IL40246A - The manufacture of phosphorus-containing condensation products,the products and their use as flameproofing agents - Google Patents

The manufacture of phosphorus-containing condensation products,the products and their use as flameproofing agents

Info

Publication number
IL40246A
IL40246A IL40246A IL4024672A IL40246A IL 40246 A IL40246 A IL 40246A IL 40246 A IL40246 A IL 40246A IL 4024672 A IL4024672 A IL 4024672A IL 40246 A IL40246 A IL 40246A
Authority
IL
Israel
Prior art keywords
process according
triazine
tetrakis
component
manufacturing
Prior art date
Application number
IL40246A
Other versions
IL40246A0 (en
Original Assignee
Ciba Geigy Ag
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Ciba Geigy Ag filed Critical Ciba Geigy Ag
Publication of IL40246A0 publication Critical patent/IL40246A0/en
Publication of IL40246A publication Critical patent/IL40246A/en

Links

Classifications

    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06MTREATMENT, NOT PROVIDED FOR ELSEWHERE IN CLASS D06, OF FIBRES, THREADS, YARNS, FABRICS, FEATHERS OR FIBROUS GOODS MADE FROM SUCH MATERIALS
    • D06M15/00Treating fibres, threads, yarns, fabrics, or fibrous goods made from such materials, with macromolecular compounds; Such treatment combined with mechanical treatment
    • D06M15/19Treating fibres, threads, yarns, fabrics, or fibrous goods made from such materials, with macromolecular compounds; Such treatment combined with mechanical treatment with synthetic macromolecular compounds
    • D06M15/37Macromolecular compounds obtained otherwise than by reactions only involving carbon-to-carbon unsaturated bonds
    • D06M15/667Macromolecular compounds obtained otherwise than by reactions only involving carbon-to-carbon unsaturated bonds containing phosphorus in the main chain
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07FACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
    • C07F9/00Compounds containing elements of Groups 5 or 15 of the Periodic Table
    • C07F9/02Phosphorus compounds
    • C07F9/547Heterocyclic compounds, e.g. containing phosphorus as a ring hetero atom
    • C07F9/6515Heterocyclic compounds, e.g. containing phosphorus as a ring hetero atom having three nitrogen atoms as the only ring hetero atoms
    • C07F9/6521Six-membered rings
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L61/00Compositions of condensation polymers of aldehydes or ketones; Compositions of derivatives of such polymers
    • C08L61/20Condensation polymers of aldehydes or ketones with only compounds containing hydrogen attached to nitrogen
    • C08L61/32Modified amine-aldehyde condensates
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06MTREATMENT, NOT PROVIDED FOR ELSEWHERE IN CLASS D06, OF FIBRES, THREADS, YARNS, FABRICS, FEATHERS OR FIBROUS GOODS MADE FROM SUCH MATERIALS
    • D06M15/00Treating fibres, threads, yarns, fabrics, or fibrous goods made from such materials, with macromolecular compounds; Such treatment combined with mechanical treatment
    • D06M15/19Treating fibres, threads, yarns, fabrics, or fibrous goods made from such materials, with macromolecular compounds; Such treatment combined with mechanical treatment with synthetic macromolecular compounds
    • D06M15/37Macromolecular compounds obtained otherwise than by reactions only involving carbon-to-carbon unsaturated bonds
    • D06M15/39Aldehyde resins; Ketone resins; Polyacetals
    • D06M15/423Amino-aldehyde resins
    • D06M15/43Amino-aldehyde resins modified by phosphorus compounds
    • D06M15/431Amino-aldehyde resins modified by phosphorus compounds by phosphines or phosphine oxides; by oxides or salts of the phosphonium radical
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B27WORKING OR PRESERVING WOOD OR SIMILAR MATERIAL; NAILING OR STAPLING MACHINES IN GENERAL
    • B27KPROCESSES, APPARATUS OR SELECTION OF SUBSTANCES FOR IMPREGNATING, STAINING, DYEING, BLEACHING OF WOOD OR SIMILAR MATERIALS, OR TREATING OF WOOD OR SIMILAR MATERIALS WITH PERMEANT LIQUIDS, NOT OTHERWISE PROVIDED FOR; CHEMICAL OR PHYSICAL TREATMENT OF CORK, CANE, REED, STRAW OR SIMILAR MATERIALS
    • B27K2240/00Purpose of the treatment
    • B27K2240/30Fireproofing
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B27WORKING OR PRESERVING WOOD OR SIMILAR MATERIAL; NAILING OR STAPLING MACHINES IN GENERAL
    • B27KPROCESSES, APPARATUS OR SELECTION OF SUBSTANCES FOR IMPREGNATING, STAINING, DYEING, BLEACHING OF WOOD OR SIMILAR MATERIALS, OR TREATING OF WOOD OR SIMILAR MATERIALS WITH PERMEANT LIQUIDS, NOT OTHERWISE PROVIDED FOR; CHEMICAL OR PHYSICAL TREATMENT OF CORK, CANE, REED, STRAW OR SIMILAR MATERIALS
    • B27K3/00Impregnating wood, e.g. impregnation pretreatment, for example puncturing; Wood impregnation aids not directly involved in the impregnation process
    • B27K3/02Processes; Apparatus
    • B27K3/15Impregnating involving polymerisation including use of polymer-containing impregnating agents
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10STECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10S428/00Stock material or miscellaneous articles
    • Y10S428/92Fire or heat protection feature
    • Y10S428/921Fire or flameproofing

