USH558H - Radation shielding pellets - Google Patents

Radation shielding pellets Download PDF

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Publication number
USH558H
USH558H US07/020,070 US2007087A USH558H US H558 H USH558 H US H558H US 2007087 A US2007087 A US 2007087A US H558 H USH558 H US H558H
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United States
Prior art keywords
pellets
shielding
outer shell
melting point
radiation
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Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Abandoned
Application number
US07/020,070
Inventor
Edmund P. Coomes
Andrzej T. Luksic
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US Department of Energy
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US Department of Energy
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Publication date
Application filed by US Department of Energy filed Critical US Department of Energy
Priority to US07/020,070 priority Critical patent/USH558H/en
Application granted granted Critical
Publication of USH558H publication Critical patent/USH558H/en
Abandoned legal-status Critical Current

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    • GPHYSICS
    • G21NUCLEAR PHYSICS; NUCLEAR ENGINEERING
    • G21FPROTECTION AGAINST X-RADIATION, GAMMA RADIATION, CORPUSCULAR RADIATION OR PARTICLE BOMBARDMENT; TREATING RADIOACTIVELY CONTAMINATED MATERIAL; DECONTAMINATION ARRANGEMENTS THEREFOR
    • G21F3/00Shielding characterised by its physical form, e.g. granules, or shape of the material
    • G21F3/04Bricks; Shields made up therefrom
    • GPHYSICS
    • G21NUCLEAR PHYSICS; NUCLEAR ENGINEERING
    • G21FPROTECTION AGAINST X-RADIATION, GAMMA RADIATION, CORPUSCULAR RADIATION OR PARTICLE BOMBARDMENT; TREATING RADIOACTIVELY CONTAMINATED MATERIAL; DECONTAMINATION ARRANGEMENTS THEREFOR
    • G21F1/00Shielding characterised by the composition of the materials
    • G21F1/02Selection of uniform shielding materials

