CS267379B1 - Process for the preparation of 3-methyl-7-n-propyl-3,7-dihydro-1H-purine-2,6-dione - Google Patents

Process for the preparation of 3-methyl-7-n-propyl-3,7-dihydro-1H-purine-2,6-dione Download PDF

Info

Publication number
CS267379B1
CS267379B1 CS883550A CS355088A CS267379B1 CS 267379 B1 CS267379 B1 CS 267379B1 CS 883550 A CS883550 A CS 883550A CS 355088 A CS355088 A CS 355088A CS 267379 B1 CS267379 B1 CS 267379B1
Authority
CS
Czechoslovakia
Prior art keywords
formula
dione
methyl
propyl
formamide
Prior art date
Application number
CS883550A
Other languages
Czech (cs)
Slovak (sk)
Other versions
CS355088A1 (en
Inventor
Alfonz Ing Csc Rybar
Milan Clen Korespondent Repas
Dusan Ing Csc Hesek
Richard Doc Ing Csc Frimm
Marian Ing Tegza
Fridrich Rndr Csc Szemes
Original Assignee
Rybar Alfonz
Milan Clen Korespondent Repas
Hesek Dusan
Frimm Richard
Tegza Marian
Szemes Fridrich
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Rybar Alfonz, Milan Clen Korespondent Repas, Hesek Dusan, Frimm Richard, Tegza Marian, Szemes Fridrich filed Critical Rybar Alfonz
Priority to CS883550A priority Critical patent/CS267379B1/en
Publication of CS355088A1 publication Critical patent/CS355088A1/en
Publication of CS267379B1 publication Critical patent/CS267379B1/en

Links

Landscapes

  • Pharmaceuticals Containing Other Organic And Inorganic Compounds (AREA)

Abstract

Zlúčenina vzorca I sa používá vo farmaceutickej chémii ako medziprodukt pri výrobě periférneho vazodilatans a hemoreologika propantofylínu. Jej výroba spočívá v tom, že sa 5- n-propylamíno-6-amíno-l-metyl-lH-pyrimidín- * 2,4-dion vzorca II formyluje pósobením formamidu a in šitu vznikajúci 5-N-(n-propyl)-formylamíno-6-amíno-l-metyl-lH-pyrimidín-2,6-dion vzorca III sa termicky cyklizuje v prostředí formamidu pri teplote 100 až 195 °C za přítomnosti kyseliny s hodnotou pKa max. 4,8, s výhodou kyseliny mravčej.The compound of formula I is used in pharmaceutical chemistry as an intermediate in the production of the peripheral vasodilator and haemorheologic propantofylline. Its production consists in the fact that 5-n-propylamino-6-amino-1-methyl-1H-pyrimidine-2,4-dione of formula II is formylated by treatment with formamide, and the resulting 5-N-(n-propyl)-formylamino-6-amino-1-methyl-1H-pyrimidine-2,6-dione of formula III is thermally cyclized in a formamide environment at a temperature of 100 to 195 °C in the presence of an acid with a pKa value of max. 4.8, preferably formic acid.

Description

Vynález sa týká spósobu přípravy 3-metyl-7n-propyl-3,7-dihydro-1H-purin-2,6-dionu vzorca I

ktorý sa používá vo farmaceutickej chémii ako medziprodukt pri výrobě periférneho vazodilatancia a hemoreologika propentofylínu.

Doposial’ sa zlúčenina vzorca I připravovala alkyláciou 3-metyl-3,7-dihydro-lH-purin-2,6dionu s n-propylhalogenidom za přítomnosti uhličitanu alkalického kovu v aprotickom rozpúšťadle A. Rybář a spol.: CS AO 263 595 alebo alkyláciou alkalickej soli 3-metyl-3,7-dihydro-lH-purin-2,6-dionu s n-propylhalogenidom v aprotickom rozpúšťadle A. Rybář a spol.: CS AO 263 595. Nevýhodou týchto postupov je, že pri nich móže vznikať ako vedfajší produkt 3-metyl-l,7-di-n-propyl-3,7-dihydro-lH-purin-2,6-dion, ktorý třeba odstraňovať.

Túto nevýhodu odstraňuje spósob přípravy zlúčeniny vzorca I podía vynálezu, podstatou ktorého je formylácia 5-n-propyIamíno-6-amíno-1-metyl-lH-pyrimidín-2,6-díonu vzorca II

pósobením formamidu a termická cyklizácia in šitu vznikajúceho 5-N-(n-propyl)-formyIamíno6-amíno-1 -metyl-1 H-pyrimidín-2,6-dionu vzorca III

v prostředí formamidu za přítomnosti kyseliny s hodnotou pKa max. 4,8.

Postup podía vynálezu sa uskutočňuje tak, že sa zlúčenina vzorca II zahrieva s prebytkom formamidu pri teplote 100 °C až 195 °C za přítomnosti kyseliny octovej, chlorovodíkovej, alebo s výhodou kyseliny mravčej. Zlúčenina vzorca I sa už počas reakcie vylučuje z reakčnej zmesi, úplné sa vylúči jej ochladenie na teplotu miestnosti. Izoluje sa odfiltrováním alebo odstředěním, premytím vodou a vysušením pri zvýšenej teplote, s výhodou vo vákuu.

