrate)〕 [Milk agent (emulsifiable concentrate)]
有効成分化合物 0.1〜30部液体担体 45〜95部界面活性剤 4.9〜15部その他 0〜10部その他として、例えば展着剤、分解防止剤等が挙げられる。 Other active ingredient compound 0.1 to 30 parts Liquid carrier 45 to 95 parts Surfactant 4.9 to 15 parts Others 0 to 10 parts, for example spreading agents, stabilizing agents and the like.
【0069】 [0069]
〔懸濁剤(suspension concentrate)〕 [Suspension (suspension concentrate)]
有効成分化合物 0.1〜70部液体担体 15〜98.89部界面活性剤 1〜12部その他 0.01〜30部その他として、例えば凍結防止剤、増粘剤等が挙げられる。 Other active ingredient compound 0.1-70 parts Liquid carrier 15 to 98.89 parts Surfactant 1 to 12 parts Others 0.01 to 30 parts, for example antifreeze agents, thickening agents, and the like.
【0070】 [0070]
〔顆粒水和剤(water dispersible granule)〕 [Water dispersible granules (water dispersible granule)]
有効成分化合物 0.1〜90部固体担体 0〜98.9部界面活性剤 1〜20部その他 0〜 10部その他として、例えば結合剤、分解防止剤等が挙げられる。 Other active ingredient compound 0.1-90 parts Solid carrier 0 to 98.9 parts Surfactant 1 to 20 parts Others 0-10 parts, such as binders, stabilizing agents and the like.
【0071】 [0071]
〔液 剤(soluble concentrate)〕 [Liquid agent (soluble concentrate)]
有効成分化合物 0.01〜70部液体担体 20〜99.99部その他 0〜 10部その他として、例えば凍結防止剤、展着剤等が挙げられる。 Other active ingredient compound 0.01-70 parts Liquid carrier 20 to 99.99 parts Others 0-10 parts, for example, an antifreezing agent, a spreading agent, and the like.
【0072】 [0072]
〔粒 剤(granule)〕 [Granules (granule)]
有効成分化合物 0.01〜80部固体担体 10〜99.99部その他 0〜10部その他として、例えば結合剤、分解防止剤等が挙げられる。 Other active ingredient compound 0.01-80 parts Solid carrier 10 to 99.99 parts Others 0 to 10 parts, such as binders, stabilizing agents and the like.
【0073】 [0073]
〔粉 剤(dustable powder)〕 [Powder agent (dustable powder)]
有効成分化合物 0.01〜30部固体担体 65〜99.99部その他 0〜5部その他として、例えばドリフト防止剤、分解防止剤等が挙げられる。 Other active ingredient compound 0.01 to 30 parts Solid carrier 65 to 99.99 parts Others 0 to 5 parts Examples of anti-drift agents, stabilizing agents and the like.
【0074】 [0074]
〔製剤例〕 [Formulation Example]
次に具体的に本発明組成物を有効成分とする農薬製剤例を示すがこれらのみに限定されるものではない。 Then they show pesticidal formulation examples to specifically present compositions the active ingredient is not limited only thereto. 尚、以下の配合例において「部」は重量部を意味する。 Incidentally, "parts" in the following formulation examples are parts by weight.
【0075】 [0075]
〔配合例1〕水和剤(wettable powder) Formulation Example 1] Wettable powder (wettable powder)
化合物No. Compound No. 1 10部化合物No. 1 10 parts of Compound No. a 10部パイロフィライト 76部ソルポール5039 2部(非イオン性界面活性剤とアニオン性界面活性剤との混合物:東邦化学工業(株)商品名) a 10 parts pyrophyllite 76 parts Sorpol 5039 2 parts (mixture of nonionic surfactant and anionic surfactant: Toho Chemical Industry Co., trade name)
カープレックス#80D 2部(合成含水珪酸:塩野義製薬(株)商品名) Carplex # 80D 2 parts (synthetic hydrous silicate: Shionogi & Co., Ltd., trade name)
以上を均一に混合粉砕して水和剤とする。 A wettable powder were uniformly mixed and ground to above.
【0076】 [0076]
〔配合例2〕乳 剤(emulsifiable concentrate) Formulation Example 2 Emulsion (emulsifiable concentrate)
化合物No. Compound No. 2 3部化合物No. 2 3 parts Compound No. b 2部キシレン 75部N−メチルピロリドン 15部ソルポール2680 5部(非イオン性界面活性剤とアニオン性界面活性剤との混合物:東邦化学工業(株)商品名) b 2 parts of xylene 75 parts of N- methylpyrrolidone 15 parts Sorpol 2680 5 parts (mixture of nonionic surfactant and anionic surfactant: Toho Chemical Industry Co., trade name)
以上を均一に混合して乳剤とする。 The emulsion was uniformly mixed more.
【0077】 [0077]
〔配合例3〕懸濁剤(suspension concentrate) Formulation Example 3 suspension (suspension concentrate)
化合物No. Compound No. 3 15部化合物No. 3 15 parts of Compound No. c 10部アグリゾールS−710 10部(非イオン性界面活性剤:花王(株)商品名) c 10 parts Agurizoru S-710 10 parts (nonionic surfactant: Kao Corporation trade name)
ルノックス1000C 0.5部(アニオン性界面活性剤:東邦化学工業(株)商品名) Lunox 1000 C-0.5 parts (Anionic surfactant: Toho Chemical Industry Co., trade name)
キサンタンガム 0.2部水 64.3部以上を均一に混合した後、湿式粉砕して懸濁剤とする。 After uniformly mixing xanthan gum 0.2 parts Water 64.3 parts The above, and suspending agent and wet grinding.
【0078】 [0078]
〔配合例4〕顆粒水和剤(water dispersible granule) Formulation Example 4 water dispersible granule (water dispersible granule)
化合物No. Compound No. 4 40部化合物No. 4 40 parts of Compound No. d 35部ハイテノールNE−15 5部(アニオン性界面活性剤:第一工業製薬(株)商品名) d 35 parts high tenor NE-15 5 parts (an anionic surfactant: Dai-ichi Kogyo Seiyaku Co., Ltd., trade name)
バニレックスN 10部(アニオン性界面活性剤:日本製紙(株)商品名) VANILLEX N 10 parts (an anionic surfactant: Nippon Paper Industries trade name)
カープレックス#80D 10部(合成含水珪酸:塩野義製薬(株)商品名) Carplex # 80D 10 parts (synthetic hydrous silicate: Shionogi & Co., Ltd., trade name)
以上を均一に混合粉砕した後、少量の水を加えて攪拌混合し、押出式造粒機で造粒し、乾燥して顆粒水和剤とする。 They were uniformly mixed and ground to above are stirred to mix with addition of a small amount of water, granulated by an extrusion granulator and dried to a water dispersible granule.
【0079】 [0079]
〔配合例5〕粒 剤(granule) Formulation Example 5 Granules (granule)
化合物No. Compound No. 5 3部化合物No. 5 3 parts of Compound No. e 2部ベントナイト 50部タルク 45部以上を均一に混合粉砕した後、少量の水を加えて攪拌混合し、押出式造粒機で造粒し、乾燥して粒剤とする。 Were uniformly mixed and pulverized to e 2 parts Bentonite 50 parts Talc 45 parts The above are stirred to mix with addition of a small amount of water, granulated by an extrusion granulator and dried to obtain granules.
【0080】 [0080]
〔配合例6〕粉 剤(dustable powder) [Formulation Example 6] Powder agent (dustable powder)
化合物No. Compound No. 6 2部化合物No. 6 2 parts of Compound No. f 1部カープレックス#80D 0.5部(ホワイトカーボン:塩野義製薬(株)商品名) f 1 part Carplex # 80D 0.5 parts (white carbon: Shionogi & Co., Ltd., trade name)
カオリナイト 95部リン酸ジイソプロピル 1.5部以上を均一に混合粉砕して粉剤とする。 A dust uniformly mixed and ground to 1.5 parts Kaolinite 95 parts diisopropyl.
【0081】 [0081]
使用に際しては上記水和剤、乳剤、フロアブル剤、粒状水和剤は水で50〜20000倍に希釈して有効成分が1ヘクタール(ha)当たり0.005〜50kgになるように散布する。 The wettable powder is in use, emulsions, flowables, granules wettable powder is sprayed as an active ingredient were diluted from 50 to 20,000-fold with water is per hectare (ha) from 0.005.
【0082】 [0082]
【実施例】 【Example】
以下に、本発明の式(1)で表されるアクリロニトリル化合物の合成例を具体的に示す。 Hereinafter, specific synthesis examples acrylonitrile compounds represented by the formula (1) of the present invention.
【0083】 [0083]
〔合成例1〕2−(4−クロロフェニル)−3−(1,3、4−トリメチルピラゾール−5−イル)−3−ヒドロキシ−アクリロニトリル(化合物No.1)の合成4−クロロフェニルアセトニトリル5.0gと1,3、4−トリメチル−5−カルボニルクロリド5.69gをテトラヒドロフラン60mlに溶解し、氷冷下にてカリウム tert−ブトキサイド8.13gを加えた。 Synthesis Example 1 2- (4-chlorophenyl) -3- (5-1,3,4-trimethyl pyrazole yl) -3-hydroxy - Synthesis of acrylonitrile (Compound No.1) 4-chlorophenyl acetonitrile 5.0g When the 1,3,4-trimethyl-5-carbonyl chloride 5.69g was dissolved in tetrahydrofuran 60 ml, was added potassium tert- butoxide 8.13g under ice-cooling. 室温で4時間撹拌した後、減圧下にて溶媒を留去し、残査に希塩酸を加えて酸性にした後、酢酸エチルで抽出、水洗、無水硫酸ナトリウムで乾燥後、減圧下で溶媒を留去し、析出した結晶をジイソプロピルエーテルで洗浄する事で標記目的化合物7.43gを得た。 After stirring for 4 hours at room temperature, the solvent was removed under reduced pressure, was acidified with dilute hydrochloric acid to the residue, extracted with ethyl acetate, washed with water, dried over anhydrous sodium sulfate, the solvent under reduced pressure distillate removed by to, and the precipitated crystals to give the title object compound 7.43g by washing with diisopropyl ether. 融点:219−220℃。 Melting point: 219-220 ℃.