Definitions

  • This invention relates in general to radiation shielding means, and more particularly to radiation shielding pellets containing at least two shielding materials within individual pellets.
  • Radiation shields often contain more than one type of material in order to provide attentuation over the entire spectrum of incident radiation.
  • One common type of shielding application requires a gamma ray shielding metal such as tungsten or steel in combination with a hydrogen-rich neutron shielding material such as lithium hydride.
  • the radiation shield Since the radiation shield must provide uniform attenuation over a large surface area, the two required materials must be prevented from separating within the shield. This means that lithium hydride in a shield must be trapped in place. If it is allowed to liquify or form vapor bubbles, portions of the shield volume will come to have an incorrect ratio of LiH versus metal, and shielding will not be uniform.
  • Prior art shielding systems have dealt with this problem by attempting to maintain all portions of the shield below the melting point of LiH.
  • the interior of the shield was filled with a honeycomb-like structure of tungsten or steel with LiH placed in the cells of the honeycomb.
  • the metallic honeycomb conducted heat away from the LiH and to the outer surface of the shield.
  • honeycomb structures are difficult to fabricate, particularly if an active cooling means, such as a fluid flow heat removal system, is required.
  • honeycombs and cooling pipes required to maintain LiH in solid form tend to be heavy. This makes them undesirable for use in systems requiring active cooling which must be launched into space.
  • shielding materials into pellets, wherein the exterior of each capsule is formed of a high melting point gamma ray shielding material, such as steel or tungsten, and the interior is formed of a lower melting point neutron shielding substance, such as lithium hydride.
  • FIG. 1 is a diagram of a shield containing pelletized shielding material.
  • FIG. 2 is a diagram of an individual pellet.
  • FIG. 3 is a diagram illustrating one method of manufacture 8 for pellets of shielding material.
  • FIG. 4 is a diagram of an actively cooled shield constructed using pellets of shielding material.
  • FIG. 1 is a diagram of a shield containing pelletized shielding material.
  • Shield retaining wall 10 may be of any convenient shape or material consistent with structural requirements.
  • Pellets of shielding material 20 are used as fill within the shield.
  • Pellets 20 may be of any convenient size. However, pellets of about one-quarter inch length are conveniently handled and placed into shields of odd shapes.
  • FIG. 2 is a diagram of an individual pellet.
  • the outer shell of the pellet 21 is composed of a high melting point material, for example tungsten, molybdenumn, depleted uranium, or iron. This material will inhibit the passage of particular types of radiation and not inhibit to the same extent other types of radiation.
  • Filling 22 comprises another type of shielding material. Ideally, this material will have shielding properties complementary to those of the outer shell. Thus, the radiation which the material in the outer shell does not shield against tends to be absorbed by materials inside the pellets.
  • Lithium hydride is a typical material that can be used for filling of pellets.
  • the filling material may be any substance which is rich in hydrogen. Thus, paraffins, plastics, and other hydrocarbon-rich materials could be used. If a thick outer shell is employed, water would also be a suitable filling material.
  • the outer shell material will be a heavy metal with a higher melting point than the filling. Typically, a hydrogen-rich pellet filling will retard neutrons, and a heavy metal shell will act against gamma rays.
  • outer shell 21 should be chosen to be of sufficient thickness so as to resist internal pressures exerted when filling 22 is heated. Adequate thickness may be determined by constructing pellets with shells of varying thickness and then heating them to the maximum rated temperature of the shield. For quarter inch pellets of steel or tungsten, filled with lithium hydride, a shell of one-sixteenth inch thickness will be adequate for temperatures of 500 degrees
  • FIG. 3 is a diagram illustrating one method of manufacture for pellets of shielding material.
  • Lengths of steel or tungsten tubing 100 are filled with liquid lithium hydride, which is then allowed to solidify.
  • Crimping tool 110 is then used to crimp the tubing at quarter-inch intervals in order to form crimped sections of tubing 115.
  • Arc welder 120 is then applied to the tubing in order to seal the ends of individual crimped sections.
  • saw 130 is used to cut crimped sections of the tubing into individual pellets.
  • FIG. 4 is a diagram of a shield constructed using shielding pellets.
  • Container 400 is filled with a bed of shielding pellets, 410.
  • Container 400 may be made in any convenient shape. It functions merely to physically restrain pellet bed 410 and to provide a containier for cooling fluid 420, which flows through the pellet bed. Cooling fluid 420 enters container 400 via inlet port 430, picks up heat from shielding pellet bed 410, and exits via outlet port 431. Thus, heat is conveyed from the shield.

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  • Physics & Mathematics (AREA)
  • Engineering & Computer Science (AREA)
  • General Engineering & Computer Science (AREA)
  • High Energy & Nuclear Physics (AREA)
  • Powder Metallurgy (AREA)

Abstract

Radiation pellets having an outer shell, preferably, of Mo, W or depleted Und an inner filling of lithium hydride wherein the outer shell material has a greater melting point than does the inner filling material.

