EP0865652B1 - Container with a radioactive body - Google Patents
Container with a radioactive body Download PDFInfo
- Publication number
- EP0865652B1 EP0865652B1 EP96939924A EP96939924A EP0865652B1 EP 0865652 B1 EP0865652 B1 EP 0865652B1 EP 96939924 A EP96939924 A EP 96939924A EP 96939924 A EP96939924 A EP 96939924A EP 0865652 B1 EP0865652 B1 EP 0865652B1
- Authority
- EP
- European Patent Office
- Prior art keywords
- container
- zeolite
- fill
- activated charcoal
- fuel rods
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Expired - Lifetime
Links
Images
Classifications
-
- G—PHYSICS
- G21—NUCLEAR PHYSICS; NUCLEAR ENGINEERING
- G21F—PROTECTION AGAINST X-RADIATION, GAMMA RADIATION, CORPUSCULAR RADIATION OR PARTICLE BOMBARDMENT; TREATING RADIOACTIVELY CONTAMINATED MATERIAL; DECONTAMINATION ARRANGEMENTS THEREFOR
- G21F1/00—Shielding characterised by the composition of the materials
-
- G—PHYSICS
- G21—NUCLEAR PHYSICS; NUCLEAR ENGINEERING
- G21F—PROTECTION AGAINST X-RADIATION, GAMMA RADIATION, CORPUSCULAR RADIATION OR PARTICLE BOMBARDMENT; TREATING RADIOACTIVELY CONTAMINATED MATERIAL; DECONTAMINATION ARRANGEMENTS THEREFOR
- G21F5/00—Transportable or portable shielded containers
- G21F5/005—Containers for solid radioactive wastes, e.g. for ultimate disposal
-
- Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
- Y10S—TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
- Y10S422/00—Chemical apparatus and process disinfecting, deodorizing, preserving, or sterilizing
- Y10S422/903—Radioactive material apparatus
Definitions
- Containers with radioactive bodies are, for example, from the US-A-4 950 426 is known. However, this document contains predominantly only indications of slight or at most moderate radiant waste.
- Fuel rods that contain radioactive nuclear fuel in one contain a sealing tube which represents a capsule, to be filled with copper granulate between the fuel rods and then around the nuclear reactor fuel element at high temperatures and high pressure a gas-tight container to be made of copper sheet.
- This sealed gastight Container is placed in a well in a repository, that is in granite and that with bentonite clay filled as a barrier against radioactive emitters (radionuclides) becomes.
- the copper granulate in the copper sheet container is said to give this container mechanical stability.
- the invention has for its object the retention that way for radioactive emitters (Radionuclides) formed barriers (i.e. the cladding tubes of the Fuel rods and the container).
- the bed of zeolite and / or activated carbon in the container also leaves enough empty volume to accommodate vacant ones Noble gases, so that there is no high internal pressure in the container can train. Nevertheless, the bed of zeolite and / or activated carbon sufficient thermal conductivity for removal of post-decay heat from the fuel rods. Also poses the fill an additional heat capacity in the container
- the bed, especially if it contains activated carbon, also has a good moderating effect on neutrons and therefore reduces the hardness of neutron radiation from the radioactive substance in the fuel rods can go out. Also for shielding gamma radiation from the fuel rods runs out, the bulk can contribute, finally the bed also provides a mechanical buffer for the fuel rods stored in the container.
- This nuclear reactor fuel element 3 has fuel rods 4 and guide tubes 5.
- the fuel rods 4 are filled with spent nuclear fuel, for example UO 2 and / or U / PuO 2 , which contains radionuclides.
- This nuclear fuel is in each case in a cladding tube of the fuel rods 4, for example made of a zirconium alloy, which is closed at both tube ends with a plug made of zirconium alloy. These zirconium alloy plugs are welded gas-tight to the cladding tube.
- the guide tubes 5 were used to guide control rods and are open at at least one tube end. They do not contain radionuclides.