【0084】 [0084]
〔合成例2〕2−(4−クロロフェニル)−3−ピバロイルオキシ−3−(1,3、4−トリメチルピラゾール−5−イル)アクリロニトリル(化合物No.2)の合成2−(4−クロロフェニル)−3−(1,3、4−トリメチルピラゾール−5−イル)−3−ヒドロキシ−アクリロニトリル1.5gをテトラヒドロフラン20mlに溶解し、カリウム tert−ブトキサイド0.64gを加えた後、ピバロイルクロリド0.75gを滴下し、室温で一晩撹拌した。 Synthesis Example 2 2- (4-chlorophenyl) -3-pivaloyloxy-3- (5-1,3,4-trimethyl pyrazole yl) Synthesis of 2- (4-chlorophenyl) acrylonitrile (Compound No.2) - 3- (5-1,3,4-trimethyl pyrazole yl) -3-hydroxy - acrylonitrile 1.5g was dissolved in tetrahydrofuran 20 ml, was added to potassium tert- butoxide 0.64 g, pivaloyl chloride 0. was added dropwise 75 g, it was stirred overnight at room temperature. 反応混合物を水中に注ぎ酢酸エチルで抽出、水洗、無水硫酸ナトリウムで乾燥後、減圧下で溶媒を留去して得られた油状物をジイソプロピルエーテルから結晶化する事で、標記目的化合物1.37gを得た。 The reaction mixture was extracted with ethyl acetate poured into water, washed with water, dried over anhydrous sodium sulfate, by crystallizing the oily substance obtained by distilling off the solvent under reduced pressure from diisopropyl ether, the title object compound 1.37g It was obtained. 融点:148℃。 Mp: 148 ° C..
【0085】 [0085]
上記合成例に準じて、前記の第1表に記載した式(1)で表されるアクリロニトリル化合物を合成した。 According to the above synthesis example was synthesized acrylonitrile compound represented by the formula (1) described in Table 1 above. 合成した化合物の物性を第4表に記載した。 The physical properties of the synthesized compounds are listed in Table 4.
【0086】 [0086]
【表4】 [Table 4]
【0087】 [0087]
次に、本発明の有用性を明らかにするため、効力試験例を具体的に以下に示す。 Then, to clarify the usefulness of the present invention, specifically the following efficacy test examples.
【0088】 [0088]
〔試験例1〕 ミカンサビダニに対する効力試験上記の第4表に記載された化合物と、前記の第3表に記載された化合物を、各々10%乳剤(化合物によっては25%水和剤)に製剤し、その製剤を展着剤の入った水で希釈して、所定濃度の薬液を調製した。 Formulations and compounds described in Table 4 Efficacy Test The relative Test Example 1 tangerine rust mite, the compounds described in Table 3 above, each 10% emulsion (25% Wettable powders by compounds) and, it was diluted with water containing the formulation exhibition of wear agent, to prepare a predetermined concentration of the chemical solution. 次に、ミカンサビダニが寄生したみかん果実から、寄生部の果皮を切りとって小さな切片(5mm×5mm程度)を作り、クリスタルバイオレットを入れた0.3%寒天溶液を用いてシャーレ内に固定したのち、実体顕微鏡下で切片上の全てのサビダニ幼虫および必要な場合は一部の成虫を除去し、一切片あたりのサビダニ成虫数が20〜30頭となるように調整した。 Next, the mandarin fruit tangerine rust mite is parasitic, cut and peel the parasitic section makes small sections (about 5 mm × 5 mm), then fixed to the dish with 0.3% agar solution containing the crystal violet If all the sections of rust mite larvae and required under stereomicroscope to remove a portion of the adult, was adjusted to rust mite number adults per any piece is 20 to 30 animals. こうして準備した供試切片に所定濃度の薬液を各5ml散布処理し、風乾後に孔のあいた蓋をして25℃の恒温室に収容した。 Thus the chemical with a predetermined concentration was each 5ml sprayed preparation was subjected 試切 pieces were housed in a constant temperature chamber of to 25 ° C. a lid apertured after air drying. 4日後の死虫数を調査し、下記の計算式から死虫率を算出した。 The number of dead insects was investigated after 4 days, was calculated the mortality from the following calculation formula. 尚、試験は2区制で行なった。 The test was carried out in the 2nd district system.
【0089】 [0089]
死虫率(%)=死虫数/供試虫数×100 Mortality (%) = dead insects / number tested insects Number × 100
各薬液濃度に対する死虫率から、プロビット法に基づいて半数致死濃度(LC 50値)を求めた。 From the mortality for each chemical concentration, it was determined median lethal concentration (LC 50 value) based on probit method. 更に共力効果(相乗効果)の程度を判定するために通常用いられているSun & Johnson法(ジャーナル オブ エコノミック エントモロジー誌、1960年、第55巻、887頁)の式を用いて、共力係数を計算した。 Further synergistic effect Sun & Johnson method commonly used to determine the extent of (synergy) (Journal of Economic entomopox biology magazine, 1960, Vol. 55, 887 pp) using the formula, synergists the coefficient was calculated. 共力係数は次に示す式で表される。 Synergistic factor is expressed by the following formula.
【0090】 [0090]
共力係数=混合剤の実際の毒性指数/混合剤の理論的毒性指数×100 Theoretical toxicity index × 100 of the actual toxicity index / admixture synergistic factor = admixtures
但し、 However,
混合剤の実際の毒性指数:[A]のLC 50 /[A][B]混合剤のLC 50 ×100 Actual toxicity index of admixtures: LC 50 × 100 of LC 50 / [A] [B ] admixture [A]
混合剤の理論的毒性指数:([A]の毒性指数×[A][B]混合剤の中の[A]の%+[B]の毒性指数×[A][B]混合剤中の[B]の%)/100 Admixtures Theoretical toxicity index (toxicity index × the [A] [A] [B] in admixture [A] of the% + [B] toxicity index × [A] [B] in admixture of % of [B]) / 100
[A]:式(1)で表されるアクリロニトリル化合物[B]:化合物群Aから選ばれる化合物%:[A]と[B]の総重量に対する重量百分率[A]の毒性指数:100 [A]: an acrylonitrile compound represented by the formula (1) [B]: Compound% selected from the group of compounds A: Toxicity index of [A] and the weight percentage of the total weight of the [B] [A]: 100
[B]の毒性指数:([A]のLC 50 /[B]のLC 50 )×100 Toxicity index of [B]: (LC 50 of LC 50 / [B] of [A]) × 100
である。 It is.
【0091】 [0091]
この共力係数の値が100より大きいほど相乗効果が高く、100に等しいときは相加的効果、100より小さくなるほど拮抗効果が高くなる、ということを示す。 The value of the co-force coefficient higher synergistic effect larger than 100, additive effect, is small becomes higher antagonizing effect than 100 higher when equal to 100 indicates that.
【0092】 [0092]
試験の結果、下記の化合物の組合わせにおいて、共力係数が100よりも大きくなった。 Results of the test, the combination of the following compounds, synergists coefficient is greater than 100.
