CN111559789A - Rotary spiral bubbling dielectric barrier discharge pollutant treatment device - Google Patents
Rotary spiral bubbling dielectric barrier discharge pollutant treatment device Download PDFInfo
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- CN111559789A CN111559789A CN202010434745.4A CN202010434745A CN111559789A CN 111559789 A CN111559789 A CN 111559789A CN 202010434745 A CN202010434745 A CN 202010434745A CN 111559789 A CN111559789 A CN 111559789A
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- C—CHEMISTRY; METALLURGY
- C02—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F1/00—Treatment of water, waste water, or sewage
- C02F1/48—Treatment of water, waste water, or sewage with magnetic or electric fields
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
- B01D53/32—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols by electrical effects other than those provided for in group B01D61/00
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- B—PERFORMING OPERATIONS; TRANSPORTING
- B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
- B01D—SEPARATION
- B01D2259/00—Type of treatment
- B01D2259/80—Employing electric, magnetic, electromagnetic or wave energy, or particle radiation
- B01D2259/818—Employing electrical discharges or the generation of a plasma
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- C—CHEMISTRY; METALLURGY
- C02—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F2101/00—Nature of the contaminant
- C02F2101/30—Organic compounds
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- C—CHEMISTRY; METALLURGY
- C02—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F—TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
- C02F2201/00—Apparatus for treatment of water, waste water or sewage
- C02F2201/48—Devices for applying magnetic or electric fields
Abstract
The invention discloses a rotary spiral bubbling dielectric barrier discharge pollutant treatment device, which is characterized in that: comprises a water tank and a rotary spiral body; the water outlet of the water tank is connected with the water drainage pipe, the water inlet of the water tank is connected with the water inlet pipe, and the grounding electrode is grounded; the air inlet of the interface end of the rotary spiral body is connected with an air inlet pipe, and the high-voltage electrode is connected with a high-voltage power supply; the rotary spiral body is fixed in the water tank through a bearing, the position of the rotary spiral body is fixed but the rotary spiral body can rotate, and the interface end of the rotary spiral body is arranged outside the water tank and is connected with the motor through a belt, so that the whole rotary spiral body is driven to rotate; the surface of the rotary spiral body is provided with a plurality of micro channels, the spiral high-voltage electrode rod is wrapped in the rotary spiral body, and the micro channels are an aeration area and a discharge area during working. The invention can increase gas-liquid contact area during discharging, improve mass transfer efficiency and efficiently treat pollutants.
Description
Technical Field
The invention belongs to the technical field of pollutant treatment, and particularly relates to a rotary spiral bubbling dielectric barrier discharge pollutant treatment device.
Background
The environmental problem is one of the key problems which need to be solved urgently by human development, and the most urgent is how to treat the serious pollution of water resources. The treatment method for easily degradable sewage is mature and has good treatment effect, but the high-efficiency treatment method for high-concentration and difficultly degradable wastewater discharged by industries such as metallurgical electroplating, textile printing and dyeing, chemical pharmacy, petroleum/coal chemical industry and the like is urgently researched. At present, scholars at home and abroad mostly adopt an advanced oxidation technology to treat the high-concentration organic sewage, and the effectiveness of the technology is verified through theory and experiments, so that the technology becomes a research hotspot of the current global water treatment technology.
The material will exhibit different aggregation states at different temperature ranges or at different energy ranges. It is believed that plasma is a fourth type of material state of aggregation that is distinct from conventional solids, liquids, and gases. The natural plasma is widely present in the vast universe, and in fact 99% of the substances in the universe exist in a plasma state. The concept of the fourth physical state of plasma was proposed by the british physicist Crockes in 1879, but until 1928 the american chemist Langmuir first adopted "plasma" to mean the ionized gas produced by glow discharge, and "plasma" was translated into "plasma" at the earliest arrival in china and was later changed into "plasma".
Among advanced oxidation technologies, plasma water treatment technology is currently the focus of attention. It integrates the actions of high-energy electron radiation, ozone oxidation and ultraviolet light decomposition into one body, and can obtain good treatment effect. At present, dielectric barrier discharge, sliding arc discharge, corona discharge, glow discharge, radio frequency microwave discharge and the like are mainly adopted for generating plasma in water treatment.
