DE1045603B - Light stabilizers - Google Patents

Light stabilizers

Info

Publication number
DE1045603B
DE1045603B DEM34398A DEM0034398A DE1045603B DE 1045603 B DE1045603 B DE 1045603B DE M34398 A DEM34398 A DE M34398A DE M0034398 A DEM0034398 A DE M0034398A DE 1045603 B DE1045603 B DE 1045603B
Authority
DE
Germany
Prior art keywords
light stabilizers
aqueous
substances
cinnamale
acetic acid
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Pending
Application number
DEM34398A
Other languages
German (de)
Inventor
Dr Heinrich Baron
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Merck KGaA
Original Assignee
E Merck AG
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by E Merck AG filed Critical E Merck AG
Priority to DEM34398A priority Critical patent/DE1045603B/en
Publication of DE1045603B publication Critical patent/DE1045603B/en
Pending legal-status Critical Current

Links

Classifications

    • AHUMAN NECESSITIES
    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61QSPECIFIC USE OF COSMETICS OR SIMILAR TOILETRY PREPARATIONS
    • A61Q17/00Barrier preparations; Preparations brought into direct contact with the skin for affording protection against external influences, e.g. sunlight, X-rays or other harmful rays, corrosive materials, bacteria or insect stings
    • A61Q17/04Topical preparations for affording protection against sunlight or other radiation; Topical sun tanning preparations
    • AHUMAN NECESSITIES
    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61KPREPARATIONS FOR MEDICAL, DENTAL OR TOILETRY PURPOSES
    • A61K8/00Cosmetics or similar toiletry preparations
    • A61K8/18Cosmetics or similar toiletry preparations characterised by the composition
    • A61K8/30Cosmetics or similar toiletry preparations characterised by the composition containing organic compounds
    • A61K8/33Cosmetics or similar toiletry preparations characterised by the composition containing organic compounds containing oxygen
    • A61K8/36Carboxylic acids; Salts or anhydrides thereof

Landscapes

  • Health & Medical Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Animal Behavior & Ethology (AREA)
  • General Health & Medical Sciences (AREA)
  • Public Health (AREA)
  • Veterinary Medicine (AREA)
  • Emergency Medicine (AREA)
  • Birds (AREA)
  • Epidemiology (AREA)
  • Dermatology (AREA)
  • Cosmetics (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Description

Lichtschutzmittel Es sind bereits zahlreicheSubstanzen vorgeschlagen worden, die als Lichtschutzmittel in Emulsionen, Salben, Pudern usw. Verwendung finden, welche auf die Haut aufgetragen werden sollen. Diesen Substanzen haftet jedoch entweder der Nachteil an, daß sie bei empfindlicher Haut Reizungserscheinungen hervorrufen, oder daß sie das UV-Licht nicht in genügendem AusmaB absorbieren, so daß für eine zweckentsprechende Anwendung unbequem große Substanzmengen erforderlich sind. Entweder muß man dann entsprechend große Salbenmengen auf die Haut bringen, oder man muß die Substanzen in relativ hoher Konzentration verwenden, was ebenfalls Unzuträglichkeiten, z. B. stärkere Reizungen oder die Gefahr der Zersetzung, mit sich bringt. Andere Lichtschutzmittel, z. B. die Natriumsalze und Ester substituierter Acryl-bzw. Crotonsäuren, neigen zur Autoxydation und Verfärbung der damit hergestellten Anwendungsformen.Light stabilizers Numerous substances have already been proposed been used as light stabilizers in emulsions, ointments, powders, etc. find which to apply to the skin. Adheres to these substances however, either the disadvantage is that they cause irritation in sensitive skin cause, or that they do not absorb the UV light to a sufficient extent, so that inconveniently large amounts of substance are required for an appropriate application are. Either you then have to apply a correspondingly large amount of ointment to the skin, or you have to use the substances in a relatively high concentration, which is also Inconveniences, e.g. B. stronger irritation or the risk of decomposition, with brings itself. Other light stabilizers, e.g. B. the sodium salts and esters substituted Acrylic or Crotonic acids tend to auto-oxidize and discolour those produced with them Application forms.