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Textile Engineering (AREA)
  • Engineering & Computer Science (AREA)
  • Health & Medical Sciences (AREA)
  • General Health & Medical Sciences (AREA)
  • Molecular Biology (AREA)
  • Biochemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Treatments For Attaching Organic Compounds To Fibrous Goods (AREA)
  • Compositions Of Macromolecular Compounds (AREA)

Abstract

The subject of the invention is a process for the manufacture of water-soluble condensation products of hydroxymethylphosphonium compounds and a 1,3,5-triazine characterised in that (a) 1 mol of a tetrakis-(hydroxymethyl)-phosphonium compound is condensed with (b) 0.02 to 0.1 mol, preferably 0.05 to 0.1 mol of optionally methylolated 1,3,5-triazine which is substituted by at least one primary amino group, at 40 DEG to 120 DEG C, optionally in the presence of formaldehyde or a formaldehyde-releasing agent and optionally in the presence of an inert organic solvent, the condensation is optionally thereafter continued at temperatures of 100 DEG to 150 DEG C and, if appropriate, free hydroxyl groups are etherified at least partially with at least one alkanol with 1 to 4 carbon atoms and, if appropriate, the salts of the condensation products are converted into the corresponding hydroxides. [US3887553A]

Claims (1)

1. Y/HAT WE CLAIM IS: 1. Process for the manufacture of water-soluble condensation products of hydroxymethyl-phosphoniu compounds and a 1 ,3 ,5-triazine , characterised in that 1 mol of a tetrakis-(hydroxymethyl )-phosphonium compound is condensed v/ith 0.02 to 0.1 mol of optionally methylolated 1,3,5-triazine, which is substituted by at least one primary amino group, at 40 to 120°C, optionally in the presence of formaldehyde or a formaldehyde-releasing agent and optionally in the presence of an inert organic solvent, the condensation is optionally continued at temperatures of 100 to 150°C and, if appropriate, free hydroxyl groups are etherified at least partially with at least one alkanol with 1 to 4 carbon atoms* 2. Process according to Claim 1, characterised in that the condensation is carried out at 70 to 110°C. 3. Process according to Claim 1 or 2, characterised in that the condensation is carried out in the presence of at least one inert aromatic hydrocarbon as the solvent. 4. Process according to Claim 3, characterised in that at least one xylene is used as the solvent. 5. Process according to one of Claims 1 to 4, characterised in that the two starting materials are condensed with one another in a molar ratio of 1:0.05 to 1:0.1. 6. Process according to one of Claims 1 to 5, characterised in that a tetrakis-(hydroxy-methyl)-phosphonium salt or tetrakis-(hydroxy-methyl)-phosphonium hydroxide is used. 7. Process according to Claim 6, characterised in that a tetrakis-(hydroxymethyl)-phosphonium salt is used. 8. Process according to Claim 7, characterised in that a tetrakis-(hydroxymethyl)-phosphonium halide is used. 9. Process according to Claim 8, characterised in that tetrakis-(hydroxymethyl)-phosphoniiim chloride is used. 10. Process according to one of Claims 1 to 9, characterised in that a compound of the formula is used as the 1,3,5-triazine, wherein R^ denotes amino, hydroxyl or hydrogen and 2 denotes amino, hydroxyl, hydrogen, methyl, phenyl or l-dialkylphosphono-(alkyl) '^, with n "being 1 or 2.. 11. Process according to Claim 10, characterised in that a compound of the formula in used as the 1,3 ,5-triazine , wherein ^ denotes amino or hydroxyl and ^ denotes amino, hydroxyl, hydrogen or 1-diethyl-phosphonoethyl. 12. Process according to Claim 11, characterised in that l-diethylphosphonoethyl-l,3,5-triazine or preferably melamine is used as the 1,3,5-triazine. 13. Process according to one of Clainel to 12, 40246/2 ' ' " ■ " J. characterised in that after completion of the reaction the salts of the condensation products are converted into the corresponding hydroxides. 14. The condensation products obtainable according to the process of one of Claims 1 to I3. 15. Process for flameproofing organic fibre materials, characterised in that an aqueous preparation is applied to these materials which contains at least 1) a water-soluble condensation product of a hydroxymethyl-phosphonium compound and.a 1,3,5-triazine, which is obtained by condensing 1 mol of a tetrakis- hydroxy-methyl)-phosphonium compound with 0.02 to 0.1 mol of optionally methylolated 1,3 ,5-triazine, which is substituted by at least one primary amino group, at 40 to 120°C, . optionally in the presence of formaldehyde or a formaldehyde- releasing agent, and optionally in the presence of an inert organic solvent and optionally subsequently continuing the condensation at temperatures of 100 to 150°C, and if appropriate, etherifying free hydroxyl groups at least partially with at least one alkanol with 1 to 4 carbon atoms, and 2) a polyfunctional epoxide having at least two epoxide groups which are derived from polyhydric phenols or a polyalkylenepolyamine , an arainoplast-forming finished in accordance with the wet batch, moist batch, ammonia fixing or thermofixing process. 16. Process according to Claim 15, characterised in that the treated materials are dried and subjected to a heat treatment. ■ . 7. ' Process according to Claim 16, characterised in that when manufacturing the component (l) the condensation is . carried out at 70 to 110°C. 18. Process according to Claim 15 or 16, characterised in that when manufacturing the component (1) the condensation is carried out in the presence of at least one inert aromatic hydrocarbon as the solvent. 19. Process according to Claim 18, characterised in that when manufacturing the component (1) at least one xylene is used as the solvent. 20. Process according to one of Claims 16 to I9, characterised in that when manufacturing the component, (1) the two starting materials are condensed with one another in a molar ratio of 1:0.05 to 1 : 0.1. 2-1. Process according to one of Claims 16 to 20, characterised in that. hen manufacturing the component (1) a tetrakis-(hydroxymethyl)-phosphonium salt or tetrakis-(hydroxymethyl)-phosphonium hydroxide is used. 22. Process according to Claim 21, characterised in that when manufacturing the component (1) a tetrakis-(hydroxymethyl) phosphonium salt is used. 23. Process according to Claim 22, characterised in that when manufacturing the component (1) a tetrakis-(hydroxymethyl) phosphonium halide is used. 24. Process according to Claim 2-3, characterised in that when manufacturing 'the component (1) tetrakis- (hydr'oxymethyl)-phosphonium chloride is used. 25. Process according to one of Claims 16 to 24, characterised in that when manufacturing the component (l) a compound of the formula 40246/2 is used as the 1,3,5-triazine, v/herein denotes amino, hydroxyl or hydrogen and R2 denotes amino, hydroxyl, hydrogen, methyl, phenyl or l-dialkylphosphono-(allyl)n_^, with n "being 1 or 2. 26. Process according to Claim 25, characterised in that when manufacturing the component (l a compound of the formula - I N I II is used as the 1,3,5-triazine, wherein denotes amino or hydroxyl and denotes amino , hydroxyl, hydrogen or 1-diethyl-phosphonoethyl. 27. Process according to claim 26, characterised in that v/hen manufacturing the component (l) the 1,3,5-triazine used is l-diethylphosphonoethyl-1,3 ,5-triazine or preferably melamine. 28. Process according to one of Claims 16 to 2 , characterised in that when manufacturing the component (l), after completion of the reaction, the salts of. the condensation products are converted into the corresponding hydroxides. 40246/2 29· Process according to Claim 23 characterized in that a methylolurea or a methylolmelamine is used as the component (2). 30. Process according to one of Claims 16 to 29» characterized in that fibre material of polyamides , cellulose, cellulose-polyester or polyester is flameproofed. 31. Process according to Claim 30, characterized in that fabrics of wool or polyester or mixed fabrics of polyester-cellulose are flameproofed. 32· Process according^ to one of Claims 15 to 31f characterized in that the fibre material is dried at temperatures of up to 100°C and subjected to a heat treatment at above 100°C, 33? t e organic fibre materials provided with a flameproof finish by the process according to one of Claims 15 to 32. 34. The aqueous preparations used for carrying out the process according to one of Claims 15 to 32.
IL40246A 1972-01-14 1972-08-29 The manufacture of phosphorus-containing condensation products,the products and their use as flameproofing agents IL40246A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CH52172 1972-01-14

