CN111638235B - XACT-based radioactive waste solidification structure detection method - Google Patents

XACT-based radioactive waste solidification structure detection method Download PDF

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CN111638235B
CN111638235B CN202010661687.9A CN202010661687A CN111638235B CN 111638235 B CN111638235 B CN 111638235B CN 202010661687 A CN202010661687 A CN 202010661687A CN 111638235 B CN111638235 B CN 111638235B
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radioactive waste
similarity
solidification structure
detection
xact
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CN111638235A (en
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刘明哲
罗锐
刘祥和
黄瑶
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Chengdu Univeristy of Technology
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    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N23/00Investigating or analysing materials by the use of wave or particle radiation, e.g. X-rays or neutrons, not covered by groups G01N3/00 – G01N17/00, G01N21/00 or G01N22/00
    • G01N23/22Investigating or analysing materials by the use of wave or particle radiation, e.g. X-rays or neutrons, not covered by groups G01N3/00 – G01N17/00, G01N21/00 or G01N22/00 by measuring secondary emission from the material
    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N29/00Investigating or analysing materials by the use of ultrasonic, sonic or infrasonic waves; Visualisation of the interior of objects by transmitting ultrasonic or sonic waves through the object
    • G01N29/04Analysing solids
    • G01N29/06Visualisation of the interior, e.g. acoustic microscopy
    • G01N29/0654Imaging
    • G01N29/0672Imaging by acoustic tomography
    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N29/00Investigating or analysing materials by the use of ultrasonic, sonic or infrasonic waves; Visualisation of the interior of objects by transmitting ultrasonic or sonic waves through the object
    • G01N29/44Processing the detected response signal, e.g. electronic circuits specially adapted therefor
    • G01N29/4409Processing the detected response signal, e.g. electronic circuits specially adapted therefor by comparison
    • G01N29/4427Processing the detected response signal, e.g. electronic circuits specially adapted therefor by comparison with stored values, e.g. threshold values
    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N2223/00Investigating materials by wave or particle radiation
    • G01N2223/07Investigating materials by wave or particle radiation secondary emission
    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N2223/00Investigating materials by wave or particle radiation
    • G01N2223/10Different kinds of radiation or particles
    • G01N2223/101Different kinds of radiation or particles electromagnetic radiation
    • G01N2223/1016X-ray
    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N2223/00Investigating materials by wave or particle radiation
    • G01N2223/50Detectors
    • G01N2223/508Detectors photo-acoustic
    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N2223/00Investigating materials by wave or particle radiation
    • G01N2223/60Specific applications or type of materials
    • G01N2223/626Specific applications or type of materials radioactive material

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Abstract

The invention discloses a radioactive waste curing structure detection method based on XACT, which aims at the defects of the existing radioactive waste curing structure detection technology and provides a radioactive waste curing structure performance detection method based on XACT.