- the storage container 2 is made of a granulate 6 a zeolite filled up. This bed 6 does not need to be compressed, and with it are the fuel rods 4 and inevitably the guide tubes 5 of the nuclear reactor fuel element 3 backfilled.
- the container 2 is made of steel and is gas-tight welded to both ends with a steel plate.
- Figure 2 is the container 2 which is the nuclear reactor fuel element 3 with the spent fuel rods in a hole used, for example, in a salt dome a repository. Is located in this hole the outside of the container 2 a further bed 7, the is also granules of a zeolite. In this bed 7 the container 2 is completely embedded.
- the beds 6 and 7 made of zeolite in FIGS. 1 and 2 activated carbon can also be added. Zeolites turn into Ullmann's "Encyclopedia of Technical Chemistry", volume 24, pages 575 to 578, 1983, and on Ullmann's "Encyclopedia of Technischen Chemie”, volume 17, pages 9 to 17, 1979. Zeolite is particularly suitable for the beds 6 and 7 of type A, preferably at least one of the substances MgA, CaA and SrA.
- Such a type A zeolite can also be used with silver be doped so that it is particularly good radioactive iodine holds back, possibly from a leak in the cladding tube Fuel rod 4 emerges, but then in front of the wall of the Container 2 is retained, the retention effect by the zeolite of the bed 6 in the container 2 is thus reinforced is.
- Chabazite are also well suited for zeolite fillings and mordenite.
- Zeolites, for example, are particularly suitable with the trade name "Zeolon Molecular Sieves" the 400 Series, 500 Series, 700 Series and 900 Series that bind Cs and Sr via ion exchange.
Landscapes
- Physics & Mathematics (AREA)
- Engineering & Computer Science (AREA)
- General Engineering & Computer Science (AREA)
- High Energy & Nuclear Physics (AREA)
- Filling Or Discharging Of Gas Storage Vessels (AREA)
- Solid-Sorbent Or Filter-Aiding Compositions (AREA)
- Medical Preparation Storing Or Oral Administration Devices (AREA)
Description
Behälter mit radioaktiven Körpern sind beispielsweise aus der US-A-4 950 426 bekannt. In diesem Dokument finden sich aber überwiegend nur Hinweise auf leicht oder allenfalls mittelstark strahlenden Abfall.Containers with radioactive bodies are, for example, from the US-A-4 950 426 is known. However, this document contains predominantly only indications of slight or at most moderate radiant waste.
Es ist bekannt, ein abgebranntes Kernreaktorbrennelement mit Brennstäben, die radioaktiven Kernbrennstoff in einem eine dichtverschlossene Kapsel darstellenden Hüllrohr enthalten, mit Kupfergranulat zwischen den Brennstäben zu verfüllen und anschließend um das Kernreaktorbrennelement bei hohen Temperaturen und hohem Druck einen gasdicht verschlossenen Behälter aus Kupferblech anzubringen. Dieser gasdicht verschlossene Behälter wird in einem Endlager in ein Bohrloch eingebracht, das sich in Granit befindet und das mit Bentonit-Lehm als Barriere gegen radioaktive Strahler (Radionuklide) zugefüllt wird. Das Kupfergranulat in dem Behälter aus Kupferblech soll diesem Behälter mechanische Stabilität verleihen.It is known to have a spent nuclear reactor fuel element Fuel rods that contain radioactive nuclear fuel in one contain a sealing tube which represents a capsule, to be filled with copper granulate between the fuel rods and then around the nuclear reactor fuel element at high temperatures and high pressure a gas-tight container to be made of copper sheet. This sealed gastight Container is placed in a well in a repository, that is in granite and that with bentonite clay filled as a barrier against radioactive emitters (radionuclides) becomes. The copper granulate in the copper sheet container is said to give this container mechanical stability.
