CN109266307A - A kind of high-temp resistant fire-retarding type adhesive waterproof coil - Google Patents
A kind of high-temp resistant fire-retarding type adhesive waterproof coil Download PDFInfo
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- CN109266307A CN109266307A CN201811134248.1A CN201811134248A CN109266307A CN 109266307 A CN109266307 A CN 109266307A CN 201811134248 A CN201811134248 A CN 201811134248A CN 109266307 A CN109266307 A CN 109266307A
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- type adhesive
- adhesive waterproof
- asphalt
- resistant fire
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- C—CHEMISTRY; METALLURGY
- C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
- C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
- C09J195/00—Adhesives based on bituminous materials, e.g. asphalt, tar, pitch
-
- C—CHEMISTRY; METALLURGY
- C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
- C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
- C09J11/00—Features of adhesives not provided for in group C09J9/00, e.g. additives
- C09J11/02—Non-macromolecular additives
- C09J11/04—Non-macromolecular additives inorganic
-
- C—CHEMISTRY; METALLURGY
- C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
- C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
- C09J7/00—Adhesives in the form of films or foils
- C09J7/30—Adhesives in the form of films or foils characterised by the adhesive composition
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K3/00—Use of inorganic substances as compounding ingredients
- C08K3/18—Oxygen-containing compounds, e.g. metal carbonyls
- C08K3/20—Oxides; Hydroxides
- C08K3/22—Oxides; Hydroxides of metals
- C08K2003/2217—Oxides; Hydroxides of metals of magnesium
- C08K2003/2224—Magnesium hydroxide
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K3/00—Use of inorganic substances as compounding ingredients
- C08K3/18—Oxygen-containing compounds, e.g. metal carbonyls
- C08K3/24—Acids; Salts thereof
- C08K3/26—Carbonates; Bicarbonates
- C08K2003/265—Calcium, strontium or barium carbonate
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2201/00—Properties
- C08L2201/02—Flame or fire retardant/resistant
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2201/00—Properties
- C08L2201/08—Stabilised against heat, light or radiation or oxydation
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2205/00—Polymer mixtures characterised by other features
- C08L2205/02—Polymer mixtures characterised by other features containing two or more polymers of the same C08L -group
- C08L2205/025—Polymer mixtures characterised by other features containing two or more polymers of the same C08L -group containing two or more polymers of the same hierarchy C08L, and differing only in parameters such as density, comonomer content, molecular weight, structure
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2205/00—Polymer mixtures characterised by other features
- C08L2205/03—Polymer mixtures characterised by other features containing three or more polymers in a blend
- C08L2205/035—Polymer mixtures characterised by other features containing three or more polymers in a blend containing four or more polymers in a blend
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2207/00—Properties characterising the ingredient of the composition
- C08L2207/10—Peculiar tacticity
Abstract
The present invention provides a kind of high-temp resistant fire-retarding type adhesive waterproof coils, including upper surface isolation film, self-adhesion sizing material, tire base and lower surface isolation film；The self-adhesion sizing material, raw material including following parts by weight, 70# asphalt or 10-20 parts of 20-30 parts of 90# asphalt, 5-10 parts of 10# asphalt, aromatic naphtha and cycloalkanes oil mixture, 20-30 parts of SBS modifier, 5-10 parts of polypropylene, 5-10 parts of phenolic resin, 5-10 parts of SBR, 10-15 parts of rubber powder, 5-10 parts of light calcium, fire retardant 2-6 parts of mixing.A kind of high-temp resistant fire-retarding type adhesive waterproof coil provided by the invention, traditional adhesive waterproof coil is overcome because the low coiled material under high temperature environment of high temperature resistance is not easy to construct, the mutability under long term high temperature environment, disadvantage easy to aging, and the invention has good flame retardant effect, and adhesive strength is bigger.
Description
Technical field
The invention belongs to water-proof building material technical fields, more particularly, to a kind of high-temp resistant fire-retarding type self-adhesion waterproof roll
Material.
Background technique
Adhesive waterproof coil is because of its easy construction, and the advantages that good water-proof effect, market is using more and more extensive.But due to certainly
The high temperature resistant of viscous waterproof roll only has 70 degree, and mutability causes construction inconvenient under high temperature environment, for a long time shadow under high temperature environment
Ring service life.Unnecessary loss is easily caused along with flammability is easy under high temperature, waterproof effect is influenced, leads to anti-water system
The failure of system.