Description

XACT-based radioactive waste solidification structure detection method
Technical Field
The invention relates to the field of radioactive waste detection, in particular to a radioactive waste solidification structure detection method based on XACT.
Background
The ultrasonic waves generated by water under X-ray irradiation were detected by Bowen et al, university of Arizona, USA, and the study of the photoacoustic effect based on X-rays was slowly focused until X-ray-excited acoustic tomography technique X-ray Induced Acoustic Computed Tomography, XACT was first proposed by the Xiang team, university of Oklamate, 2013, which uses the principle of a combination of optical and acoustic propagation, specifically: when the substance is irradiated by pulse light, the substance absorbs the energy of the pulse light to cause the transient temperature rise to cause the thermal expansion of the region, so that the outward radiation ultrasonic phenomenon is generated, which is essentially two kinds of conversion including photo-thermal and thermo-acoustic processes, and the generated ultrasonic waves express the tissue structure and performance parameters inside the substance in the outward radiation propagation process, so that the nondestructive detection of the radioactive solid structure can be realized.
Radioactive waste is a substance that contains or is contaminated with radionuclides at concentrations or activities that are greater than the clean solution level prescribed by the national regulatory agency and that is expected to be no longer in use. It is mainly derived from processes such as nuclear fuel production, reactor operation, nuclear fuel post-treatment, and nuclear facility retirement, and improper management and disposal of radioactive waste can have adverse effects on human health and the environment now and in the future. The radioactive waste solidification is to convert gas, liquid or solid waste with certain radioactivity into a monolithic solid object with performance indexes meeting the disposal requirements, and the purpose is to form an object which is suitable for loading, unloading, transporting or temporary storage and has the performance meeting the disposal requirements.
The conventional radioactive curing structure mainly comprises the detection of the mechanical property, compressive strength, impact resistance, water resistance, leaching resistance and the like of the radioactive waste curing structure, however, the conventional radioactive waste curing body performance detection utilizes sampling random screening to test the items as a reference standard for judging whether the batch of curing packaging structure meets the requirements, so that some radioactive waste curing bodies cured in the same batch must be damaged in the detection process, or curing bodies with the structure performance which does not reach the standard are missed in the random detection process, thereby causing unnecessary radiation injury to the environment and human beings. In addition, the traditional detection method has long detection time and most items to be detected, and cannot be used for real-time and rapid detection, so that time and labor are consumed in the whole process.
Disclosure of Invention
The invention aims to provide a detection method for the performance of a radioactive waste solidification structure based on XACT, and aims to provide a method for quickly and timely detecting the performance of the radioactive waste solidification structure aiming at the defects of the traditional detection technology. .
In order to achieve the above purpose, the technical scheme adopted by the invention is as follows:
a radioactive waste solidification structure detection method based on XACT, comprising the steps of:
step 01, manufacturing a plurality of groups of radioactive waste solidified bodies aiming at different radioactive waste solidification modes;
step 02, irradiating the prepared radioactive waste solidified body through suitable pulsed X-rays generated by an X-ray emission device;
step 03, collecting ultrasonic signals converted by pulsed X rays produced by an X-ray emission device in a solidified body through an ultrasonic signal collector;
step 04, the radioactive waste solidified bodies are subjected to performance test by a traditional detection method one by one, and ultrasonic signals of the radioactive waste solidified bodies which are qualified in detection are used as ultrasonic signal comparison databases of XACT detection;
step 05, performing XACT detection on the radioactive waste solidification structure to be detected, and collecting ultrasonic signals of the radioactive waste solidification structure to be detected one by one;
step 06, comparing the ultrasonic signals of the detected radioactive waste solidification structure with the data of the database by using an acoustic wave similarity comparison tool to calculate the similarity;
step 07, making reasonable logic judgment according to the similarity, namely waiting for further processing of the qualified radioactive waste solidification structure with high similarity, and waiting for further processing of the unqualified radioactive waste solidification structure with low similarity or without a similar signal;
step 08, sampling the radioactive waste solidification structure, and performing performance test by adopting a traditional detection method;
step 09, the radioactive waste solidified structure determined to be unqualified in the steps 07 and 08 is crushed and re-manufactured into a new radioactive waste solidified structure to be detected, the detection is carried out again in the step 05, and the radioactive waste solidified structure determined to be qualified in the steps 07 and 08 is stored.
Further, the method for generating the proper pulsed X-rays by the X-ray emitting device comprises the following steps: the wavelength of the X-rays generated by the X-ray emitting device is adjusted, so that the radioactive waste solidified body can be used for collecting ultrasonic signals with good signals by the ultrasonic signal collector.
Further, sampling the radioactive waste solidification structure refers to sampling the radioactive waste solidification bodies which are judged to be qualified and unqualified in the step 07, performing performance test by adopting a traditional detection method to detect the accuracy of the judgment, and using the test data to enrich and correct the data of the ultrasonic signal comparison database.
Compared with the prior art, the invention has the following beneficial effects:
(1) According to the detection method for the radioactive waste curing structure based on XACT, the prepared standard sample is subjected to XACT detection, the standard sample is subjected to performance test by the traditional detection method, and then the ultrasonic signals of the qualified standard sample are extracted to establish a database capable of determining whether the detected radioactive waste curing structure reaches the industry and national standards. The ultrasonic signals of the radioactive waste curing structure to be detected are detected and collected through XACT, and compared with the data of the database, whether the radioactive waste curing structure to be detected is qualified or not can be rapidly judged, so that the radiation hazard caused by damaging a part of radioactive waste curing bodies in each detection is changed, and the problem that unqualified curing bodies are missed due to random spot check in the traditional detection mode is avoided.
