IL43340A - A copolymer formed by the polymerization of two acrylic monomers and shaped articles formed therefrom - Google Patents

A copolymer formed by the polymerization of two acrylic monomers and shaped articles formed therefrom

Info

Publication number
IL43340A
IL43340A IL43340A IL4334073A IL43340A IL 43340 A IL43340 A IL 43340A IL 43340 A IL43340 A IL 43340A IL 4334073 A IL4334073 A IL 4334073A IL 43340 A IL43340 A IL 43340A
Authority
IL
Israel
Prior art keywords
copolymer
shaped article
acrylate
methyl
saturated
Prior art date
Application number
IL43340A
Other languages
Hebrew (he)
Other versions
IL43340A0 (en
Original Assignee
Corneal Sciences
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Corneal Sciences filed Critical Corneal Sciences
Publication of IL43340A0 publication Critical patent/IL43340A0/en
Publication of IL43340A publication Critical patent/IL43340A/en

Links

Classifications

    • GPHYSICS
    • G02OPTICS
    • G02BOPTICAL ELEMENTS, SYSTEMS OR APPARATUS
    • G02B1/00Optical elements characterised by the material of which they are made; Optical coatings for optical elements
    • G02B1/04Optical elements characterised by the material of which they are made; Optical coatings for optical elements made of organic materials, e.g. plastics
    • G02B1/041Lenses
    • G02B1/043Contact lenses
    • AHUMAN NECESSITIES
    • A01AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
    • A01NPRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
    • A01N25/00Biocides, pest repellants or attractants, or plant growth regulators, characterised by their forms, or by their non-active ingredients or by their methods of application, e.g. seed treatment or sequential application; Substances for reducing the noxious effect of the active ingredients to organisms other than pests
    • A01N25/08Biocides, pest repellants or attractants, or plant growth regulators, characterised by their forms, or by their non-active ingredients or by their methods of application, e.g. seed treatment or sequential application; Substances for reducing the noxious effect of the active ingredients to organisms other than pests containing solids as carriers or diluents
    • A01N25/10Macromolecular compounds
    • AHUMAN NECESSITIES
    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61KPREPARATIONS FOR MEDICAL, DENTAL OR TOILETRY PURPOSES
    • A61K6/00Preparations for dentistry
    • A61K6/80Preparations for artificial teeth, for filling teeth or for capping teeth
    • A61K6/884Preparations for artificial teeth, for filling teeth or for capping teeth comprising natural or synthetic resins
    • A61K6/887Compounds obtained by reactions only involving carbon-to-carbon unsaturated bonds
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B01PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01DSEPARATION
    • B01D71/00Semi-permeable membranes for separation processes or apparatus characterised by the material; Manufacturing processes specially adapted therefor
    • B01D71/06Organic material
    • B01D71/40Polymers of unsaturated acids or derivatives thereof, e.g. salts, amides, imides, nitriles, anhydrides, esters
    • B01D71/401Polymers based on the polymerisation of acrylic acid, e.g. polyacrylate
    • B01D71/4011Polymethylmethacrylate
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F220/00Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical or a salt, anhydride ester, amide, imide or nitrile thereof
    • C08F220/02Monocarboxylic acids having less than ten carbon atoms; Derivatives thereof
    • C08F220/10Esters
    • C08F220/26Esters containing oxygen in addition to the carboxy oxygen
    • C08F220/28Esters containing oxygen in addition to the carboxy oxygen containing no aromatic rings in the alcohol moiety
    • C08F220/282Esters containing oxygen in addition to the carboxy oxygen containing no aromatic rings in the alcohol moiety and containing two or more oxygen atoms

Landscapes

  • Health & Medical Sciences (AREA)
  • Chemical & Material Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Physics & Mathematics (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Health & Medical Sciences (AREA)
  • Organic Chemistry (AREA)
  • Optics & Photonics (AREA)
  • Polymers & Plastics (AREA)
  • Medicinal Chemistry (AREA)
  • Oral & Maxillofacial Surgery (AREA)
  • General Physics & Mathematics (AREA)
  • Agronomy & Crop Science (AREA)
  • Veterinary Medicine (AREA)
  • Engineering & Computer Science (AREA)
  • Plant Pathology (AREA)
  • Epidemiology (AREA)
  • Dentistry (AREA)
  • Wood Science & Technology (AREA)
  • Zoology (AREA)
  • Environmental Sciences (AREA)
  • Pest Control & Pesticides (AREA)
  • Public Health (AREA)
  • Plastic & Reconstructive Surgery (AREA)
  • Animal Behavior & Ethology (AREA)
  • Toxicology (AREA)
  • Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
  • Eyeglasses (AREA)
  • Materials For Medical Uses (AREA)
  • Polymerisation Methods In General (AREA)