Description

GOVERNMENT CONTRACT
This invention was made or conceived in the course of or under a contract with the U.S. Department of Energy.
BACKGROUND OF THE INVENTION
This invention relates in general to radiation shielding means, and more particularly to radiation shielding pellets containing at least two shielding materials within individual pellets.
Radiation shields often contain more than one type of material in order to provide attentuation over the entire spectrum of incident radiation. One common type of shielding application requires a gamma ray shielding metal such as tungsten or steel in combination with a hydrogen-rich neutron shielding material such as lithium hydride.
Since the radiation shield must provide uniform attenuation over a large surface area, the two required materials must be prevented from separating within the shield. This means that lithium hydride in a shield must be trapped in place. If it is allowed to liquify or form vapor bubbles, portions of the shield volume will come to have an incorrect ratio of LiH versus metal, and shielding will not be uniform.
Prior art shielding systems have dealt with this problem by attempting to maintain all portions of the shield below the melting point of LiH. The interior of the shield was filled with a honeycomb-like structure of tungsten or steel with LiH placed in the cells of the honeycomb. The metallic honeycomb conducted heat away from the LiH and to the outer surface of the shield.
However, honeycomb structures are difficult to fabricate, particularly if an active cooling means, such as a fluid flow heat removal system, is required. Moreover, honeycombs and cooling pipes required to maintain LiH in solid form tend to be heavy. This makes them undesirable for use in systems requiring active cooling which must be launched into space.
In addition, in shields wherein lithium hydride is cast and allowed to solidify, cracks often develop in the solid lithium hydride. These permit radiation to stream through.
OBJECTS OF THE INVENTION
Thus, it is one object of this invention to provide a radiation shield, incorporating more than one type of material, which is easy to fabricate.
It is a further object to provide a pelletized radiation shielding material which can operate at elevated temperatures without failure, despite liquifaction or cracking of the hydrogen-rich neutron absorbing material.
It is a further object to provide a shield which is light weight and therefore particularly suitable for space applications.
SUMMARY OF THE INVENTION
These and other objects are obtained by forming shielding materials into pellets, wherein the exterior of each capsule is formed of a high melting point gamma ray shielding material, such as steel or tungsten, and the interior is formed of a lower melting point neutron shielding substance, such as lithium hydride.
BRIEF DESCRIPTION OF THE DRAWINGS
FIG. 1 is a diagram of a shield containing pelletized shielding material.
FIG. 2 is a diagram of an individual pellet.
FIG. 3 is a diagram illustrating one method of manufacture 8 for pellets of shielding material.
FIG. 4 is a diagram of an actively cooled shield constructed using pellets of shielding material.
DESCRIPTION OF THE PREFERRED EMBODIMENT
FIG. 1 is a diagram of a shield containing pelletized shielding material. Shield retaining wall 10 may be of any convenient shape or material consistent with structural requirements. Pellets of shielding material 20 are used as fill within the shield. Pellets 20 may be of any convenient size. However, pellets of about one-quarter inch length are conveniently handled and placed into shields of odd shapes.
FIG. 2 is a diagram of an individual pellet. The outer shell of the pellet 21 is composed of a high melting point material, for example tungsten, molybdenumn, depleted uranium, or iron. This material will inhibit the passage of particular types of radiation and not inhibit to the same extent other types of radiation.
Filling 22 comprises another type of shielding material. Ideally, this material will have shielding properties complementary to those of the outer shell. Thus, the radiation which the material in the outer shell does not shield against tends to be absorbed by materials inside the pellets. Lithium hydride is a typical material that can be used for filling of pellets. Typically, the filling material may be any substance which is rich in hydrogen. Thus, paraffins, plastics, and other hydrocarbon-rich materials could be used. If a thick outer shell is employed, water would also be a suitable filling material. Typically, the outer shell material will be a heavy metal with a higher melting point than the filling. Typically, a hydrogen-rich pellet filling will retard neutrons, and a heavy metal shell will act against gamma rays.
As pellet 20 heats during use of the shield, filling 22 will eventually crack, melt, and perhaps, vaporize. Thus, outer shell 21 should be chosen to be of sufficient thickness so as to resist internal pressures exerted when filling 22 is heated. Adequate thickness may be determined by constructing pellets with shells of varying thickness and then heating them to the maximum rated temperature of the shield. For quarter inch pellets of steel or tungsten, filled with lithium hydride, a shell of one-sixteenth inch thickness will be adequate for temperatures of 500 degrees
FIG. 3 is a diagram illustrating one method of manufacture for pellets of shielding material. Lengths of steel or tungsten tubing 100 are filled with liquid lithium hydride, which is then allowed to solidify. Crimping tool 110 is then used to crimp the tubing at quarter-inch intervals in order to form crimped sections of tubing 115. Arc welder 120 is then applied to the tubing in order to seal the ends of individual crimped sections. Finally, saw 130 is used to cut crimped sections of the tubing into individual pellets.
FIG. 4 is a diagram of a shield constructed using shielding pellets. Container 400 is filled with a bed of shielding pellets, 410. Container 400 may be made in any convenient shape. It functions merely to physically restrain pellet bed 410 and to provide a containier for cooling fluid 420, which flows through the pellet bed. Cooling fluid 420 enters container 400 via inlet port 430, picks up heat from shielding pellet bed 410, and exits via outlet port 431. Thus, heat is conveyed from the shield.
The foregoing is a description of a preferred embodiment of this invention. However, the invention need not be limited to particular types of shielding materials or pellet sizes.