Der Erfindung liegt die Aufgabe zugrunde, das Rückhaltevermögen der auf diese Weise für radioaktive Strahler (Radionuklide) gebildeten Barrieren (d.h. der Hüllrohre der Brennstäbe und des Behälters) zu verbessern.The invention has for its object the retention that way for radioactive emitters (Radionuclides) formed barriers (i.e. the cladding tubes of the Fuel rods and the container).
Diese Aufgabe löst ein erfindungsgemäß gasdicht verschlossener Behälter gemäß Patentanspruch 1, in dem mehrere abgebrannte Brennstäbe in einer Schüttung aus Zeolith und/oder Aktivkohle eingebettet sind.This object is achieved by a gas-tight closure according to the invention Container according to claim 1, in which several spent fuel rods in one Bed of zeolite and / or activated carbon are embedded.
Zeolith und Aktivkohle ab- bzw. adsorbieren - abgesehen von Edelgasen - nicht- bzw. leicht flüchtige Radionuklide und bieten damit die Möglichkeit zu drastischer Reduzierung freigesetzter Radioaktivität im Falle einer Undichtigkeit der Hüllrohre. Dies gilt insbesondere auch für radioaktives Jod, Cäsium und Strontium. Zeolith und Aktivkohle entlasten also die Barrierenfunktion des Behälters für radioaktive Strahler (Radionuklide).Absorb or adsorb zeolite and activated carbon - apart from Noble gases - non-volatile or readily volatile radionuclides and offer thus the possibility of a drastic reduction in released Radioactivity in the event of a leak in the cladding tubes. This applies in particular to radioactive iodine, cesium and strontium. Zeolite and activated carbon relieve the burden Barrier function of the container for radioactive sources (Radionuclides).
Die Schüttung aus Zeolith und/oder Aktivkohle im Behälter läßt auch genügend Leervolumen zur Aufnahme von freigewordenen Edelgasen, so daß sich im Behälter kein hoher Innendruck ausbilden kann. Trotzdem hat die Schüttung aus Zeolith und/oder Aktivkohle genügend Wärmeleitfähigkeit zum Abführen von Nachzerfallswärme aus den Brennstäben. Außerdem stellt die Schüttung eine zusätzliche Wärmekapazität im Behälter dar. Die Schüttung, insbesondere wenn sie Aktivkohle enthält, hat ferner eine gute Moderationswirkung auf Neutronen und verringert deshalb die Härte von Neutronenstrahlung, die von der radioaktiven Substanz in den Brennstäben ausgehen kann. Auch zur Abschirmung von Gammastrahlung, die von den Brennstäben ausgeht, kann die Schüttung beitragen, Schließlich stellt die Schüttung auch noch einen mechanischen Puffer für die im Behälter eingelagerten Brennstäbe dar. Diese werden durch die Schüttung vor Beschädigung beim Transport oder bei der Handhabung des Behälters zusätzlich geschützt ist. Von der Schüttung absorbierte Radionuklide begeben sich aufgrund chemischer Gesetze in Gleichgewichts zustände und verlieren dadurch ihre Neigung zur Migration, so daß die Schüttung eine Langzeitlagerung der Kapsel sicher gewährleistet.The bed of zeolite and / or activated carbon in the container also leaves enough empty volume to accommodate vacant ones Noble gases, so that there is no high internal pressure in the container can train. Nevertheless, the bed of zeolite and / or activated carbon sufficient thermal conductivity for removal of post-decay heat from the fuel rods. Also poses the fill an additional heat capacity in the container The bed, especially if it contains activated carbon, also has a good moderating effect on neutrons and therefore reduces the hardness of neutron radiation from the radioactive substance in the fuel rods can go out. Also for shielding gamma radiation from the fuel rods runs out, the bulk can contribute, finally the bed also provides a mechanical buffer for the fuel rods stored in the container. These are due to the fill from damage during transport or at the handling of the container is additionally protected. From radionuclides absorbed in the bed emanate due to chemical laws in equilibrium and lose thereby their tendency to migrate, so that the fill a Long-term storage of the capsule is guaranteed.