Dielectric barrier discharge is an effective way to generate low temperature plasma, and particularly refers to a discharge form with insulating dielectric inserted into the discharge space. The dielectric barrier discharge can perform stable and uniform discharge at high voltage and normal pressure because the dielectric barrier discharge has the characteristics of corona discharge and glow discharge at the same time, and the electron density of the dielectric barrier discharge is high. Compared with other discharge forms, the dielectric barrier discharge form device has lower cost, higher energy utilization rate and higher energy utilization rate.
At present, a multi-type plasma reaction device is developed and applied to water treatment, but still has a plurality of defects which are difficult to overcome in the aspects of mass transfer, discharge efficiency improvement and the like. How to consider the promotion of the discharge efficiency and the enhancement of the mass transfer, thereby promoting the whole treatment efficiency, increasing the economic benefit and becoming the development direction of the plasma reaction device.
Disclosure of Invention
In view of one or more of the above-identified deficiencies in the prior art, the present invention provides a rotating spiral-bubble dielectric barrier discharge contaminant management device.
In order to achieve the above object, the present invention provides a device for treating pollutants by a rotating spiral bubbling dielectric barrier discharge, which is characterized in that: comprises a water tank (1) and a rotary spiral body (8); the water inlet (2) of the water tank (1) is connected with the water inlet pipe, the water outlet (3) is connected with the water drainage pipe, and the ground electrode (6) is grounded; the rotary spiral body (8) is connected with the water tank (1) through a bearing (7) and a hollow bearing (10), and the position of the rotary spiral body (8) is fixed but can rotate; the spiral electrode rod (9) is arranged in the rotary spiral body (8), the shape of the spiral electrode rod (9) is consistent with that of the rotary spiral body (8), but the diameter of the spiral electrode rod is slightly smaller; one end of the spiral electrode rod (9) penetrates through the hollow bearing (10) and enters the rotary interface end (11), and the spiral electrode rod (9) is cylindrical in the rotary interface end (11); a belt pulley (12) is arranged outside the rotary interface end (11) and is connected with an external motor through a belt, so that the rotary interface end (11), the spiral electrode rod (9) and the rotary spiral body (8) are driven to rotate; the rotary interface end (11) is connected with the fixed interface end (15) through a bearing 2 (14), the spiral electrode rod (9) in the fixed interface end (15) is connected with the high-voltage electrode interface (5) through a conductive bearing (13), and the high-voltage electrode interface (5) is connected with a high-voltage power supply high-voltage electrode; the fixed interface end (15) is connected with the air inlet (4) of the air inlet pipeline.
By adopting the scheme, when the device works, the external motor drives the rotary interface end (11) to rotate through the belt, and the rotary interface end (11) drives the rotary screw body (8) and the spiral electrode rod (9) to move through the hollow bearing (10); the treatment liquid enters the water tank (2) through the water inlet (2), the grounded ground electrode (6) is submerged, the rotary spiral body (8) is submerged, and finally the treatment liquid is discharged through the water discharge pipe (3); the air inlet (4) is connected with an air inlet pipeline, air enters the rotary spiral body (8) through the fixed interface end (15) and the rotary interface end (11), and liquid in the water tank is aerated through a micro-channel on the rotary spiral body (8); the spiral electrode bar (9) is connected with a high-voltage electrode of an external high-voltage power supply through a high-voltage electrode interface (5), the spiral electrode bar (9) is blocked by an insulating medium and discharges liquid in the water tank (1) through a micro-channel on the rotary spiral body (8), and the analysis of the working characteristics is as follows:
firstly, the treatment liquid is disturbed by its rotation due to the provision of the rotary screw (8).
Second, a plasma is formed by the discharge of the spiral electrode rod (9) to generate a large amount of active substances, which are aerated into the treatment liquid through the micro-channels on the rotating spiral body (8).
Thirdly, due to the disturbance and aeration of the rotary spiral body (8), the uniform and rapid diffusion of the active substances generated by the discharge is further accelerated.
Fourthly, when in discharge, the spiral electrode bar (9) is blocked by the insulating medium, so that spark discharge is avoided, uniform and stable plasma is obtained, and the discharge process has the advantages of short pulse delay, wide applicable voltage frequency range, strong adaptability and the like after being blocked by the insulating medium.
Fifth, due to the arrangement of the gas inlet (4), the plasma in the reactor can be generated in different gas phase components, so that different active substances can be generated to cope with different processing environments.
Sixthly, since the discharge area is near the liquid and is directly contacted with water, the discharge can be timely cooled, and the device can stably operate for a long time.