Summary of the invention
In view of this, the present invention is directed to propose a kind of high-temp resistant fire-retarding type adhesive waterproof coil, high temperature resistant of the present invention reach
110 DEG C, easily-deformable under high temperature environment to overcome, easy firing, adhesive strength is reduced significantly, and the service life of waterproof roll is low etc.
Situation greatlys improve the service life of coiled material since mixture is modified.
In order to achieve the above objectives, the technical scheme of the present invention is realized as follows:
A kind of high-temp resistant fire-retarding type adhesive waterproof coil, including upper surface isolation film, self-adhesion sizing material, tire base and lower surface
Isolation film；
70# asphalt or 20-30 parts of 90# asphalt, 5-10 parts of 10# pitch, aromatic naphtha and cycloalkanes oil mixture 10-
20 parts, 20-30 parts of SBS modifier (1401 and 4303 mixtures), 5-10 parts of polypropylene, 5-10 parts of phenolic resin, SBR 5-
10 parts, 10-15 parts of rubber powder, 5-10 parts of light calcium mix fire retardant 2-6 parts.
Preferably, the 10# pitch, index are as follows:
| Project | Technical indicator |
| Needle penetration | 8-13 |
| Ductility | ≥30mm |
| Softening point | ≥100℃ |
Preferably, the naphthenic oil, index are as follows:
| Project | Technical indicator |
| Viscosity | 2000—6000map.s |
| Flash-point | ≥200℃ |
| Pour point | It -25 DEG C, easily flows |
Preferably, the asphalt is the heavy-duty road asphalt oil of middle Petroleum Production, model 70# or 90#
One kind, index is as follows:
The phenolic resin, index are as follows:
The aromatic naphtha is preferably the hydrocarbon containing phenyl ring, and index is as follows:
| Project | Technical indicator |
| Appearance | Black is bright, free from admixture, free from extraneous odour |
| Pour point | - 25 DEG C of 4h flowings |
| Flash-point | ≥200℃ |
The SBR modifying agent is the monomers such as graft phenylethene and the butadiene-styrene rubber that generates on the basis of butadiene-styrene rubber, it
Other than having the characteristics that significantly improve the cryogenic property of pitch, also have the characteristics that be obviously improved high temperature performance of asphalt, skill
Art index is as follows:
| Project | Technical indicator |
| Appearance | Without agglomeration, milky, no-sundries |
| Ash content | ≤ 55% |
The SBS modifier is the mixture of SBS1401 and SBS4303.
Preferably, in aromatic naphtha and cycloalkanes oil mixture, the mass ratio of aromatic naphtha and naphthenic oil be 1:(1~: 1.5)；Institute
Stating SBS modifier is SBS1401 and SBS4303 mixture；And the two mass ratio is 1:(1~2).
Preferably, the rubber powder is rubber powder, and mesh number is 40 mesh, and 40 mesh percent of pass are >=95%.The SBR is
Butadiene-styrene rubber, ash content≤55%.
PP GRANULES (pp) is preferably isotactic polypropylene resin, which has excellent UV resistant irradiation and resistance to old
Change performance, when poly- third particle is added to heated bitumen, when asphalt temperature is between 160~180 DEG C, poly- third particle is stirred in blender
Uniform mixture is formed in sticky state and pitch under the action of paddle, improves the weak of pitch easily-deformable trickling under the high temperature conditions
Point, index are as follows:
The light calcium is preferably precipitated calcium carbonate, and index is as follows:
The mixing fire retardant, magnesium hydroxide, index are as follows；
| Project | Technical indicator |
| Content of magnesia >= | 63.0 |
| Calcium oxide content≤ | 1.0 |
| Acid non-soluble substance content≤ | 0.2 |
| Moisture≤ | 2.5 |
| Chloride content≤ | 0.15 |
| Iron content≤ | 0.25 |
| Calcination vector >= | 28.0 |
| Sieve residue (75 μm of testing sieves)≤ | 0.5 |
The present invention also provides a kind of method for preparing high-temp resistant fire-retarding type adhesive waterproof coil as described above, including it is as follows
Preparation step, 20-30 parts of 70# or 90# asphalt, 5-10 parts of 10# pitch, aromatic naphtha and 10-20 parts of cycloalkanes oil mixture；It presses
Formula rate metering, is added to above-mentioned raw materials in 1# agitator tank, 165 DEG C -170 DEG C of heating temperature, again to melt completely after metering
Change and 5-10 parts of 20-30 parts of SBS modifier (1401 and 4303 mixture), polypropylene agitating and heatings, 170 DEG C of heating temperature-is added
180 DEG C until particle melts completely；Then 5-10 parts of phenolic resin are added simultaneously, 5-10 parts of SBR, 10-15 parts of rubber powder, mixing
2-6 parts of agitating and heatings of fire retardant, 170 DEG C -180 DEG C of temperature, until particle thawing stirs evenly (60-90min)；Pass through colloid again
