EP1047083A1 - A neutron amplifier assembly - Google Patents

A neutron amplifier assembly Download PDF

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Publication number
EP1047083A1
EP1047083A1 EP19990107327 EP99107327A EP1047083A1 EP 1047083 A1 EP1047083 A1 EP 1047083A1 EP 19990107327 EP19990107327 EP 19990107327 EP 99107327 A EP99107327 A EP 99107327A EP 1047083 A1 EP1047083 A1 EP 1047083A1
Authority
EP
European Patent Office
Prior art keywords
neutron
cylinder
layer
fissile material
assembly according
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Granted
Application number
EP19990107327
Other languages
German (de)
French (fr)
Other versions
EP1047083B1 (en
Inventor
Joseph Magill
Paolo Peerani
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
European Community
Original Assignee
EUROPEAN COMMUNITY
European Community EC Luxemburg
European Economic Community
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Priority to AT99107327T priority Critical patent/ATE246394T1/en
Application filed by EUROPEAN COMMUNITY, European Community EC Luxemburg, European Economic Community filed Critical EUROPEAN COMMUNITY
Priority to PT99107327T priority patent/PT1047083E/en
Priority to ES99107327T priority patent/ES2204023T3/en
Priority to DK99107327T priority patent/DK1047083T3/en
Priority to EP99107327A priority patent/EP1047083B1/en
Priority to DE69909962T priority patent/DE69909962T2/en
Priority to JP2000612962A priority patent/JP2002542496A/en
Priority to CA002368547A priority patent/CA2368547A1/en
Priority to PCT/EP2000/003179 priority patent/WO2000063921A1/en
Publication of EP1047083A1 publication Critical patent/EP1047083A1/en
Priority to NO20014840A priority patent/NO20014840L/en
Application granted granted Critical
Publication of EP1047083B1 publication Critical patent/EP1047083B1/en
Priority to US10/698,459 priority patent/US20040228433A1/en
Anticipated expiration legal-status Critical
Expired - Lifetime legal-status Critical Current

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    • GPHYSICS
    • G21NUCLEAR PHYSICS; NUCLEAR ENGINEERING
    • G21GCONVERSION OF CHEMICAL ELEMENTS; RADIOACTIVE SOURCES
    • G21G4/00Radioactive sources
    • G21G4/02Neutron sources