Gegenstand der Patentansprüche 2 bis 11 sind vorteilhafte
Weiterbildungen des Behälters nach Patentanspruch 1.The subject of
Die Erfindung und ihre Vorteile seien anhand der Zeichnung an zwei Ausführungsbeispielen näher erläutert:
- Figur 1
- zeigt schematisiert einen Querschnitt durch einen Transport- und/oder Lagerbehälter mit einem bestrahlten Kernreaktorbrennelement,
Figur 2- zeigt schematisiert im Querschnitt den Lagerbehälter nach Fig. 1 in einem Endlager.
- Figure 1
- schematically shows a cross section through a transport and / or storage container with an irradiated nuclear reactor fuel element,
- Figure 2
- shows schematically in cross section the storage container of FIG. 1 in a repository.
Im langgestreckten Lagerbehälter 2 nach Fig. 1 befindet sich
ein Kernreaktorbrennelement 3, dessen quadratischer Umriß gestrichelt
angedeutet ist. Dieses Kernreaktorbrennelement 3
weist Brennstäbe 4, und Führungsrohre 5 auf. Die Brennstäbe 4
sind mit abgebranntem Kernbrennstoff, z.B. UO2 und/oder
U/PuO2, gefüllt, der Radionuklide enthält. Dieser Kernbrennstoff
befindet sich jeweils in einem Hüllrohr der Brennstäbe
4, z.B. aus einer Zirkoniumlegierung, das an beiden Rohrenden
jeweils mit einem Stopfen aus Zirkoniumlegierung verschlossen
ist. Diese Stopfen aus Zirkoniumlegierung sind mit dem Hüllrohr
gasdicht verschweißt. Die Führungsrohre 5 dienten zum
Führen von Steuerstäben und sind an mindestens einem Rohrende
offen. Sie enthalten keine Radionuklide.In the
Der Lagerbehälter 2 ist mit einer Schüttung 6 aus Granulat
eines Zeoliths aufgefüllt. Diese Schüttung 6 braucht nicht
zusammengepreßt zu sein, und mit ihr sind auch die Brennstäbe
4 und zwangsläufig die Führungsrohre 5 des Kernreaktorbrennelements
3 hinterfüllt. Der Behälter 2 besteht aus Stahl und
ist an beiden Enden mit einer Stahlplatte gasdicht verschweißt.The
In Figur 2 ist der Behälter 2, der das Kernreaktorbrennelement
3 mit den abgebrannten Brennstäben enthält, in eine Bohrung
eingesetzt, die sich beispielsweise in einem Salzstock
eines Endlagers befindet. In dieser Bohrung befindet sich auf
der Außenseite des Behälters 2 eine weitere Schüttung 7, die
ebenfalls Granulat eines Zeoliths ist. In dieser Schüttung 7
ist der Behälter 2 vollständig eingebettet.In Figure 2 is the
Den Schüttungen 6 und 7 aus Zeolith in den Figuren 1 und 2
kann auch Aktivkohle beigemischt sein. Zu Zeolithen wird auf
Ullmanns "Enzyklopädie der Technischen Chemie", Band 24, Seiten
575 bis 578, 1983, und auf Ullmanns "Enzyklopädie der
Technischen Chemie", Band 17, Seiten 9 bis 17, 1979 verwiesen.