The material of 1# tank is poured into 2# material-compound tank by colloid mill, is eventually adding light calcium temperature by mill grinding, milling time >=60min
165 DEG C -175 DEG C of degree stirs (90-120min), the material prepared is added to centre using Melt Pump after stirring
In material stock tank；
Material in intermediate material stock tank is put into painting oil sump, by roller by self-adhesion sizing material being coated uniformly on property tire base,
Application temperature is 170-180 DEG C, while compound upper isolation film, cools down through sizing, obtains high-temp resistant fire-retarding type adhesive waterproof coil
High-temp resistant fire-retarding type adhesive waterproof coil provided by the invention has good high temperature resistance, flame retardant property waterproof
Performance and preferable ageing-resistant performance, relative to existing high-temp resistant fire-retarding type adhesive waterproof coil have longer service life,
Easy construction, better waterproof performance are set fire engineering especially suitable for high temperature.Simultaneously because raw material are easy to get, preparation process letter
Just, easy for construction, securely and reliably, so that it is of the invention, suitable for large-scale industrial production and it is widely used.
Comprehensive difference of the high-temp resistant fire-retarding type adhesive waterproof coil provided by the invention in performance see the table below 1.
Table 1
Specific embodiment
In addition to being defined, technical term used in following embodiment has universal with those skilled in the art of the invention
The identical meanings of understanding.Test reagent used in following embodiment is unless otherwise specified conventional biochemical reagent；It is described
Experimental method is unless otherwise specified conventional method.
Below with reference to embodiment, the present invention will be described in detail.
Embodiment 1
By 22 parts of 70# asphalt, 8 parts of 10# pitch, (aromatic naphtha and cycloalkanes oil mixture, and the mass ratio of the two be 1:
1) 12 parts,；It measures by formula rate, above-mentioned raw materials is added in 1# agitator tank again after metering, 165 DEG C -170 of heating temperature
DEG C, to melt 22 parts of addition SBS modifier (SBS1401 and 4303 mixtures, and the mass ratio of the two is 1:1.2) completely, gather
6 parts of agitating and heatings of propylene, 170 DEG C -180 DEG C of heating temperature is until particle melts completely；Then 6 parts of phenolic resin are added simultaneously,
2 parts of 7 parts of SBR, 15 parts of rubber powder, fire retardant (magnesium hydroxide) agitating and heatings, 170 DEG C -180 DEG C of temperature, until particle melts stirring
Uniformly (60-90min)；It is ground again by colloid mill, the material of 1# tank is poured by milling time >=60min by colloid mill
In 2# material-compound tank, 165 DEG C -175 DEG C of light calcium temperature are eventually adding, is stirred (90-120min), melt is utilized after stirring
The material prepared is added in intermediate material stock tank by pump；
Material in intermediate material stock tank is put into painting oil sump, by roller by self-adhesion sizing material being coated uniformly on property tire base,
Application temperature is 170-180 DEG C, while compound upper isolation film, cools down through sizing, obtains high-temp resistant fire-retarding type adhesive waterproof coil.
Embodiment 2
By 24 parts of 70# asphalt, 6 parts of 10# pitch, (aromatic naphtha and cycloalkanes oil mixture, and the mass ratio 1 of the two:
1.3) 14 parts；It measures by formula rate, above-mentioned raw materials is added in 1# agitator tank again after metering, 165 DEG C -170 of heating temperature
DEG C, to melt completely be added 24 parts of SBS modifier (SBS1401 and SBS4303 mixture, and the mass ratio of the two is 1:1.5),
7 parts of agitating and heatings of polypropylene, 170 DEG C -180 DEG C of heating temperature is until particle melts completely；Then phenolic resin 5 is added simultaneously
Part, SBR5 parts, 2 parts of 13 parts of rubber powder, fire retardant (magnesium hydroxide) agitating and heatings, 170 DEG C -180 DEG C of temperature, until particle thawing is stirred
Mix uniform (60-90min)；It is ground again by colloid mill, milling time >=60min pours into the material of 1# tank by colloid mill
Into 2# material-compound tank, 165 DEG C -175 DEG C of light calcium temperature are eventually adding, is stirred (90-120min), using molten after stirring
The material prepared is added in intermediate material stock tank by body pump；
Material in intermediate material stock tank is put into painting oil sump, by roller by self-adhesion sizing material being coated uniformly on property tire base,
Application temperature is 170-180 DEG C, while compound upper isolation film, cools down through sizing, obtains high-temp resistant fire-retarding type adhesive waterproof coil.