Furthermore, the spiral electrode bar (9) is made of cylindrical flaky and meshed conductive materials; the outer surface of the insulating layer is coated with a layer of insulating medium, which can be made of any one of ceramics, quartz glass and polytetrafluoroethylene.
Furthermore, the rotary spiral body (8) can be made of any one of ceramics, quartz glass and polytetrafluoroethylene materials; the outer surface of which contains a number of channels with a diameter of 100 microns.
Further, the hollow bearing (10) can adopt a pore plate to ensure that gas can smoothly pass through.
Furthermore, the high-voltage electrode interface (5) needs to be made of rigid materials, and an insulating layer with enough thickness needs to be arranged on the outer portion of the high-voltage electrode interface.
Furthermore, the conductive bearing (13) needs to be made of a conductive material to meet the high-voltage conductive requirement, and meanwhile, an insulating layer with enough thickness needs to be arranged outside.
Preferably, the bottom of the fixed interface end (15) can be provided with a fixed bracket to prevent the rotation of the rotary interface end (11) when rotating, and the bottom of the water tank (1) can be provided with a damping bracket to reduce the vibration caused by the rotation.
The invention has the beneficial effects that:
firstly, the treatment liquid is disturbed by its rotation due to the provision of the rotary screw (8).
Second, a plasma is formed by the discharge of the spiral electrode rod (9) to generate a large amount of active substances, which are aerated into the treatment liquid through the micro-channels on the rotating spiral body (8).
Thirdly, due to the disturbance and aeration of the rotary spiral body (8), the uniform and rapid diffusion of the active substances generated by the discharge is further accelerated.
Fourthly, when in discharge, the spiral electrode bar (9) is blocked by the insulating medium, so that spark discharge is avoided, uniform and stable plasma is obtained, and the discharge process has the advantages of short pulse delay, wide applicable voltage frequency range, strong adaptability and the like after being blocked by the insulating medium.
Fifth, due to the arrangement of the gas inlet (4), the plasma in the reactor can be generated in different gas phase components, so that different active substances can be generated to cope with different processing environments.
Sixthly, since the discharge area is near the liquid and is directly contacted with water, the discharge can be timely cooled, and the device can stably operate for a long time.
Seventh, the invention can be used for wastewater treatment, waste gas treatment, synchronous treatment of wastewater and waste gas, no selectivity to pollutants, and flexible treatment capacity.
Drawings
Fig. 1 is a general schematic of the present invention.
Fig. 2 is a schematic view of an interface end of the present invention.
Fig. 3 is a schematic view of a rotary screw of the present invention.
Detailed Description
The invention is further illustrated by the following examples in conjunction with the accompanying drawings:
example (b): referring to fig. 1: a rotating spiral bubbling dielectric barrier discharge pollutant treatment device is characterized in that: comprises a water tank (1) and a rotary spiral body (8);
the water inlet (2) of the water tank (1) is connected with the water inlet pipe, the water outlet (3) is connected with the water drainage pipe, and the ground electrode (6) is grounded; the rotary spiral body (8) is connected with the water tank (1) through a bearing (7) and a hollow bearing (10), and the position of the rotary spiral body (8) is fixed but can rotate;
the spiral electrode rod (9) is arranged in the rotary spiral body (8), the shape of the spiral electrode rod (9) is consistent with that of the rotary spiral body (8), but the diameter of the spiral electrode rod is slightly smaller; one end of the spiral electrode rod (9) penetrates through the hollow bearing (10) and enters the rotary interface end (11), and the spiral electrode rod (9) is cylindrical in the rotary interface end (11);
a belt pulley (12) is arranged outside the rotary interface end (11) and is connected with an external motor through a belt, so that the rotary interface end (11), the spiral electrode rod (9) and the rotary spiral body (8) are driven to rotate; the rotary interface end (11) is connected with the fixed interface end (15) through a bearing 2 (14), the spiral electrode rod (9) in the fixed interface end (15) is connected with the high-voltage electrode interface (5) through a conductive bearing (13), and the high-voltage electrode interface (5) is connected with a high-voltage power supply high-voltage electrode; the fixed interface end (15) is connected with the air inlet (4) of the air inlet pipeline.