(2) The radioactive waste solidified body which is judged to be qualified and unqualified after XACT detection is sampled at random, and the performance test is carried out by adopting a traditional detection method, so that the judgment accuracy of the batch of solidified structures is detected, the data supplement obtained by the test is fed into a database, and the database is continuously enriched, corrected and perfected, thereby continuously improving the accuracy of the data of the database and finding out the value of the best defined similarity. Over time, the detection method of damaging the solidified body of the waste in the conventional detection is completely replaced.
(3) According to the invention, by adjusting the wavelength of the X-rays generated by the X-ray emitting device, the radioactive waste solidified body can be used for collecting the ultrasonic signals with good signals by the ultrasonic signal collector, so that the detection accuracy is improved.
Drawings
Fig. 1 is a flowchart of a radioactive waste curing structure detection method based on XACT according to an embodiment of the present invention.
Fig. 2 is a schematic diagram of an XACT detection working principle according to an embodiment of the present invention.
In the above figures, the reference numerals correspond to the component names as follows:
1-X-ray suitable for different solidifying materials, 2-radioactive waste solidifying bodies of different materials, 3-ultrasonic signals converted by the X-ray and 4-ultrasonic signal acquisition devices.
Detailed Description
The invention will now be further described with reference to the accompanying drawings and examples, embodiments of which include, but are not limited to, the following examples.
Referring to fig. 1 to 2, a method for detecting a radioactive waste solidification structure based on XACT (X-ray Induced Acoustic Computed Tomography, X-ray excited acoustic tomography) includes the steps of:
and step 01, manufacturing a plurality of groups of radioactive waste solidified bodies according to different radioactive waste solidification modes. The multi-group radioactive waste solidified bodies with uniform structures are manufactured by different materials such as cement solidification, asphalt solidification, glass solidification and plastic solidification in a traditional mode, the radioactive waste solidified bodies are completely represented, and the radioactive waste solidified bodies are used as standard samples for subsequent acquisition of ultrasonic signals.
Step 02, irradiating the prepared radioactive waste solidified body, namely the standard sample, with suitable pulsed X-rays generated by an X-ray emission device. The wavelength of the X-rays generated by the X-ray emission device is adjusted, so that the radioactive waste solidified body can be collected by the ultrasonic signal collector to obtain an ultrasonic signal with good signal, and the detection accuracy is improved.
And 03, collecting ultrasonic signals converted by the pulsed X-rays produced by the X-ray emission device in the solidified body through an ultrasonic signal collector.
Step 04, the radioactive waste solidified bodies are subjected to performance test by a traditional detection method one by one, ultrasonic signals of the radioactive waste solidified bodies which are qualified in traditional detection are used as ultrasonic signal comparison databases for XACT detection, reliability of manual detection data after standard samples are strictly manufactured is achieved, reliable data are stored to establish databases reaching industry and national standards, accuracy is high, a more accurate and convenient mode is provided for subsequent detection, and meanwhile trouble is reduced for subsequent correction of the databases.
And 05, carrying out XACT detection on the radioactive waste solidification structure to be detected, and collecting ultrasonic signals of the radioactive waste solidification structure to be detected one by one.
And 06, comparing the ultrasonic signals of the detected radioactive waste solidification structure with the ultrasonic signals by using an acoustic wave similarity comparison tool to calculate the similarity of the data of the database. The sound wave similarity comparison tool is an existing software, such as Matlab, spss and other computer tools, calculates the similarity between the sound wave to be detected and the sound wave in the comparison database, and can refer to KTV singing to judge and score.
And step 07, making reasonable logic judgment according to the degree of similarity, namely waiting for further processing as a qualified radioactive waste solidification structure with high similarity, and waiting for further processing as an unqualified radioactive waste solidification structure with low similarity or without a similar signal. The starting similarity may be randomly determined by a value and then the size of this similarity is corrected by a subsequent sample check. For example, when the similarity value is initially higher, random detection finds that many cured structures that are judged to be unacceptable by taking the higher similarity value as a standard are acceptable, and then the similarity needs to be correspondingly reduced. Meanwhile, the similarity for the standard determination may be different depending on the radioactive material of the cured structure.
The ultrasonic signals of the radioactive waste curing structure to be detected are detected and collected through XACT, and compared with the data of the database, whether the radioactive waste curing structure to be detected is qualified or not can be rapidly judged, so that the radiation hazard caused by damaging a part of radioactive waste curing bodies in each detection is changed, and the problem that unqualified curing bodies are missed due to random spot check in the traditional detection mode is avoided.
And 08, sampling the radioactive waste solidification structure, and performing performance test by adopting a traditional detection method, so as to judge whether the radioactive waste solidification structure of the batch is accurate or not. And the data supplement obtained by the test is fed into the database, and the database is continuously enriched, corrected and perfected, so that the accuracy of the data of the database is continuously improved. Over time, the detection method of damaging the solidified body of the waste in the conventional detection is completely replaced.
Step 09, the radioactive waste solidification structure determined to be unqualified in step 07 and step 08 is crushed and re-manufactured into a new radioactive waste solidification structure to be detected, and the detection is carried out again in step 05, and the radioactive waste solidification structure determined to be qualified in step 07 and step 08 is subjected to waste storage, so that the accuracy of XACT detection is further improved.
The above embodiments are only preferred embodiments of the present invention, and not intended to limit the scope of the present invention, but all changes made by adopting the design principle of the present invention and performing non-creative work on the basis thereof shall fall within the scope of the present invention.