【0093】 [0093]
共力係数が100よりも大きくなった化合物の組合せ:1+v,1+df,1+dg,1+gh,1+gk,1+gl,1+gp,1+gr,1+gt,1+gy,1+gz,1+ha,1+hd,1+hg,1+ht,1+hu,1+il,1+iq,1+jy,1+kl,1+kp,1+ly,2+v,2+df,2+dg,2+gh,2+gk,2+gl,2+gp,2+gr,2+gt,2+gy,2+gz,2+ha,2+hd,2+hg,2+ht,2+hu,2+il,2+iq,2+jy,2+kl,2+kp,2+ly,3+v,3+df,3+dg,3+gh,3+gk,3+gl,3+gp,3+gr,3+gt,3+gy,3+gz,3+ha,3+hd,3+hg,3+ht,3+hu,3+il,3+iq,3 Combination of compounds synergistic factor is greater than 100: 1 + v, 1 + df, 1 + dg, 1 + gh, 1 + gk, 1 + gl, 1 + gp, 1 + gr, 1 + gt, 1 + gy, 1 + gz, 1 + ha, 1 + hd, 1 + hg, 1 + ht, 1 + hu, 1 + il, 1 + iq, 1 + jy, 1 + kl, 1 + kp, 1 + ly, 2 + v, 2 + df, 2 + dg, 2 + gh, 2 + gk, 2 + gl, 2 + gp, 2 + gr, 2 + gt, 2 + gy, 2 + gz, 2 + ha, 2 + hd, 2 + hg, 2 + ht, 2 + hu, 2 + il, 2 + iq, 2 + jy, 2 + kl, 2 + kp, 2 + ly, 3 + v, 3 + df, 3 + dg, 3 + gh, 3 + gk, 3 + gl, 3 + gp, 3 + gr, 3 + gt, 3 + gy, 3 + gz, 3 + ha, 3 + hd, 3 + hg, 3 + ht, 3 + hu, 3 + il, 3 + iq, 3 jy,3+kl,3+kp,3+ly,4+v,4+df,4+dg,4+gh,4+gk,4+gl,4+gp,4+gr,4+gt,4+gy,4+gz,4+ha,4+hd,4+hg,4+ht,4+hu,4+il,4+iq,4+jy,4+kl,4+kp,4+ly,5+v,5+df,5+dg,5+gh,5+gk,5+gl,5+gp,5+gr,5+gt,5+gy,5+gz,5+ha,5+hd,5+hg,5+ht,5+hu,5+il,5+iq,5+jy,5+kl,5+kp,5+ly,6+v,6+df,6+dg,6+gh,6+gk,6+gl,6+gp,6+gr,6+gt,6+gy,6+gz,6+ha,6+hd,6+hg,6+ht,6+hu,6+il,6+iq,6+jy,6+ jy, 3 + kl, 3 + kp, 3 + ly, 4 + v, 4 + df, 4 + dg, 4 + gh, 4 + gk, 4 + gl, 4 + gp, 4 + gr, 4 + gt, 4 + gy, 4 + gz, 4 + ha, 4 + hd, 4 + hg, 4 + ht, 4 + hu, 4 + il, 4 + iq, 4 + jy, 4 + kl, 4 + kp, 4 + ly, 5 + v, 5 + df, 5 + dg, 5 + gh, 5 + gk, 5 + gl, 5 + gp, 5 + gr, 5 + gt, 5 + gy, 5 + gz, 5 + ha, 5 + hd, 5 + hg, 5 + ht, 5 + hu, 5 + il, 5 + iq, 5 + jy, 5 + kl, 5 + kp, 5 + ly, 6 + v, 6 + df, 6 + dg, 6 + gh, 6 + gk, 6 + gl, 6 + gp, 6 + gr, 6 + gt, 6 + gy, 6 + gz, 6 + ha, 6 + hd, 6 + hg, 6 + ht, 6 + hu, 6 + il, 6 + iq, 6 + jy, 6 + l,6+kp,6+ly,7+v,7+df,7+dg,7+gh,7+gk,7+gl,7+gp,7+gr,7+gt,7+gy,7+gz,7+ha,7+hd,7+hg,7+ht,7+hu,7+il,7+iq,7+jy,7+kl,7+kp,7+ly,8+v,8+df,8+dg,8+gh,8+gk,8+gl,8+gp,8+gr,8+gt,8+gy,8+gz,8+ha,8+hd,8+hg,8+ht,8+hu,8+il,8+iq,8+jy,8+kl,8+kp,8+ly,9+v,9+df,9+dg,9+gh,9+gk,9+gl,9+gp,9+gr,9+gt,9+gy,9+gz,9+ha,9+hd,9+hg,9+ht,9+hu,9+il,9+iq,9+jy,9+kl,9+kp l, 6 + kp, 6 + ly, 7 + v, 7 + df, 7 + dg, 7 + gh, 7 + gk, 7 + gl, 7 + gp, 7 + gr, 7 + gt, 7 + gy, 7 + gz, 7 + ha, 7 + hd, 7 + hg, 7 + ht, 7 + hu, 7 + il, 7 + iq, 7 + jy, 7 + kl, 7 + kp, 7 + ly, 8 + v, 8 + df, 8 + dg, 8 + gh, 8 + gk, 8 + gl, 8 + gp, 8 + gr, 8 + gt, 8 + gy, 8 + gz, 8 + ha, 8 + hd, 8 + hg, 8 + ht, 8 + hu, 8 + il, 8 + iq, 8 + jy, 8 + kl, 8 + kp, 8 + ly, 9 + v, 9 + df, 9 + dg, 9 + gh, 9 + gk, 9 + gl, 9 + gp, 9 + gr, 9 + gt, 9 + gy, 9 + gz, 9 + ha, 9 + hd, 9 + hg, 9 + ht, 9 + hu, 9 + il, 9 + iq, 9 + jy, 9 + kl, 9 + kp ,9+ly,10+v,10+df,10+dg,10+gh,10+gk,10+gl,10+gp,10+gr,10+gt,10+gy,10+gz,10+ha,10+hd,10+hg,10+ht,10+hu,10+il,10+iq,10+jy,10+kl,10+kp,10+ly,11+v,11+df,11+dg,11+gh,11+gk,11+gl,11+gp,11+gr,11+gt,11+gy,11+gz,11+ha,11+hd,11+hg,11+ht,11+hu,11+il,11+iq,11+jy,11+kl,11+kp,11+ly,12+v,12+df,12+dg,12+gh,12+gk,12+gl,12+gp,12+gr,12+gt,12+gy,12+gz, , 9 + ly, 10 + v, 10 + df, 10 + dg, 10 + gh, 10 + gk, 10 + gl, 10 + gp, 10 + gr, 10 + gt, 10 + gy, 10 + gz, 10 + ha, 10 + hd, 10 + hg, 10 + ht, 10 + hu, 10 + il, 10 + iq, 10 + jy, 10 + kl, 10 + kp, 10 + ly, 11 + v, 11 + df , 11 + dg, 11 + gh, 11 + gk, 11 + gl, 11 + gp, 11 + gr, 11 + gt, 11 + gy, 11 + gz, 11 + ha, 11 + hd, 11 + hg, 11 + ht, 11 + hu, 11 + il, 11 + iq, 11 + jy, 11 + kl, 11 + kp, 11 + ly, 12 + v, 12 + df, 12 + dg, 12 + gh, 12 + gk , 12 + gl, 12 + gp, 12 + gr, 12 + gt, 12 + gy, 12 + gz, 2+ha,12+hd,12+hg,12+ht,12+hu,12+il,12+iq,12+jy,12+kl,12+kp,12+ly,13+v,13+df,13+dg,13+gh,13+gk,13+gl,13+gp,13+gr,13+gt,13+gy,13+gz,13+ha,13+hd,13+hg,13+ht,13+hu,13+il,13+iq,13+jy,13+kl,13+kp,13+ly,14+v,14+df,14+dg,14+gh,14+gk,14+gl,14+gp,14+gr,14+gt,14+gy,14+gz,14+ha,14+hd,14+hg,14+ht,14+hu,14+il,14+iq,14+jy,14+kl,14+kp,14+ly,15+v, 2 + ha, 12 + hd, 12 + hg, 12 + ht, 12 + hu, 12 + il, 12 + iq, 12 + jy, 12 + kl, 12 + kp, 12 + ly, 13 + v, 13 + df, 13 + dg, 13 + gh, 13 + gk, 13 + gl, 13 + gp, 13 + gr, 13 + gt, 13 + gy, 13 + gz, 13 + ha, 13 + hd, 13 + hg, 13 + ht, 13 + hu, 13 + il, 13 + iq, 13 + jy, 13 + kl, 13 + kp, 13 + ly, 14 + v, 14 + df, 14 + dg, 14 + gh, 14 + gk, 14 + gl, 14 + gp, 14 + gr, 14 + gt, 14 + gy, 14 + gz, 14 + ha, 14 + hd, 14 + hg, 14 + ht, 14 + hu, 14 + il, 14 + iq, 14 + jy, 14 + kl, 14 + kp, 14 + ly, 15 + v, 5+df,15+dg,15+gh,15+gk,15+gl,15+gp,15+gr,15+gt,15+gy,15+gz,15+ha,15+hd,15+hg,15+ht,15+hu,15+il,15+iq,15+jy,15+kl,15+kp,15+ly,16+v,16+df,16+dg,16+gh,16+gk,16+gl,16+gp,16+gr,16+gt,16+gy,16+gz,16+ha,16+hd,16+hg,16+ht,16+hu,16+il,16+iq,16+jy,16+kl,16+kp,16+ly,17+v,17+df,17+dg,17+gh,17+gk,17+gl,17+gp,17+gr,17+gt,17+gy,17+gz,17+ha,17+hd, 5 + df, 15 + dg, 15 + gh, 15 + gk, 15 + gl, 15 + gp, 15 + gr, 15 + gt, 15 + gy, 15 + gz, 15 + ha, 15 + hd, 15 + hg, 15 + ht, 15 + hu, 15 + il, 15 + iq, 15 + jy, 15 + kl, 15 + kp, 15 + ly, 16 + v, 16 + df, 16 + dg, 16 + gh, 16 + gk, 16 + gl, 16 + gp, 16 + gr, 16 + gt, 16 + gy, 16 + gz, 16 + ha, 16 + hd, 16 + hg, 16 + ht, 16 + hu, 16 + il, 16 + iq, 16 + jy, 16 + kl, 16 + kp, 16 + ly, 17 + v, 17 + df, 17 + dg, 17 + gh, 17 + gk, 17 + gl, 17 + gp, 17 + gr, 17 + gt, 17 + gy, 17 + gz, 17 + ha, 17 + hd, 17+hg,17+ht,17+hu,17+il,17+iq,17+jy,17+kl,17+kp,17+ly,18+v,18+df,18+dg,18+gh,18+gk,18+gl,18+gp,18+gr,18+gt,18+gy,18+gz,18+ha,18+hd,18+hg,18+ht,18+hu,18+il,18+iq,18+jy,18+kl,18+kp,18+ly,19+v,19+df,19+dg,19+gh,19+gk,19+gl,19+gp,19+gr,19+gt,19+gy,19+gz,19+ha,19+hd,19+hg,19+ht,19+hu,19+il,19+iq,19+jy,19+kl,19+kp,19+ly,20+v,20+df,20+dg, 17 + hg, 17 + ht, 17 + hu, 17 + il, 17 + iq, 17 + jy, 17 + kl, 17 + kp, 17 + ly, 18 + v, 18 + df, 18 + dg, 18 + gh, 18 + gk, 18 + gl, 18 + gp, 18 + gr, 18 + gt, 18 + gy, 18 + gz, 18 + ha, 18 + hd, 18 + hg, 18 + ht, 18 + hu, 18 + il, 18 + iq, 