Furthermore, the spiral electrode bar (9) is made of cylindrical flaky and meshed conductive materials; the outer surface of the insulating layer is coated with a layer of insulating medium, which can be made of any one of ceramics, quartz glass and polytetrafluoroethylene.
Furthermore, the rotary spiral body (8) can be made of any one of ceramics, quartz glass and polytetrafluoroethylene materials; the outer surface of which contains a number of channels with a diameter of 100 microns.
Further, the hollow bearing (10) can adopt a pore plate to ensure that gas can smoothly pass through.
Furthermore, the high-voltage electrode interface (5) needs to be made of rigid materials, and an insulating layer with enough thickness needs to be arranged on the outer portion of the high-voltage electrode interface.
Furthermore, the conductive bearing (13) needs to be made of a conductive material to meet the high-voltage conductive requirement, and meanwhile, an insulating layer with enough thickness needs to be arranged outside.
Preferably, the bottom of the fixed interface end (15) can be provided with a fixed bracket to prevent the rotation of the rotary interface end (11) when rotating, and the bottom of the water tank (1) can be provided with a damping bracket to reduce the vibration caused by the rotation.
In addition, a water supply device can be arranged in front of the water inlet (2), an air supply device can be arranged in front of the air inlet (4), and the belt pulley (12) can be connected with a motor through a belt.
When the spiral electrode rotating machine works, an external motor drives a rotating interface end (11) to rotate through a belt, the rotating interface end (11) drives a rotating spiral body (8) and a spiral electrode rod (9) to move through a hollow bearing (10), and the rotating speed is maintained at 60 r/min; the treatment liquid enters the water tank (2) through the water inlet (2), the grounded ground electrode (6) is submerged, the rotary spiral body (8) is submerged, and finally the treatment liquid is discharged through the water discharge pipe (3); the air inlet (4) is connected with an air inlet pipeline, air enters the rotary spiral body (8) through the fixed interface end (15) and the rotary interface end (11), and liquid in the water tank is aerated through a micro-channel on the rotary spiral body (8); the spiral electrode bar (9) is connected with a high-voltage electrode of an external high-voltage power supply through a high-voltage electrode interface (5), the spiral electrode bar (9) is blocked by an insulating medium and discharges liquid in the water tank (1) through a micro-channel on the rotary spiral body (8), and the analysis of the working characteristics is as follows:
firstly, the treatment liquid is disturbed by its rotation due to the provision of the rotary screw (8).
Second, a plasma is formed by the discharge of the spiral electrode rod (9) to generate a large amount of active substances, which are aerated into the treatment liquid through the micro-channels on the rotating spiral body (8).
Thirdly, due to the disturbance and aeration of the rotary spiral body (8), the uniform and rapid diffusion of the active substances generated by the discharge is further accelerated.
Fourthly, when in discharge, the spiral electrode bar (9) is blocked by the insulating medium, so that spark discharge is avoided, uniform and stable plasma is obtained, and the discharge process has the advantages of short pulse delay, wide applicable voltage frequency range, strong adaptability and the like after being blocked by the insulating medium.
Fifth, due to the arrangement of the gas inlet (4), the plasma in the reactor can be generated in different gas phase components, so that different active substances can be generated to cope with different processing environments.
Sixthly, since the discharge area is near the liquid and is directly contacted with water, the discharge can be timely cooled, and the device can stably operate for a long time.
The invention has three working states:
firstly, only organic wastewater is treated; this state is also the main working state of the device; firstly, wastewater is introduced from a water inlet (2), then gas is introduced from a gas inlet (4), then a motor is started to enable a rotary spiral body (8) to start rotating, when the grounded ground electrode (6) is submerged in the wastewater firstly and then the rotary spiral body (8) is submerged, and the micro-channel on the rotary spiral body (8) starts aeration, a high-voltage power supply is started to start discharge treatment, and the wastewater finally flows out from a water outlet (3), so that the long-term stable operation can be realized.
Secondly, only organic waste gas is treated; firstly, tap water is introduced from the water inlet (2), then waste gas is introduced from the air inlet (4), then the motor is started to enable the rotary spiral body (8) to start rotating, when the tap water submerges the grounded ground electrode (6) and then submerges the rotary spiral body (8), and the micro-channel on the rotary spiral body (8) starts aeration, the high-voltage power supply is started to start discharge treatment, and the tap water flows out from the water outlet (3), so that the long-term stable operation can be realized.