Besonders geeignet ist für die Schüttungen 6 und 7 Zeolith
vom Typ A, vorzugsweise mindestens einer der Stoffe MgA,
CaA und SrA. Ein solches Zeolith vom Typ A kann auch mit Silber
dotiert sein, so daß es besonders gut radioaktives Jod
zurückhält, das möglicherweise aus einem Leck im Hüllrohr eines
Brennstabs 4 austritt, dann aber schon vor der Wand des
Behälters 2 zurückgehalten wird, deren Rückhaltewirkung durch
das Zeolith der Schüttung 6 im Behälter 2 also noch verstärkt
ist. Gut geeignet für Zeolithschüttungen sind auch Chabazit
und Mordenit. Besonders gut geeignet sind beispielsweise Zeolithe
mit der Handelsbezeichnung "Zeolon Molecular Sieves"
der 400 Series, 500 Series, 700 Series und 900 Series, die
über Ionenaustausch Cs und Sr binden.The
Partikel aus mindestens einem der Stoffe Metallgrieß, MnO2,
Al2O3, MgO, SuO2, ZrO2 und Silikat, die mindestens einer der
Schüttungen 6 und 7 beigemischt werden, erhöhen die Wärmeleitfähigkeit
dieser Schüttungen 6 und 7 zum Abführen von
Nachzerfallswärme von den Brennstäben 4.Particles of at least one of the materials metal grit, MnO 2 , Al 2 O 3 , MgO, SuO 2 , ZrO 2 and silicate, which are mixed in at least one of the
Claims (11)
- Container (2) sealed in a gastight manner and having several spent fuel rods (4) which are embedded in a fill (6) consisting of zeolite and/or activated charcoal.
- Container (2) according to claim 1,
characterized by steel walls and steel plates at its ends, the steel plates being welded in a gastight manner to the steel walls. - Container (2) according to claim 1 or 2,
having a fuel element (3) which contains the fuel rods (4) and through which the fill (6) passes. - Container (2) according to claim 3,
characterized in that there is room for only one fuel element (3) therein. - Container (2) according to one of claims 1 to 3, characterized in that the fill (6) is formed from a granulated material consisting of the zeolite and/or the activated charcoal.
- Container (2) according to one of claims 1 to 5, characterized by another fill (7) consisting of zeolite and/or activated charcoal, in particular a fill consisting of granulated material of zeolite and/or activated charcoal, on its outer side.
- Container (2) according to one of claims 1 to 6, characterized in that the zeolite is of Type A.
- Container (2) according to claim 7,
characterized in that the zeolite is formed at least from one of the substances MgA, CaA and SrA. - Container (2) according to claim 7 or 8,
characterized in that the zeolite is doped with silver. - Container (2) according to one of claims 1 to 6, characterized in that the zeolite is formed at least from one of the substances chabazite and mordenite.
- Container (2) according to one of claims 1 to 10, characterized in that particles consisting of at least one of the substances metal grit, MnO2, Al2O3, MgO, Sno2, ZrO2 and silicate are admixed to the zeolite and/or the activated charcoal.
Applications Claiming Priority (3)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
DE19545761 | 1995-12-07 | ||
DE19545761A DE19545761A1 (en) | 1995-12-07 | 1995-12-07 | Containers with a radioactive body |
PCT/EP1996/005205 WO1997021227A1 (en) | 1995-12-07 | 1996-11-25 | Container with a radioactive body |
Publications (2)
Publication Number | Publication Date |
---|---|
EP0865652A1 EP0865652A1 (en) | 1998-09-23 |
EP0865652B1 true EP0865652B1 (en) | 1999-06-02 |
Family
ID=7779513
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
EP96939924A Expired - Lifetime EP0865652B1 (en) | 1995-12-07 | 1996-11-25 | Container with a radioactive body |
Country Status (5)
Country | Link |
---|---|
US (1) | US6699439B1 (en) |
EP (1) | EP0865652B1 (en) |
DE (2) | DE19545761A1 (en) |
ES (1) | ES2133198T3 (en) |
WO (1) | WO1997021227A1 (en) |