18 + jy, 18 + kl, 18 + kp, 18 + ly, 19 + v, 19 + df, 19 + dg, 19 + gh, 19 + gk, 19 + gl, 19 + gp, 19 + gr, 19 + gt, 19 + gy, 19 + gz, 19 + ha, 19 + hd, 19 + hg, 19 + ht, 19 + hu, 19 + il, 19 + iq, 19 + jy, 19 + kl, 19 + kp, 19 + ly, 20 + v, 20 + df, 20 + dg, 0+gh,20+gk,20+gl,20+gp,20+gr,20+gt,20+gy,20+gz,20+ha,20+hd,20+hg,20+ht,20+hu,20+il,20+iq,20+jy,20+kl,20+kp,20+ly,21+v,21+df,21+dg,21+gh,21+gk,21+gl,21+gp,21+gr,21+gt,21+gy,21+gz,21+ha,21+hd,21+hg,21+ht,21+hu,21+il,21+iq,21+jy,21+kl,21+kp,21+ly,22+v,22+df,22+dg,22+gh,22+gk,22+gl,22+gp,22+gr,22+gt,22+gy,22+gz,22+ha,22+hd,22+hg,22+ht 0 + gh, 20 + gk, 20 + gl, 20 + gp, 20 + gr, 20 + gt, 20 + gy, 20 + gz, 20 + ha, 20 + hd, 20 + hg, 20 + ht, 20 + hu, 20 + il, 20 + iq, 20 + jy, 20 + kl, 20 + kp, 20 + ly, 21 + v, 21 + df, 21 + dg, 21 + gh, 21 + gk, 21 + gl, 21 + gp, 21 + gr, 21 + gt, 21 + gy, 21 + gz, 21 + ha, 21 + hd, 21 + hg, 21 + ht, 21 + hu, 21 + il, 21 + iq, 21 + jy, 21 + kl, 21 + kp, 21 + ly, 22 + v, 22 + df, 22 + dg, 22 + gh, 22 + gk, 22 + gl, 22 + gp, 22 + gr, 22 + gt, 22 + gy, 22 + gz, 22 + ha, 22 + hd, 22 + hg, 22 + ht 22+hu,22+il,22+iq,22+jy,22+kl,22+kp,22+ly,23+v,23+df,23+dg,23+gh,23+gk,23+gl,23+gp,23+gr,23+gt,23+gy,23+gz,23+ha,23+hd,23+hg,23+ht,23+hu,23+il,23+iq,23+jy,23+kl,23+kp,23+ly,24+v,24+df,24+dg,24+gh,24+gk,24+gl,24+gp,24+gr,24+gt,24+gy,24+gz,24+ha,24+hd,24+hg,24+ht,24+hu,24+il,24+iq,24+jy,24+kl,24+kp,24+ly,25+v,25+df,25+dg,25+gh,25+gk, 22 + hu, 22 + il, 22 + iq, 22 + jy, 22 + kl, 22 + kp, 22 + ly, 23 + v, 23 + df, 23 + dg, 23 + gh, 23 + gk, 23 + gl, 23 + gp, 23 + gr, 23 + gt, 23 + gy, 23 + gz, 23 + ha, 23 + hd, 23 + hg, 23 + ht, 23 + hu, 23 + il, 23 + iq, 23 + jy, 23 + kl, 23 + kp, 23 + ly, 24 + v, 24 + df, 24 + dg, 24 + gh, 24 + gk, 24 + gl, 24 + gp, 24 + gr, 24 + gt, 24 + gy, 24 + gz, 24 + ha, 24 + hd, 24 + hg, 24 + ht, 24 + hu, 24 + il, 24 + iq, 24 + jy, 24 + kl, 24 + kp, 24 + ly, 25 + v, 25 + df, 25 + dg, 25 + gh, 25 + gk, 25+gl,25+gp,25+gr,25+gt,25+gy,25+gz,25+ha,25+hd,25+hg,25+ht,25+hu,25+il,25+iq,25+jy,25+kl,25+kp,25+ly,26+v,26+df,26+dg,26+gh,26+gk,26+gl,26+gp,26+gr,26+gt,26+gy,26+gz,26+ha,26+hd,26+hg,26+ht,26+hu,26+il,26+iq,26+jy,26+kl,26+kp,26+ly,27+v,27+df,27+dg,27+gh,27+gk,27+gl,27+gp,27+gr,27+gt,27+gy,27+gz,27+ha,27+hd,27+hg,27+ht,27+hu,27+il 25 + gl, 25 + gp, 25 + gr, 25 + gt, 25 + gy, 25 + gz, 25 + ha, 25 + hd, 25 + hg, 25 + ht, 25 + hu, 25 + il, 25 + iq, 25 + jy, 25 + kl, 25 + kp, 25 + ly, 26 + v, 26 + df, 26 + dg, 26 + gh, 26 + gk, 26 + gl, 26 + gp, 26 + gr, 26 + gt, 26 + gy, 26 + gz, 26 + ha, 26 + hd, 26 + hg, 26 + ht, 26 + hu, 26 + il, 26 + iq, 26 + jy, 26 + kl, 26 + kp, 26 + ly, 27 + v, 27 + df, 27 + dg, 27 + gh, 27 + gk, 27 + gl, 27 + gp, 27 + gr, 27 + gt, 27 + gy, 27 + gz, 27 + ha, 27 + hd, 27 + hg, 27 + ht, 27 + hu, 27 + il 27+iq,27+jy,27+kl,27+kp,27+ly,28+v,28+df,28+dg,28+gh,28+gk,28+gl,28+gp,28+gr,28+gt,28+gy,28+gz,28+ha,28+hd,28+hg,28+ht,28+hu,28+il,28+iq,28+jy,28+kl,28+kp,28+ly,29+v,29+df,29+dg,29+gh,29+gk,29+gl,29+gp,29+gr,29+gt,29+gy,29+gz,29+ha,29+hd,29+hg,29+ht,29+hu,29+il,29+iq,29+jy,29+kl,29+kp,29+ly,30+v,30+df,30+dg,30+gh,30+gk,30+gl,30+gp 27 + iq, 27 + jy, 27 + kl, 27 + kp, 27 + ly, 28 + v, 28 + df, 28 + dg, 28 + gh, 28 + gk, 28 + gl, 28 + gp, 28 + gr, 28 + gt, 28 + gy, 28 + gz, 28 + ha, 28 + hd, 28 + hg, 28 + ht, 28 + hu, 28 + il, 28 + iq, 28 + jy, 28 + kl, 28 + kp, 28 + ly, 29 + v, 29 + df, 29 + dg, 29 + gh, 29 + gk, 29 + gl, 29 + gp, 29 + gr, 29 + gt, 29 + gy, 29 + gz, 29 + ha, 29 + hd, 29 + hg, 29 + ht, 29 + hu, 29 + il, 29 + iq, 29 + jy, 29 + kl, 29 + kp, 29 + ly, 30 + v, 30 + df, 30 + dg, 30 + gh, 30 + gk, 30 + gl, 30 + gp 30+gr,30+gt,30+gy,30+gz,30+ha,30+hd,30+hg,30+ht,30+hu,30+il,30+iq,30+jy,30+kl,30+kp,30+ly,31+v,31+df,31+dg,31+gh,31+gk,31+gl,31+gp,31+gr,31+gt,31+gy,31+gz,31+ha,31+hd,31+hg,31+ht,31+hu,31+il,31+iq,31+jy,31+kl,31+kp,31+ly,32+v,32+df,32+dg,32+gh,32+gk,32+gl,32+gp,32+gr,32+gt,32+gy,32+gz,32+ha,32+hd,32+hg,32+ht,32+hu,32+il,32+iq,32+jy 30 + gr, 30 + gt, 30 + gy, 30 + gz, 30 + ha, 30 + hd, 30 + hg, 30 + ht, 30 + hu, 30 + il, 30 + iq, 30 + jy, 30 + kl, 30 + kp, 30 + ly, 31 + v, 31 + df, 31 + dg, 31 + gh, 31 + gk, 31 + gl, 31 + gp, 31 + gr, 31 + gt, 31 + gy, 31 + gz, 31 + ha, 31 + hd, 31 + hg, 31 + ht, 31 + hu, 31 + il, 31 + iq, 31 + jy, 31 + kl, 31 + kp, 31 + ly, 32 + v, 32 + df, 32 + dg, 32 + gh, 32 + gk, 32 + gl, 32 + gp, 32 + gr, 32 + gt, 32 + gy, 32 + gz, 32 + ha, 32 + hd, 32 + hg, 32 + ht, 32 + hu, 32 + il, 32 + iq, 32 + jy ,32+kl,32+kp,32+ly,33+v,33+df,33+dg,33+gh,33+gk,33+gl,33+gp,33+gr,33+gt,33+gy,33+gz,33+ha,33+hd,33+hg,33+ht,33+hu,33+il,33+iq,33+jy,33+kl,33+kp,33+ly,34+v,34+df,34+dg,34+gh,34+gk,34+gl,34+gp,34+gr,34+gt,34+gy,34+gz,34+ha,34+hd,34+hg,34+ht,34+hu,34+il,34+iq,34+jy,34+kl,34+kp,34+ly,35+v,35+df,35+dg,35+gh,35+gk,35+gl,35+gp,35+gr,35+gt , 32 + kl, 32 + kp, 32 + ly, 33 + v, 33 + df, 33 + dg, 33 + gh, 33 + gk, 33 + gl, 33 + gp, 33 + gr, 33 + gt, 33 + gy, 33 + gz, 33 + ha, 33 + hd, 33 + hg, 33 + ht, 33 + hu, 33 + il, 33 + iq, 33 + jy, 33 + kl, 33 + kp, 33 + ly , 34 + v, 34 + df, 34 + dg, 34 + gh, 34 + gk, 34 + gl, 34 + gp, 34 + gr, 34 + gt, 34 + gy, 34 + gz, 34 + ha, 34 + hd, 34 + hg, 34 + ht, 34 + hu, 34 + il, 34 + iq, 34 + jy, 34 + kl, 34 + kp, 34 + ly, 35 + v, 35 + df, 35 + dg , 35 + gh, 35 + gk, 35 + gl, 35 + gp, 35 + gr, 35 + gt 35+gy,35+gz,35+ha,35+hd,35+hg,35+ht,35+hu,35+il,35+iq,35+jy,35+kl,35+kp,35+ly,36+v,36+df,36+dg,36+gh,36+gk,36+gl,36+gp,36+gr,36+gt,36+gy,36+gz,36+ha,36+hd,36+hg,36+ht,36+hu,36+il,36+iq,36+jy,36+kl,36+kp,36+ly,37+v,37+df,37+dg,37+gh,37+gk,37+gl,37+gp,37+gr,37+gt,37+gy,37+gz,37+ha,37+hd,37+hg,37+ht,37+hu,37+il,37+iq,37+jy,37+kl,37+k 35 + gy, 35 + gz, 35 + ha, 35 + hd, 35 + hg, 35 + ht, 35 + hu, 35 + il, 35 + iq, 35 + jy, 35 + kl, 35 + kp, 35 + ly, 36 + v, 36 + df, 36 + dg, 36 + gh, 36 + gk, 36 + gl, 36 + gp, 36 + gr, 36 + gt, 36 + gy, 36 + gz, 36 + ha, 36 + hd, 36 + hg, 36 + ht, 36 + hu, 36 + il, 36 + iq, 36 + jy, 36 + kl, 36 + kp, 36 + ly, 37 + v, 37 + df, 37 + dg, 37 + gh, 37 + gk, 37 + gl, 37 + gp, 37 + gr, 37 + gt, 37 + gy, 37 + gz, 37 + ha, 37 + hd, 37 + hg, 37 + ht, 37 + hu, 37 + il, 37 + iq, 37 + jy, 37 + kl, 37 + k ,37+ly,38+v,38+df,38+dg,38+gh,38+gk,38+gl,38+gp,38+gr,38+gt,38+gy,38+gz,38+ha,38+hd,38+hg,38+ht,38+hu,38+il,38+iq,38+jy,38+kl,38+kp,38+ly,39+v,39+df,39+dg,39+gh,39+gk,39+gl,39+gp,39+gr,39+gt,39+gy,39+gz,39+ha,39+hd,39+hg,39+ht,39+hu,39+il,39+iq,39+jy,39+kl,39+kp,39+ly,40+v,40+df,40+dg,40+gh,40+gk,40+gl,40+gp,40+gr,40+gt,40+gy,40+gz , 37 + ly, 38 + v, 38 + df, 38 + dg, 38 + gh, 38 + gk, 38 + gl, 38 + gp, 38 + gr, 38 + gt, 38 + gy, 38 + gz, 38 + ha, 38 + hd, 38 + hg, 38 + ht, 38 + hu, 38 + il, 38 + iq, 38 + jy, 38 + kl, 38 + kp, 38 + ly, 39 + v, 39 + df , 39 + dg, 39 + gh, 39 + gk, 39 + gl, 39 + gp, 39 + gr, 39 + gt, 39 + gy, 39 + gz, 39 + ha, 39 + hd, 39 + hg, 39 + ht, 39 + hu, 39 + il, 39 + iq, 39 + jy, 39 + kl, 39 + kp, 39 + ly, 40 + v, 40 + df, 40 + dg, 40 + gh, 40 + gk , 40 + gl, 40 + gp, 40 + gr, 40 + gt, 40 + gy, 40 + gz ,40+ha,40+hd,40+hg,40+ht,40+hu,40+il,40+iq,40+jy,40+kl,40+kp,40+ly,41+v,41+df,41+dg,41+gh,41+gk,41+gl,41+gp,41+gr,41+gt,41+gy,41+gz,41+ha,41+hd,41+hg,41+ht,41+hu,41+il,41+iq,41+jy,41+kl,41+kp,41+ly,42+v,42+df,42+dg,42+gh,42+gk,42+gl,42+gp,42+gr,42+gt,42+gy,42+gz,42+ha,42+hd,42+hg,42+ht,42+hu,42+il,42+iq,42+jy,42+kl,42+kp,42+ly,43+v , 40 + ha, 40 + hd, 40 + hg, 40 + ht, 40 + hu, 40 + il, 40 + iq, 40 + jy, 40 + kl, 40 + kp, 40 + ly, 41 + v, 41 + df, 41 + dg, 41 + gh, 41 + gk, 41 + gl, 41 + gp, 41 + gr, 41 + gt, 41 + gy, 41 + gz, 41 + ha, 41 + hd, 41 + hg , 41 + ht, 41 + hu, 41 + il, 41 + iq, 41 + jy, 41 + kl, 41 + kp, 41 + ly, 42 + v, 42 + df, 42 + dg, 42 + gh, 42 + gk, 42 ​​+ gl, 42 + gp, 42 + gr, 42 + gt, 42 + gy, 42 + gz, 42 + ha, 42 + hd, 42 + hg, 42 + ht, 42 + hu, 42 + il , 42 + iq, 42 + jy, 42 + kl, 42 + kp, 42 + ly, 43 + v 43+df,43+dg,43+gh,43+gk,43+gl,43+gp,43+gr,43+gt,43+gy,43+gz,43+ha,43+hd,43+hg,43+ht,43+hu,43+il,43+iq,43+jy,43+kl,43+kp,43+ly. 43 + df, 43 + dg, 43 + gh, 43 + gk, 43 + gl, 43 + gp, 43 + gr, 43 + gt, 43 + gy, 43 + gz, 43 + ha, 43 + hd, 43 + hg, 43 + ht, 43 + hu, 43 + il, 43 + iq, 43 + jy, 43 + kl, 43 + kp, 43 + ly.
【0094】 [0094]
【発明の効果】 【Effect of the invention】
本発明組成物及び本発明方法は、各種病害虫に対して優れた相乗的防除効果を奏する。 The present invention compositions and method of the present invention exhibits an excellent synergistic pesticidal effect against various pests.

Claims (6)

  1. 以下の式(1)で表されるアクリロニトリル化合物の1種以上と、以下の化合物群Aより選ばれる化合物の1種以上を含有する殺虫、殺ダニ、殺線虫、殺菌又は殺バクテリア組成物。 Insecticides containing one or more of the following formulas (1) and one or more acrylonitrile compounds represented by compounds selected from the following compound group A, acaricidal, nematicidal, fungicidal or bactericidal composition.
    式(1): Equation (1):
    [式中、 Aは、 [In the formula, A,
    であり、 It is in,
    Bは、H、CR 、CHR 、C 〜C ハロアルキル、テトラヒドロピラニル、Si(CH 、SO Re、SO NHRb、SO NRaRb、C(S)NHRb、C(S)NRaRb、C(O)Rf、P(O)RgRh、P(S)RgRh、アルカリ金属、アルカリ土類金属またはNHRiRjRkであり、 B is, H, CR 1 R 2 R 3, CHR 1 R 2, C 1 ~C 4 haloalkyl, tetrahydropyranyl, Si (CH 3) 3, SO 2 Re, SO 2 NHRb, SO 2 NRaRb, C (S ) NHRb, C (S) NRaRb, C (O) Rf, a P (O) RgRh, P (S) RgRh, alkali metal, alkaline earth metal or NHRiRjRk,
    Gは、H、ハロゲン、C 〜C アルキル、Rcで置換されたC 〜C アルキル、C 〜C ハロアルキル、C 〜C アルキルで置換されていてもよいC 〜C シクロアルキル、C 〜C アルコキシ、C 〜C アルケニルオキシ、C 〜C アルキニルオキシ、C 〜C ハロアルコキシ、C 〜C アルキルスルフェニル、C 〜C アルキルスルフィニル、C 〜C アルキルスルホニル、C 〜C アルケニルスルフェニル、C 〜C アルケニルスルフィニル、C 〜C アルケニルスルホニル、C 〜C アルキニルスルフェニル、C 〜C アルキニルスルフィニル、C 〜C アルキニルスルホニル、C 〜C ハロアルキルスルフェニル、C 〜C ハロアルキルスル G is, H, halogen, C 1 -C 6 alkyl, C 1 -C 4 alkyl substituted by Rc, C 1 ~C 4 haloalkyl, C 1 -C 3 alkyl C 3 optionally substituted with -C 6 cycloalkyl, C 1 -C 6 alkoxy, C 2 -C 4 alkenyloxy, C 2 -C 4 alkynyloxy, C 1 -C 4 haloalkoxy, C 1 -C 4 alkylsulfenyl, C 1 -C 4 alkyl sulfinyl, C 1 -C 4 alkylsulfonyl, C 2 -C 4 alkenyl Le phenyl, C 2 -C 4 alkenylsulfinyl, C 2 -C 4 alkenylsulfonyl, C 2 -C 4 alkyl Nils Le phenyl, C 2 -C 4 alkynyl sulfinyl, C 2 -C 4 alkynylsulfonyl, C 1 -C 4 haloalkylsulfenyl, C 1 -C 4 haloalkylsulfenyl ィニル、C 〜C ハロアルキルスルホニル、C 〜C ハロアルケニルスルフェニル、C 〜C ハロアルケニルスルフィニル、C 〜C ハロアルケニルスルホニル、NO 、CN、−NU 、ナフチル、Rcで置換されたメトキシ、C 〜C アルコキシカルボニル、C 〜C アルコキシアルキル、C 〜C アルキルカルボニル、C 〜C ハロアルキルカルボニル、C 〜C アルキルカルボニルオキシ、C 〜C ハロアルキルカルボニルオキシ、C 〜C ジアルキルアミノカルボニルオキシ、Zで置換されていてもよいフェニル、Zで置換されていてもよいフェノキシ、Zで置換されていてもよいベンゾイル、Zで置換されていてもよいピリジル、Zで置換されていてもよいピリジルオ Iniru, C 1 -C 4 haloalkylsulfonyl, C 2 -C 4 halo alkenyl Le phenyl, C 2 -C 4 halo alkenylsulfinyl, C 2 -C 4 haloalkenyl sulfonyl, NO 2, CN, -NU 1 U 2, naphthyl , methoxy substituted with Rc, C 2 -C 5 alkoxycarbonyl, C 2 -C 4 alkoxyalkyl, C 2 -C 4 alkylcarbonyl, C 2 -C 4 haloalkylcarbonyl, C 2 -C 5 alkylcarbonyloxy, C 2 -C 5 halo alkylcarbonyloxy, C 3 -C 7 dialkylaminocarbonyloxy, phenyl optionally substituted by Z, which may be substituted with Z phenoxy, optionally substituted by Z benzoyl, with Z optionally substituted pyridyl, optionally substituted by Z Pirijiruo シ、Zで置換されていてもよいチエニル、隣接した置換位置で結合したメチレンジオキシ、隣接した置換位置で結合したハロメチレンジオキシ及び−N=CT の中から選ばれる1ないし4個の置換基、または隣接した置換位置で結合したアルキレン基によって形成される5ないし8員環であり、 Shi, thienyl which may be substituted with Z, adjacent methylenedioxy bound to a substituted position, to 1 selected from halo methylenedioxy and -N = CT 2 T 3 bound in adjacent substitution positions 4 a number of substituents or 5 is formed by an alkylene group bonded at the adjacent substituting position to 8-membered ring,