Hlavnou výhodou poslupu podía vynálezu je 1-stupňová příprava zlúčeniny vzorca I zo zlúčeniny vzorca II. Výťažky zlúčeniny vzorca I sa pohybujú okolo 80 % teorie. V ďalšom je predmet vynálezu popísaný v príkladoch prevedenia bez toho, že by sa na tieto obmedzoval. Příklad 1

Zmes 9,9 g zlúčeniny vzorca íí, 50 ml formamidu a 2,5 ml kyseliny mravčej sa zahrieva pri teplote kúpeía 185 °C počas 4 h. Po tejto době sa nechá samovolné vychladnúť, pričom z reakčnej zmesi kryštalizuje zlúčenina vzorca I. Po premytí vodou a vysušení pri zvýšenej teplote sa získá 8,25 g (79,2 % teorie) zlúčeniny vzorca 1 s 1.1.248 °C až 251 °C. Pre C9H|2N4O2 (208,2) vypočítané: 51,91 %C, 5,81 % H. 26,91 %N; nájdené: 51,69 % C, 6,00 % H, 27,08 % N. Produkt reakcie je chromatograficky totožný so zlúčeninou vzorca I připravenou podfa CS AO 263 595. Příklad 2

Zmes 9,9 g zlúčeniny vzorca II, 50 ml formamidu a 2,5 ml kyseliny octovej sa zahrieva do varu (teplota kúpeía 185 °C) počas 4 h. Po tomto čase s nechá samovolné vychladnúť, pričom vykrystalizuje zlúčenina vzorca I. Po niekofkohodinovom dochladení na teplotu okolo 0 °C sa produkt odsaje, premyje vodou a vysuší pri zvýšenej teplote vo vákuu. Získá sa 8,4 g (80,8 % teorie) zlúčeniny vzorca I s 1.1. 248 až 250 °C.

The invention relates to a process for the preparation of 3-methyl-7n-propyl-3,7-dihydro-1H-purine-2,6-dione of the formula I

which is used in pharmaceutical chemistry as an intermediate in the production of peripheral vasodilators and hemorrhages of propentophyllin.

To date, the compound of formula I has been prepared by alkylating 3-methyl-3,7-dihydro-1H-purine-2,6-dione with n-propyl halide in the presence of an alkali metal carbonate in aprotic solvent A. Rybář et al. of the 3-methyl-3,7-dihydro-1H-purine-2,6-dione alkaline salt with n-propyl halide in aprotic solvent A. Rybář et al .: CS AO 263 595. as by-product 3-methyl-1,7-di-n-propyl-3,7-dihydro-1H-purine-2,6-dione, which is to be removed.

This drawback is overcome by the preparation of the compound of formula (I) according to the invention, the subject of which is the formylation of 5-n-propylamino-6-amino-1-methyl-1H-pyrimidine-2,6-dione of formula II

by formamide and thermal cyclization of the resulting 5-N- (n-propyl) -formylamino-6-amino-1-methyl-1H-pyrimidine-2,6-dione of formula III

in formamide in the presence of acid with a pKa value of max 4.8.

The process of the invention is carried out by heating the compound of formula II with excess formamide at 100 ° C to 195 ° C in the presence of acetic acid, hydrochloric acid, or preferably formic acid. The compound of formula (I) is already precipitated from the reaction mixture during the reaction and is completely eliminated from cooling to room temperature. It is isolated by filtration or centrifugation, washing with water and drying at elevated temperature, preferably under vacuum.

The main advantage of the sequence according to the invention is the 1-step preparation of the compound of formula I from the compound of formula II. The yields of the compound of formula I are about 80% of theory. In the following, the invention will be described in the examples without limiting it. Example 1

A mixture of 9.9 g of the compound of formula (Ii), 50 ml of formamide and 2.5 ml of formic acid is heated at a bath temperature of 185 ° C for 4 h. with water and drying at elevated temperature, 8.25 g (79.2% of theory) of the compound of formula I with 1.148 ° C to 251 ° C are obtained. For C9H12N4O2 (208.2) calculated: 51.91% C, 5.81% H 26.91% N; Found: C, 51.69; H, 6.00; N, 27.08. The product of the reaction is identical to the compound of formula (I) prepared in accordance with AO 263,595.

A mixture of 9.9 g of the compound of formula II, 50 ml of formamide and 2.5 ml of acetic acid is heated to boiling (bath temperature 185 ° C) for 4 h. After this time it is allowed to cool spontaneously, whereby the compound of formula I crystallizes. cooling to about 0 ° C, the product is filtered off with suction, washed with water and dried under vacuum at elevated temperature. 8.4 g (80.8% of theory) of the compound of formula I with 1.1 are obtained. 248-250 ° C.