Thirdly, synchronously treating the waste water and the waste gas; firstly, wastewater is introduced from a water inlet (2), then waste gas is introduced from an air inlet (4), then a motor is started to enable a rotary spiral body (8) to start rotating, when the grounded ground electrode (6) is submerged in the wastewater and then the rotary spiral body (8) is submerged, and the micro-channel on the rotary spiral body (8) starts aeration, a high-voltage power supply is started to start discharge treatment, the wastewater flows out from a water outlet (3), and the long-term stable operation can be realized.
Therefore, the invention can be used for treating waste water and waste gas, and can realize the synchronous treatment of waste water and waste gas.
The foregoing detailed description of the preferred embodiments of the invention has been presented. It should be understood that numerous modifications and variations could be devised by those skilled in the art in light of the present teachings without departing from the inventive concepts. Therefore, the technical solutions available to those skilled in the art through logic analysis, reasoning and limited experiments based on the prior art according to the concept of the present invention should be within the scope of protection defined by the claims.
Claims (7)
1. The invention discloses a rotary spiral bubbling dielectric barrier discharge pollutant treatment device, which is characterized in that: comprises a water tank (1) and a rotary spiral body (8);
the water inlet (2) of the water tank (1) is connected with the water inlet pipe, the water outlet (3) is connected with the water drainage pipe, and the ground electrode (6) is grounded; the rotary spiral body (8) is connected with the water tank (1) through a bearing (7) and a hollow bearing (10), and the position of the rotary spiral body (8) is fixed but can rotate;
the spiral electrode rod (9) is arranged in the rotary spiral body (8), the shape of the spiral electrode rod (9) is consistent with that of the rotary spiral body (8), but the diameter of the spiral electrode rod is slightly smaller; one end of the spiral electrode rod (9) penetrates through the hollow bearing (10) and enters the rotary interface end (11), and the spiral electrode rod (9) is cylindrical in the rotary interface end (11);
a belt pulley (12) is arranged outside the rotary interface end (11) and is connected with an external motor through a belt, so that the rotary interface end (11), the spiral electrode rod (9) and the rotary spiral body (8) are driven to rotate; the rotary interface end (11) is connected with the fixed interface end (15) through a bearing 2 (14), the spiral electrode rod (9) in the fixed interface end (15) is connected with the high-voltage electrode interface (5) through a conductive bearing (13), and the high-voltage electrode interface (5) is connected with a high-voltage power supply high-voltage electrode; the fixed interface end (15) is connected with the air inlet (4) of the air inlet pipeline.
2. A spiral-bubble dielectric barrier discharge contaminant treatment device, as claimed in claim 1, wherein: the spiral electrode bar (9) is made of cylindrical flaky and meshed conductive materials; the outer surface of the insulating layer is coated with a layer of insulating medium, which can be made of any one of ceramics, quartz glass and polytetrafluoroethylene.
3. A spiral-bubble dielectric barrier discharge contaminant treatment device, as claimed in claim 1, wherein: the rotary spiral body (8) can be made of any one of ceramics, quartz glass and polytetrafluoroethylene materials; the outer surface of which contains a number of channels with a diameter of 100 microns.
4. A spiral-bubble dielectric barrier discharge contaminant treatment device, as claimed in claim 1, wherein: the hollow bearing (10) can adopt a pore plate to ensure that gas can smoothly pass through.
5. A spiral-bubble dielectric barrier discharge contaminant treatment device, as claimed in claim 1, wherein: the high-voltage electrode interface (5) is made of rigid materials, and an insulating layer with enough thickness is required on the outer portion.
6. A spiral-bubble dielectric barrier discharge contaminant treatment device, as claimed in claim 1, wherein: the conductive bearing (13) needs to be made of a conductive material to meet the high-voltage conductive requirement, and meanwhile, an insulating layer with enough thickness needs to be arranged outside.
7. A spiral-bubble dielectric barrier discharge contaminant treatment device, as claimed in claim 1, wherein: the bottom of the fixed interface end (15) can be provided with a fixed support to prevent the rotation of the rotary interface end (11), and the bottom of the water tank (1) can be provided with a damping support to reduce the vibration caused by the rotation.
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Cited By (1)
Publication number | Priority date | Publication date | Assignee | Title |
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CN113828252A (en) * | 2021-09-22 | 2021-12-24 | 湖南大学 | Novel efficient reaction device for preparing ammonia by low-temperature plasma concerted catalysis |
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