GB579303A - Improvements relating to the production of cyclic amidines or salts thereof - Google Patents
Improvements relating to the production of cyclic amidines or salts thereofInfo
- Publication number
- GB579303A GB579303A GB1027744A GB1027744A GB579303A GB 579303 A GB579303 A GB 579303A GB 1027744 A GB1027744 A GB 1027744A GB 1027744 A GB1027744 A GB 1027744A GB 579303 A GB579303 A GB 579303A
- Authority
- GB
- United Kingdom
- Prior art keywords
- benzenesulphonate
- oxime
- benzene
- extracted
- general formula
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Expired
Links
Landscapes
- Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
- Hydrogenated Pyridines (AREA)
Abstract
Amidines of the general formula:-<FORM:0579303/IV/1> or salts thereof, wherein R represents a chain of methylene or alkyl substituted methylene radicals and R1 and R2 are each a hydrocarbon radical or hydrogen, or one is a hydrocarbon radical and the other a hydrogen atom, are produced (a) by reaction of ammonia or a primary or secondary amine with a sulphonic ester of the general formula:- <FORM:0579303/IV/2> where R has the significance above and X is a hydrocarbon radical. The sulphonic ester is obtained by reaction of: (a) a lactam having the general formula:- <FORM:0579303/IV/3> or (b) a ketoxime of the general formula:- <FORM:0579303/IV/4> with a sulphonyl halide, R again representing a chain of methylene or alkyl-substituted methylene radicals. In examples: (1) benzenesulphonyl chloride is added to cyclohexanone oxime in 2.25 N. sodium hydroxide and acetone and the oxime benzenesulphonate is extracted with benzene and treated with aniline prior to adding caustic soda to liberate 2-phenyliminohexamethylene imine; (2) e -caprolactam in pyridine-benzene is stirred with benzene-sulphonyl chloride at room temperature and aniline is added, 2-phenyliminohexamethyleneimine being isolated from the aqueous extract as in (1); (3) 2-phenyl cyclopentanone is added to hydroxylamine hydrochloride in 4.45 N. sodium hydroxide and the resulting solution of sodium cyclopentanone oxime is cooled to about - 5 DEG C., benzenesulphonyl chloride is added, cyclopentanone oxime benzenesulphonate is benzene-extracted and reaction with aniline is effected prior to isolating 2-phenyliminopiperidine on adding caustic soda (4) cyclopentanone oxime benzenesulphonate prepared as in (3) is extracted with nitrobenzene ammonia being introduced into the stirred solution, and on warming to 80 DEG C. an exothermic reaction is initiated and 2-iminopiperidine benzenesulphonate is crystallized from the mixture; (5) cyclohexanone oxime benzenesulphonate prepared as in (4) is extracted with nitrobenzene, ammonia is introduced and the mother liquor, evaporated to dryness in vacuo, yields 2-iminohexamethyleneimine benzenesulphonate.
Priority Applications (1)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
GB1027744A GB579303A (en) | 1944-05-26 | 1944-05-26 | Improvements relating to the production of cyclic amidines or salts thereof |
Applications Claiming Priority (1)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
GB1027744A GB579303A (en) | 1944-05-26 | 1944-05-26 | Improvements relating to the production of cyclic amidines or salts thereof |
Publications (1)
Publication Number | Publication Date |
---|---|
GB579303A true GB579303A (en) | 1946-07-30 |
Family
ID=9964878
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
GB1027744A Expired GB579303A (en) | 1944-05-26 | 1944-05-26 | Improvements relating to the production of cyclic amidines or salts thereof |
Country Status (1)
Country | Link |
---|---|
GB (1) | GB579303A (en) |
Cited By (1)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
EP0212479A1 (en) * | 1985-08-20 | 1987-03-04 | Bayer Ag | Use of lactam amides as efficiency improvers in animals |
-
1944
- 1944-05-26 GB GB1027744A patent/GB579303A/en not_active Expired
Cited By (1)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
EP0212479A1 (en) * | 1985-08-20 | 1987-03-04 | Bayer Ag | Use of lactam amides as efficiency improvers in animals |
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