Vorliegende Erfindung beruht auf der Feststellung, daß die Cinnamalessigsäure und/oder deren Salze, UV-Strahlen der Erythem erzeugenden Wellenlängen in so starkem Maße abschirmen, daß bereits ein Zusatz son 0,5 bis 1 I/o dieser Verbindungen zu den üblichen, insbesondere hydrophilen Salbengrundlagen u. ä. ausreicht, um eine vollständige Abschirmung der Sonnenbrand erzeugenden Strahlen zu erreichen. The present invention is based on the discovery that cinnamale acetic acid and / or their salts, UV rays of erythema generating wavelengths in such strong Shield dimensions that add 0.5 to 1 I / o of these connections the usual, especially hydrophilic ointment bases and the like to achieve complete shielding of the sunburn-causing rays.

Cinnamalessigsäure bzw. ihre Salze sind für den menschlichen Organismus ungiftig und zeigen eine überragend gute Verträglichkeit mit der menschlichen Haut. Auch werden diese Verbindungen durch Einwirkung ultravioletter Strahlen während der üblichen Dauer des Sonnenbades nicht verändert bzw. zerstört, so daß Reizungserscheinungen der Haut durch EntstehenaggressiverZersetzungsprodukte ausgeschlossen sind. Ein weiterer Vorteil der erfindungsgemäßen Stoffe besteht darin, daß sie geschmack-und geruchlos und höchstens leicht gelbgefärbt sind. Zu den erfindungsgemäßen Verbindungen gehört die Cinnamalessigsäure selbst sowie ihre ungefärbten oder schwach gefärbten Salze mit für den betreffenden Verwendungszweck nicht störenden Alkalien, Erdalkalien oder anderen Metallen.Cinnamale acetic acid and its salts are for the human organism non-toxic and show outstanding compatibility with human skin. Also, these compounds are exposed during exposure to ultraviolet rays the usual duration of sunbathing is not changed or destroyed, so that irritation symptoms of the skin due to the formation of aggressive decomposition products. A Another advantage of the substances according to the invention is that they taste and are odorless and at most slightly yellow in color. The compounds according to the invention belongs to the cinnamale acetic acid itself as well as its uncolored or faintly colored Salts with alkalis and alkaline earths which do not interfere with the intended use or other metals.

Es sind bereits ähnlich gebaute Lichtschutzsubstanzen, wie z. B. Cinnamalacetophenon, Dibenzalaceton oder Abkömmlinge des Phenylbutadiens, die keine Carboxylgruppe enthalten, bekannt. Diese Substanzen absorbieren jedoch zum Teil nicht in dem für kosmetische Lichtschutzsubstanzen interessierenden UV-Bereich von 280 bis 300mu und haben insbesondere den Nachteil, daß sie nicht wasserlöslich sind, so daß wäßrige oder wäßrig-alkoholische Lichtschutzpräparate, die sich als besonders vorteilhaft erwiesen haben, daraus nicht hergestellt werden können. Zum Teil sind diese Verbindungen auch stark hautreizend, so daß sie schon deswegen für kosmetische Zwecke ungeeignet sind. There are already similarly built light protection substances such. B. Cinnamalacetophenone, dibenzalacetone or derivatives of phenylbutadiene that do not have any Contain carboxyl group, known. However, some of these substances absorb not in the UV range of 280 to 300mu and have the particular disadvantage that they are not water-soluble, so that aqueous or aqueous-alcoholic light protection preparations, which are particularly have proven advantageous, cannot be produced from it. Partly are these compounds are also highly irritating to the skin, so that they are therefore suitable for cosmetic use Purposes are unsuitable.

Demgegenüber sind die Lichtschutzsubstanzen nach derErfindung gut wasserlöslich, so daß wäßrigeLichtschutzpräparate daraus hergestellt werden können, die neben besserer UV-Absorption den Vorteil geringerer Toxizität gegenüber lipoidlöslichen Präparaten besitzen. On the other hand, the photoprotective substances according to the invention are good water-soluble, so that aqueous light protection preparations can be made from it, which, in addition to better UV absorption, have the advantage of lower toxicity compared to lipoid-soluble ones Own preparations.

Als geeignete Anwendungsform der gemäß vorliegender Erfindung beanspruchten Lichtschutzsubstanzen eignen sich wäßrige oder wäßrig-alkoholische Lösungen, denen gegebenenfalls noch Insekten abwehrende Verbindungen, Parfüms, die Hautbräunung fördernde Stoffe zugefügt sein können. As a suitable application form those claimed according to the present invention Light protection substances are aqueous or aqueous-alcoholic solutions, which possibly also insect repellent compounds, perfumes, skin tanning promoting substances can be added.