Embodiment 3
By 25 parts of 70# asphalt, 5 parts of 10# pitch, (aromatic naphtha and cycloalkanes oil mixture, and the two mass ratio 1:1.5)
15 parts；It measures by formula rate, above-mentioned raw materials is added in 1# agitator tank again after metering, 165 DEG C -170 DEG C of heating temperature, to
Melt completely and 25 parts, 7 parts of polypropylene of SBS modifier (SBS1404 and 4303 mixtures, and the mass ratio of the two is 1:2) is added
Agitating and heating, 170 DEG C -180 DEG C of heating temperature is until particle melts completely；Then 6 parts of phenolic resin are added simultaneously, 5 parts of SBR,
2 parts of 10 parts of rubber powder, fire retardant (magnesium hydroxide) agitating and heatings, 170 DEG C -180 DEG C of temperature, until particle thawing stirs evenly (60-
90min)；It is ground again by colloid mill, the material of 1# tank is poured into 2# material-compound tank by colloid mill by milling time >=60min
In, 165 DEG C -175 DEG C of light calcium temperature are eventually adding, stirs (90-120min), will be prepared after stirring using Melt Pump
Material be added in intermediate material stock tank；
Material in intermediate material stock tank is put into painting oil sump, by roller by self-adhesion sizing material being coated uniformly on property tire base,
Application temperature is 170-180 DEG C, while compound upper isolation film, cools down through sizing, obtains high-temp resistant fire-retarding type adhesive waterproof coil.
Embodiment 4
Using the preparation method of same embodiment 1, self-adhesion sizing material other compositions are constant, change 70# pitch in formula into 90# drip
A kind of high-temp resistant fire-retarding type self-adhesive coiled material that blueness obtains.
Comparative example 1
Using the preparation method of same embodiment 1, self-adhesion sizing material other compositions are constant, change 70# pitch in formula into 90# drip
A kind of high-temp resistant fire-retarding type self-adhesive coiled material of fire retardant acquisition is not added in blueness, self-adhesion prescription of mixed materials
The various embodiments described above and the performance test results of comparative example product obtained are as shown in the table.
The foregoing is merely illustrative of the preferred embodiments of the present invention, is not intended to limit the invention, all in essence of the invention
Within mind and principle, any modification, equivalent replacement, improvement and so on be should all be included in the protection scope of the present invention.
Claims (10)
1. a kind of high-temp resistant fire-retarding type adhesive waterproof coil, it is characterised in that: including upper surface isolation film, self-adhesion sizing material, tire base
And lower surface isolation film；
The self-adhesion sizing material, the raw material including following parts by weight, 70# asphalt or 20-30 parts of 90# asphalt, 10# stone
10-20 parts of 5-10 parts of oil asphalt, aromatic naphtha and cycloalkanes oil mixture, 20-30 parts of SBS modifier, 5-10 parts of polypropylene, phenolic aldehyde tree
5-10 parts of rouge, 5-10 parts of SBR, 10-15 parts of rubber powder, 5-10 parts of light calcium, fire retardant 2-6 parts of mixing.
2. high-temp resistant fire-retarding type adhesive waterproof coil according to claim 1, it is characterised in that: the 70# asphalt
Needle penetration 60-80, softening point >=50 DEG C, ductility >=1000mm；The needle penetration 80-90 of the 90# asphalt, softening point >=
50 DEG C, ductility >=1000mm；The needle penetration 8-13 of the 10# asphalt, softening point >=100 DEG C, ductility >=30mm.
3. high-temp resistant fire-retarding type adhesive waterproof coil according to claim 1, it is characterised in that: aromatic naphtha and naphthenic oil are mixed
Close in object, the mass ratio of aromatic naphtha and naphthenic oil be 1:(1~: 1.5)；The SBS modifier is SBS1401 and SBS4303 mixed
Close object；And the two mass ratio is 1:(1~2).