Claims (2)

PREDMET VYNÁLEZUOBJECT OF THE INVENTION 1. Spósob přípravy 3-metyl-7-n-propyl-3,7dihydro-lH-purin-2,6-dionu vzorca I vyznačujúci sa tým, že sa 5-n-propylamíno-A process for the preparation of 3-methyl-7-n-propyl-3,7-dihydro-1H-purine-2,6-dione of the formula I, characterized in that 5-n-propylamino- CS 267 379 Bl formyluje pósobením formamidu a in šitu vznikajúci 5-N-(n-propyl)-formylamíno-6-amíno-lmetyl-lH-pyrimidín-2,6-dion vzorce ÍII sa termicky cyklizuje v prostředí formamidu pri teplote 100 až 195 °C za přítomnosti kyseliny s hodnotou pKa max. 4,8,CS 267 379 B1 is formalized by the action of formamide and the in situ 5-N- (n-propyl) -formylamino-6-amino-1-methyl-1H-pyrimidine-2,6-dione of formula II is thermally cyclized in the formamide at temperatures of 100 to 195 ° C in the presence of acid with pKa max. 4.8. 2. Spósob podía bodu 1 vyznačujúci sa tým, že sa reakcia uskutočňuje za přítomnosti kyseliny octovej, chlorovodíkovej alebo s výhodou kyseliny tnravčej.2. Process according to claim 1, characterized in that the reaction is carried out in the presence of acetic acid, hydrochloric acid or preferably formic acid.
CS883550A 1988-05-25 1988-05-25 Process for the preparation of 3-methyl-7-n-propyl-3,7-dihydro-1H-purine-2,6-dione CS267379B1 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
CS883550A CS267379B1 (en) 1988-05-25 1988-05-25 Process for the preparation of 3-methyl-7-n-propyl-3,7-dihydro-1H-purine-2,6-dione

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CS883550A CS267379B1 (en) 1988-05-25 1988-05-25 Process for the preparation of 3-methyl-7-n-propyl-3,7-dihydro-1H-purine-2,6-dione

Publications (2)

Publication Number Publication Date
CS355088A1 CS355088A1 (en) 1989-06-13
CS267379B1 true CS267379B1 (en) 1990-02-12

Family

ID=5375907

Family Applications (1)

Application Number Title Priority Date Filing Date
CS883550A CS267379B1 (en) 1988-05-25 1988-05-25 Process for the preparation of 3-methyl-7-n-propyl-3,7-dihydro-1H-purine-2,6-dione

Country Status (1)

Country Link
CS (1) CS267379B1 (en)

Also Published As

Publication number Publication date
CS355088A1 (en) 1989-06-13

Similar Documents

Publication Publication Date Title
Blicke et al. Reactions of 1, 3-Dimethyl-5, 6-diaminouracil
Weiner Reaction of phenyl isocyanate with N, N-dimethylformamide
US4758667A (en) Process for the preparation of 2-(imidazolin-2-yl)-3-pyridine- and -3-quinolinecarboxylic acids
US3049544A (en) Method for the preparation of
RU2158266C2 (en) Method of preparing purine compounds, intermediate compounds used therein, and method of preparation thereof
IL25802A (en) Pyrazinimidoylguanidines and their preparation
CS267379B1 (en) Process for the preparation of 3-methyl-7-n-propyl-3,7-dihydro-1H-purine-2,6-dione
IL39729A (en) Pyridine derivatives
US4886881A (en) Preparation of 2-amino triazines
SU854272A3 (en) Method of producing racemitic p-oxyphenyl-5-hydantion
US3549626A (en) Process for preparing 1-loweralkyl-5-nitroimidazoles
US2820050A (en) Substituted propionitriles and preparation of the same
EP0295218A1 (en) A process for the preparation of 2,4-diamino-6-(1-piperidinyl)-pyrimidine N-oxide
US4395547A (en) Process for preparing 1-substituted-6-n-propyl-8-methylimidazo[1,5-d]-as-triazin-4(3H)-ones
RU2043993C1 (en) Method for production of hexahydrate of trisodium phosphonoformiate
JPH0645620B2 (en) Method for methylating xanthines
JPH0573738B2 (en)
US3673178A (en) Process for preparing 2-{8 2-(arylamino)-vinyl{9 -1-(lower alkyl)-3-h-indolium salt dyes
US3225048A (en) Process for the preparation of 2,6-diketo-8-thiapurines
JP2626710B2 (en) Method for synthesizing 4-amino-1,2,4- (4H) triazole derivative
Hajpál et al. Synthesis of 6‐(2‐nitrobenzyl)‐3, 5‐dioxo‐2, 3, 4, 5‐tetrahydro‐as‐triazine and some derivatives
Eid et al. Condensed 1, 2, 4‐triazines. Regioselective condensations with benzo [h] quinoline‐5, 6‐dione
Zvilichovsky et al. Synthesis and properties of 7-hydroxyxanthine and its derivatives
US3270011A (en) 5, 7-disubstituted-2, 3, 6, 8-tetraketo-pyrimido [5, 4-b] 1, 4-thiazines
JPS6126910B2 (en)