Claims (2)

1. A radioactive waste solidification structure detection method based on XACT, comprising the steps of:
step 01, manufacturing a plurality of groups of radioactive waste solidified bodies aiming at different radioactive waste solidification modes;
step 02, irradiating the prepared radioactive waste solidified body through suitable pulsed X-rays generated by an X-ray emission device;
step 03, collecting ultrasonic signals converted by pulsed X rays produced by an X-ray emission device in a solidified body through an ultrasonic signal collector;
step 04, the radioactive waste solidified bodies are subjected to performance test by a traditional detection method one by one, and ultrasonic signals of the radioactive waste solidified bodies which are qualified in detection are used as ultrasonic signal comparison databases of XACT detection;
step 05, performing XACT detection on the radioactive waste solidification structure to be detected, and collecting ultrasonic signals of the radioactive waste solidification structure to be detected one by one;
step 06, comparing the ultrasonic signals of the detected radioactive waste solidification structure with the data of the database by using an acoustic wave similarity comparison tool to calculate the similarity;
step 07, making reasonable logic judgment according to the similarity, namely waiting for further processing of the qualified radioactive waste solidification structure with high similarity, and waiting for further processing of the unqualified radioactive waste solidification structure with low similarity or without a similar signal; the initial similarity is a value determined randomly, and the size of the similarity is corrected through subsequent sampling inspection; if the similarity value is higher at first, random detection finds that many cured structures which are judged to be unqualified by taking the higher similarity value as a standard are qualified, and then the similarity needs to be correspondingly reduced at the moment; meanwhile, according to different radioactive materials of the curing structure, the similarity used for judging as a standard has certain difference;
step 08, sampling the radioactive waste solidification structure, and performing performance test by adopting a traditional detection method; the step of sampling the radioactive waste solidification structure refers to sampling the radioactive waste solidification structure which is judged to be qualified and unqualified in the step 07, performing performance test by adopting a traditional detection method so as to detect the accuracy of judgment, and using test data to enrich and correct the data of an ultrasonic signal comparison database;
step 09, the radioactive waste solidified structure determined to be unqualified in the steps 07 and 08 is crushed and re-manufactured into a new radioactive waste solidified structure to be detected, the detection is carried out again in the step 05, and the radioactive waste solidified structure determined to be qualified in the steps 07 and 08 is stored.
2. The method for detecting a radioactive waste solidification structure based on XACT according to claim 1, wherein the method for generating a suitable pulsed X-ray by the X-ray emitting device comprises: the wavelength of the X-rays generated by the X-ray emitting device is adjusted, so that the radioactive waste solidified body can be used for collecting ultrasonic signals with good signals by the ultrasonic signal collector.
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