Cited By (1)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE10116029A1 (en) * | 2001-03-30 | 2002-08-22 | Framatome Anp Gmbh | Transport container with internal arrangement of fuel rods for nuclear reactor, also contains medium to trap aerosols and radiolytic gases |
Families Citing this family (7)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE19757843C1 (en) * | 1997-12-24 | 1999-08-12 | Nuklear Service Gmbh Gns | Storage containers for the intermediate and / or final storage of spent fuel elements |
US7309807B2 (en) | 2003-02-28 | 2007-12-18 | The Nanosteel Company, Inc. | Method of containing radioactive contamination |
US7199375B2 (en) * | 2004-10-12 | 2007-04-03 | Bard Brachytherapy, Inc. | Radiation shielding container that encloses a vial of one or more radioactive seeds |
NO20044434D0 (en) * | 2004-10-19 | 2004-10-19 | Nuclear Prot Products As | Long-term storage container and process for making it |
DE202011102838U1 (en) * | 2011-07-02 | 2011-12-27 | Ewald von Hagen | Radiation protection offset for the prevention and discharge of radioactive radiation in mining |
WO2018064572A1 (en) * | 2016-09-29 | 2018-04-05 | Elysium Industries Ltd. | Silver chloride waste form and apparatus |
US10878972B2 (en) | 2019-02-21 | 2020-12-29 | Deep Isolation, Inc. | Hazardous material repository systems and methods |
Family Cites Families (9)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
FR319398A (en) | 1902-03-08 | 1902-11-11 | Buysse | Automatic sorter for potatoes, vegetables, fruits, grains, etc. |
DE3169709D1 (en) * | 1980-10-13 | 1985-05-09 | Euratom | A method of encapsulating materials in a zeolite in a stable manner |
RU1299369C (en) * | 1985-07-26 | 1993-02-23 | Предприятие П/Я В-2679 | Packing unit for transporting and storing radio-active and fissionable materials |
US4778628A (en) * | 1986-05-15 | 1988-10-18 | The United States Of America As Represented By The United States Department Of Energy | Underground waste barrier structure |
US4891164A (en) * | 1986-08-28 | 1990-01-02 | The Standard Oil Company | Method for separating and immobilizing radioactive materials |
JPH0631882B2 (en) * | 1987-01-19 | 1994-04-27 | 鹿島建設株式会社 | Waste treatment facility |
FR2624301B1 (en) * | 1987-12-02 | 1990-03-30 | Commissariat Energie Atomique | DEVICE FOR CONDITIONING RADIOACTIVE OR TOXIC WASTE CONTAINING BORATE IONS, AND MANUFACTURING METHOD THEREOF |
US4950426A (en) * | 1989-03-31 | 1990-08-21 | Westinghouse Electric Corp. | Granular fill material for nuclear waste containing modules |
US5169566A (en) * | 1990-05-18 | 1992-12-08 | E. Khashoggi Industries | Engineered cementitious contaminant barriers and their method of manufacture |
-
1995
- 1995-12-07 DE DE19545761A patent/DE19545761A1/en not_active Withdrawn
-
1996
- 1996-11-25 WO PCT/EP1996/005205 patent/WO1997021227A1/en active IP Right Grant
- 1996-11-25 EP EP96939924A patent/EP0865652B1/en not_active Expired - Lifetime
- 1996-11-25 ES ES96939924T patent/ES2133198T3/en not_active Expired - Lifetime
- 1996-11-25 DE DE59602126T patent/DE59602126D1/en not_active Expired - Lifetime
-
1998
- 1998-06-08 US US09/093,574 patent/US6699439B1/en not_active Expired - Fee Related
Cited By (1)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE10116029A1 (en) * | 2001-03-30 | 2002-08-22 | Framatome Anp Gmbh | Transport container with internal arrangement of fuel rods for nuclear reactor, also contains medium to trap aerosols and radiolytic gases |
Also Published As
Publication number | Publication date |
---|---|
US6699439B1 (en) | 2004-03-02 |
EP0865652A1 (en) | 1998-09-23 |
DE19545761A1 (en) | 1997-06-12 |
WO1997021227A1 (en) | 1997-06-12 |
ES2133198T3 (en) | 1999-09-01 |
DE59602126D1 (en) | 1999-07-08 |
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