Definitions

  • This invention refers to a neutron amplifier assembly comprising a slightly subcritical array of fissile material which is subjected to a primary neutron flux.
  • a neutron flux is used not only for research purposes but also for irradiating goods, for cancer treatment and even for controlling a nuclear power generator.
  • a high neutron intensity above 10 17 s -1 would be useful for many purposes.
  • Such a high flux is beyond the practical possibilities of modern accelerators, even in combination with a spallation target. It is therefore an object of the present invention to provide a neutron amplifier assembly which supplies an intense and readily controllable neutron flux.
  • Figure 1 shows schematically in cross-section a first embodiment of the assembly according to the invention.
  • Figure 3 shows a variant which is conceived to produce a high flux of fast neutrons.
  • Figure 4 is an improved embodiment with two subcritical arrays in series.
  • the fissile material is Am 242m .
  • This material constitutes a thin layer 1 on the inner surface of a hollow cylinder 2 of circular cross-section, made of a neutron moderator material such as graphite or beryllium.
  • a spallation target 3 is located which is intended to receive a proton beam from an accelerator (not shown) along the axial direction of the cylinder 2.
  • the cylinder height and its inner diameter are both 1 m, the diameter of the target 3 being 30 cm.
  • the thickness of the layer 1 is in the micrometer range and will be specified later. This thickness depends upon the type of fissile material and its concentration in this layer. In any case it must be sufficiently small in order to allow fast neutrons to pass there-through without interaction, whereas thermal neutrons are trapped.
  • Neutrons starting from the target 3 may be either thermal or fast neutrons.
  • Thermal neutrons react immediately with the layer 1 and generate fast neutrons whereas fast neutrons pass there-through without interaction. In both cases fast neutrons penetrate into the graphite cylinder 2 and become thermalized. If these neutrons penetrate again into the layer 1 they cause more fissions. Those which escape from the cylinder at its outside constitute the output of the amplifier assembly.
  • the thickness of the fissile material layer on the inner surface of the graphite cylinder should be such that the arrangement does not become critical, but a criticality factor k eff close to 1 should be achieved in order to enhance the neutron amplification gain.
  • the arrangement will be subcritical. If for example the criticality factor k eff is 0.95 then its neutron amplification factor will become 20.
  • the invention is not restricted to the embodiment described above.
  • the invention is also applicable to materials others than pure fissile materials, in which the fissile material is present in the layer at a substantially reduced amount.
  • the neutron source can instead of a spallation target consist of a neutron emitter such as Californium.
  • the cylinder 2 is not necessarily of circular cross-section as shown in the drawings.
  • the cross-section might be square or present an inner corrugated shape like a star. In this latter case the overall diameter of the cylinder 2 can be reduced whilst maintaining the same surface area of fissile material.
  • the heat production in the arrangement is rather low: Taking the above cited example of a 150 MeV accelerator supplying a proton current of 2 mA (corresponding to 300 kW power output) and a neutron amplification factor of 20 due to the layer 1 of fissile material, the neutron intensity will become about 2,5 ⁇ 10 17 s -1 . Since the neutron generation rate is approximately equal to the rate of fissioning, the maximum heat generation rate is about 8 MW. This heat can be easily extracted through coolant channels in the graphite cylinder.
  • the arrangement according to figure 1 should be completed, as shown in figure 3, by a further layer 4 of fissile material on the outer surface of the graphite cylinder 2 and optionally by a metal casing 5 around this layer, especially made of tungsten.
  • This second layer 4 is again transparent to fast neutrons as it interacts only with neutrons which have been thermalized in the graphite cylinder. These neutrons cause fissions which result in fast neutrons. A part of these fast neutrons escapes through the casing whereas others return into the graphite cylinder and cause further fissions in one of the layers of fissile materials.
  • two or more layers of fissile material are located, preferably in a concentric axial configuration, between the spallation target and the inner diameter of the graphite cylinder.
  • a concentric axial configuration between the spallation target and the inner diameter of the graphite cylinder.
  • one additional layer 6 of fissile material is added which is either self-supporting or deposited on a metal tube, for example made of tungsten (not shown).
  • one or more moderator rods can be inserted in a controlled manner into the free space inside the graphite cylinder. This insertion increases the criticality factor and allows a fine control of the neutron amplification factor and of the criticality factor, in order to take into account inhomogeneities of the thin layers and their burn-up.

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  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Physics & Mathematics (AREA)
  • Engineering & Computer Science (AREA)
  • General Engineering & Computer Science (AREA)
  • High Energy & Nuclear Physics (AREA)
  • Chemical & Material Sciences (AREA)
  • Particle Accelerators (AREA)
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  • Tires In General (AREA)
  • Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
  • Semiconductor Lasers (AREA)
  • Monitoring And Testing Of Nuclear Reactors (AREA)

Abstract

This invention relates to a neutron amplifier assembly comprising an array of fissile material which is subjected to a primary neutron flux.
According to the invention a thin layer (1) of fissile material is located on the inner surface of a hollow support cylinder (2) of moderator material, the fissile material layer thickness and the inner diameter of said cylinder being chosen such that the array is close to criticality.