Im folgenden seien einige unter die Erfindung fallende Rezepte für kosmetische Lichtschutzmittel angeführt. Die Herstellung erfolgt unter Beachtung der in der kosmetischen Industrie erarbeiteten Verfahren. The following are some of the recipes for which the invention relates cosmetic sunscreens listed. The production takes place under consideration of the procedures developed in the cosmetic industry.

1. Wäßrig alkoholische Lichtschutzlösung, nicht fettend : Cinnamalessigsäure 1,0 Teile Triäthanolamin 0,9" Sorbit (700/o Trockensubstanz enthaltend)....................... 5,0" n-Propanol...................... 40, 0" Parfum 0, 3" Wasser.......................... 52,8" 2. Wäßrige Lichtschutzlösung : Cinnamalessigsaure.............. 1, 0 Teile Natriumcarbonat (10 Mol Kristallwasser)....................... 0,82" Parfüm, wasserlöslich 1,0,. 1. Aqueous alcoholic light protection solution, non-greasy: cinnamale acetic acid 1.0 parts triethanolamine 0.9 "sorbitol (containing 700 / o dry matter) ....................... 5.0 "n-propanol ...................... 40.0" perfume 0.3 "water ........... ............... 52.8 "2. Aqueous light protection solution: cinnamale acetic acid .............. 1.0 parts Sodium carbonate (10 mol of crystal water) ....................... 0.82 "perfume, soluble in water 1.0 ,.

Sorbit (70°/o Trockensubstanz enthaltend)....................... 5,0 Wasser.......................... 100,0,. Sorbitol (containing 70% dry matter) ....................... 5.0 water .......................... 100.0 ,.

Claims (1)

PATENTANSPRUCH Lichtschutzmittel für den kosmetischen Gebrauch, gekennzeichnet durch einen Gehalt an Cinnamalessigsäure und/oder ein ein Salz oder mehrerenSalzen derCinnamalessigsäure in wäßriger oder alkoholisch-wäßriger Lösung. PATENT CLAIM Light stabilizers for cosmetic use, marked by a content of cinnamale acetic acid and / or a salt or several salts dercinnamalenacetic acid in aqueous or alcoholic-aqueous solution. In Betracht gezogene Druckschriften : Deutsche Patentschriften Nr. 652 929,762 869 ; USA.-Patentschrift Nr. 2 134 947. Considered publications: German Patent Specifications No. 652,929,762,869; U.S. Patent No. 2,134,947.
DEM34398A 1957-06-06 1957-06-06 Light stabilizers Pending DE1045603B (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
DEM34398A DE1045603B (en) 1957-06-06 1957-06-06 Light stabilizers

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DEM34398A DE1045603B (en) 1957-06-06 1957-06-06 Light stabilizers

Publications (1)

Publication Number Publication Date
DE1045603B true DE1045603B (en) 1958-12-04

Family

ID=7302012

Family Applications (1)

Application Number Title Priority Date Filing Date
DEM34398A Pending DE1045603B (en) 1957-06-06 1957-06-06 Light stabilizers

Country Status (1)

Country Link
DE (1) DE1045603B (en)

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
FR2395024A1 (en) * 1977-06-23 1979-01-19 Henkel Kgaa COSMETIC PRODUCTS FOR PROTECTION AGAINST LIGHT AND MORE SPECIFICALLY THE LIGHT OF THE REGION HAS ULTRAVIOLET SPECTRUM

Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE652929C (en) * 1936-02-25 1937-11-10 Chem Fab Means for shielding ultraviolet rays
US2134947A (en) * 1935-09-13 1938-11-01 Isermann Samuel Protective cosmetic
DE762869C (en) * 1941-02-25 1952-11-17 Ig Farbenindustrie Ag Filter that absorbs ultraviolet rays

Patent Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2134947A (en) * 1935-09-13 1938-11-01 Isermann Samuel Protective cosmetic
DE652929C (en) * 1936-02-25 1937-11-10 Chem Fab Means for shielding ultraviolet rays
DE762869C (en) * 1941-02-25 1952-11-17 Ig Farbenindustrie Ag Filter that absorbs ultraviolet rays

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
FR2395024A1 (en) * 1977-06-23 1979-01-19 Henkel Kgaa COSMETIC PRODUCTS FOR PROTECTION AGAINST LIGHT AND MORE SPECIFICALLY THE LIGHT OF THE REGION HAS ULTRAVIOLET SPECTRUM

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