Claims (42)

Claiffls:
1. A copolymer formed by the polymerisation of two acrylic monomers, said first monomer being hydrophilic and conforming to the formula: R .0 OH CH2 = C - C - 0 - (CH2)n - CH - CHgOH where R is hydrogen or methyl and n is a whole integer having a value of from 0 to 4, and said second monomer being substantially water insoluble and conorming to the formula: A U CH2 o C - C - OR' where R is as above described and R1 is al&yl having from 1 to 6 carbon atoms, the mole ratio of said first acrylate to said second acrylate varying between 1:3 and 20:1,
2. The copolymer of claim 1 where the mole ratio of said first acrylate to said second acrylate varies between 1:1 and 10:1.
3. The copolymer of claim 1 where the mole ratio of said first acrylate to said second acrylate varies between 1.2:1 and 2:1.
4. The copolymer of claim 1 where R is methyl.
5. The copolymer of claim 1 where R and R' are methyl and n is 1.
6. The copolymer of claim 1 wherein said first monomer is 2,3-dihydroxypropyl methacrylate, said second monomer is methyl methacrylate and the mole ratio of the 2,3-dihydroxypropyl methacrylate to the methyl methacrylate varies between about 1.2:1 and 3:1.
7. · The copolymer of claim 6 where the ratio is about 1.3 to 1»
8. The copolymer of claim 6 formed in the presence of 0.02 weight percent of a catalyst based upon the weight of the 2,3-dihycLroxypropyl methacrylate.
9. · A shaped article formed from the copolymer of claim 1.
10. · The shaped article of claim 9 saturated with a drug.
11. · The shaped article of claim 9 saturated with water.
12. * The shaped article of claim 9 saturated with a pesticide.
13. The shaped article of claim 9 being saturated with an aqueous liquid containing a physiologically active solute.
14. The shaped article of claim 13 where said solute is bacteriostatic.
15. 5. The shaped article of claim 9 in the form of a contact lens.
16. The contact lens of claim 15 having anterior or posterior peripheral curvature or multiple peripheral curvatures.
17. The shaped article of claim 9 being formed with a plurality of openings therethrough, said openings defining passages through said article. i
18. A shaped article formed from the copolymer of claim 6i.
19. » The shaped article of claim 18 saturated with a drug.
20. The shaped article of claim 18 hydrated with water.
21. The shaped article of claim 18 saturated with a pesticide.
22. The shaped article of claim 18 saturated with an aqueous liquid containing a physiologically active 30lute.
23. · The shaped article of claim 22 where the solute is bacteriostatic.
24. The shaped article of claim 18 in the form of a contact lens.
25. The. shaped article of claim 24 hydrated with water.
26. The contact lens of claim 24 having anterior and/or posterior peripheral curvature or multiple peripheral curvatures.
27. · The shaped article of claim 18 being formed with a plurality of openings therethrough, said openings defining passages through said article.
28. The shaped article of claim 18 in the form of an intrauterine device.
29. · -A process for preparing a copolymerio structure comprising mixing two aorylates together in the substantial absence of water or other diluent, said first aerylate being hydrophilic and conforming to the formula: H O OH CH = C - C - 0 - (CHj - CH - CH OH 2 2 n 2 where R is hydrogen or methyl and n is a whole integer having a; value of from 0 to 4» and said second acrylate being substantially water insoluble and conforming 43540/3 where R is as above described and R' is alkyl having from 1 to 6 carbon atoms, the molar ratio of said first aorylate to said second aorylate Varying between 1:3 and 20:1 and causing said mixture to react so as to form a shape-retaining body of copolymer of said two acrylatea.
30. The process of claim 29 wherein said copolymer is formed by bulk polymerization in the substantial absence of water or other diluent.
31. · The process of claim 30 wherein the reaction temperature for the o polymerization reaction ie about 40 C.
32. The process of claim 29 wherein a hydrated round button formed from said copolymer having a thickness of 3 mm and a diameter of 12 mm will appear slightly milky when viewed through its cross-section.
33. * The process of claim 29 wherein said copolymer is formed by bulk polymerization of 2,3-dlhydroxypropyl methacrylate and methyl methacrylate in the substantial absence of water or other diluent, the molar ratio of 2,3-dihydroxypropyl methacrylate to methyl methacrylate ranging between about 1 :1 and 10:1.
34. The process of claim 33 wherein a hydrated round button formed from said copolymer having a thickness of 3 mm and a diameter of 12 mm will appear slightly milky when viewed through its cross-section.
35. The process of claim 29 including the step of hydrating the copolymer to form a hydrogel.
36. The process of claim 29 where the mole ratio of said first aorylate to said second acrylate varies between about 1:1 and 10:1.
37. · The process of claim 29 where the mole ratio of said first acrylate to said second acrylate varies between about 1.2:1 and 2:1*
38. The process of claim 29 where R and R1 are methyl and n is 1.
39. » The process of claim ;33 where the reaction temperature is about 40°C.
40. The process of claim 29 where a catalyst is used In an amount of about 0.02$ by weight of said first aerylate,
41. The process of claim 40 where the catalyst is lsopropylpercarbonate.
42. A contact lens formed by copolymer!Bation of 2,3-dihydroxypropyl methacrylate and methyl raethacrylate,said lens being a hydrogel which when hydrated swells linearly between about 17 and 19$, absorbs about 37 to 42$ liquid and has a durometer hardness of between about 46 to 49. 43· The contact lens of claim 4fl having a thickness varying between 0.05 mm and 0,15 mm*. 20 * l The copolymer of claim 1, further comprising from about 1 to about % by weight, based on said first monomer, of a epoxy compound conforming to the formulat I II U CH2 «0 -0 0 - (OHg)n - OH - CHg. 1+5. The copolymer of claim ht wherein the epoxy compound is present in an amount of from about 1 ·¾¾ to about 2·2# by weight based on said flrat monomer* ι·Ε. MULPORD Attorney for Applicants
IL43340A 1972-10-02 1973-09-30 A copolymer formed by the polymerization of two acrylic monomers and shaped articles formed therefrom IL43340A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US29401972A 1972-10-02 1972-10-02