Description

  • This invention refers to a neutron amplifier assembly comprising a slightly subcritical array of fissile material which is subjected to a primary neutron flux.
  • A neutron flux is used not only for research purposes but also for irradiating goods, for cancer treatment and even for controlling a nuclear power generator. For example, a high neutron intensity above 1017 s-1 would be useful for many purposes. Such a high flux is beyond the practical possibilities of modern accelerators, even in combination with a spallation target. It is therefore an object of the present invention to provide a neutron amplifier assembly which supplies an intense and readily controllable neutron flux.
  • This object is achieved according to the invention by the neutron amplifier assembly as defined in claim 1. For further improvements of this assembly reference is made to the secondary claims.
  • The invention will now be described in detail by means of some preferred embodiments and the enclosed drawings.
  • Figure 1 shows schematically in cross-section a first embodiment of the assembly according to the invention.
  • Figure 2 shows the relation between the mass and layer thickness of fissile material in the hollow cylindrical arrangement of given dimensions for keff = 1.
  • Figure 3 shows a variant which is conceived to produce a high flux of fast neutrons.
  • Figure 4 is an improved embodiment with two subcritical arrays in series.
  • According to a first embodiment shown in figure 1, the fissile material is Am242m. This material constitutes a thin layer 1 on the inner surface of a hollow cylinder 2 of circular cross-section, made of a neutron moderator material such as graphite or beryllium. Along the axis of this cylinder a spallation target 3 is located which is intended to receive a proton beam from an accelerator (not shown) along the axial direction of the cylinder 2. As an example, the cylinder height and its inner diameter are both 1 m, the diameter of the target 3 being 30 cm.
  • The thickness of the layer 1 is in the micrometer range and will be specified later. This thickness depends upon the type of fissile material and its concentration in this layer. In any case it must be sufficiently small in order to allow fast neutrons to pass there-through without interaction, whereas thermal neutrons are trapped.
  • Neutrons starting from the target 3 may be either thermal or fast neutrons.
  • Thermal neutrons react immediately with the layer 1 and generate fast neutrons whereas fast neutrons pass there-through without interaction. In both cases fast neutrons penetrate into the graphite cylinder 2 and become thermalized. If these neutrons penetrate again into the layer 1 they cause more fissions. Those which escape from the cylinder at its outside constitute the output of the amplifier assembly.
  • It should be noted that the thickness of the fissile material layer on the inner surface of the graphite cylinder should be such that the arrangement does not become critical, but a criticality factor keff close to 1 should be achieved in order to enhance the neutron amplification gain.
  • The tables following here-after show, for a cylinder having an inner diameter  equal to its height, the thickness of a layer of Am242m and U235 respectively required for various inner cylinder diameters  necessary to make the system critical.
     (cm) critical thickness (cm) critical mass (kg)
    10 0.4 2.6
    20 0.063 1.6
    30 0.005 0.25
    40 0.001 0.1
    60 0.0004 0.08
    Table 1. Layer thickness of Am242m metal and corresponding mass required for criticality for various cylinder diameters .
     (cm) critical thickness (cm) critical mass (kg)
    10 2 14
    20 0.8 20
    40 0.15 14
    60 0.023 5
    100 0.007 4
    Table 2. Layer thickness of U235 metal and corresponding mass required for criticality for various cylinder diameters .
  • These values are also represented in the plot of Figure 2 as small circles and crosses respectively. One can for example deduce there-from that criticality is obtained with an Am242m layer thickness of 4 µm on the inner surface (diameter 60 cm) of a graphite cylinder (axial length 60 cm). The overall critical mass of fissile material is under these circumstances only 80 g which is considerably less than the (bare) critical mass of a solid spere of the same material (4.7 kg).
  • Thus if a thickness below 4 pm is chosen then the arrangement will be subcritical. If for example the criticality factor keff is 0.95 then its neutron amplification factor will become 20.
  • A commercial cyclotron supplying a proton beam of 150 MeV produces in a lead spallation target about 1 neutron per proton. Due to the layer of fissile material this neutron produces on average M neutrons where M ≈ 1/(1 - keff). For the case of keff= 0.95, M is approximately 20.
  • The invention is not restricted to the embodiment described above. One could employ other fissile materials, such as U235 (see table 2 and figure 2). It should further be noted that the invention is also applicable to materials others than pure fissile materials, in which the fissile material is present in the layer at a substantially reduced amount.
  • It is also possible to cover the inner layer 1 of fissile material with a layer of moderator material in order to reduce damages in the fissile material layer due to high energy neutrons.
  • The neutron source can instead of a spallation target consist of a neutron emitter such as Californium.
  • The cylinder 2 is not necessarily of circular cross-section as shown in the drawings. In fact, the cross-section might be square or present an inner corrugated shape like a star. In this latter case the overall diameter of the cylinder 2 can be reduced whilst maintaining the same surface area of fissile material.
  • The heat production in the arrangement is rather low: Taking the above cited example of a 150 MeV accelerator supplying a proton current of 2 mA (corresponding to 300 kW power output) and a neutron amplification factor of 20 due to the layer 1 of fissile material, the neutron intensity will become about 2,5·1017 s-1. Since the neutron generation rate is approximately equal to the rate of fissioning, the maximum heat generation rate is about 8 MW. This heat can be easily extracted through coolant channels in the graphite cylinder.
  • In case that not a thermal neutron flux but a fast neutron flux is desired, the arrangement according to figure 1 should be completed, as shown in figure 3, by a further layer 4 of fissile material on the outer surface of the graphite cylinder 2 and optionally by a metal casing 5 around this layer, especially made of tungsten. This second layer 4 is again transparent to fast neutrons as it interacts only with neutrons which have been thermalized in the graphite cylinder. These neutrons cause fissions which result in fast neutrons. A part of these fast neutrons escapes through the casing whereas others return into the graphite cylinder and cause further fissions in one of the layers of fissile materials.
  • According to a further improvement of the present invention two or more layers of fissile material are located, preferably in a concentric axial configuration, between the spallation target and the inner diameter of the graphite cylinder. Such an example is sketched in figure 4. Here, one additional layer 6 of fissile material is added which is either self-supporting or deposited on a metal tube, for example made of tungsten (not shown).
  • As a further improvement, one or more moderator rods (not shown) can be inserted in a controlled manner into the free space inside the graphite cylinder. This insertion increases the criticality factor and allows a fine control of the neutron amplification factor and of the criticality factor, in order to take into account inhomogeneities of the thin layers and their burn-up.