    Y、Y 及びY は、各々独立にH、ハロゲン、C 〜C アルキル、C 〜C ハロアルキル、C 〜C アルコキシ、C 〜C ハロアルコキシ、C 〜C アルキルスルフェニル、C 〜C アルキルスルフィニル、C 〜C アルキルスルホニル、C 〜C ハロアルキルスルフェニル、C 〜C ハロアルキルスルフィニル、C 〜C ハロアルキルスルホニル、NO またはCNであるか、または隣接した置換位置で結合したアルキレン基によって形成される5員環、6員環、7員環もしくは8員環であり、 Y, Y 1 and Y 2 are each independently H, halogen, C 1 -C 4 alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 alkoxy, C 1 -C 4 haloalkoxy, C 1 -C 4 alkylsulfenyl, C 1 -C 4 alkylsulfinyl, C 1 -C 4 alkylsulfonyl, C 1 -C 4 haloalkylsulfenyl, C 1 -C 4 haloalkylsulfinyl, C 1 -C 4 haloalkylsulfonyl, NO 2 or CN 5-membered ring formed by an alkylene group, or bound in adjacent substitution positions is a 6-membered ring, 7-membered ring or 8-membered ring,
    は、H、C 〜C アルキルまたはC 〜C ハロアルキルであり、 Y 3 is, H, a C 1 -C 4 alkyl or C 1 -C 4 haloalkyl,
    Zは、各々独立して、ハロゲン、C 〜C アルキル、C 〜C ハロアルキル、C 〜C アルコキシ、C 〜C ハロアルコキシ、C 〜C アルキルスルフェニル、C 〜C アルキルスルフィニル、C 〜C アルキルスルホニル、C 〜C アルケニルスルフェニル、C 〜C アルケニルスルフィニル、C 〜C アルケニルスルホニル、C 〜C ハロアルキルスルフェニル、C 〜C ハロアルキルスルフィニル、C 〜C ハロアルキルスルホニル、NO 、CN、−NU 及びC 〜C アルコキシカルボニルの中から選ばれる1ないし5個の置換基であり、 Z are each independently halogen, C 1 -C 4 alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 alkoxy, C 1 -C 4 haloalkoxy, C 1 -C 4 alkylsulfenyl, C 1 -C 4 alkylsulfinyl, C 1 -C 4 alkylsulfonyl, C 2 -C 4 alkenyl Le phenyl, C 2 -C 4 alkenylsulfinyl, C 2 -C 4 alkenylsulfonyl, C 1 -C 4 haloalkylsulfenyl, C 1 -C 4 haloalkylsulfinyl, a C 1 -C 4 haloalkylsulfonyl, nO 2, CN, 1 to 5 substituents selected from among -NU 1 U 2 and C 2 -C 5 alkoxycarbonyl,
    、R 、R 及びRaは、各々独立にC 〜C アルキルであり、 R 1, R 2, R 3 and Ra is C 1 -C 6 alkyl each independently,
    Rbは、H、C 〜C アルキル、またはT で置換されていてもよいフェニルであり、 Rb is, H, a C 1 -C 6 alkyl or phenyl optionally substituted with T 1,,
    Rcは、ハロゲン、C 〜C アルキル、C 〜C アルコキシ及びC 〜C ハロアルキルの中から任意に選ばれる1種以上で置換されていてもよいフェニルであり、 Rc is halogen, C 1 -C 4 alkyl, C 1 -C 4 alkoxy and C 1 -C 4 phenyl optionally substituted with one or more selected arbitrarily from among haloalkyl,
    Rdは、ハロゲン、C 〜C アルキル及びC 〜C ハロアルキルの中から任意に選ばれる1種以上で置換されていてもよいベンゾイルであり、 Rd is halogen, C 1 -C 4 alkyl and C 1 -C 4 optionally benzoyl optionally substituted with one or more selected arbitrarily from among haloalkyl,
    Reは、C 〜C アルキル、C 〜C ハロアルキル、またはT で置換されていてもよいフェニルであり、 Re is a C 1 -C 4 alkyl, C 1 -C 4 haloalkyl or phenyl optionally substituted with T 1,,
    Rfは、C 〜C 20アルキル、C 〜C アルケニル、C 〜C ハロアルキル、C 〜C アルコキシアルキル、C 〜C ハロシクロアルキル、Rcで置換されたC 〜C アルキル、C 〜C アルキルで置換されていてもよいC 〜C シクロアルキル、Rcで置換されたシクロアルキル、Rc及びC 〜C アルキルで置換されたシクロプロピル、Rc及びハロゲンで置換されたC 〜C シクロアルキル基、T 及びC 〜C アルキルで置換されたシクロプロピル基、Rcで置換されたC 〜C アルケニル、C 〜C アルコキシ、C 〜C ハロアルコキシ、C 〜C アルケニルオキシ、C 〜C アルキルで置換されていてもよいC 〜C シクロアルコキシ、ベンジルオキシ Rf is, C 1 -C 20 alkyl, C 2 -C 6 alkenyl, C 1 -C 6 haloalkyl, C 2 -C 4 alkoxyalkyl, C 3 -C 6 halocycloalkyl, C 1 -C substituted with Rc 4 alkyl, C 1 -C 4 optionally substituted by alkyl C 3 -C 7 cycloalkyl, cycloalkyl substituted with Rc, Rc and C 1 -C 4 alkyl substituted cyclopropyl, Rc and halogen in substituted C 3 -C 4 cycloalkyl group, T 2, and C 1 -C 4 alkyl substituted cyclopropyl group, C 2 -C 4 alkenyl substituted with Rc, C 1 ~C 6 alkoxy, C 1 -C 4 haloalkoxy, C 2 -C 5 alkenyloxy, C 1 -C 3 may be alkyl substituted C 3 -C 6 cycloalkoxy, benzyloxy 、COORa、−NU 、T で置換されていてもよいフェニル、T で置換されていてもよいフェノキシ、ナフチル、T で置換されていてもよいピリジルまたはA−1〜A−140であり、 , COORa, -NU 1 U 2, T 3 optionally substituted by phenyl, optionally substituted with T 3 phenoxy, naphthyl, T 1 pyridyl or A-1~A- be substituted by is 140,
    Rg及びRhは各々独立に、OH、フェニル、C 〜C アルキル、C 〜C アルコキシまたはC 〜C アルキルスルフェニルであり、 Rg and Rh are each independently, OH, phenyl, C 1 -C 6 alkyl, C 1 -C 6 alkoxy or C 1 -C 4 alkylsulfenyl,
    Ri、Rj及びRkは各々独立に、H、C 〜C アルキル、C 〜C アルケニル、C 〜C アルキル基で置換されていてもよいC 〜C シクロアルキル基またはベンジルであるか、あるいはRi、Rj及びRkのうちの2個が、それぞれが結合している窒素原子と共に酸素原子、窒素原子または硫黄原子を含有していてもよい5ないし8員環基を形成してもよく、 Ri, Rj and Rk are each independently, H, C 1 -C 6 alkyl, C 1 -C 4 alkenyl, optionally substituted with C 1 -C 3 alkyl group C 3 -C 6 cycloalkyl group or a benzyl or is, or Ri, 2 pieces of Rj and Rk are an oxygen atom together with the nitrogen atom to which each is attached, to 5 which may contain a nitrogen atom or a sulfur atom to form a 8-membered ring group at best,
    は、ハロゲン、C 〜C アルキル、C 〜C ハロアルキルまたはC 〜C アルコキシであり、 T 1 is halogen, C 1 -C 4 alkyl, C 1 -C 4 haloalkyl or C 1 -C 4 alkoxy,
    は、ハロゲンで置換されていてもよいC 〜C アルケニルであり、 T 2 are a good C 2 -C 4 alkenyl optionally substituted by halogen,
    は、ハロゲン、C 〜C アルキル、C 〜C ハロアルキル、C 〜C アルコキシ、C 〜C ハロアルコキシ、C 〜C アルキルスルフェニル、C 〜C アルキルスルフィニル、C 〜C アルキルスルホニル、C 〜C ハロアルキルスルフェニル、C 〜C ハロアルキルスルフィニル、C 〜C ハロアルキルスルホニル、NO 、CN、CHO、−NU 、フェニル及びフェノキシの中から任意に選ばれる1ないし5個の置換基であり、 T 3 is halogen, C 1 -C 4 alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 alkoxy, C 1 -C 4 haloalkoxy, C 1 -C 4 alkylsulfenyl, C 1 -C 4 alkyl sulfinyl, C 1 -C 4 alkylsulfonyl, C 1 -C 4 haloalkylsulfenyl, C 1 -C 4 haloalkylsulfinyl, C 1 -C 4 haloalkylsulfonyl, NO 2, CN, CHO, -NU 1 U 2, phenyl and it 1 is arbitrarily selected from among phenoxy are 5 substituents,
    及びU は、各々独立に、H、C 〜C アルキル、COORa、フェニルまたはベンジルを表すか、あるいはU とU とが結合している窒素原子と共に酸素原子、窒素原子または硫黄原子を含有していてもよい5ないし8員環基を形成してもよく、 U 1 and U 2 are each independently, H, C 1 -C 6 alkyl, COORa, or represents phenyl or benzyl, or U 1 and U 2 and an oxygen atom together with the nitrogen atom to which they are attached a nitrogen atom or 5 to may contain a sulfur atom may form a 8-membered ring group,
    mは、置換基の数を表し、0、1、2または3であり、 m represents the number of substituents is 0, 1, 2 or 3,
    nは、置換基の数を表し、0、1、2、3または4であり、 n represents the number of substituents is 0, 1, 2, 3 or 4,
    pは、置換基の数を表し、0、1または2であり、 p represents the number of substituents is 0, 1 or 2,
    qは、置換基の数を表し、0または1である。 q represents the number of substituents is 0 or 1. (但し、m、n及びpが2以上の整数を表す場合は、その置換基は同一か相互に異なってもよい。)]。 (Where, m, when the n and p is an integer of 2 or more, the substituents may be different in the same or another.).