Publications (2)

Publication Number Publication Date
IL43340A0 IL43340A0 (en) 1973-11-28
IL43340A true IL43340A (en) 1976-07-30

Family

ID=23131552

Family Applications (1)

Application Number Title Priority Date Filing Date
IL43340A IL43340A (en) 1972-10-02 1973-09-30 A copolymer formed by the polymerization of two acrylic monomers and shaped articles formed therefrom

Country Status (19)

Country Link
JP (2) JPS5750803B2 (en)
AR (1) AR216881A1 (en)
AT (1) AT339596B (en)
BE (1) BE805215A (en)
BR (1) BR7307579D0 (en)
CA (1) CA1002235A (en)
CH (1) CH621562A5 (en)
DD (2) DD109880A5 (en)
DE (1) DE2349528C2 (en)
DK (1) DK150526C (en)
ES (1) ES419240A1 (en)
FR (1) FR2201307B1 (en)
GB (1) GB1419437A (en)
IL (1) IL43340A (en)
IT (1) IT995537B (en)
NL (1) NL177601C (en)
SE (1) SE398647B (en)
SU (1) SU609473A3 (en)
ZA (1) ZA737138B (en)

Families Citing this family (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB2150147A (en) * 1983-11-25 1985-06-26 Donald James Highgate Materials for use in forming casts
JPS6233110A (en) * 1985-08-02 1987-02-13 Daikin Ind Ltd Dental material

Also Published As

Publication number Publication date
DD109880A5 (en) 1974-11-20
AT339596B (en) 1977-10-25
IL43340A0 (en) 1973-11-28
DE2349528C2 (en) 1983-07-21
DK150526B (en) 1987-03-16
FR2201307A1 (en) 1974-04-26
GB1419437A (en) 1975-12-31
CH621562A5 (en) 1981-02-13
JPS49116187A (en) 1974-11-06
JPS589121A (en) 1983-01-19
ES419240A1 (en) 1976-03-01
SE398647B (en) 1978-01-09
DK150526C (en) 1987-09-28
FR2201307B1 (en) 1977-08-05
IT995537B (en) 1975-11-20
AU6070173A (en) 1975-03-27
NL7313318A (en) 1974-04-04
DD113556A5 (en) 1975-06-12
JPS5750803B2 (en) 1982-10-29
ZA737138B (en) 1975-04-30
CA1002235A (en) 1976-12-21
JPS6232456B2 (en) 1987-07-15
NL177601C (en) 1985-10-16
DE2349528A1 (en) 1974-04-18
NL177601B (en) 1985-05-17
BR7307579D0 (en) 1974-08-22
ATA842673A (en) 1977-02-15
AR216881A1 (en) 1980-02-15
SU609473A3 (en) 1978-05-30
BE805215A (en) 1974-03-25

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