Claims (7)

  1. A neutron amplifier assembly comprising an array of fissile material which is subjected to a primary neutron flux, characterized by a thin layer (1) of fissile material on the inner surface of a hollow support cylinder (2) of moderator material, the fissile material layer thickness and the inner diameter of said cylinder being chosen such that the array is close to criticality.
  2. An assembly according to claim 1, characterized in that at least one further thin cylindrical layer (5) of fissile material is placed in said cylinder at a distance from the previous layer (1), its diameter and thickness being chosen such that the overall configuration constitutes again a nearly critical array.
  3. An assembly according to claim 1, characterized in that the primary neutron flux is generated by a neutron emitter situated in the centre of the assembly.
  4. An assembly according to claim 3, characterized in that the neutron emitter is constituted by a spallation target (3) intended to be bombarded by accelerated particles.
  5. An assembly according to any one of the preceding claims, characterized in that the hollow cylinder (2) is made from graphite.
  6. An assembly according to any one of the preceding claims, characterized in that the hollow cylinder (2) is surrounded by a layer (4) of fissile material.
  7. An assembly according to any one of the preceding claims, characterized in that at least one moderator material rod is movably inserted into the free space in the hollow cylinder (2).
EP99107327A 1999-04-20 1999-04-20 A neutron amplifier assembly Expired - Lifetime EP1047083B1 (en)

Priority Applications (11)