    化合物群A:アシベンゾラルーS−メチル、アシルアミノベンザミド、アンバム、アムプロピルホス、アニラジン、アザコナゾール、アゾキシストロビン、ベナラキシル、ベノダニル、ベノミル、ベンチアゾール、ベンザマクリル、ビナパクリル、ビフェニル、ビテルタノール、ベトキサジン、ボルドー液、ブラストサイジン−S、ブロモコナゾール、ブピリメート、ブチオベート、カルシウムポリスルフィド、キャプタフォール、キャプタン、カッパーオキシクロリド、カルプロパミド、カルベンダジン、カルボキシン、CGA−279202、キノメチオネート、クロベンチアゾン、クロルフェナゾール、クロロネブ、クロロタロニル、クロゾリネート、クフラネブ、シモキサニル、シプロコナゾール、シプロジニル、シプロフラム、ダ Compounds A: Ashibenzoraru S- methyl, acylamino benzalkonium bromide, Anbamu, Am propyl phosphite, Anirajin, azaconazole, azoxystrobin, benalaxyl, Benodaniru, benomyl, bench azole, Benzamakuriru, binapacryl, biphenyl, bitertanol, Betokisajin, Bordeaux mixture, blasticidin -S, Bro Mokona tetrazole, bupirimate, buthiobate, calcium polysulfide, cap data fall, captan, copper oxychloride, carpropamid, carbendazim Jin, carboxin, CGA-two hundred seventy-nine thousand two hundred and two, Kinomechioneto, black bench azone, chlorobenzene phenazine tetrazole, chloroneb , chlorothalonil, chlozolinate, Kufuranebu, cymoxanil, cyproconazole, cyprodinil, Shipurofuramu, da メット、デバカルブ、ジクロロフェン、ジクロブトラゾール、ジクロフラニド、ジクロメジン、ジクロラン、ジエトフェンカルブ、ジクロシメット、ジフェノコナゾール、ジフルメトリン、ジメチリモール、ジメトモルフ、ジニコナゾール、ジニコナゾール−M、ジノカップ、ジフェニルアミン、ジピリチオン、ジタリムホス、ジチアノン、ドデモルフ、ドジン、ドラゾクソロン、エデフェノホス、エポキシコナゾール、エタコナゾール、エチリモル、エトリジアノール、ファモキサゾン、フェナリモル、フェブコナゾール、フェナミドン、フェンダゾスラム、フェンフラム、フェンヘキサミド、フェンピクロニル、フェンプロピジン、フェンプロピモルフ、フェンチン、フェルバン、フェリムゾン、フルアジナム、フルジオキソニル、フ Met, Debakarubu, dichlorophen, Axis Rob tiger tetrazole, Jikurofuranido, Jikuromejin, dichloran, diethofencarb, diclocymet, difenoconazole, Jifurumetorin, dimethirimol, dimethomorph, diniconazole, diniconazole -M, dinocap, diphenylamine, Jipirichion, Jitarimuhosu, dithianon, dodemorph, dodine, Dorazokusoron, Edefenohosu, epoxiconazole, Etakonazoru, Echirimoru, Etorijianoru, Famokisazon, fenarimol, Febukonazoru, fenamidone, fender zone slum, Fenfuramu, fenhexamid, fenpiclonil, fenpropidin, fenpropimorph, fentin, Feruban, ferimzone, fluazinam, fludioxonil, off オロイミド、フルキンコナゾール、フルシラゾール、フルスルファミド、フルトラニル、フルトリアフォール、フォルペット、フォセチル−アルミニウム、フベリダゾール、フララキシル、フラメトピル、グアザチン、ヘキサクロロベンゼン、ヘキサコナゾール、ヒメキサゾール、イマザリル、イミベンコナゾール、イミノクタジン、イプコナゾール、イプロベンホス、イプロジオン、イソプロチオラン、イプロバリカルブ、カスガマイシン、クレソキシム−メチル、マンカッパー、マンコゼブ、マンネブ、メパニピリム、メプロニル、メタラキシル、メトコナゾール、メタスルホカルブ、メチラム、メトミノストロビン、ミクロブタニル、MTF−753、ナバム、ニッケルビス(ジメチルジチオカーバメート)、ニトロタール−イソプロ Oroimido, fluquinconazole, flusilazole, flusulfamide, flutolanil, full-thoria fall, folpet, fosetyl - aluminum, fuberidazole, furalaxyl, furametpyr, guazatine, hexachlorobenzene, hexaconazole, hymexazol, imazalil, imibenconazole, iminoctadine, ipconazole, iprobenfos, iprodione, isoprothiolane, iprovalicarb, kasugamycin, kresoxim - methyl, Man copper, mancozeb, maneb, mepanipyrim, mepronil, metalaxyl, metconazole, methasulfocarb, metiram, metominostrobin, myclobutanil, MTF-753, Nabamu, nickel bis ( dimethyldithiocarbamate), Nitorotaru - isoproterenol ピル、ヌアリモル、NNF−9425、オクチリノン、オフレース、オキサジキシル、オキシカルボキシン、オキポコナゾールフマール酸塩、ペフラゾエート、ペンコナゾール、ペンシクロン、フタライド、ピペラリン、ポリオキシン、炭酸水素カリウム、プロベナゾール、プロクロラズ、プロシミドン、プロパモカルブ塩酸塩、プロピコナゾール、プロピネブ、ピラゾホス、ピリフェノックス、ピリメタニル、ピロキュロン、キノメチオネート、キノキシフェン、キントゼン、RH7281、炭酸水素ナトリウム、次亜塩素酸ナトリウム、硫黄、スピロキサミン、テブコナゾール、テクナゼン、テトラコナゾール、チアベンダゾール、チアジアジン、チフルザミド、チオファネート−メチル、チラム、トルクロホス−メチル、トリルフラニ Pills, nuarimol, NNF-9425, octhilinone, ofurace, oxadixyl, oxycarboxin, Oki Poco Nazo Ruch Mar salt, pefurazoate, penconazole, pencycuron, phthalide, Piperarin, polyoxin, potassium hydrogen carbonate, probenazole, prochloraz, procymidone, propamocarb hydrochloride salt, propiconazole, propineb, pyrazophos, pyrifenox, pyrimethanil, Pirokyuron, Kinomechioneto, quinoxyfen, quintozene, RH7281, sodium bicarbonate, sodium hypochlorite, sulfur, spiroxamine, tebuconazole, Tekunazen, Tetraconazole tetrazole, thiabendazole, thiadiazine, thifluzamide, thiophanate - methyl, thiram, tolclofos - methyl, Torirufurani 、トリアジメホン、トリアジメノール、トリアゾキシド、トリシクラゾール、トリデモルフ、トリフルミゾール、トリホリン、トリチコナゾール、バリダマイシン、ビンクロゾリン、硫酸亜鉛、ジネブ、ジラム、シイタケ菌糸体抽出物、ストレプトマイシン、テクロフタラム、オキシテトラサイクリン、オキソリニックアシド、アルドキシカルブ、カズサホス、フォスチアゼート、フォスチエタン、オキサミル、フェナミホス、アセキノシル、ブロモプロピレート、チノメチオネート、クロロベンジラート、サイヘキサチン、ジコフォール、ジエノクロール、エトキサゾール、フェナザキン、フェンブタチンオキシド、フェンプロパトリン、フェンプロキシメート、ハルフェンプロックス、ヘキシチアゾックス、ミルベメクチン、プロパル , Triadimefon, triadimenol, triazoxide, tricyclazole, tridemorph, triflumizole, triforine, triticonazole, validamycin, vinclozolin, zinc sulfate, zineb, ziram, shiitake mycelium extract, streptomycin, tecloftalam, oxytetracycline, oxolinic A Sid, aldoxycarb, cadusafos, fosthiazate, Fosuchietan, oxamyl, fenamiphos, acequinocyl, bromopropylate, Chinomechioneto, chlorobenzal iophendylate, Saihekisachin, dicofol, Jienokuroru, etoxazole, fenazaquin, fenbutatin oxide, fenpropathrin, Fen proxy formate, Hull Fen PROX, hexythiazox, milbemectin, Puroparu ット、ピリダベン、ピリミジフェン、テブフェンピラド、アバメクチン、アセフェート、アセタミピリド、アルディカルブ、アレスリン、アジンホス−メチル、ベンジオカルブ、ベンフラカルブ、ベンスルタップ、ブプロフェジン、ブトカルボキシン、カルバリル、カルボフラン、カルボスルファン、カルタップ、クロルフェナピル、クロルピリホス、クロルフェンビンホス、クロルフルアズロン、クロチアニジン、クロマフェノジド、クロピリホス−メチル、シクロプロトリン、シフルトリン、ベータ−シフルトリン、シペルメトリン、シロマジン、シハロトリン、ラムダ−シハロトリン、デルタメトリン、ジアフェンチウロン、ダイアジノン、ジアクロデン、ジフルベンズロン、ジメチルビンホス、ジオフェノラン、ジスルフォトン、ジ Tsu DOO, pyridaben, pyrimidifen, tebufenpyrad, abamectin, acephate, Asetamipirido, aldicarb, allethrin, azinphos - methyl, bendiocarb, benfuracarb, bensultap, buprofezin, Butokarubokishin, carbaryl, carbofuran, carbosulfan, cartap, chlorfenapyr, chlorpyrifos, chlorfenvinphos, chlorfluazuron, clothianidin, chromafenozide, Kuropirihosu - methyl, cyclopropyl, cyfluthrin, beta - cyfluthrin, cypermethrin, cyromazine, cyhalothrin, lambda - cyhalothrin, deltamethrin, diafenthiuron, diazinon, Jiakuroden, diflubenzuron, dimethyl bottle phosphite, diofenolan, Jisurufoton, di メトエート、エマメクチンベンゾエート、EPN、エスフェンバレレート、エチオフェンカルブ、エチプロール、エトフェンプロックス、エトリムホス、フェニトロチオン、フェノブカルブ、フェノキシカーブ、フェンプロパトリン、フェンバレレート、フィプロニル、フルアクリピリム、フルシトリネート、フルフェノクスウロン、フルフェンプロックス、タウ−フルバリネート、ホノホス、フォルメタネート、フォルモチオン、フラチオカルブ、ハロフェノジド、ヘキサフルムロン、ヒドラメチルノン、イミダクロプリド、イソフェンホス、インドキサカルブ、イソプロカルブ、イソキサチオン、ルフェヌウロン、マラチオン、メタルデヒド、メタミドホス、メチダチオン、メタクリホス、メタルカルブ、メソミル、メソプレン、メトキ Metoeto, emamectin benzoate, EPN, esfenvalerate, ethiofencarb, ethiprole, etofenprox, etrimfos, fenitrothion, fenobucarb, phenoxy curve, fenpropathrin, fenvalerate, fipronil, fluacrypyrim, flucythrinate, flufenoxuron uronic full Fen flufenprox tau - fluvalinate, fonofos, folder meth sulfonates, formothion, furathiocarb, halofenozide, hexaflumuron, hydramethylnon, imidacloprid, isofenphos, indoxacarb, isoprocarb, isoxathion, Rufenuuron, malathion, Metarudehido, methamidophos, methidathion, Metakurihosu, Metarukarubu, methomyl, methoprene, methoxide クロール、メトキシフェノジド、モノクロトホス、ムスカルーレ、ニジノテフラン、ニテンピラム、オメトエート、オキシデメトン−メチル、オキサミル、パラチオン、パラチオン−メチル、ペルメトリン、フェントエート、フォキシム、ホレート、ホサロン、ホスメット、ホスファミドン、ピリミカルブ、ピリミホス−メチル、プロフェノホス、プロトリフェンブト、ピメトロジン、ピラクロホス、ピリプロキシフェン、ロテノン、スルプロホス、シラフルオフェン、スピノサド、スルホテップ、テブフェノジド、テフルベンズロン、テフルトリン、テルブホス、テトラクロロビンホス、チアクロプリド、チオシクラム、チオジカルブ、チアメトキサム、チオファノックス、チオメトン、トルフェンピラド、トラロメスリン、トリクロル Crawl, methoxyfenozide, monocrotophos, Musukarure, two dinotefuran, nitenpyram, omethoate, oxydemeton - methyl, oxamyl, parathion, parathion - methyl, permethrin, phenthoate, phoxim, phorate, phosalone, phosmet, phosphamidon, pirimicarb, pirimiphos - methyl, profenofos, Pro triphenedioxazine butoxide, pymetrozine, pyraclofos, pyriproxyfen, rotenone, sulprofos, silafluofen, spinosad, sulfotep, tebufenozide, teflubenzuron, tefluthrin, terbufos, tetrachloride robin phosphite, thiacloprid, thiocyclam, thiodicarb, thiamethoxam, thiofanox, thiometon, tolfenpyrad, tralomethrin, trichloroacetic ン、トリアズロン、トリフルムロン、バミドチオン及びエチオン。 Down, Toriazuron, triflumuron, vamidothion and ethion.
  2. 請求項1記載の式(1)で表されるアクリロニトリル化合物の1種以上と、以下の化合物群Bより選ばれる化合物の1種以上を含有する殺ダニ組成物。 Acaricidal compositions containing one or more with one or more of the following compounds a compound selected from B of claim 1 acrylonitrile compound represented by the formula (1) as claimed.
    化合物群B:アセキノシル、ブロモプロピレート、チノメチオネート、ジコフォール、エトキサゾール、フェンブタチンオキシド、ミルベメクチン、プロパルギット、ピリダベン、アバメクチン、アルディカルブ、クロルピリフォス、ジフルベンズロン、クロルフェナピル、フェントエート、エマメクチンベンゾエート、メチダチオン、オキサミル、カルシウムポリスルフィド、マンコゼブ、マンネブ及びエチオン。 Compound group B: acequinocyl, bromopropylate, Chinomechioneto, dicofol, etoxazole, fenbutatin oxide, milbemectin, propargite, pyridaben, abamectin, aldicarb, chlorpyrifos, diflubenzuron, chlorfenapyr, phenthoate, emamectin benzoate, methidathion, oxamyl, calcium polysulfide, mancozeb, maneb and ethion.
  3. ハダニ、フシダニ又はホコリダニの防除に用いる請求項2記載の殺ダニ組成物。 Spider mites, Fushidani or dust mite claim 2 acaricidal composition according used for controlling.
  4. 請求項1記載の式(1)で表されるアクリロニトリル化合物の1種以上と、請求項1記載の化合物群Aより選ばれる化合物の1種以上を同時に、又は近接して処理することを特徴とする、害虫又は病害の防除方法。 And one or more of claims 1 acrylonitrile compound represented by the formula (1) as claimed, and wherein simultaneously, or close to the process of one or more of claims 1 compounds compound selected from A according to method for controlling pests or disease.
  5. 請求項1記載の式(1)で表されるアクリロニトリル化合物の1種以上と、請求項2記載の化合物群Bより選ばれる化合物の1種以上を同時に、又は近接して処理することを特徴とする、ダニの防除方法。 And one or more of claims 1 acrylonitrile compound represented by the formula (1) as claimed, and wherein simultaneously, or close to the process of one or more of claims 2 compounds compound selected from B according the method for controlling mites.
  6. 請求項1記載の式(1)で表されるアクリロニトリル化合物の1種以上と、請求項2記載の化合物群Bより選ばれる化合物の1種以上を同時に、又は近接して処理することを特徴とする、ハダニ、フシダニ又はホコリダニの防除方法。 And one or more of claims 1 acrylonitrile compound represented by the formula (1) as claimed, and wherein simultaneously, or close to the process of one or more of claims 2 compounds compound selected from B according to, spider mites, Fushidani or dust mite control methods.
JP2002322041A 2002-11-06 2002-11-06 Insecticidal, acaricidal, nematicidal, fungicidal or bactericidal composition, and method for controlling disease and insect pest Pending JP2004155693A (en)

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Cited By (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2007145221A1 (en) * 2006-06-13 2007-12-21 Nissan Chemical Industries, Ltd. Aqueous suspension agricultural chemical composition
WO2010095427A1 (en) 2009-02-17 2010-08-26 株式会社日本触媒 Polyacrylic acid-based water-absorbing resin powder and method for producing the same
JP2014012686A (en) * 2006-07-06 2014-01-23 Bayer Cropscience Ag Pesticide composition comprising pyridylethylbenzamide derivative and insecticidal compound
CN104904722A (en) * 2015-05-19 2015-09-16 陕西上格之路生物科学有限公司 Mite killing composition containing cyenopyrafen and pyridaben
CN104920393A (en) * 2015-05-19 2015-09-23 陕西上格之路生物科学有限公司 Acaricidal composition containing cyenopyrafen and abamectin

Cited By (8)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2007145221A1 (en) * 2006-06-13 2007-12-21 Nissan Chemical Industries, Ltd. Aqueous suspension agricultural chemical composition
JP5339055B2 (en) * 2006-06-13 2013-11-13 日産化学工業株式会社 Pesticidal composition
US9408385B2 (en) 2006-07-06 2016-08-09 Bayer Cropscience Ag Pesticidal composition comprising a pyridylethylbenzamide derivative and an insecticide compound
JP2014012686A (en) * 2006-07-06 2014-01-23 Bayer Cropscience Ag Pesticide composition comprising pyridylethylbenzamide derivative and insecticidal compound
JP2016065093A (en) * 2006-07-06 2016-04-28 バイエル・クロップサイエンス・アクチェンゲゼルシャフト Pesticide composition containing pyridyl ethyl benzamide derivative and insecticidal compound
WO2010095427A1 (en) 2009-02-17 2010-08-26 株式会社日本触媒 Polyacrylic acid-based water-absorbing resin powder and method for producing the same
CN104904722A (en) * 2015-05-19 2015-09-16 陕西上格之路生物科学有限公司 Mite killing composition containing cyenopyrafen and pyridaben
CN104920393A (en) * 2015-05-19 2015-09-23 陕西上格之路生物科学有限公司 Acaricidal composition containing cyenopyrafen and abamectin

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