Claims (6)

What we claim is:
1. Radiation sheilding pellets comprising:
an outer shell of radiation shielding material having a first melting point; and
an inner filling of radiation shielding material having a second melting point,
wherein said first melting point is greater than said second melting point.
2. The pellets of claim 1 wherein said outer shell comprises a metal effective for shielding against gamma rays.
3. The pellets of claim 2 wherein said metal is selected from the group containing: iron, molybdenum, tungsten, depleted uranium, and alloys thereof.
4. The pellets of claim 1 wherein said inner filling comprises lithium hydride.
5. The pellets of claim 2 wherein said inner filling comprises lithium hydride and said outer shell is selected from the group containing tungsten, iron, molybdenum, depleted uranium, and alloys thereof.
6. A bed of radiation shielding pellets comprising pellets and retention means effective for maintaining a plurality of said pellets in position with repect to one another and also effective for containment of a cooling fluid in contact with said pellets,
wherein said pellets comprise an outer shell of a first shielding material and an inner filling of a second shielding material; and
wherein said retention means further comprises means for admission and exit of said cooling fluid.
US07/020,070 1987-02-27 1987-02-27 Radation shielding pellets Abandoned USH558H (en)

Priority Applications (1)

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US07/020,070 USH558H (en) 1987-02-27 1987-02-27 Radation shielding pellets

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Application Number Priority Date Filing Date Title
US07/020,070 USH558H (en) 1987-02-27 1987-02-27 Radation shielding pellets

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Publication Number Publication Date
USH558H true USH558H (en) 1988-12-06

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Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4997619A (en) * 1989-10-13 1991-03-05 The Babcock & Wilcox Company Shield for a nuclear reactor
US5015863A (en) * 1989-05-31 1991-05-14 Sumitomo Heavy Industries, Ltd. Radiation shield and shielding material with excellent heat-transferring property
US20080198960A1 (en) * 2007-02-20 2008-08-21 Keegan C Patrick Nuclear reactor vessel fuel thermal insulating barrier
US9193105B1 (en) 2011-08-31 2015-11-24 Consolidated Nuclear Security, LLC Casting fine grained, fully dense, strong inorganic materials

Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4130459A (en) 1976-03-29 1978-12-19 Westinghouse Electric Corp. Poison and diluent system for nuclear power plants
US4507359A (en) 1980-12-22 1985-03-26 Chomerics, Inc. Electromagnetic shielding
US4657784A (en) 1986-03-10 1987-04-14 Ecolab Inc. Process for encapsulating particles with at least two coating layers having different melting points

Patent Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4130459A (en) 1976-03-29 1978-12-19 Westinghouse Electric Corp. Poison and diluent system for nuclear power plants
US4507359A (en) 1980-12-22 1985-03-26 Chomerics, Inc. Electromagnetic shielding
US4657784A (en) 1986-03-10 1987-04-14 Ecolab Inc. Process for encapsulating particles with at least two coating layers having different melting points

Cited By (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US5015863A (en) * 1989-05-31 1991-05-14 Sumitomo Heavy Industries, Ltd. Radiation shield and shielding material with excellent heat-transferring property
US4997619A (en) * 1989-10-13 1991-03-05 The Babcock & Wilcox Company Shield for a nuclear reactor
US20080198960A1 (en) * 2007-02-20 2008-08-21 Keegan C Patrick Nuclear reactor vessel fuel thermal insulating barrier
US8401142B2 (en) * 2007-02-20 2013-03-19 Westinghouse Electric Company Llc Nuclear reactor vessel fuel thermal insulating barrier
US9193105B1 (en) 2011-08-31 2015-11-24 Consolidated Nuclear Security, LLC Casting fine grained, fully dense, strong inorganic materials

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