Application Number Priority Date Filing Date Title
PT99107327T PT1047083E (en) 1999-04-20 1999-04-20 NEUTRAL AMPLIFIER STRUCTURE
ES99107327T ES2204023T3 (en) 1999-04-20 1999-04-20 NEUTRON AMPLIFIER ASSEMBLY.
DK99107327T DK1047083T3 (en) 1999-04-20 1999-04-20 neutron
EP99107327A EP1047083B1 (en) 1999-04-20 1999-04-20 A neutron amplifier assembly
DE69909962T DE69909962T2 (en) 1999-04-20 1999-04-20 Neutronverstärkersanlage
AT99107327T ATE246394T1 (en) 1999-04-20 1999-04-20 NEUTRON AMPLIFIER SYSTEM
JP2000612962A JP2002542496A (en) 1999-04-20 2000-04-10 Neutron amplifier assembly
CA002368547A CA2368547A1 (en) 1999-04-20 2000-04-10 A neutron amplifier assembly
PCT/EP2000/003179 WO2000063921A1 (en) 1999-04-20 2000-04-10 A neutron amplifier assembly
NO20014840A NO20014840L (en) 1999-04-20 2001-10-04 Nöytronforsterkerenhet
US10/698,459 US20040228433A1 (en) 1999-04-20 2003-11-03 Neutron amplifier assembly

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
EP99107327A EP1047083B1 (en) 1999-04-20 1999-04-20 A neutron amplifier assembly

Publications (2)

Publication Number Publication Date
EP1047083A1 true EP1047083A1 (en) 2000-10-25
EP1047083B1 EP1047083B1 (en) 2003-07-30

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ID=8237956

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Application Number Title Priority Date Filing Date
EP99107327A Expired - Lifetime EP1047083B1 (en) 1999-04-20 1999-04-20 A neutron amplifier assembly

Country Status (10)

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EP (1) EP1047083B1 (en)
JP (1) JP2002542496A (en)
AT (1) ATE246394T1 (en)
CA (1) CA2368547A1 (en)
DE (1) DE69909962T2 (en)
DK (1) DK1047083T3 (en)
ES (1) ES2204023T3 (en)
NO (1) NO20014840L (en)
PT (1) PT1047083E (en)
WO (1) WO2000063921A1 (en)

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB2625606A (en) * 2022-11-02 2024-06-26 Aurelia Lumina Ltd Power source

Families Citing this family (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP7074615B2 (en) * 2018-08-27 2022-05-24 株式会社東芝 Neutron supply device and neutron supply method

Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB850876A (en) * 1957-04-24 1960-10-12 Dow Chemical Co Neutron amplifier
US3778627A (en) * 1973-04-17 1973-12-11 Atomic Energy Commission High intensity, pulsed thermal neutron source
SU786619A1 (en) * 1979-07-16 1991-08-15 Предприятие П/Я Г-4665 Two-stage multiplier of neutrons
WO1995024043A1 (en) * 1994-03-04 1995-09-08 Ion Beam Applications S.A. Method for producing thermal neutrons, device therefor, and use thereof for producing radioisotopes

Patent Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB850876A (en) * 1957-04-24 1960-10-12 Dow Chemical Co Neutron amplifier
US3778627A (en) * 1973-04-17 1973-12-11 Atomic Energy Commission High intensity, pulsed thermal neutron source
SU786619A1 (en) * 1979-07-16 1991-08-15 Предприятие П/Я Г-4665 Two-stage multiplier of neutrons
WO1995024043A1 (en) * 1994-03-04 1995-09-08 Ion Beam Applications S.A. Method for producing thermal neutrons, device therefor, and use thereof for producing radioisotopes

Non-Patent Citations (1)

* Cited by examiner, † Cited by third party
Title
DATABASE WPI Week 9220, Derwent World Patents Index; AN 92-164686, XP002116849 *

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB2625606A (en) * 2022-11-02 2024-06-26 Aurelia Lumina Ltd Power source

Also Published As

Publication number Publication date
NO20014840D0 (en) 2001-10-04
CA2368547A1 (en) 2000-10-26
DE69909962T2 (en) 2004-05-27
EP1047083B1 (en) 2003-07-30
ES2204023T3 (en) 2004-04-16
ATE246394T1 (en) 2003-08-15
WO2000063921A1 (en) 2000-10-26
JP2002542496A (en) 2002-12-10
DE69909962D1 (en) 2003-09-04
DK1047083T3 (en) 2003-11-24
NO20014840L (en) 2001-10-04
PT1047083E (en) 2003-12-31

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