4. high-temp resistant fire-retarding type adhesive waterproof coil according to claim 1, it is characterised in that: the phenolic resin specific gravity
1.18-1.22,95 DEG C -115 DEG C of softening point, free phenol content 0.5%-3.5%.
5. high-temp resistant fire-retarding type adhesive waterproof coil according to claim 1, it is characterised in that: the aromatic naphtha dodges
Point >=200 DEG C can be flowed under -20 DEG C of low-temperature conditions of pour point, viscosity >=6000mpa.s/25 DEG C；The naphthenic oil, flash-point >=
It 200 DEG C, can flow under -25 DEG C of low-temperature conditions of pour point, viscosity >=2000mpa.s/25 DEG C.
6. high-temp resistant fire-retarding type adhesive waterproof coil according to claim 1, it is characterised in that: the rubber powder is rubber powder
End, 40 mesh percent of pass are >=95%；The SBR is butadiene-styrene rubber, ash content≤55%；The polypropylene, melting refer to
Number >=15g/10min.
7. high-temp resistant fire-retarding type adhesive waterproof coil according to claim 1, it is characterised in that: the light calcium, it is aqueous
Amount≤0.1%, fineness: 200 mesh percent of pass >=95%.
8. high-temp resistant fire-retarding type adhesive waterproof coil according to claim 1, it is characterised in that: the mixing fire retardant is
Magnesium hydroxide.
9. a kind of method for preparing high-temp resistant fire-retarding type adhesive waterproof coil as described in any one of claims 1 to 8, feature
It is: includes the following steps, by 70# asphalt or 20-30 parts of 90# asphalt, 5-10 parts of 10# pitch, aromatic naphtha and ring
10-20 parts of alkane oil mixture；It measures, above-mentioned raw materials is added in 1# agitator tank again after metering, heating temperature by formula rate
165 DEG C -170 DEG C, 5-10 parts of SBS modifier 20-30 parts, polypropylene agitating and heatings, heating temperature 170 is added to melt completely
DEG C -180 DEG C until particle melts completely；Then 5-10 parts of phenolic resin are added simultaneously, 5-10 parts of SBR, 10-15 parts of rubber powder, mixes
Fire retardant 2-6 parts of agitating and heating is closed, 170 DEG C -180 DEG C of temperature, is stirred evenly until particle melts, mixing time 60-
90min；It is ground again by colloid mill, the material of 1# tank is poured into 2# material-compound tank by colloid mill by milling time >=60min
In, it is eventually adding 165 DEG C -175 DEG C of light calcium temperature, stirs 90-120min, will be prepared after stirring using Melt Pump
Material is added in intermediate material stock tank；
Material in intermediate material stock tank is put into painting oil sump, by, by self-adhesion sizing material being coated uniformly on property tire base, coating to roller
Temperature is 170-180 DEG C, while compound upper isolation film, cools down through sizing, obtains high-temp resistant fire-retarding type adhesive waterproof coil.
10. described in any item high-temp resistant fire-retarding type adhesive waterproof coils or as claimed in claim 9 according to claim 1~8
Application of the waterproof roll that preparation method obtains in water proof building or water-proof building material.
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| CN201811134248.1A CN109266307A (en) | 2018-09-27 | 2018-09-27 | A kind of high-temp resistant fire-retarding type adhesive waterproof coil |
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| CN110041826A (en) * | 2019-04-23 | 2019-07-23 | 临沂木子原热能科技有限公司 | A kind of new waterproof film |
| CN110054904A (en) * | 2019-04-25 | 2019-07-26 | 山东红花防水建材有限公司 | A kind of high-polymer self-adhesion waterproof coiled material and preparation method thereof, application |
| CN111978920A (en) * | 2020-08-26 | 2020-11-24 | 甘肃宇邦建筑防水材料有限公司 | Anti-aging waterproof self-adhesive coiled material and preparation method thereof |
| CN113969135A (en) * | 2021-10-26 | 2022-01-25 | 中国石油化工股份有限公司 | Reactive self-adhesive waterproof coiled material and preparation method and application thereof |
| CN114591631A (en) * | 2022-04-26 | 2022-06-07 | 河南蓝翎环科防水材料有限公司 | Asphalt-based synthetic polymer waterproof material and production process thereof |
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| CN110041826A (en) * | 2019-04-23 | 2019-07-23 | 临沂木子原热能科技有限公司 | A kind of new waterproof film |
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