Publications (2)

Publication Number Publication Date
IL40246A0 IL40246A0 (en) 1972-10-29
IL40246A true IL40246A (en) 1976-06-30

Family

ID=4188903

Family Applications (1)

Application Number Title Priority Date Filing Date
IL40246A IL40246A (en) 1972-01-14 1972-08-29 The manufacture of phosphorus-containing condensation products,the products and their use as flameproofing agents

Country Status (18)

Country Link
US (1) US3887553A (en)
JP (1) JPS4880896A (en)
AR (1) AR199880A1 (en)
AT (1) AT317837B (en)
AU (1) AU470571B2 (en)
BE (1) BE788595A (en)
BR (1) BR7206195D0 (en)
CA (1) CA981677A (en)
CH (2) CH52172A4 (en)
CS (1) CS158744B2 (en)
DE (1) DE2242714A1 (en)
FR (1) FR2167497B1 (en)
GB (1) GB1388604A (en)
IL (1) IL40246A (en)
IT (1) IT972347B (en)
NL (1) NL7212267A (en)
SU (1) SU529811A3 (en)
ZA (1) ZA725954B (en)

Families Citing this family (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3994971A (en) * 1971-09-10 1976-11-30 Ciba-Geigy Corporation Phosphorus-containing condensation products
US4020224A (en) * 1974-07-22 1977-04-26 Monsanto Research Corporation Flame retardant method
US3989702A (en) * 1974-07-22 1976-11-02 Monsanto Research Corporation Flame retardant
CA1032941A (en) * 1974-12-10 1978-06-13 Encoat Chemicals Limited Substituted ammonium polyphosphate composition
GB8702055D0 (en) * 1987-01-30 1987-03-04 Albright & Wilson Wood treatment process
US4927929A (en) * 1988-08-01 1990-05-22 Synthetic Products Company Melamine salts of alkyl acid phosphates
US5047458A (en) * 1988-08-01 1991-09-10 Synthetic Products Company Melamine salts of alkyl acid phosphates as flame retardants for polymers

Family Cites Families (10)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
NL83058C (en) * 1952-04-22
US2809941A (en) * 1952-04-22 1957-10-15 Wilson A Reeves Producing phosphorus containing amino resins and flameproofing organic textiles
US2772188A (en) * 1953-11-18 1956-11-27 Wilson A Reeves Ammonia insolubilized methylol-phosphorus polymers and cellulosic materials impregnated therewith
US2911322A (en) * 1957-10-29 1959-11-03 Klein Elias Field treatment for making cellulosic fabrics flameproof and resistant to certain chemical warfare gases
US2993746A (en) * 1959-03-27 1961-07-25 Thomas D Miles Treatment of thpc flame-resistant fabrics with strong mineral acids to improve theirtear strength and products produced thereby
NL129265C (en) * 1959-10-05 1900-01-01
CH418289A (en) * 1964-07-10 1967-02-15 Ciba Geigy Process for simultaneously making cellulose-containing textiles flame-proof and rot-proof
US3551422A (en) * 1968-03-27 1970-12-29 Stevens & Co Inc J P N-(oxymethyl) derivatives of phosphonopolyamino-s-triazines
CH501093A (en) * 1968-07-09 1970-08-14 Ciba Geigy Ag Process for making cellulose-containing textile materials flame-resistant
US3654274A (en) * 1970-06-09 1972-04-04 Us Agriculture Phosphorus-containing triazines

Also Published As

Publication number Publication date
IL40246A0 (en) 1972-10-29
IT972347B (en) 1974-05-20
AR199880A1 (en) 1974-10-08
JPS4880896A (en) 1973-10-29
DE2242714A1 (en) 1973-07-19
BR7206195D0 (en) 1973-09-25
NL7212267A (en) 1973-07-17
FR2167497B1 (en) 1977-08-05
CS158744B2 (en) 1974-11-25
US3887553A (en) 1975-06-03
CH546297A (en) 1974-02-28
CA981677A (en) 1976-01-13
BE788595A (en) 1973-03-08
SU529811A3 (en) 1976-09-25
CH52172A4 (en) 1973-05-15
AT317837B (en) 1974-09-10
FR2167497A1 (en) 1973-08-24
AU4619672A (en) 1974-03-07
GB1388604A (en) 1975-03-26
ZA725954B (en) 1973-06-27
AU470571B2 (en) 1976-03-18

Similar Documents

Publication Publication Date Title
US3832227A (en) Use of triazinylaminoalkyl phosphonates for the flameproofing of textiles
US3878245A (en) Process for the manufacture of phosphorus-containing condensation products, the products and their use as flameproofing agents
IL40246A (en) The manufacture of phosphorus-containing condensation products,the products and their use as flameproofing agents
US3763281A (en) Ureidoalkylphosphonates
HUT57294A (en) Method for treating clothes
IL40238A (en) The manufacture of phosphorus-containing condensation products,the products and their use as flameproofing agents
US4148602A (en) Phosphoramide-hydroxymethyl phosphine condensation products for textile fire retardation
US3864076A (en) Process for flameproofing organic fibers with phosphorus-containing condensation products and the products produced
US3619113A (en) Flame-retardant finish for cellulosic textile materials
US2785145A (en) Siliconate-aminoplast compositions and textiles coated therewith
US3079279A (en) Blends of imidazolidinones and aminoplasts and method for finishing cellulose containing textile material
US3931310A (en) Phosphorus-containing condensation products
US3082118A (en) Novel mercurated acrylamide compounds and germicidal textile finishes
US3903336A (en) Use of phosphorus-containing condensation products as flameproofing agents for fibre mixtures of polyester and cellulose
US3994971A (en) Phosphorus-containing condensation products
US4044006A (en) Oxazine containing ureidoalkylphosphonates
US4145547A (en) Ureidoalkylphosphonates and their use for the flameproofing of textiles
IL40236A (en) Manufacture of condensation products containing phosphorus,the products and their use as flameproofing agents
US3907898A (en) Process for the manufacture of polycondensation products containing phosphorus, the products and their use as flameproofing agents
US4020262A (en) Method of applying phosphoramide-hydroxymethyl phosphine condensation products for textile fire retardation
US3671611A (en) Phosphorus acid esters
US3874911A (en) Process for the manufacture of phosphorus-containing condensation products, the products and their use as flameproofing agents
IL40241A (en) The manufacture of phosphorus-containing condensation products,the products and their use as flameproofing agents
IL40242A (en) The manufacture of phosphorus-containing condensation products,the products and their use as flameproofing agents
IL40239A (en) The manufacture of phosphorus-containing condensation products,the products and their use as flameproofing agents